ap-4-10.dvi Acta Polytechnica Vol. 50 No. 4/2010 Capillary Discharge Parameter Assessment for X-ray Laser Pumping J. Hübner Abstract This paper assigns optimum capillary discharge characteristics with respect to reaching the maximum emission gain on wavelength l = 18.2 nm and corresponding to Balmer α transition H-like carbon. The computer modelling of the capil- lary discharge evolution is carried out using the NPINCH programme, using a one-dimensional physical model based on MHD equations. The information about the capillary discharge evolution is processed in FLY, FLYPAPER, FLYSPEC programmes, enabling the population to be modelled on specific levels during capillary discharge. Keywords: capillary discharge, X-ray laser, MHD (magnetohydrodynamic) simulation, population inversion, gain optimal- ization, carbon. 1 Introduction Non-stationaryplasmaof a fast capillary electrical dis- charge was studied as a potential active medium for a soft X-ray laser. The aim was to achieve an optimum set of characteristics for lasing at 18.2 nm wavelength H-like carbon C5+ in an alumina capillary. Optimum in the sense of reachingamaximumgainvalue for each set of parameters. Capillary pinch dynamics is determined by many selected parameters: capillary geometry (radius and capillary length), the substance of the capillary, the initial filling pressure, and the electric current time dependance. This dependance, in particular, is given by an electric circuit which is joined to the capillary. A capillary discharge Z-pinch acting as a medium for a soft X-ray laser uses ASE, the “Amplified Spon- taneous Emission” effect, and electron-collisional re- combination pumping. The main variable for ASE is the gain, and the most important goal of this paper is to find specific parameters of a capillary to obtain the maximum gain. Electron-collisional recombination, sometimes re- ferred to as “three body” recombination, is the in- verse process to electron-collisional ionization fromex- cited levels. The combined recombination and radia- tive downward cascading process is illustrated by the equation X(i+1)+o +2e → X i+ n + e → X i+ u + e (1) It is assumed that the ions exist plentifully in the initial state, which is one stage of ionization higher than that of the lasing ions. Note that this is not a self-containedpopulation-replenishment scheme. Hence, replenishment depends upon further reioniza- tion, which is provided in our case by the release of the next current pulse. It was assumed that ablation from inner walls has only an imperceptible effect, and so it was not in- cluded in the calculations. The capillary discharge plasma quantities were calculated by means of the NPINCH [2] code under the one-dimensional, two- temperature, one-fluidMHDapproximation. The out- put data was then processed by means of the FLY code, which enables the creation of a history file of the population on the individual levels along the capillary axis. On the basis of the populations history, the gain and the gain history can be calculated. 2 Optimization Optimization itself involves searching the maximum in the four-dimensional space of the parameters. Two parameters relate to the current-impulse shape, the third parameter is initial density (or pressure), and the fourth is the radius of the capillary. The right choice in the range of parameters is of fundamental importance. The results of our study should be instrumental for experimenters in the CAPEX-U [4] project. The range of parameters there- fore has to be related to their experimental equipment, with the view to verifying the results. Consequently, the choice of the first parameter was obvious because an alumina capillary r = 1.6 mm in radius is used in CAPEX-U. The choice of the current pulse had to coincide with the source in CAPEX-U. The electric current in a capillary was fitted from measuring by function. If it = I0 sin ( πt 2t0 ) exp ( − t t1 ) (2) The chosen parameters are therefore associated with equation 2: current peak value Imax and dI/dt|t=0. Two cases were calculated Imax ≈ 30 kA and Imax ≈ 60 kA, on behalf of dI/dt|t=0 the area within the range of value 0.5 ·1012–2.5 ·1012 A/s was chosen. 52 Acta Polytechnica Vol. 50 No. 4/2010 Table 1: Parameters of pulse shape for Imax =30 kA dI/dt|t=0 Imax tmax I0 t0 t1 (A/s) (kA) (ns) (kA) (ns) (ns) 0.750 · 1012 30.023 67.6 33.900 71 570 0.923 · 1012 30.031 54 33.082 56.3 570 1.000 · 1012 30.003 49.5 32.786 51.5 570 1.250 · 1012 30.049 39.4 32.229 40.5 570 1.500 · 1012 30.015 32.5 31.799 33.3 570 Table 2: Parameters of pulse shape for Imax =60 kA dI/dt|t=0 Imax tmax I0 t0 t1 A/s (kA) (ns) (kA) (ns) (ns) 0.923 ·1012 60.056 115.15 74.213 126.3 570 1.000 ·1012 60.029 105.05 72.765 114.3 570 1.250 ·1012 60.006 82.020 69.630 87.5 570 1.500 ·1012 60.044 67.878 67.8 71 570 1.750 ·1012 60.027 57.57 66.51 59.7 570 2.000 ·1012 60.002 50 65.27 51.5 570 2.250 ·1012 60.005 43.63 64.88 45.3 570 2.500 ·1012 60.095 39.59 64.45 40.5 570 The last parameter is initial density N, accord- ing to the theoretical analysis and in order to achieve the gain maximum, the maximum electron den- sity for carbon has to be Ne ≈ 3 · 1020. To accomplish this requirement, we chose the range N =0.5 · 1017–5 ·1017 cm−3. 3 Gain evaluation The selected parameters for each case served as input data for NPINCH. A very useful output of the calcu- lation was the dens.dat file, which contained a time history of electron and ion density, and electron tem- perature. This file futher served as input for the FLY and the FLYPAPER code, and by means of these we obtained the time histories of populations on set lev- els N3 for level n = 3 and N2 for level n = 2 H-like carbon ions. Inversion function F [3] is represented by Equation 3, where the statistical weights gu/gl are for our transition 9/4, and Nl, Nu presents the lower and upper laser state population densities. F =1− ( 2.25 N1 Nu ) (3) The cross-section with corresponding coefficients for our transition λul = 13.3818 · 10−7 cm, Aul = 5.72 · 1010 s−1 can be illustrated as σstim = λ3 8πcΔλ/λ Aul = 1.62 · 104 · (18.2178)3 · 5.72 ·1010 8 · π ·2.997925 · 1010 · √ 2π = (4) 2.966136 · 10−15cm2 And finally, G after cross-section substitution can be illustrated as G =2.966136 · 10−15NuF cm−1 (5) For each calculation, we listed the parameter data, information about the maximum value and the time of reaching gain, the pinch time (the time when the maximum of electron density Ne is reached). 4 Imax =30 kA The results for Imax = 30 kA, are in Fig. 1. The maximum gain value was achieved at dI/dt|t=0 = 1 ·1012 A/s, initial carbon density 1.4 ·1017 cm−3 and Gmax ≈ 0.05 cm−1. The calculated data resembled the Gauss function, so they were fitted by this func- tion, and the deviation between the calculated data and the fitted function was minimal. The most infor- mation is shown in Fig. 2. The best gainwas achieved when the time of reaching currentmaximumwas equal to the pinch time. Fig. 1: Maximum Gmax against initial density for various current derivations at Imax =30 kA. The data is fitted by the Gauss function Fig. 2: Comparison of the achieving time ofmaximumgain TG, and current TI in dependence on dI/dt|t=0 5 Imax = 60 kA For the casewhere Imax =60 kA is chosen, the results are shown in thenextfigure. Themaximumgainvalue 53 Acta Polytechnica Vol. 50 No. 4/2010 Gmax was reachedatdI/dt|t=0 =2.25·1012 A/s, initial carbon density 4.1 · 1017 cm−3 and Gmax ≈ 3.4 cm−1. This data too was fitted by the Gauss function. Fig. 3: Maximum Gmax against initial density for various current derivations at Imax =60 kA. The data is fitted by the Gauss function Fig. 4: Comparison of achieving time ofmaximumgain TG and current TI in dependence on dI/dt|t=0 6 Example Now we can take a closer look at a particular case to show the history of certain variables. The param- eters of a capillary discharge N0 = 4.0 · 1017 cm−3, dI/dt|t=0 = 2 · 1012 A/s, r0 = 1.6 mm and Imax = 60 kAhave been chosen. We will plot the curve for an individual quantity, such as electron density, electron temperature, inversion of population, and gain. Fig. 5: Behaviour of electron density for parameters N0 = 4.0·1017 cm−3, dI/dt|t=0 =2·1012 A/s, r0 =1.6 mmand, Imax =60 kA Fig. 6: Behaviour of electron temperature for parameters N0 =4.0·1017 cm−3, dI/dt|t=0 =2·1012 A/s, r0 =1.6mm, and Imax =60 kA Fig. 7: Behaviour of the population on levels n = 2 a n = 3 for parameters N0 =4.0 · 1017 cm−3, dI/dt|t=0 = 2 ·1012 A/s, r0 =1.6 mm, and Imax =60 kA Fig. 8: Behaviour of inversion function F and gain (cm−1). In addition, the figure contains a marked pinch time tp = 44nsand time of reaching currentmaximum tImax =55 for parameters N0 =4.0 ·1017 cm−3, dI/dt|t=0 =2 ·1012 A/s, r0 =1.6 mm and Imax =60 kA Figures 6 and 7 demonstrate the behaviour of elec- tron density and temperature. They show pinch time tp =44 ns, Nemax =3.8 ·1020 cm−3, Temax =110 eV. After that, a rapid drop in these quantities followsdue to adiabatic expansion. The electron density drops by nearly two orders in 5 ns and the electron temperature drops by nearly 90 eV. These are ideal conditions for creating population inversion at the desired levels. 54 Acta Polytechnica Vol. 50 No. 4/2010 Figure 8 shows that at time 46.5 ns, 2.5 ns after pinch time, both the inversion function and gain had an above zero value. At time 47.2 ns, the gain maxi- mum Gmax =3.2 cm −1 is reached, and just about one ns later the inversion function also reaches its max- imum and starts to fall steadily. However, the gain begins to drop very rapidly, due to rapid density de- cay of the whole mass (both electrons and ions, which are lasing) along to axix. It follows from the gain be- haviour that the hypothetical laser pulse could be 2 ns in length. Howdoes the initial density influence the pinchbe- haviour? With increasing initial density themaximum density also increases. At the same time, the pich time is delayed. The effect is totally contrary to the elec- tron temperature. As the initial density increases the maximum electron temperature value decreases. 7 Conclusion The optimal conditions for achieving maximum gain for initial density and electric current pulse shape have been obtained for two different current maxima, Imax = 30 kA, Imax = 60 kA and capillary radius r = 1.6 mm. Figures 2 and 4 show clearly that the time of achieving the currentmaximum and the pinch time have to be synchronized for optimal current dif- ferentiation at zero time, so that both times will be almost identical. Gmax = 0.05 cm −1 was achieved at N0 = 1.4 · 1017 cm−3, dI/dt|t=0 =1 ·1012 A/s, r0 =1.6 mm and Imax =30 kA. Gmax = 3.4 cm −1 was achieved at N0 = 4.1 · 1017 cm−3, dI/dt|t=0 = 2.25 · 1012 A/s, r0 = 1.6 mm and Imax =60 kA. The assumed pulse length is 2 ns. Acknowledgement The research described in this paper was supervised by Ing. Pavel Vrba, CSc., IPP AS CR in Prague, and was supportedby theCzechGrantAgencyundergrant No. 202/08/057. References [1] Rocca, J. J.: Table-top soft x-ray lasers,Review of Scientific Instruments, 1999, vol. 70, no. 10. [2] Razinkova, T. L., Sasorov, P. V.: Program NPINCH na počítání dynamiky z-pinče, Moskva, 1998. [3] Elton, R. C.: X-Ray Laser, Academic Press, New York, 1990. [4] Koláček, K. et al.: 10th ICXRL2006, Berlin, Ger- many (poster – 14 09 Kolacek.pdf). Jakub Hübner E-mail: bukajus@centrum.cz Dept. of Physical Electronics Faculty of Nuclear Science and Physical Engineering Czech Technical University Břehová 7, 115 19 Prague 1, Czech Republic 55