Format And Type Fonts CHEMICAL ENGINEERING TRANSACTIONS VOL. 39, 2014 A publication of The Italian Association of Chemical Engineering www.aidic.it/cet Guest Editors: Petar Sabev Varbanov, Jiří Jaromír Klemeš, Peng Yen Liew, Jun Yow Yong Copyright © 2014, AIDIC Servizi S.r.l., ISBN 978-88-95608-30-3; ISSN 2283-9216 DOI: 10.3303/CET1439240 Please cite this article as: Pan M., Bulatov I., Smith R., 2014, Recent methods for retrofitting heat exchanger networks with heat transfer intensifications, Chemical Engineering Transactions, 39, 1435-1440 DOI:10.3303/CET1439240 1435 Recent Methods for Retrofitting Heat Exchanger Networks with Heat Transfer Intensifications Ming Pan*, Igor Bulatov, Robin Smith Centre for Process Integration, The University of Manchester, Sackville street, Manchester, M13 9PL, UK ming.pan@manchester.ac.uk This paper presents an overview of recent optimization approaches for retrofitting heat exchanger networks (HENs) with heat transfer intensified techniques. The developed methods includes the heuristic rules for finding suitable enhanced exchangers in HENs, and the SA-based optimization method and MILP-based iterative mathematical programming method for optimizing HEN retrofit problems. An industrial case is investigated with the different optimization methods in several typical retrofit scenarios, providing a better understanding of implementing intensification techniques in suitable exchangers to achieve the best energy saving in a whole retrofitted HEN. 1. Introduction The most efficient way to decrease energy consumption and the release of greenhouse gases from the process industries is to increase heat recovery. The cleanest energy is the energy saved by improved efficiency. In major process industries including oil refining, petrochemical processes, food, cement, steel, pulp and paper, where very substantial energy savings can be made. Calculations indicate that the energy consumption could be decreased by 30 % purely by using intensification technology in the critical parts of the heat recovery system (Pan et al., 2012). Various new ways have recently been developed to significantly enhance heat exchanger performance. These techniques do not need to be applied through the whole heat recovery system, but mainly at those critical parts that limit the system performance. Recently, the approaches of implementing heat transfer intensification techniques have be considered in more details. Pan et al. (2011) firstly proposed a novel MILP-based method to solve HEN retrofit problems with intensified heat transfer techniques. Wang et al. (2012a) proposed a detailed model for predicting exchanger performances and developed five heuristic rules to identify suitable heat exchangers for intensification. For modelling detailed intensified techniques, Pan et al. (2013a) focused on the recent achievements of tube-side and shell-side enhancement techniques, considered different techniques in the same cases to compare their performances, and investigated their combinations. Intensified heat transfer techniques are also considered to reduce fouling effect in enhanced exchangers (Pan et al., 2013b). To combine the advantages of intensification and the conventional retrofit methods, Pan et al. (2013c) successfully found valid retrofitted structures for retrofitting HEN with heat transfer intensification, which can achieve significant energy saving without expensive cost from too many modifications. Sreepathi and Rangaiah (2014) proposed several exchanger reassignment strategies for HEN retrofitting. One of those was developed and used in multi-objective optimization. Liu et al. (2014) applied hybrid genetic algorithm to obtain the optimal retrofitted HEN with full utilization of the existing heat exchangers and structures. Kang and Liu (2014) presented a retrofitting approach for heat exchanger networks (HENs) for single- period and multiple-period operations, aiming at the improvement of operation flexibility of HENs. Based on the aforementioned researches, this paper provides an overview of recent optimization approaches for retrofitting heat exchanger networks (HENs) with heat transfer intensified techniques. The conventional approaches (heuristic based, simulated annealing based and MILP-based) are investigated in an industrial case study to illustrate their efficiencies of solving HEN retrofit problems with heat transfer intensification. 1436 2. Conventional approaches of retrofitting HENs with heat transfer intensification The existing methods for retrofitting HENs can be divided into three categories, thermodynamic analysis (e.g. Heuristic Rules), stochastic optimization methods (e.g. Simulated Annealing), and deterministic programming methods (e.g. MILP). The optimization procedures and required models of the most efficient approaches based on the above categories are briefly introduced in this section. More details of these methods have been reported by Wang et al. (2012a), Wang et al. (2012b) and Pan et al. (2012). 2.1 Heuristic rule approach The heuristic rules proposed by Wang et al. (2012a) are used to consider aspects of the reduction in the use of utilities, and the selection of suitable heat exchangers to be enhanced. Retrofit problems can be dealt without involving complex calculations. The optimization procedure includes five steps (namely five rules): Rule 1: searching for exchangers in utility path. The candidates for intensification should be on utility path. The exchangers on the same stream with a utility exchanger can affect the duty of the utility exchanger directly. Rule 2: sensitivity analysis. Based on the heat exchangers selected with Rule 1, sensitivity tables are used to quantify impact of heat transfer intensity on utility consumption of the HEN. High sensitivity exchanger can be a good candidate for intensification. Rule 3: checking pinching match. Pinching match is the bottleneck of heat recovery network. Normally, the pinching match will have a very small heat transfer temperature difference. Rule 4: enhancing candidates in sequence. Once the best exchanger selected based on Rule 2 is enhanced, sensitivity analysis (Rule 2) is applied again to all candidate exchangers to find the next best one. Rule 5: enhancing pinching match. Enhancing pinching match can be considered in the situation of no good candidate for the heat transfer enhancement, or the potential for energy savings from enhancing promising candidates may be very low. Based on the heuristic rules 1-5, suitable candidates in HEN are selected, and the optimal solution of HEN retrofit can be obtained. 2.2 Stochastic optimization method Stochastic optimization methods are optimization methods that generate and use random variables. Simulated annealing (SA) is a generic probabilistic metaheuristic for the global optimization problem of locating a good approximation to the global optimum of a given function in a large search space. The SA- based optimization method adopted in this paper is based on the approach proposed by Wang et al. (2012b). In the SA method, continuous variables include exchanger duties, stream flowrates, stream temperatures, and exchanger heat transfer coefficients; while discrete variables include adding intensification techniques, deleting intensification techniques. Thus, adding intensification techniques and deleting intensification techniques are described as the SA moves, which can create a network with a small random difference from the trial situation as follows: Intensification is randomly added to tube side or shell side or both in an exchanger with an increasing ratio of heat transfer coefficient. The maximum increasing ratio of heat transfer coefficient according to enhancement device is described in constraints. Moreover, the maximum number of exchangers to be enhanced can be set as too many modifications on exchangers are not common in practical industry. The objective function is to minimize the energy consumption or the total retrofit cost of networks. After a SA move is made, the new network will be accepted if the objective value is improved; otherwise, the new network will be denied. Repeat the above procedure in a sufficient long computing time, an optimal retrofitted network with heat transfer intensification can be found. Two calculation approaches (duty-based and area-based) are used for determining heat exchanger performances. In duty-based approach, the inlet temperatures, stream capacities and heat load in an exchanger are known, thus exchanger area can be calculated directly from Eq(1)-Eq(3), where EX is the set of all exchangers, HTIex, HTOex, CTIex and CTOex are inlet and outlet temperatures of hot and cold streams in exchanger ex, Qex is the duty of exchanger ex, HFCPex and CFCPex are heat-flow capacities (the multiplication between heat capacity and flow-rate) of hot and cold streams in exchanger ex, LMTDex is the logarithmic mean temperature difference of exchanger ex, EXAex is area of exchanger ex, and Uex is the heat transfer coefficient of exchanger ex. 1437 ex ex exex HFCP Q HTIHTO , EXex (1) ex ex exex CFCP Q CTICTO , EXex (2) exex ex ex LMTDU Q EXA , EXex (3) In area-based approach, exchanger area is known and fixed, but heat load (Qex) is unknown. The calculation of heat load (Qex) requires a iterative procedure of Eq(1)-Eq(3), and an estimated value of heat load is needed in the initial condition. Even though the area-based approach leads to a longer computing time, it presents practical HEN retrofit process with heat transfer intensification directly, and avoids minimum approach temperature violation. 2.3 Deterministic programming method A deterministic algorithm is an algorithm which, given a particular input, will always produce the same output, with the underlying machine always passing through the same sequence of states. MILP-based iterative methods proposed by Pan et al. (2012) have been widely used for retrofitting HENs with heat transfer intensification recently. The optimization approach includes an MILP-based model and an iteration algorithm. First of all, logarithmic mean temperature difference (LMTD) is initialized with initial stream temperatures, as shown in Eq(4), where HTI’ex, HTO’ex, CTI’ex and CTO’ex are inlet and outlet initial temperatures of hot and cold streams in exchanger ex. exexexex exexexex ex ICTOHT/OCTIHTln ICTOHTOCTIHT DLMT , EXex (4) Then, a set of binary variables is proposed: EEXex =1, if an intensification technique is implemented in exchanger ex; otherwise, it is 0. Thus, the heat transfer coefficients of intensified exchangers can be formulated as: exexex EEXMINUU 1 , EXex (5) exexex EEXMAXUU 1 , EXex (6) where MAXUex and MINUex are the upper and lower bounds of heat transfer coefficient when a intensification technique is implemented in exchanger ex. The constraints of heat transfer (HBAex and HBBex) and energy balance (AEBex and BEBex) in an exchanger are shown in Eq(7)-Eq(10). exexexexexexex DLMTUEXAHTOHTIPHFCHBA , EXex (7) exexexexexexex HTOHTIPHFCDLMTUEXAHBB , EXex (8) exexexexexexex CTOCTIPCFCHTOHTIPHFCAEB , EXex (9) exexexexexexex HTOHTIPHFCCTOCTIPCFCBEB , EXex (10) The minimum temperature difference (∆Tmin) is restricted in Eq(11) and Eq(12). min TCTOHTI exex , EXex (11) min TCTIHTO exex , EXex (12) The stream temperature differences (DAHTIex and DBHTIex) are presented in Eq(13) and Eq(14). Other temperature differences, such as DAHTOex, DBHTOe, DACTIex, DBCTIex, DACTOex and DBCTOex are formulated in the same way. 1438 exexex IHTHTIDAHTI , EXex (13) exexex HTIIHTDBHTI , EXex (14) Eq(15) presents energy saving (QS) after in the retrofit, where EXhu and EXcu are the set of all exchangers consuming hot and cold utilities; OCTIex and OHTIex are the original inlet temperatures of cold stream and hot stream in exchanger ex before retrofit. cuhu EXex exexex EXex exexex HTIOHTIPHFCOCTICTIPCFCQS (15) The objective of the MILP-based method is to minimize the summation of difference in energy balances, heat transfers and stream temperatures with the restrictions of an estimated energy saving value (QS’), as shown in Eq(16) and Eq(17). SQQS (16) EXex EXex exexexexexex EXex exex EXex exexexex BEBAEBDBHTODAHTODBHTIDAHTI HBBHBADBCTODACTODBCTIDACTIObj (17) The MILP-based model for maximum energy saving consists of an objective function given in Eq(17) and model constraints given from Eq(4)-Eq(16). Since the MILP-based model has been built, an iteration algorithm (two iteration loops) is used to find the optimal solution for HEN retrofit problems. In the first loop, the MILP-based model is solved repeatedly to obtain a feasible solution for HEN retrofit under certain energy saving. In the second loop, the maximum value of energy saving is searched, and the feasible solution under the maximum energy saving can be found by using the procedure proposed in the first loop. 3. Case study Figure 1: An industrial scale HEN for the case study C1 C2 C3 CU H1 H2 H3 H4 H5 H6 H7 H8 H 9 H10 H11 HU 30 30 29 29 21 21 28 28 27 27 26 26 24 24 20 20 4 4 18 18 17 17 16 16 23 23 13 13 22 22 12 12 6 6 5 5 3 3 1 1 2 2 25 25 31 31 19 19 15 15 14 14 7 7 11 11 10 10 8 8 9 9 H Hot stream: HU Hot utility: C Cold stream: CU Cold utility: 1439 The example investigated in this paper is an industrial scale HEN, as shown in Figure 1. The retrofit objective is to reduce the hot utility (HU) consumption, namely, reduce the heat duty of heat exchanger 30 (target exchanger). The stream data and initial exchanger data can be found in Tables 1 and 2. Moreover, the heat-flow capacities of hot utility and cold utility are 93 kW/ºC and 9,652.5 kW/ºC, the inlet temperatures of hot utility and cold utility are 1,500 ºC and 12.45 ºC, the minimum temperature difference approaches (∆Tmin) before and after heat transfer intensification are 19 ºC and 5 ºC. Table 1: Stream details in case study Stream C1 C2 C3 H1 H2 H3 H4 H5 H6 H7 H8 H9 H10 H11 FCP (kW/ºC) 323 358.5 474 14.2 181.5 113 100 22.2 39.5 28.0 176 24.5 25.0 69.6 Tin (ºC) 33.5 91.34 151 335 253.2 294 212 213 174 364 290 284 240 179 Tout (ºC) 95.6 157.3 352 69.4 116.1 130 156 61.7 43.3 65.6 211 65.6 57.8 69.3 Table 2: Exchanger details in original HEN EXs HTIex (ºC) HTOex (ºC) CTIex (ºC) CTOex (ºC) LMTDex (ºC) EXAex (m 2 ) Uex (kW/m 2 ·ºC) Duty (kW) 1 117.220 66.284 33.510 40.523 51.660 174.990 0.12509 1130.8 2 131.237 130.000 14.194 14.208 116.416 11.666 0.10292 139.8 3 174.400 76.670 33.510 57.450 74.024 116.660 0.44702 3860.3 4 284.200 174.731 156.731 162.390 54.291 174.990 0.28230 2682.0 5 212.440 156.050 48.986 66.454 125.521 100.000 0.44880 5633.4 6 174.444 85.701 66.454 85.606 45.500 650.000 0.20884 6176.5 7 66.284 61.670 12.998 13.009 50.939 20.000 0.10054 102.4 8 76.670 62.200 12.527 12.586 56.573 30.000 0.33677 571.6 9 62.200 43.330 12.450 12.527 39.535 55.560 0.33933 745.4 10 171.093 57.780 12.586 12.880 90.200 277.800 0.11305 2832.8 11 85.701 69.300 12.880 12.998 64.218 55.560 0.31994 1141.5 12 169.050 117.220 85.606 89.174 52.070 22.224 0.99432 1150.6 13 221.101 147.201 89.174 95.590 87.473 38.060 0.62153 2069.2 14 147.201 65.560 13.009 13.246 86.996 85.720 0.30654 2285.9 15 109.340 69.440 13.246 13.304 74.344 42.860 0.17781 566.6 16 198.376 131.237 91.340 133.665 51.308 128.580 1.15000 7586.7 17 335.400 109.340 91.340 109.248 82.246 207.690 0.18792 3210.1 18 174.731 139.686 121.457 123.852 31.809 207.690 0.12996 858.6 19 139.686 65.560 13.304 13.492 83.862 138.460 0.15640 1816.1 20 206.228 141.852 123.852 156.444 31.243 1384.600 0.27010 11684.2 21 178.700 174.444 156.444 157.270 19.665 27.692 0.54395 296.2 22 212.680 169.050 151.050 153.093 34.741 83.076 0.33560 968.6 23 240.070 171.093 153.093 156.731 42.634 41.538 0.97373 1724.4 24 253.200 206.228 162.390 180.376 57.110 1038.450 0.14375 8525.4 25 222.747 210.900 13.978 14.194 202.682 66.660 0.15433 2085.1 26 293.700 198.376 180.376 203.101 44.923 299.970 0.79934 10771.6 27 248.975 221.101 203.101 204.747 29.175 233.310 0.11466 780.5 28 290.380 222.747 204.747 229.860 35.065 1020.000 0.33281 11903.4 29 364.260 248.975 229.860 236.670 57.142 240.000 0.23538 3228.0 30 1500.000 912.546 236.670 351.930 891.221 180.000 0.34056 54633.2 31 141.852 116.050 13.492 13.978 114.751 60.000 0.68018 4683.1 In this case study, three typical optimization approaches are used to solve the retrofit problem. They are heuristic rule approach (Wang et al., 2012a), SA optimization approach (Wang et al., 2012b), and MILP- based iterative approach (Pan et al., 2012). Intensified technique is implemented to directly increase the overall heat transfer coefficients of enhanced exchangers. It is assumed that the maximum intensified coefficient of each exchanger is two times of its original value. The optimal solutions based on the three optimization approaches are shown in Table 3. As presented in Table 3, heat transfer coefficients increase in the intensified exchangers, all exchangers remain unchanged area, and the optimal solution based on the MILP-based approach requires less 1440 computing time and give the best solution. It is noted that the MILP-based method can quickly find the most appropriate heat exchangers for intensification. Table 3: Optimal solutions based on the three optimization approaches Optimization approaches Intensified exchangers (U: kW/m 2 ·°C) Energy saving (kW) Computing time Heuristic rule approach (Wang et al., 2012a) EX20 (0.348), EX24 (0.155), EX26 (1.2), EX28 (0.448) 1904.2 SA optimization approach (Wang et al., 2012b) Duty-based EX4 (0.407), EX20 (0.3), EX23 (1.444), EX28 (0.413) 1118.6 2~3 h Partial area- based EX4 (0.367), EX6 (0.211), EX12 (1.092), EX18 (0.151), EX28 (0.407) 929.0 22~24 h Area-based EX20 (0.397), EX24 (0.195), EX26 (0.878), EX28 (0.425), EX29 (0.336) 2114.0 22~24 h MILP-based iterative approach (Pan et al., 2012) EX20 (0.385), EX24 (0.192), EX26 (0.851), EX28 (0.442), EX29 (0.35) 2161.4 < 1 min 4. Conclusions Many conventional optimization approaches have been widely studied for retrofitting HENs with heat transfer intensification. However, most of the reported methods are still in the research stage and far from being used in industrial application. 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