id	sid	tid	token	lemma	pos
cet-13155	1	1	cet	cet	PROPN
cet-13155	1	2	vol	vol	NOUN
cet-13155	1	3	99	99	NUM
cet-13155	1	4	doi	doi	NOUN
cet-13155	1	5	:	:	PUNCT
cet-13155	1	6	10.3303	10.3303	NUM
cet-13155	1	7	/	/	SYM
cet-13155	1	8	cet2399077	cet2399077	NOUN
cet-13155	1	9	paper	paper	NOUN
cet-13155	1	10	received	receive	VERB
cet-13155	1	11	:	:	PUNCT
cet-13155	1	12	30	30	NUM
cet-13155	1	13	january	january	NOUN
cet-13155	1	14	2023	2023	NUM
cet-13155	1	15	;	;	PUNCT
cet-13155	1	16	revised	revise	VERB
cet-13155	1	17	:	:	PUNCT
cet-13155	1	18	30	30	NUM
cet-13155	1	19	march	march	NOUN
cet-13155	1	20	2023	2023	NUM
cet-13155	1	21	;	;	PUNCT
cet-13155	1	22	accepted	accept	VERB
cet-13155	1	23	:	:	PUNCT
cet-13155	1	24	18	18	NUM
cet-13155	1	25	april	april	PROPN
cet-13155	1	26	2023	2023	NUM
cet-13155	1	27	please	please	INTJ
cet-13155	1	28	cite	cite	VERB
cet-13155	1	29	this	this	DET
cet-13155	1	30	article	article	NOUN
cet-13155	1	31	as	as	ADP
cet-13155	1	32	:	:	PUNCT
cet-13155	1	33	parra	parra	PROPN
cet-13155	1	34	o.	o.	PROPN
cet-13155	1	35	,	,	PUNCT
cet-13155	1	36	portillo	portillo	PROPN
cet-13155	1	37	a.	a.	PROPN
cet-13155	1	38	,	,	PUNCT
cet-13155	1	39	erena	erena	PROPN
cet-13155	1	40	j.	j.	PROPN
cet-13155	1	41	,	,	PUNCT
cet-13155	1	42	ateka	ateka	PROPN
cet-13155	1	43	a.	a.	PROPN
cet-13155	1	44	,	,	PUNCT
cet-13155	1	45	bilbao	bilbao	PROPN
cet-13155	1	46	j.	j.	PROPN
cet-13155	1	47	,	,	PUNCT
cet-13155	1	48	2023	2023	NUM
cet-13155	1	49	,	,	PUNCT
cet-13155	1	50	in2o3	in2o3	PROPN
cet-13155	1	51	-	-	NOUN
cet-13155	1	52	zro2	zro2	PROPN
cet-13155	1	53	as	as	ADP
cet-13155	1	54	alternative	alternative	NOUN
cet-13155	1	55	to	to	ADP
cet-13155	1	56	cu	cu	NOUN
cet-13155	1	57	-	-	PUNCT
cet-13155	1	58	based	base	VERB
cet-13155	1	59	catalysts	catalyst	NOUN
cet-13155	1	60	for	for	ADP
cet-13155	1	61	methanol	methanol	NOUN
cet-13155	1	62	production	production	NOUN
cet-13155	1	63	step	step	NOUN
cet-13155	1	64	in	in	ADP
cet-13155	1	65	the	the	DET
cet-13155	1	66	co2	co2	NOUN
cet-13155	1	67	to	to	ADP
cet-13155	1	68	hydrocarbon	hydrocarbon	NOUN
cet-13155	1	69	process	process	NOUN
cet-13155	1	70	,	,	PUNCT
cet-13155	1	71	chemical	chemical	ADJ
cet-13155	1	72	engineering	engineering	NOUN
cet-13155	1	73	transactions	transaction	NOUN
cet-13155	1	74	,	,	PUNCT
cet-13155	1	75	99	99	NUM
cet-13155	1	76	,	,	PUNCT
cet-13155	1	77	457	457	NUM
cet-13155	1	78	-	-	SYM
cet-13155	1	79	462	462	NUM
cet-13155	1	80	doi:10.3303	doi:10.3303	NOUN
cet-13155	1	81	/	/	SYM
cet-13155	1	82	cet2399077	cet2399077	NOUN
cet-13155	1	83	chemical	chemical	PROPN
cet-13155	1	84	engineering	engineering	NOUN
cet-13155	1	85	transactions	transaction	NOUN
cet-13155	1	86	vol	vol	NOUN
cet-13155	1	87	.	.	PROPN
cet-13155	1	88	99	99	NUM
cet-13155	1	89	,	,	PUNCT
cet-13155	1	90	2023	2023	NUM
cet-13155	1	91	a	a	DET
cet-13155	1	92	publication	publication	NOUN
cet-13155	1	93	of	of	ADP
cet-13155	1	94	the	the	DET
cet-13155	1	95	italian	italian	ADJ
cet-13155	1	96	association	association	NOUN
cet-13155	1	97	of	of	ADP
cet-13155	1	98	chemical	chemical	PROPN
cet-13155	1	99	engineering	engineering	NOUN
cet-13155	1	100	online	online	ADV
cet-13155	1	101	at	at	ADP
cet-13155	1	102	www.cetjournal.it	www.cetjournal.it	PROPN
cet-13155	1	103	guest	guest	NOUN
cet-13155	1	104	editors	editor	NOUN
cet-13155	1	105	:	:	PUNCT
cet-13155	1	106	sauro	sauro	PROPN
cet-13155	1	107	pierucci	pierucci	PROPN
cet-13155	1	108	,	,	PUNCT
cet-13155	1	109	flavio	flavio	PROPN
cet-13155	1	110	manenti	manenti	VERB
cet-13155	1	111	copyright	copyright	NOUN
cet-13155	1	112	©	©	PROPN
cet-13155	1	113	2023	2023	NUM
cet-13155	1	114	,	,	PUNCT
cet-13155	1	115	aidic	aidic	ADJ
cet-13155	1	116	servizi	servizi	PROPN
cet-13155	1	117	s.r.l	s.r.l	PROPN
cet-13155	1	118	.	.	PUNCT
cet-13155	2	1	isbn	isbn	ADJ
cet-13155	2	2	978	978	NUM
cet-13155	2	3	-	-	SYM
cet-13155	2	4	88	88	NUM
cet-13155	2	5	-	-	PUNCT
cet-13155	2	6	95608	95608	NUM
cet-13155	2	7	-	-	PUNCT
cet-13155	2	8	98	98	NUM
cet-13155	2	9	-	-	SYM
cet-13155	2	10	3	3	NUM
cet-13155	2	11	;	;	PUNCT
cet-13155	2	12	issn	issn	PROPN
cet-13155	2	13	2283	2283	NUM
cet-13155	2	14	-	-	SYM
cet-13155	2	15	9216	9216	NUM
cet-13155	2	16	in2o3	in2o3	PROPN
cet-13155	2	17	-	-	PUNCT
cet-13155	2	18	zro2	zro2	PROPN
cet-13155	2	19	as	as	ADP
cet-13155	2	20	alternative	alternative	NOUN
cet-13155	2	21	to	to	ADP
cet-13155	2	22	cu	cu	NOUN
cet-13155	2	23	-	-	PUNCT
cet-13155	2	24	based	base	VERB
cet-13155	2	25	catalysts	catalyst	NOUN
cet-13155	2	26	for	for	ADP
cet-13155	2	27	methanol	methanol	NOUN
cet-13155	2	28	production	production	NOUN
cet-13155	2	29	step	step	NOUN
cet-13155	2	30	in	in	ADP
cet-13155	2	31	the	the	DET
cet-13155	2	32	co2	co2	NOUN
cet-13155	2	33	to	to	ADP
cet-13155	2	34	hydrocarbon	hydrocarbon	NOUN
cet-13155	2	35	process	process	NOUN
cet-13155	2	36	onintze	onintze	PROPN
cet-13155	2	37	parra	parra	PROPN
cet-13155	2	38	*	*	PROPN
cet-13155	2	39	,	,	PUNCT
cet-13155	2	40	ander	ander	PROPN
cet-13155	2	41	portillo	portillo	PROPN
cet-13155	2	42	,	,	PUNCT
cet-13155	2	43	javier	javier	PROPN
cet-13155	2	44	ereña	ereña	PROPN
cet-13155	2	45	,	,	PUNCT
cet-13155	2	46	ainara	ainara	ADV
cet-13155	2	47	ateka	ateka	NOUN
cet-13155	2	48	,	,	PUNCT
cet-13155	2	49	javier	javier	PROPN
cet-13155	2	50	bilbao	bilbao	PROPN
cet-13155	2	51	department	department	PROPN
cet-13155	2	52	of	of	ADP
cet-13155	2	53	chemical	chemical	PROPN
cet-13155	2	54	engineering	engineering	NOUN
cet-13155	2	55	,	,	PUNCT
cet-13155	2	56	university	university	NOUN
cet-13155	2	57	of	of	ADP
cet-13155	2	58	the	the	DET
cet-13155	2	59	basque	basque	ADJ
cet-13155	2	60	country	country	NOUN
cet-13155	2	61	,	,	PUNCT
cet-13155	2	62	upv	upv	PROPN
cet-13155	2	63	/	/	SYM
cet-13155	2	64	ehu	ehu	PROPN
cet-13155	2	65	,	,	PUNCT
cet-13155	2	66	p.o	p.o	PROPN
cet-13155	2	67	.	.	PROPN
cet-13155	2	68	box	box	PROPN
cet-13155	2	69	644	644	NUM
cet-13155	2	70	,	,	PUNCT
cet-13155	2	71	48080	48080	PROPN
cet-13155	2	72	bilbao	bilbao	PROPN
cet-13155	2	73	,	,	PUNCT
cet-13155	3	1	spain	spain	PROPN
cet-13155	3	2	onintze.parra@ehu.eus	onintze.parra@ehu.eus	PROPN
cet-13155	3	3	as	as	ADP
cet-13155	3	4	a	a	DET
cet-13155	3	5	consequence	consequence	NOUN
cet-13155	3	6	of	of	ADP
cet-13155	3	7	the	the	DET
cet-13155	3	8	increasing	increase	VERB
cet-13155	3	9	greenhouse	greenhouse	NOUN
cet-13155	3	10	gas	gas	NOUN
cet-13155	3	11	emissions	emission	NOUN
cet-13155	3	12	,	,	PUNCT
cet-13155	3	13	co2	co2	NOUN
cet-13155	3	14	valorization	valorization	NOUN
cet-13155	3	15	processes	process	NOUN
cet-13155	3	16	are	be	AUX
cet-13155	3	17	gaining	gain	VERB
cet-13155	3	18	importance	importance	NOUN
cet-13155	3	19	in	in	ADP
cet-13155	3	20	the	the	DET
cet-13155	3	21	last	last	ADJ
cet-13155	3	22	decades	decade	NOUN
cet-13155	3	23	.	.	PUNCT
cet-13155	4	1	amongst	amongst	ADP
cet-13155	4	2	the	the	DET
cet-13155	4	3	most	most	ADV
cet-13155	4	4	attractive	attractive	ADJ
cet-13155	4	5	processes	process	NOUN
cet-13155	4	6	for	for	ADP
cet-13155	4	7	co2	co2	NOUN
cet-13155	4	8	utilization	utilization	NOUN
cet-13155	4	9	,	,	PUNCT
cet-13155	4	10	its	its	PRON
cet-13155	4	11	conversion	conversion	NOUN
cet-13155	4	12	into	into	ADP
cet-13155	4	13	hydrocarbons	hydrocarbon	NOUN
cet-13155	4	14	stands	stand	VERB
cet-13155	4	15	out	out	ADP
cet-13155	4	16	,	,	PUNCT
cet-13155	4	17	in	in	ADP
cet-13155	4	18	particular	particular	ADJ
cet-13155	4	19	by	by	ADP
cet-13155	4	20	means	mean	NOUN
cet-13155	4	21	of	of	ADP
cet-13155	4	22	catalytic	catalytic	ADJ
cet-13155	4	23	processes	process	NOUN
cet-13155	4	24	with	with	ADP
cet-13155	4	25	syngas	syngas	NOUN
cet-13155	4	26	co	co	NOUN
cet-13155	4	27	-	-	NOUN
cet-13155	4	28	feeding	feeding	NOUN
cet-13155	4	29	.	.	PUNCT
cet-13155	5	1	with	with	ADP
cet-13155	5	2	this	this	DET
cet-13155	5	3	purpose	purpose	NOUN
cet-13155	5	4	,	,	PUNCT
cet-13155	5	5	an	an	DET
cet-13155	5	6	in2o3	in2o3	PROPN
cet-13155	5	7	-	-	PUNCT
cet-13155	5	8	zro2	zro2	PROPN
cet-13155	5	9	(	(	PUNCT
cet-13155	5	10	inzr	inzr	NOUN
cet-13155	5	11	)	)	PUNCT
cet-13155	5	12	catalyst	catalyst	NOUN
cet-13155	5	13	alternative	alternative	NOUN
cet-13155	5	14	to	to	ADP
cet-13155	5	15	the	the	DET
cet-13155	5	16	traditional	traditional	ADJ
cet-13155	5	17	cu	cu	PROPN
cet-13155	5	18	-	-	PUNCT
cet-13155	5	19	zno	zno	NOUN
cet-13155	5	20	-	-	ADJ
cet-13155	5	21	zro2	zro2	PROPN
cet-13155	5	22	(	(	PUNCT
cet-13155	5	23	cuznzr	cuznzr	NOUN
cet-13155	5	24	)	)	PUNCT
cet-13155	5	25	for	for	ADP
cet-13155	5	26	methanol	methanol	NOUN
cet-13155	5	27	synthesis	synthesis	NOUN
cet-13155	5	28	(	(	PUNCT
cet-13155	5	29	as	as	ADP
cet-13155	5	30	the	the	DET
cet-13155	5	31	first	first	ADJ
cet-13155	5	32	stage	stage	NOUN
cet-13155	5	33	of	of	ADP
cet-13155	5	34	the	the	DET
cet-13155	5	35	direct	direct	ADJ
cet-13155	5	36	synthesis	synthesis	NOUN
cet-13155	5	37	of	of	ADP
cet-13155	5	38	hydrocarbons	hydrocarbon	NOUN
cet-13155	5	39	from	from	ADP
cet-13155	5	40	co2	co2	NOUN
cet-13155	5	41	/	/	SYM
cet-13155	5	42	co	co	NOUN
cet-13155	5	43	hydrogenation	hydrogenation	NOUN
cet-13155	5	44	)	)	PUNCT
cet-13155	5	45	was	be	AUX
cet-13155	5	46	assessed	assess	VERB
cet-13155	5	47	.	.	PUNCT
cet-13155	6	1	afterwards	afterwards	ADV
cet-13155	6	2	,	,	PUNCT
cet-13155	6	3	both	both	DET
cet-13155	6	4	catalysts	catalyst	NOUN
cet-13155	6	5	were	be	AUX
cet-13155	6	6	tested	test	VERB
cet-13155	6	7	in	in	ADP
cet-13155	6	8	tandem	tandem	NOUN
cet-13155	6	9	with	with	ADP
cet-13155	6	10	hzm-5	hzm-5	PUNCT
cet-13155	6	11	zeolite	zeolite	NOUN
cet-13155	6	12	for	for	ADP
cet-13155	6	13	the	the	DET
cet-13155	6	14	production	production	NOUN
cet-13155	6	15	of	of	ADP
cet-13155	6	16	fuel	fuel	NOUN
cet-13155	6	17	-	-	PUNCT
cet-13155	6	18	range	range	NOUN
cet-13155	6	19	hydrocarbons	hydrocarbon	NOUN
cet-13155	6	20	.	.	PUNCT
cet-13155	7	1	the	the	DET
cet-13155	7	2	catalysts	catalyst	NOUN
cet-13155	7	3	were	be	AUX
cet-13155	7	4	characterized	characterize	VERB
cet-13155	7	5	by	by	ADP
cet-13155	7	6	several	several	ADJ
cet-13155	7	7	techniques	technique	NOUN
cet-13155	7	8	and	and	CCONJ
cet-13155	7	9	ascertained	ascertain	VERB
cet-13155	7	10	by	by	ADP
cet-13155	7	11	means	mean	NOUN
cet-13155	7	12	of	of	ADP
cet-13155	7	13	reaction	reaction	NOUN
cet-13155	7	14	runs	run	NOUN
cet-13155	7	15	at	at	ADP
cet-13155	7	16	different	different	ADJ
cet-13155	7	17	operating	operating	NOUN
cet-13155	7	18	conditions	condition	NOUN
cet-13155	7	19	,	,	PUNCT
cet-13155	7	20	aiming	aim	VERB
cet-13155	7	21	to	to	PART
cet-13155	7	22	assess	assess	VERB
cet-13155	7	23	the	the	DET
cet-13155	7	24	effect	effect	NOUN
cet-13155	7	25	of	of	ADP
cet-13155	7	26	temperature	temperature	NOUN
cet-13155	7	27	on	on	ADP
cet-13155	7	28	the	the	DET
cet-13155	7	29	performance	performance	NOUN
cet-13155	7	30	.	.	PUNCT
cet-13155	8	1	even	even	ADV
cet-13155	8	2	if	if	SCONJ
cet-13155	8	3	cuznzr	cuznzr	NOUN
cet-13155	8	4	resulted	result	VERB
cet-13155	8	5	in	in	ADP
cet-13155	8	6	higher	high	ADJ
cet-13155	8	7	methanol	methanol	NOUN
cet-13155	8	8	production	production	NOUN
cet-13155	8	9	,	,	PUNCT
cet-13155	8	10	inzr	inzr	ADJ
cet-13155	8	11	catalyst	catalyst	NOUN
cet-13155	8	12	proved	prove	VERB
cet-13155	8	13	to	to	PART
cet-13155	8	14	be	be	AUX
cet-13155	8	15	the	the	DET
cet-13155	8	16	most	most	ADV
cet-13155	8	17	adequate	adequate	ADJ
cet-13155	8	18	catalyst	catalyst	NOUN
cet-13155	8	19	for	for	ADP
cet-13155	8	20	the	the	DET
cet-13155	8	21	integrated	integrate	VERB
cet-13155	8	22	process	process	NOUN
cet-13155	8	23	,	,	PUNCT
cet-13155	8	24	since	since	SCONJ
cet-13155	8	25	cuznzr	cuznzr	ADJ
cet-13155	8	26	sintered	sinter	VERB
cet-13155	8	27	at	at	ADP
cet-13155	8	28	temperatures	temperature	NOUN
cet-13155	8	29	above	above	ADP
cet-13155	8	30	300	300	NUM
cet-13155	8	31	ºc	ºc	NOUN
cet-13155	8	32	(	(	PUNCT
cet-13155	8	33	needed	need	VERB
cet-13155	8	34	for	for	ADP
cet-13155	8	35	the	the	DET
cet-13155	8	36	conversion	conversion	NOUN
cet-13155	8	37	of	of	ADP
cet-13155	8	38	methanol	methanol	NOUN
cet-13155	8	39	to	to	ADP
cet-13155	8	40	hydrocarbons	hydrocarbon	NOUN
cet-13155	8	41	)	)	PUNCT
cet-13155	8	42	.	.	PUNCT
cet-13155	9	1	with	with	ADP
cet-13155	9	2	inzr	inzr	NOUN
cet-13155	9	3	/	/	SYM
cet-13155	9	4	hzsm-5	hzsm-5	NOUN
cet-13155	9	5	catalyst	catalyst	NOUN
cet-13155	9	6	,	,	PUNCT
cet-13155	9	7	c5	c5	PROPN
cet-13155	9	8	+	+	CCONJ
cet-13155	9	9	hydrocarbon	hydrocarbon	NOUN
cet-13155	9	10	yield	yield	NOUN
cet-13155	9	11	near	near	ADP
cet-13155	9	12	20	20	NUM
cet-13155	9	13	%	%	NOUN
cet-13155	9	14	was	be	AUX
cet-13155	9	15	obtained	obtain	VERB
cet-13155	9	16	at	at	ADP
cet-13155	9	17	420	420	NUM
cet-13155	9	18	ºc	ºc	NUM
cet-13155	9	19	and	and	CCONJ
cet-13155	9	20	50	50	NUM
cet-13155	9	21	bar	bar	NOUN
cet-13155	9	22	,	,	PUNCT
cet-13155	9	23	with	with	ADP
cet-13155	9	24	a	a	DET
cet-13155	9	25	cox	cox	PROPN
cet-13155	9	26	conversion	conversion	NOUN
cet-13155	9	27	of	of	ADP
cet-13155	9	28	23	23	NUM
cet-13155	9	29	%	%	NOUN
cet-13155	9	30	,	,	PUNCT
cet-13155	9	31	by	by	ADP
cet-13155	9	32	feeding	feed	VERB
cet-13155	9	33	a	a	DET
cet-13155	9	34	co2	co2	NOUN
cet-13155	9	35	/	/	SYM
cet-13155	9	36	co	co	NOUN
cet-13155	9	37	equimolar	equimolar	NOUN
cet-13155	9	38	mixture	mixture	NOUN
cet-13155	9	39	,	,	PUNCT
cet-13155	9	40	and	and	CCONJ
cet-13155	9	41	with	with	ADP
cet-13155	9	42	a	a	DET
cet-13155	9	43	h2	h2	PROPN
cet-13155	9	44	/	/	SYM
cet-13155	9	45	cox	cox	PROPN
cet-13155	9	46	ratio	ratio	NOUN
cet-13155	9	47	of	of	ADP
cet-13155	9	48	3	3	NUM
cet-13155	9	49	.	.	NOUN
cet-13155	9	50	1	1	NUM
cet-13155	9	51	.	.	X
cet-13155	10	1	introduction	introduction	NOUN
cet-13155	10	2	climate	climate	NOUN
cet-13155	10	3	change	change	NOUN
cet-13155	10	4	,	,	PUNCT
cet-13155	10	5	rising	rise	VERB
cet-13155	10	6	co2	co2	NOUN
cet-13155	10	7	emissions	emission	NOUN
cet-13155	10	8	and	and	CCONJ
cet-13155	10	9	global	global	ADJ
cet-13155	10	10	warming	warming	NOUN
cet-13155	10	11	have	have	AUX
cet-13155	10	12	put	put	VERB
cet-13155	10	13	carbon	carbon	NOUN
cet-13155	10	14	capture	capture	NOUN
cet-13155	10	15	and	and	CCONJ
cet-13155	10	16	utilization	utilization	NOUN
cet-13155	10	17	(	(	PUNCT
cet-13155	10	18	ccu	ccu	NOUN
cet-13155	10	19	)	)	PUNCT
cet-13155	10	20	technologies	technology	NOUN
cet-13155	10	21	in	in	ADP
cet-13155	10	22	the	the	DET
cet-13155	10	23	spotlight	spotlight	NOUN
cet-13155	10	24	.	.	PUNCT
cet-13155	11	1	among	among	ADP
cet-13155	11	2	the	the	DET
cet-13155	11	3	most	most	ADV
cet-13155	11	4	attractive	attractive	ADJ
cet-13155	11	5	co2	co2	NOUN
cet-13155	11	6	utilization	utilization	NOUN
cet-13155	11	7	processes	process	NOUN
cet-13155	11	8	,	,	PUNCT
cet-13155	11	9	its	its	PRON
cet-13155	11	10	conversion	conversion	NOUN
cet-13155	11	11	into	into	ADP
cet-13155	11	12	hydrocarbons	hydrocarbon	NOUN
cet-13155	11	13	stands	stand	VERB
cet-13155	11	14	out	out	ADP
cet-13155	11	15	(	(	PUNCT
cet-13155	11	16	saeidi	saeidi	PROPN
cet-13155	11	17	et	et	PROPN
cet-13155	11	18	al	al	PROPN
cet-13155	11	19	.	.	PROPN
cet-13155	11	20	,	,	PUNCT
cet-13155	11	21	2021	2021	NUM
cet-13155	11	22	)	)	PUNCT
cet-13155	11	23	,	,	PUNCT
cet-13155	11	24	especially	especially	ADV
cet-13155	11	25	through	through	ADP
cet-13155	11	26	catalytic	catalytic	ADJ
cet-13155	11	27	processes	process	NOUN
cet-13155	11	28	,	,	PUNCT
cet-13155	11	29	which	which	PRON
cet-13155	11	30	can	can	AUX
cet-13155	11	31	also	also	ADV
cet-13155	11	32	be	be	AUX
cet-13155	11	33	performed	perform	VERB
cet-13155	11	34	co	co	ADJ
cet-13155	11	35	-	-	VERB
cet-13155	11	36	feeding	feed	VERB
cet-13155	11	37	sustainably	sustainably	ADV
cet-13155	11	38	obtained	obtain	VERB
cet-13155	11	39	syngas	syngas	NOUN
cet-13155	11	40	(	(	PUNCT
cet-13155	11	41	from	from	ADP
cet-13155	11	42	biomass	biomass	NOUN
cet-13155	11	43	or	or	CCONJ
cet-13155	11	44	waste	waste	NOUN
cet-13155	11	45	)	)	PUNCT
cet-13155	11	46	.	.	PUNCT
cet-13155	12	1	currently	currently	ADV
cet-13155	12	2	,	,	PUNCT
cet-13155	12	3	addressing	address	VERB
cet-13155	12	4	the	the	DET
cet-13155	12	5	need	need	NOUN
cet-13155	12	6	for	for	ADP
cet-13155	12	7	using	use	VERB
cet-13155	12	8	sustainably	sustainably	ADV
cet-13155	12	9	sourced	source	VERB
cet-13155	12	10	fuels	fuel	NOUN
cet-13155	12	11	as	as	ADP
cet-13155	12	12	consequence	consequence	NOUN
cet-13155	12	13	of	of	ADP
cet-13155	12	14	the	the	DET
cet-13155	12	15	fossil	fossil	ADJ
cet-13155	12	16	fuels	fuel	NOUN
cet-13155	12	17	scarcity	scarcity	NOUN
cet-13155	12	18	,	,	PUNCT
cet-13155	12	19	research	research	NOUN
cet-13155	12	20	is	be	AUX
cet-13155	12	21	focused	focus	VERB
cet-13155	12	22	on	on	ADP
cet-13155	12	23	the	the	DET
cet-13155	12	24	production	production	NOUN
cet-13155	12	25	of	of	ADP
cet-13155	12	26	hydrocarbons	hydrocarbon	NOUN
cet-13155	12	27	by	by	ADP
cet-13155	12	28	co2	co2	NOUN
cet-13155	12	29	/	/	SYM
cet-13155	12	30	co	co	NOUN
cet-13155	12	31	hydrogenation	hydrogenation	NOUN
cet-13155	12	32	.	.	PUNCT
cet-13155	13	1	these	these	DET
cet-13155	13	2	processes	process	NOUN
cet-13155	13	3	may	may	AUX
cet-13155	13	4	be	be	AUX
cet-13155	13	5	conducted	conduct	VERB
cet-13155	13	6	following	follow	VERB
cet-13155	13	7	:	:	PUNCT
cet-13155	13	8	(	(	PUNCT
cet-13155	13	9	i	i	NOUN
cet-13155	13	10	)	)	PUNCT
cet-13155	13	11	the	the	DET
cet-13155	13	12	modified	modify	VERB
cet-13155	13	13	fischer	fischer	PROPN
cet-13155	13	14	tropsch	tropsch	PROPN
cet-13155	13	15	route	route	PROPN
cet-13155	13	16	(	(	PUNCT
cet-13155	13	17	kim	kim	PROPN
cet-13155	13	18	et	et	PROPN
cet-13155	13	19	al	al	PROPN
cet-13155	13	20	.	.	PROPN
cet-13155	13	21	,	,	PUNCT
cet-13155	13	22	2022	2022	NUM
cet-13155	13	23	)	)	PUNCT
cet-13155	13	24	,	,	PUNCT
cet-13155	13	25	in	in	ADP
cet-13155	13	26	which	which	PRON
cet-13155	13	27	co2	co2	NOUN
cet-13155	13	28	is	be	AUX
cet-13155	13	29	firstly	firstly	ADV
cet-13155	13	30	converted	convert	VERB
cet-13155	13	31	to	to	PART
cet-13155	13	32	co	co	VERB
cet-13155	13	33	(	(	PUNCT
cet-13155	13	34	through	through	ADP
cet-13155	13	35	the	the	DET
cet-13155	13	36	rwgs	rwgs	NOUN
cet-13155	13	37	reaction	reaction	NOUN
cet-13155	13	38	)	)	PUNCT
cet-13155	13	39	,	,	PUNCT
cet-13155	13	40	and	and	CCONJ
cet-13155	13	41	later	later	ADV
cet-13155	13	42	converted	convert	VERB
cet-13155	13	43	into	into	ADP
cet-13155	13	44	hydrocarbons	hydrocarbon	NOUN
cet-13155	13	45	by	by	ADP
cet-13155	13	46	the	the	DET
cet-13155	13	47	traditional	traditional	ADJ
cet-13155	13	48	fischer	fischer	NOUN
cet-13155	13	49	tropsch	tropsch	PROPN
cet-13155	13	50	synthesis	synthesis	NOUN
cet-13155	13	51	;	;	PUNCT
cet-13155	13	52	and	and	CCONJ
cet-13155	13	53	(	(	PUNCT
cet-13155	13	54	ii	ii	NOUN
cet-13155	13	55	)	)	PUNCT
cet-13155	13	56	the	the	DET
cet-13155	13	57	route	route	NOUN
cet-13155	13	58	with	with	ADP
cet-13155	13	59	oxygenates	oxygenate	NOUN
cet-13155	13	60	(	(	PUNCT
cet-13155	13	61	methanol	methanol	NOUN
cet-13155	13	62	/	/	SYM
cet-13155	13	63	dme	dme	PROPN
cet-13155	13	64	)	)	PUNCT
cet-13155	13	65	as	as	ADP
cet-13155	13	66	intermediates	intermediate	NOUN
cet-13155	13	67	(	(	PUNCT
cet-13155	13	68	ateka	ateka	PROPN
cet-13155	13	69	et	et	PROPN
cet-13155	13	70	al	al	PROPN
cet-13155	13	71	.	.	PROPN
cet-13155	13	72	,	,	PUNCT
cet-13155	13	73	2022	2022	NUM
cet-13155	13	74	)	)	PUNCT
cet-13155	13	75	.	.	PUNCT
cet-13155	14	1	meanwhile	meanwhile	ADV
cet-13155	14	2	,	,	PUNCT
cet-13155	14	3	the	the	DET
cet-13155	14	4	latter	latter	ADJ
cet-13155	14	5	can	can	AUX
cet-13155	14	6	be	be	AUX
cet-13155	14	7	performed	perform	VERB
cet-13155	14	8	through	through	ADP
cet-13155	14	9	indirect	indirect	ADJ
cet-13155	14	10	or	or	CCONJ
cet-13155	14	11	direct	direct	ADJ
cet-13155	14	12	routes	route	NOUN
cet-13155	14	13	.	.	PUNCT
cet-13155	15	1	the	the	DET
cet-13155	15	2	indirect	indirect	ADJ
cet-13155	15	3	synthesis	synthesis	NOUN
cet-13155	15	4	consists	consist	VERB
cet-13155	15	5	of	of	ADP
cet-13155	15	6	two	two	NUM
cet-13155	15	7	reaction	reaction	NOUN
cet-13155	15	8	stages	stage	NOUN
cet-13155	15	9	:	:	PUNCT
cet-13155	15	10	(	(	PUNCT
cet-13155	15	11	i	i	NOUN
cet-13155	15	12	)	)	PUNCT
cet-13155	15	13	the	the	DET
cet-13155	15	14	synthesis	synthesis	NOUN
cet-13155	15	15	of	of	ADP
cet-13155	15	16	methanol	methanol	NOUN
cet-13155	15	17	by	by	ADP
cet-13155	15	18	co2	co2	NOUN
cet-13155	15	19	/	/	SYM
cet-13155	15	20	co	co	NOUN
cet-13155	15	21	hydrogenation	hydrogenation	NOUN
cet-13155	15	22	(	(	PUNCT
cet-13155	15	23	eqs	eqs	X
cet-13155	15	24	(	(	PUNCT
cet-13155	15	25	1	1	NUM
cet-13155	15	26	)	)	PUNCT
cet-13155	15	27	and	and	CCONJ
cet-13155	15	28	(	(	PUNCT
cet-13155	15	29	2	2	NUM
cet-13155	15	30	)	)	PUNCT
cet-13155	15	31	)	)	PUNCT
cet-13155	15	32	in	in	ADP
cet-13155	15	33	a	a	DET
cet-13155	15	34	first	first	ADJ
cet-13155	15	35	stage	stage	NOUN
cet-13155	15	36	and	and	CCONJ
cet-13155	15	37	(	(	PUNCT
cet-13155	15	38	ii	ii	NOUN
cet-13155	15	39	)	)	PUNCT
cet-13155	15	40	its	its	PRON
cet-13155	15	41	subsequent	subsequent	ADJ
cet-13155	15	42	conversion	conversion	NOUN
cet-13155	15	43	to	to	ADP
cet-13155	15	44	higher	high	ADJ
cet-13155	15	45	hydrocarbons	hydrocarbon	NOUN
cet-13155	15	46	.	.	PUNCT
cet-13155	16	1	co2	co2	NOUN
cet-13155	16	2	+	+	CCONJ
cet-13155	16	3	3h2	3h2	NUM
cet-13155	16	4	↔	↔	PROPN
cet-13155	16	5	ch3oh	ch3oh	NOUN
cet-13155	17	1	+	+	NUM
cet-13155	17	2	h2o	h2o	PROPN
cet-13155	17	3	(	(	PUNCT
cet-13155	17	4	1	1	NUM
cet-13155	17	5	)	)	PUNCT
cet-13155	17	6	co	co	NOUN
cet-13155	18	1	+	+	NUM
cet-13155	18	2	2h2	2h2	NUM
cet-13155	18	3	↔	↔	PROPN
cet-13155	18	4	ch3oh	ch3oh	X
cet-13155	18	5	(	(	PUNCT
cet-13155	18	6	2	2	NUM
cet-13155	18	7	)	)	PUNCT
cet-13155	18	8	methanol	methanol	NOUN
cet-13155	18	9	synthesis	synthesis	NOUN
cet-13155	18	10	is	be	AUX
cet-13155	18	11	attributed	attribute	VERB
cet-13155	18	12	to	to	ADP
cet-13155	18	13	the	the	DET
cet-13155	18	14	reaction	reaction	NOUN
cet-13155	18	15	mechanism	mechanism	NOUN
cet-13155	18	16	with	with	ADP
cet-13155	18	17	formate	formate	NOUN
cet-13155	18	18	ions	ion	NOUN
cet-13155	18	19	(	(	PUNCT
cet-13155	18	20	hcoo	hcoo	NOUN
cet-13155	18	21	*	*	PUNCT
cet-13155	18	22	)	)	PUNCT
cet-13155	18	23	as	as	ADP
cet-13155	18	24	intermediate	intermediate	ADJ
cet-13155	18	25	species	specie	NOUN
cet-13155	18	26	,	,	PUNCT
cet-13155	18	27	and	and	CCONJ
cet-13155	18	28	to	to	ADP
cet-13155	18	29	the	the	DET
cet-13155	18	30	further	further	ADJ
cet-13155	18	31	hydrogenation	hydrogenation	NOUN
cet-13155	18	32	of	of	ADP
cet-13155	18	33	co2	co2	NOUN
cet-13155	18	34	(	(	PUNCT
cet-13155	18	35	grabow	grabow	PROPN
cet-13155	18	36	and	and	CCONJ
cet-13155	18	37	mavrikakis	mavrikaki	NOUN
cet-13155	18	38	,	,	PUNCT
cet-13155	18	39	2011	2011	NUM
cet-13155	18	40	)	)	PUNCT
cet-13155	18	41	.	.	PUNCT
cet-13155	19	1	these	these	DET
cet-13155	19	2	reactions	reaction	NOUN
cet-13155	19	3	are	be	AUX
cet-13155	19	4	exothermic	exothermic	ADJ
cet-13155	19	5	,	,	PUNCT
cet-13155	19	6	and	and	CCONJ
cet-13155	19	7	thus	thus	ADV
cet-13155	19	8	,	,	PUNCT
cet-13155	19	9	they	they	PRON
cet-13155	19	10	are	be	AUX
cet-13155	19	11	favored	favor	VERB
cet-13155	19	12	at	at	ADP
cet-13155	19	13	low	low	ADJ
cet-13155	19	14	temperature	temperature	NOUN
cet-13155	19	15	and	and	CCONJ
cet-13155	19	16	high	high	ADJ
cet-13155	19	17	pressure	pressure	NOUN
cet-13155	19	18	,	,	PUNCT
cet-13155	19	19	demanding	demand	VERB
cet-13155	19	20	highly	highly	ADV
cet-13155	19	21	active	active	ADJ
cet-13155	19	22	catalysts	catalyst	NOUN
cet-13155	19	23	working	work	VERB
cet-13155	19	24	in	in	ADP
cet-13155	19	25	these	these	DET
cet-13155	19	26	reaction	reaction	NOUN
cet-13155	19	27	conditions	condition	NOUN
cet-13155	19	28	(	(	PUNCT
cet-13155	19	29	zhang	zhang	X
cet-13155	19	30	et	et	PROPN
cet-13155	19	31	al	al	PROPN
cet-13155	19	32	.	.	PROPN
cet-13155	19	33	,	,	PUNCT
cet-13155	19	34	2021	2021	NUM
cet-13155	19	35	)	)	PUNCT
cet-13155	19	36	.	.	PUNCT
cet-13155	20	1	in	in	ADP
cet-13155	20	2	this	this	DET
cet-13155	20	3	field	field	NOUN
cet-13155	20	4	,	,	PUNCT
cet-13155	20	5	metallic	metallic	ADJ
cet-13155	20	6	oxides	oxide	NOUN
cet-13155	20	7	are	be	AUX
cet-13155	20	8	the	the	DET
cet-13155	20	9	most	most	ADV
cet-13155	20	10	suitable	suitable	ADJ
cet-13155	20	11	alternatives	alternative	NOUN
cet-13155	20	12	,	,	PUNCT
cet-13155	20	13	although	although	SCONJ
cet-13155	20	14	temperature	temperature	NOUN
cet-13155	20	15	above	above	ADP
cet-13155	20	16	250	250	NUM
cet-13155	20	17	ºc	ºc	PROPN
cet-13155	20	18	is	be	AUX
cet-13155	20	19	needed	need	VERB
cet-13155	20	20	in	in	ADP
cet-13155	20	21	order	order	NOUN
cet-13155	20	22	to	to	PART
cet-13155	20	23	favor	favor	VERB
cet-13155	20	24	the	the	DET
cet-13155	20	25	reaction	reaction	NOUN
cet-13155	20	26	rate	rate	NOUN
cet-13155	20	27	of	of	ADP
cet-13155	20	28	methanol	methanol	NOUN
cet-13155	20	29	formation	formation	NOUN
cet-13155	20	30	(	(	PUNCT
cet-13155	20	31	samiee	samiee	NOUN
cet-13155	20	32	and	and	CCONJ
cet-13155	20	33	457	457	NUM
cet-13155	20	34	mailto:onintze.parra@ehu.eus	mailto:onintze.parra@ehu.eus	NOUN
cet-13155	20	35	gandzha	gandzha	NOUN
cet-13155	20	36	,	,	PUNCT
cet-13155	20	37	2019	2019	NUM
cet-13155	20	38	)	)	PUNCT
cet-13155	20	39	.	.	PUNCT
cet-13155	21	1	nonetheless	nonetheless	ADV
cet-13155	21	2	,	,	PUNCT
cet-13155	21	3	it	it	PRON
cet-13155	21	4	will	will	AUX
cet-13155	21	5	also	also	ADV
cet-13155	21	6	boost	boost	VERB
cet-13155	21	7	the	the	DET
cet-13155	21	8	side	side	NOUN
cet-13155	21	9	formation	formation	NOUN
cet-13155	21	10	of	of	ADP
cet-13155	21	11	co	co	X
cet-13155	21	12	by	by	ADP
cet-13155	21	13	the	the	DET
cet-13155	21	14	reverse	reverse	ADJ
cet-13155	21	15	water	water	NOUN
cet-13155	21	16	gas	gas	NOUN
cet-13155	21	17	shift	shift	NOUN
cet-13155	21	18	(	(	PUNCT
cet-13155	21	19	rwgs	rwgs	NOUN
cet-13155	21	20	)	)	PUNCT
cet-13155	21	21	reaction	reaction	NOUN
cet-13155	21	22	(	(	PUNCT
cet-13155	21	23	eq	eq	NOUN
cet-13155	21	24	(	(	PUNCT
cet-13155	21	25	3	3	NUM
cet-13155	21	26	)	)	PUNCT
cet-13155	21	27	)	)	PUNCT
cet-13155	21	28	and	and	CCONJ
cet-13155	21	29	the	the	DET
cet-13155	21	30	methanation	methanation	NOUN
cet-13155	21	31	reactions	reaction	NOUN
cet-13155	21	32	(	(	PUNCT
cet-13155	21	33	eqs	eqs	X
cet-13155	21	34	(	(	PUNCT
cet-13155	21	35	4	4	NUM
cet-13155	21	36	)	)	PUNCT
cet-13155	21	37	and	and	CCONJ
cet-13155	21	38	(	(	PUNCT
cet-13155	21	39	5	5	NUM
cet-13155	21	40	)	)	PUNCT
cet-13155	21	41	)	)	PUNCT
cet-13155	21	42	.	.	PUNCT
cet-13155	22	1	co2	co2	NOUN
cet-13155	22	2	+	+	PROPN
cet-13155	22	3	h2	h2	NOUN
cet-13155	22	4	↔	↔	PROPN
cet-13155	22	5	co	co	NOUN
cet-13155	22	6	+	+	PROPN
cet-13155	22	7	h2o	h2o	PROPN
cet-13155	22	8	(	(	PUNCT
cet-13155	22	9	3	3	X
cet-13155	22	10	)	)	PUNCT
cet-13155	22	11	co2	co2	NOUN
cet-13155	22	12	+	+	CCONJ
cet-13155	22	13	4h2	4h2	NUM
cet-13155	22	14	↔	↔	PROPN
cet-13155	22	15	ch4	ch4	NOUN
cet-13155	22	16	+	+	CCONJ
cet-13155	22	17	2h2o	2h2o	NUM
cet-13155	22	18	(	(	PUNCT
cet-13155	22	19	4	4	NUM
cet-13155	22	20	)	)	PUNCT
cet-13155	22	21	co	co	NOUN
cet-13155	23	1	+	+	NOUN
cet-13155	23	2	3h2	3h2	NUM
cet-13155	23	3	↔	↔	PROPN
cet-13155	23	4	ch4	ch4	NOUN
cet-13155	23	5	+	+	CCONJ
cet-13155	23	6	h2o	h2o	PROPN
cet-13155	23	7	(	(	PUNCT
cet-13155	23	8	5	5	NUM
cet-13155	23	9	)	)	PUNCT
cet-13155	23	10	the	the	DET
cet-13155	23	11	synthesized	synthesize	VERB
cet-13155	23	12	methanol	methanol	NOUN
cet-13155	23	13	is	be	AUX
cet-13155	23	14	converted	convert	VERB
cet-13155	23	15	into	into	ADP
cet-13155	23	16	hydrocarbons	hydrocarbon	NOUN
cet-13155	23	17	by	by	ADP
cet-13155	23	18	means	mean	NOUN
cet-13155	23	19	of	of	ADP
cet-13155	23	20	an	an	DET
cet-13155	23	21	acid	acid	NOUN
cet-13155	23	22	catalyst	catalyst	NOUN
cet-13155	23	23	,	,	PUNCT
cet-13155	23	24	typically	typically	ADV
cet-13155	23	25	zeolites	zeolite	NOUN
cet-13155	23	26	.	.	PUNCT
cet-13155	24	1	this	this	DET
cet-13155	24	2	reaction	reaction	NOUN
cet-13155	24	3	stage	stage	NOUN
cet-13155	24	4	(	(	PUNCT
cet-13155	24	5	eq	eq	NOUN
cet-13155	24	6	(	(	PUNCT
cet-13155	24	7	6	6	NUM
cet-13155	24	8	)	)	PUNCT
cet-13155	24	9	)	)	PUNCT
cet-13155	24	10	is	be	AUX
cet-13155	24	11	favored	favor	VERB
cet-13155	24	12	at	at	ADP
cet-13155	24	13	high	high	ADJ
cet-13155	24	14	temperature	temperature	NOUN
cet-13155	24	15	(	(	PUNCT
cet-13155	24	16	>	>	SYM
cet-13155	24	17	300	300	NUM
cet-13155	24	18	ºc	ºc	NUM
cet-13155	24	19	)	)	PUNCT
cet-13155	24	20	and	and	CCONJ
cet-13155	24	21	takes	take	VERB
cet-13155	24	22	places	place	NOUN
cet-13155	24	23	by	by	ADP
cet-13155	24	24	way	way	NOUN
cet-13155	24	25	of	of	ADP
cet-13155	24	26	the	the	DET
cet-13155	24	27	dual	dual	ADJ
cet-13155	24	28	cycle	cycle	NOUN
cet-13155	24	29	mechanism	mechanism	NOUN
cet-13155	24	30	with	with	ADP
cet-13155	24	31	olefins	olefin	NOUN
cet-13155	24	32	and	and	CCONJ
cet-13155	24	33	arenes	arene	NOUN
cet-13155	24	34	as	as	ADP
cet-13155	24	35	intermediates	intermediate	NOUN
cet-13155	24	36	.	.	PUNCT
cet-13155	25	1	2𝐶𝐻3𝑂𝐻	2𝐶𝐻3𝑂𝐻	NUM
cet-13155	26	1	+	+	NOUN
cet-13155	26	2	𝐻2𝑂	𝐻2𝑂	PRON
cet-13155	26	3	⇋	⇋	PUNCT
cet-13155	26	4	−𝐻2𝑂	−𝐻2𝑂	ADV
cet-13155	26	5	𝐶𝐻3𝑂𝐶𝐻3	𝐶𝐻3𝑂𝐶𝐻3	NOUN
cet-13155	26	6	−𝐻2𝑂	−𝐻2𝑂	ADV
cet-13155	26	7	→	→	PUNCT
cet-13155	26	8	𝐿𝑖𝑔ℎ𝑡	𝐿𝑖𝑔ℎ𝑡	PROPN
cet-13155	26	9	𝑂𝑙𝑒𝑓𝑖𝑛𝑠	𝑂𝑙𝑒𝑓𝑖𝑛𝑠	PROPN
cet-13155	26	10	⟶	⟶	NOUN
cet-13155	26	11	𝑛/𝑖𝑠𝑜𝑝𝑎𝑟𝑎𝑓𝑓𝑖𝑛𝑠	𝑛/𝑖𝑠𝑜𝑝𝑎𝑟𝑎𝑓𝑓𝑖𝑛𝑠	CCONJ
cet-13155	26	12	𝐻𝑖𝑔ℎ𝑒𝑟	𝐻𝑖𝑔ℎ𝑒𝑟	PROPN
cet-13155	26	13	𝑂𝑙𝑒𝑓𝑖𝑛𝑠	𝑂𝑙𝑒𝑓𝑖𝑛𝑠	PROPN
cet-13155	26	14	𝐴𝑟𝑜𝑚𝑎𝑡𝑖𝑐𝑠/𝑛𝑎𝑝𝑡ℎ𝑒𝑛𝑒𝑠	𝐴𝑟𝑜𝑚𝑎𝑡𝑖𝑐𝑠/𝑛𝑎𝑝𝑡ℎ𝑒𝑛𝑒𝑠	PROPN
cet-13155	26	15	(	(	PUNCT
cet-13155	26	16	6	6	NUM
cet-13155	26	17	)	)	PUNCT
cet-13155	26	18	as	as	SCONJ
cet-13155	26	19	pointed	point	VERB
cet-13155	26	20	out	out	ADP
cet-13155	26	21	above	above	ADV
cet-13155	26	22	,	,	PUNCT
cet-13155	26	23	the	the	DET
cet-13155	26	24	hydrogenation	hydrogenation	NOUN
cet-13155	26	25	of	of	ADP
cet-13155	26	26	co2	co2	NOUN
cet-13155	26	27	/	/	SYM
cet-13155	26	28	co	co	NOUN
cet-13155	26	29	can	can	AUX
cet-13155	26	30	be	be	AUX
cet-13155	26	31	also	also	ADV
cet-13155	26	32	carried	carry	VERB
cet-13155	26	33	out	out	ADP
cet-13155	26	34	by	by	ADP
cet-13155	26	35	the	the	DET
cet-13155	26	36	direct	direct	ADJ
cet-13155	26	37	route	route	NOUN
cet-13155	26	38	,	,	PUNCT
cet-13155	26	39	integrating	integrate	VERB
cet-13155	26	40	both	both	DET
cet-13155	26	41	reaction	reaction	NOUN
cet-13155	26	42	stages	stage	NOUN
cet-13155	26	43	in	in	ADP
cet-13155	26	44	the	the	DET
cet-13155	26	45	same	same	ADJ
cet-13155	26	46	reactor	reactor	NOUN
cet-13155	26	47	.	.	PUNCT
cet-13155	27	1	for	for	ADP
cet-13155	27	2	this	this	DET
cet-13155	27	3	purpose	purpose	NOUN
cet-13155	27	4	,	,	PUNCT
cet-13155	27	5	tandem	tandem	NOUN
cet-13155	27	6	catalysts	catalyst	NOUN
cet-13155	27	7	,	,	PUNCT
cet-13155	27	8	consisting	consist	VERB
cet-13155	27	9	of	of	ADP
cet-13155	27	10	a	a	DET
cet-13155	27	11	metallic	metallic	ADJ
cet-13155	27	12	oxide	oxide	NOUN
cet-13155	27	13	and	and	CCONJ
cet-13155	27	14	a	a	DET
cet-13155	27	15	zeotype	zeotype	NOUN
cet-13155	27	16	,	,	PUNCT
cet-13155	27	17	are	be	AUX
cet-13155	27	18	used	use	VERB
cet-13155	27	19	.	.	PUNCT
cet-13155	28	1	in	in	ADP
cet-13155	28	2	order	order	NOUN
cet-13155	28	3	to	to	PART
cet-13155	28	4	achieve	achieve	VERB
cet-13155	28	5	high	high	ADJ
cet-13155	28	6	conversion	conversion	NOUN
cet-13155	28	7	,	,	PUNCT
cet-13155	28	8	optimizing	optimize	VERB
cet-13155	28	9	the	the	DET
cet-13155	28	10	operating	operating	NOUN
cet-13155	28	11	conditions	condition	NOUN
cet-13155	28	12	is	be	AUX
cet-13155	28	13	fundamental	fundamental	ADJ
cet-13155	28	14	for	for	ADP
cet-13155	28	15	ensuring	ensure	VERB
cet-13155	28	16	both	both	CCONJ
cet-13155	28	17	high	high	ADJ
cet-13155	28	18	methanol	methanol	NOUN
cet-13155	28	19	synthesis	synthesis	NOUN
cet-13155	28	20	and	and	CCONJ
cet-13155	28	21	consequently	consequently	ADV
cet-13155	28	22	,	,	PUNCT
cet-13155	28	23	high	high	ADJ
cet-13155	28	24	formation	formation	NOUN
cet-13155	28	25	of	of	ADP
cet-13155	28	26	hydrocarbons	hydrocarbon	NOUN
cet-13155	28	27	.	.	PUNCT
cet-13155	29	1	therefore	therefore	ADV
cet-13155	29	2	,	,	PUNCT
cet-13155	29	3	the	the	DET
cet-13155	29	4	thermal	thermal	ADJ
cet-13155	29	5	limitation	limitation	NOUN
cet-13155	29	6	of	of	ADP
cet-13155	29	7	cu	cu	PROPN
cet-13155	29	8	-	-	PUNCT
cet-13155	29	9	based	base	VERB
cet-13155	29	10	catalysts	catalyst	NOUN
cet-13155	29	11	due	due	ADP
cet-13155	29	12	to	to	ADP
cet-13155	29	13	the	the	DET
cet-13155	29	14	sintering	sintering	NOUN
cet-13155	29	15	of	of	ADP
cet-13155	29	16	cu	cu	PROPN
cet-13155	29	17	in	in	ADP
cet-13155	29	18	the	the	DET
cet-13155	29	19	conditions	condition	NOUN
cet-13155	29	20	required	require	VERB
cet-13155	29	21	for	for	ADP
cet-13155	29	22	the	the	DET
cet-13155	29	23	integrated	integrate	VERB
cet-13155	29	24	process	process	NOUN
cet-13155	29	25	makes	make	VERB
cet-13155	29	26	the	the	DET
cet-13155	29	27	screening	screening	NOUN
cet-13155	29	28	of	of	ADP
cet-13155	29	29	an	an	DET
cet-13155	29	30	active	active	ADJ
cet-13155	29	31	and	and	CCONJ
cet-13155	29	32	stable	stable	ADJ
cet-13155	29	33	catalyst	catalyst	NOUN
cet-13155	29	34	a	a	DET
cet-13155	29	35	key	key	ADJ
cet-13155	29	36	target	target	NOUN
cet-13155	29	37	for	for	ADP
cet-13155	29	38	enhancing	enhance	VERB
cet-13155	29	39	the	the	DET
cet-13155	29	40	direct	direct	ADJ
cet-13155	29	41	synthesis	synthesis	NOUN
cet-13155	29	42	of	of	ADP
cet-13155	29	43	hydrocarbons	hydrocarbon	NOUN
cet-13155	29	44	from	from	ADP
cet-13155	29	45	co2	co2	NOUN
cet-13155	29	46	/	/	SYM
cet-13155	29	47	co	co	NOUN
cet-13155	29	48	hydrogenation	hydrogenation	NOUN
cet-13155	29	49	.	.	PUNCT
cet-13155	30	1	in	in	ADP
cet-13155	30	2	this	this	DET
cet-13155	30	3	regard	regard	NOUN
cet-13155	30	4	,	,	PUNCT
cet-13155	30	5	this	this	DET
cet-13155	30	6	work	work	NOUN
cet-13155	30	7	aims	aim	VERB
cet-13155	30	8	to	to	PART
cet-13155	30	9	deepen	deepen	VERB
cet-13155	30	10	in	in	ADP
cet-13155	30	11	the	the	DET
cet-13155	30	12	study	study	NOUN
cet-13155	30	13	of	of	ADP
cet-13155	30	14	an	an	DET
cet-13155	30	15	alternative	alternative	ADJ
cet-13155	30	16	in2o3	in2o3	PROPN
cet-13155	30	17	-	-	ADJ
cet-13155	30	18	zro2	zro2	ADJ
cet-13155	30	19	metallic	metallic	ADJ
cet-13155	30	20	catalyst	catalyst	NOUN
cet-13155	30	21	for	for	ADP
cet-13155	30	22	methanol	methanol	NOUN
cet-13155	30	23	synthesis	synthesis	NOUN
cet-13155	30	24	,	,	PUNCT
cet-13155	30	25	and	and	CCONJ
cet-13155	30	26	in	in	ADP
cet-13155	30	27	the	the	DET
cet-13155	30	28	optimization	optimization	NOUN
cet-13155	30	29	of	of	ADP
cet-13155	30	30	the	the	DET
cet-13155	30	31	operating	operating	NOUN
cet-13155	30	32	conditions	condition	NOUN
cet-13155	30	33	,	,	PUNCT
cet-13155	30	34	pursuing	pursue	VERB
cet-13155	30	35	the	the	DET
cet-13155	30	36	avoidance	avoidance	NOUN
cet-13155	30	37	of	of	ADP
cet-13155	30	38	sintering	sintering	NOUN
cet-13155	30	39	and	and	CCONJ
cet-13155	30	40	the	the	DET
cet-13155	30	41	feasibility	feasibility	NOUN
cet-13155	30	42	in	in	ADP
cet-13155	30	43	the	the	DET
cet-13155	30	44	integrated	integrate	VERB
cet-13155	30	45	co	co	NOUN
cet-13155	30	46	and	and	CCONJ
cet-13155	30	47	co2	co2	NOUN
cet-13155	30	48	hydrogenation	hydrogenation	NOUN
cet-13155	30	49	into	into	ADP
cet-13155	30	50	hydrocarbons	hydrocarbon	NOUN
cet-13155	30	51	.	.	PUNCT
cet-13155	31	1	for	for	ADP
cet-13155	31	2	that	that	PRON
cet-13155	31	3	,	,	PUNCT
cet-13155	31	4	in2o3	in2o3	PROPN
cet-13155	31	5	-	-	PUNCT
cet-13155	31	6	zro2	zro2	PROPN
cet-13155	31	7	(	(	PUNCT
cet-13155	31	8	inzr	inzr	NOUN
cet-13155	31	9	)	)	PUNCT
cet-13155	31	10	and	and	CCONJ
cet-13155	31	11	cuozno	cuozno	NOUN
cet-13155	31	12	-	-	PUNCT
cet-13155	31	13	zro2	zro2	PROPN
cet-13155	31	14	(	(	PUNCT
cet-13155	31	15	cuznzr	cuznzr	NOUN
cet-13155	31	16	)	)	PUNCT
cet-13155	31	17	catalysts	catalyst	NOUN
cet-13155	31	18	were	be	AUX
cet-13155	31	19	tested	test	VERB
cet-13155	31	20	initially	initially	ADV
cet-13155	31	21	under	under	ADP
cet-13155	31	22	several	several	ADJ
cet-13155	31	23	operating	operating	NOUN
cet-13155	31	24	conditions	condition	NOUN
cet-13155	31	25	,	,	PUNCT
cet-13155	31	26	in	in	ADP
cet-13155	31	27	order	order	NOUN
cet-13155	31	28	to	to	PART
cet-13155	31	29	compare	compare	VERB
cet-13155	31	30	their	their	PRON
cet-13155	31	31	effectiveness	effectiveness	NOUN
cet-13155	31	32	in	in	ADP
cet-13155	31	33	methanol	methanol	NOUN
cet-13155	31	34	synthesis	synthesis	NOUN
cet-13155	31	35	step	step	NOUN
cet-13155	31	36	.	.	PUNCT
cet-13155	32	1	afterwards	afterwards	ADV
cet-13155	32	2	,	,	PUNCT
cet-13155	32	3	the	the	DET
cet-13155	32	4	catalysts	catalyst	NOUN
cet-13155	32	5	were	be	AUX
cet-13155	32	6	assessed	assess	VERB
cet-13155	32	7	in	in	ADP
cet-13155	32	8	tandem	tandem	NOUN
cet-13155	32	9	with	with	ADP
cet-13155	32	10	hzsm-5	hzsm-5	NOUN
cet-13155	32	11	zeolite	zeolite	NOUN
cet-13155	32	12	(	(	PUNCT
cet-13155	32	13	inzr	inzr	NOUN
cet-13155	32	14	/	/	SYM
cet-13155	32	15	h5	h5	NOUN
cet-13155	32	16	and	and	CCONJ
cet-13155	32	17	cuznzr	cuznzr	ADJ
cet-13155	32	18	/	/	SYM
cet-13155	32	19	h5	h5	NOUN
cet-13155	32	20	)	)	PUNCT
cet-13155	32	21	as	as	SCONJ
cet-13155	32	22	to	to	PART
cet-13155	32	23	observe	observe	VERB
cet-13155	32	24	the	the	DET
cet-13155	32	25	effect	effect	NOUN
cet-13155	32	26	of	of	ADP
cet-13155	32	27	operating	operate	VERB
cet-13155	32	28	in	in	ADP
cet-13155	32	29	the	the	DET
cet-13155	32	30	integrated	integrate	VERB
cet-13155	32	31	process	process	NOUN
cet-13155	32	32	.	.	PUNCT
cet-13155	33	1	2	2	X
cet-13155	33	2	.	.	X
cet-13155	33	3	experimental	experimental	ADJ
cet-13155	33	4	section	section	NOUN
cet-13155	33	5	2.1	2.1	NUM
cet-13155	33	6	preparation	preparation	NOUN
cet-13155	33	7	and	and	CCONJ
cet-13155	33	8	characterization	characterization	NOUN
cet-13155	33	9	of	of	ADP
cet-13155	33	10	the	the	DET
cet-13155	33	11	catalysts	catalyst	NOUN
cet-13155	33	12	the	the	DET
cet-13155	33	13	metallic	metallic	ADJ
cet-13155	33	14	catalysts	catalyst	NOUN
cet-13155	33	15	(	(	PUNCT
cet-13155	33	16	cuznzr	cuznzr	ADJ
cet-13155	33	17	and	and	CCONJ
cet-13155	33	18	inzr	inzr	NOUN
cet-13155	33	19	)	)	PUNCT
cet-13155	33	20	used	use	VERB
cet-13155	33	21	for	for	ADP
cet-13155	33	22	the	the	DET
cet-13155	33	23	methanol	methanol	NOUN
cet-13155	33	24	synthesis	synthesis	NOUN
cet-13155	33	25	step	step	NOUN
cet-13155	33	26	were	be	AUX
cet-13155	33	27	synthesized	synthesize	VERB
cet-13155	33	28	by	by	ADP
cet-13155	33	29	coprecipitation	coprecipitation	NOUN
cet-13155	33	30	,	,	PUNCT
cet-13155	33	31	following	follow	VERB
cet-13155	33	32	the	the	DET
cet-13155	33	33	methods	method	NOUN
cet-13155	33	34	proposed	propose	VERB
cet-13155	33	35	by	by	ADP
cet-13155	33	36	sanchez	sanchez	PROPN
cet-13155	33	37	-	-	PUNCT
cet-13155	33	38	contador	contador	NOUN
cet-13155	33	39	et	et	PROPN
cet-13155	33	40	al	al	PROPN
cet-13155	33	41	.	.	PROPN
cet-13155	34	1	(	(	PUNCT
cet-13155	34	2	2018	2018	NUM
cet-13155	34	3	)	)	PUNCT
cet-13155	34	4	and	and	CCONJ
cet-13155	34	5	portillo	portillo	VERB
cet-13155	34	6	et	et	PROPN
cet-13155	34	7	al	al	PROPN
cet-13155	34	8	.	.	PROPN
cet-13155	35	1	(	(	PUNCT
cet-13155	35	2	2022	2022	NUM
cet-13155	35	3	)	)	PUNCT
cet-13155	35	4	.	.	PUNCT
cet-13155	36	1	for	for	ADP
cet-13155	36	2	preparing	prepare	VERB
cet-13155	36	3	cuznzr	cuznzr	NOUN
cet-13155	36	4	catalyst	catalyst	NOUN
cet-13155	36	5	,	,	PUNCT
cet-13155	36	6	with	with	ADP
cet-13155	36	7	a	a	DET
cet-13155	36	8	cu	cu	PROPN
cet-13155	36	9	:	:	PUNCT
cet-13155	36	10	zn	zn	NUM
cet-13155	36	11	:	:	PUNCT
cet-13155	36	12	zr	zr	NOUN
cet-13155	36	13	ratio	ratio	NOUN
cet-13155	36	14	of	of	ADP
cet-13155	36	15	2/1/1	2/1/1	NUM
cet-13155	36	16	,	,	PUNCT
cet-13155	36	17	an	an	DET
cet-13155	36	18	aqueous	aqueous	ADJ
cet-13155	36	19	solution	solution	NOUN
cet-13155	36	20	of	of	ADP
cet-13155	36	21	cu(no3)2	cu(no3)2	ADJ
cet-13155	36	22	,	,	PUNCT
cet-13155	36	23	zn(no3)2	zn(no3)2	NOUN
cet-13155	36	24	and	and	CCONJ
cet-13155	36	25	zro(no3)2	zro(no3)2	PROPN
cet-13155	36	26	(	(	PUNCT
cet-13155	36	27	1	1	NUM
cet-13155	36	28	m	m	NOUN
cet-13155	36	29	)	)	PUNCT
cet-13155	36	30	and	and	CCONJ
cet-13155	36	31	an	an	DET
cet-13155	36	32	aqueous	aqueous	ADJ
cet-13155	36	33	solution	solution	NOUN
cet-13155	36	34	of	of	ADP
cet-13155	36	35	na2co3	na2co3	ADJ
cet-13155	36	36	(	(	PUNCT
cet-13155	36	37	1	1	NUM
cet-13155	36	38	m	m	NOUN
cet-13155	36	39	)	)	PUNCT
cet-13155	36	40	as	as	SCONJ
cet-13155	36	41	precipitant	precipitant	NOUN
cet-13155	36	42	agent	agent	NOUN
cet-13155	36	43	were	be	AUX
cet-13155	36	44	prepared	prepare	VERB
cet-13155	36	45	,	,	PUNCT
cet-13155	36	46	and	and	CCONJ
cet-13155	36	47	added	add	VERB
cet-13155	36	48	dropwise	dropwise	NOUN
cet-13155	36	49	over	over	ADP
cet-13155	36	50	distilled	distil	VERB
cet-13155	36	51	water	water	NOUN
cet-13155	36	52	at	at	ADP
cet-13155	36	53	a	a	DET
cet-13155	36	54	constant	constant	ADJ
cet-13155	36	55	temperature	temperature	NOUN
cet-13155	36	56	of	of	ADP
cet-13155	36	57	70	70	NUM
cet-13155	36	58	ºc	ºc	NOUN
cet-13155	36	59	and	and	CCONJ
cet-13155	36	60	a	a	DET
cet-13155	36	61	ph	ph	NOUN
cet-13155	36	62	of	of	ADP
cet-13155	36	63	7	7	NUM
cet-13155	36	64	.	.	PUNCT
cet-13155	37	1	after	after	ADP
cet-13155	37	2	the	the	DET
cet-13155	37	3	co	co	NOUN
cet-13155	37	4	-	-	NOUN
cet-13155	37	5	precipitation	precipitation	NOUN
cet-13155	37	6	,	,	PUNCT
cet-13155	37	7	the	the	DET
cet-13155	37	8	catalyst	catalyst	NOUN
cet-13155	37	9	was	be	AUX
cet-13155	37	10	aged	age	VERB
cet-13155	37	11	at	at	ADP
cet-13155	37	12	the	the	DET
cet-13155	37	13	aforementioned	aforementioned	ADJ
cet-13155	37	14	conditions	condition	NOUN
cet-13155	37	15	for	for	ADP
cet-13155	37	16	1	1	NUM
cet-13155	37	17	h	h	NOUN
cet-13155	37	18	,	,	PUNCT
cet-13155	37	19	filtered	filter	VERB
cet-13155	37	20	and	and	CCONJ
cet-13155	37	21	washed	wash	VERB
cet-13155	37	22	to	to	PART
cet-13155	37	23	eliminate	eliminate	VERB
cet-13155	37	24	na+	na+	NOUN
cet-13155	37	25	ions	ion	NOUN
cet-13155	37	26	.	.	PUNCT
cet-13155	38	1	afterwards	afterwards	ADV
cet-13155	38	2	,	,	PUNCT
cet-13155	38	3	the	the	DET
cet-13155	38	4	obtained	obtain	VERB
cet-13155	38	5	solution	solution	NOUN
cet-13155	38	6	was	be	AUX
cet-13155	38	7	dried	dry	VERB
cet-13155	38	8	at	at	ADP
cet-13155	38	9	room	room	NOUN
cet-13155	38	10	temperature	temperature	NOUN
cet-13155	38	11	for	for	ADP
cet-13155	38	12	12	12	NUM
cet-13155	38	13	h	h	NOUN
cet-13155	38	14	,	,	PUNCT
cet-13155	38	15	and	and	CCONJ
cet-13155	38	16	another	another	DET
cet-13155	38	17	12	12	NUM
cet-13155	38	18	h	h	NOUN
cet-13155	38	19	at	at	ADP
cet-13155	38	20	110	110	NUM
cet-13155	38	21	ºc	ºc	NOUN
cet-13155	38	22	.	.	PUNCT
cet-13155	39	1	finally	finally	ADV
cet-13155	39	2	,	,	PUNCT
cet-13155	39	3	the	the	DET
cet-13155	39	4	obtained	obtain	VERB
cet-13155	39	5	catalyst	catalyst	NOUN
cet-13155	39	6	was	be	AUX
cet-13155	39	7	calcined	calcine	VERB
cet-13155	39	8	at	at	ADP
cet-13155	39	9	300	300	NUM
cet-13155	39	10	ºc	ºc	NOUN
cet-13155	39	11	for	for	ADP
cet-13155	39	12	10	10	NUM
cet-13155	39	13	h.	h.	NOUN
cet-13155	39	14	as	as	ADP
cet-13155	39	15	for	for	ADP
cet-13155	39	16	the	the	DET
cet-13155	39	17	inzr	inzr	ADJ
cet-13155	39	18	catalyst	catalyst	NOUN
cet-13155	39	19	,	,	PUNCT
cet-13155	39	20	with	with	ADP
cet-13155	39	21	an	an	DET
cet-13155	39	22	atomic	atomic	NOUN
cet-13155	39	23	in	in	ADP
cet-13155	39	24	:	:	PUNCT
cet-13155	39	25	zr	zr	NOUN
cet-13155	39	26	ratio	ratio	NOUN
cet-13155	39	27	of	of	ADP
cet-13155	39	28	2/1	2/1	NUM
cet-13155	39	29	,	,	PUNCT
cet-13155	39	30	the	the	DET
cet-13155	39	31	procedure	procedure	NOUN
cet-13155	39	32	was	be	AUX
cet-13155	39	33	similar	similar	ADJ
cet-13155	39	34	as	as	SCONJ
cet-13155	39	35	outlined	outline	VERB
cet-13155	39	36	above	above	ADV
cet-13155	39	37	.	.	PUNCT
cet-13155	40	1	in	in	ADP
cet-13155	40	2	this	this	DET
cet-13155	40	3	case	case	NOUN
cet-13155	40	4	,	,	PUNCT
cet-13155	40	5	in(no3)3	in(no3)3	NOUN
cet-13155	40	6	and	and	CCONJ
cet-13155	40	7	zr(no3)4	zr(no3)4	NOUN
cet-13155	40	8	nitrates	nitrate	NOUN
cet-13155	40	9	were	be	AUX
cet-13155	40	10	employed	employ	VERB
cet-13155	40	11	,	,	PUNCT
cet-13155	40	12	and	and	CCONJ
cet-13155	40	13	(	(	PUNCT
cet-13155	40	14	nh4)2co3	nh4)2co3	NOUN
cet-13155	40	15	was	be	AUX
cet-13155	40	16	used	use	VERB
cet-13155	40	17	as	as	ADP
cet-13155	40	18	precipitating	precipitate	VERB
cet-13155	40	19	agent	agent	NOUN
cet-13155	40	20	.	.	PUNCT
cet-13155	41	1	after	after	ADP
cet-13155	41	2	aging	age	VERB
cet-13155	41	3	,	,	PUNCT
cet-13155	41	4	filtering	filtering	NOUN
cet-13155	41	5	and	and	CCONJ
cet-13155	41	6	washing	washing	NOUN
cet-13155	41	7	,	,	PUNCT
cet-13155	41	8	the	the	DET
cet-13155	41	9	obtained	obtain	VERB
cet-13155	41	10	solution	solution	NOUN
cet-13155	41	11	was	be	AUX
cet-13155	41	12	dried	dry	VERB
cet-13155	41	13	and	and	CCONJ
cet-13155	41	14	calcined	calcine	VERB
cet-13155	41	15	at	at	ADP
cet-13155	41	16	500	500	NUM
cet-13155	41	17	ºc	ºc	NOUN
cet-13155	41	18	for	for	ADP
cet-13155	41	19	1	1	NUM
cet-13155	41	20	h.	h.	NOUN
cet-13155	41	21	the	the	DET
cet-13155	41	22	acid	acid	PROPN
cet-13155	41	23	catalyst	catalyst	NOUN
cet-13155	41	24	was	be	AUX
cet-13155	41	25	a	a	DET
cet-13155	41	26	commercial	commercial	ADJ
cet-13155	41	27	hzsm-5	hzsm-5	NOUN
cet-13155	41	28	(	(	PUNCT
cet-13155	41	29	obtained	obtain	VERB
cet-13155	41	30	by	by	ADP
cet-13155	41	31	zeolyst	zeolyst	PROPN
cet-13155	41	32	international	international	PROPN
cet-13155	41	33	)	)	PUNCT
cet-13155	41	34	with	with	ADP
cet-13155	41	35	a	a	DET
cet-13155	41	36	si	si	PROPN
cet-13155	41	37	/	/	SYM
cet-13155	41	38	al	al	PROPN
cet-13155	41	39	ratio	ratio	NOUN
cet-13155	41	40	of	of	ADP
cet-13155	41	41	140	140	NUM
cet-13155	41	42	.	.	PUNCT
cet-13155	42	1	the	the	DET
cet-13155	42	2	zeolite	zeolite	NOUN
cet-13155	42	3	was	be	AUX
cet-13155	42	4	obtained	obtain	VERB
cet-13155	42	5	in	in	ADP
cet-13155	42	6	ammonium	ammonium	NOUN
cet-13155	42	7	form	form	NOUN
cet-13155	42	8	and	and	CCONJ
cet-13155	42	9	calcined	calcine	VERB
cet-13155	42	10	at	at	ADP
cet-13155	42	11	575	575	NUM
cet-13155	42	12	ºc	ºc	NOUN
cet-13155	42	13	for	for	ADP
cet-13155	42	14	2	2	NUM
cet-13155	42	15	hours	hour	NOUN
cet-13155	42	16	for	for	ADP
cet-13155	42	17	obtaining	obtain	VERB
cet-13155	42	18	the	the	DET
cet-13155	42	19	acidic	acidic	ADJ
cet-13155	42	20	form	form	NOUN
cet-13155	42	21	.	.	PUNCT
cet-13155	43	1	the	the	DET
cet-13155	43	2	tandem	tandem	NOUN
cet-13155	43	3	catalysts	catalyst	NOUN
cet-13155	43	4	(	(	PUNCT
cet-13155	43	5	inzr	inzr	NOUN
cet-13155	43	6	/	/	SYM
cet-13155	43	7	h5	h5	NOUN
cet-13155	43	8	and	and	CCONJ
cet-13155	43	9	cuznzr	cuznzr	ADJ
cet-13155	43	10	/	/	SYM
cet-13155	43	11	h5	h5	NOUN
cet-13155	43	12	)	)	PUNCT
cet-13155	43	13	were	be	AUX
cet-13155	43	14	prepared	prepare	VERB
cet-13155	43	15	by	by	ADP
cet-13155	43	16	physical	physical	ADJ
cet-13155	43	17	mixture	mixture	NOUN
cet-13155	43	18	of	of	ADP
cet-13155	43	19	the	the	DET
cet-13155	43	20	metallic	metallic	ADJ
cet-13155	43	21	and	and	CCONJ
cet-13155	43	22	acid	acid	ADJ
cet-13155	43	23	catalyst	catalyst	NOUN
cet-13155	43	24	,	,	PUNCT
cet-13155	43	25	with	with	ADP
cet-13155	43	26	a	a	DET
cet-13155	43	27	metalilc	metalilc	NOUN
cet-13155	43	28	/	/	SYM
cet-13155	43	29	acid	acid	NOUN
cet-13155	43	30	mass	mass	NOUN
cet-13155	43	31	ratio	ratio	NOUN
cet-13155	43	32	of	of	ADP
cet-13155	43	33	1/1	1/1	NUM
cet-13155	43	34	.	.	PUNCT
cet-13155	44	1	this	this	DET
cet-13155	44	2	configuration	configuration	NOUN
cet-13155	44	3	was	be	AUX
cet-13155	44	4	selected	select	VERB
cet-13155	44	5	to	to	PART
cet-13155	44	6	shift	shift	VERB
cet-13155	44	7	the	the	DET
cet-13155	44	8	equilibrium	equilibrium	NOUN
cet-13155	44	9	of	of	ADP
cet-13155	44	10	the	the	DET
cet-13155	44	11	first	first	ADJ
cet-13155	44	12	reaction	reaction	NOUN
cet-13155	44	13	-	-	PUNCT
cet-13155	44	14	stage	stage	NOUN
cet-13155	44	15	(	(	PUNCT
cet-13155	44	16	methanol	methanol	NOUN
cet-13155	44	17	synthesis	synthesis	NOUN
cet-13155	44	18	)	)	PUNCT
cet-13155	44	19	by	by	ADP
cet-13155	44	20	favoring	favor	VERB
cet-13155	44	21	the	the	DET
cet-13155	44	22	synergy	synergy	NOUN
cet-13155	44	23	between	between	ADP
cet-13155	44	24	the	the	DET
cet-13155	44	25	metallic	metallic	NOUN
cet-13155	44	26	and	and	CCONJ
cet-13155	44	27	the	the	DET
cet-13155	44	28	acid	acid	NOUN
cet-13155	44	29	catalyst	catalyst	NOUN
cet-13155	44	30	when	when	SCONJ
cet-13155	44	31	physically	physically	ADV
cet-13155	44	32	mixing	mix	VERB
cet-13155	44	33	them	they	PRON
cet-13155	44	34	.	.	PUNCT
cet-13155	45	1	2.2	2.2	NUM
cet-13155	45	2	reaction	reaction	NOUN
cet-13155	45	3	and	and	CCONJ
cet-13155	45	4	analysis	analysis	NOUN
cet-13155	45	5	equipment	equipment	NOUN
cet-13155	45	6	the	the	DET
cet-13155	45	7	catalytic	catalytic	ADJ
cet-13155	45	8	reactions	reaction	NOUN
cet-13155	45	9	were	be	AUX
cet-13155	45	10	carried	carry	VERB
cet-13155	45	11	out	out	ADP
cet-13155	45	12	in	in	ADP
cet-13155	45	13	an	an	DET
cet-13155	45	14	automated	automate	VERB
cet-13155	45	15	reaction	reaction	NOUN
cet-13155	45	16	equipment	equipment	NOUN
cet-13155	45	17	(	(	PUNCT
cet-13155	45	18	pid	pid	X
cet-13155	45	19	eng	eng	PROPN
cet-13155	45	20	&	&	CCONJ
cet-13155	45	21	tech	tech	PROPN
cet-13155	45	22	microactivity	microactivity	NOUN
cet-13155	45	23	reference	reference	NOUN
cet-13155	45	24	)	)	PUNCT
cet-13155	45	25	provided	provide	VERB
cet-13155	45	26	with	with	ADP
cet-13155	45	27	an	an	DET
cet-13155	45	28	isothermal	isothermal	ADJ
cet-13155	45	29	fixed	fix	VERB
cet-13155	45	30	bed	bed	NOUN
cet-13155	45	31	reactor	reactor	NOUN
cet-13155	45	32	made	make	VERB
cet-13155	45	33	of	of	ADP
cet-13155	45	34	stainless	stainless	ADJ
cet-13155	45	35	steel	steel	NOUN
cet-13155	45	36	and	and	CCONJ
cet-13155	45	37	with	with	ADP
cet-13155	45	38	an	an	DET
cet-13155	45	39	internal	internal	ADJ
cet-13155	45	40	ceramic	ceramic	ADJ
cet-13155	45	41	coating	coating	NOUN
cet-13155	45	42	.	.	PUNCT
cet-13155	46	1	the	the	DET
cet-13155	46	2	catalytic	catalytic	ADJ
cet-13155	46	3	bed	bed	NOUN
cet-13155	46	4	consisted	consist	VERB
cet-13155	46	5	of	of	ADP
cet-13155	46	6	a	a	DET
cet-13155	46	7	mixture	mixture	NOUN
cet-13155	46	8	of	of	ADP
cet-13155	46	9	the	the	DET
cet-13155	46	10	catalyst	catalyst	NOUN
cet-13155	46	11	and	and	CCONJ
cet-13155	46	12	an	an	DET
cet-13155	46	13	inert	inert	ADJ
cet-13155	46	14	sic	sic	NOUN
cet-13155	46	15	solid	solid	ADJ
cet-13155	46	16	,	,	PUNCT
cet-13155	46	17	with	with	ADP
cet-13155	46	18	the	the	DET
cet-13155	46	19	aim	aim	NOUN
cet-13155	46	20	of	of	ADP
cet-13155	46	21	avoiding	avoid	VERB
cet-13155	46	22	preferential	preferential	ADJ
cet-13155	46	23	flow	flow	NOUN
cet-13155	46	24	paths	path	NOUN
cet-13155	46	25	and	and	CCONJ
cet-13155	46	26	ensuring	ensure	VERB
cet-13155	46	27	isothermal	isothermal	ADJ
cet-13155	46	28	conditions	condition	NOUN
cet-13155	46	29	in	in	ADP
cet-13155	46	30	the	the	DET
cet-13155	46	31	bed	bed	NOUN
cet-13155	46	32	.	.	PUNCT
cet-13155	47	1	the	the	DET
cet-13155	47	2	feed	feed	NOUN
cet-13155	47	3	and	and	CCONJ
cet-13155	47	4	products	product	NOUN
cet-13155	47	5	streams	stream	NOUN
cet-13155	47	6	were	be	AUX
cet-13155	47	7	analyzed	analyze	VERB
cet-13155	47	8	on	on	ADP
cet-13155	47	9	-	-	PUNCT
cet-13155	47	10	line	line	NOUN
cet-13155	47	11	by	by	ADP
cet-13155	47	12	means	mean	NOUN
cet-13155	47	13	of	of	ADP
cet-13155	47	14	a	a	DET
cet-13155	47	15	varian	varian	PROPN
cet-13155	47	16	cp-4900	cp-4900	NOUN
cet-13155	47	17	(	(	PUNCT
cet-13155	47	18	agilent	agilent	PROPN
cet-13155	47	19	)	)	PUNCT
cet-13155	47	20	micro	micro	NOUN
cet-13155	47	21	chromatograph	chromatograph	NOUN
cet-13155	47	22	,	,	PUNCT
cet-13155	47	23	equipped	equip	VERB
cet-13155	47	24	with	with	ADP
cet-13155	47	25	three	three	NUM
cet-13155	47	26	analytical	analytical	ADJ
cet-13155	47	27	modules	module	NOUN
cet-13155	47	28	with	with	ADP
cet-13155	47	29	tcd	tcd	NOUN
cet-13155	47	30	detectors	detector	NOUN
cet-13155	47	31	:	:	PUNCT
cet-13155	47	32	molecular	molecular	ADJ
cet-13155	47	33	sieve	sieve	NOUN
cet-13155	47	34	(	(	PUNCT
cet-13155	47	35	ms-5	ms-5	ADV
cet-13155	47	36	)	)	PUNCT
cet-13155	47	37	,	,	PUNCT
cet-13155	47	38	porapak	porapak	VERB
cet-13155	47	39	q	q	PROPN
cet-13155	47	40	(	(	PUNCT
cet-13155	47	41	ppq	ppq	PROPN
cet-13155	47	42	)	)	PUNCT
cet-13155	47	43	and	and	CCONJ
cet-13155	47	44	5	5	NUM
cet-13155	47	45	cb	cb	PROPN
cet-13155	47	46	column	column	NOUN
cet-13155	47	47	(	(	PUNCT
cet-13155	47	48	cpsil	cpsil	PROPN
cet-13155	47	49	)	)	PUNCT
cet-13155	47	50	.	.	PUNCT
cet-13155	48	1	a	a	DET
cet-13155	48	2	more	more	ADV
cet-13155	48	3	detailed	detailed	ADJ
cet-13155	48	4	configuration	configuration	NOUN
cet-13155	48	5	of	of	ADP
cet-13155	48	6	the	the	DET
cet-13155	48	7	experimental	experimental	ADJ
cet-13155	48	8	setup	setup	NOUN
cet-13155	48	9	is	be	AUX
cet-13155	48	10	described	describe	VERB
cet-13155	48	11	elsewhere	elsewhere	ADV
cet-13155	48	12	(	(	PUNCT
cet-13155	48	13	ateka	ateka	PROPN
cet-13155	48	14	,	,	PUNCT
cet-13155	48	15	2016	2016	NUM
cet-13155	48	16	)	)	PUNCT
cet-13155	48	17	.	.	PUNCT
cet-13155	49	1	458	458	NUM
cet-13155	50	1	the	the	DET
cet-13155	50	2	reaction	reaction	NOUN
cet-13155	50	3	runs	run	VERB
cet-13155	50	4	with	with	ADP
cet-13155	50	5	the	the	DET
cet-13155	50	6	metallic	metallic	ADJ
cet-13155	50	7	catalysts	catalyst	NOUN
cet-13155	50	8	were	be	AUX
cet-13155	50	9	performed	perform	VERB
cet-13155	50	10	under	under	ADP
cet-13155	50	11	the	the	DET
cet-13155	50	12	succeeding	succeed	VERB
cet-13155	50	13	conditions	condition	NOUN
cet-13155	50	14	:	:	PUNCT
cet-13155	50	15	310	310	NUM
cet-13155	50	16	-	-	SYM
cet-13155	50	17	430	430	NUM
cet-13155	50	18	ºc	ºc	NOUN
cet-13155	50	19	;	;	PUNCT
cet-13155	50	20	50	50	NUM
cet-13155	50	21	bar	bar	NOUN
cet-13155	50	22	;	;	PUNCT
cet-13155	50	23	co2/(co+co2	co2/(co+co2	PROPN
cet-13155	50	24	)	)	PUNCT
cet-13155	50	25	ratio	ratio	NOUN
cet-13155	50	26	,	,	PUNCT
cet-13155	50	27	0.5	0.5	NUM
cet-13155	50	28	;	;	PUNCT
cet-13155	50	29	h2/(co+co2	h2/(co+co2	PROPN
cet-13155	50	30	)	)	PUNCT
cet-13155	50	31	ratio	ratio	NOUN
cet-13155	50	32	,	,	PUNCT
cet-13155	50	33	3	3	NUM
cet-13155	50	34	;	;	PUNCT
cet-13155	50	35	space	space	NOUN
cet-13155	50	36	time	time	NOUN
cet-13155	50	37	,	,	PUNCT
cet-13155	50	38	6	6	NUM
cet-13155	50	39	gcat	gcat	NOUN
cet-13155	50	40	h	h	NOUN
cet-13155	50	41	molc-1	molc-1	PROPN
cet-13155	50	42	(	(	PUNCT
cet-13155	50	43	only	only	ADV
cet-13155	50	44	metallic	metallic	ADJ
cet-13155	50	45	catalyst	catalyst	NOUN
cet-13155	50	46	)	)	PUNCT
cet-13155	50	47	.	.	PUNCT
cet-13155	51	1	regarding	regard	VERB
cet-13155	51	2	the	the	DET
cet-13155	51	3	reactions	reaction	NOUN
cet-13155	51	4	with	with	ADP
cet-13155	51	5	the	the	DET
cet-13155	51	6	tandem	tandem	NOUN
cet-13155	51	7	catalysts	catalyst	NOUN
cet-13155	51	8	,	,	PUNCT
cet-13155	51	9	the	the	DET
cet-13155	51	10	reactions	reaction	NOUN
cet-13155	51	11	were	be	AUX
cet-13155	51	12	carried	carry	VERB
cet-13155	51	13	out	out	ADP
cet-13155	51	14	under	under	ADP
cet-13155	51	15	the	the	DET
cet-13155	51	16	following	following	ADJ
cet-13155	51	17	conditions	condition	NOUN
cet-13155	51	18	:	:	PUNCT
cet-13155	51	19	340	340	NUM
cet-13155	51	20	ºc	ºc	NOUN
cet-13155	51	21	,	,	PUNCT
cet-13155	51	22	380	380	NUM
cet-13155	51	23	ºc	ºc	NUM
cet-13155	51	24	and	and	CCONJ
cet-13155	51	25	420	420	NUM
cet-13155	51	26	ºc	ºc	NOUN
cet-13155	51	27	;	;	PUNCT
cet-13155	51	28	50	50	NUM
cet-13155	51	29	bar	bar	NOUN
cet-13155	51	30	;	;	PUNCT
cet-13155	51	31	co2/(co+co2	co2/(co+co2	PROPN
cet-13155	51	32	)	)	PUNCT
cet-13155	51	33	ratio	ratio	NOUN
cet-13155	51	34	,	,	PUNCT
cet-13155	51	35	0.5	0.5	NUM
cet-13155	51	36	;	;	PUNCT
cet-13155	51	37	h2/(co+co2	h2/(co+co2	PROPN
cet-13155	51	38	)	)	PUNCT
cet-13155	51	39	ratio	ratio	NOUN
cet-13155	51	40	,	,	PUNCT
cet-13155	51	41	3	3	NUM
cet-13155	51	42	;	;	PUNCT
cet-13155	51	43	space	space	NOUN
cet-13155	51	44	time	time	NOUN
cet-13155	51	45	,	,	PUNCT
cet-13155	51	46	12	12	NUM
cet-13155	51	47	gcat	gcat	NOUN
cet-13155	51	48	h	h	NOUN
cet-13155	51	49	molc1	molc1	NOUN
cet-13155	51	50	(	(	PUNCT
cet-13155	51	51	metallic	metallic	ADJ
cet-13155	51	52	and	and	CCONJ
cet-13155	51	53	acid	acid	ADJ
cet-13155	51	54	catalysts	catalyst	NOUN
cet-13155	51	55	)	)	PUNCT
cet-13155	51	56	.	.	PUNCT
cet-13155	52	1	the	the	DET
cet-13155	52	2	results	result	NOUN
cet-13155	52	3	of	of	ADP
cet-13155	52	4	the	the	DET
cet-13155	52	5	reactions	reaction	NOUN
cet-13155	52	6	are	be	AUX
cet-13155	52	7	the	the	DET
cet-13155	52	8	average	average	ADJ
cet-13155	52	9	value	value	NOUN
cet-13155	52	10	of	of	ADP
cet-13155	52	11	three	three	NUM
cet-13155	52	12	tested	test	VERB
cet-13155	52	13	reactions	reaction	NOUN
cet-13155	52	14	,	,	PUNCT
cet-13155	52	15	in	in	ADP
cet-13155	52	16	which	which	PRON
cet-13155	52	17	carbon	carbon	NOUN
cet-13155	52	18	balance	balance	NOUN
cet-13155	52	19	was	be	AUX
cet-13155	52	20	closed	close	VERB
cet-13155	52	21	above	above	ADP
cet-13155	52	22	95	95	NUM
cet-13155	52	23	%	%	NOUN
cet-13155	52	24	.	.	PUNCT
cet-13155	53	1	2.3	2.3	NUM
cet-13155	53	2	reaction	reaction	NOUN
cet-13155	53	3	indices	indice	VERB
cet-13155	53	4	the	the	DET
cet-13155	53	5	conversion	conversion	NOUN
cet-13155	53	6	of	of	ADP
cet-13155	53	7	co2	co2	NOUN
cet-13155	53	8	and	and	CCONJ
cet-13155	53	9	cox	cox	PROPN
cet-13155	53	10	(	(	PUNCT
cet-13155	53	11	co2+co	co2+co	NOUN
cet-13155	53	12	)	)	PUNCT
cet-13155	53	13	were	be	AUX
cet-13155	53	14	calculated	calculate	VERB
cet-13155	53	15	in	in	ADP
cet-13155	53	16	accordance	accordance	NOUN
cet-13155	53	17	with	with	ADP
cet-13155	53	18	the	the	DET
cet-13155	53	19	following	follow	VERB
cet-13155	53	20	expressions	expression	NOUN
cet-13155	53	21	:	:	PUNCT
cet-13155	54	1	xco2	xco2	PROPN
cet-13155	54	2	=	=	PUNCT
cet-13155	54	3	fco2	fco2	ADJ
cet-13155	54	4	0	0	NUM
cet-13155	55	1	−	−	ADP
cet-13155	55	2	fco2	fco2	ADJ
cet-13155	55	3	fco2	fco2	PROPN
cet-13155	55	4	0	0	NUM
cet-13155	55	5	(	(	PUNCT
cet-13155	55	6	6	6	NUM
cet-13155	55	7	)	)	PUNCT
cet-13155	55	8	xcox	xcox	X
cet-13155	56	1	=	=	PUNCT
cet-13155	56	2	fcox	fcox	ADJ
cet-13155	56	3	0	0	PUNCT
cet-13155	57	1	−	−	NOUN
cet-13155	57	2	fcox	fcox	ADJ
cet-13155	57	3	fcox	fcox	PROPN
cet-13155	57	4	0	0	PUNCT
cet-13155	58	1	(	(	PUNCT
cet-13155	58	2	7	7	NUM
cet-13155	58	3	)	)	PUNCT
cet-13155	58	4	where	where	SCONJ
cet-13155	58	5	f0	f0	ADJ
cet-13155	58	6	co2	co2	NOUN
cet-13155	58	7	and	and	CCONJ
cet-13155	58	8	f0	f0	PROPN
cet-13155	58	9	cox	cox	PROPN
cet-13155	58	10	are	be	AUX
cet-13155	58	11	the	the	DET
cet-13155	58	12	inlet	inlet	ADJ
cet-13155	58	13	molar	molar	ADJ
cet-13155	58	14	flow	flow	NOUN
cet-13155	58	15	rates	rate	NOUN
cet-13155	58	16	in	in	ADP
cet-13155	58	17	content	content	NOUN
cet-13155	58	18	of	of	ADP
cet-13155	58	19	c	c	NOUN
cet-13155	58	20	atoms	atom	NOUN
cet-13155	58	21	of	of	ADP
cet-13155	58	22	co2	co2	NOUN
cet-13155	58	23	and	and	CCONJ
cet-13155	58	24	cox	cox	PROPN
cet-13155	58	25	,	,	PUNCT
cet-13155	58	26	respectively	respectively	ADV
cet-13155	58	27	,	,	PUNCT
cet-13155	58	28	and	and	CCONJ
cet-13155	58	29	fco2	fco2	ADJ
cet-13155	58	30	and	and	CCONJ
cet-13155	58	31	fcox	fcox	ADJ
cet-13155	58	32	are	be	AUX
cet-13155	58	33	the	the	DET
cet-13155	58	34	outlet	outlet	ADJ
cet-13155	58	35	molar	molar	ADJ
cet-13155	58	36	flow	flow	NOUN
cet-13155	58	37	rates	rate	NOUN
cet-13155	58	38	in	in	ADP
cet-13155	58	39	content	content	NOUN
cet-13155	58	40	of	of	ADP
cet-13155	58	41	c	c	NOUN
cet-13155	58	42	atoms	atom	NOUN
cet-13155	58	43	of	of	ADP
cet-13155	58	44	co2	co2	NOUN
cet-13155	58	45	and	and	CCONJ
cet-13155	58	46	cox	cox	PROPN
cet-13155	58	47	respectively	respectively	ADV
cet-13155	58	48	.	.	PUNCT
cet-13155	59	1	the	the	DET
cet-13155	59	2	yield	yield	NOUN
cet-13155	59	3	of	of	ADP
cet-13155	59	4	each	each	DET
cet-13155	59	5	i	i	PROPN
cet-13155	59	6	product	product	NOUN
cet-13155	59	7	(	(	PUNCT
cet-13155	59	8	yi	yi	PROPN
cet-13155	59	9	,	,	PUNCT
cet-13155	59	10	except	except	SCONJ
cet-13155	59	11	for	for	ADP
cet-13155	59	12	co	co	NOUN
cet-13155	59	13	and	and	CCONJ
cet-13155	59	14	co2	co2	NOUN
cet-13155	59	15	)	)	PUNCT
cet-13155	59	16	was	be	AUX
cet-13155	59	17	measured	measure	VERB
cet-13155	59	18	as	as	SCONJ
cet-13155	59	19	follows	follow	VERB
cet-13155	59	20	:	:	PUNCT
cet-13155	60	1	yi	yi	PROPN
cet-13155	60	2	=	=	SYM
cet-13155	60	3	ni	ni	PROPN
cet-13155	60	4	·	·	PUNCT
cet-13155	60	5	fi	fi	NOUN
cet-13155	60	6	fcox	fcox	ADJ
cet-13155	60	7	0	0	NUM
cet-13155	60	8	·	·	SYM
cet-13155	60	9	100	100	NUM
cet-13155	60	10	(	(	PUNCT
cet-13155	60	11	8)	8)	NUM
cet-13155	60	12	where	where	SCONJ
cet-13155	60	13	ni	ni	PROPN
cet-13155	60	14	is	be	AUX
cet-13155	60	15	the	the	DET
cet-13155	60	16	number	number	NOUN
cet-13155	60	17	of	of	ADP
cet-13155	60	18	carbon	carbon	NOUN
cet-13155	60	19	atoms	atom	NOUN
cet-13155	60	20	for	for	ADP
cet-13155	60	21	the	the	DET
cet-13155	60	22	i	i	PROPN
cet-13155	60	23	product	product	NOUN
cet-13155	60	24	and	and	CCONJ
cet-13155	60	25	fi	fi	NOUN
cet-13155	60	26	the	the	DET
cet-13155	60	27	molar	molar	ADJ
cet-13155	60	28	flow	flow	NOUN
cet-13155	60	29	rate	rate	NOUN
cet-13155	60	30	of	of	ADP
cet-13155	60	31	the	the	DET
cet-13155	60	32	i	i	PROPN
cet-13155	60	33	in	in	ADP
cet-13155	60	34	the	the	DET
cet-13155	60	35	products	product	NOUN
cet-13155	60	36	stream	stream	NOUN
cet-13155	60	37	.	.	PUNCT
cet-13155	61	1	3	3	X
cet-13155	61	2	.	.	NOUN
cet-13155	61	3	results	result	VERB
cet-13155	61	4	3.1	3.1	NUM
cet-13155	61	5	alternative	alternative	ADJ
cet-13155	61	6	catalysts	catalyst	NOUN
cet-13155	61	7	for	for	ADP
cet-13155	61	8	methanol	methanol	NOUN
cet-13155	61	9	synthesis	synthesis	NOUN
cet-13155	61	10	in	in	ADP
cet-13155	61	11	this	this	DET
cet-13155	61	12	section	section	NOUN
cet-13155	61	13	,	,	PUNCT
cet-13155	61	14	a	a	DET
cet-13155	61	15	comparison	comparison	NOUN
cet-13155	61	16	of	of	ADP
cet-13155	61	17	the	the	DET
cet-13155	61	18	traditional	traditional	ADJ
cet-13155	61	19	cuznzr	cuznzr	NOUN
cet-13155	61	20	and	and	CCONJ
cet-13155	61	21	the	the	DET
cet-13155	61	22	alternative	alternative	ADJ
cet-13155	61	23	inzr	inzr	ADJ
cet-13155	61	24	metallic	metallic	ADJ
cet-13155	61	25	catalysts	catalyst	NOUN
cet-13155	61	26	was	be	AUX
cet-13155	61	27	performed	perform	VERB
cet-13155	61	28	.	.	PUNCT
cet-13155	62	1	as	as	SCONJ
cet-13155	62	2	stated	state	VERB
cet-13155	62	3	above	above	ADV
cet-13155	62	4	,	,	PUNCT
cet-13155	62	5	the	the	DET
cet-13155	62	6	integrated	integrate	VERB
cet-13155	62	7	process	process	NOUN
cet-13155	62	8	requires	require	VERB
cet-13155	62	9	higher	high	ADJ
cet-13155	62	10	temperature	temperature	NOUN
cet-13155	62	11	to	to	PART
cet-13155	62	12	yield	yield	VERB
cet-13155	62	13	hydrocarbons	hydrocarbon	NOUN
cet-13155	62	14	.	.	PUNCT
cet-13155	63	1	accordingly	accordingly	ADV
cet-13155	63	2	,	,	PUNCT
cet-13155	63	3	reaction	reaction	NOUN
cet-13155	63	4	runs	run	NOUN
cet-13155	63	5	were	be	AUX
cet-13155	63	6	performed	perform	VERB
cet-13155	63	7	between	between	ADP
cet-13155	63	8	310	310	NUM
cet-13155	63	9	ºc	ºc	NUM
cet-13155	63	10	and	and	CCONJ
cet-13155	63	11	430	430	NUM
cet-13155	63	12	ºc	ºc	PROPN
cet-13155	63	13	.	.	PROPN
cet-13155	63	14	figures	figures	PROPN
cet-13155	63	15	1a	1a	PROPN
cet-13155	63	16	and	and	CCONJ
cet-13155	63	17	1b	1b	NUM
cet-13155	63	18	show	show	VERB
cet-13155	63	19	the	the	DET
cet-13155	63	20	effect	effect	NOUN
cet-13155	63	21	of	of	ADP
cet-13155	63	22	the	the	DET
cet-13155	63	23	temperature	temperature	NOUN
cet-13155	63	24	on	on	ADP
cet-13155	63	25	methanol	methanol	NOUN
cet-13155	63	26	and	and	CCONJ
cet-13155	63	27	on	on	ADP
cet-13155	63	28	undesired	undesired	ADJ
cet-13155	63	29	methane	methane	NOUN
cet-13155	63	30	yield	yield	NOUN
cet-13155	63	31	,	,	PUNCT
cet-13155	63	32	respectively	respectively	ADV
cet-13155	63	33	.	.	PUNCT
cet-13155	64	1	as	as	SCONJ
cet-13155	64	2	seen	see	VERB
cet-13155	64	3	in	in	ADP
cet-13155	64	4	figure	figure	NOUN
cet-13155	64	5	1a	1a	NOUN
cet-13155	64	6	,	,	PUNCT
cet-13155	64	7	the	the	DET
cet-13155	64	8	traditional	traditional	ADJ
cet-13155	64	9	cuznzr	cuznzr	ADJ
cet-13155	64	10	catalyst	catalyst	NOUN
cet-13155	64	11	exhibited	exhibit	VERB
cet-13155	64	12	higher	high	ADJ
cet-13155	64	13	methanol	methanol	NOUN
cet-13155	64	14	yield	yield	NOUN
cet-13155	64	15	than	than	ADP
cet-13155	64	16	the	the	DET
cet-13155	64	17	alternative	alternative	ADJ
cet-13155	64	18	inzr	inzr	ADJ
cet-13155	64	19	catalyst	catalyst	NOUN
cet-13155	64	20	at	at	ADP
cet-13155	64	21	lower	low	ADJ
cet-13155	64	22	temperature	temperature	NOUN
cet-13155	64	23	(	(	PUNCT
cet-13155	64	24	14.5	14.5	NUM
cet-13155	64	25	%	%	NOUN
cet-13155	64	26	vs.	vs.	ADP
cet-13155	64	27	3.6	3.6	NUM
cet-13155	64	28	%	%	NOUN
cet-13155	64	29	at	at	ADP
cet-13155	64	30	310	310	NUM
cet-13155	64	31	ºc	ºc	NOUN
cet-13155	64	32	)	)	PUNCT
cet-13155	64	33	.	.	PUNCT
cet-13155	65	1	at	at	ADP
cet-13155	65	2	this	this	DET
cet-13155	65	3	temperature	temperature	NOUN
cet-13155	65	4	,	,	PUNCT
cet-13155	65	5	inzr	inzr	ADJ
cet-13155	65	6	catalyst	catalyst	NOUN
cet-13155	65	7	is	be	AUX
cet-13155	65	8	not	not	PART
cet-13155	65	9	as	as	ADV
cet-13155	65	10	active	active	ADJ
cet-13155	65	11	as	as	ADP
cet-13155	65	12	cuznzr	cuznzr	NOUN
cet-13155	65	13	,	,	PUNCT
cet-13155	65	14	and	and	CCONJ
cet-13155	65	15	thus	thus	ADV
cet-13155	65	16	it	it	PRON
cet-13155	65	17	required	require	VERB
cet-13155	65	18	higher	high	ADJ
cet-13155	65	19	reaction	reaction	NOUN
cet-13155	65	20	temperature	temperature	NOUN
cet-13155	65	21	to	to	PART
cet-13155	65	22	increase	increase	VERB
cet-13155	65	23	methanol	methanol	NOUN
cet-13155	65	24	yield	yield	NOUN
cet-13155	65	25	,	,	PUNCT
cet-13155	65	26	leading	lead	VERB
cet-13155	65	27	to	to	ADP
cet-13155	65	28	the	the	DET
cet-13155	65	29	maximum	maximum	ADJ
cet-13155	65	30	yield	yield	NOUN
cet-13155	65	31	at	at	ADP
cet-13155	65	32	340	340	NUM
cet-13155	65	33	ºc	ºc	NOUN
cet-13155	65	34	.	.	PUNCT
cet-13155	66	1	however	however	ADV
cet-13155	66	2	,	,	PUNCT
cet-13155	66	3	even	even	ADV
cet-13155	66	4	at	at	ADP
cet-13155	66	5	this	this	DET
cet-13155	66	6	temperature	temperature	NOUN
cet-13155	66	7	,	,	PUNCT
cet-13155	66	8	cuznzr	cuznzr	NOUN
cet-13155	66	9	showed	show	VERB
cet-13155	66	10	better	well	ADJ
cet-13155	66	11	results	result	NOUN
cet-13155	66	12	than	than	ADP
cet-13155	66	13	inzr	inzr	NOUN
cet-13155	66	14	.	.	PUNCT
cet-13155	67	1	nonetheless	nonetheless	ADV
cet-13155	67	2	,	,	PUNCT
cet-13155	67	3	with	with	ADP
cet-13155	67	4	cuznzr	cuznzr	ADJ
cet-13155	67	5	catalyst	catalyst	NOUN
cet-13155	67	6	,	,	PUNCT
cet-13155	67	7	methanol	methanol	NOUN
cet-13155	67	8	yield	yield	NOUN
cet-13155	67	9	decreased	decrease	VERB
cet-13155	67	10	at	at	ADP
cet-13155	67	11	higher	high	ADJ
cet-13155	67	12	temperature	temperature	NOUN
cet-13155	67	13	(	(	PUNCT
cet-13155	67	14	due	due	ADP
cet-13155	67	15	to	to	ADP
cet-13155	67	16	the	the	DET
cet-13155	67	17	thermodynamic	thermodynamic	ADJ
cet-13155	67	18	limitation	limitation	NOUN
cet-13155	67	19	)	)	PUNCT
cet-13155	67	20	,	,	PUNCT
cet-13155	67	21	driving	drive	VERB
cet-13155	67	22	the	the	DET
cet-13155	67	23	methanol	methanol	NOUN
cet-13155	67	24	yield	yield	NOUN
cet-13155	67	25	to	to	ADP
cet-13155	67	26	less	less	ADJ
cet-13155	67	27	than	than	ADP
cet-13155	67	28	1	1	NUM
cet-13155	67	29	%	%	NOUN
cet-13155	67	30	at	at	ADP
cet-13155	67	31	430	430	NUM
cet-13155	67	32	ºc	ºc	NOUN
cet-13155	67	33	.	.	PUNCT
cet-13155	68	1	cu	cu	PROPN
cet-13155	68	2	-	-	PUNCT
cet-13155	68	3	based	base	VERB
cet-13155	68	4	catalysts	catalyst	NOUN
cet-13155	68	5	are	be	AUX
cet-13155	68	6	known	know	VERB
cet-13155	68	7	to	to	ADP
cet-13155	68	8	sinter	sinter	PROPN
cet-13155	68	9	at	at	ADP
cet-13155	68	10	temperatures	temperature	NOUN
cet-13155	68	11	above	above	ADP
cet-13155	68	12	300	300	NUM
cet-13155	68	13	ºc	ºc	NOUN
cet-13155	68	14	(	(	PUNCT
cet-13155	68	15	sanchez	sanchez	NOUN
cet-13155	68	16	-	-	PUNCT
cet-13155	68	17	contador	contador	NOUN
cet-13155	68	18	,	,	PUNCT
cet-13155	68	19	2018	2018	NUM
cet-13155	68	20	)	)	PUNCT
cet-13155	68	21	,	,	PUNCT
cet-13155	68	22	which	which	PRON
cet-13155	68	23	makes	make	VERB
cet-13155	68	24	them	they	PRON
cet-13155	68	25	unsuitable	unsuitable	ADJ
cet-13155	68	26	for	for	ADP
cet-13155	68	27	process	process	NOUN
cet-13155	68	28	requiring	require	VERB
cet-13155	68	29	high	high	ADJ
cet-13155	68	30	temperatures	temperature	NOUN
cet-13155	68	31	.	.	PUNCT
cet-13155	69	1	therefore	therefore	ADV
cet-13155	69	2	,	,	PUNCT
cet-13155	69	3	cuznzr	cuznzr	VERB
cet-13155	69	4	better	well	ADJ
cet-13155	69	5	activity	activity	NOUN
cet-13155	69	6	might	might	AUX
cet-13155	69	7	not	not	PART
cet-13155	69	8	be	be	AUX
cet-13155	69	9	so	so	ADV
cet-13155	69	10	significant	significant	ADJ
cet-13155	69	11	at	at	ADP
cet-13155	69	12	the	the	DET
cet-13155	69	13	temperatures	temperature	NOUN
cet-13155	69	14	required	require	VERB
cet-13155	69	15	for	for	ADP
cet-13155	69	16	the	the	DET
cet-13155	69	17	integrated	integrate	VERB
cet-13155	69	18	process	process	NOUN
cet-13155	69	19	,	,	PUNCT
cet-13155	69	20	in	in	ADP
cet-13155	69	21	which	which	PRON
cet-13155	69	22	a	a	DET
cet-13155	69	23	stable	stable	ADJ
cet-13155	69	24	catalyst	catalyst	NOUN
cet-13155	69	25	is	be	AUX
cet-13155	69	26	required	require	VERB
cet-13155	69	27	.	.	PUNCT
cet-13155	70	1	as	as	ADP
cet-13155	70	2	for	for	ADP
cet-13155	70	3	the	the	DET
cet-13155	70	4	methane	methane	NOUN
cet-13155	70	5	yield	yield	NOUN
cet-13155	70	6	,	,	PUNCT
cet-13155	70	7	figure	figure	NOUN
cet-13155	70	8	1b	1b	NUM
cet-13155	70	9	,	,	PUNCT
cet-13155	70	10	with	with	SCONJ
cet-13155	70	11	both	both	PRON
cet-13155	70	12	catalysts	catalyst	NOUN
cet-13155	70	13	methane	methane	NOUN
cet-13155	70	14	increased	increase	VERB
cet-13155	70	15	with	with	ADP
cet-13155	70	16	rising	rise	VERB
cet-13155	70	17	temperature	temperature	NOUN
cet-13155	70	18	.	.	PUNCT
cet-13155	71	1	this	this	PRON
cet-13155	71	2	occurred	occur	VERB
cet-13155	71	3	as	as	ADP
cet-13155	71	4	a	a	DET
cet-13155	71	5	result	result	NOUN
cet-13155	71	6	of	of	ADP
cet-13155	71	7	the	the	DET
cet-13155	71	8	cracking	cracking	NOUN
cet-13155	71	9	of	of	ADP
cet-13155	71	10	olefins	olefin	NOUN
cet-13155	71	11	and	and	CCONJ
cet-13155	71	12	the	the	DET
cet-13155	71	13	decomposition	decomposition	NOUN
cet-13155	71	14	of	of	ADP
cet-13155	71	15	methanol	methanol	NOUN
cet-13155	71	16	(	(	PUNCT
cet-13155	71	17	portillo	portillo	PROPN
cet-13155	71	18	et	et	PROPN
cet-13155	71	19	al	al	PROPN
cet-13155	71	20	.	.	PROPN
cet-13155	71	21	,	,	PUNCT
cet-13155	71	22	2022	2022	NUM
cet-13155	71	23	)	)	PUNCT
cet-13155	71	24	,	,	PUNCT
cet-13155	71	25	and	and	CCONJ
cet-13155	71	26	the	the	DET
cet-13155	71	27	methane	methane	NOUN
cet-13155	71	28	production	production	NOUN
cet-13155	71	29	accounted	account	VERB
cet-13155	71	30	for	for	ADP
cet-13155	71	31	almost	almost	ADV
cet-13155	71	32	1.5	1.5	NUM
cet-13155	71	33	%	%	NOUN
cet-13155	71	34	at	at	ADP
cet-13155	71	35	430	430	NUM
cet-13155	71	36	ºc	ºc	NOUN
cet-13155	71	37	,	,	PUNCT
cet-13155	71	38	almost	almost	ADV
cet-13155	71	39	doubling	double	VERB
cet-13155	71	40	methanol	methanol	NOUN
cet-13155	71	41	yield	yield	NOUN
cet-13155	71	42	(	(	PUNCT
cet-13155	71	43	0.8	0.8	NUM
cet-13155	71	44	%	%	NOUN
cet-13155	71	45	)	)	PUNCT
cet-13155	71	46	.	.	PUNCT
cet-13155	72	1	the	the	DET
cet-13155	72	2	rising	rise	VERB
cet-13155	72	3	trend	trend	NOUN
cet-13155	72	4	of	of	ADP
cet-13155	72	5	methane	methane	NOUN
cet-13155	72	6	production	production	NOUN
cet-13155	72	7	is	be	AUX
cet-13155	72	8	nearly	nearly	ADV
cet-13155	72	9	the	the	DET
cet-13155	72	10	same	same	ADJ
cet-13155	72	11	for	for	ADP
cet-13155	72	12	both	both	DET
cet-13155	72	13	catalysts	catalyst	NOUN
cet-13155	72	14	,	,	PUNCT
cet-13155	72	15	allowing	allow	VERB
cet-13155	72	16	concluding	conclude	VERB
cet-13155	72	17	that	that	SCONJ
cet-13155	72	18	the	the	DET
cet-13155	72	19	tendency	tendency	NOUN
cet-13155	72	20	is	be	AUX
cet-13155	72	21	related	relate	VERB
cet-13155	72	22	to	to	ADP
cet-13155	72	23	the	the	DET
cet-13155	72	24	operating	operating	NOUN
cet-13155	72	25	conditions	condition	NOUN
cet-13155	72	26	,	,	PUNCT
cet-13155	72	27	regardless	regardless	ADV
cet-13155	72	28	the	the	DET
cet-13155	72	29	catalyst	catalyst	NOUN
cet-13155	72	30	used	use	VERB
cet-13155	72	31	.	.	PUNCT
cet-13155	73	1	459	459	NUM
cet-13155	73	2	figure	figure	NOUN
cet-13155	73	3	1	1	NUM
cet-13155	73	4	:	:	PUNCT
cet-13155	73	5	effect	effect	NOUN
cet-13155	73	6	of	of	ADP
cet-13155	73	7	the	the	DET
cet-13155	73	8	temperature	temperature	NOUN
cet-13155	73	9	on	on	ADP
cet-13155	73	10	(	(	PUNCT
cet-13155	73	11	a	a	DET
cet-13155	73	12	)	)	PUNCT
cet-13155	73	13	methanol	methanol	NOUN
cet-13155	73	14	yield	yield	NOUN
cet-13155	73	15	and	and	CCONJ
cet-13155	73	16	(	(	PUNCT
cet-13155	73	17	b	b	NOUN
cet-13155	73	18	)	)	PUNCT
cet-13155	73	19	methane	methane	NOUN
cet-13155	73	20	yield	yield	NOUN
cet-13155	73	21	with	with	ADP
cet-13155	73	22	cuznzr	cuznzr	ADJ
cet-13155	73	23	and	and	CCONJ
cet-13155	73	24	inzr	inzr	ADJ
cet-13155	73	25	metallic	metallic	ADJ
cet-13155	73	26	oxide	oxide	NOUN
cet-13155	73	27	catalysts	catalyst	NOUN
cet-13155	73	28	.	.	PUNCT
cet-13155	74	1	reaction	reaction	NOUN
cet-13155	74	2	conditions	condition	NOUN
cet-13155	74	3	:	:	PUNCT
cet-13155	74	4	50	50	NUM
cet-13155	74	5	bar	bar	NOUN
cet-13155	74	6	;	;	PUNCT
cet-13155	74	7	space	space	NOUN
cet-13155	74	8	time	time	NOUN
cet-13155	74	9	,	,	PUNCT
cet-13155	74	10	6	6	NUM
cet-13155	74	11	gcat	gcat	NOUN
cet-13155	74	12	h	h	NOUN
cet-13155	74	13	molc-1	molc-1	NOUN
cet-13155	74	14	;	;	PUNCT
cet-13155	74	15	h2	h2	PROPN
cet-13155	74	16	/	/	SYM
cet-13155	74	17	cox	cox	PROPN
cet-13155	74	18	,	,	PUNCT
cet-13155	74	19	3	3	NUM
cet-13155	74	20	.	.	NOUN
cet-13155	74	21	3.2	3.2	NUM
cet-13155	74	22	alternative	alternative	ADJ
cet-13155	74	23	tandem	tandem	NOUN
cet-13155	74	24	catalysts	catalyst	NOUN
cet-13155	74	25	for	for	ADP
cet-13155	74	26	hydrocarbons	hydrocarbon	NOUN
cet-13155	74	27	synthesis	synthesis	NOUN
cet-13155	74	28	as	as	SCONJ
cet-13155	74	29	mentioned	mention	VERB
cet-13155	74	30	above	above	ADV
cet-13155	74	31	,	,	PUNCT
cet-13155	74	32	working	work	VERB
cet-13155	74	33	in	in	ADP
cet-13155	74	34	a	a	DET
cet-13155	74	35	single	single	ADJ
cet-13155	74	36	stage	stage	NOUN
cet-13155	74	37	has	have	VERB
cet-13155	74	38	several	several	ADJ
cet-13155	74	39	benefits	benefit	NOUN
cet-13155	74	40	,	,	PUNCT
cet-13155	74	41	such	such	ADJ
cet-13155	74	42	as	as	ADP
cet-13155	74	43	a	a	DET
cet-13155	74	44	lower	low	ADJ
cet-13155	74	45	economic	economic	ADJ
cet-13155	74	46	investment	investment	NOUN
cet-13155	74	47	due	due	ADP
cet-13155	74	48	to	to	ADP
cet-13155	74	49	the	the	DET
cet-13155	74	50	use	use	NOUN
cet-13155	74	51	of	of	ADP
cet-13155	74	52	a	a	DET
cet-13155	74	53	single	single	ADJ
cet-13155	74	54	reactor	reactor	NOUN
cet-13155	74	55	.	.	PUNCT
cet-13155	75	1	nonetheless	nonetheless	ADV
cet-13155	75	2	,	,	PUNCT
cet-13155	75	3	the	the	DET
cet-13155	75	4	main	main	ADJ
cet-13155	75	5	advantage	advantage	NOUN
cet-13155	75	6	of	of	ADP
cet-13155	75	7	working	work	VERB
cet-13155	75	8	in	in	ADP
cet-13155	75	9	a	a	DET
cet-13155	75	10	single	single	ADJ
cet-13155	75	11	stage	stage	NOUN
cet-13155	75	12	is	be	AUX
cet-13155	75	13	the	the	DET
cet-13155	75	14	shifting	shifting	NOUN
cet-13155	75	15	of	of	ADP
cet-13155	75	16	the	the	DET
cet-13155	75	17	equilibrium	equilibrium	NOUN
cet-13155	75	18	,	,	PUNCT
cet-13155	75	19	as	as	SCONJ
cet-13155	75	20	methanol	methanol	NOUN
cet-13155	75	21	immediately	immediately	ADV
cet-13155	75	22	converts	convert	VERB
cet-13155	75	23	into	into	ADP
cet-13155	75	24	higher	high	ADJ
cet-13155	75	25	hydrocarbons	hydrocarbon	NOUN
cet-13155	75	26	when	when	SCONJ
cet-13155	75	27	operating	operate	VERB
cet-13155	75	28	in	in	ADP
cet-13155	75	29	the	the	DET
cet-13155	75	30	same	same	ADJ
cet-13155	75	31	reactor	reactor	NOUN
cet-13155	75	32	.	.	PUNCT
cet-13155	76	1	this	this	DET
cet-13155	76	2	way	way	NOUN
cet-13155	76	3	,	,	PUNCT
cet-13155	76	4	the	the	DET
cet-13155	76	5	role	role	NOUN
cet-13155	76	6	of	of	ADP
cet-13155	76	7	the	the	DET
cet-13155	76	8	synergy	synergy	NOUN
cet-13155	76	9	between	between	ADP
cet-13155	76	10	the	the	DET
cet-13155	76	11	metallic	metallic	NOUN
cet-13155	76	12	and	and	CCONJ
cet-13155	76	13	the	the	DET
cet-13155	76	14	acid	acid	NOUN
cet-13155	76	15	catalyst	catalyst	NOUN
cet-13155	76	16	becomes	become	VERB
cet-13155	76	17	an	an	DET
cet-13155	76	18	essential	essential	ADJ
cet-13155	76	19	aspect	aspect	NOUN
cet-13155	76	20	.	.	PUNCT
cet-13155	77	1	therefore	therefore	ADV
cet-13155	77	2	,	,	PUNCT
cet-13155	77	3	cuznzr	cuznzr	ADJ
cet-13155	77	4	and	and	CCONJ
cet-13155	77	5	inzr	inzr	NOUN
cet-13155	77	6	were	be	AUX
cet-13155	77	7	tested	test	VERB
cet-13155	77	8	in	in	ADP
cet-13155	77	9	tandem	tandem	NOUN
cet-13155	77	10	with	with	ADP
cet-13155	77	11	hzsm-5	hzsm-5	NOUN
cet-13155	77	12	zeolite	zeolite	NOUN
cet-13155	77	13	(	(	PUNCT
cet-13155	77	14	cuznzr	cuznzr	NOUN
cet-13155	77	15	/	/	SYM
cet-13155	77	16	h5	h5	NOUN
cet-13155	77	17	and	and	CCONJ
cet-13155	77	18	inzr	inzr	NOUN
cet-13155	77	19	/	/	SYM
cet-13155	77	20	h5	h5	PROPN
cet-13155	77	21	)	)	PUNCT
cet-13155	77	22	,	,	PUNCT
cet-13155	77	23	as	as	SCONJ
cet-13155	77	24	to	to	PART
cet-13155	77	25	prove	prove	VERB
cet-13155	77	26	whether	whether	SCONJ
cet-13155	77	27	these	these	DET
cet-13155	77	28	metallic	metallic	ADJ
cet-13155	77	29	oxide	oxide	NOUN
cet-13155	77	30	catalysts	catalyst	NOUN
cet-13155	77	31	were	be	AUX
cet-13155	77	32	feasible	feasible	ADJ
cet-13155	77	33	for	for	ADP
cet-13155	77	34	operating	operate	VERB
cet-13155	77	35	in	in	ADP
cet-13155	77	36	the	the	DET
cet-13155	77	37	integrated	integrate	VERB
cet-13155	77	38	cox	cox	PROPN
cet-13155	77	39	to	to	ADP
cet-13155	77	40	hydrocarbons	hydrocarbon	NOUN
cet-13155	77	41	process	process	NOUN
cet-13155	77	42	.	.	PUNCT
cet-13155	78	1	since	since	SCONJ
cet-13155	78	2	methanol	methanol	NOUN
cet-13155	78	3	synthesis	synthesis	NOUN
cet-13155	78	4	step	step	NOUN
cet-13155	78	5	is	be	AUX
cet-13155	78	6	favored	favor	VERB
cet-13155	78	7	at	at	ADP
cet-13155	78	8	low	low	ADJ
cet-13155	78	9	temperature	temperature	NOUN
cet-13155	78	10	(	(	PUNCT
cet-13155	78	11	and	and	CCONJ
cet-13155	78	12	high	high	ADJ
cet-13155	78	13	pressure	pressure	NOUN
cet-13155	78	14	)	)	PUNCT
cet-13155	78	15	and	and	CCONJ
cet-13155	78	16	methanol	methanol	NOUN
cet-13155	78	17	to	to	ADP
cet-13155	78	18	hydrocarbons	hydrocarbon	NOUN
cet-13155	78	19	(	(	PUNCT
cet-13155	78	20	mth	mth	NOUN
cet-13155	78	21	)	)	PUNCT
cet-13155	78	22	reactions	reaction	NOUN
cet-13155	78	23	are	be	AUX
cet-13155	78	24	favored	favor	VERB
cet-13155	78	25	at	at	ADP
cet-13155	78	26	high	high	ADJ
cet-13155	78	27	temperature	temperature	NOUN
cet-13155	78	28	,	,	PUNCT
cet-13155	78	29	optimizing	optimize	VERB
cet-13155	78	30	the	the	DET
cet-13155	78	31	operating	operating	NOUN
cet-13155	78	32	conditions	condition	NOUN
cet-13155	78	33	for	for	ADP
cet-13155	78	34	boosting	boost	VERB
cet-13155	78	35	the	the	DET
cet-13155	78	36	whole	whole	ADJ
cet-13155	78	37	process	process	NOUN
cet-13155	78	38	in	in	ADP
cet-13155	78	39	a	a	DET
cet-13155	78	40	single	single	ADJ
cet-13155	78	41	stage	stage	NOUN
cet-13155	78	42	is	be	AUX
cet-13155	78	43	a	a	DET
cet-13155	78	44	key	key	ADJ
cet-13155	78	45	feature	feature	NOUN
cet-13155	78	46	.	.	PUNCT
cet-13155	79	1	figures	figure	NOUN
cet-13155	79	2	3	3	NUM
cet-13155	79	3	and	and	CCONJ
cet-13155	79	4	4	4	NUM
cet-13155	79	5	display	display	VERB
cet-13155	79	6	the	the	DET
cet-13155	79	7	yield	yield	NOUN
cet-13155	79	8	of	of	ADP
cet-13155	79	9	the	the	DET
cet-13155	79	10	desired	desire	VERB
cet-13155	79	11	products	product	NOUN
cet-13155	79	12	,	,	PUNCT
cet-13155	79	13	i.e.	i.e.	X
cet-13155	79	14	,	,	PUNCT
cet-13155	79	15	methanol	methanol	NOUN
cet-13155	79	16	when	when	SCONJ
cet-13155	79	17	the	the	DET
cet-13155	79	18	reactions	reaction	NOUN
cet-13155	79	19	were	be	AUX
cet-13155	79	20	carried	carry	VERB
cet-13155	79	21	out	out	ADP
cet-13155	79	22	with	with	ADP
cet-13155	79	23	the	the	DET
cet-13155	79	24	metallic	metallic	ADJ
cet-13155	79	25	cuznzr	cuznzr	ADJ
cet-13155	79	26	and	and	CCONJ
cet-13155	79	27	inzr	inzr	ADJ
cet-13155	79	28	catalysts	catalyst	NOUN
cet-13155	79	29	and	and	CCONJ
cet-13155	79	30	fuel	fuel	NOUN
cet-13155	79	31	-	-	PUNCT
cet-13155	79	32	range	range	NOUN
cet-13155	79	33	hydrocarbons	hydrocarbon	NOUN
cet-13155	79	34	(	(	PUNCT
cet-13155	79	35	c5	c5	PROPN
cet-13155	79	36	+	+	PROPN
cet-13155	79	37	hydrocarbons	hydrocarbon	NOUN
cet-13155	79	38	)	)	PUNCT
cet-13155	79	39	when	when	SCONJ
cet-13155	79	40	tandem	tandem	NOUN
cet-13155	79	41	catalysts	catalyst	NOUN
cet-13155	79	42	were	be	AUX
cet-13155	79	43	tested	test	VERB
cet-13155	79	44	.	.	PUNCT
cet-13155	80	1	it	it	PRON
cet-13155	80	2	can	can	AUX
cet-13155	80	3	be	be	AUX
cet-13155	80	4	observed	observe	VERB
cet-13155	80	5	that	that	SCONJ
cet-13155	80	6	,	,	PUNCT
cet-13155	80	7	as	as	SCONJ
cet-13155	80	8	concluded	conclude	VERB
cet-13155	80	9	before	before	ADV
cet-13155	80	10	,	,	PUNCT
cet-13155	80	11	obtaining	obtain	VERB
cet-13155	80	12	a	a	DET
cet-13155	80	13	higher	high	ADJ
cet-13155	80	14	methanol	methanol	NOUN
cet-13155	80	15	production	production	NOUN
cet-13155	80	16	with	with	ADP
cet-13155	80	17	the	the	DET
cet-13155	80	18	cuznzr	cuznzr	NOUN
cet-13155	80	19	than	than	ADP
cet-13155	80	20	with	with	ADP
cet-13155	80	21	inzr	inzr	NOUN
cet-13155	80	22	did	do	AUX
cet-13155	80	23	not	not	PART
cet-13155	80	24	result	result	VERB
cet-13155	80	25	in	in	ADP
cet-13155	80	26	a	a	DET
cet-13155	80	27	better	well	ADJ
cet-13155	80	28	performance	performance	NOUN
cet-13155	80	29	with	with	ADP
cet-13155	80	30	tandem	tandem	NOUN
cet-13155	80	31	configuration	configuration	NOUN
cet-13155	80	32	,	,	PUNCT
cet-13155	80	33	evidencing	evidence	VERB
cet-13155	80	34	that	that	SCONJ
cet-13155	80	35	achieving	achieve	VERB
cet-13155	80	36	a	a	DET
cet-13155	80	37	successful	successful	ADJ
cet-13155	80	38	synergy	synergy	NOUN
cet-13155	80	39	among	among	ADP
cet-13155	80	40	catalysts	catalyst	NOUN
cet-13155	80	41	is	be	AUX
cet-13155	80	42	more	more	ADV
cet-13155	80	43	significant	significant	ADJ
cet-13155	80	44	than	than	ADP
cet-13155	80	45	combining	combine	VERB
cet-13155	80	46	the	the	DET
cet-13155	80	47	best	good	ADJ
cet-13155	80	48	catalysts	catalyst	NOUN
cet-13155	80	49	in	in	ADP
cet-13155	80	50	the	the	DET
cet-13155	80	51	same	same	ADJ
cet-13155	80	52	conditions	condition	NOUN
cet-13155	80	53	.	.	PUNCT
cet-13155	81	1	in	in	ADP
cet-13155	81	2	fact	fact	NOUN
cet-13155	81	3	,	,	PUNCT
cet-13155	81	4	as	as	SCONJ
cet-13155	81	5	observed	observe	VERB
cet-13155	81	6	in	in	ADP
cet-13155	81	7	figure	figure	NOUN
cet-13155	81	8	3	3	NUM
cet-13155	81	9	,	,	PUNCT
cet-13155	81	10	even	even	ADV
cet-13155	81	11	if	if	SCONJ
cet-13155	81	12	at	at	ADP
cet-13155	81	13	low	low	ADJ
cet-13155	81	14	temperature	temperature	NOUN
cet-13155	81	15	,	,	PUNCT
cet-13155	81	16	high	high	ADJ
cet-13155	81	17	methanol	methanol	NOUN
cet-13155	81	18	production	production	NOUN
cet-13155	81	19	was	be	AUX
cet-13155	81	20	obtained	obtain	VERB
cet-13155	81	21	,	,	PUNCT
cet-13155	81	22	virtually	virtually	ADV
cet-13155	81	23	no	no	DET
cet-13155	81	24	hydrocarbons	hydrocarbon	NOUN
cet-13155	81	25	were	be	AUX
cet-13155	81	26	yielded	yield	VERB
cet-13155	81	27	at	at	ADP
cet-13155	81	28	340	340	NUM
cet-13155	81	29	ºc	ºc	NOUN
cet-13155	81	30	(	(	PUNCT
cet-13155	81	31	~0.1	~0.1	NOUN
cet-13155	81	32	%	%	INTJ
cet-13155	81	33	)	)	PUNCT
cet-13155	81	34	.	.	PUNCT
cet-13155	82	1	at	at	ADP
cet-13155	82	2	this	this	DET
cet-13155	82	3	temperature	temperature	NOUN
cet-13155	82	4	,	,	PUNCT
cet-13155	82	5	the	the	DET
cet-13155	82	6	methanol	methanol	NOUN
cet-13155	82	7	was	be	AUX
cet-13155	82	8	selectively	selectively	ADV
cet-13155	82	9	dehydrated	dehydrate	VERB
cet-13155	82	10	to	to	ADP
cet-13155	82	11	dimethyl	dimethyl	PROPN
cet-13155	82	12	ether	ether	NOUN
cet-13155	82	13	over	over	ADP
cet-13155	82	14	the	the	DET
cet-13155	82	15	hzsm-5	hzsm-5	NOUN
cet-13155	82	16	zeolite	zeolite	NOUN
cet-13155	82	17	and	and	CCONJ
cet-13155	82	18	the	the	DET
cet-13155	82	19	hydrocarbon	hydrocarbon	NOUN
cet-13155	82	20	pool	pool	NOUN
cet-13155	82	21	mechanism	mechanism	NOUN
cet-13155	82	22	did	do	AUX
cet-13155	82	23	require	require	VERB
cet-13155	82	24	higher	high	ADJ
cet-13155	82	25	temperature	temperature	NOUN
cet-13155	82	26	to	to	PART
cet-13155	82	27	activate	activate	VERB
cet-13155	82	28	.	.	PUNCT
cet-13155	83	1	as	as	SCONJ
cet-13155	83	2	temperature	temperature	NOUN
cet-13155	83	3	increased	increase	VERB
cet-13155	83	4	,	,	PUNCT
cet-13155	83	5	hydrocarbons	hydrocarbon	NOUN
cet-13155	83	6	started	start	VERB
cet-13155	83	7	to	to	PART
cet-13155	83	8	form	form	VERB
cet-13155	83	9	over	over	ADP
cet-13155	83	10	the	the	DET
cet-13155	83	11	zeolite	zeolite	NOUN
cet-13155	83	12	(	(	PUNCT
cet-13155	83	13	mainly	mainly	ADV
cet-13155	83	14	c2	c2	PROPN
cet-13155	83	15	-	-	PUNCT
cet-13155	83	16	c4	c4	NOUN
cet-13155	83	17	paraffins	paraffin	NOUN
cet-13155	83	18	)	)	PUNCT
cet-13155	83	19	.	.	PUNCT
cet-13155	84	1	however	however	ADV
cet-13155	84	2	,	,	PUNCT
cet-13155	84	3	as	as	ADP
cet-13155	84	4	a	a	DET
cet-13155	84	5	consequence	consequence	NOUN
cet-13155	84	6	of	of	ADP
cet-13155	84	7	the	the	DET
cet-13155	84	8	decline	decline	NOUN
cet-13155	84	9	of	of	ADP
cet-13155	84	10	the	the	DET
cet-13155	84	11	cuznzr	cuznzr	ADJ
cet-13155	84	12	catalyst	catalyst	NOUN
cet-13155	84	13	due	due	ADP
cet-13155	84	14	to	to	ADP
cet-13155	84	15	the	the	DET
cet-13155	84	16	thermal	thermal	ADJ
cet-13155	84	17	sintering	sintering	NOUN
cet-13155	84	18	,	,	PUNCT
cet-13155	84	19	the	the	DET
cet-13155	84	20	c5	c5	PROPN
cet-13155	84	21	+	+	PROPN
cet-13155	84	22	hydrocarbons	hydrocarbon	NOUN
cet-13155	84	23	yield	yield	NOUN
cet-13155	84	24	did	do	AUX
cet-13155	84	25	not	not	PART
cet-13155	84	26	exceed	exceed	VERB
cet-13155	84	27	3	3	NUM
cet-13155	84	28	%	%	NOUN
cet-13155	84	29	in	in	ADP
cet-13155	84	30	any	any	DET
cet-13155	84	31	case	case	NOUN
cet-13155	84	32	.	.	PUNCT
cet-13155	85	1	it	it	PRON
cet-13155	85	2	can	can	AUX
cet-13155	85	3	be	be	AUX
cet-13155	85	4	thus	thus	ADV
cet-13155	85	5	concluded	conclude	VERB
cet-13155	85	6	that	that	SCONJ
cet-13155	85	7	cuznzr	cuznzr	NOUN
cet-13155	85	8	/	/	SYM
cet-13155	85	9	h5	h5	PROPN
cet-13155	85	10	tandem	tandem	PROPN
cet-13155	85	11	catalyst	catalyst	NOUN
cet-13155	85	12	is	be	AUX
cet-13155	85	13	a	a	DET
cet-13155	85	14	feasible	feasible	ADJ
cet-13155	85	15	catalyst	catalyst	NOUN
cet-13155	85	16	for	for	ADP
cet-13155	85	17	dimethyl	dimethyl	NOUN
cet-13155	85	18	ether	ether	NOUN
cet-13155	85	19	production	production	NOUN
cet-13155	85	20	,	,	PUNCT
cet-13155	85	21	but	but	CCONJ
cet-13155	85	22	it	it	PRON
cet-13155	85	23	is	be	AUX
cet-13155	85	24	not	not	PART
cet-13155	85	25	a	a	DET
cet-13155	85	26	good	good	ADJ
cet-13155	85	27	choice	choice	NOUN
cet-13155	85	28	for	for	ADP
cet-13155	85	29	fuel	fuel	NOUN
cet-13155	85	30	-	-	PUNCT
cet-13155	85	31	range	range	NOUN
cet-13155	85	32	hydrocarbons	hydrocarbon	NOUN
cet-13155	85	33	production	production	NOUN
cet-13155	85	34	as	as	SCONJ
cet-13155	85	35	targeted	target	VERB
cet-13155	85	36	.	.	PUNCT
cet-13155	86	1	on	on	ADP
cet-13155	86	2	the	the	DET
cet-13155	86	3	other	other	ADJ
cet-13155	86	4	hand	hand	NOUN
cet-13155	86	5	,	,	PUNCT
cet-13155	86	6	the	the	DET
cet-13155	86	7	results	result	NOUN
cet-13155	86	8	completely	completely	ADV
cet-13155	86	9	differed	differ	VERB
cet-13155	86	10	with	with	ADP
cet-13155	86	11	inzr	inzr	NOUN
cet-13155	86	12	/	/	SYM
cet-13155	86	13	h5	h5	PROPN
cet-13155	86	14	tandem	tandem	NOUN
cet-13155	86	15	catalyst	catalyst	NOUN
cet-13155	86	16	.	.	PUNCT
cet-13155	87	1	as	as	SCONJ
cet-13155	87	2	exhibited	exhibit	VERB
cet-13155	87	3	in	in	ADP
cet-13155	87	4	figure	figure	NOUN
cet-13155	87	5	4	4	NUM
cet-13155	87	6	,	,	PUNCT
cet-13155	87	7	considerably	considerably	ADV
cet-13155	87	8	lower	low	ADJ
cet-13155	87	9	methanol	methanol	NOUN
cet-13155	87	10	yield	yield	NOUN
cet-13155	87	11	was	be	AUX
cet-13155	87	12	obtained	obtain	VERB
cet-13155	87	13	with	with	ADP
cet-13155	87	14	inzr	inzr	ADJ
cet-13155	87	15	metallic	metallic	ADJ
cet-13155	87	16	catalyst	catalyst	NOUN
cet-13155	87	17	as	as	SCONJ
cet-13155	87	18	compared	compare	VERB
cet-13155	87	19	with	with	ADP
cet-13155	87	20	cuznzr	cuznzr	NOUN
cet-13155	87	21	.	.	PUNCT
cet-13155	88	1	nevertheless	nevertheless	ADV
cet-13155	88	2	,	,	PUNCT
cet-13155	88	3	inzr	inzr	NOUN
cet-13155	88	4	did	do	AUX
cet-13155	88	5	not	not	PART
cet-13155	88	6	suffer	suffer	VERB
cet-13155	88	7	any	any	DET
cet-13155	88	8	thermal	thermal	ADJ
cet-13155	88	9	sintering	sintering	NOUN
cet-13155	88	10	,	,	PUNCT
cet-13155	88	11	leading	lead	VERB
cet-13155	88	12	to	to	ADP
cet-13155	88	13	highly	highly	ADV
cet-13155	88	14	enhanced	enhance	VERB
cet-13155	88	15	results	result	NOUN
cet-13155	88	16	.	.	PUNCT
cet-13155	89	1	even	even	ADV
cet-13155	89	2	at	at	ADP
cet-13155	89	3	low	low	ADJ
cet-13155	89	4	temperature	temperature	NOUN
cet-13155	89	5	,	,	PUNCT
cet-13155	89	6	the	the	DET
cet-13155	89	7	c5	c5	PROPN
cet-13155	89	8	+	+	NOUN
cet-13155	89	9	hydrocarbon	hydrocarbon	NOUN
cet-13155	89	10	yield	yield	NOUN
cet-13155	89	11	was	be	AUX
cet-13155	89	12	higher	high	ADJ
cet-13155	89	13	than	than	ADP
cet-13155	89	14	the	the	DET
cet-13155	89	15	maximum	maximum	NOUN
cet-13155	89	16	obtained	obtain	VERB
cet-13155	89	17	with	with	ADP
cet-13155	89	18	cuznzr	cuznzr	NOUN
cet-13155	89	19	/	/	SYM
cet-13155	89	20	h5	h5	NOUN
cet-13155	89	21	(	(	PUNCT
cet-13155	89	22	4.9	4.9	NUM
cet-13155	89	23	%	%	NOUN
cet-13155	89	24	vs.	vs.	ADP
cet-13155	89	25	2.9	2.9	NUM
cet-13155	89	26	%	%	NOUN
cet-13155	89	27	)	)	PUNCT
cet-13155	89	28	.	.	PUNCT
cet-13155	90	1	as	as	SCONJ
cet-13155	90	2	temperature	temperature	NOUN
cet-13155	90	3	was	be	AUX
cet-13155	90	4	risen	rise	VERB
cet-13155	90	5	,	,	PUNCT
cet-13155	90	6	owing	owe	VERB
cet-13155	90	7	to	to	ADP
cet-13155	90	8	the	the	DET
cet-13155	90	9	favored	favor	VERB
cet-13155	90	10	mth	mth	NOUN
cet-13155	90	11	reactions	reaction	NOUN
cet-13155	90	12	,	,	PUNCT
cet-13155	90	13	hydrocarbon	hydrocarbon	NOUN
cet-13155	90	14	production	production	NOUN
cet-13155	90	15	sharply	sharply	ADV
cet-13155	90	16	increased	increase	VERB
cet-13155	90	17	.	.	PUNCT
cet-13155	91	1	in	in	ADP
cet-13155	91	2	fact	fact	NOUN
cet-13155	91	3	,	,	PUNCT
cet-13155	91	4	at	at	ADP
cet-13155	91	5	420	420	NUM
cet-13155	91	6	ºc	ºc	NOUN
cet-13155	91	7	,	,	PUNCT
cet-13155	91	8	the	the	DET
cet-13155	91	9	c5	c5	PROPN
cet-13155	91	10	+	+	CCONJ
cet-13155	91	11	yield	yield	NOUN
cet-13155	91	12	reached	reach	VERB
cet-13155	91	13	17	17	NUM
cet-13155	91	14	%	%	NOUN
cet-13155	91	15	.	.	PUNCT
cet-13155	92	1	even	even	ADV
cet-13155	92	2	if	if	SCONJ
cet-13155	92	3	almost	almost	ADV
cet-13155	92	4	no	no	DET
cet-13155	92	5	methanol	methanol	NOUN
cet-13155	92	6	was	be	AUX
cet-13155	92	7	produced	produce	VERB
cet-13155	92	8	only	only	ADV
cet-13155	92	9	with	with	ADP
cet-13155	92	10	the	the	DET
cet-13155	92	11	metallic	metallic	ADJ
cet-13155	92	12	catalyst	catalyst	NOUN
cet-13155	92	13	at	at	ADP
cet-13155	92	14	these	these	DET
cet-13155	92	15	conditions	condition	NOUN
cet-13155	92	16	,	,	PUNCT
cet-13155	92	17	the	the	DET
cet-13155	92	18	high	high	ADJ
cet-13155	92	19	hydrocarbons	hydrocarbon	NOUN
cet-13155	92	20	production	production	NOUN
cet-13155	92	21	was	be	AUX
cet-13155	92	22	obtained	obtain	VERB
cet-13155	92	23	by	by	ADP
cet-13155	92	24	dint	dint	NOUN
cet-13155	92	25	of	of	ADP
cet-13155	92	26	the	the	DET
cet-13155	92	27	displaced	displaced	ADJ
cet-13155	92	28	equilibrium	equilibrium	NOUN
cet-13155	92	29	of	of	ADP
cet-13155	92	30	the	the	DET
cet-13155	92	31	first	first	ADJ
cet-13155	92	32	step	step	NOUN
cet-13155	92	33	in	in	ADP
cet-13155	92	34	the	the	DET
cet-13155	92	35	integrated	integrate	VERB
cet-13155	92	36	process	process	NOUN
cet-13155	92	37	.	.	PUNCT
cet-13155	93	1	the	the	DET
cet-13155	93	2	great	great	ADJ
cet-13155	93	3	thermodynamic	thermodynamic	ADJ
cet-13155	93	4	advantage	advantage	NOUN
cet-13155	93	5	of	of	ADP
cet-13155	93	6	operating	operate	VERB
cet-13155	93	7	in	in	ADP
cet-13155	93	8	a	a	DET
cet-13155	93	9	single	single	ADJ
cet-13155	93	10	stage	stage	NOUN
cet-13155	93	11	is	be	AUX
cet-13155	93	12	therefore	therefore	ADV
cet-13155	93	13	evidenced	evidence	VERB
cet-13155	93	14	.	.	PUNCT
cet-13155	94	1	moreover	moreover	ADV
cet-13155	94	2	,	,	PUNCT
cet-13155	94	3	with	with	ADP
cet-13155	94	4	the	the	DET
cet-13155	94	5	inzr	inzr	NOUN
cet-13155	94	6	/	/	SYM
cet-13155	94	7	h5	h5	PROPN
cet-13155	94	8	tandem	tandem	NOUN
cet-13155	94	9	catalyst	catalyst	NOUN
cet-13155	94	10	,	,	PUNCT
cet-13155	94	11	the	the	DET
cet-13155	94	12	conversion	conversion	NOUN
cet-13155	94	13	of	of	ADP
cet-13155	94	14	co2	co2	NOUN
cet-13155	94	15	/	/	SYM
cet-13155	94	16	co	co	NOUN
cet-13155	94	17	hydrogenation	hydrogenation	NOUN
cet-13155	94	18	rocketed	rocket	VERB
cet-13155	94	19	from	from	ADP
cet-13155	94	20	1.8	1.8	NUM
cet-13155	94	21	%	%	NOUN
cet-13155	94	22	when	when	SCONJ
cet-13155	94	23	operating	operate	VERB
cet-13155	94	24	just	just	ADV
cet-13155	94	25	with	with	ADP
cet-13155	94	26	the	the	DET
cet-13155	94	27	metallic	metallic	ADJ
cet-13155	94	28	catalyst	catalyst	NOUN
cet-13155	94	29	to	to	ADP
cet-13155	94	30	23	23	NUM
cet-13155	94	31	%	%	NOUN
cet-13155	94	32	in	in	ADP
cet-13155	94	33	the	the	DET
cet-13155	94	34	integrated	integrate	VERB
cet-13155	94	35	process	process	NOUN
cet-13155	94	36	.	.	PUNCT
cet-13155	95	1	a	a	DET
cet-13155	95	2	)	)	PUNCT
cet-13155	95	3	b	b	NOUN
cet-13155	95	4	)	)	PUNCT
cet-13155	95	5	460	460	NUM
cet-13155	95	6	figure	figure	NOUN
cet-13155	95	7	3	3	NUM
cet-13155	95	8	.	.	PUNCT
cet-13155	95	9	effect	effect	NOUN
cet-13155	95	10	of	of	ADP
cet-13155	95	11	the	the	DET
cet-13155	95	12	temperature	temperature	NOUN
cet-13155	95	13	on	on	ADP
cet-13155	95	14	the	the	DET
cet-13155	95	15	yield	yield	NOUN
cet-13155	95	16	of	of	ADP
cet-13155	95	17	the	the	DET
cet-13155	95	18	desired	desire	VERB
cet-13155	95	19	product	product	NOUN
cet-13155	95	20	fraction	fraction	NOUN
cet-13155	95	21	:	:	PUNCT
cet-13155	95	22	(	(	PUNCT
cet-13155	95	23	i	i	NOUN
cet-13155	95	24	)	)	PUNCT
cet-13155	95	25	methanol	methanol	NOUN
cet-13155	95	26	(	(	PUNCT
cet-13155	95	27	with	with	ADP
cet-13155	95	28	cuznzr	cuznzr	ADJ
cet-13155	95	29	metallic	metallic	ADJ
cet-13155	95	30	catalyst	catalyst	NOUN
cet-13155	95	31	)	)	PUNCT
cet-13155	95	32	and	and	CCONJ
cet-13155	95	33	(	(	PUNCT
cet-13155	95	34	ii	ii	NOUN
cet-13155	95	35	)	)	PUNCT
cet-13155	95	36	c5	c5	PROPN
cet-13155	95	37	+	+	PROPN
cet-13155	95	38	hydrocarbons	hydrocarbon	NOUN
cet-13155	95	39	(	(	PUNCT
cet-13155	95	40	with	with	ADP
cet-13155	95	41	cuznzr	cuznzr	ADJ
cet-13155	95	42	/	/	SYM
cet-13155	95	43	h5	h5	PROPN
cet-13155	95	44	tandem	tandem	NOUN
cet-13155	95	45	catalyst	catalyst	NOUN
cet-13155	95	46	)	)	PUNCT
cet-13155	95	47	.	.	PUNCT
cet-13155	96	1	reaction	reaction	NOUN
cet-13155	96	2	conditions	condition	NOUN
cet-13155	96	3	:	:	PUNCT
cet-13155	96	4	50	50	NUM
cet-13155	96	5	bar	bar	NOUN
cet-13155	96	6	;	;	PUNCT
cet-13155	96	7	space	space	NOUN
cet-13155	96	8	time	time	NOUN
cet-13155	96	9	,	,	PUNCT
cet-13155	96	10	6	6	NUM
cet-13155	96	11	and	and	CCONJ
cet-13155	96	12	12	12	NUM
cet-13155	96	13	gcat	gcat	NOUN
cet-13155	96	14	h	h	NOUN
cet-13155	96	15	molc-1	molc-1	NOUN
cet-13155	96	16	;	;	PUNCT
cet-13155	96	17	h2	h2	PROPN
cet-13155	96	18	/	/	SYM
cet-13155	96	19	cox	cox	PROPN
cet-13155	96	20	,	,	PUNCT
cet-13155	96	21	3	3	X
cet-13155	96	22	.	.	X
cet-13155	96	23	figure	figure	NOUN
cet-13155	96	24	4	4	NUM
cet-13155	96	25	.	.	PUNCT
cet-13155	96	26	effect	effect	NOUN
cet-13155	96	27	of	of	ADP
cet-13155	96	28	the	the	DET
cet-13155	96	29	temperature	temperature	NOUN
cet-13155	96	30	on	on	ADP
cet-13155	96	31	the	the	DET
cet-13155	96	32	yield	yield	NOUN
cet-13155	96	33	of	of	ADP
cet-13155	96	34	the	the	DET
cet-13155	96	35	desired	desire	VERB
cet-13155	96	36	product	product	NOUN
cet-13155	96	37	fraction	fraction	NOUN
cet-13155	96	38	:	:	PUNCT
cet-13155	96	39	(	(	PUNCT
cet-13155	96	40	i	i	NOUN
cet-13155	96	41	)	)	PUNCT
cet-13155	96	42	methanol	methanol	NOUN
cet-13155	96	43	(	(	PUNCT
cet-13155	96	44	with	with	ADP
cet-13155	96	45	inzr	inzr	ADJ
cet-13155	96	46	metallic	metallic	ADJ
cet-13155	96	47	catalyst	catalyst	NOUN
cet-13155	96	48	)	)	PUNCT
cet-13155	96	49	and	and	CCONJ
cet-13155	96	50	(	(	PUNCT
cet-13155	96	51	ii	ii	NOUN
cet-13155	96	52	)	)	PUNCT
cet-13155	96	53	c5	c5	PROPN
cet-13155	96	54	+	+	PROPN
cet-13155	96	55	hydrocarbons	hydrocarbon	NOUN
cet-13155	96	56	(	(	PUNCT
cet-13155	96	57	with	with	ADP
cet-13155	96	58	inzr	inzr	NOUN
cet-13155	96	59	/	/	SYM
cet-13155	96	60	h5	h5	PROPN
cet-13155	96	61	tandem	tandem	NOUN
cet-13155	96	62	catalyst	catalyst	NOUN
cet-13155	96	63	)	)	PUNCT
cet-13155	96	64	.	.	PUNCT
cet-13155	97	1	reaction	reaction	NOUN
cet-13155	97	2	conditions	condition	NOUN
cet-13155	97	3	:	:	PUNCT
cet-13155	97	4	50	50	NUM
cet-13155	97	5	bar	bar	NOUN
cet-13155	97	6	;	;	PUNCT
cet-13155	97	7	space	space	NOUN
cet-13155	97	8	time	time	NOUN
cet-13155	97	9	,	,	PUNCT
cet-13155	97	10	6	6	NUM
cet-13155	97	11	and	and	CCONJ
cet-13155	97	12	12	12	NUM
cet-13155	97	13	gcat	gcat	NOUN
cet-13155	97	14	h	h	NOUN
cet-13155	97	15	molc-1	molc-1	NOUN
cet-13155	97	16	;	;	PUNCT
cet-13155	97	17	h2	h2	PROPN
cet-13155	97	18	/	/	SYM
cet-13155	97	19	cox	cox	PROPN
cet-13155	97	20	,	,	PUNCT
cet-13155	97	21	3	3	X
cet-13155	97	22	.	.	PUNCT
cet-13155	97	23	table	table	NOUN
cet-13155	97	24	1	1	NUM
cet-13155	97	25	shows	show	VERB
cet-13155	97	26	the	the	DET
cet-13155	97	27	distribution	distribution	NOUN
cet-13155	97	28	of	of	ADP
cet-13155	97	29	the	the	DET
cet-13155	97	30	obtained	obtain	VERB
cet-13155	97	31	hydrocarbons	hydrocarbon	NOUN
cet-13155	97	32	at	at	ADP
cet-13155	97	33	420	420	NUM
cet-13155	97	34	ºc	ºc	NOUN
cet-13155	97	35	.	.	PUNCT
cet-13155	97	36	isoparaffins	isoparaffin	NOUN
cet-13155	97	37	in	in	ADP
cet-13155	97	38	the	the	DET
cet-13155	97	39	c4	c4	NOUN
cet-13155	97	40	-	-	PUNCT
cet-13155	97	41	c6	c6	PROPN
cet-13155	97	42	range	range	NOUN
cet-13155	97	43	turned	turn	VERB
cet-13155	97	44	out	out	ADP
cet-13155	97	45	to	to	PART
cet-13155	97	46	be	be	AUX
cet-13155	97	47	the	the	DET
cet-13155	97	48	most	most	ADV
cet-13155	97	49	numerous	numerous	ADJ
cet-13155	97	50	produced	produce	VERB
cet-13155	97	51	hydrocarbons	hydrocarbon	NOUN
cet-13155	97	52	,	,	PUNCT
cet-13155	97	53	accounting	account	VERB
cet-13155	97	54	for	for	ADP
cet-13155	97	55	more	more	ADJ
cet-13155	97	56	than	than	ADP
cet-13155	97	57	half	half	NOUN
cet-13155	97	58	of	of	ADP
cet-13155	97	59	the	the	DET
cet-13155	97	60	obtained	obtain	VERB
cet-13155	97	61	hydrocarbon	hydrocarbon	NOUN
cet-13155	97	62	products	product	NOUN
cet-13155	97	63	.	.	PUNCT
cet-13155	98	1	almost	almost	ADV
cet-13155	98	2	no	no	DET
cet-13155	98	3	aromatics	aromatic	NOUN
cet-13155	98	4	were	be	AUX
cet-13155	98	5	produced	produce	VERB
cet-13155	98	6	,	,	PUNCT
cet-13155	98	7	and	and	CCONJ
cet-13155	98	8	olefins	olefin	NOUN
cet-13155	98	9	did	do	AUX
cet-13155	98	10	not	not	PART
cet-13155	98	11	reach	reach	VERB
cet-13155	98	12	15	15	NUM
cet-13155	98	13	%	%	NOUN
cet-13155	98	14	.	.	PUNCT
cet-13155	99	1	this	this	DET
cet-13155	99	2	composition	composition	NOUN
cet-13155	99	3	is	be	AUX
cet-13155	99	4	very	very	ADV
cet-13155	99	5	suitable	suitable	ADJ
cet-13155	99	6	for	for	ADP
cet-13155	99	7	its	its	PRON
cet-13155	99	8	incorporation	incorporation	NOUN
cet-13155	99	9	into	into	ADP
cet-13155	99	10	the	the	DET
cet-13155	99	11	gasoline	gasoline	NOUN
cet-13155	99	12	-	-	PUNCT
cet-13155	99	13	pool	pool	NOUN
cet-13155	99	14	.	.	PUNCT
cet-13155	100	1	because	because	SCONJ
cet-13155	100	2	,	,	PUNCT
cet-13155	100	3	when	when	SCONJ
cet-13155	100	4	mixed	mix	VERB
cet-13155	100	5	with	with	ADP
cet-13155	100	6	streams	stream	NOUN
cet-13155	100	7	with	with	ADP
cet-13155	100	8	high	high	ADJ
cet-13155	100	9	aromatic	aromatic	NOUN
cet-13155	100	10	(	(	PUNCT
cet-13155	100	11	such	such	ADJ
cet-13155	100	12	as	as	ADP
cet-13155	100	13	those	those	PRON
cet-13155	100	14	from	from	ADP
cet-13155	100	15	the	the	DET
cet-13155	100	16	fcc	fcc	PROPN
cet-13155	100	17	)	)	PUNCT
cet-13155	100	18	or	or	CCONJ
cet-13155	100	19	olefin	olefin	NOUN
cet-13155	100	20	content	content	NOUN
cet-13155	100	21	,	,	PUNCT
cet-13155	100	22	it	it	PRON
cet-13155	100	23	would	would	AUX
cet-13155	100	24	help	help	VERB
cet-13155	100	25	meet	meet	VERB
cet-13155	100	26	environmental	environmental	ADJ
cet-13155	100	27	requirements	requirement	NOUN
cet-13155	100	28	.	.	PUNCT
cet-13155	101	1	in	in	ADP
cet-13155	101	2	addition	addition	NOUN
cet-13155	101	3	,	,	PUNCT
cet-13155	101	4	it	it	PRON
cet-13155	101	5	is	be	AUX
cet-13155	101	6	remarkable	remarkable	ADJ
cet-13155	101	7	that	that	SCONJ
cet-13155	101	8	the	the	DET
cet-13155	101	9	produced	produce	VERB
cet-13155	101	10	hydrocarbons	hydrocarbon	NOUN
cet-13155	101	11	do	do	AUX
cet-13155	101	12	not	not	PART
cet-13155	101	13	contain	contain	VERB
cet-13155	101	14	s	s	PRON
cet-13155	101	15	or	or	CCONJ
cet-13155	101	16	n	n	CCONJ
cet-13155	101	17	,	,	PUNCT
cet-13155	101	18	pollutants	pollutant	NOUN
cet-13155	101	19	present	present	ADJ
cet-13155	101	20	in	in	ADP
cet-13155	101	21	refinery	refinery	NOUN
cet-13155	101	22	streams	stream	NOUN
cet-13155	101	23	.	.	PUNCT
cet-13155	102	1	on	on	ADP
cet-13155	102	2	the	the	DET
cet-13155	102	3	other	other	ADJ
cet-13155	102	4	hand	hand	NOUN
cet-13155	102	5	,	,	PUNCT
cet-13155	102	6	its	its	PRON
cet-13155	102	7	commercial	commercial	ADJ
cet-13155	102	8	application	application	NOUN
cet-13155	102	9	is	be	AUX
cet-13155	102	10	interesting	interesting	ADJ
cet-13155	102	11	for	for	ADP
cet-13155	102	12	the	the	DET
cet-13155	102	13	co2	co2	NOUN
cet-13155	102	14	valorization	valorization	NOUN
cet-13155	102	15	policies	policy	NOUN
cet-13155	102	16	aimed	aim	VERB
cet-13155	102	17	at	at	ADP
cet-13155	102	18	synthesizing	synthesize	VERB
cet-13155	102	19	products	product	NOUN
cet-13155	102	20	of	of	ADP
cet-13155	102	21	commercial	commercial	ADJ
cet-13155	102	22	interest	interest	NOUN
cet-13155	102	23	that	that	PRON
cet-13155	102	24	partially	partially	ADV
cet-13155	102	25	compensate	compensate	VERB
cet-13155	102	26	the	the	DET
cet-13155	102	27	costs	cost	NOUN
cet-13155	102	28	of	of	ADP
cet-13155	102	29	co2	co2	NOUN
cet-13155	102	30	capture	capture	NOUN
cet-13155	102	31	technologies	technology	NOUN
cet-13155	102	32	and	and	CCONJ
cet-13155	102	33	the	the	DET
cet-13155	102	34	higher	high	ADJ
cet-13155	102	35	cost	cost	NOUN
cet-13155	102	36	of	of	ADP
cet-13155	102	37	indium	indium	NOUN
cet-13155	102	38	-	-	PUNCT
cet-13155	102	39	based	base	VERB
cet-13155	102	40	catalysts	catalyst	NOUN
cet-13155	102	41	.	.	PUNCT
cet-13155	103	1	it	it	PRON
cet-13155	103	2	is	be	AUX
cet-13155	103	3	noteworthy	noteworthy	ADJ
cet-13155	103	4	that	that	SCONJ
cet-13155	103	5	the	the	DET
cet-13155	103	6	hydrocarbons	hydrocarbon	NOUN
cet-13155	103	7	obtained	obtain	VERB
cet-13155	103	8	with	with	ADP
cet-13155	103	9	cuznzr	cuznzr	ADJ
cet-13155	103	10	/	/	SYM
cet-13155	103	11	h5	h5	PROPN
cet-13155	103	12	were	be	AUX
cet-13155	103	13	mainly	mainly	ADV
cet-13155	103	14	5	5	NUM
cet-13155	103	15	carbon	carbon	NOUN
cet-13155	103	16	number	number	NOUN
cet-13155	103	17	paraffins	paraffin	NOUN
cet-13155	103	18	,	,	PUNCT
cet-13155	103	19	with	with	ADP
cet-13155	103	20	almost	almost	ADV
cet-13155	103	21	no	no	PRON
cet-13155	103	22	presence	presence	NOUN
cet-13155	103	23	of	of	ADP
cet-13155	103	24	naphthenic	naphthenic	ADJ
cet-13155	103	25	or	or	CCONJ
cet-13155	103	26	aromatic	aromatic	ADJ
cet-13155	103	27	compounds	compound	NOUN
cet-13155	103	28	.	.	PUNCT
cet-13155	104	1	461	461	NUM
cet-13155	104	2	table	table	NOUN
cet-13155	104	3	1	1	NUM
cet-13155	104	4	:	:	PUNCT
cet-13155	104	5	distribution	distribution	NOUN
cet-13155	104	6	of	of	ADP
cet-13155	104	7	hydrocarbons	hydrocarbon	NOUN
cet-13155	104	8	by	by	ADP
cet-13155	104	9	product	product	NOUN
cet-13155	104	10	fraction	fraction	NOUN
cet-13155	104	11	and	and	CCONJ
cet-13155	104	12	carbon	carbon	NOUN
cet-13155	104	13	number	number	NOUN
cet-13155	104	14	(	(	PUNCT
cet-13155	104	15	mol	mol	NUM
cet-13155	104	16	%	%	NOUN
cet-13155	104	17	)	)	PUNCT
cet-13155	104	18	obtained	obtain	VERB
cet-13155	104	19	with	with	ADP
cet-13155	104	20	inzr	inzr	ADJ
cet-13155	104	21	/	/	SYM
cet-13155	104	22	h5	h5	NOUN
cet-13155	104	23	catalyst	catalyst	NOUN
cet-13155	104	24	.	.	PUNCT
cet-13155	105	1	reaction	reaction	NOUN
cet-13155	105	2	conditions	condition	NOUN
cet-13155	105	3	:	:	PUNCT
cet-13155	105	4	420	420	NUM
cet-13155	105	5	ºc	ºc	NOUN
cet-13155	105	6	;	;	PUNCT
cet-13155	105	7	50	50	NUM
cet-13155	105	8	bar	bar	NOUN
cet-13155	105	9	;	;	PUNCT
cet-13155	105	10	space	space	NOUN
cet-13155	105	11	time	time	NOUN
cet-13155	105	12	,	,	PUNCT
cet-13155	105	13	12	12	NUM
cet-13155	105	14	gcat	gcat	NOUN
cet-13155	105	15	h	h	NOUN
cet-13155	105	16	molc-1	molc-1	NOUN
cet-13155	105	17	;	;	PUNCT
cet-13155	105	18	h2	h2	PROPN
cet-13155	105	19	/	/	SYM
cet-13155	105	20	cox	cox	PROPN
cet-13155	105	21	,	,	PUNCT
cet-13155	105	22	3	3	X
cet-13155	105	23	.	.	PUNCT
cet-13155	106	1	the	the	DET
cet-13155	106	2	remainder	remainder	NOUN
cet-13155	106	3	to	to	PART
cet-13155	106	4	reach	reach	VERB
cet-13155	106	5	100	100	NUM
cet-13155	106	6	%	%	NOUN
cet-13155	106	7	corresponds	correspond	NOUN
cet-13155	106	8	to	to	PART
cet-13155	106	9	oxygenate	oxygenate	VERB
cet-13155	106	10	fraction	fraction	NOUN
cet-13155	106	11	.	.	PUNCT
cet-13155	107	1	carbon	carbon	NOUN
cet-13155	107	2	number	number	NOUN
cet-13155	107	3	n	n	CCONJ
cet-13155	107	4	-	-	PUNCT
cet-13155	107	5	paraffin	paraffin	NOUN
cet-13155	107	6	isoparaffin	isoparaffin	NOUN
cet-13155	107	7	olefin	olefin	NOUN
cet-13155	107	8	naphthene	naphthene	PROPN
cet-13155	107	9	aromatic	aromatic	ADJ
cet-13155	107	10	c1	c1	PROPN
cet-13155	107	11	8.8	8.8	NUM
cet-13155	107	12	c2	c2	PROPN
cet-13155	107	13	3.0	3.0	NUM
cet-13155	107	14	3.4	3.4	NUM
cet-13155	107	15	c3	c3	NOUN
cet-13155	107	16	5.4	5.4	NUM
cet-13155	107	17	3.4	3.4	NUM
cet-13155	107	18	c4	c4	NOUN
cet-13155	107	19	11.2	11.2	NUM
cet-13155	107	20	5.4	5.4	NUM
cet-13155	107	21	c5	c5	PROPN
cet-13155	107	22	3.2	3.2	NUM
cet-13155	107	23	21.3	21.3	NUM
cet-13155	107	24	0.8	0.8	NUM
cet-13155	107	25	c6	c6	PROPN
cet-13155	107	26	2.2	2.2	NUM
cet-13155	107	27	20.1	20.1	NUM
cet-13155	107	28	2.4	2.4	NUM
cet-13155	107	29	c7	c7	NOUN
cet-13155	107	30	+	+	PROPN
cet-13155	107	31	1.4	1.4	NUM
cet-13155	107	32	4.7	4.7	NUM
cet-13155	107	33	2.2	2.2	NUM
cet-13155	107	34	4	4	NUM
cet-13155	107	35	.	.	PUNCT
cet-13155	108	1	conclusions	conclusion	NOUN
cet-13155	108	2	the	the	DET
cet-13155	108	3	production	production	NOUN
cet-13155	108	4	of	of	ADP
cet-13155	108	5	c5	c5	PROPN
cet-13155	108	6	+	+	CCONJ
cet-13155	108	7	fuel	fuel	NOUN
cet-13155	108	8	-	-	PUNCT
cet-13155	108	9	range	range	NOUN
cet-13155	108	10	hydrocarbons	hydrocarbon	NOUN
cet-13155	108	11	from	from	ADP
cet-13155	108	12	co2	co2	NOUN
cet-13155	108	13	/	/	SYM
cet-13155	108	14	co	co	NOUN
cet-13155	108	15	hydrogenation	hydrogenation	NOUN
cet-13155	108	16	is	be	AUX
cet-13155	108	17	an	an	DET
cet-13155	108	18	interesting	interesting	ADJ
cet-13155	108	19	process	process	NOUN
cet-13155	108	20	for	for	ADP
cet-13155	108	21	co2	co2	NOUN
cet-13155	108	22	valorization	valorization	NOUN
cet-13155	108	23	and	and	CCONJ
cet-13155	108	24	synthesis	synthesis	NOUN
cet-13155	108	25	of	of	ADP
cet-13155	108	26	sustainably	sustainably	ADV
cet-13155	108	27	sourced	source	VERB
cet-13155	108	28	fuels	fuel	NOUN
cet-13155	108	29	.	.	PUNCT
cet-13155	109	1	two	two	NUM
cet-13155	109	2	metallic	metallic	ADJ
cet-13155	109	3	catalysts	catalyst	NOUN
cet-13155	109	4	(	(	PUNCT
cet-13155	109	5	cuo	cuo	PROPN
cet-13155	109	6	-	-	PUNCT
cet-13155	109	7	zno	zno	NOUN
cet-13155	109	8	-	-	ADJ
cet-13155	109	9	zro2	zro2	PROPN
cet-13155	109	10	and	and	CCONJ
cet-13155	109	11	in2o3	in2o3	PROPN
cet-13155	109	12	-	-	PUNCT
cet-13155	109	13	zro2	zro2	PROPN
cet-13155	109	14	)	)	PUNCT
cet-13155	109	15	were	be	AUX
cet-13155	109	16	tested	test	VERB
cet-13155	109	17	under	under	ADP
cet-13155	109	18	different	different	ADJ
cet-13155	109	19	operating	operating	NOUN
cet-13155	109	20	conditions	condition	NOUN
cet-13155	109	21	on	on	ADP
cet-13155	109	22	co2	co2	NOUN
cet-13155	109	23	/	/	SYM
cet-13155	109	24	co	co	NOUN
cet-13155	109	25	hydrogenation	hydrogenation	NOUN
cet-13155	109	26	to	to	PART
cet-13155	109	27	methanol	methanol	VERB
cet-13155	109	28	.	.	PUNCT
cet-13155	110	1	even	even	ADV
cet-13155	110	2	cuo	cuo	PROPN
cet-13155	110	3	-	-	PUNCT
cet-13155	110	4	zno	zno	NOUN
cet-13155	110	5	-	-	PUNCT
cet-13155	110	6	zro2	zro2	PROPN
cet-13155	110	7	seemed	seem	VERB
cet-13155	110	8	a	a	DET
cet-13155	110	9	good	good	ADJ
cet-13155	110	10	alternative	alternative	NOUN
cet-13155	110	11	attending	attend	VERB
cet-13155	110	12	the	the	DET
cet-13155	110	13	high	high	ADJ
cet-13155	110	14	methanol	methanol	NOUN
cet-13155	110	15	yield	yield	NOUN
cet-13155	110	16	obtained	obtain	VERB
cet-13155	110	17	at	at	ADP
cet-13155	110	18	low	low	ADJ
cet-13155	110	19	temperature	temperature	NOUN
cet-13155	110	20	,	,	PUNCT
cet-13155	110	21	the	the	DET
cet-13155	110	22	catalyst	catalyst	NOUN
cet-13155	110	23	suffered	suffer	VERB
cet-13155	110	24	cu	cu	PROPN
cet-13155	110	25	sintered	sinter	VERB
cet-13155	110	26	at	at	ADP
cet-13155	110	27	temperature	temperature	NOUN
cet-13155	110	28	above	above	ADP
cet-13155	110	29	300	300	NUM
cet-13155	110	30	ºc	ºc	NOUN
cet-13155	110	31	,	,	PUNCT
cet-13155	110	32	leading	lead	VERB
cet-13155	110	33	to	to	ADP
cet-13155	110	34	high	high	ADJ
cet-13155	110	35	methane	methane	NOUN
cet-13155	110	36	production	production	NOUN
cet-13155	110	37	and	and	CCONJ
cet-13155	110	38	lower	low	ADJ
cet-13155	110	39	methanol	methanol	NOUN
cet-13155	110	40	yield	yield	NOUN
cet-13155	110	41	in	in	ADP
cet-13155	110	42	the	the	DET
cet-13155	110	43	conditions	condition	NOUN
cet-13155	110	44	required	require	VERB
cet-13155	110	45	for	for	ADP
cet-13155	110	46	the	the	DET
cet-13155	110	47	integrated	integrate	VERB
cet-13155	110	48	process	process	NOUN
cet-13155	110	49	.	.	PUNCT
cet-13155	111	1	on	on	ADP
cet-13155	111	2	the	the	DET
cet-13155	111	3	other	other	ADJ
cet-13155	111	4	hand	hand	NOUN
cet-13155	111	5	,	,	PUNCT
cet-13155	111	6	besides	besides	SCONJ
cet-13155	111	7	the	the	DET
cet-13155	111	8	limited	limited	ADJ
cet-13155	111	9	methanol	methanol	NOUN
cet-13155	111	10	yield	yield	NOUN
cet-13155	111	11	(	(	PUNCT
cet-13155	111	12	5	5	NUM
cet-13155	111	13	%	%	NOUN
cet-13155	111	14	)	)	PUNCT
cet-13155	111	15	obtained	obtain	VERB
cet-13155	111	16	with	with	ADP
cet-13155	111	17	in2o3	in2o3	PROPN
cet-13155	111	18	-	-	PUNCT
cet-13155	111	19	zro2	zro2	PROPN
cet-13155	111	20	at	at	ADP
cet-13155	111	21	low	low	ADJ
cet-13155	111	22	temperature	temperature	NOUN
cet-13155	111	23	,	,	PUNCT
cet-13155	111	24	at	at	ADP
cet-13155	111	25	which	which	PRON
cet-13155	111	26	hydrogenation	hydrogenation	NOUN
cet-13155	111	27	reactions	reaction	NOUN
cet-13155	111	28	are	be	AUX
cet-13155	111	29	favored	favor	VERB
cet-13155	111	30	,	,	PUNCT
cet-13155	111	31	operating	operate	VERB
cet-13155	111	32	in	in	ADP
cet-13155	111	33	tandem	tandem	NOUN
cet-13155	111	34	with	with	ADP
cet-13155	111	35	a	a	DET
cet-13155	111	36	zeolite	zeolite	NOUN
cet-13155	111	37	favorably	favorably	ADV
cet-13155	111	38	displaced	displace	VERB
cet-13155	111	39	the	the	DET
cet-13155	111	40	thermodynamic	thermodynamic	ADJ
cet-13155	111	41	equilibrium	equilibrium	NOUN
cet-13155	111	42	of	of	ADP
cet-13155	111	43	methanol	methanol	NOUN
cet-13155	111	44	formation	formation	NOUN
cet-13155	111	45	and	and	CCONJ
cet-13155	111	46	in2o3	in2o3	PROPN
cet-13155	111	47	-	-	ADJ
cet-13155	111	48	zro2	zro2	PROPN
cet-13155	111	49	/	/	SYM
cet-13155	111	50	hzsm5	hzsm5	PROPN
cet-13155	111	51	proved	prove	VERB
cet-13155	111	52	to	to	PART
cet-13155	111	53	be	be	AUX
cet-13155	111	54	an	an	DET
cet-13155	111	55	excellent	excellent	ADJ
cet-13155	111	56	catalyst	catalyst	NOUN
cet-13155	111	57	for	for	ADP
cet-13155	111	58	fuel	fuel	NOUN
cet-13155	111	59	-	-	PUNCT
cet-13155	111	60	range	range	NOUN
cet-13155	111	61	hydrocarbons	hydrocarbon	NOUN
cet-13155	111	62	production	production	NOUN
cet-13155	111	63	.	.	PUNCT
cet-13155	112	1	the	the	DET
cet-13155	112	2	c5	c5	PROPN
cet-13155	112	3	+	+	CCONJ
cet-13155	112	4	yield	yield	NOUN
cet-13155	112	5	at	at	ADP
cet-13155	112	6	high	high	ADJ
cet-13155	112	7	temperature	temperature	NOUN
cet-13155	112	8	(	(	PUNCT
cet-13155	112	9	420	420	NUM
cet-13155	112	10	ºc	ºc	NOUN
cet-13155	112	11	)	)	PUNCT
cet-13155	112	12	reached	reach	VERB
cet-13155	112	13	almost	almost	ADV
cet-13155	112	14	20	20	NUM
cet-13155	112	15	%	%	NOUN
cet-13155	112	16	,	,	PUNCT
cet-13155	112	17	and	and	CCONJ
cet-13155	112	18	the	the	DET
cet-13155	112	19	conversion	conversion	NOUN
cet-13155	112	20	was	be	AUX
cet-13155	112	21	boosted	boost	VERB
cet-13155	112	22	from	from	ADP
cet-13155	112	23	1.8	1.8	NUM
cet-13155	112	24	%	%	NOUN
cet-13155	112	25	(	(	PUNCT
cet-13155	112	26	with	with	ADP
cet-13155	112	27	just	just	ADV
cet-13155	112	28	in2o3	in2o3	PROPN
cet-13155	112	29	-	-	PUNCT
cet-13155	112	30	zro2	zro2	ADJ
cet-13155	112	31	metallic	metallic	ADJ
cet-13155	112	32	catalyst	catalyst	NOUN
cet-13155	112	33	)	)	PUNCT
cet-13155	112	34	to	to	ADP
cet-13155	112	35	23	23	NUM
cet-13155	112	36	%	%	NOUN
cet-13155	112	37	in	in	ADP
cet-13155	112	38	the	the	DET
cet-13155	112	39	integrated	integrate	VERB
cet-13155	112	40	process	process	NOUN
cet-13155	112	41	(	(	PUNCT
cet-13155	112	42	with	with	ADP
cet-13155	112	43	in2o3	in2o3	PROPN
cet-13155	112	44	-	-	PUNCT
cet-13155	112	45	zro2	zro2	ADJ
cet-13155	112	46	/	/	SYM
cet-13155	112	47	hzsm-5	hzsm-5	NOUN
cet-13155	112	48	tandem	tandem	NOUN
cet-13155	112	49	catalyst	catalyst	NOUN
cet-13155	112	50	)	)	PUNCT
cet-13155	112	51	.	.	PUNCT
cet-13155	113	1	in	in	ADP
cet-13155	113	2	addition	addition	NOUN
cet-13155	113	3	,	,	PUNCT
cet-13155	113	4	the	the	DET
cet-13155	113	5	obtained	obtain	VERB
cet-13155	113	6	hydrocarbon	hydrocarbon	NOUN
cet-13155	113	7	stream	stream	NOUN
cet-13155	113	8	was	be	AUX
cet-13155	113	9	rich	rich	ADJ
cet-13155	113	10	in	in	ADP
cet-13155	113	11	isoparaffinic	isoparaffinic	ADJ
cet-13155	113	12	compounds	compound	NOUN
cet-13155	113	13	,	,	PUNCT
cet-13155	113	14	and	and	CCONJ
cet-13155	113	15	contained	contain	VERB
cet-13155	113	16	low	low	ADJ
cet-13155	113	17	aromatic	aromatic	ADJ
cet-13155	113	18	and	and	CCONJ
cet-13155	113	19	olefin	olefin	NOUN
cet-13155	113	20	content	content	NOUN
cet-13155	113	21	,	,	PUNCT
cet-13155	113	22	resulting	result	VERB
cet-13155	113	23	in	in	ADP
cet-13155	113	24	an	an	DET
cet-13155	113	25	adequate	adequate	ADJ
cet-13155	113	26	product	product	NOUN
cet-13155	113	27	for	for	ADP
cet-13155	113	28	its	its	PRON
cet-13155	113	29	incorporation	incorporation	NOUN
cet-13155	113	30	into	into	ADP
cet-13155	113	31	the	the	DET
cet-13155	113	32	refinery	refinery	NOUN
cet-13155	113	33	gasoline	gasoline	NOUN
cet-13155	113	34	-	-	PUNCT
cet-13155	113	35	pool	pool	NOUN
cet-13155	113	36	.	.	PUNCT
cet-13155	114	1	acknowledgments	acknowledgment	NOUN
cet-13155	114	2	this	this	DET
cet-13155	114	3	work	work	NOUN
cet-13155	114	4	has	have	AUX
cet-13155	114	5	been	be	AUX
cet-13155	114	6	carried	carry	VERB
cet-13155	114	7	out	out	ADP
cet-13155	114	8	with	with	ADP
cet-13155	114	9	the	the	DET
cet-13155	114	10	financial	financial	ADJ
cet-13155	114	11	support	support	NOUN
cet-13155	114	12	of	of	ADP
cet-13155	114	13	the	the	DET
cet-13155	114	14	micinn	micinn	NOUN
cet-13155	114	15	of	of	ADP
cet-13155	114	16	spanish	spanish	ADJ
cet-13155	114	17	government	government	NOUN
cet-13155	114	18	(	(	PUNCT
cet-13155	114	19	pid2019108448rb-100	pid2019108448rb-100	PROPN
cet-13155	114	20	)	)	PUNCT
cet-13155	114	21	;	;	PUNCT
cet-13155	114	22	the	the	DET
cet-13155	114	23	basque	basque	ADJ
cet-13155	114	24	government	government	NOUN
cet-13155	114	25	(	(	PUNCT
cet-13155	114	26	it1645	it1645	PROPN
cet-13155	114	27	-	-	PUNCT
cet-13155	114	28	22	22	NUM
cet-13155	114	29	)	)	PUNCT
cet-13155	114	30	,	,	PUNCT
cet-13155	114	31	the	the	DET
cet-13155	114	32	european	european	PROPN
cet-13155	114	33	regional	regional	PROPN
cet-13155	114	34	development	development	NOUN
cet-13155	114	35	funds	fund	NOUN
cet-13155	114	36	(	(	PUNCT
cet-13155	114	37	erdf	erdf	PROPN
cet-13155	114	38	)	)	PUNCT
cet-13155	114	39	.	.	PUNCT
cet-13155	115	1	o.	o.	PROPN
cet-13155	115	2	parra	parra	PROPN
cet-13155	115	3	is	be	AUX
cet-13155	115	4	grateful	grateful	ADJ
cet-13155	115	5	for	for	ADP
cet-13155	115	6	the	the	DET
cet-13155	115	7	financial	financial	ADJ
cet-13155	115	8	support	support	NOUN
cet-13155	115	9	of	of	ADP
cet-13155	115	10	the	the	DET
cet-13155	115	11	grant	grant	NOUN
cet-13155	115	12	of	of	ADP
cet-13155	115	13	the	the	DET
cet-13155	115	14	basque	basque	ADJ
cet-13155	115	15	government	government	NOUN
cet-13155	115	16	(	(	PUNCT
cet-13155	115	17	pre_2021_1_0014	pre_2021_1_0014	NOUN
cet-13155	115	18	)	)	PUNCT
cet-13155	115	19	.	.	PUNCT
cet-13155	116	1	references	reference	NOUN
cet-13155	116	2	ateka	ateka	PROPN
cet-13155	116	3	a.	a.	PROPN
cet-13155	116	4	,	,	PUNCT
cet-13155	116	5	sierra	sierra	PROPN
cet-13155	116	6	i.	i.	PROPN
cet-13155	116	7	,	,	PUNCT
cet-13155	116	8	ereña	ereña	ADJ
cet-13155	116	9	j.	j.	PROPN
cet-13155	116	10	,	,	PUNCT
cet-13155	116	11	bilbao	bilbao	PROPN
cet-13155	116	12	j.	j.	PROPN
cet-13155	116	13	,	,	PUNCT
cet-13155	116	14	aguayo	aguayo	PROPN
cet-13155	116	15	a.t	a.t	PROPN
cet-13155	116	16	.	.	PROPN
cet-13155	116	17	,	,	PUNCT
cet-13155	116	18	2016	2016	NUM
cet-13155	116	19	,	,	PUNCT
cet-13155	116	20	performance	performance	NOUN
cet-13155	116	21	of	of	ADP
cet-13155	116	22	cuo	cuo	PROPN
cet-13155	116	23	–	–	PUNCT
cet-13155	116	24	zno	zno	PROPN
cet-13155	116	25	–	–	PUNCT
cet-13155	116	26	zro2	zro2	PROPN
cet-13155	116	27	and	and	CCONJ
cet-13155	116	28	cuo	cuo	PROPN
cet-13155	116	29	–	–	PUNCT
cet-13155	116	30	zno	zno	PROPN
cet-13155	116	31	–	–	PUNCT
cet-13155	116	32	mno	mno	PROPN
cet-13155	116	33	as	as	ADP
cet-13155	116	34	metallic	metallic	ADJ
cet-13155	116	35	functions	function	NOUN
cet-13155	116	36	and	and	CCONJ
cet-13155	116	37	sapo-18	sapo-18	PROPN
cet-13155	116	38	as	as	ADP
cet-13155	116	39	acid	acid	NOUN
cet-13155	116	40	function	function	NOUN
cet-13155	116	41	of	of	ADP
cet-13155	116	42	the	the	DET
cet-13155	116	43	catalyst	catalyst	NOUN
cet-13155	116	44	for	for	ADP
cet-13155	116	45	the	the	DET
cet-13155	116	46	synthesis	synthesis	NOUN
cet-13155	116	47	of	of	ADP
cet-13155	116	48	dme	dme	PROPN
cet-13155	116	49	co	co	ADJ
cet-13155	116	50	-	-	ADJ
cet-13155	116	51	feeding	feeding	ADJ
cet-13155	116	52	co2	co2	NOUN
cet-13155	116	53	.	.	PUNCT
cet-13155	117	1	fuel	fuel	NOUN
cet-13155	117	2	processing	processing	NOUN
cet-13155	117	3	technology	technology	NOUN
cet-13155	117	4	,	,	PUNCT
cet-13155	117	5	152	152	NUM
cet-13155	117	6	,	,	PUNCT
cet-13155	117	7	34	34	NUM
cet-13155	117	8	-	-	SYM
cet-13155	117	9	45	45	NUM
cet-13155	117	10	.	.	PUNCT
cet-13155	118	1	ateka	ateka	PROPN
cet-13155	118	2	a.	a.	PROPN
cet-13155	118	3	,	,	PUNCT
cet-13155	118	4	rodriguez	rodriguez	NOUN
cet-13155	118	5	-	-	PUNCT
cet-13155	118	6	vega	vega	PROPN
cet-13155	118	7	p.	p.	PROPN
cet-13155	118	8	,	,	PUNCT
cet-13155	118	9	ereña	ereña	ADJ
cet-13155	118	10	j.	j.	PROPN
cet-13155	118	11	,	,	PUNCT
cet-13155	118	12	aguayo	aguayo	PROPN
cet-13155	118	13	a.t	a.t	PROPN
cet-13155	118	14	.	.	PROPN
cet-13155	118	15	,	,	PUNCT
cet-13155	118	16	bilbao	bilbao	PROPN
cet-13155	118	17	j.	j.	PROPN
cet-13155	118	18	,	,	PUNCT
cet-13155	118	19	2022	2022	NUM
cet-13155	118	20	,	,	PUNCT
cet-13155	118	21	a	a	DET
cet-13155	118	22	review	review	NOUN
cet-13155	118	23	on	on	ADP
cet-13155	118	24	the	the	DET
cet-13155	118	25	valorization	valorization	NOUN
cet-13155	118	26	of	of	ADP
cet-13155	118	27	co2	co2	NOUN
cet-13155	118	28	.	.	PUNCT
cet-13155	119	1	focusing	focus	VERB
cet-13155	119	2	on	on	ADP
cet-13155	119	3	the	the	DET
cet-13155	119	4	thermodynamics	thermodynamic	NOUN
cet-13155	119	5	and	and	CCONJ
cet-13155	119	6	catalyst	catalyst	NOUN
cet-13155	119	7	design	design	NOUN
cet-13155	119	8	studies	study	NOUN
cet-13155	119	9	of	of	ADP
cet-13155	119	10	the	the	DET
cet-13155	119	11	direct	direct	ADJ
cet-13155	119	12	synthesis	synthesis	NOUN
cet-13155	119	13	of	of	ADP
cet-13155	119	14	dimethyl	dimethyl	NOUN
cet-13155	119	15	ether	ether	NOUN
cet-13155	119	16	,	,	PUNCT
cet-13155	119	17	fuel	fuel	NOUN
cet-13155	119	18	processing	processing	NOUN
cet-13155	119	19	technology	technology	NOUN
cet-13155	119	20	,	,	PUNCT
cet-13155	119	21	233	233	NUM
cet-13155	119	22	,	,	PUNCT
cet-13155	119	23	107310	107310	NUM
cet-13155	119	24	.	.	PUNCT
cet-13155	120	1	grabow	grabow	PROPN
cet-13155	120	2	l.c	l.c	PROPN
cet-13155	120	3	.	.	PROPN
cet-13155	120	4	,	,	PUNCT
cet-13155	120	5	mavrikakis	mavrikakis	PROPN
cet-13155	120	6	m.	m.	NOUN
cet-13155	120	7	,	,	PUNCT
cet-13155	120	8	2011	2011	NUM
cet-13155	120	9	,	,	PUNCT
cet-13155	120	10	mechanism	mechanism	NOUN
cet-13155	120	11	of	of	ADP
cet-13155	120	12	methanol	methanol	NOUN
cet-13155	120	13	synthesis	synthesis	NOUN
cet-13155	120	14	on	on	ADP
cet-13155	120	15	cu	cu	PROPN
cet-13155	120	16	through	through	ADP
cet-13155	120	17	co2	co2	NOUN
cet-13155	120	18	and	and	CCONJ
cet-13155	120	19	co	co	NOUN
cet-13155	120	20	hydrogenation	hydrogenation	NOUN
cet-13155	120	21	,	,	PUNCT
cet-13155	120	22	acs	acs	PROPN
cet-13155	120	23	catalysis	catalysis	NOUN
cet-13155	120	24	,	,	PUNCT
cet-13155	120	25	1	1	NUM
cet-13155	120	26	,	,	PUNCT
cet-13155	120	27	365	365	NUM
cet-13155	120	28	-	-	SYM
cet-13155	120	29	384	384	NUM
cet-13155	120	30	.	.	PUNCT
cet-13155	121	1	kim	kim	PROPN
cet-13155	121	2	h.d	h.d	PROPN
cet-13155	121	3	.	.	PROPN
cet-13155	121	4	,	,	PUNCT
cet-13155	121	5	song	song	PROPN
cet-13155	121	6	h.	h.	PROPN
cet-13155	121	7	,	,	PUNCT
cet-13155	121	8	fazeli	fazeli	PROPN
cet-13155	121	9	a.	a.	PROPN
cet-13155	121	10	,	,	PUNCT
cet-13155	121	11	eslami	eslami	VERB
cet-13155	121	12	a.a	a.a	PROPN
cet-13155	121	13	.	.	PROPN
cet-13155	121	14	,	,	PUNCT
cet-13155	121	15	noh	noh	PROPN
cet-13155	121	16	y.s	y.s	PROPN
cet-13155	121	17	.	.	PROPN
cet-13155	121	18	,	,	PUNCT
cet-13155	121	19	saeidabad	saeidabad	PROPN
cet-13155	121	20	n.g	n.g	PROPN
cet-13155	121	21	.	.	PROPN
cet-13155	121	22	,	,	PUNCT
cet-13155	121	23	lee	lee	PROPN
cet-13155	121	24	k.	k.	PROPN
cet-13155	121	25	,	,	PUNCT
cet-13155	121	26	moon	moon	PROPN
cet-13155	121	27	d.	d.	PROPN
cet-13155	121	28	j.	j.	PROPN
cet-13155	121	29	,	,	PUNCT
cet-13155	121	30	2022	2022	NUM
cet-13155	121	31	,	,	PUNCT
cet-13155	121	32	co	co	ADJ
cet-13155	121	33	/	/	ADJ
cet-13155	121	34	co2	co2	NOUN
cet-13155	121	35	hydrogenation	hydrogenation	NOUN
cet-13155	121	36	for	for	ADP
cet-13155	121	37	the	the	DET
cet-13155	121	38	production	production	NOUN
cet-13155	121	39	of	of	ADP
cet-13155	121	40	lighter	light	ADJ
cet-13155	121	41	hydrocarbons	hydrocarbon	NOUN
cet-13155	121	42	over	over	ADP
cet-13155	121	43	sapo-34	sapo-34	PROPN
cet-13155	121	44	modified	modified	ADJ
cet-13155	121	45	hybrid	hybrid	ADJ
cet-13155	121	46	fts	fts	PROPN
cet-13155	121	47	catalysts	catalyst	NOUN
cet-13155	121	48	,	,	PUNCT
cet-13155	121	49	catalysis	catalysis	NOUN
cet-13155	121	50	today	today	NOUN
cet-13155	121	51	,	,	PUNCT
cet-13155	121	52	388	388	NUM
cet-13155	121	53	-	-	SYM
cet-13155	121	54	389	389	NUM
cet-13155	121	55	,	,	PUNCT
cet-13155	121	56	410	410	NUM
cet-13155	121	57	-	-	SYM
cet-13155	121	58	416	416	NUM
cet-13155	121	59	.	.	PUNCT
cet-13155	122	1	portillo	portillo	PROPN
cet-13155	122	2	a.	a.	PROPN
cet-13155	122	3	,	,	PUNCT
cet-13155	122	4	ateka	ateka	PROPN
cet-13155	122	5	a.	a.	PROPN
cet-13155	122	6	,	,	PUNCT
cet-13155	122	7	ereña	ereña	ADJ
cet-13155	122	8	j.	j.	PROPN
cet-13155	122	9	,	,	PUNCT
cet-13155	122	10	aguayo	aguayo	PROPN
cet-13155	122	11	a.t	a.t	PROPN
cet-13155	122	12	.	.	PROPN
cet-13155	122	13	,	,	PUNCT
cet-13155	122	14	bilbao	bilbao	PROPN
cet-13155	122	15	j.	j.	PROPN
cet-13155	122	16	,	,	PUNCT
cet-13155	122	17	2022	2022	NUM
cet-13155	122	18	,	,	PUNCT
cet-13155	122	19	conditions	condition	NOUN
cet-13155	122	20	for	for	ADP
cet-13155	122	21	the	the	DET
cet-13155	122	22	joint	joint	ADJ
cet-13155	122	23	conversion	conversion	NOUN
cet-13155	122	24	of	of	ADP
cet-13155	122	25	co2	co2	NOUN
cet-13155	122	26	and	and	CCONJ
cet-13155	122	27	syngas	syngas	NOUN
cet-13155	122	28	in	in	ADP
cet-13155	122	29	the	the	DET
cet-13155	122	30	direct	direct	ADJ
cet-13155	122	31	synthesis	synthesis	NOUN
cet-13155	122	32	of	of	ADP
cet-13155	122	33	light	light	ADJ
cet-13155	122	34	olefins	olefin	NOUN
cet-13155	122	35	using	use	VERB
cet-13155	122	36	in2o3	in2o3	PROPN
cet-13155	122	37	-	-	PUNCT
cet-13155	122	38	zro2	zro2	ADJ
cet-13155	122	39	/	/	SYM
cet-13155	122	40	sapo-34	sapo-34	PROPN
cet-13155	122	41	catalyst	catalyst	NOUN
cet-13155	122	42	,	,	PUNCT
cet-13155	122	43	industrial	industrial	PROPN
cet-13155	122	44	&	&	CCONJ
cet-13155	122	45	engineering	engineer	VERB
cet-13155	122	46	chemistry	chemistry	NOUN
cet-13155	122	47	research	research	NOUN
cet-13155	122	48	,	,	PUNCT
cet-13155	122	49	61	61	NUM
cet-13155	122	50	,	,	PUNCT
cet-13155	122	51	10365	10365	NUM
cet-13155	122	52	-	-	SYM
cet-13155	122	53	10376	10376	NUM
cet-13155	122	54	.	.	PUNCT
cet-13155	123	1	saeidi	saeidi	PROPN
cet-13155	123	2	s.	s.	PROPN
cet-13155	123	3	,	,	PUNCT
cet-13155	123	4	najari	najari	PROPN
cet-13155	123	5	s.	s.	PROPN
cet-13155	123	6	,	,	PUNCT
cet-13155	123	7	hessel	hessel	PROPN
cet-13155	123	8	v.	v.	PROPN
cet-13155	123	9	,	,	PUNCT
cet-13155	123	10	wilson	wilson	PROPN
cet-13155	123	11	k.	k.	PROPN
cet-13155	123	12	,	,	PUNCT
cet-13155	123	13	keil	keil	PROPN
cet-13155	123	14	f.j	f.j	PROPN
cet-13155	123	15	.	.	PROPN
cet-13155	123	16	,	,	PUNCT
cet-13155	123	17	concepción	concepción	NOUN
cet-13155	123	18	p.	p.	NOUN
cet-13155	123	19	,	,	PUNCT
cet-13155	123	20	suib	suib	PROPN
cet-13155	123	21	s.l	s.l	PROPN
cet-13155	123	22	.	.	PROPN
cet-13155	123	23	,	,	PUNCT
cet-13155	123	24	rodrigues	rodrigue	VERB
cet-13155	123	25	a.e	a.e	PROPN
cet-13155	123	26	.	.	PROPN
cet-13155	123	27	,	,	PUNCT
cet-13155	123	28	2021	2021	NUM
cet-13155	123	29	,	,	PUNCT
cet-13155	123	30	recent	recent	ADJ
cet-13155	123	31	advances	advance	NOUN
cet-13155	123	32	in	in	ADP
cet-13155	123	33	co2	co2	NOUN
cet-13155	123	34	hydrogenation	hydrogenation	NOUN
cet-13155	123	35	to	to	ADP
cet-13155	123	36	value	value	NOUN
cet-13155	123	37	-	-	PUNCT
cet-13155	123	38	added	add	VERB
cet-13155	123	39	products	product	NOUN
cet-13155	123	40	—	—	PUNCT
cet-13155	123	41	current	current	ADJ
cet-13155	123	42	challenges	challenge	NOUN
cet-13155	123	43	and	and	CCONJ
cet-13155	123	44	future	future	ADJ
cet-13155	123	45	directions	direction	NOUN
cet-13155	123	46	,	,	PUNCT
cet-13155	123	47	progress	progress	NOUN
cet-13155	123	48	in	in	ADP
cet-13155	123	49	energy	energy	NOUN
cet-13155	123	50	and	and	CCONJ
cet-13155	123	51	combustion	combustion	NOUN
cet-13155	123	52	science	science	NOUN
cet-13155	123	53	,	,	PUNCT
cet-13155	123	54	85	85	NUM
cet-13155	123	55	,	,	PUNCT
cet-13155	123	56	100905	100905	NUM
cet-13155	123	57	.	.	PUNCT
cet-13155	124	1	samiee	samiee	PROPN
cet-13155	124	2	l.	l.	PROPN
cet-13155	124	3	,	,	PUNCT
cet-13155	124	4	ganszha	ganszha	PROPN
cet-13155	124	5	s.	s.	PROPN
cet-13155	124	6	,	,	PUNCT
cet-13155	124	7	2019	2019	NUM
cet-13155	124	8	,	,	PUNCT
cet-13155	124	9	power	power	NOUN
cet-13155	124	10	to	to	PART
cet-13155	124	11	methanol	methanol	NOUN
cet-13155	124	12	technologies	technology	NOUN
cet-13155	124	13	via	via	ADP
cet-13155	124	14	co2	co2	NOUN
cet-13155	124	15	recovery	recovery	NOUN
cet-13155	124	16	:	:	PUNCT
cet-13155	124	17	co2	co2	NOUN
cet-13155	124	18	hydrogenation	hydrogenation	NOUN
cet-13155	124	19	and	and	CCONJ
cet-13155	124	20	electrocatalytic	electrocatalytic	ADJ
cet-13155	124	21	routes	route	NOUN
cet-13155	124	22	.	.	PUNCT
cet-13155	125	1	reviews	review	NOUN
cet-13155	125	2	in	in	ADP
cet-13155	125	3	chemical	chemical	ADJ
cet-13155	125	4	engineering	engineering	NOUN
cet-13155	125	5	,	,	PUNCT
cet-13155	125	6	37	37	NUM
cet-13155	125	7	,	,	PUNCT
cet-13155	125	8	619	619	NUM
cet-13155	125	9	-	-	SYM
cet-13155	125	10	641	641	NUM
cet-13155	125	11	.	.	PUNCT
cet-13155	125	12	sánchez	sánchez	NOUN
cet-13155	125	13	-	-	PUNCT
cet-13155	125	14	contador	contador	NOUN
cet-13155	125	15	m.	m.	NOUN
cet-13155	125	16	,	,	PUNCT
cet-13155	125	17	ateka	ateka	PROPN
cet-13155	125	18	a.	a.	PROPN
cet-13155	125	19	,	,	PUNCT
cet-13155	125	20	rodriguez	rodriguez	NOUN
cet-13155	125	21	-	-	PUNCT
cet-13155	125	22	vega	vega	PROPN
cet-13155	125	23	p.	p.	PROPN
cet-13155	125	24	,	,	PUNCT
cet-13155	125	25	bilbao	bilbao	PROPN
cet-13155	125	26	j.	j.	PROPN
cet-13155	125	27	,	,	PUNCT
cet-13155	125	28	aguayo	aguayo	PROPN
cet-13155	125	29	a.t	a.t	PROPN
cet-13155	125	30	.	.	PROPN
cet-13155	125	31	,	,	PUNCT
cet-13155	125	32	2018	2018	NUM
cet-13155	125	33	,	,	PUNCT
cet-13155	125	34	optimization	optimization	NOUN
cet-13155	125	35	of	of	ADP
cet-13155	125	36	the	the	DET
cet-13155	125	37	zr	zr	PROPN
cet-13155	125	38	content	content	NOUN
cet-13155	125	39	in	in	ADP
cet-13155	125	40	the	the	DET
cet-13155	125	41	cuo	cuo	PROPN
cet-13155	125	42	-	-	PUNCT
cet-13155	125	43	zno	zno	NOUN
cet-13155	125	44	-	-	ADJ
cet-13155	125	45	zro2	zro2	ADJ
cet-13155	125	46	/	/	SYM
cet-13155	125	47	sapo-11	sapo-11	ADJ
cet-13155	125	48	catalyst	catalyst	NOUN
cet-13155	125	49	for	for	ADP
cet-13155	125	50	the	the	DET
cet-13155	125	51	selective	selective	ADJ
cet-13155	125	52	hydrogenation	hydrogenation	NOUN
cet-13155	125	53	of	of	ADP
cet-13155	125	54	co+co2	co+co2	ADJ
cet-13155	125	55	mixtures	mixture	NOUN
cet-13155	125	56	in	in	ADP
cet-13155	125	57	the	the	DET
cet-13155	125	58	direct	direct	ADJ
cet-13155	125	59	synthesis	synthesis	NOUN
cet-13155	125	60	of	of	ADP
cet-13155	125	61	dimethyl	dimethyl	NOUN
cet-13155	125	62	ether	ether	NOUN
cet-13155	125	63	,	,	PUNCT
cet-13155	125	64	industrial	industrial	PROPN
cet-13155	125	65	&	&	CCONJ
cet-13155	125	66	engineering	engineer	VERB
cet-13155	125	67	chemistry	chemistry	NOUN
cet-13155	125	68	research	research	NOUN
cet-13155	125	69	,	,	PUNCT
cet-13155	125	70	57	57	NUM
cet-13155	125	71	,	,	PUNCT
cet-13155	125	72	1169	1169	NUM
cet-13155	125	73	-	-	SYM
cet-13155	125	74	1178	1178	NUM
cet-13155	125	75	.	.	PUNCT
cet-13155	126	1	zhang	zhang	PROPN
cet-13155	126	2	s.	s.	PROPN
cet-13155	126	3	,	,	PUNCT
cet-13155	126	4	wu	wu	PROPN
cet-13155	126	5	z.	z.	PROPN
cet-13155	126	6	,	,	PUNCT
cet-13155	126	7	liu	liu	PROPN
cet-13155	126	8	x.	x.	PROPN
cet-13155	126	9	,	,	PUNCT
cet-13155	126	10	hua	hua	PROPN
cet-13155	126	11	k.	k.	PROPN
cet-13155	126	12	,	,	PUNCT
cet-13155	126	13	shao	shao	PROPN
cet-13155	126	14	z.	z.	PROPN
cet-13155	126	15	,	,	PUNCT
cet-13155	126	16	wei	wei	PROPN
cet-13155	126	17	b.	b.	PROPN
cet-13155	126	18	,	,	PUNCT
cet-13155	126	19	huang	huang	PROPN
cet-13155	126	20	c.	c.	PROPN
cet-13155	126	21	,	,	PUNCT
cet-13155	126	22	wang	wang	PROPN
cet-13155	126	23	h.	h.	PROPN
cet-13155	126	24	,	,	PUNCT
cet-13155	126	25	sun	sun	PROPN
cet-13155	126	26	y.	y.	PROPN
cet-13155	126	27	,	,	PUNCT
cet-13155	126	28	2021	2021	NUM
cet-13155	126	29	,	,	PUNCT
cet-13155	126	30	a	a	DET
cet-13155	126	31	short	short	ADJ
cet-13155	126	32	review	review	NOUN
cet-13155	126	33	of	of	ADP
cet-13155	126	34	recent	recent	ADJ
cet-13155	126	35	advances	advance	NOUN
cet-13155	126	36	in	in	ADP
cet-13155	126	37	direct	direct	ADJ
cet-13155	126	38	co2	co2	NOUN
cet-13155	126	39	hydrogenation	hydrogenation	NOUN
cet-13155	126	40	to	to	ADP
cet-13155	126	41	alcohols	alcohol	NOUN
cet-13155	126	42	,	,	PUNCT
cet-13155	126	43	topics	topic	NOUN
cet-13155	126	44	in	in	ADP
cet-13155	126	45	catalysis	catalysis	NOUN
cet-13155	126	46	,	,	PUNCT
cet-13155	126	47	64	64	NUM
cet-13155	126	48	,	,	PUNCT
cet-13155	126	49	371	371	NUM
cet-13155	126	50	-	-	SYM
cet-13155	126	51	394	394	NUM
cet-13155	126	52	.	.	PUNCT
cet-13155	127	1	462	462	NUM
cet-13155	127	2	14parra.pdf	14parra.pdf	NUM
cet-13155	127	3	in2o3	in2o3	PROPN
cet-13155	127	4	-	-	PUNCT
cet-13155	127	5	zro2	zro2	PROPN
cet-13155	127	6	as	as	ADP
cet-13155	127	7	alternative	alternative	NOUN
cet-13155	127	8	to	to	ADP
cet-13155	127	9	cu	cu	NOUN
cet-13155	127	10	-	-	PUNCT
cet-13155	127	11	based	base	VERB
cet-13155	127	12	catalysts	catalyst	NOUN
cet-13155	127	13	for	for	ADP
cet-13155	127	14	methanol	methanol	NOUN
cet-13155	127	15	production	production	NOUN
cet-13155	127	16	step	step	NOUN
cet-13155	127	17	in	in	ADP
cet-13155	127	18	the	the	DET
cet-13155	127	19	co2	co2	NOUN
cet-13155	127	20	to	to	ADP
cet-13155	127	21	hydrocarbon	hydrocarbon	NOUN
cet-13155	127	22	process	process	NOUN