id	sid	tid	token	lemma	pos
cet-14412	1	1	doi	doi	NOUN
cet-14412	1	2	:	:	PUNCT
cet-14412	1	3	10.3303	10.3303	NUM
cet-14412	1	4	/	/	SYM
cet-14412	1	5	cet24108002	cet24108002	NOUN
cet-14412	1	6	paper	paper	NOUN
cet-14412	1	7	received	receive	VERB
cet-14412	1	8	:	:	PUNCT
cet-14412	1	9	19	19	NUM
cet-14412	1	10	august	august	PROPN
cet-14412	1	11	2023	2023	NUM
cet-14412	1	12	;	;	PUNCT
cet-14412	1	13	revised	revise	VERB
cet-14412	1	14	:	:	PUNCT
cet-14412	1	15	10	10	NUM
cet-14412	1	16	november	november	PROPN
cet-14412	1	17	2023	2023	NUM
cet-14412	1	18	;	;	PUNCT
cet-14412	1	19	accepted	accept	VERB
cet-14412	1	20	:	:	PUNCT
cet-14412	1	21	19	19	NUM
cet-14412	1	22	january	january	NOUN
cet-14412	1	23	2024	2024	NUM
cet-14412	1	24	please	please	INTJ
cet-14412	1	25	cite	cite	VERB
cet-14412	1	26	this	this	DET
cet-14412	1	27	article	article	NOUN
cet-14412	1	28	as	as	ADP
cet-14412	1	29	:	:	PUNCT
cet-14412	1	30	fournier	fournier	PROPN
cet-14412	1	31	v.	v.	PROPN
cet-14412	1	32	,	,	PUNCT
cet-14412	1	33	docoslis	docoslis	PROPN
cet-14412	1	34	a.	a.	PROPN
cet-14412	1	35	,	,	PUNCT
cet-14412	1	36	2024	2024	NUM
cet-14412	1	37	,	,	PUNCT
cet-14412	1	38	monitoring	monitor	VERB
cet-14412	1	39	adsorption	adsorption	NOUN
cet-14412	1	40	kinetics	kinetic	NOUN
cet-14412	1	41	with	with	ADP
cet-14412	1	42	surface	surface	NOUN
cet-14412	1	43	-	-	PUNCT
cet-14412	1	44	enhanced	enhance	VERB
cet-14412	1	45	raman	raman	NOUN
cet-14412	1	46	scattering	scattering	NOUN
cet-14412	1	47	in	in	ADP
cet-14412	1	48	a	a	DET
cet-14412	1	49	microfluidic	microfluidic	ADJ
cet-14412	1	50	environment	environment	NOUN
cet-14412	1	51	,	,	PUNCT
cet-14412	1	52	chemical	chemical	NOUN
cet-14412	1	53	engineering	engineering	NOUN
cet-14412	1	54	transactions	transaction	NOUN
cet-14412	1	55	,	,	PUNCT
cet-14412	1	56	108	108	NUM
cet-14412	1	57	,	,	PUNCT
cet-14412	1	58	7	7	NUM
cet-14412	1	59	-	-	SYM
cet-14412	1	60	12	12	NUM
cet-14412	1	61	doi:10.3303	doi:10.3303	NOUN
cet-14412	1	62	/	/	SYM
cet-14412	1	63	cet24108002	cet24108002	NOUN
cet-14412	1	64	chemical	chemical	NOUN
cet-14412	1	65	engineering	engineering	NOUN
cet-14412	1	66	transactions	transaction	NOUN
cet-14412	1	67	vol	vol	NOUN
cet-14412	1	68	.	.	PROPN
cet-14412	1	69	108	108	NUM
cet-14412	1	70	,	,	PUNCT
cet-14412	1	71	2024	2024	NUM
cet-14412	1	72	a	a	DET
cet-14412	1	73	publication	publication	NOUN
cet-14412	1	74	of	of	ADP
cet-14412	1	75	the	the	DET
cet-14412	1	76	italian	italian	ADJ
cet-14412	1	77	association	association	NOUN
cet-14412	1	78	of	of	ADP
cet-14412	1	79	chemical	chemical	PROPN
cet-14412	1	80	engineering	engineering	NOUN
cet-14412	1	81	online	online	ADV
cet-14412	1	82	at	at	ADP
cet-14412	1	83	www.cetjournal.it	www.cetjournal.it	PROPN
cet-14412	1	84	guest	guest	NOUN
cet-14412	1	85	editors	editor	NOUN
cet-14412	1	86	:	:	PUNCT
cet-14412	1	87	carlo	carlo	PROPN
cet-14412	1	88	pirola	pirola	PROPN
cet-14412	1	89	,	,	PUNCT
cet-14412	1	90	antonio	antonio	PROPN
cet-14412	1	91	espuña	espuña	PROPN
cet-14412	1	92	copyright	copyright	NOUN
cet-14412	1	93	©	©	PROPN
cet-14412	1	94	2024	2024	NUM
cet-14412	1	95	,	,	PUNCT
cet-14412	1	96	aidic	aidic	ADJ
cet-14412	1	97	servizi	servizi	PROPN
cet-14412	1	98	s.r.l	s.r.l	NOUN
cet-14412	1	99	.	.	PUNCT
cet-14412	2	1	isbn	isbn	PROPN
cet-14412	2	2	979	979	NUM
cet-14412	2	3	-	-	SYM
cet-14412	2	4	12	12	NUM
cet-14412	2	5	-	-	PUNCT
cet-14412	2	6	81206	81206	NUM
cet-14412	2	7	-	-	SYM
cet-14412	2	8	08	08	NUM
cet-14412	2	9	-	-	SYM
cet-14412	2	10	3	3	NUM
cet-14412	3	1	;	;	PUNCT
cet-14412	3	2	issn	issn	PROPN
cet-14412	3	3	2283	2283	NUM
cet-14412	3	4	-	-	SYM
cet-14412	3	5	9216	9216	NUM
cet-14412	3	6	monitoring	monitoring	NOUN
cet-14412	3	7	adsorption	adsorption	NOUN
cet-14412	3	8	kinetics	kinetic	NOUN
cet-14412	3	9	with	with	ADP
cet-14412	3	10	surface	surface	NOUN
cet-14412	3	11	-	-	PUNCT
cet-14412	3	12	enhanced	enhance	VERB
cet-14412	3	13	raman	raman	NOUN
cet-14412	3	14	scattering	scattering	NOUN
cet-14412	3	15	in	in	ADP
cet-14412	3	16	a	a	DET
cet-14412	3	17	microfluidic	microfluidic	ADJ
cet-14412	3	18	environment	environment	NOUN
cet-14412	3	19	victoria	victoria	PROPN
cet-14412	3	20	fournier	fournier	PROPN
cet-14412	3	21	,	,	PUNCT
cet-14412	3	22	aristides	aristide	VERB
cet-14412	3	23	docoslis	docoslis	PROPN
cet-14412	3	24	*	*	PROPN
cet-14412	3	25	department	department	PROPN
cet-14412	3	26	of	of	ADP
cet-14412	3	27	chemical	chemical	PROPN
cet-14412	3	28	engineering	engineering	PROPN
cet-14412	3	29	,	,	PUNCT
cet-14412	3	30	queen	queen	PROPN
cet-14412	3	31	’s	’s	PART
cet-14412	3	32	university	university	PROPN
cet-14412	3	33	,	,	PUNCT
cet-14412	3	34	kingston	kingston	PROPN
cet-14412	3	35	,	,	PUNCT
cet-14412	3	36	on	on	ADP
cet-14412	3	37	k7l	k7l	PROPN
cet-14412	3	38	3n6	3n6	NUM
cet-14412	3	39	canada	canada	PROPN
cet-14412	3	40	docoslis@queensu.ca	docoslis@queensu.ca	PROPN
cet-14412	4	1	this	this	DET
cet-14412	4	2	article	article	NOUN
cet-14412	4	3	provides	provide	VERB
cet-14412	4	4	a	a	DET
cet-14412	4	5	proof	proof	NOUN
cet-14412	4	6	of	of	ADP
cet-14412	4	7	concept	concept	NOUN
cet-14412	4	8	on	on	ADP
cet-14412	4	9	how	how	SCONJ
cet-14412	4	10	surface	surface	NOUN
cet-14412	4	11	-	-	PUNCT
cet-14412	4	12	enhanced	enhance	VERB
cet-14412	4	13	raman	raman	NOUN
cet-14412	4	14	scattering	scattering	NOUN
cet-14412	4	15	(	(	PUNCT
cet-14412	4	16	sers	ser	NOUN
cet-14412	4	17	)	)	PUNCT
cet-14412	4	18	can	can	AUX
cet-14412	4	19	be	be	AUX
cet-14412	4	20	combined	combine	VERB
cet-14412	4	21	with	with	ADP
cet-14412	4	22	microfluidics	microfluidic	NOUN
cet-14412	4	23	towards	towards	ADP
cet-14412	4	24	the	the	DET
cet-14412	4	25	development	development	NOUN
cet-14412	4	26	of	of	ADP
cet-14412	4	27	an	an	PRON
cet-14412	4	28	in	in	ADP
cet-14412	4	29	situ	situ	ADJ
cet-14412	4	30	chemical	chemical	NOUN
cet-14412	4	31	detection	detection	NOUN
cet-14412	4	32	method	method	NOUN
cet-14412	4	33	.	.	PUNCT
cet-14412	5	1	a	a	DET
cet-14412	5	2	microfluidic	microfluidic	ADJ
cet-14412	5	3	device	device	NOUN
cet-14412	5	4	prototype	prototype	NOUN
cet-14412	5	5	was	be	AUX
cet-14412	5	6	designed	design	VERB
cet-14412	5	7	,	,	PUNCT
cet-14412	5	8	fabricated	fabricate	VERB
cet-14412	5	9	,	,	PUNCT
cet-14412	5	10	and	and	CCONJ
cet-14412	5	11	characterized	characterize	VERB
cet-14412	5	12	to	to	PART
cet-14412	5	13	demonstrate	demonstrate	VERB
cet-14412	5	14	the	the	DET
cet-14412	5	15	feasibility	feasibility	NOUN
cet-14412	5	16	of	of	ADP
cet-14412	5	17	microfluidics	microfluidic	NOUN
cet-14412	5	18	in	in	ADP
cet-14412	5	19	achieving	achieve	VERB
cet-14412	5	20	analyte	analyte	NOUN
cet-14412	5	21	transport	transport	NOUN
cet-14412	5	22	from	from	ADP
cet-14412	5	23	the	the	DET
cet-14412	5	24	sample	sample	NOUN
cet-14412	5	25	introduction	introduction	NOUN
cet-14412	5	26	site	site	NOUN
cet-14412	5	27	to	to	ADP
cet-14412	5	28	the	the	DET
cet-14412	5	29	detection	detection	NOUN
cet-14412	5	30	site	site	NOUN
cet-14412	5	31	.	.	PUNCT
cet-14412	6	1	subsequently	subsequently	ADV
cet-14412	6	2	,	,	PUNCT
cet-14412	6	3	the	the	DET
cet-14412	6	4	microfluidic	microfluidic	ADJ
cet-14412	6	5	setup	setup	NOUN
cet-14412	6	6	was	be	AUX
cet-14412	6	7	used	use	VERB
cet-14412	6	8	for	for	ADP
cet-14412	6	9	monitoring	monitor	VERB
cet-14412	6	10	the	the	DET
cet-14412	6	11	adsorption	adsorption	NOUN
cet-14412	6	12	kinetics	kinetic	NOUN
cet-14412	6	13	of	of	ADP
cet-14412	6	14	the	the	DET
cet-14412	6	15	molecule	molecule	NOUN
cet-14412	6	16	rhodamine	rhodamine	NOUN
cet-14412	6	17	6	6	NUM
cet-14412	6	18	g	g	NOUN
cet-14412	6	19	(	(	PUNCT
cet-14412	6	20	r6	r6	NOUN
cet-14412	6	21	g	g	NOUN
cet-14412	6	22	)	)	PUNCT
cet-14412	6	23	onto	onto	ADP
cet-14412	6	24	a	a	DET
cet-14412	6	25	sers	ser	NOUN
cet-14412	6	26	-	-	ADJ
cet-14412	6	27	active	active	ADJ
cet-14412	6	28	substrate	substrate	NOUN
cet-14412	6	29	;	;	PUNCT
cet-14412	6	30	an	an	DET
cet-14412	6	31	application	application	NOUN
cet-14412	6	32	,	,	PUNCT
cet-14412	6	33	for	for	ADP
cet-14412	6	34	which	which	PRON
cet-14412	6	35	only	only	ADV
cet-14412	6	36	scare	scare	VERB
cet-14412	6	37	information	information	NOUN
cet-14412	6	38	is	be	AUX
cet-14412	6	39	available	available	ADJ
cet-14412	6	40	in	in	ADP
cet-14412	6	41	the	the	DET
cet-14412	6	42	literature	literature	NOUN
cet-14412	6	43	.	.	PUNCT
cet-14412	7	1	moreover	moreover	ADV
cet-14412	7	2	,	,	PUNCT
cet-14412	7	3	this	this	DET
cet-14412	7	4	work	work	NOUN
cet-14412	7	5	demonstrates	demonstrate	VERB
cet-14412	7	6	how	how	SCONJ
cet-14412	7	7	the	the	DET
cet-14412	7	8	actual	actual	ADJ
cet-14412	7	9	concentration	concentration	NOUN
cet-14412	7	10	of	of	ADP
cet-14412	7	11	adsorbed	adsorb	VERB
cet-14412	7	12	r6	r6	PROPN
cet-14412	7	13	g	g	PROPN
cet-14412	7	14	(	(	PUNCT
cet-14412	7	15	moles	mole	NOUN
cet-14412	7	16	m-2	m-2	NOUN
cet-14412	7	17	)	)	PUNCT
cet-14412	7	18	onto	onto	ADP
cet-14412	7	19	the	the	DET
cet-14412	7	20	sers	ser	NOUN
cet-14412	7	21	substrate	substrate	NOUN
cet-14412	7	22	can	can	AUX
cet-14412	7	23	be	be	AUX
cet-14412	7	24	quantified	quantify	VERB
cet-14412	7	25	in	in	ADP
cet-14412	7	26	real	real	ADJ
cet-14412	7	27	time	time	NOUN
cet-14412	7	28	.	.	PUNCT
cet-14412	8	1	sers	ser	NOUN
cet-14412	8	2	-	-	ADJ
cet-14412	8	3	active	active	ADJ
cet-14412	8	4	substrates	substrate	NOUN
cet-14412	8	5	,	,	PUNCT
cet-14412	8	6	such	such	DET
cet-14412	8	7	the	the	DET
cet-14412	8	8	ones	one	NOUN
cet-14412	8	9	used	use	VERB
cet-14412	8	10	in	in	ADP
cet-14412	8	11	this	this	DET
cet-14412	8	12	study	study	NOUN
cet-14412	8	13	,	,	PUNCT
cet-14412	8	14	can	can	AUX
cet-14412	8	15	be	be	AUX
cet-14412	8	16	integrated	integrate	VERB
cet-14412	8	17	in	in	ADP
cet-14412	8	18	a	a	DET
cet-14412	8	19	microfluidic	microfluidic	ADJ
cet-14412	8	20	device	device	NOUN
cet-14412	8	21	for	for	ADP
cet-14412	8	22	achieving	achieve	VERB
cet-14412	8	23	reproducible	reproducible	ADJ
cet-14412	8	24	monitoring	monitoring	NOUN
cet-14412	8	25	of	of	ADP
cet-14412	8	26	the	the	DET
cet-14412	8	27	adsorption	adsorption	NOUN
cet-14412	8	28	kinetics	kinetic	NOUN
cet-14412	8	29	of	of	ADP
cet-14412	8	30	a	a	DET
cet-14412	8	31	molecule	molecule	NOUN
cet-14412	8	32	in	in	ADP
cet-14412	8	33	a	a	DET
cet-14412	8	34	liquid	liquid	ADJ
cet-14412	8	35	sample	sample	NOUN
cet-14412	8	36	,	,	PUNCT
cet-14412	8	37	or	or	CCONJ
cet-14412	8	38	for	for	ADP
cet-14412	8	39	detecting	detect	VERB
cet-14412	8	40	and	and	CCONJ
cet-14412	8	41	reporting	report	VERB
cet-14412	8	42	the	the	DET
cet-14412	8	43	concentration	concentration	NOUN
cet-14412	8	44	of	of	ADP
cet-14412	8	45	an	an	DET
cet-14412	8	46	unknown	unknown	ADJ
cet-14412	8	47	target	target	NOUN
cet-14412	8	48	molecule	molecule	NOUN
cet-14412	8	49	during	during	ADP
cet-14412	8	50	a	a	DET
cet-14412	8	51	diagnostic	diagnostic	ADJ
cet-14412	8	52	assay	assay	NOUN
cet-14412	8	53	.	.	PUNCT
cet-14412	9	1	1	1	X
cet-14412	9	2	.	.	X
cet-14412	9	3	introduction	introduction	NOUN
cet-14412	9	4	the	the	DET
cet-14412	9	5	increasing	increase	VERB
cet-14412	9	6	need	need	NOUN
cet-14412	9	7	for	for	ADP
cet-14412	9	8	point	point	NOUN
cet-14412	9	9	-	-	PUNCT
cet-14412	9	10	of	of	ADP
cet-14412	9	11	-	-	PUNCT
cet-14412	9	12	care	care	NOUN
cet-14412	9	13	(	(	PUNCT
cet-14412	9	14	poc	poc	NOUN
cet-14412	9	15	)	)	PUNCT
cet-14412	9	16	diagnostic	diagnostic	ADJ
cet-14412	9	17	devices	device	NOUN
cet-14412	9	18	creates	create	VERB
cet-14412	9	19	a	a	DET
cet-14412	9	20	strong	strong	ADJ
cet-14412	9	21	incentive	incentive	NOUN
cet-14412	9	22	to	to	PART
cet-14412	9	23	integrate	integrate	VERB
cet-14412	9	24	established	establish	VERB
cet-14412	9	25	laboratory	laboratory	NOUN
cet-14412	9	26	chemical	chemical	NOUN
cet-14412	9	27	detection	detection	NOUN
cet-14412	9	28	and	and	CCONJ
cet-14412	9	29	quantification	quantification	NOUN
cet-14412	9	30	methods	method	NOUN
cet-14412	9	31	with	with	ADP
cet-14412	9	32	microfluidic	microfluidic	ADJ
cet-14412	9	33	,	,	PUNCT
cet-14412	9	34	lab	lab	NOUN
cet-14412	9	35	-	-	PUNCT
cet-14412	9	36	on	on	ADP
cet-14412	9	37	-	-	PUNCT
cet-14412	9	38	a	a	DET
cet-14412	9	39	-	-	PUNCT
cet-14412	9	40	chip	chip	NOUN
cet-14412	9	41	(	(	PUNCT
cet-14412	9	42	loc	loc	NOUN
cet-14412	9	43	)	)	PUNCT
cet-14412	9	44	,	,	PUNCT
cet-14412	9	45	systems	system	NOUN
cet-14412	9	46	(	(	PUNCT
cet-14412	9	47	maria	maria	PROPN
cet-14412	9	48	et	et	PROPN
cet-14412	9	49	al	al	PROPN
cet-14412	9	50	.	.	PROPN
cet-14412	9	51	,	,	PUNCT
cet-14412	9	52	2017	2017	NUM
cet-14412	9	53	;	;	PUNCT
cet-14412	9	54	juncker	juncker	NOUN
cet-14412	9	55	et	et	PROPN
cet-14412	9	56	al	al	PROPN
cet-14412	9	57	.	.	PROPN
cet-14412	9	58	,	,	PUNCT
cet-14412	9	59	2002	2002	NUM
cet-14412	9	60	)	)	PUNCT
cet-14412	9	61	.	.	PUNCT
cet-14412	10	1	the	the	DET
cet-14412	10	2	incorporation	incorporation	NOUN
cet-14412	10	3	of	of	ADP
cet-14412	10	4	microfluidics	microfluidic	NOUN
cet-14412	10	5	into	into	ADP
cet-14412	10	6	chemical	chemical	ADJ
cet-14412	10	7	analysis	analysis	NOUN
cet-14412	10	8	allow	allow	VERB
cet-14412	10	9	for	for	ADP
cet-14412	10	10	greater	great	ADJ
cet-14412	10	11	control	control	NOUN
cet-14412	10	12	of	of	ADP
cet-14412	10	13	the	the	DET
cet-14412	10	14	introduction	introduction	NOUN
cet-14412	10	15	of	of	ADP
cet-14412	10	16	analyte	analyte	NOUN
cet-14412	10	17	to	to	ADP
cet-14412	10	18	the	the	DET
cet-14412	10	19	detection	detection	NOUN
cet-14412	10	20	method	method	NOUN
cet-14412	10	21	of	of	ADP
cet-14412	10	22	choice	choice	NOUN
cet-14412	10	23	.	.	PUNCT
cet-14412	11	1	surface	surface	NOUN
cet-14412	11	2	-	-	PUNCT
cet-14412	11	3	enhanced	enhance	VERB
cet-14412	11	4	raman	raman	NOUN
cet-14412	11	5	scattering	scattering	NOUN
cet-14412	11	6	(	(	PUNCT
cet-14412	11	7	sers	ser	NOUN
cet-14412	11	8	)	)	PUNCT
cet-14412	11	9	is	be	AUX
cet-14412	11	10	an	an	DET
cet-14412	11	11	advantageous	advantageous	ADJ
cet-14412	11	12	detection	detection	NOUN
cet-14412	11	13	method	method	NOUN
cet-14412	11	14	due	due	ADP
cet-14412	11	15	to	to	ADP
cet-14412	11	16	its	its	PRON
cet-14412	11	17	non	non	ADJ
cet-14412	11	18	-	-	ADJ
cet-14412	11	19	destructive	destructive	ADJ
cet-14412	11	20	,	,	PUNCT
cet-14412	11	21	rapid	rapid	ADJ
cet-14412	11	22	,	,	PUNCT
cet-14412	11	23	chemically	chemically	ADV
cet-14412	11	24	specific	specific	ADJ
cet-14412	11	25	and	and	CCONJ
cet-14412	11	26	ultrasensitive	ultrasensitive	ADJ
cet-14412	11	27	detection	detection	NOUN
cet-14412	11	28	characteristics	characteristic	NOUN
cet-14412	11	29	.	.	PUNCT
cet-14412	12	1	applications	application	NOUN
cet-14412	12	2	of	of	ADP
cet-14412	12	3	a	a	DET
cet-14412	12	4	variety	variety	NOUN
cet-14412	12	5	of	of	ADP
cet-14412	12	6	sers	ser	NOUN
cet-14412	12	7	detection	detection	NOUN
cet-14412	12	8	methods	method	NOUN
cet-14412	12	9	in	in	ADP
cet-14412	12	10	loc	loc	NOUN
cet-14412	12	11	devices	device	NOUN
cet-14412	12	12	have	have	AUX
cet-14412	12	13	been	be	AUX
cet-14412	12	14	reported	report	VERB
cet-14412	12	15	in	in	ADP
cet-14412	12	16	literature	literature	NOUN
cet-14412	12	17	(	(	PUNCT
cet-14412	12	18	white	white	PROPN
cet-14412	12	19	et	et	PROPN
cet-14412	12	20	al	al	PROPN
cet-14412	12	21	.	.	PROPN
cet-14412	12	22	,	,	PUNCT
cet-14412	12	23	2013	2013	NUM
cet-14412	12	24	;	;	PUNCT
cet-14412	12	25	kong	kong	PROPN
cet-14412	12	26	et	et	PROPN
cet-14412	12	27	al	al	PROPN
cet-14412	12	28	.	.	PROPN
cet-14412	12	29	,	,	PUNCT
cet-14412	12	30	2018	2018	NUM
cet-14412	12	31	;	;	PUNCT
cet-14412	12	32	andreou	andreou	NOUN
cet-14412	12	33	et	et	PROPN
cet-14412	12	34	al	al	PROPN
cet-14412	12	35	.	.	PROPN
cet-14412	12	36	,	,	PUNCT
cet-14412	12	37	2013	2013	NUM
cet-14412	12	38	)	)	PUNCT
cet-14412	12	39	.	.	PUNCT
cet-14412	13	1	these	these	DET
cet-14412	13	2	applications	application	NOUN
cet-14412	13	3	show	show	VERB
cet-14412	13	4	success	success	NOUN
cet-14412	13	5	at	at	ADP
cet-14412	13	6	overcoming	overcome	VERB
cet-14412	13	7	various	various	ADJ
cet-14412	13	8	limitations	limitation	NOUN
cet-14412	13	9	of	of	ADP
cet-14412	13	10	the	the	DET
cet-14412	13	11	sers	ser	NOUN
cet-14412	13	12	detection	detection	NOUN
cet-14412	13	13	method	method	NOUN
cet-14412	13	14	by	by	ADP
cet-14412	13	15	demonstrating	demonstrate	VERB
cet-14412	13	16	ease	ease	NOUN
cet-14412	13	17	of	of	ADP
cet-14412	13	18	use	use	NOUN
cet-14412	13	19	,	,	PUNCT
cet-14412	13	20	speed	speed	NOUN
cet-14412	13	21	of	of	ADP
cet-14412	13	22	measurement	measurement	NOUN
cet-14412	13	23	,	,	PUNCT
cet-14412	13	24	accuracy	accuracy	NOUN
cet-14412	13	25	and	and	CCONJ
cet-14412	13	26	reproducibility	reproducibility	NOUN
cet-14412	13	27	of	of	ADP
cet-14412	13	28	results	result	NOUN
cet-14412	13	29	.	.	PUNCT
cet-14412	14	1	however	however	ADV
cet-14412	14	2	,	,	PUNCT
cet-14412	14	3	current	current	ADJ
cet-14412	14	4	sers	ser	NOUN
cet-14412	14	5	detection	detection	NOUN
cet-14412	14	6	methods	method	NOUN
cet-14412	14	7	incorporated	incorporate	VERB
cet-14412	14	8	into	into	ADP
cet-14412	14	9	loc	loc	NOUN
cet-14412	14	10	devices	device	NOUN
cet-14412	14	11	all	all	PRON
cet-14412	14	12	share	share	VERB
cet-14412	14	13	a	a	DET
cet-14412	14	14	similar	similar	ADJ
cet-14412	14	15	disadvantage	disadvantage	NOUN
cet-14412	14	16	:	:	PUNCT
cet-14412	14	17	samples	sample	NOUN
cet-14412	14	18	must	must	AUX
cet-14412	14	19	be	be	AUX
cet-14412	14	20	mixed	mix	VERB
cet-14412	14	21	with	with	ADP
cet-14412	14	22	nanoparticles	nanoparticle	NOUN
cet-14412	14	23	before	before	ADP
cet-14412	14	24	being	be	AUX
cet-14412	14	25	loaded	load	VERB
cet-14412	14	26	into	into	ADP
cet-14412	14	27	the	the	DET
cet-14412	14	28	device	device	NOUN
cet-14412	14	29	.	.	PUNCT
cet-14412	15	1	this	this	DET
cet-14412	15	2	sample	sample	NOUN
cet-14412	15	3	preparation	preparation	NOUN
cet-14412	15	4	step	step	NOUN
cet-14412	15	5	increases	increase	VERB
cet-14412	15	6	the	the	DET
cet-14412	15	7	difficulty	difficulty	NOUN
cet-14412	15	8	of	of	ADP
cet-14412	15	9	use	use	NOUN
cet-14412	15	10	of	of	ADP
cet-14412	15	11	the	the	DET
cet-14412	15	12	device	device	NOUN
cet-14412	15	13	in	in	ADP
cet-14412	15	14	a	a	DET
cet-14412	15	15	poc	poc	NOUN
cet-14412	15	16	diagnostic	diagnostic	ADJ
cet-14412	15	17	setting	setting	NOUN
cet-14412	15	18	and	and	CCONJ
cet-14412	15	19	presents	present	VERB
cet-14412	15	20	the	the	DET
cet-14412	15	21	issue	issue	NOUN
cet-14412	15	22	of	of	ADP
cet-14412	15	23	nanoparticles	nanoparticle	NOUN
cet-14412	15	24	crashing	crash	VERB
cet-14412	15	25	out	out	ADP
cet-14412	15	26	of	of	ADP
cet-14412	15	27	solution	solution	NOUN
cet-14412	15	28	before	before	ADP
cet-14412	15	29	sample	sample	NOUN
cet-14412	15	30	loading	loading	NOUN
cet-14412	15	31	.	.	PUNCT
cet-14412	16	1	recently	recently	ADV
cet-14412	16	2	,	,	PUNCT
cet-14412	16	3	a	a	DET
cet-14412	16	4	patented	patented	ADJ
cet-14412	16	5	technique	technique	NOUN
cet-14412	16	6	that	that	PRON
cet-14412	16	7	creates	create	VERB
cet-14412	16	8	sers	ser	NOUN
cet-14412	16	9	-	-	ADJ
cet-14412	16	10	active	active	ADJ
cet-14412	16	11	substrates	substrate	NOUN
cet-14412	16	12	with	with	ADP
cet-14412	16	13	the	the	DET
cet-14412	16	14	use	use	NOUN
cet-14412	16	15	of	of	ADP
cet-14412	16	16	electric	electric	ADJ
cet-14412	16	17	field	field	NOUN
cet-14412	16	18	-	-	PUNCT
cet-14412	16	19	directed	direct	VERB
cet-14412	16	20	nanoparticle	nanoparticle	NOUN
cet-14412	16	21	assembly	assembly	NOUN
cet-14412	16	22	has	have	AUX
cet-14412	16	23	been	be	AUX
cet-14412	16	24	developed	develop	VERB
cet-14412	16	25	in	in	ADP
cet-14412	16	26	our	our	PRON
cet-14412	16	27	lab	lab	NOUN
cet-14412	16	28	(	(	PUNCT
cet-14412	16	29	bacon	bacon	NOUN
cet-14412	16	30	at	at	ADP
cet-14412	16	31	al	al	PROPN
cet-14412	16	32	.	.	PROPN
cet-14412	16	33	,	,	PUNCT
cet-14412	16	34	2022	2022	NUM
cet-14412	16	35	;	;	PUNCT
cet-14412	16	36	dies	die	VERB
cet-14412	16	37	et	et	PROPN
cet-14412	16	38	al	al	PROPN
cet-14412	16	39	.	.	PROPN
cet-14412	16	40	,	,	PUNCT
cet-14412	16	41	2017	2017	NUM
cet-14412	16	42	)	)	PUNCT
cet-14412	16	43	.	.	PUNCT
cet-14412	17	1	the	the	DET
cet-14412	17	2	produced	produce	VERB
cet-14412	17	3	sers	ser	NOUN
cet-14412	17	4	substrates	substrate	NOUN
cet-14412	17	5	have	have	AUX
cet-14412	17	6	been	be	AUX
cet-14412	17	7	shown	show	VERB
cet-14412	17	8	to	to	PART
cet-14412	17	9	amplify	amplify	VERB
cet-14412	17	10	the	the	DET
cet-14412	17	11	conventional	conventional	ADJ
cet-14412	17	12	raman	raman	NOUN
cet-14412	17	13	signal	signal	NOUN
cet-14412	17	14	by	by	ADP
cet-14412	17	15	more	more	ADJ
cet-14412	17	16	than	than	ADP
cet-14412	17	17	106	106	NUM
cet-14412	17	18	-	-	NOUN
cet-14412	17	19	fold	fold	ADJ
cet-14412	17	20	.	.	PUNCT
cet-14412	18	1	the	the	DET
cet-14412	18	2	substrates	substrate	NOUN
cet-14412	18	3	have	have	AUX
cet-14412	18	4	been	be	AUX
cet-14412	18	5	successful	successful	ADJ
cet-14412	18	6	in	in	ADP
cet-14412	18	7	the	the	DET
cet-14412	18	8	detection	detection	NOUN
cet-14412	18	9	and	and	CCONJ
cet-14412	18	10	quantification	quantification	NOUN
cet-14412	18	11	of	of	ADP
cet-14412	18	12	a	a	DET
cet-14412	18	13	variety	variety	NOUN
cet-14412	18	14	of	of	ADP
cet-14412	18	15	samples	sample	NOUN
cet-14412	18	16	,	,	PUNCT
cet-14412	18	17	including	include	VERB
cet-14412	18	18	illicit	illicit	ADJ
cet-14412	18	19	drugs	drug	NOUN
cet-14412	18	20	[	[	X
cet-14412	18	21	wilson	wilson	PROPN
cet-14412	18	22	et	et	PROPN
cet-14412	18	23	al	al	PROPN
cet-14412	18	24	.	.	PROPN
cet-14412	18	25	,	,	PUNCT
cet-14412	18	26	2021	2021	NUM
cet-14412	18	27	]	]	PUNCT
cet-14412	18	28	,	,	PUNCT
cet-14412	18	29	environmental	environmental	ADJ
cet-14412	18	30	pollutants	pollutant	NOUN
cet-14412	19	1	[	[	X
cet-14412	19	2	raveendran	raveendran	VERB
cet-14412	19	3	et	et	PROPN
cet-14412	19	4	al	al	PROPN
cet-14412	19	5	.	.	PROPN
cet-14412	19	6	,	,	PUNCT
cet-14412	19	7	2021	2021	NUM
cet-14412	19	8	]	]	PUNCT
cet-14412	19	9	,	,	PUNCT
cet-14412	19	10	and	and	CCONJ
cet-14412	19	11	food	food	NOUN
cet-14412	19	12	adulterants	adulterant	NOUN
cet-14412	19	13	(	(	PUNCT
cet-14412	19	14	dies	die	VERB
cet-14412	19	15	et	et	PROPN
cet-14412	19	16	al	al	PROPN
cet-14412	19	17	.	.	PROPN
cet-14412	19	18	,	,	PUNCT
cet-14412	19	19	2018	2018	NUM
cet-14412	19	20	)	)	PUNCT
cet-14412	19	21	.	.	PUNCT
cet-14412	20	1	however	however	ADV
cet-14412	20	2	,	,	PUNCT
cet-14412	20	3	all	all	DET
cet-14412	20	4	the	the	DET
cet-14412	20	5	tests	test	NOUN
cet-14412	20	6	were	be	AUX
cet-14412	20	7	performed	perform	VERB
cet-14412	20	8	by	by	ADP
cet-14412	20	9	following	follow	VERB
cet-14412	20	10	the	the	DET
cet-14412	20	11	standard	standard	ADJ
cet-14412	20	12	method	method	NOUN
cet-14412	20	13	of	of	ADP
cet-14412	20	14	“	"	PUNCT
cet-14412	20	15	drop	drop	NOUN
cet-14412	20	16	-	-	PUNCT
cet-14412	20	17	casting	casting	NOUN
cet-14412	20	18	”	"	PUNCT
cet-14412	20	19	,	,	PUNCT
cet-14412	20	20	i.e.	i.e.	X
cet-14412	20	21	,	,	PUNCT
cet-14412	20	22	placing	place	VERB
cet-14412	20	23	a	a	DET
cet-14412	20	24	droplet	droplet	NOUN
cet-14412	20	25	of	of	ADP
cet-14412	20	26	the	the	DET
cet-14412	20	27	liquid	liquid	ADJ
cet-14412	20	28	sample	sample	NOUN
cet-14412	20	29	on	on	ADP
cet-14412	20	30	the	the	DET
cet-14412	20	31	surface	surface	NOUN
cet-14412	20	32	of	of	ADP
cet-14412	20	33	the	the	DET
cet-14412	20	34	sensor	sensor	NOUN
cet-14412	20	35	and	and	CCONJ
cet-14412	20	36	waiting	wait	VERB
cet-14412	20	37	for	for	SCONJ
cet-14412	20	38	the	the	DET
cet-14412	20	39	liquid	liquid	NOUN
cet-14412	20	40	in	in	ADP
cet-14412	20	41	the	the	DET
cet-14412	20	42	droplet	droplet	NOUN
cet-14412	20	43	to	to	PART
cet-14412	20	44	evaporate	evaporate	VERB
cet-14412	20	45	.	.	PUNCT
cet-14412	21	1	a	a	DET
cet-14412	21	2	major	major	ADJ
cet-14412	21	3	disadvantage	disadvantage	NOUN
cet-14412	21	4	of	of	ADP
cet-14412	21	5	drop	drop	NOUN
cet-14412	21	6	-	-	PUNCT
cet-14412	21	7	casting	casting	NOUN
cet-14412	21	8	is	be	AUX
cet-14412	21	9	that	that	SCONJ
cet-14412	21	10	it	it	PRON
cet-14412	21	11	results	result	VERB
cet-14412	21	12	in	in	ADP
cet-14412	21	13	an	an	DET
cet-14412	21	14	uneven	uneven	ADJ
cet-14412	21	15	target	target	NOUN
cet-14412	21	16	molecule	molecule	NOUN
cet-14412	21	17	distribution	distribution	NOUN
cet-14412	21	18	on	on	ADP
cet-14412	21	19	the	the	DET
cet-14412	21	20	surface	surface	NOUN
cet-14412	21	21	,	,	PUNCT
cet-14412	21	22	consequentially	consequentially	ADV
cet-14412	21	23	impeding	impede	VERB
cet-14412	21	24	the	the	DET
cet-14412	21	25	reproducibility	reproducibility	NOUN
cet-14412	21	26	and	and	CCONJ
cet-14412	21	27	reliability	reliability	NOUN
cet-14412	21	28	of	of	ADP
cet-14412	21	29	the	the	DET
cet-14412	21	30	detection	detection	NOUN
cet-14412	21	31	method	method	NOUN
cet-14412	21	32	.	.	PUNCT
cet-14412	22	1	the	the	DET
cet-14412	22	2	cause	cause	NOUN
cet-14412	22	3	of	of	ADP
cet-14412	22	4	uneven	uneven	ADJ
cet-14412	22	5	distribution	distribution	NOUN
cet-14412	22	6	can	can	AUX
cet-14412	22	7	be	be	AUX
cet-14412	22	8	attributed	attribute	VERB
cet-14412	22	9	to	to	ADP
cet-14412	22	10	droplet	droplet	ADJ
cet-14412	22	11	evaporation	evaporation	NOUN
cet-14412	22	12	that	that	PRON
cet-14412	22	13	results	result	VERB
cet-14412	22	14	in	in	ADP
cet-14412	22	15	the	the	DET
cet-14412	22	16	“	"	PUNCT
cet-14412	22	17	coffee	coffee	NOUN
cet-14412	22	18	-	-	PUNCT
cet-14412	22	19	ring	ring	NOUN
cet-14412	22	20	”	"	PUNCT
cet-14412	22	21	effect	effect	NOUN
cet-14412	22	22	that	that	PRON
cet-14412	22	23	concentrates	concentrate	VERB
cet-14412	22	24	analyte	analyte	NOUN
cet-14412	22	25	deposition	deposition	NOUN
cet-14412	22	26	towards	towards	ADP
cet-14412	22	27	the	the	DET
cet-14412	22	28	outer	outer	ADJ
cet-14412	22	29	circumference	circumference	NOUN
cet-14412	22	30	of	of	ADP
cet-14412	22	31	the	the	DET
cet-14412	22	32	drop	drop	NOUN
cet-14412	22	33	(	(	PUNCT
cet-14412	22	34	shur	shur	NOUN
cet-14412	22	35	et	et	PROPN
cet-14412	22	36	al	al	PROPN
cet-14412	22	37	.	.	PROPN
cet-14412	22	38	,	,	PUNCT
cet-14412	22	39	2015	2015	NUM
cet-14412	22	40	)	)	PUNCT
cet-14412	22	41	.	.	PUNCT
cet-14412	23	1	another	another	DET
cet-14412	23	2	limitation	limitation	NOUN
cet-14412	23	3	to	to	ADP
cet-14412	23	4	the	the	DET
cet-14412	23	5	dropcast	dropcast	ADJ
cet-14412	23	6	method	method	NOUN
cet-14412	23	7	is	be	AUX
cet-14412	23	8	the	the	DET
cet-14412	23	9	amount	amount	NOUN
cet-14412	23	10	of	of	ADP
cet-14412	23	11	time	time	NOUN
cet-14412	23	12	needed	need	VERB
cet-14412	23	13	for	for	SCONJ
cet-14412	23	14	evaporation	evaporation	NOUN
cet-14412	23	15	to	to	PART
cet-14412	23	16	occur	occur	VERB
cet-14412	23	17	.	.	PUNCT
cet-14412	24	1	the	the	DET
cet-14412	24	2	slow	slow	ADJ
cet-14412	24	3	rate	rate	NOUN
cet-14412	24	4	of	of	ADP
cet-14412	24	5	introduction	introduction	NOUN
cet-14412	24	6	of	of	ADP
cet-14412	24	7	target	target	NOUN
cet-14412	24	8	7	7	NUM
cet-14412	24	9	mailto:docoslis@queensu.ca	mailto:docoslis@queensu.ca	NOUN
cet-14412	24	10	molecule	molecule	NOUN
cet-14412	24	11	to	to	ADP
cet-14412	24	12	sers	ser	NOUN
cet-14412	24	13	substrate	substrate	NOUN
cet-14412	24	14	impedes	impede	VERB
cet-14412	24	15	the	the	DET
cet-14412	24	16	use	use	NOUN
cet-14412	24	17	of	of	ADP
cet-14412	24	18	the	the	DET
cet-14412	24	19	technique	technique	NOUN
cet-14412	24	20	in	in	ADP
cet-14412	24	21	poc	poc	NOUN
cet-14412	24	22	diagnostics	diagnostic	NOUN
cet-14412	24	23	,	,	PUNCT
cet-14412	24	24	since	since	SCONJ
cet-14412	24	25	measurements	measurement	NOUN
cet-14412	24	26	need	need	VERB
cet-14412	24	27	to	to	PART
cet-14412	24	28	be	be	AUX
cet-14412	24	29	taken	take	VERB
cet-14412	24	30	instantaneously	instantaneously	ADV
cet-14412	24	31	.	.	PUNCT
cet-14412	25	1	before	before	SCONJ
cet-14412	25	2	these	these	DET
cet-14412	25	3	new	new	ADJ
cet-14412	25	4	sers	ser	NOUN
cet-14412	25	5	substrates	substrate	NOUN
cet-14412	25	6	can	can	AUX
cet-14412	25	7	be	be	AUX
cet-14412	25	8	implemented	implement	VERB
cet-14412	25	9	into	into	ADP
cet-14412	25	10	poc	poc	NOUN
cet-14412	25	11	diagnostics	diagnostic	NOUN
cet-14412	25	12	,	,	PUNCT
cet-14412	25	13	new	new	ADJ
cet-14412	25	14	sample	sample	NOUN
cet-14412	25	15	introduction	introduction	NOUN
cet-14412	25	16	methods	method	NOUN
cet-14412	25	17	must	must	AUX
cet-14412	25	18	be	be	AUX
cet-14412	25	19	investigated	investigate	VERB
cet-14412	25	20	such	such	ADJ
cet-14412	25	21	that	that	DET
cet-14412	25	22	target	target	NOUN
cet-14412	25	23	molecules	molecule	NOUN
cet-14412	25	24	are	be	AUX
cet-14412	25	25	arranged	arrange	VERB
cet-14412	25	26	evenly	evenly	ADV
cet-14412	25	27	on	on	ADP
cet-14412	25	28	the	the	DET
cet-14412	25	29	substrates	substrate	NOUN
cet-14412	25	30	,	,	PUNCT
cet-14412	25	31	resulting	result	VERB
cet-14412	25	32	in	in	ADP
cet-14412	25	33	greater	great	ADJ
cet-14412	25	34	reproducibility	reproducibility	NOUN
cet-14412	25	35	and	and	CCONJ
cet-14412	25	36	reliability	reliability	NOUN
cet-14412	25	37	.	.	PUNCT
cet-14412	26	1	a	a	DET
cet-14412	26	2	uniform	uniform	NOUN
cet-14412	26	3	and	and	CCONJ
cet-14412	26	4	gradual	gradual	ADJ
cet-14412	26	5	sample	sample	NOUN
cet-14412	26	6	introduction	introduction	NOUN
cet-14412	26	7	into	into	ADP
cet-14412	26	8	the	the	DET
cet-14412	26	9	sers	ser	NOUN
cet-14412	26	10	-	-	ADJ
cet-14412	26	11	active	active	ADJ
cet-14412	26	12	surface	surface	NOUN
cet-14412	26	13	may	may	AUX
cet-14412	26	14	also	also	ADV
cet-14412	26	15	help	help	VERB
cet-14412	26	16	overcome	overcome	VERB
cet-14412	26	17	limitations	limitation	NOUN
cet-14412	26	18	with	with	ADP
cet-14412	26	19	the	the	DET
cet-14412	26	20	ability	ability	NOUN
cet-14412	26	21	of	of	ADP
cet-14412	26	22	sers	ser	NOUN
cet-14412	26	23	to	to	PART
cet-14412	26	24	provide	provide	VERB
cet-14412	26	25	quantifiable	quantifiable	ADJ
cet-14412	26	26	results	result	NOUN
cet-14412	26	27	.	.	PUNCT
cet-14412	27	1	therefore	therefore	ADV
cet-14412	27	2	,	,	PUNCT
cet-14412	27	3	the	the	DET
cet-14412	27	4	combination	combination	NOUN
cet-14412	27	5	of	of	ADP
cet-14412	27	6	these	these	DET
cet-14412	27	7	new	new	ADJ
cet-14412	27	8	sers	ser	NOUN
cet-14412	27	9	substrates	substrate	NOUN
cet-14412	27	10	with	with	ADP
cet-14412	27	11	microfluidics	microfluidic	NOUN
cet-14412	27	12	appears	appear	VERB
cet-14412	27	13	to	to	PART
cet-14412	27	14	hold	hold	VERB
cet-14412	27	15	promise	promise	NOUN
cet-14412	27	16	for	for	ADP
cet-14412	27	17	overcoming	overcome	VERB
cet-14412	27	18	some	some	PRON
cet-14412	27	19	of	of	ADP
cet-14412	27	20	the	the	DET
cet-14412	27	21	main	main	ADJ
cet-14412	27	22	disadvantages	disadvantage	NOUN
cet-14412	27	23	that	that	PRON
cet-14412	27	24	presently	presently	ADV
cet-14412	27	25	exist	exist	VERB
cet-14412	27	26	with	with	ADP
cet-14412	27	27	the	the	DET
cet-14412	27	28	application	application	NOUN
cet-14412	27	29	of	of	ADP
cet-14412	27	30	the	the	DET
cet-14412	27	31	method	method	NOUN
cet-14412	27	32	in	in	ADP
cet-14412	27	33	the	the	DET
cet-14412	27	34	field	field	NOUN
cet-14412	27	35	.	.	PUNCT
cet-14412	28	1	this	this	DET
cet-14412	28	2	article	article	NOUN
cet-14412	28	3	is	be	AUX
cet-14412	28	4	a	a	DET
cet-14412	28	5	demonstration	demonstration	NOUN
cet-14412	28	6	of	of	ADP
cet-14412	28	7	how	how	SCONJ
cet-14412	28	8	sers	ser	NOUN
cet-14412	28	9	-	-	ADJ
cet-14412	28	10	active	active	ADJ
cet-14412	28	11	substrates	substrate	NOUN
cet-14412	28	12	can	can	AUX
cet-14412	28	13	be	be	AUX
cet-14412	28	14	combined	combine	VERB
cet-14412	28	15	with	with	ADP
cet-14412	28	16	microfluidics	microfluidic	NOUN
cet-14412	28	17	toward	toward	ADP
cet-14412	28	18	the	the	DET
cet-14412	28	19	development	development	NOUN
cet-14412	28	20	of	of	ADP
cet-14412	28	21	an	an	PRON
cet-14412	28	22	in	in	ADP
cet-14412	28	23	situ	situ	ADJ
cet-14412	28	24	chemical	chemical	NOUN
cet-14412	28	25	detection	detection	NOUN
cet-14412	28	26	method	method	NOUN
cet-14412	28	27	that	that	PRON
cet-14412	28	28	can	can	AUX
cet-14412	28	29	be	be	AUX
cet-14412	28	30	used	use	VERB
cet-14412	28	31	as	as	ADP
cet-14412	28	32	a	a	DET
cet-14412	28	33	poc	poc	NOUN
cet-14412	28	34	diagnostic	diagnostic	ADJ
cet-14412	28	35	device	device	NOUN
cet-14412	28	36	.	.	PUNCT
cet-14412	29	1	a	a	DET
cet-14412	29	2	microfluidic	microfluidic	ADJ
cet-14412	29	3	device	device	NOUN
cet-14412	29	4	prototype	prototype	NOUN
cet-14412	29	5	was	be	AUX
cet-14412	29	6	designed	design	VERB
cet-14412	29	7	,	,	PUNCT
cet-14412	29	8	fabricated	fabricate	VERB
cet-14412	29	9	,	,	PUNCT
cet-14412	29	10	and	and	CCONJ
cet-14412	29	11	characterized	characterize	VERB
cet-14412	29	12	to	to	PART
cet-14412	29	13	demonstrate	demonstrate	VERB
cet-14412	29	14	the	the	DET
cet-14412	29	15	feasibility	feasibility	NOUN
cet-14412	29	16	of	of	ADP
cet-14412	29	17	microfluidics	microfluidic	NOUN
cet-14412	29	18	in	in	ADP
cet-14412	29	19	achieving	achieve	VERB
cet-14412	29	20	analyte	analyte	NOUN
cet-14412	29	21	transport	transport	NOUN
cet-14412	29	22	from	from	ADP
cet-14412	29	23	loading	load	VERB
cet-14412	29	24	to	to	ADP
cet-14412	29	25	detection	detection	NOUN
cet-14412	29	26	site	site	NOUN
cet-14412	29	27	.	.	PUNCT
cet-14412	30	1	more	more	ADV
cet-14412	30	2	importantly	importantly	ADV
cet-14412	30	3	,	,	PUNCT
cet-14412	30	4	this	this	DET
cet-14412	30	5	basic	basic	ADJ
cet-14412	30	6	microfluidic	microfluidic	ADJ
cet-14412	30	7	setup	setup	NOUN
cet-14412	30	8	is	be	AUX
cet-14412	30	9	used	use	VERB
cet-14412	30	10	here	here	ADV
cet-14412	30	11	for	for	ADP
cet-14412	30	12	monitoring	monitor	VERB
cet-14412	30	13	the	the	DET
cet-14412	30	14	adsorption	adsorption	NOUN
cet-14412	30	15	kinetics	kinetic	NOUN
cet-14412	30	16	of	of	ADP
cet-14412	30	17	the	the	DET
cet-14412	30	18	molecule	molecule	NOUN
cet-14412	30	19	rhodamine	rhodamine	NOUN
cet-14412	30	20	6	6	NUM
cet-14412	30	21	g	g	NOUN
cet-14412	30	22	(	(	PUNCT
cet-14412	30	23	r6	r6	NOUN
cet-14412	30	24	g	g	NOUN
cet-14412	30	25	)	)	PUNCT
cet-14412	30	26	onto	onto	ADP
cet-14412	30	27	a	a	DET
cet-14412	30	28	sers	ser	NOUN
cet-14412	30	29	-	-	ADJ
cet-14412	30	30	active	active	ADJ
cet-14412	30	31	substrate	substrate	NOUN
cet-14412	30	32	;	;	PUNCT
cet-14412	30	33	an	an	DET
cet-14412	30	34	application	application	NOUN
cet-14412	30	35	,	,	PUNCT
cet-14412	30	36	for	for	ADP
cet-14412	30	37	which	which	PRON
cet-14412	30	38	only	only	ADV
cet-14412	30	39	scare	scare	VERB
cet-14412	30	40	information	information	NOUN
cet-14412	30	41	is	be	AUX
cet-14412	30	42	available	available	ADJ
cet-14412	30	43	in	in	ADP
cet-14412	30	44	the	the	DET
cet-14412	30	45	literature	literature	NOUN
cet-14412	30	46	.	.	PUNCT
cet-14412	31	1	in	in	ADP
cet-14412	31	2	fact	fact	NOUN
cet-14412	31	3	,	,	PUNCT
cet-14412	31	4	we	we	PRON
cet-14412	31	5	take	take	VERB
cet-14412	31	6	this	this	DET
cet-14412	31	7	application	application	NOUN
cet-14412	31	8	a	a	DET
cet-14412	31	9	step	step	NOUN
cet-14412	31	10	further	far	ADV
cet-14412	31	11	by	by	ADP
cet-14412	31	12	showing	show	VERB
cet-14412	31	13	how	how	SCONJ
cet-14412	31	14	to	to	PART
cet-14412	31	15	quantify	quantify	VERB
cet-14412	31	16	in	in	ADP
cet-14412	31	17	real	real	ADJ
cet-14412	31	18	time	time	NOUN
cet-14412	31	19	the	the	DET
cet-14412	31	20	actual	actual	ADJ
cet-14412	31	21	concentration	concentration	NOUN
cet-14412	31	22	of	of	ADP
cet-14412	31	23	adsorbed	adsorb	VERB
cet-14412	31	24	r6	r6	NOUN
cet-14412	31	25	g	g	NOUN
cet-14412	31	26	onto	onto	ADP
cet-14412	31	27	the	the	DET
cet-14412	31	28	sers	ser	NOUN
cet-14412	31	29	substrate	substrate	NOUN
cet-14412	31	30	.	.	PUNCT
cet-14412	32	1	we	we	PRON
cet-14412	32	2	offer	offer	VERB
cet-14412	32	3	a	a	DET
cet-14412	32	4	proof	proof	NOUN
cet-14412	32	5	of	of	ADP
cet-14412	32	6	concept	concept	NOUN
cet-14412	32	7	on	on	ADP
cet-14412	32	8	how	how	SCONJ
cet-14412	32	9	we	we	PRON
cet-14412	32	10	can	can	AUX
cet-14412	32	11	use	use	VERB
cet-14412	32	12	a	a	DET
cet-14412	32	13	sers	ser	NOUN
cet-14412	32	14	-	-	ADJ
cet-14412	32	15	active	active	ADJ
cet-14412	32	16	substrate	substrate	NOUN
cet-14412	32	17	embedded	embed	VERB
cet-14412	32	18	in	in	ADP
cet-14412	32	19	a	a	DET
cet-14412	32	20	diagnostic	diagnostic	ADJ
cet-14412	32	21	microfluidic	microfluidic	ADJ
cet-14412	32	22	device	device	NOUN
cet-14412	32	23	to	to	PART
cet-14412	32	24	detect	detect	VERB
cet-14412	32	25	and	and	CCONJ
cet-14412	32	26	report	report	VERB
cet-14412	32	27	the	the	DET
cet-14412	32	28	concentration	concentration	NOUN
cet-14412	32	29	of	of	ADP
cet-14412	32	30	an	an	DET
cet-14412	32	31	unknown	unknown	ADJ
cet-14412	32	32	target	target	NOUN
cet-14412	32	33	molecule	molecule	NOUN
cet-14412	32	34	in	in	ADP
cet-14412	32	35	an	an	DET
cet-14412	32	36	aqueous	aqueous	ADJ
cet-14412	32	37	solution	solution	NOUN
cet-14412	32	38	as	as	ADP
cet-14412	32	39	a	a	DET
cet-14412	32	40	function	function	NOUN
cet-14412	32	41	of	of	ADP
cet-14412	32	42	time	time	NOUN
cet-14412	32	43	.	.	PUNCT
cet-14412	33	1	2	2	X
cet-14412	33	2	.	.	X
cet-14412	33	3	experimental	experimental	ADJ
cet-14412	33	4	details	detail	NOUN
cet-14412	33	5	materials	material	NOUN
cet-14412	33	6	.	.	PUNCT
cet-14412	34	1	polydimethylsiloxane	polydimethylsiloxane	NOUN
cet-14412	34	2	(	(	PUNCT
cet-14412	34	3	pdms	pdms	NOUN
cet-14412	34	4	)	)	PUNCT
cet-14412	34	5	,	,	PUNCT
cet-14412	34	6	sylgard	sylgard	NOUN
cet-14412	34	7	™	™	ADJ
cet-14412	34	8	elastomer	elastomer	NOUN
cet-14412	34	9	kit	kit	NOUN
cet-14412	34	10	with	with	ADP
cet-14412	34	11	monomer	monomer	NOUN
cet-14412	34	12	and	and	CCONJ
cet-14412	34	13	curing	cure	VERB
cet-14412	34	14	agent	agent	NOUN
cet-14412	34	15	,	,	PUNCT
cet-14412	34	16	was	be	AUX
cet-14412	34	17	purchased	purchase	VERB
cet-14412	34	18	from	from	ADP
cet-14412	34	19	dow	dow	PROPN
cet-14412	34	20	corning	corning	PROPN
cet-14412	34	21	corporation	corporation	NOUN
cet-14412	34	22	(	(	PUNCT
cet-14412	34	23	midland	midland	PROPN
cet-14412	34	24	,	,	PUNCT
cet-14412	34	25	mi	mi	PROPN
cet-14412	34	26	,	,	PUNCT
cet-14412	34	27	usa	usa	PROPN
cet-14412	34	28	)	)	PUNCT
cet-14412	34	29	.	.	PUNCT
cet-14412	35	1	polylactic	polylactic	ADJ
cet-14412	35	2	acid	acid	NOUN
cet-14412	35	3	(	(	PUNCT
cet-14412	35	4	pla	pla	NOUN
cet-14412	35	5	)	)	PUNCT
cet-14412	35	6	3d	3d	NOUN
cet-14412	35	7	printer	printer	NOUN
cet-14412	35	8	filament	filament	NOUN
cet-14412	35	9	was	be	AUX
cet-14412	35	10	purchased	purchase	VERB
cet-14412	35	11	from	from	ADP
cet-14412	35	12	amz3d	amz3d	PROPN
cet-14412	35	13	.	.	PROPN
cet-14412	35	14	diiodomethane	diiodomethane	PROPN
cet-14412	35	15	(	(	PUNCT
cet-14412	35	16	99	99	NUM
cet-14412	35	17	%	%	NOUN
cet-14412	35	18	)	)	PUNCT
cet-14412	35	19	and	and	CCONJ
cet-14412	35	20	rhodamine	rhodamine	ADJ
cet-14412	35	21	6	6	NUM
cet-14412	35	22	g	g	NOUN
cet-14412	35	23	(	(	PUNCT
cet-14412	35	24	r6	r6	NOUN
cet-14412	35	25	g	g	NOUN
cet-14412	35	26	,	,	PUNCT
cet-14412	35	27	99	99	NUM
cet-14412	35	28	%	%	NOUN
cet-14412	35	29	)	)	PUNCT
cet-14412	35	30	were	be	AUX
cet-14412	35	31	purchased	purchase	VERB
cet-14412	35	32	from	from	ADP
cet-14412	35	33	sigma	sigma	PROPN
cet-14412	35	34	-	-	PUNCT
cet-14412	35	35	aldrich	aldrich	PROPN
cet-14412	35	36	(	(	PUNCT
cet-14412	35	37	oakville	oakville	PROPN
cet-14412	35	38	,	,	PUNCT
cet-14412	35	39	on	on	ADP
cet-14412	35	40	)	)	PUNCT
cet-14412	35	41	.	.	PUNCT
cet-14412	36	1	silver	silver	ADJ
cet-14412	36	2	nanoparticles	nanoparticle	NOUN
cet-14412	36	3	(	(	PUNCT
cet-14412	36	4	agnps	agnps	ADJ
cet-14412	36	5	)	)	PUNCT
cet-14412	36	6	,	,	PUNCT
cet-14412	36	7	50	50	NUM
cet-14412	36	8	nm	nm	NOUN
cet-14412	36	9	in	in	ADP
cet-14412	36	10	diameter	diameter	NOUN
cet-14412	36	11	,	,	PUNCT
cet-14412	36	12	were	be	AUX
cet-14412	36	13	bought	buy	VERB
cet-14412	36	14	from	from	ADP
cet-14412	36	15	cytodiagnostics	cytodiagnostics	PROPN
cet-14412	36	16	inc	inc	PROPN
cet-14412	36	17	.	.	PROPN
cet-14412	36	18	(	(	PUNCT
cet-14412	36	19	burlington	burlington	PROPN
cet-14412	36	20	,	,	PUNCT
cet-14412	36	21	on	on	ADP
cet-14412	36	22	)	)	PUNCT
cet-14412	36	23	.	.	PUNCT
cet-14412	37	1	polished	polished	ADJ
cet-14412	37	2	silicon	silicon	NOUN
cet-14412	37	3	wafers	wafer	NOUN
cet-14412	37	4	(	(	PUNCT
cet-14412	37	5	4	4	NUM
cet-14412	37	6	”	"	PUNCT
cet-14412	37	7	diameter	diameter	NOUN
cet-14412	37	8	)	)	PUNCT
cet-14412	37	9	with	with	ADP
cet-14412	37	10	a	a	DET
cet-14412	37	11	thermally	thermally	ADV
cet-14412	37	12	grown	grow	VERB
cet-14412	37	13	sio2	sio2	NOUN
cet-14412	37	14	layer	layer	NOUN
cet-14412	37	15	(	(	PUNCT
cet-14412	37	16	0.5	0.5	NUM
cet-14412	37	17	µm	µm	NOUN
cet-14412	37	18	)	)	PUNCT
cet-14412	37	19	were	be	AUX
cet-14412	37	20	purchased	purchase	VERB
cet-14412	37	21	from	from	ADP
cet-14412	37	22	university	university	NOUN
cet-14412	37	23	wafer	wafer	NOUN
cet-14412	37	24	(	(	PUNCT
cet-14412	37	25	south	south	PROPN
cet-14412	37	26	boston	boston	PROPN
cet-14412	37	27	,	,	PUNCT
cet-14412	37	28	ma	ma	PROPN
cet-14412	37	29	,	,	PUNCT
cet-14412	37	30	usa	usa	PROPN
cet-14412	37	31	)	)	PUNCT
cet-14412	37	32	.	.	PUNCT
cet-14412	38	1	millipore	millipore	PROPN
cet-14412	38	2	®	®	PROPN
cet-14412	38	3	water	water	NOUN
cet-14412	38	4	(	(	PUNCT
cet-14412	38	5	18.2	18.2	NUM
cet-14412	38	6	mω	mω	NOUN
cet-14412	38	7	cm	cm	NOUN
cet-14412	38	8	)	)	PUNCT
cet-14412	38	9	was	be	AUX
cet-14412	38	10	used	use	VERB
cet-14412	38	11	in	in	ADP
cet-14412	38	12	all	all	DET
cet-14412	38	13	experiments	experiment	NOUN
cet-14412	38	14	to	to	PART
cet-14412	38	15	prepare	prepare	VERB
cet-14412	38	16	r6	r6	NOUN
cet-14412	38	17	g	g	NOUN
cet-14412	38	18	stock	stock	NOUN
cet-14412	38	19	solutions	solution	NOUN
cet-14412	38	20	.	.	PUNCT
cet-14412	39	1	methods	method	NOUN
cet-14412	39	2	microfluidic	microfluidic	ADJ
cet-14412	39	3	device	device	NOUN
cet-14412	39	4	.	.	PUNCT
cet-14412	40	1	a	a	DET
cet-14412	40	2	negative	negative	ADJ
cet-14412	40	3	mold	mold	NOUN
cet-14412	40	4	of	of	ADP
cet-14412	40	5	the	the	DET
cet-14412	40	6	microfluidic	microfluidic	ADJ
cet-14412	40	7	prototype	prototype	NOUN
cet-14412	40	8	was	be	AUX
cet-14412	40	9	designed	design	VERB
cet-14412	40	10	and	and	CCONJ
cet-14412	40	11	modelled	model	VERB
cet-14412	40	12	using	use	VERB
cet-14412	40	13	solidworks	solidwork	NOUN
cet-14412	40	14	.	.	PUNCT
cet-14412	41	1	the	the	DET
cet-14412	41	2	mold	mold	NOUN
cet-14412	41	3	was	be	AUX
cet-14412	41	4	printed	print	VERB
cet-14412	41	5	using	use	VERB
cet-14412	41	6	a	a	DET
cet-14412	41	7	3d	3d	NUM
cet-14412	41	8	fdm	fdm	NOUN
cet-14412	41	9	(	(	PUNCT
cet-14412	41	10	fusion	fusion	NOUN
cet-14412	41	11	deposition	deposition	NOUN
cet-14412	41	12	modeling	modeling	NOUN
cet-14412	41	13	)	)	PUNCT
cet-14412	41	14	printer	printer	NOUN
cet-14412	41	15	(	(	PUNCT
cet-14412	41	16	iiip	iiip	PROPN
cet-14412	41	17	mini	mini	ADJ
cet-14412	41	18	3d	3d	PROPN
cet-14412	41	19	printer	printer	NOUN
cet-14412	41	20	)	)	PUNCT
cet-14412	41	21	,	,	PUNCT
cet-14412	41	22	with	with	ADP
cet-14412	41	23	pla	pla	NOUN
cet-14412	41	24	as	as	ADP
cet-14412	41	25	the	the	DET
cet-14412	41	26	print	print	NOUN
cet-14412	41	27	material	material	NOUN
cet-14412	41	28	.	.	PUNCT
cet-14412	42	1	prototypes	prototype	NOUN
cet-14412	42	2	were	be	AUX
cet-14412	42	3	cast	cast	VERB
cet-14412	42	4	in	in	ADP
cet-14412	42	5	pdms	pdms	NOUN
cet-14412	42	6	using	use	VERB
cet-14412	42	7	a	a	DET
cet-14412	42	8	monomer	monomer	NOUN
cet-14412	42	9	base	base	NOUN
cet-14412	42	10	-	-	PUNCT
cet-14412	42	11	to	to	ADP
cet-14412	42	12	-	-	PUNCT
cet-14412	42	13	curing	cure	VERB
cet-14412	42	14	agent	agent	NOUN
cet-14412	42	15	ratio	ratio	NOUN
cet-14412	42	16	of	of	ADP
cet-14412	42	17	10:1	10:1	NUM
cet-14412	42	18	.	.	PUNCT
cet-14412	43	1	each	each	DET
cet-14412	43	2	batch	batch	NOUN
cet-14412	43	3	was	be	AUX
cet-14412	43	4	mixed	mix	VERB
cet-14412	43	5	for	for	ADP
cet-14412	43	6	5	5	NUM
cet-14412	43	7	minutes	minute	NOUN
cet-14412	43	8	and	and	CCONJ
cet-14412	43	9	degassed	degas	VERB
cet-14412	43	10	in	in	ADP
cet-14412	43	11	a	a	DET
cet-14412	43	12	vacuum	vacuum	NOUN
cet-14412	43	13	at	at	ADP
cet-14412	43	14	0.7	0.7	NUM
cet-14412	43	15	mpa	mpa	NOUN
cet-14412	43	16	for	for	ADP
cet-14412	43	17	30	30	NUM
cet-14412	43	18	minutes	minute	NOUN
cet-14412	43	19	before	before	ADP
cet-14412	43	20	being	be	AUX
cet-14412	43	21	poured	pour	VERB
cet-14412	43	22	into	into	ADP
cet-14412	43	23	the	the	DET
cet-14412	43	24	mold	mold	NOUN
cet-14412	43	25	.	.	PUNCT
cet-14412	44	1	microfluidic	microfluidic	ADJ
cet-14412	44	2	chips	chip	NOUN
cet-14412	44	3	were	be	AUX
cet-14412	44	4	allowed	allow	VERB
cet-14412	44	5	to	to	PART
cet-14412	44	6	cure	cure	VERB
cet-14412	44	7	on	on	ADP
cet-14412	44	8	a	a	DET
cet-14412	44	9	hotplate	hotplate	NOUN
cet-14412	44	10	at	at	ADP
cet-14412	44	11	80	80	NUM
cet-14412	44	12	˚c	˚c	PROPN
cet-14412	44	13	for	for	ADP
cet-14412	44	14	2	2	NUM
cet-14412	44	15	-	-	SYM
cet-14412	44	16	3	3	NUM
cet-14412	44	17	hours	hour	NOUN
cet-14412	44	18	.	.	PUNCT
cet-14412	45	1	the	the	DET
cet-14412	45	2	pdms	pdms	ADJ
cet-14412	45	3	chip	chip	NOUN
cet-14412	45	4	was	be	AUX
cet-14412	45	5	rendered	render	VERB
cet-14412	45	6	hydrophilic	hydrophilic	ADJ
cet-14412	45	7	through	through	ADP
cet-14412	45	8	oxygen	oxygen	NOUN
cet-14412	45	9	plasma	plasma	NOUN
cet-14412	45	10	treatment	treatment	NOUN
cet-14412	45	11	,	,	PUNCT
cet-14412	45	12	using	use	VERB
cet-14412	45	13	a	a	DET
cet-14412	45	14	harrick	harrick	NOUN
cet-14412	45	15	plasma	plasma	NOUN
cet-14412	45	16	cleaner	cleaner	NOUN
cet-14412	45	17	(	(	PUNCT
cet-14412	45	18	model	model	NOUN
cet-14412	45	19	:	:	PUNCT
cet-14412	45	20	pdc32	pdc32	PROPN
cet-14412	45	21	g	g	NOUN
cet-14412	45	22	)	)	PUNCT
cet-14412	45	23	for	for	ADP
cet-14412	45	24	5	5	NUM
cet-14412	45	25	minutes	minute	NOUN
cet-14412	45	26	.	.	PUNCT
cet-14412	46	1	microfluidic	microfluidic	ADJ
cet-14412	46	2	prototypes	prototype	NOUN
cet-14412	46	3	were	be	AUX
cet-14412	46	4	assembled	assemble	VERB
cet-14412	46	5	by	by	ADP
cet-14412	46	6	contacting	contact	VERB
cet-14412	46	7	the	the	DET
cet-14412	46	8	pdms	pdms	ADJ
cet-14412	46	9	chips	chip	NOUN
cet-14412	46	10	with	with	ADP
cet-14412	46	11	glass	glass	NOUN
cet-14412	46	12	substrates	substrate	NOUN
cet-14412	46	13	and	and	CCONJ
cet-14412	46	14	letting	let	VERB
cet-14412	46	15	them	they	PRON
cet-14412	46	16	bond	bond	NOUN
cet-14412	46	17	on	on	ADP
cet-14412	46	18	a	a	DET
cet-14412	46	19	hotplate	hotplate	NOUN
cet-14412	46	20	at	at	ADP
cet-14412	46	21	80	80	NUM
cet-14412	46	22	˚c	˚c	PROPN
cet-14412	46	23	for	for	ADP
cet-14412	46	24	20	20	NUM
cet-14412	46	25	minutes	minute	NOUN
cet-14412	46	26	.	.	PUNCT
cet-14412	47	1	inlet	inlet	VERB
cet-14412	47	2	and	and	CCONJ
cet-14412	47	3	outlet	outlet	NOUN
cet-14412	47	4	reservoirs	reservoir	NOUN
cet-14412	47	5	each	each	PRON
cet-14412	47	6	have	have	VERB
cet-14412	47	7	a	a	DET
cet-14412	47	8	radius	radius	NOUN
cet-14412	47	9	of	of	ADP
cet-14412	47	10	3	3	NUM
cet-14412	47	11	mm	mm	NOUN
cet-14412	47	12	for	for	ADP
cet-14412	47	13	sers	ser	NOUN
cet-14412	47	14	substrate	substrate	NOUN
cet-14412	47	15	integration	integration	NOUN
cet-14412	47	16	.	.	PUNCT
cet-14412	48	1	the	the	DET
cet-14412	48	2	channel	channel	NOUN
cet-14412	48	3	connecting	connect	VERB
cet-14412	48	4	the	the	DET
cet-14412	48	5	reservoirs	reservoir	NOUN
cet-14412	48	6	has	have	VERB
cet-14412	48	7	a	a	DET
cet-14412	48	8	length	length	NOUN
cet-14412	48	9	of	of	ADP
cet-14412	48	10	30	30	NUM
cet-14412	48	11	mm	mm	NOUN
cet-14412	48	12	and	and	CCONJ
cet-14412	48	13	a	a	DET
cet-14412	48	14	crosssectional	crosssectional	ADJ
cet-14412	48	15	area	area	NOUN
cet-14412	48	16	of	of	ADP
cet-14412	48	17	1	1	NUM
cet-14412	48	18	mm	mm	NOUN
cet-14412	48	19	by	by	ADP
cet-14412	48	20	1	1	NUM
cet-14412	48	21	mm	mm	NOUN
cet-14412	48	22	.	.	PUNCT
cet-14412	49	1	sample	sample	NOUN
cet-14412	49	2	preparation	preparation	NOUN
cet-14412	49	3	and	and	CCONJ
cet-14412	49	4	fluorescence	fluorescence	NOUN
cet-14412	49	5	measurements	measurement	NOUN
cet-14412	49	6	.	.	PUNCT
cet-14412	50	1	six	six	NUM
cet-14412	50	2	aliquots	aliquot	NOUN
cet-14412	50	3	(	(	PUNCT
cet-14412	50	4	1	1	NUM
cet-14412	50	5	ml	ml	NOUN
cet-14412	50	6	)	)	PUNCT
cet-14412	50	7	of	of	ADP
cet-14412	50	8	agnp	agnp	NOUN
cet-14412	50	9	dispersion	dispersion	NOUN
cet-14412	50	10	were	be	AUX
cet-14412	50	11	concentrated	concentrate	VERB
cet-14412	50	12	through	through	ADP
cet-14412	50	13	centrifugation	centrifugation	NOUN
cet-14412	50	14	at	at	ADP
cet-14412	50	15	3600	3600	NUM
cet-14412	50	16	g	g	NOUN
cet-14412	50	17	for	for	ADP
cet-14412	50	18	30	30	NUM
cet-14412	50	19	minutes	minute	NOUN
cet-14412	50	20	.	.	PUNCT
cet-14412	51	1	the	the	DET
cet-14412	51	2	supernatant	supernatant	NOUN
cet-14412	51	3	was	be	AUX
cet-14412	51	4	discarded	discard	VERB
cet-14412	51	5	from	from	ADP
cet-14412	51	6	each	each	DET
cet-14412	51	7	sample	sample	NOUN
cet-14412	51	8	and	and	CCONJ
cet-14412	51	9	the	the	DET
cet-14412	51	10	isolated	isolated	ADJ
cet-14412	51	11	agnps	agnps	NOUN
cet-14412	51	12	were	be	AUX
cet-14412	51	13	placed	place	VERB
cet-14412	51	14	into	into	ADP
cet-14412	51	15	r6	r6	PROPN
cet-14412	51	16	g	g	NOUN
cet-14412	51	17	solutions	solution	NOUN
cet-14412	51	18	of	of	ADP
cet-14412	51	19	five	five	NUM
cet-14412	51	20	concentrations	concentration	NOUN
cet-14412	51	21	(	(	PUNCT
cet-14412	51	22	5	5	NUM
cet-14412	51	23	*	*	SYM
cet-14412	51	24	10	10	NUM
cet-14412	51	25	-	-	SYM
cet-14412	51	26	8	8	NUM
cet-14412	51	27	m	m	NOUN
cet-14412	51	28	,	,	PUNCT
cet-14412	51	29	10	10	NUM
cet-14412	51	30	-	-	SYM
cet-14412	51	31	7	7	NUM
cet-14412	51	32	m	m	NOUN
cet-14412	51	33	,	,	PUNCT
cet-14412	51	34	5	5	NUM
cet-14412	51	35	*	*	SYM
cet-14412	51	36	10	10	NUM
cet-14412	51	37	-	-	SYM
cet-14412	51	38	7	7	NUM
cet-14412	51	39	m	m	NOUN
cet-14412	51	40	,	,	PUNCT
cet-14412	51	41	106	106	NUM
cet-14412	51	42	m	m	NOUN
cet-14412	51	43	and	and	CCONJ
cet-14412	51	44	5	5	NUM
cet-14412	51	45	*	*	NUM
cet-14412	51	46	10	10	NUM
cet-14412	51	47	-	-	SYM
cet-14412	51	48	6	6	NUM
cet-14412	51	49	m	m	NOUN
cet-14412	51	50	)	)	PUNCT
cet-14412	51	51	and	and	CCONJ
cet-14412	51	52	a	a	DET
cet-14412	51	53	control	control	NOUN
cet-14412	51	54	solution	solution	NOUN
cet-14412	51	55	of	of	ADP
cet-14412	51	56	water	water	NOUN
cet-14412	51	57	(	(	PUNCT
cet-14412	51	58	5	5	NUM
cet-14412	51	59	ml	ml	NOUN
cet-14412	51	60	each	each	PRON
cet-14412	51	61	)	)	PUNCT
cet-14412	51	62	.	.	PUNCT
cet-14412	52	1	solutions	solution	NOUN
cet-14412	52	2	of	of	ADP
cet-14412	52	3	r6	r6	PROPN
cet-14412	52	4	g	g	PROPN
cet-14412	52	5	were	be	AUX
cet-14412	52	6	sonicated	sonicate	VERB
cet-14412	52	7	to	to	PART
cet-14412	52	8	ensure	ensure	VERB
cet-14412	52	9	full	full	ADJ
cet-14412	52	10	dispersion	dispersion	NOUN
cet-14412	52	11	of	of	ADP
cet-14412	52	12	agnps	agnps	PROPN
cet-14412	52	13	and	and	CCONJ
cet-14412	52	14	were	be	AUX
cet-14412	52	15	left	leave	VERB
cet-14412	52	16	to	to	PART
cet-14412	52	17	adsorb	adsorb	VERB
cet-14412	52	18	for	for	ADP
cet-14412	52	19	24	24	NUM
cet-14412	52	20	hours	hour	NOUN
cet-14412	52	21	.	.	PUNCT
cet-14412	53	1	solutions	solution	NOUN
cet-14412	53	2	were	be	AUX
cet-14412	53	3	centrifuged	centrifuge	VERB
cet-14412	53	4	again	again	ADV
cet-14412	53	5	at	at	ADP
cet-14412	53	6	the	the	DET
cet-14412	53	7	same	same	ADJ
cet-14412	53	8	conditions	condition	NOUN
cet-14412	53	9	,	,	PUNCT
cet-14412	53	10	followed	follow	VERB
cet-14412	53	11	by	by	ADP
cet-14412	53	12	removing	remove	VERB
cet-14412	53	13	the	the	DET
cet-14412	53	14	supernatant	supernatant	NOUN
cet-14412	53	15	.	.	PUNCT
cet-14412	54	1	the	the	DET
cet-14412	54	2	supernatant	supernatant	NOUN
cet-14412	54	3	was	be	AUX
cet-14412	54	4	retained	retain	VERB
cet-14412	54	5	and	and	CCONJ
cet-14412	54	6	used	use	VERB
cet-14412	54	7	for	for	ADP
cet-14412	54	8	fluorescence	fluorescence	NOUN
cet-14412	54	9	spectroscopy	spectroscopy	NOUN
cet-14412	54	10	measurements	measurement	NOUN
cet-14412	54	11	.	.	PUNCT
cet-14412	55	1	fluoresce	fluoresce	ADP
cet-14412	55	2	spectral	spectral	ADJ
cet-14412	55	3	data	datum	NOUN
cet-14412	55	4	was	be	AUX
cet-14412	55	5	collected	collect	VERB
cet-14412	55	6	using	use	VERB
cet-14412	55	7	a	a	DET
cet-14412	55	8	pti	pti	PROPN
cet-14412	55	9	quantamaster	quantamaster	NOUN
cet-14412	55	10	™	™	PROPN
cet-14412	55	11	80	80	NUM
cet-14412	55	12	fluorometer	fluorometer	NOUN
cet-14412	55	13	with	with	ADP
cet-14412	55	14	a	a	DET
cet-14412	55	15	xenon	xenon	NOUN
cet-14412	55	16	arc	arc	NOUN
cet-14412	55	17	lamp	lamp	NOUN
cet-14412	55	18	and	and	CCONJ
cet-14412	55	19	dual	dual	ADJ
cet-14412	55	20	pmt	pmt	PROPN
cet-14412	55	21	detectors	detector	NOUN
cet-14412	55	22	.	.	PUNCT
cet-14412	56	1	data	datum	NOUN
cet-14412	56	2	was	be	AUX
cet-14412	56	3	collected	collect	VERB
cet-14412	56	4	using	use	VERB
cet-14412	56	5	the	the	DET
cet-14412	56	6	emission	emission	NOUN
cet-14412	56	7	scan	scan	NOUN
cet-14412	56	8	method	method	NOUN
cet-14412	56	9	over	over	ADP
cet-14412	56	10	a	a	DET
cet-14412	56	11	range	range	NOUN
cet-14412	56	12	of	of	ADP
cet-14412	56	13	500	500	NUM
cet-14412	56	14	nm	nm	NOUN
cet-14412	56	15	to	to	ADP
cet-14412	56	16	650	650	NUM
cet-14412	56	17	nm	nm	NOUN
cet-14412	56	18	with	with	ADP
cet-14412	56	19	an	an	DET
cet-14412	56	20	excitation	excitation	NOUN
cet-14412	56	21	wavelength	wavelength	NOUN
cet-14412	56	22	of	of	ADP
cet-14412	56	23	532	532	NUM
cet-14412	56	24	nm	nm	NOUN
cet-14412	56	25	,	,	PUNCT
cet-14412	56	26	step	step	NOUN
cet-14412	56	27	size	size	NOUN
cet-14412	56	28	of	of	ADP
cet-14412	56	29	0.5	0.5	NUM
cet-14412	56	30	nm	nm	NOUN
cet-14412	56	31	,	,	PUNCT
cet-14412	56	32	integration	integration	NOUN
cet-14412	56	33	time	time	NOUN
cet-14412	56	34	of	of	ADP
cet-14412	56	35	1	1	NUM
cet-14412	56	36	second	second	ADJ
cet-14412	56	37	and	and	CCONJ
cet-14412	56	38	a	a	DET
cet-14412	56	39	blank	blank	ADJ
cet-14412	56	40	water	water	NOUN
cet-14412	56	41	sample	sample	NOUN
cet-14412	56	42	as	as	ADP
cet-14412	56	43	the	the	DET
cet-14412	56	44	background	background	NOUN
cet-14412	56	45	.	.	PUNCT
cet-14412	57	1	a	a	DET
cet-14412	57	2	total	total	NOUN
cet-14412	57	3	of	of	ADP
cet-14412	57	4	three	three	NUM
cet-14412	57	5	spectra	spectra	NOUN
cet-14412	57	6	were	be	AUX
cet-14412	57	7	collected	collect	VERB
cet-14412	57	8	for	for	ADP
cet-14412	57	9	each	each	DET
cet-14412	57	10	sample	sample	NOUN
cet-14412	57	11	tested	test	VERB
cet-14412	57	12	to	to	PART
cet-14412	57	13	determine	determine	VERB
cet-14412	57	14	the	the	DET
cet-14412	57	15	experimental	experimental	ADJ
cet-14412	57	16	error	error	NOUN
cet-14412	57	17	.	.	PUNCT
cet-14412	58	1	sers	ser	NOUN
cet-14412	58	2	substrate	substrate	NOUN
cet-14412	58	3	fabrication	fabrication	NOUN
cet-14412	58	4	.	.	PUNCT
cet-14412	59	1	the	the	DET
cet-14412	59	2	procedure	procedure	NOUN
cet-14412	59	3	is	be	AUX
cet-14412	59	4	described	describe	VERB
cet-14412	59	5	in	in	ADP
cet-14412	59	6	detail	detail	NOUN
cet-14412	59	7	in	in	ADP
cet-14412	59	8	dies	die	NOUN
cet-14412	59	9	et	et	PROPN
cet-14412	59	10	al	al	PROPN
cet-14412	59	11	.	.	PROPN
cet-14412	59	12	,	,	PUNCT
cet-14412	59	13	2017	2017	NUM
cet-14412	59	14	.	.	PUNCT
cet-14412	60	1	briefly	briefly	ADV
cet-14412	60	2	,	,	PUNCT
cet-14412	60	3	the	the	DET
cet-14412	60	4	microchip	microchip	NOUN
cet-14412	60	5	electrodes	electrode	NOUN
cet-14412	60	6	were	be	AUX
cet-14412	60	7	fabricated	fabricate	VERB
cet-14412	60	8	at	at	ADP
cet-14412	60	9	the	the	DET
cet-14412	60	10	nanofabrication	nanofabrication	PROPN
cet-14412	60	11	kingston	kingston	PROPN
cet-14412	60	12	facility	facility	PROPN
cet-14412	60	13	(	(	PUNCT
cet-14412	60	14	nfk	nfk	NOUN
cet-14412	60	15	,	,	PUNCT
cet-14412	60	16	innovation	innovation	NOUN
cet-14412	60	17	park	park	NOUN
cet-14412	60	18	,	,	PUNCT
cet-14412	60	19	kingston	kingston	PROPN
cet-14412	60	20	,	,	PUNCT
cet-14412	60	21	on	on	ADP
cet-14412	60	22	)	)	PUNCT
cet-14412	60	23	.	.	PUNCT
cet-14412	61	1	the	the	DET
cet-14412	61	2	negative	negative	ADJ
cet-14412	61	3	photoresist	photoresist	NOUN
cet-14412	61	4	su-8	su-8	PUNCT
cet-14412	61	5	(	(	PUNCT
cet-14412	61	6	microchem	microchem	PROPN
cet-14412	61	7	corp	corp	PROPN
cet-14412	61	8	,	,	PUNCT
cet-14412	61	9	westborough	westborough	PROPN
cet-14412	61	10	,	,	PUNCT
cet-14412	61	11	ma	ma	PROPN
cet-14412	61	12	)	)	PUNCT
cet-14412	61	13	and	and	CCONJ
cet-14412	61	14	maskless	maskless	NOUN
cet-14412	61	15	photolithography	photolithography	NOUN
cet-14412	61	16	were	be	AUX
cet-14412	61	17	used	use	VERB
cet-14412	61	18	to	to	PART
cet-14412	61	19	transfer	transfer	VERB
cet-14412	61	20	the	the	DET
cet-14412	61	21	microelectrode	microelectrode	NOUN
cet-14412	61	22	pattern	pattern	NOUN
cet-14412	61	23	on	on	ADP
cet-14412	61	24	to	to	ADP
cet-14412	61	25	silicon	silicon	NOUN
cet-14412	61	26	wafers	wafer	NOUN
cet-14412	61	27	.	.	PUNCT
cet-14412	62	1	subsequent	subsequent	ADJ
cet-14412	62	2	electron	electron	NOUN
cet-14412	62	3	beam	beam	NOUN
cet-14412	62	4	metal	metal	NOUN
cet-14412	62	5	film	film	NOUN
cet-14412	62	6	evaporation	evaporation	NOUN
cet-14412	62	7	and	and	CCONJ
cet-14412	62	8	lift	lift	VERB
cet-14412	62	9	off	off	ADP
cet-14412	62	10	completed	complete	VERB
cet-14412	62	11	the	the	DET
cet-14412	62	12	microchips	microchip	NOUN
cet-14412	62	13	.	.	PUNCT
cet-14412	63	1	a	a	DET
cet-14412	63	2	layer	layer	NOUN
cet-14412	63	3	of	of	ADP
cet-14412	63	4	chrome	chrome	NOUN
cet-14412	63	5	(	(	PUNCT
cet-14412	63	6	5	5	NUM
cet-14412	63	7	µm	µm	NOUN
cet-14412	63	8	)	)	PUNCT
cet-14412	63	9	was	be	AUX
cet-14412	63	10	implemented	implement	VERB
cet-14412	63	11	on	on	ADP
cet-14412	63	12	the	the	DET
cet-14412	63	13	silicon	silicon	NOUN
cet-14412	63	14	wafer	wafer	NOUN
cet-14412	63	15	to	to	PART
cet-14412	63	16	enhance	enhance	VERB
cet-14412	63	17	the	the	DET
cet-14412	63	18	8	8	NUM
cet-14412	63	19	adhesion	adhesion	NOUN
cet-14412	63	20	of	of	ADP
cet-14412	63	21	gold	gold	NOUN
cet-14412	63	22	electrodes	electrode	NOUN
cet-14412	63	23	(	(	PUNCT
cet-14412	63	24	100	100	NUM
cet-14412	63	25	µm	µm	ADP
cet-14412	63	26	thickness	thickness	NOUN
cet-14412	63	27	)	)	PUNCT
cet-14412	63	28	.	.	PUNCT
cet-14412	64	1	next	next	ADV
cet-14412	64	2	,	,	PUNCT
cet-14412	64	3	agnps	agnps	PROPN
cet-14412	64	4	were	be	AUX
cet-14412	64	5	assembled	assemble	VERB
cet-14412	64	6	by	by	ADP
cet-14412	64	7	dispensing	dispense	VERB
cet-14412	64	8	a	a	DET
cet-14412	64	9	10	10	NUM
cet-14412	64	10	µl	µl	NOUN
cet-14412	64	11	drop	drop	NOUN
cet-14412	64	12	over	over	ADP
cet-14412	64	13	the	the	DET
cet-14412	64	14	center	center	NOUN
cet-14412	64	15	of	of	ADP
cet-14412	64	16	the	the	DET
cet-14412	64	17	microelectrodes	microelectrode	NOUN
cet-14412	64	18	.	.	PUNCT
cet-14412	65	1	each	each	DET
cet-14412	65	2	sers	ser	NOUN
cet-14412	65	3	substrate	substrate	NOUN
cet-14412	65	4	was	be	AUX
cet-14412	65	5	allowed	allow	VERB
cet-14412	65	6	to	to	PART
cet-14412	65	7	accumulate	accumulate	VERB
cet-14412	65	8	on	on	ADP
cet-14412	65	9	the	the	DET
cet-14412	65	10	microchip	microchip	NOUN
cet-14412	65	11	for	for	ADP
cet-14412	65	12	5	5	NUM
cet-14412	65	13	minutes	minute	NOUN
cet-14412	65	14	at	at	ADP
cet-14412	65	15	an	an	DET
cet-14412	65	16	ac	ac	PROPN
cet-14412	65	17	frequency	frequency	NOUN
cet-14412	65	18	of	of	ADP
cet-14412	65	19	10	10	NUM
cet-14412	65	20	hz	hz	VERB
cet-14412	65	21	and	and	CCONJ
cet-14412	65	22	a	a	DET
cet-14412	65	23	peak	peak	NOUN
cet-14412	65	24	-	-	PUNCT
cet-14412	65	25	to	to	ADP
cet-14412	65	26	-	-	PUNCT
cet-14412	65	27	peak	peak	NOUN
cet-14412	65	28	voltage	voltage	NOUN
cet-14412	65	29	of	of	ADP
cet-14412	65	30	3	3	NUM
cet-14412	65	31	v.	v.	ADP
cet-14412	65	32	microchips	microchip	NOUN
cet-14412	65	33	were	be	AUX
cet-14412	65	34	rinsed	rinse	VERB
cet-14412	65	35	with	with	ADP
cet-14412	65	36	water	water	NOUN
cet-14412	65	37	and	and	CCONJ
cet-14412	65	38	dried	dry	VERB
cet-14412	65	39	under	under	ADP
cet-14412	65	40	a	a	DET
cet-14412	65	41	stream	stream	NOUN
cet-14412	65	42	of	of	ADP
cet-14412	65	43	air	air	NOUN
cet-14412	65	44	before	before	ADP
cet-14412	65	45	use	use	NOUN
cet-14412	65	46	in	in	ADP
cet-14412	65	47	further	further	ADJ
cet-14412	65	48	experiments	experiment	NOUN
cet-14412	65	49	.	.	PUNCT
cet-14412	66	1	figure	figure	VERB
cet-14412	66	2	1	1	NUM
cet-14412	66	3	:	:	PUNCT
cet-14412	66	4	(	(	PUNCT
cet-14412	66	5	a	a	X
cet-14412	66	6	)	)	PUNCT
cet-14412	66	7	mold	mold	NOUN
cet-14412	66	8	of	of	ADP
cet-14412	66	9	microfluidic	microfluidic	ADJ
cet-14412	66	10	prototype	prototype	NOUN
cet-14412	66	11	.	.	PUNCT
cet-14412	67	1	(	(	PUNCT
cet-14412	67	2	b	b	X
cet-14412	67	3	)	)	PUNCT
cet-14412	67	4	schematic	schematic	ADJ
cet-14412	67	5	depicting	depict	VERB
cet-14412	67	6	the	the	DET
cet-14412	67	7	cross	cross	NOUN
cet-14412	67	8	sectional	sectional	ADJ
cet-14412	67	9	view	view	NOUN
cet-14412	67	10	of	of	ADP
cet-14412	67	11	the	the	DET
cet-14412	67	12	assembled	assemble	VERB
cet-14412	67	13	microfluidic	microfluidic	ADJ
cet-14412	67	14	device	device	NOUN
cet-14412	67	15	during	during	ADP
cet-14412	67	16	a	a	DET
cet-14412	67	17	sers	ser	NOUN
cet-14412	67	18	measurement	measurement	NOUN
cet-14412	67	19	.	.	PUNCT
cet-14412	68	1	(	(	PUNCT
cet-14412	68	2	c	c	X
cet-14412	68	3	)	)	PUNCT
cet-14412	68	4	sers	ser	NOUN
cet-14412	68	5	-	-	ADJ
cet-14412	68	6	active	active	ADJ
cet-14412	68	7	dendritic	dendritic	ADJ
cet-14412	68	8	agnp	agnp	PROPN
cet-14412	68	9	structures	structure	NOUN
cet-14412	68	10	formed	form	VERB
cet-14412	68	11	in	in	ADP
cet-14412	68	12	the	the	DET
cet-14412	68	13	interelectrode	interelectrode	ADJ
cet-14412	68	14	spaces	space	NOUN
cet-14412	68	15	.	.	PUNCT
cet-14412	69	1	(	(	PUNCT
cet-14412	69	2	d	d	X
cet-14412	69	3	)	)	PUNCT
cet-14412	69	4	sem	sem	NOUN
cet-14412	69	5	image	image	NOUN
cet-14412	69	6	showing	show	VERB
cet-14412	69	7	details	detail	NOUN
cet-14412	69	8	on	on	ADP
cet-14412	69	9	the	the	DET
cet-14412	69	10	agnp	agnp	NOUN
cet-14412	69	11	structure	structure	NOUN
cet-14412	69	12	.	.	PUNCT
cet-14412	70	1	adsorption	adsorption	NOUN
cet-14412	70	2	measurements	measurement	NOUN
cet-14412	70	3	.	.	PUNCT
cet-14412	71	1	sers	ser	NOUN
cet-14412	71	2	substrates	substrate	NOUN
cet-14412	71	3	affixed	affix	VERB
cet-14412	71	4	at	at	ADP
cet-14412	71	5	the	the	DET
cet-14412	71	6	bottom	bottom	NOUN
cet-14412	71	7	of	of	ADP
cet-14412	71	8	the	the	DET
cet-14412	71	9	receiving	receive	VERB
cet-14412	71	10	reservoir	reservoir	NOUN
cet-14412	71	11	of	of	ADP
cet-14412	71	12	the	the	DET
cet-14412	71	13	microfluidic	microfluidic	ADJ
cet-14412	71	14	cell	cell	NOUN
cet-14412	71	15	were	be	AUX
cet-14412	71	16	placed	place	VERB
cet-14412	71	17	under	under	ADP
cet-14412	71	18	the	the	DET
cet-14412	71	19	raman	raman	NOUN
cet-14412	71	20	microscope	microscope	NOUN
cet-14412	71	21	.	.	PUNCT
cet-14412	72	1	solutions	solution	NOUN
cet-14412	72	2	of	of	ADP
cet-14412	72	3	known	know	VERB
cet-14412	72	4	concentration	concentration	NOUN
cet-14412	72	5	of	of	ADP
cet-14412	72	6	r6	r6	NOUN
cet-14412	72	7	g	g	PROPN
cet-14412	72	8	were	be	AUX
cet-14412	72	9	dispensed	dispense	VERB
cet-14412	72	10	in	in	ADP
cet-14412	72	11	the	the	DET
cet-14412	72	12	feeding	feeding	NOUN
cet-14412	72	13	reservoir	reservoir	NOUN
cet-14412	72	14	and	and	CCONJ
cet-14412	72	15	were	be	AUX
cet-14412	72	16	let	let	VERB
cet-14412	72	17	to	to	PART
cet-14412	72	18	flow	flow	VERB
cet-14412	72	19	over	over	ADP
cet-14412	72	20	the	the	DET
cet-14412	72	21	sers	ser	NOUN
cet-14412	72	22	substrate	substrate	NOUN
cet-14412	72	23	in	in	ADP
cet-14412	72	24	the	the	DET
cet-14412	72	25	receiving	receive	VERB
cet-14412	72	26	reservoir	reservoir	NOUN
cet-14412	72	27	.	.	PUNCT
cet-14412	73	1	adsorption	adsorption	NOUN
cet-14412	73	2	was	be	AUX
cet-14412	73	3	monitored	monitor	VERB
cet-14412	73	4	over	over	ADP
cet-14412	73	5	time	time	NOUN
cet-14412	73	6	such	such	ADJ
cet-14412	73	7	that	that	SCONJ
cet-14412	73	8	sers	ser	NOUN
cet-14412	73	9	measurements	measurement	NOUN
cet-14412	73	10	were	be	AUX
cet-14412	73	11	taken	take	VERB
cet-14412	73	12	through	through	ADP
cet-14412	73	13	the	the	DET
cet-14412	73	14	air	air	NOUN
cet-14412	73	15	and	and	CCONJ
cet-14412	73	16	aqueous	aqueous	ADJ
cet-14412	73	17	solution	solution	NOUN
cet-14412	73	18	above	above	ADP
cet-14412	73	19	the	the	DET
cet-14412	73	20	chip	chip	NOUN
cet-14412	73	21	.	.	PUNCT
cet-14412	74	1	the	the	DET
cet-14412	74	2	sers	ser	NOUN
cet-14412	74	3	spectra	spectra	PROPN
cet-14412	74	4	were	be	AUX
cet-14412	74	5	collected	collect	VERB
cet-14412	74	6	using	use	VERB
cet-14412	74	7	a	a	DET
cet-14412	74	8	horiba	horiba	PROPN
cet-14412	74	9	-	-	PUNCT
cet-14412	74	10	jobin	jobin	PROPN
cet-14412	74	11	yvon	yvon	PROPN
cet-14412	74	12	raman	raman	PROPN
cet-14412	74	13	spectrometer	spectrometer	NOUN
cet-14412	74	14	(	(	PUNCT
cet-14412	74	15	model	model	NOUN
cet-14412	74	16	:	:	PUNCT
cet-14412	74	17	labram	labram	PROPN
cet-14412	74	18	)	)	PUNCT
cet-14412	74	19	with	with	ADP
cet-14412	74	20	a	a	DET
cet-14412	74	21	632.8	632.8	NUM
cet-14412	74	22	nm	nm	NOUN
cet-14412	74	23	he	he	PRON
cet-14412	74	24	/	/	SYM
cet-14412	74	25	ne	ne	PROPN
cet-14412	74	26	laser	laser	NOUN
cet-14412	74	27	(	(	PUNCT
cet-14412	74	28	17	17	NUM
cet-14412	74	29	mw	mw	NOUN
cet-14412	74	30	)	)	PUNCT
cet-14412	74	31	,	,	PUNCT
cet-14412	74	32	1800	1800	NUM
cet-14412	74	33	l	l	NOUN
cet-14412	74	34	mm-1	mm-1	PUNCT
cet-14412	74	35	grating	grate	VERB
cet-14412	74	36	and	and	CCONJ
cet-14412	74	37	an	an	DET
cet-14412	74	38	olympus	olympus	PROPN
cet-14412	74	39	bx-41	bx-41	PRON
cet-14412	74	40	microscope	microscope	NOUN
cet-14412	74	41	system	system	NOUN
cet-14412	74	42	.	.	PUNCT
cet-14412	75	1	the	the	DET
cet-14412	75	2	spectra	spectra	NOUN
cet-14412	75	3	were	be	AUX
cet-14412	75	4	measured	measure	VERB
cet-14412	75	5	with	with	ADP
cet-14412	75	6	10x	10x	NOUN
cet-14412	75	7	microscope	microscope	NOUN
cet-14412	75	8	objective	objective	NOUN
cet-14412	75	9	for	for	ADP
cet-14412	75	10	3x5	3x5	NUM
cet-14412	75	11	s	s	NOUN
cet-14412	75	12	for	for	ADP
cet-14412	75	13	each	each	DET
cet-14412	75	14	measurement	measurement	NOUN
cet-14412	75	15	.	.	PUNCT
cet-14412	76	1	a	a	DET
cet-14412	76	2	background	background	NOUN
cet-14412	76	3	baseline	baseline	NOUN
cet-14412	76	4	correction	correction	NOUN
cet-14412	76	5	and	and	CCONJ
cet-14412	76	6	savitsky	savitsky	NOUN
cet-14412	76	7	-	-	PUNCT
cet-14412	76	8	golay	golay	NOUN
cet-14412	76	9	filter	filter	NOUN
cet-14412	76	10	was	be	AUX
cet-14412	76	11	applied	apply	VERB
cet-14412	76	12	to	to	ADP
cet-14412	76	13	all	all	DET
cet-14412	76	14	spectral	spectral	ADJ
cet-14412	76	15	data	datum	NOUN
cet-14412	76	16	using	use	VERB
cet-14412	76	17	matlab	matlab	PROPN
cet-14412	76	18	.	.	PUNCT
cet-14412	77	1	adsorption	adsorption	NOUN
cet-14412	77	2	isotherm	isotherm	NOUN
cet-14412	77	3	model	model	NOUN
cet-14412	77	4	fitting	fitting	ADJ
cet-14412	77	5	was	be	AUX
cet-14412	77	6	also	also	ADV
cet-14412	77	7	performed	perform	VERB
cet-14412	77	8	using	use	VERB
cet-14412	77	9	an	an	DET
cet-14412	77	10	open	open	ADJ
cet-14412	77	11	-	-	PUNCT
cet-14412	77	12	source	source	NOUN
cet-14412	77	13	matlab	matlab	PROPN
cet-14412	77	14	code11	code11	X
cet-14412	77	15	.	.	PUNCT
cet-14412	78	1	3	3	X
cet-14412	78	2	.	.	NOUN
cet-14412	78	3	results	result	NOUN
cet-14412	78	4	and	and	CCONJ
cet-14412	78	5	discussion	discussion	NOUN
cet-14412	78	6	to	to	PART
cet-14412	78	7	be	be	AUX
cet-14412	78	8	able	able	ADJ
cet-14412	78	9	to	to	PART
cet-14412	78	10	quantify	quantify	VERB
cet-14412	78	11	the	the	DET
cet-14412	78	12	concentration	concentration	NOUN
cet-14412	78	13	of	of	ADP
cet-14412	78	14	adsorbed	adsorb	VERB
cet-14412	78	15	r6	r6	NOUN
cet-14412	78	16	g	g	PROPN
cet-14412	78	17	on	on	ADP
cet-14412	78	18	the	the	DET
cet-14412	78	19	sers	ser	NOUN
cet-14412	78	20	substrate	substrate	NOUN
cet-14412	78	21	,	,	PUNCT
cet-14412	78	22	an	an	DET
cet-14412	78	23	adsorption	adsorption	NOUN
cet-14412	78	24	isotherm	isotherm	NOUN
cet-14412	78	25	was	be	AUX
cet-14412	78	26	first	first	ADV
cet-14412	78	27	created	create	VERB
cet-14412	78	28	that	that	PRON
cet-14412	78	29	correlates	correlate	VERB
cet-14412	78	30	the	the	DET
cet-14412	78	31	amount	amount	NOUN
cet-14412	78	32	of	of	ADP
cet-14412	78	33	r6	r6	NOUN
cet-14412	78	34	g	g	PROPN
cet-14412	78	35	(	(	PUNCT
cet-14412	78	36	moles	mole	NOUN
cet-14412	78	37	m-2	m-2	NOUN
cet-14412	78	38	)	)	PUNCT
cet-14412	78	39	adsorbed	adsorb	VERB
cet-14412	78	40	on	on	ADP
cet-14412	78	41	the	the	DET
cet-14412	78	42	agnp	agnp	NOUN
cet-14412	78	43	to	to	ADP
cet-14412	78	44	the	the	DET
cet-14412	78	45	concentration	concentration	NOUN
cet-14412	78	46	of	of	ADP
cet-14412	78	47	r6	r6	NOUN
cet-14412	78	48	g	g	NOUN
cet-14412	78	49	in	in	ADP
cet-14412	78	50	solution	solution	NOUN
cet-14412	78	51	(	(	PUNCT
cet-14412	78	52	moles	mole	NOUN
cet-14412	78	53	l-1	l-1	NUM
cet-14412	78	54	)	)	PUNCT
cet-14412	78	55	at	at	ADP
cet-14412	78	56	equilibrium	equilibrium	NOUN
cet-14412	78	57	.	.	PUNCT
cet-14412	79	1	this	this	DET
cet-14412	79	2	correlation	correlation	NOUN
cet-14412	79	3	is	be	AUX
cet-14412	79	4	subsequently	subsequently	ADV
cet-14412	79	5	used	use	VERB
cet-14412	79	6	to	to	PART
cet-14412	79	7	link	link	VERB
cet-14412	79	8	the	the	DET
cet-14412	79	9	sers	ser	NOUN
cet-14412	79	10	signal	signal	PROPN
cet-14412	79	11	intensity	intensity	NOUN
cet-14412	79	12	to	to	ADP
cet-14412	79	13	the	the	DET
cet-14412	79	14	concentration	concentration	NOUN
cet-14412	79	15	of	of	ADP
cet-14412	79	16	adsorbed	adsorb	VERB
cet-14412	79	17	r6	r6	PROPN
cet-14412	79	18	g	g	NOUN
cet-14412	79	19	,	,	PUNCT
cet-14412	79	20	as	as	SCONJ
cet-14412	79	21	described	describe	VERB
cet-14412	79	22	below	below	ADV
cet-14412	79	23	.	.	PUNCT
cet-14412	80	1	this	this	PRON
cet-14412	80	2	is	be	AUX
cet-14412	80	3	possible	possible	ADJ
cet-14412	80	4	due	due	ADP
cet-14412	80	5	to	to	ADP
cet-14412	80	6	the	the	DET
cet-14412	80	7	unique	unique	ADJ
cet-14412	80	8	advantage	advantage	NOUN
cet-14412	80	9	of	of	ADP
cet-14412	80	10	the	the	DET
cet-14412	80	11	present	present	ADJ
cet-14412	80	12	sers	ser	NOUN
cet-14412	80	13	substrate	substrate	NOUN
cet-14412	80	14	fabrication	fabrication	NOUN
cet-14412	80	15	technique	technique	NOUN
cet-14412	80	16	,	,	PUNCT
cet-14412	80	17	namely	namely	ADV
cet-14412	80	18	,	,	PUNCT
cet-14412	80	19	the	the	DET
cet-14412	80	20	agnps	agnps	PROPN
cet-14412	80	21	used	use	VERB
cet-14412	80	22	for	for	ADP
cet-14412	80	23	constructing	construct	VERB
cet-14412	80	24	the	the	DET
cet-14412	80	25	adsorption	adsorption	NOUN
cet-14412	80	26	isotherm	isotherm	NOUN
cet-14412	80	27	also	also	ADV
cet-14412	80	28	serve	serve	VERB
cet-14412	80	29	as	as	ADP
cet-14412	80	30	building	build	VERB
cet-14412	80	31	blocks	block	NOUN
cet-14412	80	32	of	of	ADP
cet-14412	80	33	the	the	DET
cet-14412	80	34	dendritic	dendritic	ADJ
cet-14412	80	35	sers	ser	NOUN
cet-14412	80	36	.	.	PUNCT
cet-14412	81	1	fig	fig	NOUN
cet-14412	81	2	.	.	PUNCT
cet-14412	82	1	1c	1c	NOUN
cet-14412	82	2	is	be	AUX
cet-14412	82	3	a	a	DET
cet-14412	82	4	top	top	ADJ
cet-14412	82	5	-	-	PUNCT
cet-14412	82	6	down	down	ADP
cet-14412	82	7	microscope	microscope	NOUN
cet-14412	82	8	image	image	NOUN
cet-14412	82	9	of	of	ADP
cet-14412	82	10	the	the	DET
cet-14412	82	11	dendritic	dendritic	ADJ
cet-14412	82	12	substrates	substrate	NOUN
cet-14412	82	13	formed	form	VERB
cet-14412	82	14	in	in	ADP
cet-14412	82	15	the	the	DET
cet-14412	82	16	gaps	gap	NOUN
cet-14412	82	17	between	between	ADP
cet-14412	82	18	planar	planar	ADJ
cet-14412	82	19	microelectrodes	microelectrode	NOUN
cet-14412	82	20	using	use	VERB
cet-14412	82	21	our	our	PRON
cet-14412	82	22	electric	electric	ADJ
cet-14412	82	23	field	field	NOUN
cet-14412	82	24	-	-	PUNCT
cet-14412	82	25	guided	guide	VERB
cet-14412	82	26	agnp	agnp	NOUN
cet-14412	82	27	assembly	assembly	NOUN
cet-14412	82	28	technique	technique	NOUN
cet-14412	82	29	,	,	PUNCT
cet-14412	82	30	while	while	SCONJ
cet-14412	82	31	fig	fig	NOUN
cet-14412	82	32	.	.	PUNCT
cet-14412	83	1	1d	1d	NUM
cet-14412	83	2	is	be	AUX
cet-14412	83	3	an	an	DET
cet-14412	83	4	sem	sem	NOUN
cet-14412	83	5	image	image	NOUN
cet-14412	83	6	showing	show	VERB
cet-14412	83	7	details	detail	NOUN
cet-14412	83	8	of	of	ADP
cet-14412	83	9	that	that	DET
cet-14412	83	10	sers	ser	NOUN
cet-14412	83	11	-	-	PUNCT
cet-14412	83	12	active	active	ADJ
cet-14412	83	13	agnp	agnp	NOUN
cet-14412	83	14	structure	structure	NOUN
cet-14412	83	15	.	.	PUNCT
cet-14412	84	1	the	the	DET
cet-14412	84	2	enhancement	enhancement	NOUN
cet-14412	84	3	factor	factor	NOUN
cet-14412	84	4	provided	provide	VERB
cet-14412	84	5	by	by	ADP
cet-14412	84	6	these	these	DET
cet-14412	84	7	ag	ag	PROPN
cet-14412	84	8	dendritic	dendritic	ADJ
cet-14412	84	9	substrates	substrate	NOUN
cet-14412	84	10	was	be	AUX
cet-14412	84	11	found	find	VERB
cet-14412	84	12	to	to	PART
cet-14412	84	13	be	be	AUX
cet-14412	84	14	equal	equal	ADJ
cet-14412	84	15	to	to	ADP
cet-14412	84	16	4x105	4x105	NUM
cet-14412	84	17	(	(	PUNCT
cet-14412	84	18	dies	die	VERB
cet-14412	84	19	et	et	PROPN
cet-14412	84	20	al	al	PROPN
cet-14412	84	21	.	.	PROPN
cet-14412	84	22	,	,	PUNCT
cet-14412	84	23	2017	2017	NUM
cet-14412	84	24	)	)	PUNCT
cet-14412	84	25	.	.	PUNCT
cet-14412	85	1	a	a	DET
cet-14412	85	2	step	step	NOUN
cet-14412	85	3	-	-	PUNCT
cet-14412	85	4	by	by	ADP
cet-14412	85	5	-	-	PUNCT
cet-14412	85	6	step	step	NOUN
cet-14412	85	7	presentation	presentation	NOUN
cet-14412	85	8	of	of	ADP
cet-14412	85	9	the	the	DET
cet-14412	85	10	method	method	NOUN
cet-14412	85	11	that	that	PRON
cet-14412	85	12	allows	allow	VERB
cet-14412	85	13	quantification	quantification	NOUN
cet-14412	85	14	of	of	ADP
cet-14412	85	15	adsorbed	adsorb	VERB
cet-14412	85	16	r6	r6	NOUN
cet-14412	85	17	g	g	PROPN
cet-14412	85	18	is	be	AUX
cet-14412	85	19	described	describe	VERB
cet-14412	85	20	below	below	ADV
cet-14412	85	21	.	.	PUNCT
cet-14412	86	1	construction	construction	NOUN
cet-14412	86	2	of	of	ADP
cet-14412	86	3	the	the	DET
cet-14412	86	4	r6	r6	NOUN
cet-14412	86	5	g	g	PROPN
cet-14412	86	6	adsorption	adsorption	NOUN
cet-14412	86	7	isotherm	isotherm	NOUN
cet-14412	86	8	.	.	PUNCT
cet-14412	87	1	first	first	ADV
cet-14412	87	2	,	,	PUNCT
cet-14412	87	3	a	a	DET
cet-14412	87	4	calibration	calibration	NOUN
cet-14412	87	5	curve	curve	NOUN
cet-14412	87	6	for	for	ADP
cet-14412	87	7	measuring	measure	VERB
cet-14412	87	8	the	the	DET
cet-14412	87	9	concentration	concentration	NOUN
cet-14412	87	10	of	of	ADP
cet-14412	87	11	r6	r6	NOUN
cet-14412	87	12	g	g	PROPN
cet-14412	87	13	in	in	ADP
cet-14412	87	14	solution	solution	NOUN
cet-14412	87	15	was	be	AUX
cet-14412	87	16	constructed	construct	VERB
cet-14412	87	17	using	use	VERB
cet-14412	87	18	fluorescence	fluorescence	NOUN
cet-14412	87	19	spectroscopy	spectroscopy	NOUN
cet-14412	87	20	.	.	PUNCT
cet-14412	88	1	a	a	DET
cet-14412	88	2	control	control	NOUN
cet-14412	88	3	(	(	PUNCT
cet-14412	88	4	di	di	NOUN
cet-14412	88	5	water	water	NOUN
cet-14412	88	6	)	)	PUNCT
cet-14412	88	7	and	and	CCONJ
cet-14412	88	8	five	five	NUM
cet-14412	88	9	aqueous	aqueous	ADJ
cet-14412	88	10	solutions	solution	NOUN
cet-14412	88	11	of	of	ADP
cet-14412	88	12	r6	r6	NOUN
cet-14412	88	13	g	g	NOUN
cet-14412	88	14	ranging	range	VERB
cet-14412	88	15	in	in	ADP
cet-14412	88	16	concentration	concentration	NOUN
cet-14412	88	17	from	from	ADP
cet-14412	88	18	5	5	NUM
cet-14412	88	19	*	*	SYM
cet-14412	88	20	10	10	NUM
cet-14412	88	21	-	-	SYM
cet-14412	88	22	8	8	NUM
cet-14412	88	23	m	m	NOUN
cet-14412	88	24	to	to	ADP
cet-14412	88	25	5	5	NUM
cet-14412	88	26	*	*	SYM
cet-14412	88	27	10	10	NUM
cet-14412	88	28	-	-	SYM
cet-14412	88	29	6	6	NUM
cet-14412	88	30	m	m	NOUN
cet-14412	88	31	were	be	AUX
cet-14412	88	32	used	use	VERB
cet-14412	88	33	for	for	ADP
cet-14412	88	34	the	the	DET
cet-14412	88	35	measurements	measurement	NOUN
cet-14412	88	36	(	(	PUNCT
cet-14412	88	37	fig	fig	NOUN
cet-14412	88	38	.	.	PUNCT
cet-14412	89	1	2a	2a	NUM
cet-14412	89	2	)	)	PUNCT
cet-14412	89	3	.	.	PUNCT
cet-14412	90	1	background	background	NOUN
cet-14412	90	2	noise	noise	NOUN
cet-14412	90	3	correction	correction	NOUN
cet-14412	90	4	and	and	CCONJ
cet-14412	90	5	linear	linear	PROPN
cet-14412	90	6	regression	regression	NOUN
cet-14412	90	7	analyses	analysis	NOUN
cet-14412	90	8	were	be	AUX
cet-14412	90	9	performed	perform	VERB
cet-14412	90	10	on	on	ADP
cet-14412	90	11	the	the	DET
cet-14412	90	12	data	datum	NOUN
cet-14412	90	13	.	.	PUNCT
cet-14412	91	1	data	datum	NOUN
cet-14412	91	2	point	point	NOUN
cet-14412	91	3	regression	regression	NOUN
cet-14412	91	4	produced	produce	VERB
cet-14412	91	5	a	a	DET
cet-14412	91	6	linear	linear	ADJ
cet-14412	91	7	correlation	correlation	NOUN
cet-14412	91	8	(	(	PUNCT
cet-14412	91	9	r2=0.999	r2=0.999	X
cet-14412	91	10	)	)	PUNCT
cet-14412	91	11	.	.	PUNCT
cet-14412	92	1	next	next	ADJ
cet-14412	92	2	,	,	PUNCT
cet-14412	92	3	50	50	NUM
cet-14412	92	4	nm	nm	NOUN
cet-14412	92	5	agnps	agnps	ADJ
cet-14412	92	6	(	(	PUNCT
cet-14412	92	7	concentration	concentration	NOUN
cet-14412	92	8	:	:	PUNCT
cet-14412	92	9	2x1010	2x1010	NUM
cet-14412	92	10	nanoparticles	nanoparticle	NOUN
cet-14412	92	11	/	/	SYM
cet-14412	92	12	ml	ml	ADP
cet-14412	92	13	;	;	PUNCT
cet-14412	92	14	corresponding	correspond	VERB
cet-14412	92	15	surface	surface	NOUN
cet-14412	92	16	area	area	NOUN
cet-14412	92	17	:	:	PUNCT
cet-14412	92	18	2.28	2.28	NUM
cet-14412	92	19	cm2	cm2	NOUN
cet-14412	92	20	/	/	SYM
cet-14412	92	21	ml	ml	VERB
cet-14412	92	22	)	)	PUNCT
cet-14412	92	23	dispersed	disperse	VERB
cet-14412	92	24	into	into	ADP
cet-14412	92	25	the	the	DET
cet-14412	92	26	control	control	NOUN
cet-14412	92	27	and	and	CCONJ
cet-14412	92	28	five	five	NUM
cet-14412	92	29	aqueous	aqueous	ADJ
cet-14412	92	30	solutions	solution	NOUN
cet-14412	92	31	of	of	ADP
cet-14412	92	32	r6	r6	NOUN
cet-14412	92	33	g	g	PROPN
cet-14412	92	34	were	be	AUX
cet-14412	92	35	used	use	VERB
cet-14412	92	36	to	to	PART
cet-14412	92	37	generate	generate	VERB
cet-14412	92	38	the	the	DET
cet-14412	92	39	adsorption	adsorption	NOUN
cet-14412	92	40	isotherm	isotherm	NOUN
cet-14412	92	41	.	.	PUNCT
cet-14412	93	1	in	in	ADP
cet-14412	93	2	each	each	DET
cet-14412	93	3	case	case	NOUN
cet-14412	93	4	,	,	PUNCT
cet-14412	93	5	the	the	DET
cet-14412	93	6	surface	surface	NOUN
cet-14412	93	7	concentration	concentration	NOUN
cet-14412	93	8	(	(	PUNCT
cet-14412	93	9	mole	mole	NOUN
cet-14412	93	10	m-2	m-2	NOUN
cet-14412	93	11	)	)	PUNCT
cet-14412	93	12	of	of	ADP
cet-14412	93	13	r6	r6	PROPN
cet-14412	93	14	g	g	PROPN
cet-14412	93	15	adsorbed	adsorb	VERB
cet-14412	93	16	onto	onto	ADP
cet-14412	93	17	the	the	DET
cet-14412	93	18	agnps	agnps	PROPN
cet-14412	93	19	was	be	AUX
cet-14412	93	20	calculated	calculate	VERB
cet-14412	93	21	by	by	ADP
cet-14412	93	22	concentration	concentration	NOUN
cet-14412	93	23	difference	difference	NOUN
cet-14412	93	24	(	(	PUNCT
cet-14412	93	25	initial	initial	ADJ
cet-14412	93	26	vs.	vs.	X
cet-14412	93	27	equilibrium	equilibrium	NOUN
cet-14412	93	28	)	)	PUNCT
cet-14412	93	29	and	and	CCONJ
cet-14412	93	30	knowledge	knowledge	NOUN
cet-14412	93	31	of	of	ADP
cet-14412	93	32	the	the	DET
cet-14412	93	33	total	total	ADJ
cet-14412	93	34	surface	surface	NOUN
cet-14412	93	35	area	area	NOUN
cet-14412	93	36	provided	provide	VERB
cet-14412	93	37	by	by	ADP
cet-14412	93	38	the	the	DET
cet-14412	93	39	agnps	agnps	PROPN
cet-14412	93	40	.	.	PUNCT
cet-14412	94	1	adsorption	adsorption	NOUN
cet-14412	94	2	equilibrium	equilibrium	NOUN
cet-14412	94	3	was	be	AUX
cet-14412	94	4	assumed	assume	VERB
cet-14412	94	5	to	to	PART
cet-14412	94	6	be	be	AUX
cet-14412	94	7	reached	reach	VERB
cet-14412	94	8	within	within	ADP
cet-14412	94	9	24	24	NUM
cet-14412	94	10	hours	hour	NOUN
cet-14412	94	11	.	.	PUNCT
cet-14412	95	1	after	after	ADP
cet-14412	95	2	allowing	allow	VERB
cet-14412	95	3	24	24	NUM
cet-14412	95	4	hours	hour	NOUN
cet-14412	95	5	for	for	ADP
cet-14412	95	6	r6	r6	NOUN
cet-14412	95	7	g	g	PROPN
cet-14412	95	8	molecules	molecule	NOUN
cet-14412	95	9	to	to	PART
cet-14412	95	10	adsorb	adsorb	VERB
cet-14412	95	11	onto	onto	ADP
cet-14412	95	12	agnps	agnps	NOUN
cet-14412	95	13	in	in	ADP
cet-14412	95	14	the	the	DET
cet-14412	95	15	solution	solution	NOUN
cet-14412	95	16	,	,	PUNCT
cet-14412	95	17	agnps	agnps	PROPN
cet-14412	95	18	were	be	AUX
cet-14412	95	19	centrifuged	centrifuge	VERB
cet-14412	95	20	out	out	ADP
cet-14412	95	21	of	of	ADP
cet-14412	95	22	the	the	DET
cet-14412	95	23	solution	solution	NOUN
cet-14412	95	24	.	.	PUNCT
cet-14412	96	1	fluorescence	fluorescence	NOUN
cet-14412	96	2	spectroscopy	spectroscopy	NOUN
cet-14412	96	3	were	be	AUX
cet-14412	96	4	obtained	obtain	VERB
cet-14412	96	5	for	for	ADP
cet-14412	96	6	the	the	DET
cet-14412	96	7	remaining	remain	VERB
cet-14412	96	8	supernatants	supernatant	NOUN
cet-14412	96	9	of	of	ADP
cet-14412	96	10	each	each	DET
cet-14412	96	11	solution	solution	NOUN
cet-14412	96	12	.	.	PUNCT
cet-14412	97	1	unknown	unknown	ADJ
cet-14412	97	2	concentrations	concentration	NOUN
cet-14412	97	3	of	of	ADP
cet-14412	97	4	supernatant	supernatant	NOUN
cet-14412	97	5	solutions	solution	NOUN
cet-14412	97	6	were	be	AUX
cet-14412	97	7	determined	determine	VERB
cet-14412	97	8	by	by	ADP
cet-14412	97	9	using	use	VERB
cet-14412	97	10	the	the	DET
cet-14412	97	11	calibration	calibration	NOUN
cet-14412	97	12	curve	curve	NOUN
cet-14412	97	13	for	for	ADP
cet-14412	97	14	r6	r6	PROPN
cet-14412	97	15	g	g	PROPN
cet-14412	97	16	(	(	PUNCT
cet-14412	97	17	fig	fig	NOUN
cet-14412	97	18	.	.	PUNCT
cet-14412	97	19	2a	2a	NUM
cet-14412	97	20	)	)	PUNCT
cet-14412	97	21	.	.	PUNCT
cet-14412	98	1	the	the	DET
cet-14412	98	2	concentration	concentration	NOUN
cet-14412	98	3	of	of	ADP
cet-14412	98	4	each	each	DET
cet-14412	98	5	supernatant	supernatant	NOUN
cet-14412	98	6	was	be	AUX
cet-14412	98	7	assumed	assume	VERB
cet-14412	98	8	to	to	PART
cet-14412	98	9	be	be	AUX
cet-14412	98	10	equivalent	equivalent	ADJ
cet-14412	98	11	to	to	ADP
cet-14412	98	12	the	the	DET
cet-14412	98	13	equilibrium	equilibrium	NOUN
cet-14412	98	14	bulk	bulk	ADJ
cet-14412	98	15	concentration	concentration	NOUN
cet-14412	98	16	at	at	ADP
cet-14412	98	17	adsorption	adsorption	NOUN
cet-14412	98	18	equilibrium	equilibrium	NOUN
cet-14412	98	19	.	.	PUNCT
cet-14412	99	1	figure	figure	NOUN
cet-14412	99	2	2b	2b	PROPN
cet-14412	99	3	shows	show	VERB
cet-14412	99	4	the	the	DET
cet-14412	99	5	r6	r6	NOUN
cet-14412	99	6	g	g	NOUN
cet-14412	99	7	adsorption	adsorption	NOUN
cet-14412	99	8	isotherm	isotherm	NOUN
cet-14412	99	9	generated	generate	VERB
cet-14412	99	10	from	from	ADP
cet-14412	99	11	experimental	experimental	ADJ
cet-14412	99	12	data	datum	NOUN
cet-14412	99	13	.	.	PUNCT
cet-14412	100	1	the	the	DET
cet-14412	100	2	r6	r6	PROPN
cet-14412	100	3	g	g	PROPN
cet-14412	100	4	adsorption	adsorption	NOUN
cet-14412	100	5	isotherm	isotherm	NOUN
cet-14412	100	6	was	be	AUX
cet-14412	100	7	fit	fit	ADJ
cet-14412	100	8	with	with	ADP
cet-14412	100	9	a	a	DET
cet-14412	100	10	linear	linear	ADJ
cet-14412	100	11	model	model	NOUN
cet-14412	100	12	.	.	PUNCT
cet-14412	101	1	9	9	NUM
cet-14412	101	2	figure	figure	NOUN
cet-14412	101	3	2	2	NUM
cet-14412	101	4	:	:	PUNCT
cet-14412	101	5	(	(	PUNCT
cet-14412	101	6	a	a	X
cet-14412	101	7	)	)	PUNCT
cet-14412	101	8	calibration	calibration	NOUN
cet-14412	101	9	curves	curve	NOUN
cet-14412	101	10	for	for	ADP
cet-14412	101	11	r6	r6	NOUN
cet-14412	101	12	g	g	NOUN
cet-14412	101	13	in	in	ADP
cet-14412	101	14	solution	solution	NOUN
cet-14412	101	15	;	;	PUNCT
cet-14412	101	16	(	(	PUNCT
cet-14412	101	17	b	b	X
cet-14412	101	18	)	)	PUNCT
cet-14412	101	19	r6	r6	NOUN
cet-14412	101	20	g	g	PROPN
cet-14412	101	21	isotherm	isotherm	NOUN
cet-14412	101	22	correlating	correlate	VERB
cet-14412	101	23	raman	raman	NOUN
cet-14412	101	24	intensity	intensity	NOUN
cet-14412	101	25	and	and	CCONJ
cet-14412	101	26	r6	r6	NOUN
cet-14412	101	27	g	g	NOUN
cet-14412	101	28	adsorption	adsorption	NOUN
cet-14412	101	29	.	.	PUNCT
cet-14412	102	1	the	the	DET
cet-14412	102	2	sers	ser	NOUN
cet-14412	102	3	intensity	intensity	NOUN
cet-14412	102	4	can	can	AUX
cet-14412	102	5	be	be	AUX
cet-14412	102	6	correlated	correlate	VERB
cet-14412	102	7	to	to	ADP
cet-14412	102	8	the	the	DET
cet-14412	102	9	concentration	concentration	NOUN
cet-14412	102	10	of	of	ADP
cet-14412	102	11	analyte	analyte	NOUN
cet-14412	102	12	in	in	ADP
cet-14412	102	13	solution	solution	NOUN
cet-14412	102	14	.	.	PUNCT
cet-14412	103	1	the	the	DET
cet-14412	103	2	raman	raman	ADJ
cet-14412	103	3	spectra	spectra	NOUN
cet-14412	103	4	for	for	ADP
cet-14412	103	5	r6	r6	PROPN
cet-14412	103	6	g	g	PROPN
cet-14412	103	7	has	have	VERB
cet-14412	103	8	several	several	ADJ
cet-14412	103	9	distinct	distinct	ADJ
cet-14412	103	10	,	,	PUNCT
cet-14412	103	11	strong	strong	ADJ
cet-14412	103	12	peaks	peak	NOUN
cet-14412	103	13	from	from	ADP
cet-14412	103	14	which	which	PRON
cet-14412	103	15	intensity	intensity	NOUN
cet-14412	103	16	can	can	AUX
cet-14412	103	17	be	be	AUX
cet-14412	103	18	monitored	monitor	VERB
cet-14412	103	19	.	.	PUNCT
cet-14412	104	1	here	here	ADV
cet-14412	104	2	,	,	PUNCT
cet-14412	104	3	changes	change	NOUN
cet-14412	104	4	in	in	ADP
cet-14412	104	5	the	the	DET
cet-14412	104	6	r6	r6	NOUN
cet-14412	104	7	g	g	PROPN
cet-14412	104	8	spectrum	spectrum	NOUN
cet-14412	104	9	intensity	intensity	NOUN
cet-14412	104	10	are	be	AUX
cet-14412	104	11	monitored	monitor	VERB
cet-14412	104	12	using	use	VERB
cet-14412	104	13	the	the	DET
cet-14412	104	14	strong	strong	ADJ
cet-14412	104	15	c	c	NOUN
cet-14412	104	16	-	-	PUNCT
cet-14412	104	17	c	c	NOUN
cet-14412	104	18	in	in	ADP
cet-14412	104	19	-	-	PUNCT
cet-14412	104	20	plane	plane	NOUN
cet-14412	104	21	bending	bending	NOUN
cet-14412	104	22	peak	peak	NOUN
cet-14412	104	23	at	at	ADP
cet-14412	104	24	612	612	NUM
cet-14412	104	25	cm-1	cm-1	NOUN
cet-14412	104	26	.	.	PUNCT
cet-14412	105	1	a	a	DET
cet-14412	105	2	calibration	calibration	NOUN
cet-14412	105	3	curve	curve	NOUN
cet-14412	105	4	following	follow	VERB
cet-14412	105	5	this	this	DET
cet-14412	105	6	characteristic	characteristic	ADJ
cet-14412	105	7	peak	peak	NOUN
cet-14412	105	8	intensity	intensity	NOUN
cet-14412	105	9	was	be	AUX
cet-14412	105	10	constructed	construct	VERB
cet-14412	105	11	using	use	VERB
cet-14412	105	12	sers	ser	NOUN
cet-14412	105	13	spectroscopy	spectroscopy	VERB
cet-14412	105	14	for	for	ADP
cet-14412	105	15	five	five	NUM
cet-14412	105	16	aqueous	aqueous	ADJ
cet-14412	105	17	solutions	solution	NOUN
cet-14412	105	18	of	of	ADP
cet-14412	105	19	r6	r6	NOUN
cet-14412	105	20	g	g	NOUN
cet-14412	105	21	ranging	range	VERB
cet-14412	105	22	in	in	ADP
cet-14412	105	23	concentration	concentration	NOUN
cet-14412	105	24	from	from	ADP
cet-14412	105	25	5	5	NUM
cet-14412	105	26	*	*	SYM
cet-14412	105	27	10	10	NUM
cet-14412	105	28	-	-	SYM
cet-14412	105	29	8	8	NUM
cet-14412	105	30	m	m	NOUN
cet-14412	105	31	to	to	ADP
cet-14412	105	32	5	5	NUM
cet-14412	105	33	*	*	SYM
cet-14412	105	34	10	10	NUM
cet-14412	105	35	-	-	SYM
cet-14412	105	36	6	6	NUM
cet-14412	105	37	m	m	NOUN
cet-14412	105	38	(	(	PUNCT
cet-14412	105	39	fig	fig	NOUN
cet-14412	105	40	.	.	PUNCT
cet-14412	106	1	3a	3a	NUM
cet-14412	106	2	)	)	PUNCT
cet-14412	106	3	.	.	PUNCT
cet-14412	107	1	a	a	DET
cet-14412	107	2	linear	linear	ADJ
cet-14412	107	3	regression	regression	NOUN
cet-14412	107	4	analysis	analysis	NOUN
cet-14412	107	5	was	be	AUX
cet-14412	107	6	performed	perform	VERB
cet-14412	107	7	on	on	ADP
cet-14412	107	8	the	the	DET
cet-14412	107	9	data	datum	NOUN
cet-14412	107	10	and	and	CCONJ
cet-14412	107	11	the	the	DET
cet-14412	107	12	calibration	calibration	NOUN
cet-14412	107	13	curve	curve	NOUN
cet-14412	107	14	also	also	ADV
cet-14412	107	15	demonstrated	demonstrate	VERB
cet-14412	107	16	a	a	DET
cet-14412	107	17	strong	strong	ADJ
cet-14412	107	18	linear	linear	ADJ
cet-14412	107	19	dependence	dependence	NOUN
cet-14412	107	20	(	(	PUNCT
cet-14412	107	21	r2=0.9868	r2=0.9868	PROPN
cet-14412	107	22	)	)	PUNCT
cet-14412	107	23	.	.	PUNCT
cet-14412	108	1	distribution	distribution	NOUN
cet-14412	108	2	of	of	ADP
cet-14412	108	3	r6	r6	NOUN
cet-14412	108	4	g	g	NOUN
cet-14412	108	5	on	on	ADP
cet-14412	108	6	the	the	DET
cet-14412	108	7	sers	ser	NOUN
cet-14412	108	8	substrate	substrate	NOUN
cet-14412	108	9	through	through	ADP
cet-14412	108	10	adsorption	adsorption	NOUN
cet-14412	108	11	allows	allow	VERB
cet-14412	108	12	for	for	ADP
cet-14412	108	13	correlation	correlation	NOUN
cet-14412	108	14	of	of	ADP
cet-14412	108	15	raman	raman	NOUN
cet-14412	108	16	intensity	intensity	NOUN
cet-14412	108	17	with	with	ADP
cet-14412	108	18	concentration	concentration	NOUN
cet-14412	108	19	of	of	ADP
cet-14412	108	20	r6	r6	NOUN
cet-14412	108	21	g	g	NOUN
cet-14412	108	22	on	on	ADP
cet-14412	108	23	the	the	DET
cet-14412	108	24	sers	ser	NOUN
cet-14412	108	25	substrate	substrate	NOUN
cet-14412	108	26	.	.	PUNCT
cet-14412	109	1	the	the	DET
cet-14412	109	2	experimental	experimental	ADJ
cet-14412	109	3	r6	r6	PROPN
cet-14412	109	4	g	g	PROPN
cet-14412	109	5	adsorption	adsorption	NOUN
cet-14412	109	6	isotherm	isotherm	VERB
cet-14412	109	7	onto	onto	ADP
cet-14412	109	8	agnps	agnps	ADJ
cet-14412	109	9	(	(	PUNCT
cet-14412	109	10	fig	fig	NOUN
cet-14412	109	11	.	.	PUNCT
cet-14412	110	1	3b	3b	NUM
cet-14412	110	2	)	)	PUNCT
cet-14412	110	3	predicts	predict	VERB
cet-14412	110	4	the	the	DET
cet-14412	110	5	concentration	concentration	NOUN
cet-14412	110	6	of	of	ADP
cet-14412	110	7	r6	r6	NOUN
cet-14412	110	8	g	g	PROPN
cet-14412	110	9	that	that	PRON
cet-14412	110	10	will	will	AUX
cet-14412	110	11	be	be	AUX
cet-14412	110	12	adsorbed	adsorb	VERB
cet-14412	110	13	onto	onto	ADP
cet-14412	110	14	an	an	DET
cet-14412	110	15	agnps	agnps	ADJ
cet-14412	110	16	surface	surface	NOUN
cet-14412	110	17	dependent	dependent	ADJ
cet-14412	110	18	on	on	ADP
cet-14412	110	19	bulk	bulk	ADJ
cet-14412	110	20	equilibrium	equilibrium	NOUN
cet-14412	110	21	concentration	concentration	NOUN
cet-14412	110	22	.	.	PUNCT
cet-14412	111	1	the	the	DET
cet-14412	111	2	sers	ser	NOUN
cet-14412	111	3	measurements	measurement	NOUN
cet-14412	111	4	were	be	AUX
cet-14412	111	5	performed	perform	VERB
cet-14412	111	6	after	after	ADP
cet-14412	111	7	equilibrium	equilibrium	NOUN
cet-14412	111	8	has	have	AUX
cet-14412	111	9	been	be	AUX
cet-14412	111	10	reached	reach	VERB
cet-14412	111	11	between	between	ADP
cet-14412	111	12	r6	r6	NOUN
cet-14412	111	13	g	g	NOUN
cet-14412	111	14	molecules	molecule	NOUN
cet-14412	111	15	and	and	CCONJ
cet-14412	111	16	the	the	DET
cet-14412	111	17	agnp	agnp	NOUN
cet-14412	111	18	substrate	substrate	NOUN
cet-14412	111	19	.	.	PUNCT
cet-14412	112	1	through	through	ADP
cet-14412	112	2	this	this	DET
cet-14412	112	3	assumption	assumption	NOUN
cet-14412	112	4	,	,	PUNCT
cet-14412	112	5	sers	ser	NOUN
cet-14412	112	6	signal	signal	PROPN
cet-14412	112	7	intensities	intensity	NOUN
cet-14412	112	8	measured	measure	VERB
cet-14412	112	9	for	for	ADP
cet-14412	112	10	known	know	VERB
cet-14412	112	11	initial	initial	ADJ
cet-14412	112	12	bulk	bulk	ADJ
cet-14412	112	13	r6	r6	NOUN
cet-14412	112	14	g	g	NOUN
cet-14412	112	15	concentrations	concentration	NOUN
cet-14412	112	16	can	can	AUX
cet-14412	112	17	be	be	AUX
cet-14412	112	18	correlated	correlate	VERB
cet-14412	112	19	to	to	ADP
cet-14412	112	20	the	the	DET
cet-14412	112	21	adsorbed	adsorb	VERB
cet-14412	112	22	r6	r6	NOUN
cet-14412	112	23	g	g	PROPN
cet-14412	112	24	concentrations	concentration	NOUN
cet-14412	112	25	for	for	ADP
cet-14412	112	26	the	the	DET
cet-14412	112	27	same	same	ADJ
cet-14412	112	28	known	know	VERB
cet-14412	112	29	initial	initial	ADJ
cet-14412	112	30	bulk	bulk	ADJ
cet-14412	112	31	r6	r6	NOUN
cet-14412	112	32	g	g	NOUN
cet-14412	112	33	concentrations	concentration	NOUN
cet-14412	112	34	.	.	PUNCT
cet-14412	113	1	figure	figure	NOUN
cet-14412	113	2	3b	3b	NOUN
cet-14412	113	3	demonstrates	demonstrate	VERB
cet-14412	113	4	the	the	DET
cet-14412	113	5	direct	direct	ADJ
cet-14412	113	6	correlation	correlation	NOUN
cet-14412	113	7	of	of	ADP
cet-14412	113	8	r6	r6	NOUN
cet-14412	113	9	g	g	PROPN
cet-14412	113	10	adsorbed	adsorb	VERB
cet-14412	113	11	concentration	concentration	NOUN
cet-14412	113	12	versus	versus	ADP
cet-14412	113	13	raman	raman	NOUN
cet-14412	113	14	intensity	intensity	NOUN
cet-14412	113	15	.	.	PUNCT
cet-14412	114	1	the	the	DET
cet-14412	114	2	regressed	regress	VERB
cet-14412	114	3	data	datum	NOUN
cet-14412	114	4	in	in	ADP
cet-14412	114	5	figure	figure	NOUN
cet-14412	114	6	3b	3b	NOUN
cet-14412	114	7	show	show	VERB
cet-14412	114	8	a	a	DET
cet-14412	114	9	linear	linear	ADJ
cet-14412	114	10	correlation	correlation	NOUN
cet-14412	114	11	(	(	PUNCT
cet-14412	114	12	r2=0.9911	r2=0.9911	PROPN
cet-14412	114	13	)	)	PUNCT
cet-14412	114	14	and	and	CCONJ
cet-14412	114	15	validates	validate	VERB
cet-14412	114	16	its	its	PRON
cet-14412	114	17	use	use	NOUN
cet-14412	114	18	in	in	ADP
cet-14412	114	19	determining	determine	VERB
cet-14412	114	20	the	the	DET
cet-14412	114	21	concentration	concentration	NOUN
cet-14412	114	22	of	of	ADP
cet-14412	114	23	r6	r6	NOUN
cet-14412	114	24	g	g	PROPN
cet-14412	114	25	adsorbed	adsorb	VERB
cet-14412	114	26	on	on	ADP
cet-14412	114	27	the	the	DET
cet-14412	114	28	surface	surface	NOUN
cet-14412	114	29	of	of	ADP
cet-14412	114	30	sers	ser	NOUN
cet-14412	114	31	substrates	substrate	NOUN
cet-14412	114	32	from	from	ADP
cet-14412	114	33	raman	raman	NOUN
cet-14412	114	34	intensity	intensity	NOUN
cet-14412	114	35	values	value	NOUN
cet-14412	114	36	.	.	PUNCT
cet-14412	115	1	figure	figure	VERB
cet-14412	115	2	3	3	NUM
cet-14412	115	3	:	:	PUNCT
cet-14412	115	4	(	(	PUNCT
cet-14412	115	5	a	a	X
cet-14412	115	6	)	)	PUNCT
cet-14412	115	7	r6	r6	NOUN
cet-14412	115	8	g	g	PROPN
cet-14412	115	9	sers	ser	NOUN
cet-14412	115	10	intensity	intensity	NOUN
cet-14412	115	11	(	(	PUNCT
cet-14412	115	12	612	612	NUM
cet-14412	115	13	cm-1	cm-1	NOUN
cet-14412	115	14	peak	peak	NOUN
cet-14412	115	15	)	)	PUNCT
cet-14412	115	16	vs.	vs.	ADP
cet-14412	115	17	r6	r6	NOUN
cet-14412	115	18	g	g	NOUN
cet-14412	115	19	in	in	ADP
cet-14412	115	20	solution	solution	NOUN
cet-14412	115	21	;	;	PUNCT
cet-14412	115	22	(	(	PUNCT
cet-14412	115	23	b	b	X
cet-14412	115	24	)	)	PUNCT
cet-14412	115	25	correlation	correlation	NOUN
cet-14412	115	26	between	between	ADP
cet-14412	115	27	sers	ser	NOUN
cet-14412	115	28	signal	signal	PROPN
cet-14412	115	29	intensity	intensity	NOUN
cet-14412	115	30	(	(	PUNCT
cet-14412	115	31	612	612	NUM
cet-14412	115	32	cm-1	cm-1	NOUN
cet-14412	115	33	peak	peak	NOUN
cet-14412	115	34	)	)	PUNCT
cet-14412	115	35	and	and	CCONJ
cet-14412	115	36	adsorbed	adsorb	VERB
cet-14412	115	37	r6	r6	PROPN
cet-14412	115	38	g.	g.	PROPN
cet-14412	115	39	kinetics	kinetic	NOUN
cet-14412	115	40	of	of	ADP
cet-14412	115	41	r6	r6	NOUN
cet-14412	115	42	g	g	NOUN
cet-14412	115	43	adsorption	adsorption	NOUN
cet-14412	115	44	.	.	PUNCT
cet-14412	116	1	figure	figure	NOUN
cet-14412	116	2	4	4	NUM
cet-14412	116	3	shows	show	VERB
cet-14412	116	4	an	an	DET
cet-14412	116	5	example	example	NOUN
cet-14412	116	6	of	of	ADP
cet-14412	116	7	how	how	SCONJ
cet-14412	116	8	the	the	DET
cet-14412	116	9	progression	progression	NOUN
cet-14412	116	10	of	of	ADP
cet-14412	116	11	r6	r6	NOUN
cet-14412	116	12	g	g	NOUN
cet-14412	116	13	adsorption	adsorption	NOUN
cet-14412	116	14	onto	onto	ADP
cet-14412	116	15	the	the	DET
cet-14412	116	16	sers	ser	NOUN
cet-14412	116	17	substrate	substrate	NOUN
cet-14412	116	18	can	can	AUX
cet-14412	116	19	be	be	AUX
cet-14412	116	20	monitored	monitor	VERB
cet-14412	116	21	by	by	ADP
cet-14412	116	22	recording	record	VERB
cet-14412	116	23	the	the	DET
cet-14412	116	24	intensity	intensity	NOUN
cet-14412	116	25	of	of	ADP
cet-14412	116	26	the	the	DET
cet-14412	116	27	sers	ser	NOUN
cet-14412	116	28	spectra	spectra	PROPN
cet-14412	116	29	.	.	PUNCT
cet-14412	117	1	the	the	DET
cet-14412	117	2	complete	complete	ADJ
cet-14412	117	3	set	set	NOUN
cet-14412	117	4	of	of	ADP
cet-14412	117	5	results	result	NOUN
cet-14412	117	6	from	from	ADP
cet-14412	117	7	this	this	DET
cet-14412	117	8	study	study	NOUN
cet-14412	117	9	are	be	AUX
cet-14412	117	10	presented	present	VERB
cet-14412	117	11	in	in	ADP
cet-14412	117	12	fig	fig	NOUN
cet-14412	117	13	.	.	PUNCT
cet-14412	118	1	5	5	X
cet-14412	118	2	.	.	PUNCT
cet-14412	118	3	sers	ser	NOUN
cet-14412	118	4	substrates	substrate	NOUN
cet-14412	118	5	were	be	AUX
cet-14412	118	6	exposed	expose	VERB
cet-14412	118	7	to	to	ADP
cet-14412	118	8	aqueous	aqueous	ADJ
cet-14412	118	9	solutions	solution	NOUN
cet-14412	118	10	of	of	ADP
cet-14412	118	11	r6	r6	NOUN
cet-14412	118	12	g	g	NOUN
cet-14412	118	13	at	at	ADP
cet-14412	118	14	initial	initial	ADJ
cet-14412	118	15	bulk	bulk	ADJ
cet-14412	118	16	concentrations	concentration	NOUN
cet-14412	118	17	of	of	ADP
cet-14412	118	18	5	5	NUM
cet-14412	118	19	*	*	SYM
cet-14412	118	20	10	10	NUM
cet-14412	118	21	-	-	SYM
cet-14412	118	22	7	7	NUM
cet-14412	118	23	m	m	NOUN
cet-14412	118	24	,	,	PUNCT
cet-14412	118	25	1	1	NUM
cet-14412	118	26	*	*	SYM
cet-14412	118	27	10	10	NUM
cet-14412	118	28	-	-	SYM
cet-14412	118	29	6	6	NUM
cet-14412	118	30	m	m	NOUN
cet-14412	118	31	and	and	CCONJ
cet-14412	118	32	5	5	NUM
cet-14412	118	33	*	*	NUM
cet-14412	118	34	10	10	NUM
cet-14412	118	35	-	-	SYM
cet-14412	118	36	6	6	NUM
cet-14412	118	37	m.	m.	NOUN
cet-14412	118	38	adsorption	adsorption	NOUN
cet-14412	118	39	kinetics	kinetic	NOUN
cet-14412	118	40	of	of	ADP
cet-14412	118	41	r6	r6	PROPN
cet-14412	118	42	g	g	PROPN
cet-14412	118	43	onto	onto	ADP
cet-14412	118	44	sers	ser	NOUN
cet-14412	118	45	substrates	substrate	NOUN
cet-14412	118	46	were	be	AUX
cet-14412	118	47	studied	study	VERB
cet-14412	118	48	to	to	PART
cet-14412	118	49	determine	determine	VERB
cet-14412	118	50	adsorption	adsorption	NOUN
cet-14412	118	51	times	time	NOUN
cet-14412	118	52	and	and	CCONJ
cet-14412	118	53	final	final	ADJ
cet-14412	118	54	plateau	plateau	NOUN
cet-14412	118	55	intensities	intensity	NOUN
cet-14412	118	56	.	.	PUNCT
cet-14412	119	1	plateau	plateau	NOUN
cet-14412	119	2	intensities	intensity	NOUN
cet-14412	119	3	were	be	AUX
cet-14412	119	4	reached	reach	VERB
cet-14412	119	5	at	at	ADP
cet-14412	119	6	different	different	ADJ
cet-14412	119	7	times	time	NOUN
cet-14412	119	8	depending	depend	VERB
cet-14412	119	9	on	on	ADP
cet-14412	119	10	solution	solution	NOUN
cet-14412	119	11	concentration	concentration	NOUN
cet-14412	119	12	.	.	PUNCT
cet-14412	120	1	this	this	PRON
cet-14412	120	2	was	be	AUX
cet-14412	120	3	expected	expect	VERB
cet-14412	120	4	as	as	SCONJ
cet-14412	120	5	the	the	DET
cet-14412	120	6	rate	rate	NOUN
cet-14412	120	7	of	of	ADP
cet-14412	120	8	this	this	DET
cet-14412	120	9	phenomenon	phenomenon	NOUN
cet-14412	120	10	is	be	AUX
cet-14412	120	11	mass	mass	NOUN
cet-14412	120	12	transferred	transfer	VERB
cet-14412	120	13	controlled	control	VERB
cet-14412	120	14	,	,	PUNCT
cet-14412	120	15	meaning	mean	VERB
cet-14412	120	16	that	that	SCONJ
cet-14412	120	17	higher	high	ADJ
cet-14412	120	18	rates	rate	NOUN
cet-14412	120	19	of	of	ADP
cet-14412	120	20	adsorption	adsorption	NOUN
cet-14412	120	21	for	for	ADP
cet-14412	120	22	the	the	DET
cet-14412	120	23	same	same	ADJ
cet-14412	120	24	molecule	molecule	NOUN
cet-14412	120	25	should	should	AUX
cet-14412	120	26	be	be	AUX
cet-14412	120	27	expected	expect	VERB
cet-14412	120	28	at	at	ADP
cet-14412	120	29	higher	high	ADJ
cet-14412	120	30	bulk	bulk	ADJ
cet-14412	120	31	concentrations	concentration	NOUN
cet-14412	120	32	.	.	PUNCT
cet-14412	121	1	as	as	SCONJ
cet-14412	121	2	can	can	AUX
cet-14412	121	3	be	be	AUX
cet-14412	121	4	seen	see	VERB
cet-14412	121	5	,	,	PUNCT
cet-14412	121	6	the	the	DET
cet-14412	121	7	plateau	plateau	NOUN
cet-14412	121	8	value	value	NOUN
cet-14412	121	9	takes	take	VERB
cet-14412	121	10	longer	long	ADV
cet-14412	121	11	to	to	PART
cet-14412	121	12	be	be	AUX
cet-14412	121	13	reached	reach	VERB
cet-14412	121	14	at	at	ADP
cet-14412	121	15	lower	low	ADJ
cet-14412	121	16	bulk	bulk	ADJ
cet-14412	121	17	concentrations	concentration	NOUN
cet-14412	121	18	.	.	PUNCT
cet-14412	122	1	although	although	SCONJ
cet-14412	122	2	plateau	plateau	NOUN
cet-14412	122	3	concentrations	concentration	NOUN
cet-14412	122	4	are	be	AUX
cet-14412	122	5	reached	reach	VERB
cet-14412	122	6	within	within	ADP
cet-14412	122	7	about	about	ADP
cet-14412	122	8	2,000	2,000	NUM
cet-14412	122	9	s	s	NOUN
cet-14412	122	10	for	for	ADP
cet-14412	122	11	the	the	DET
cet-14412	122	12	most	most	ADV
cet-14412	122	13	concentrated	concentrated	ADJ
cet-14412	122	14	solutions	solution	NOUN
cet-14412	122	15	,	,	PUNCT
cet-14412	122	16	adsorption	adsorption	NOUN
cet-14412	122	17	still	still	ADV
cet-14412	122	18	appears	appear	VERB
cet-14412	122	19	to	to	PART
cet-14412	122	20	take	take	VERB
cet-14412	122	21	place	place	NOUN
cet-14412	122	22	at	at	ADP
cet-14412	122	23	the	the	DET
cet-14412	122	24	lowest	low	ADJ
cet-14412	122	25	concentration	concentration	NOUN
cet-14412	122	26	.	.	PUNCT
cet-14412	123	1	in	in	ADP
cet-14412	123	2	addition	addition	NOUN
cet-14412	123	3	to	to	ADP
cet-14412	123	4	allowing	allow	VERB
cet-14412	123	5	us	we	PRON
cet-14412	123	6	to	to	PART
cet-14412	123	7	measure	measure	VERB
cet-14412	123	8	10	10	NUM
cet-14412	123	9	the	the	DET
cet-14412	123	10	actual	actual	ADJ
cet-14412	123	11	kinetics	kinetic	NOUN
cet-14412	123	12	of	of	ADP
cet-14412	123	13	the	the	DET
cet-14412	123	14	adsorption	adsorption	NOUN
cet-14412	123	15	process	process	NOUN
cet-14412	123	16	,	,	PUNCT
cet-14412	123	17	these	these	DET
cet-14412	123	18	measurements	measurement	NOUN
cet-14412	123	19	also	also	ADV
cet-14412	123	20	give	give	VERB
cet-14412	123	21	us	we	PRON
cet-14412	123	22	an	an	DET
cet-14412	123	23	indication	indication	NOUN
cet-14412	123	24	of	of	ADP
cet-14412	123	25	the	the	DET
cet-14412	123	26	wait	wait	NOUN
cet-14412	123	27	times	time	NOUN
cet-14412	123	28	that	that	PRON
cet-14412	123	29	need	need	VERB
cet-14412	123	30	to	to	PART
cet-14412	123	31	be	be	AUX
cet-14412	123	32	observed	observe	VERB
cet-14412	123	33	in	in	ADP
cet-14412	123	34	in	in	ADP
cet-14412	123	35	situ	situ	ADJ
cet-14412	123	36	measurements	measurement	NOUN
cet-14412	123	37	for	for	ADP
cet-14412	123	38	obtaining	obtain	VERB
cet-14412	123	39	an	an	DET
cet-14412	123	40	accurate	accurate	ADJ
cet-14412	123	41	reading	reading	NOUN
cet-14412	123	42	that	that	PRON
cet-14412	123	43	corresponds	correspond	VERB
cet-14412	123	44	to	to	ADP
cet-14412	123	45	the	the	DET
cet-14412	123	46	equilibrium	equilibrium	NOUN
cet-14412	123	47	value	value	NOUN
cet-14412	123	48	.	.	PUNCT
cet-14412	124	1	if	if	SCONJ
cet-14412	124	2	measurements	measurement	NOUN
cet-14412	124	3	are	be	AUX
cet-14412	124	4	taken	take	VERB
cet-14412	124	5	too	too	ADV
cet-14412	124	6	fast	fast	ADV
cet-14412	124	7	,	,	PUNCT
cet-14412	124	8	this	this	PRON
cet-14412	124	9	will	will	AUX
cet-14412	124	10	result	result	VERB
cet-14412	124	11	in	in	ADP
cet-14412	124	12	false	false	ADJ
cet-14412	124	13	concentration	concentration	NOUN
cet-14412	124	14	readings	reading	NOUN
cet-14412	124	15	.	.	PUNCT
cet-14412	125	1	our	our	PRON
cet-14412	125	2	observed	observed	ADJ
cet-14412	125	3	time	time	NOUN
cet-14412	125	4	scales	scale	NOUN
cet-14412	125	5	agree	agree	VERB
cet-14412	125	6	with	with	ADP
cet-14412	125	7	other	other	ADJ
cet-14412	125	8	researchers	researcher	NOUN
cet-14412	125	9	(	(	PUNCT
cet-14412	125	10	tripathi	tripathi	NOUN
cet-14412	125	11	et	et	PROPN
cet-14412	125	12	al	al	PROPN
cet-14412	125	13	.	.	PROPN
cet-14412	125	14	,	,	PUNCT
cet-14412	125	15	2015	2015	NUM
cet-14412	125	16	)	)	PUNCT
cet-14412	125	17	who	who	PRON
cet-14412	125	18	performed	perform	VERB
cet-14412	125	19	similar	similar	ADJ
cet-14412	125	20	adsorption	adsorption	NOUN
cet-14412	125	21	measurements	measurement	NOUN
cet-14412	125	22	on	on	ADP
cet-14412	125	23	a	a	DET
cet-14412	125	24	different	different	ADJ
cet-14412	125	25	type	type	NOUN
cet-14412	125	26	of	of	ADP
cet-14412	125	27	sers	ser	NOUN
cet-14412	125	28	-	-	ADJ
cet-14412	125	29	active	active	ADJ
cet-14412	125	30	substrates	substrate	NOUN
cet-14412	125	31	for	for	ADP
cet-14412	125	32	numerous	numerous	ADJ
cet-14412	125	33	chemical	chemical	ADJ
cet-14412	125	34	compounds	compound	NOUN
cet-14412	125	35	.	.	PUNCT
cet-14412	126	1	these	these	DET
cet-14412	126	2	researchers	researcher	NOUN
cet-14412	126	3	also	also	ADV
cet-14412	126	4	showed	show	VERB
cet-14412	126	5	that	that	SCONJ
cet-14412	126	6	adsorption	adsorption	NOUN
cet-14412	126	7	isotherms	isotherm	NOUN
cet-14412	126	8	thus	thus	ADV
cet-14412	126	9	constructed	construct	VERB
cet-14412	126	10	can	can	AUX
cet-14412	126	11	yield	yield	VERB
cet-14412	126	12	the	the	DET
cet-14412	126	13	equilibrium	equilibrium	NOUN
cet-14412	126	14	constants	constant	NOUN
cet-14412	126	15	of	of	ADP
cet-14412	126	16	adsorption	adsorption	NOUN
cet-14412	126	17	and	and	CCONJ
cet-14412	126	18	binding	bind	VERB
cet-14412	126	19	energies	energy	NOUN
cet-14412	126	20	of	of	ADP
cet-14412	126	21	the	the	DET
cet-14412	126	22	molecules	molecule	NOUN
cet-14412	126	23	.	.	PUNCT
cet-14412	127	1	figure	figure	VERB
cet-14412	127	2	4	4	NUM
cet-14412	127	3	:	:	PUNCT
cet-14412	127	4	example	example	NOUN
cet-14412	127	5	of	of	ADP
cet-14412	127	6	sers	ser	NOUN
cet-14412	127	7	spectra	spectra	PROPN
cet-14412	127	8	intensity	intensity	PROPN
cet-14412	127	9	change	change	NOUN
cet-14412	127	10	during	during	ADP
cet-14412	127	11	r6	r6	NOUN
cet-14412	127	12	g	g	NOUN
cet-14412	127	13	adsorption	adsorption	NOUN
cet-14412	127	14	(	(	PUNCT
cet-14412	127	15	concentration	concentration	NOUN
cet-14412	127	16	:	:	PUNCT
cet-14412	127	17	5x10	5x10	NUM
cet-14412	127	18	-	-	SYM
cet-14412	127	19	6	6	NUM
cet-14412	127	20	m	m	NOUN
cet-14412	127	21	)	)	PUNCT
cet-14412	127	22	.	.	PUNCT
cet-14412	128	1	figure	figure	VERB
cet-14412	128	2	5	5	NUM
cet-14412	128	3	:	:	PUNCT
cet-14412	128	4	adsorption	adsorption	NOUN
cet-14412	128	5	kinetics	kinetic	NOUN
cet-14412	128	6	of	of	ADP
cet-14412	128	7	r6	r6	PROPN
cet-14412	128	8	g	g	PROPN
cet-14412	128	9	on	on	ADP
cet-14412	128	10	the	the	DET
cet-14412	128	11	silver	silver	ADJ
cet-14412	128	12	sers	ser	NOUN
cet-14412	128	13	-	-	ADJ
cet-14412	128	14	active	active	ADJ
cet-14412	128	15	substrate	substrate	NOUN
cet-14412	128	16	.	.	PUNCT
cet-14412	129	1	(	(	PUNCT
cet-14412	129	2	a	a	X
cet-14412	129	3	)	)	PUNCT
cet-14412	129	4	sers	ser	NOUN
cet-14412	129	5	signal	signal	PROPN
cet-14412	129	6	intensity	intensity	NOUN
cet-14412	129	7	;	;	PUNCT
cet-14412	129	8	(	(	PUNCT
cet-14412	129	9	b	b	X
cet-14412	129	10	)	)	PUNCT
cet-14412	129	11	corresponding	correspond	VERB
cet-14412	129	12	surface	surface	NOUN
cet-14412	129	13	concentration	concentration	NOUN
cet-14412	129	14	of	of	ADP
cet-14412	129	15	adsorbed	adsorb	VERB
cet-14412	129	16	r6	r6	PROPN
cet-14412	129	17	g.	g.	PROPN
cet-14412	129	18	conc	conc	PROPN
cet-14412	129	19	.	.	PUNCT
cet-14412	129	20	:	:	PUNCT
cet-14412	130	1	5x10	5x10	NUM
cet-14412	130	2	-	-	SYM
cet-14412	130	3	7	7	NUM
cet-14412	130	4	m	m	NOUN
cet-14412	130	5	(	(	PUNCT
cet-14412	130	6	•	•	NOUN
cet-14412	130	7	)	)	PUNCT
cet-14412	130	8	,	,	PUNCT
cet-14412	130	9	1x10	1x10	PROPN
cet-14412	130	10	-	-	SYM
cet-14412	130	11	6	6	NUM
cet-14412	130	12	m	m	NOUN
cet-14412	130	13	(	(	PUNCT
cet-14412	130	14	•	•	NOUN
cet-14412	130	15	)	)	PUNCT
cet-14412	130	16	,	,	PUNCT
cet-14412	130	17	5x10	5x10	NUM
cet-14412	130	18	-	-	SYM
cet-14412	130	19	6	6	NUM
cet-14412	130	20	m	m	NOUN
cet-14412	130	21	(	(	PUNCT
cet-14412	130	22	•	•	NOUN
cet-14412	130	23	)	)	PUNCT
cet-14412	130	24	.	.	PUNCT
cet-14412	131	1	the	the	DET
cet-14412	131	2	corresponding	corresponding	ADJ
cet-14412	131	3	concentrations	concentration	NOUN
cet-14412	131	4	of	of	ADP
cet-14412	131	5	r6	r6	NOUN
cet-14412	131	6	g	g	PROPN
cet-14412	131	7	adsorbed	adsorb	VERB
cet-14412	131	8	onto	onto	ADP
cet-14412	131	9	sers	ser	NOUN
cet-14412	131	10	substrate	substrate	NOUN
cet-14412	131	11	as	as	SCONJ
cet-14412	131	12	a	a	DET
cet-14412	131	13	function	function	NOUN
cet-14412	131	14	of	of	ADP
cet-14412	131	15	time	time	NOUN
cet-14412	131	16	can	can	AUX
cet-14412	131	17	be	be	AUX
cet-14412	131	18	calculated	calculate	VERB
cet-14412	131	19	from	from	ADP
cet-14412	131	20	the	the	DET
cet-14412	131	21	experimental	experimental	ADJ
cet-14412	131	22	data	datum	NOUN
cet-14412	131	23	depicted	depict	VERB
cet-14412	131	24	in	in	ADP
cet-14412	131	25	figures	figure	NOUN
cet-14412	131	26	3b	3b	NOUN
cet-14412	131	27	and	and	CCONJ
cet-14412	131	28	5a	5a	NUM
cet-14412	131	29	.	.	PUNCT
cet-14412	132	1	the	the	DET
cet-14412	132	2	kinetics	kinetic	NOUN
cet-14412	132	3	of	of	ADP
cet-14412	132	4	r6	r6	PROPN
cet-14412	132	5	g	g	PROPN
cet-14412	132	6	adsorbed	adsorb	VERB
cet-14412	132	7	onto	onto	ADP
cet-14412	132	8	agnps	agnps	ADJ
cet-14412	132	9	substrates	substrate	NOUN
cet-14412	132	10	in	in	ADP
cet-14412	132	11	figure	figure	NOUN
cet-14412	132	12	5d	5d	PROPN
cet-14412	132	13	illustrates	illustrate	VERB
cet-14412	132	14	the	the	DET
cet-14412	132	15	adsorption	adsorption	NOUN
cet-14412	132	16	rate	rate	NOUN
cet-14412	132	17	upon	upon	SCONJ
cet-14412	132	18	contact	contact	NOUN
cet-14412	132	19	of	of	ADP
cet-14412	132	20	sers	ser	NOUN
cet-14412	132	21	substrates	substrate	NOUN
cet-14412	132	22	with	with	ADP
cet-14412	132	23	sample	sample	NOUN
cet-14412	132	24	solutions	solution	NOUN
cet-14412	132	25	.	.	PUNCT
cet-14412	133	1	knowledge	knowledge	NOUN
cet-14412	133	2	of	of	ADP
cet-14412	133	3	this	this	DET
cet-14412	133	4	phenomenon	phenomenon	NOUN
cet-14412	133	5	over	over	ADP
cet-14412	133	6	time	time	NOUN
cet-14412	133	7	allows	allow	VERB
cet-14412	133	8	for	for	ADP
cet-14412	133	9	a	a	DET
cet-14412	133	10	wider	wide	ADJ
cet-14412	133	11	range	range	NOUN
cet-14412	133	12	of	of	ADP
cet-14412	133	13	application	application	NOUN
cet-14412	133	14	for	for	ADP
cet-14412	133	15	this	this	DET
cet-14412	133	16	sers	ser	NOUN
cet-14412	133	17	detection	detection	NOUN
cet-14412	133	18	method	method	NOUN
cet-14412	133	19	.	.	PUNCT
cet-14412	134	1	adsorption	adsorption	NOUN
cet-14412	134	2	concentration	concentration	NOUN
cet-14412	134	3	as	as	ADP
cet-14412	134	4	a	a	DET
cet-14412	134	5	function	function	NOUN
cet-14412	134	6	of	of	ADP
cet-14412	134	7	time	time	NOUN
cet-14412	134	8	,	,	PUNCT
cet-14412	134	9	figure	figure	NOUN
cet-14412	134	10	5b	5b	NUM
cet-14412	134	11	,	,	PUNCT
cet-14412	134	12	paired	pair	VERB
cet-14412	134	13	with	with	ADP
cet-14412	134	14	sers	ser	NOUN
cet-14412	134	15	intensity	intensity	NOUN
cet-14412	134	16	correlated	correlate	VERB
cet-14412	134	17	to	to	ADP
cet-14412	134	18	adsorption	adsorption	NOUN
cet-14412	134	19	concentration	concentration	NOUN
cet-14412	134	20	,	,	PUNCT
cet-14412	134	21	figure	figure	NOUN
cet-14412	134	22	2a	2a	NUM
cet-14412	134	23	,	,	PUNCT
cet-14412	134	24	shows	show	VERB
cet-14412	134	25	a	a	DET
cet-14412	134	26	potential	potential	ADJ
cet-14412	134	27	method	method	NOUN
cet-14412	134	28	for	for	ADP
cet-14412	134	29	immediate	immediate	ADJ
cet-14412	134	30	analyte	analyte	NOUN
cet-14412	134	31	concentration	concentration	NOUN
cet-14412	134	32	detection	detection	NOUN
cet-14412	134	33	in	in	ADP
cet-14412	134	34	sample	sample	NOUN
cet-14412	134	35	solutions	solution	NOUN
cet-14412	134	36	.	.	PUNCT
cet-14412	135	1	in	in	ADP
cet-14412	135	2	theory	theory	NOUN
cet-14412	135	3	,	,	PUNCT
cet-14412	135	4	the	the	DET
cet-14412	135	5	detection	detection	NOUN
cet-14412	135	6	of	of	ADP
cet-14412	135	7	target	target	NOUN
cet-14412	135	8	molecules	molecule	NOUN
cet-14412	135	9	can	can	AUX
cet-14412	135	10	be	be	AUX
cet-14412	135	11	determined	determine	VERB
cet-14412	135	12	immediately	immediately	ADV
cet-14412	135	13	through	through	ADP
cet-14412	135	14	adsorption	adsorption	NOUN
cet-14412	135	15	kinetics	kinetic	NOUN
cet-14412	135	16	.	.	PUNCT
cet-14412	136	1	however	however	ADV
cet-14412	136	2	,	,	PUNCT
cet-14412	136	3	figure	figure	NOUN
cet-14412	136	4	5b	5b	NOUN
cet-14412	136	5	demonstrates	demonstrate	VERB
cet-14412	136	6	that	that	SCONJ
cet-14412	136	7	quantification	quantification	NOUN
cet-14412	136	8	of	of	ADP
cet-14412	136	9	the	the	DET
cet-14412	136	10	detection	detection	NOUN
cet-14412	136	11	becomes	become	VERB
cet-14412	136	12	more	more	ADV
cet-14412	136	13	accurate	accurate	ADJ
cet-14412	136	14	as	as	SCONJ
cet-14412	136	15	adsorption	adsorption	NOUN
cet-14412	136	16	reaches	reach	VERB
cet-14412	136	17	equilibrium	equilibrium	NOUN
cet-14412	136	18	,	,	PUNCT
cet-14412	136	19	where	where	SCONJ
cet-14412	136	20	error	error	NOUN
cet-14412	136	21	bars	bar	NOUN
cet-14412	136	22	between	between	ADP
cet-14412	136	23	the	the	DET
cet-14412	136	24	three	three	NUM
cet-14412	136	25	concentrations	concentration	NOUN
cet-14412	136	26	show	show	VERB
cet-14412	136	27	greater	great	ADJ
cet-14412	136	28	separation	separation	NOUN
cet-14412	136	29	.	.	PUNCT
cet-14412	137	1	4	4	X
cet-14412	137	2	.	.	X
cet-14412	137	3	conclusions	conclusion	NOUN
cet-14412	137	4	a	a	DET
cet-14412	137	5	microfluidic	microfluidic	ADJ
cet-14412	137	6	device	device	NOUN
cet-14412	137	7	prototype	prototype	NOUN
cet-14412	137	8	was	be	AUX
cet-14412	137	9	developed	develop	VERB
cet-14412	137	10	to	to	PART
cet-14412	137	11	introduce	introduce	VERB
cet-14412	137	12	sample	sample	NOUN
cet-14412	137	13	to	to	ADP
cet-14412	137	14	a	a	DET
cet-14412	137	15	sers	ser	NOUN
cet-14412	137	16	substrate	substrate	NOUN
cet-14412	137	17	in	in	ADP
cet-14412	137	18	a	a	DET
cet-14412	137	19	controlled	control	VERB
cet-14412	137	20	manner	manner	NOUN
cet-14412	137	21	.	.	PUNCT
cet-14412	138	1	an	an	DET
cet-14412	138	2	adsorption	adsorption	NOUN
cet-14412	138	3	isotherm	isotherm	NOUN
cet-14412	138	4	was	be	AUX
cet-14412	138	5	generated	generate	VERB
cet-14412	138	6	for	for	ADP
cet-14412	138	7	r6	r6	NOUN
cet-14412	138	8	g	g	PROPN
cet-14412	138	9	adsorption	adsorption	NOUN
cet-14412	138	10	onto	onto	ADP
cet-14412	138	11	agnps	agnps	NOUN
cet-14412	138	12	by	by	ADP
cet-14412	138	13	using	use	VERB
cet-14412	138	14	fluorescence	fluorescence	NOUN
cet-14412	138	15	spectroscopy	spectroscopy	NOUN
cet-14412	138	16	.	.	PUNCT
cet-14412	139	1	the	the	DET
cet-14412	139	2	amount	amount	NOUN
cet-14412	139	3	of	of	ADP
cet-14412	139	4	r6	r6	NOUN
cet-14412	139	5	g	g	PROPN
cet-14412	139	6	adsorbed	adsorb	VERB
cet-14412	139	7	onto	onto	ADP
cet-14412	139	8	a	a	DET
cet-14412	139	9	known	know	VERB
cet-14412	139	10	surface	surface	NOUN
cet-14412	139	11	area	area	NOUN
cet-14412	139	12	of	of	ADP
cet-14412	139	13	agnps	agnps	PROPN
cet-14412	139	14	at	at	ADP
cet-14412	139	15	equilibrium	equilibrium	NOUN
cet-14412	139	16	was	be	AUX
cet-14412	139	17	determined	determine	VERB
cet-14412	139	18	and	and	CCONJ
cet-14412	139	19	an	an	DET
cet-14412	139	20	adsorption	adsorption	NOUN
cet-14412	139	21	isotherm	isotherm	NOUN
cet-14412	139	22	was	be	AUX
cet-14412	139	23	generated	generate	VERB
cet-14412	139	24	by	by	ADP
cet-14412	139	25	estimating	estimate	VERB
cet-14412	139	26	bulk	bulk	ADJ
cet-14412	139	27	r6	r6	NOUN
cet-14412	139	28	g	g	NOUN
cet-14412	139	29	concentration	concentration	NOUN
cet-14412	139	30	at	at	ADP
cet-14412	139	31	equilibrium	equilibrium	NOUN
cet-14412	139	32	through	through	ADP
cet-14412	139	33	deduction	deduction	NOUN
cet-14412	139	34	.	.	PUNCT
cet-14412	140	1	for	for	ADP
cet-14412	140	2	the	the	DET
cet-14412	140	3	range	range	NOUN
cet-14412	140	4	of	of	ADP
cet-14412	140	5	concentrations	concentration	NOUN
cet-14412	140	6	used	use	VERB
cet-14412	140	7	,	,	PUNCT
cet-14412	140	8	the	the	DET
cet-14412	140	9	adsorption	adsorption	NOUN
cet-14412	140	10	isotherm	isotherm	NOUN
cet-14412	140	11	was	be	AUX
cet-14412	140	12	given	give	VERB
cet-14412	140	13	a	a	DET
cet-14412	140	14	linear	linear	ADJ
cet-14412	140	15	fit	fit	NOUN
cet-14412	140	16	.	.	PUNCT
cet-14412	141	1	however	however	ADV
cet-14412	141	2	,	,	PUNCT
cet-14412	141	3	more	more	ADJ
cet-14412	141	4	data	datum	NOUN
cet-14412	141	5	must	must	AUX
cet-14412	141	6	be	be	AUX
cet-14412	141	7	gathered	gather	VERB
cet-14412	141	8	to	to	PART
cet-14412	141	9	confirm	confirm	VERB
cet-14412	141	10	whether	whether	SCONJ
cet-14412	141	11	:	:	PUNCT
cet-14412	141	12	(	(	PUNCT
cet-14412	141	13	1	1	X
cet-14412	141	14	)	)	PUNCT
cet-14412	141	15	the	the	DET
cet-14412	141	16	fit	fit	NOUN
cet-14412	141	17	is	be	AUX
cet-14412	141	18	linear	linear	ADJ
cet-14412	141	19	and	and	CCONJ
cet-14412	141	20	represents	represent	VERB
cet-14412	141	21	the	the	DET
cet-14412	141	22	linear	linear	ADJ
cet-14412	141	23	region	region	NOUN
cet-14412	141	24	of	of	ADP
cet-14412	141	25	a	a	DET
cet-14412	141	26	langmuir	langmuir	PROPN
cet-14412	141	27	isotherm	isotherm	PROPN
cet-14412	141	28	;	;	PUNCT
cet-14412	141	29	(	(	PUNCT
cet-14412	141	30	2	2	X
cet-14412	141	31	)	)	PUNCT
cet-14412	141	32	the	the	DET
cet-14412	141	33	fit	fit	NOUN
cet-14412	141	34	is	be	AUX
cet-14412	141	35	not	not	PART
cet-14412	141	36	linear	linear	ADJ
cet-14412	141	37	,	,	PUNCT
cet-14412	141	38	and	and	CCONJ
cet-14412	141	39	a	a	DET
cet-14412	141	40	full	full	ADJ
cet-14412	141	41	langmuir	langmuir	PROPN
cet-14412	141	42	isotherm	isotherm	PROPN
cet-14412	141	43	is	be	AUX
cet-14412	141	44	seen	see	VERB
cet-14412	141	45	within	within	ADP
cet-14412	141	46	this	this	DET
cet-14412	141	47	region	region	NOUN
cet-14412	141	48	of	of	ADP
cet-14412	141	49	concentrations	concentration	NOUN
cet-14412	141	50	.	.	PUNCT
cet-14412	142	1	the	the	DET
cet-14412	142	2	adsorption	adsorption	NOUN
cet-14412	142	3	kinetics	kinetic	NOUN
cet-14412	142	4	of	of	ADP
cet-14412	142	5	r6	r6	PROPN
cet-14412	142	6	g	g	PROPN
cet-14412	142	7	onto	onto	ADP
cet-14412	142	8	agnps	agnps	PROPN
cet-14412	142	9	was	be	AUX
cet-14412	142	10	studied	study	VERB
cet-14412	142	11	using	use	VERB
cet-14412	142	12	raman	raman	NOUN
cet-14412	142	13	intensities	intensity	NOUN
cet-14412	142	14	over	over	ADP
cet-14412	142	15	time	time	NOUN
cet-14412	142	16	.	.	PUNCT
cet-14412	143	1	using	use	VERB
cet-14412	143	2	a	a	DET
cet-14412	143	3	series	series	NOUN
cet-14412	143	4	of	of	ADP
cet-14412	143	5	analytical	analytical	ADJ
cet-14412	143	6	steps	step	NOUN
cet-14412	143	7	,	,	PUNCT
cet-14412	143	8	sers	ser	NOUN
cet-14412	143	9	intensity	intensity	NOUN
cet-14412	143	10	was	be	AUX
cet-14412	143	11	found	find	VERB
cet-14412	143	12	to	to	PART
cet-14412	143	13	have	have	VERB
cet-14412	143	14	a	a	DET
cet-14412	143	15	linear	linear	ADJ
cet-14412	143	16	correlation	correlation	NOUN
cet-14412	143	17	to	to	PART
cet-14412	143	18	adsorbed	adsorb	VERB
cet-14412	143	19	r6	r6	NOUN
cet-14412	143	20	g	g	PROPN
cet-14412	143	21	concentration	concentration	NOUN
cet-14412	143	22	on	on	ADP
cet-14412	143	23	the	the	DET
cet-14412	143	24	surface	surface	NOUN
cet-14412	143	25	of	of	ADP
cet-14412	143	26	sers	ser	NOUN
cet-14412	143	27	11	11	NUM
cet-14412	143	28	substrates	substrate	NOUN
cet-14412	143	29	for	for	ADP
cet-14412	143	30	the	the	DET
cet-14412	143	31	range	range	NOUN
cet-14412	143	32	of	of	ADP
cet-14412	143	33	concentrations	concentration	NOUN
cet-14412	143	34	tested	test	VERB
cet-14412	143	35	(	(	PUNCT
cet-14412	143	36	5	5	NUM
cet-14412	143	37	*	*	SYM
cet-14412	143	38	10	10	NUM
cet-14412	143	39	-	-	SYM
cet-14412	143	40	8	8	NUM
cet-14412	143	41	to	to	PART
cet-14412	143	42	5	5	NUM
cet-14412	143	43	*	*	SYM
cet-14412	143	44	10	10	NUM
cet-14412	143	45	-	-	SYM
cet-14412	143	46	6	6	NUM
cet-14412	143	47	)	)	PUNCT
cet-14412	143	48	.	.	PUNCT
cet-14412	144	1	proof	proof	NOUN
cet-14412	144	2	of	of	ADP
cet-14412	144	3	concept	concept	NOUN
cet-14412	144	4	was	be	AUX
cet-14412	144	5	demonstrated	demonstrate	VERB
cet-14412	144	6	for	for	ADP
cet-14412	144	7	a	a	DET
cet-14412	144	8	new	new	ADJ
cet-14412	144	9	method	method	NOUN
cet-14412	144	10	that	that	PRON
cet-14412	144	11	can	can	AUX
cet-14412	144	12	be	be	AUX
cet-14412	144	13	used	use	VERB
cet-14412	144	14	to	to	PART
cet-14412	144	15	rapidly	rapidly	ADV
cet-14412	144	16	determine	determine	VERB
cet-14412	144	17	the	the	DET
cet-14412	144	18	adsorbed	adsorb	VERB
cet-14412	144	19	concentration	concentration	NOUN
cet-14412	144	20	of	of	ADP
cet-14412	144	21	r6	r6	NOUN
cet-14412	144	22	g	g	NOUN
cet-14412	144	23	on	on	ADP
cet-14412	144	24	the	the	DET
cet-14412	144	25	surface	surface	NOUN
cet-14412	144	26	of	of	ADP
cet-14412	144	27	agnps	agnps	ADJ
cet-14412	144	28	sers	ser	NOUN
cet-14412	144	29	substrates	substrate	NOUN
cet-14412	144	30	and	and	CCONJ
cet-14412	144	31	concentration	concentration	NOUN
cet-14412	144	32	of	of	ADP
cet-14412	144	33	r6	r6	NOUN
cet-14412	144	34	g	g	NOUN
cet-14412	144	35	in	in	ADP
cet-14412	144	36	a	a	DET
cet-14412	144	37	sample	sample	NOUN
cet-14412	144	38	within	within	ADP
cet-14412	144	39	the	the	DET
cet-14412	144	40	order	order	NOUN
cet-14412	144	41	of	of	ADP
cet-14412	144	42	magnitude	magnitude	NOUN
cet-14412	144	43	.	.	PUNCT
cet-14412	145	1	acknowledgements	acknowledgement	NOUN
cet-14412	145	2	the	the	DET
cet-14412	145	3	authors	author	NOUN
cet-14412	145	4	would	would	AUX
cet-14412	145	5	like	like	VERB
cet-14412	145	6	to	to	PART
cet-14412	145	7	thank	thank	VERB
cet-14412	145	8	drs	drs	PROPN
cet-14412	145	9	.	.	PUNCT
cet-14412	146	1	joshua	joshua	PROPN
cet-14412	146	2	raveendran	raveendran	PROPN
cet-14412	146	3	and	and	CCONJ
cet-14412	146	4	hannah	hannah	PROPN
cet-14412	146	5	bacon	bacon	NOUN
cet-14412	146	6	for	for	ADP
cet-14412	146	7	their	their	PRON
cet-14412	146	8	technical	technical	ADJ
cet-14412	146	9	assistance	assistance	NOUN
cet-14412	146	10	and	and	CCONJ
cet-14412	146	11	canada	canada	PROPN
cet-14412	146	12	foundation	foundation	PROPN
cet-14412	146	13	for	for	ADP
cet-14412	146	14	innovation	innovation	NOUN
cet-14412	146	15	for	for	ADP
cet-14412	146	16	the	the	DET
cet-14412	146	17	support	support	NOUN
cet-14412	146	18	though	though	SCONJ
cet-14412	146	19	the	the	DET
cet-14412	146	20	john	john	PROPN
cet-14412	146	21	r.	r.	PROPN
cet-14412	146	22	evans	evans	PROPN
cet-14412	146	23	leaders	leaders	PROPN
cet-14412	146	24	fund	fund	PROPN
cet-14412	146	25	.	.	PUNCT
cet-14412	147	1	references	reference	NOUN
cet-14412	147	2	andreou	andreou	PROPN
cet-14412	147	3	c.	c.	PROPN
cet-14412	147	4	,	,	PUNCT
cet-14412	147	5	hoonejani	hoonejani	PROPN
cet-14412	147	6	m.r	m.r	PROPN
cet-14412	147	7	.	.	PROPN
cet-14412	147	8	,	,	PUNCT
cet-14412	147	9	barmi	barmi	PROPN
cet-14412	147	10	m.r	m.r	PROPN
cet-14412	147	11	.	.	PROPN
cet-14412	147	12	,	,	PUNCT
cet-14412	147	13	moskovits	moskovits	PROPN
cet-14412	147	14	m.	m.	NOUN
cet-14412	147	15	,	,	PUNCT
cet-14412	147	16	meinhart	meinhart	NOUN
cet-14412	147	17	c.d	c.d	PROPN
cet-14412	147	18	.	.	PROPN
cet-14412	147	19	,	,	PUNCT
cet-14412	147	20	2013	2013	NUM
cet-14412	147	21	,	,	PUNCT
cet-14412	147	22	rapid	rapid	ADJ
cet-14412	147	23	detection	detection	NOUN
cet-14412	147	24	of	of	ADP
cet-14412	147	25	drugs	drug	NOUN
cet-14412	147	26	of	of	ADP
cet-14412	147	27	abuse	abuse	NOUN
cet-14412	147	28	in	in	ADP
cet-14412	147	29	saliva	saliva	NOUN
cet-14412	147	30	using	use	VERB
cet-14412	147	31	surface	surface	NOUN
cet-14412	147	32	enhanced	enhance	VERB
cet-14412	147	33	raman	raman	NOUN
cet-14412	147	34	spectroscopy	spectroscopy	NOUN
cet-14412	147	35	and	and	CCONJ
cet-14412	147	36	microfluidics	microfluidic	NOUN
cet-14412	147	37	,	,	PUNCT
cet-14412	147	38	acs	acs	PROPN
cet-14412	147	39	nano	nano	NOUN
cet-14412	147	40	,	,	PUNCT
cet-14412	147	41	7:8	7:8	NUM
cet-14412	147	42	,	,	PUNCT
cet-14412	147	43	71577164	71577164	NUM
cet-14412	147	44	.	.	PUNCT
cet-14412	148	1	doi:10.1021	doi:10.1021	PROPN
cet-14412	148	2	/	/	SYM
cet-14412	148	3	nn402563f	nn402563f	PROPN
cet-14412	148	4	.	.	PUNCT
cet-14412	148	5	bacon	bacon	PROPN
cet-14412	148	6	,	,	PUNCT
cet-14412	148	7	h.	h.	PROPN
cet-14412	148	8	,	,	PUNCT
cet-14412	148	9	docoslis	docoslis	PROPN
cet-14412	148	10	,	,	PUNCT
cet-14412	148	11	a.	a.	PROPN
cet-14412	148	12	,	,	PUNCT
cet-14412	148	13	escobedo	escobedo	PROPN
cet-14412	148	14	c.	c.	PROPN
cet-14412	148	15	,	,	PUNCT
cet-14412	148	16	2022	2022	NUM
cet-14412	148	17	,	,	PUNCT
cet-14412	148	18	reconfigurable	reconfigurable	ADJ
cet-14412	148	19	surface	surface	NOUN
cet-14412	148	20	enhanced	enhance	VERB
cet-14412	148	21	raman	raman	NOUN
cet-14412	148	22	spectroscopy	spectroscopy	NOUN
cet-14412	148	23	device	device	NOUN
cet-14412	148	24	and	and	CCONJ
cet-14412	148	25	method	method	NOUN
cet-14412	148	26	therefor	therefor	ADV
cet-14412	148	27	,	,	PUNCT
cet-14412	148	28	us	us	PROPN
cet-14412	148	29	patent	patent	NOUN
cet-14412	148	30	11,237,112	11,237,112	NUM
cet-14412	148	31	.	.	PUNCT
cet-14412	149	1	dies	die	VERB
cet-14412	149	2	h.	h.	PROPN
cet-14412	149	3	,	,	PUNCT
cet-14412	149	4	raveendran	raveendran	PROPN
cet-14412	149	5	j.	j.	PROPN
cet-14412	149	6	,	,	PUNCT
cet-14412	149	7	escobedo	escobedo	PROPN
cet-14412	149	8	c.	c.	PROPN
cet-14412	149	9	,	,	PUNCT
cet-14412	149	10	docoslis	docoslis	PROPN
cet-14412	149	11	a.	a.	PROPN
cet-14412	149	12	,	,	PUNCT
cet-14412	149	13	2017	2017	NUM
cet-14412	149	14	,	,	PUNCT
cet-14412	149	15	in	in	ADP
cet-14412	149	16	situ	situ	ADJ
cet-14412	149	17	assembly	assembly	NOUN
cet-14412	149	18	of	of	ADP
cet-14412	149	19	active	active	ADJ
cet-14412	149	20	surface	surface	NOUN
cet-14412	149	21	-	-	PUNCT
cet-14412	149	22	enhanced	enhance	VERB
cet-14412	149	23	raman	raman	NOUN
cet-14412	149	24	scattering	scattering	NOUN
cet-14412	149	25	substrates	substrate	NOUN
cet-14412	149	26	via	via	ADP
cet-14412	149	27	electric	electric	ADJ
cet-14412	149	28	field	field	NOUN
cet-14412	149	29	-	-	PUNCT
cet-14412	149	30	guided	guide	VERB
cet-14412	149	31	growth	growth	NOUN
cet-14412	149	32	of	of	ADP
cet-14412	149	33	dendritic	dendritic	ADJ
cet-14412	149	34	nanoparticle	nanoparticle	NOUN
cet-14412	149	35	structures	structure	NOUN
cet-14412	149	36	,	,	PUNCT
cet-14412	149	37	nanoscale	nanoscale	NOUN
cet-14412	149	38	,	,	PUNCT
cet-14412	149	39	9:23	9:23	NUM
cet-14412	149	40	,	,	PUNCT
cet-14412	149	41	7847	7847	NUM
cet-14412	149	42	-	-	SYM
cet-14412	149	43	7857	7857	NUM
cet-14412	149	44	.	.	PUNCT
cet-14412	150	1	doi:10.1039	doi:10.1039	NOUN
cet-14412	150	2	/	/	SYM
cet-14412	150	3	c7nr01743j	c7nr01743j	PROPN
cet-14412	150	4	.	.	PROPN
cet-14412	150	5	dies	die	VERB
cet-14412	150	6	h.	h.	PROPN
cet-14412	150	7	,	,	PUNCT
cet-14412	150	8	siampani	siampani	PROPN
cet-14412	150	9	m.	m.	PROPN
cet-14412	150	10	,	,	PUNCT
cet-14412	150	11	escobedo	escobedo	PROPN
cet-14412	150	12	c.	c.	PROPN
cet-14412	150	13	,	,	PUNCT
cet-14412	150	14	docoslis	docoslis	PROPN
cet-14412	150	15	a.	a.	PROPN
cet-14412	150	16	,	,	PUNCT
cet-14412	150	17	2018	2018	NUM
cet-14412	150	18	,	,	PUNCT
cet-14412	150	19	direct	direct	ADJ
cet-14412	150	20	detection	detection	NOUN
cet-14412	150	21	of	of	ADP
cet-14412	150	22	toxic	toxic	ADJ
cet-14412	150	23	contaminants	contaminant	NOUN
cet-14412	150	24	in	in	ADP
cet-14412	150	25	minimally	minimally	ADV
cet-14412	150	26	processed	process	VERB
cet-14412	150	27	food	food	NOUN
cet-14412	150	28	products	product	NOUN
cet-14412	150	29	using	use	VERB
cet-14412	150	30	dendritic	dendritic	ADJ
cet-14412	150	31	surface	surface	NOUN
cet-14412	150	32	-	-	PUNCT
cet-14412	150	33	enhanced	enhance	VERB
cet-14412	150	34	raman	raman	NOUN
cet-14412	150	35	scattering	scattering	NOUN
cet-14412	150	36	substrates	substrate	NOUN
cet-14412	150	37	,	,	PUNCT
cet-14412	150	38	sensors	sensor	NOUN
cet-14412	150	39	,	,	PUNCT
cet-14412	150	40	18:8	18:8	NUM
cet-14412	150	41	,	,	PUNCT
cet-14412	150	42	2726	2726	NUM
cet-14412	150	43	.	.	PUNCT
cet-14412	151	1	doi.org/10.3390/s18082726	doi.org/10.3390/s18082726	X
cet-14412	151	2	.	.	PUNCT
cet-14412	151	3	juncker	juncker	PROPN
cet-14412	151	4	d.	d.	PROPN
cet-14412	151	5	,	,	PUNCT
cet-14412	151	6	schmid	schmid	PROPN
cet-14412	151	7	h.	h.	PROPN
cet-14412	151	8	,	,	PUNCT
cet-14412	151	9	drechsler	drechsler	NOUN
cet-14412	151	10	,	,	PUNCT
cet-14412	151	11	u.	u.	PROPN
cet-14412	151	12	,	,	PUNCT
cet-14412	151	13	wolf	wolf	PROPN
cet-14412	151	14	,	,	PUNCT
cet-14412	151	15	h.	h.	PROPN
cet-14412	151	16	,	,	PUNCT
cet-14412	151	17	wolf	wolf	PROPN
cet-14412	151	18	,	,	PUNCT
cet-14412	151	19	m.	m.	NOUN
cet-14412	151	20	,	,	PUNCT
cet-14412	151	21	michel	michel	PROPN
cet-14412	151	22	,	,	PUNCT
cet-14412	151	23	b.	b.	PROPN
cet-14412	151	24	,	,	PUNCT
cet-14412	151	25	de	de	X
cet-14412	151	26	rooij	rooij	PROPN
cet-14412	151	27	,	,	PUNCT
cet-14412	151	28	n.	n.	NOUN
cet-14412	151	29	,	,	PUNCT
cet-14412	151	30	delamarche	delamarche	PROPN
cet-14412	151	31	,	,	PUNCT
cet-14412	151	32	e.	e.	PROPN
cet-14412	151	33	,	,	PUNCT
cet-14412	151	34	2002	2002	NUM
cet-14412	151	35	,	,	PUNCT
cet-14412	151	36	autonomous	autonomous	ADJ
cet-14412	151	37	microfluidic	microfluidic	ADJ
cet-14412	151	38	capillary	capillary	ADJ
cet-14412	151	39	system	system	NOUN
cet-14412	151	40	,	,	PUNCT
cet-14412	151	41	analytical	analytical	ADJ
cet-14412	151	42	chemistry	chemistry	NOUN
cet-14412	151	43	,	,	PUNCT
cet-14412	151	44	74	74	NUM
cet-14412	151	45	,	,	PUNCT
cet-14412	151	46	24	24	NUM
cet-14412	151	47	,	,	PUNCT
cet-14412	151	48	6139	6139	NUM
cet-14412	151	49	-	-	SYM
cet-14412	151	50	6144	6144	NUM
cet-14412	151	51	.	.	PUNCT
cet-14412	152	1	doi:10.1021	doi:10.1021	ADJ
cet-14412	152	2	/	/	SYM
cet-14412	152	3	ac0261449	ac0261449	PROPN
cet-14412	152	4	kong	kong	PROPN
cet-14412	152	5	x.	x.	PROPN
cet-14412	152	6	,	,	PUNCT
cet-14412	152	7	chong	chong	PROPN
cet-14412	152	8	x.	x.	PROPN
cet-14412	152	9	,	,	PUNCT
cet-14412	152	10	squire	squire	PROPN
cet-14412	152	11	k.	k.	PROPN
cet-14412	152	12	,	,	PUNCT
cet-14412	152	13	wang	wang	PROPN
cet-14412	152	14	a.x	a.x	PROPN
cet-14412	152	15	.	.	PROPN
cet-14412	152	16	,	,	PUNCT
cet-14412	152	17	2018	2018	NUM
cet-14412	152	18	,	,	PUNCT
cet-14412	152	19	microfluidic	microfluidic	ADJ
cet-14412	152	20	diatomite	diatomite	ADJ
cet-14412	152	21	analytical	analytical	ADJ
cet-14412	152	22	devices	device	NOUN
cet-14412	152	23	for	for	ADP
cet-14412	152	24	illicit	illicit	ADJ
cet-14412	152	25	drug	drug	NOUN
cet-14412	152	26	sensing	sense	VERB
cet-14412	152	27	with	with	ADP
cet-14412	152	28	ppb	ppb	NOUN
cet-14412	152	29	-	-	PUNCT
cet-14412	152	30	level	level	NOUN
cet-14412	152	31	sensitivity	sensitivity	NOUN
cet-14412	152	32	,	,	PUNCT
cet-14412	152	33	sensors	sensor	NOUN
cet-14412	152	34	and	and	CCONJ
cet-14412	152	35	actuators	actuator	NOUN
cet-14412	152	36	b	b	X
cet-14412	152	37	:	:	PUNCT
cet-14412	152	38	chemical	chemical	NOUN
cet-14412	152	39	,	,	PUNCT
cet-14412	152	40	15:259	15:259	NUM
cet-14412	152	41	,	,	PUNCT
cet-14412	152	42	587	587	NUM
cet-14412	152	43	-	-	SYM
cet-14412	152	44	595	595	NUM
cet-14412	152	45	.	.	PUNCT
cet-14412	153	1	doi.org/10.1016/j.snb.2017.12.038	doi.org/10.1016/j.snb.2017.12.038	PROPN
cet-14412	153	2	.	.	PUNCT
cet-14412	154	1	maria	maria	PROPN
cet-14412	154	2	m.s	m.s	PROPN
cet-14412	154	3	.	.	PROPN
cet-14412	154	4	,	,	PUNCT
cet-14412	154	5	rakesh	rakesh	PROPN
cet-14412	154	6	p.e	p.e	PROPN
cet-14412	154	7	.	.	PROPN
cet-14412	154	8	,	,	PUNCT
cet-14412	154	9	chandra	chandra	PROPN
cet-14412	154	10	t.s	t.s	PROPN
cet-14412	154	11	.	.	PROPN
cet-14412	154	12	,	,	PUNCT
cet-14412	154	13	sen	sen	PROPN
cet-14412	154	14	a.k	a.k	PROPN
cet-14412	154	15	.	.	PROPN
cet-14412	154	16	,	,	PUNCT
cet-14412	154	17	2017	2017	NUM
cet-14412	154	18	,	,	PUNCT
cet-14412	154	19	capillary	capillary	ADJ
cet-14412	154	20	flowdriven	flowdriven	NOUN
cet-14412	154	21	microfluidic	microfluidic	ADJ
cet-14412	154	22	device	device	NOUN
cet-14412	154	23	with	with	ADP
cet-14412	154	24	wettability	wettability	NOUN
cet-14412	154	25	gradient	gradient	NOUN
cet-14412	154	26	and	and	CCONJ
cet-14412	154	27	sedimentation	sedimentation	NOUN
cet-14412	154	28	effects	effect	NOUN
cet-14412	154	29	for	for	ADP
cet-14412	154	30	blood	blood	NOUN
cet-14412	154	31	plasma	plasma	NOUN
cet-14412	154	32	separation	separation	NOUN
cet-14412	154	33	,	,	PUNCT
cet-14412	154	34	scientific	scientific	ADJ
cet-14412	154	35	reports	report	NOUN
cet-14412	154	36	7:43457	7:43457	NUM
cet-14412	154	37	.	.	PUNCT
cet-14412	154	38	doi:10.1038	doi:10.1038	NOUN
cet-14412	154	39	/	/	SYM
cet-14412	154	40	srep43457	srep43457	PROPN
cet-14412	154	41	.	.	PUNCT
cet-14412	155	1	raveendran	raveendran	PROPN
cet-14412	155	2	j.	j.	PROPN
cet-14412	155	3	,	,	PUNCT
cet-14412	155	4	docoslis	docoslis	PROPN
cet-14412	155	5	,	,	PUNCT
cet-14412	155	6	a.	a.	NOUN
cet-14412	155	7	,	,	PUNCT
cet-14412	155	8	2021	2021	NUM
cet-14412	155	9	,	,	PUNCT
cet-14412	155	10	detection	detection	NOUN
cet-14412	155	11	and	and	CCONJ
cet-14412	155	12	quantification	quantification	NOUN
cet-14412	155	13	of	of	ADP
cet-14412	155	14	toxicants	toxicant	NOUN
cet-14412	155	15	in	in	ADP
cet-14412	155	16	food	food	NOUN
cet-14412	155	17	and	and	CCONJ
cet-14412	155	18	water	water	NOUN
cet-14412	155	19	using	use	VERB
cet-14412	155	20	ag	ag	PROPN
cet-14412	155	21	–	–	PUNCT
cet-14412	155	22	au	au	ADV
cet-14412	155	23	core	core	NOUN
cet-14412	155	24	-	-	PUNCT
cet-14412	155	25	shell	shell	NOUN
cet-14412	155	26	fractal	fractal	ADJ
cet-14412	155	27	sers	ser	NOUN
cet-14412	155	28	nanostructures	nanostructure	NOUN
cet-14412	155	29	and	and	CCONJ
cet-14412	155	30	multivariate	multivariate	NOUN
cet-14412	155	31	analysis	analysis	NOUN
cet-14412	155	32	,	,	PUNCT
cet-14412	155	33	talanta	talanta	ADJ
cet-14412	155	34	,	,	PUNCT
cet-14412	155	35	231	231	NUM
cet-14412	155	36	,	,	PUNCT
cet-14412	155	37	122383	122383	NUM
cet-14412	155	38	.	.	PUNCT
cet-14412	156	1	doi.org/10.1016/j.talanta.2021.122383	doi.org/10.1016/j.talanta.2021.122383	NOUN
cet-14412	156	2	shur	shur	NOUN
cet-14412	156	3	v.	v.	PROPN
cet-14412	156	4	ya	ya	PROPN
cet-14412	156	5	.	.	PUNCT
cet-14412	156	6	et	et	PROPN
cet-14412	157	1	al	al	PROPN
cet-14412	157	2	.	.	PROPN
cet-14412	157	3	,	,	PUNCT
cet-14412	157	4	2015	2015	NUM
cet-14412	157	5	,	,	PUNCT
cet-14412	157	6	coffee	coffee	NOUN
cet-14412	157	7	ring	ring	NOUN
cet-14412	157	8	effect	effect	NOUN
cet-14412	157	9	during	during	ADP
cet-14412	157	10	drying	dry	VERB
cet-14412	157	11	of	of	ADP
cet-14412	157	12	colloid	colloid	NOUN
cet-14412	157	13	drop	drop	NOUN
cet-14412	157	14	:	:	PUNCT
cet-14412	157	15	experiment	experiment	NOUN
cet-14412	157	16	and	and	CCONJ
cet-14412	157	17	computer	computer	NOUN
cet-14412	157	18	simulation	simulation	NOUN
cet-14412	157	19	,	,	PUNCT
cet-14412	157	20	ferroelectrics	ferroelectric	NOUN
cet-14412	157	21	,	,	PUNCT
cet-14412	157	22	476	476	NUM
cet-14412	157	23	,	,	PUNCT
cet-14412	157	24	47	47	NUM
cet-14412	157	25	-	-	SYM
cet-14412	157	26	53	53	NUM
cet-14412	157	27	.	.	PUNCT
cet-14412	158	1	doi:10.1080/00150193.2015.998156	doi:10.1080/00150193.2015.998156	PROPN
cet-14412	158	2	.	.	PUNCT
cet-14412	159	1	tripathi	tripathi	PROPN
cet-14412	159	2	a.	a.	PROPN
cet-14412	159	3	,	,	PUNCT
cet-14412	159	4	emmons	emmons	PROPN
cet-14412	159	5	e.d	e.d	PROPN
cet-14412	159	6	.	.	PROPN
cet-14412	159	7	,	,	PUNCT
cet-14412	159	8	fountain	fountain	PROPN
cet-14412	159	9	a.w	a.w	PROPN
cet-14412	159	10	.	.	PROPN
cet-14412	159	11	,	,	PUNCT
cet-14412	159	12	guicheteau	guicheteau	PROPN
cet-14412	159	13	j.a	j.a	PROPN
cet-14412	159	14	.	.	PROPN
cet-14412	159	15	,	,	PUNCT
cet-14412	159	16	moskovits	moskovits	PROPN
cet-14412	159	17	m.	m.	NOUN
cet-14412	159	18	,	,	PUNCT
cet-14412	159	19	christesen	christesen	PROPN
cet-14412	159	20	s.d	s.d	PROPN
cet-14412	159	21	.	.	PROPN
cet-14412	159	22	,	,	PUNCT
cet-14412	159	23	2015	2015	NUM
cet-14412	159	24	,	,	PUNCT
cet-14412	159	25	critical	critical	ADJ
cet-14412	159	26	role	role	NOUN
cet-14412	159	27	of	of	ADP
cet-14412	159	28	adsorption	adsorption	NOUN
cet-14412	159	29	equilibria	equilibrium	NOUN
cet-14412	159	30	on	on	ADP
cet-14412	159	31	the	the	DET
cet-14412	159	32	determination	determination	NOUN
cet-14412	159	33	of	of	ADP
cet-14412	159	34	surfaceenhanced	surfaceenhanced	ADJ
cet-14412	159	35	raman	raman	NOUN
cet-14412	159	36	enhancement	enhancement	NOUN
cet-14412	159	37	,	,	PUNCT
cet-14412	159	38	acs	acs	PROPN
cet-14412	159	39	nano	nano	NOUN
cet-14412	159	40	,	,	PUNCT
cet-14412	159	41	9:1	9:1	NUM
cet-14412	159	42	,	,	PUNCT
cet-14412	159	43	584	584	NUM
cet-14412	159	44	-	-	SYM
cet-14412	159	45	593	593	NUM
cet-14412	159	46	.	.	PUNCT
cet-14412	160	1	doi:10.1021	doi:10.1021	ADJ
cet-14412	160	2	/	/	SYM
cet-14412	160	3	nn5058936	nn5058936	PROPN
cet-14412	160	4	.	.	PUNCT
cet-14412	160	5	white	white	PROPN
cet-14412	160	6	i.m	i.m	PROPN
cet-14412	160	7	.	.	PROPN
cet-14412	160	8	,	,	PUNCT
cet-14412	160	9	yazdi	yazdi	PROPN
cet-14412	160	10	s.h	s.h	PROPN
cet-14412	160	11	.	.	PROPN
cet-14412	160	12	,	,	PUNCT
cet-14412	160	13	2013	2013	NUM
cet-14412	160	14	,	,	PUNCT
cet-14412	160	15	multiplexed	multiplexed	ADJ
cet-14412	160	16	detection	detection	NOUN
cet-14412	160	17	of	of	ADP
cet-14412	160	18	aquaculture	aquaculture	NOUN
cet-14412	160	19	fungicides	fungicide	NOUN
cet-14412	160	20	using	use	VERB
cet-14412	160	21	a	a	DET
cet-14412	160	22	pump	pump	NOUN
cet-14412	160	23	-	-	PUNCT
cet-14412	160	24	free	free	ADJ
cet-14412	160	25	optofluidic	optofluidic	ADJ
cet-14412	160	26	sers	ser	NOUN
cet-14412	160	27	microsystem	microsystem	PROPN
cet-14412	160	28	,	,	PUNCT
cet-14412	160	29	analyst	analyst	NOUN
cet-14412	160	30	,	,	PUNCT
cet-14412	160	31	138	138	NUM
cet-14412	160	32	,	,	PUNCT
cet-14412	160	33	100	100	NUM
cet-14412	160	34	-	-	SYM
cet-14412	160	35	103	103	NUM
cet-14412	160	36	.	.	PUNCT
cet-14412	161	1	doi:10.1039	doi:10.1039	NOUN
cet-14412	161	2	/	/	PUNCT
cet-14412	162	1	c2an36232e	c2an36232e	PROPN
cet-14412	162	2	wilson	wilson	PROPN
cet-14412	162	3	n.g	n.g	PROPN
cet-14412	162	4	.	.	PROPN
cet-14412	162	5	,	,	PUNCT
cet-14412	162	6	raveendran	raveendran	PROPN
cet-14412	162	7	j.	j.	PROPN
cet-14412	162	8	,	,	PUNCT
cet-14412	162	9	docoslis	docoslis	PROPN
cet-14412	162	10	,	,	PUNCT
cet-14412	162	11	a.	a.	NOUN
cet-14412	162	12	,	,	PUNCT
cet-14412	162	13	2021	2021	NUM
cet-14412	162	14	,	,	PUNCT
cet-14412	162	15	portable	portable	ADJ
cet-14412	162	16	identification	identification	NOUN
cet-14412	162	17	of	of	ADP
cet-14412	162	18	fentanyl	fentanyl	ADJ
cet-14412	162	19	analogues	analogue	NOUN
cet-14412	162	20	in	in	ADP
cet-14412	162	21	drugs	drug	NOUN
cet-14412	162	22	using	use	VERB
cet-14412	162	23	surface	surface	NOUN
cet-14412	162	24	-	-	PUNCT
cet-14412	162	25	enhanced	enhance	VERB
cet-14412	162	26	raman	raman	NOUN
cet-14412	162	27	scattering	scattering	NOUN
cet-14412	162	28	,	,	PUNCT
cet-14412	162	29	sensors	sensor	NOUN
cet-14412	162	30	and	and	CCONJ
cet-14412	162	31	actuators	actuator	NOUN
cet-14412	162	32	b	b	X
cet-14412	162	33	:	:	PUNCT
cet-14412	162	34	chemical	chemical	NOUN
cet-14412	162	35	,	,	PUNCT
cet-14412	162	36	330	330	NUM
cet-14412	162	37	,	,	PUNCT
cet-14412	162	38	129303	129303	NUM
cet-14412	162	39	.	.	PUNCT
cet-14412	163	1	doi.org/10.1016/j.snb.2020.129303	doi.org/10.1016/j.snb.2020.129303	ADJ
cet-14412	163	2	.	.	PROPN
cet-14412	163	3	12	12	NUM
cet-14412	163	4	252docoslis-pagato.pdf	252docoslis-pagato.pdf	NUM
cet-14412	163	5	monitoring	monitoring	NOUN
cet-14412	163	6	adsorption	adsorption	NOUN
cet-14412	163	7	kinetics	kinetic	NOUN
cet-14412	163	8	with	with	ADP
cet-14412	163	9	surface	surface	NOUN
cet-14412	163	10	-	-	PUNCT
cet-14412	163	11	enhanced	enhance	VERB
cet-14412	163	12	raman	raman	NOUN
cet-14412	163	13	scattering	scattering	NOUN
cet-14412	163	14	in	in	ADP
cet-14412	163	15	a	a	DET
cet-14412	163	16	microfluidic	microfluidic	ADJ
cet-14412	163	17	environment	environment	NOUN