id	sid	tid	token	lemma	pos
cet-14418	1	1	doi	doi	NOUN
cet-14418	1	2	:	:	PUNCT
cet-14418	1	3	10.3303	10.3303	NUM
cet-14418	1	4	/	/	SYM
cet-14418	1	5	cet24108008	cet24108008	NOUN
cet-14418	1	6	paper	paper	NOUN
cet-14418	1	7	received	receive	VERB
cet-14418	1	8	:	:	PUNCT
cet-14418	1	9	04	04	NUM
cet-14418	1	10	december	december	PROPN
cet-14418	1	11	2023	2023	NUM
cet-14418	1	12	;	;	PUNCT
cet-14418	1	13	revised	revise	VERB
cet-14418	1	14	:	:	PUNCT
cet-14418	1	15	21	21	NUM
cet-14418	1	16	december	december	PROPN
cet-14418	1	17	2023	2023	NUM
cet-14418	1	18	;	;	PUNCT
cet-14418	1	19	accepted	accept	VERB
cet-14418	1	20	:	:	PUNCT
cet-14418	1	21	19	19	NUM
cet-14418	1	22	january	january	NOUN
cet-14418	1	23	2024	2024	NUM
cet-14418	1	24	please	please	INTJ
cet-14418	1	25	cite	cite	VERB
cet-14418	1	26	this	this	DET
cet-14418	1	27	article	article	NOUN
cet-14418	1	28	as	as	ADP
cet-14418	1	29	:	:	PUNCT
cet-14418	1	30	takagishi	takagishi	PROPN
cet-14418	1	31	y.	y.	PROPN
cet-14418	1	32	,	,	PUNCT
cet-14418	1	33	baba	baba	PROPN
cet-14418	1	34	r.	r.	PROPN
cet-14418	1	35	,	,	PUNCT
cet-14418	1	36	yamashita	yamashita	PROPN
cet-14418	1	37	t.	t.	PROPN
cet-14418	1	38	,	,	PUNCT
cet-14418	1	39	adachi	adachi	PROPN
cet-14418	1	40	w.	w.	PROPN
cet-14418	1	41	,	,	PUNCT
cet-14418	1	42	2024	2024	NUM
cet-14418	1	43	,	,	PUNCT
cet-14418	1	44	multi	multi	ADJ
cet-14418	1	45	-	-	ADJ
cet-14418	1	46	scale	scale	ADJ
cet-14418	1	47	simulations	simulation	NOUN
cet-14418	1	48	in	in	ADP
cet-14418	1	49	a	a	DET
cet-14418	1	50	catalytic	catalytic	ADJ
cet-14418	1	51	reactor	reactor	NOUN
cet-14418	1	52	considering	consider	VERB
cet-14418	1	53	three	three	NUM
cet-14418	1	54	-	-	PUNCT
cet-14418	1	55	dimensional	dimensional	ADJ
cet-14418	1	56	pellet	pellet	NOUN
cet-14418	1	57	geometry	geometry	NOUN
cet-14418	1	58	,	,	PUNCT
cet-14418	1	59	chemical	chemical	NOUN
cet-14418	1	60	engineering	engineering	NOUN
cet-14418	1	61	transactions	transaction	NOUN
cet-14418	1	62	,	,	PUNCT
cet-14418	1	63	108	108	NUM
cet-14418	1	64	,	,	PUNCT
cet-14418	1	65	43	43	NUM
cet-14418	1	66	-	-	SYM
cet-14418	1	67	48	48	NUM
cet-14418	1	68	doi:10.3303	doi:10.3303	NOUN
cet-14418	1	69	/	/	SYM
cet-14418	1	70	cet24108008	cet24108008	NOUN
cet-14418	1	71	chemical	chemical	NOUN
cet-14418	1	72	engineering	engineering	NOUN
cet-14418	1	73	transactions	transaction	NOUN
cet-14418	1	74	vol	vol	NOUN
cet-14418	1	75	.	.	PROPN
cet-14418	1	76	108	108	NUM
cet-14418	1	77	,	,	PUNCT
cet-14418	1	78	2024	2024	NUM
cet-14418	1	79	a	a	DET
cet-14418	1	80	publication	publication	NOUN
cet-14418	1	81	of	of	ADP
cet-14418	1	82	the	the	DET
cet-14418	1	83	italian	italian	ADJ
cet-14418	1	84	association	association	NOUN
cet-14418	1	85	of	of	ADP
cet-14418	1	86	chemical	chemical	PROPN
cet-14418	1	87	engineering	engineering	NOUN
cet-14418	1	88	online	online	ADV
cet-14418	1	89	at	at	ADP
cet-14418	1	90	www.cetjournal.it	www.cetjournal.it	PROPN
cet-14418	1	91	guest	guest	NOUN
cet-14418	1	92	editors	editor	NOUN
cet-14418	1	93	:	:	PUNCT
cet-14418	1	94	carlo	carlo	PROPN
cet-14418	1	95	pirola	pirola	PROPN
cet-14418	1	96	,	,	PUNCT
cet-14418	1	97	antonio	antonio	PROPN
cet-14418	1	98	espuña	espuña	PROPN
cet-14418	1	99	copyright	copyright	NOUN
cet-14418	1	100	©	©	PROPN
cet-14418	1	101	2024	2024	NUM
cet-14418	1	102	,	,	PUNCT
cet-14418	1	103	aidic	aidic	ADJ
cet-14418	1	104	servizi	servizi	PROPN
cet-14418	1	105	s.r.l	s.r.l	NOUN
cet-14418	1	106	.	.	PUNCT
cet-14418	2	1	isbn	isbn	PROPN
cet-14418	2	2	979	979	NUM
cet-14418	2	3	-	-	SYM
cet-14418	2	4	12	12	NUM
cet-14418	2	5	-	-	PUNCT
cet-14418	2	6	81206	81206	NUM
cet-14418	2	7	-	-	SYM
cet-14418	2	8	08	08	NUM
cet-14418	2	9	-	-	SYM
cet-14418	2	10	3	3	NUM
cet-14418	2	11	;	;	PUNCT
cet-14418	2	12	issn	issn	PROPN
cet-14418	2	13	2283	2283	NUM
cet-14418	2	14	-	-	SYM
cet-14418	2	15	9216	9216	NUM
cet-14418	2	16	multi	multi	ADJ
cet-14418	2	17	-	-	ADJ
cet-14418	2	18	scale	scale	ADJ
cet-14418	2	19	simulations	simulation	NOUN
cet-14418	2	20	in	in	ADP
cet-14418	2	21	a	a	DET
cet-14418	2	22	catalytic	catalytic	ADJ
cet-14418	2	23	reactor	reactor	NOUN
cet-14418	2	24	considering	consider	VERB
cet-14418	2	25	three	three	NUM
cet-14418	2	26	-	-	PUNCT
cet-14418	2	27	dimensional	dimensional	ADJ
cet-14418	2	28	pellet	pellet	NOUN
cet-14418	2	29	geometry	geometry	NOUN
cet-14418	2	30	yoichi	yoichi	PROPN
cet-14418	2	31	takagishi	takagishi	PROPN
cet-14418	2	32	*	*	PROPN
cet-14418	2	33	,	,	PUNCT
cet-14418	2	34	ryohei	ryohei	PROPN
cet-14418	2	35	baba	baba	PROPN
cet-14418	2	36	,	,	PUNCT
cet-14418	2	37	takeshi	takeshi	PROPN
cet-14418	2	38	yamashita	yamashita	PROPN
cet-14418	2	39	,	,	PUNCT
cet-14418	2	40	wataru	wataru	PROPN
cet-14418	2	41	adachi	adachi	PROPN
cet-14418	2	42	computational	computational	PROPN
cet-14418	2	43	science	science	NOUN
cet-14418	2	44	center	center	NOUN
cet-14418	2	45	,	,	PUNCT
cet-14418	2	46	kobelco	kobelco	PROPN
cet-14418	2	47	research	research	PROPN
cet-14418	2	48	institute	institute	PROPN
cet-14418	2	49	inc	inc	PROPN
cet-14418	2	50	.	.	PROPN
cet-14418	2	51	,	,	PUNCT
cet-14418	2	52	1	1	NUM
cet-14418	2	53	-	-	SYM
cet-14418	2	54	1	1	NUM
cet-14418	2	55	-	-	SYM
cet-14418	2	56	5	5	NUM
cet-14418	2	57	,	,	PUNCT
cet-14418	2	58	takatsukadai	takatsukadai	PROPN
cet-14418	2	59	,	,	PUNCT
cet-14418	2	60	nishi	nishi	NOUN
cet-14418	2	61	-	-	PUNCT
cet-14418	2	62	ku	ku	PROPN
cet-14418	2	63	,	,	PUNCT
cet-14418	2	64	kobe	kobe	PROPN
cet-14418	2	65	,	,	PUNCT
cet-14418	2	66	651	651	NUM
cet-14418	2	67	-	-	SYM
cet-14418	2	68	2271	2271	NUM
cet-14418	2	69	,	,	PUNCT
cet-14418	2	70	japan	japan	PROPN
cet-14418	2	71	takagishi.yoichi@kki.kobelco.com	takagishi.yoichi@kki.kobelco.com	PROPN
cet-14418	2	72	catalytic	catalytic	ADJ
cet-14418	2	73	reactors	reactor	NOUN
cet-14418	2	74	that	that	PRON
cet-14418	2	75	convert	convert	VERB
cet-14418	2	76	carbon	carbon	NOUN
cet-14418	2	77	dioxide	dioxide	NOUN
cet-14418	2	78	into	into	ADP
cet-14418	2	79	methanol	methanol	NOUN
cet-14418	2	80	are	be	AUX
cet-14418	2	81	one	one	NUM
cet-14418	2	82	of	of	ADP
cet-14418	2	83	the	the	DET
cet-14418	2	84	key	key	ADJ
cet-14418	2	85	technologies	technology	NOUN
cet-14418	2	86	in	in	ADP
cet-14418	2	87	carbon	carbon	NOUN
cet-14418	2	88	recycling	recycling	NOUN
cet-14418	2	89	.	.	PUNCT
cet-14418	3	1	various	various	ADJ
cet-14418	3	2	numerical	numerical	ADJ
cet-14418	3	3	simulations	simulation	NOUN
cet-14418	3	4	have	have	AUX
cet-14418	3	5	been	be	AUX
cet-14418	3	6	conducted	conduct	VERB
cet-14418	3	7	to	to	PART
cet-14418	3	8	study	study	VERB
cet-14418	3	9	catalytic	catalytic	ADJ
cet-14418	3	10	reactors	reactor	NOUN
cet-14418	3	11	,	,	PUNCT
cet-14418	3	12	including	include	VERB
cet-14418	3	13	multi	multi	ADJ
cet-14418	3	14	-	-	ADJ
cet-14418	3	15	step	step	ADJ
cet-14418	3	16	chemical	chemical	NOUN
cet-14418	3	17	reactions	reaction	NOUN
cet-14418	3	18	,	,	PUNCT
cet-14418	3	19	flow	flow	NOUN
cet-14418	3	20	,	,	PUNCT
cet-14418	3	21	reaction	reaction	NOUN
cet-14418	3	22	heat	heat	NOUN
cet-14418	3	23	,	,	PUNCT
cet-14418	3	24	heat	heat	NOUN
cet-14418	3	25	transfer	transfer	NOUN
cet-14418	3	26	,	,	PUNCT
cet-14418	3	27	and	and	CCONJ
cet-14418	3	28	diffusion	diffusion	NOUN
cet-14418	3	29	.	.	PUNCT
cet-14418	4	1	however	however	ADV
cet-14418	4	2	,	,	PUNCT
cet-14418	4	3	in	in	ADP
cet-14418	4	4	most	most	ADJ
cet-14418	4	5	cases	case	NOUN
cet-14418	4	6	,	,	PUNCT
cet-14418	4	7	the	the	DET
cet-14418	4	8	microstructures	microstructure	NOUN
cet-14418	4	9	of	of	ADP
cet-14418	4	10	the	the	DET
cet-14418	4	11	catalyst	catalyst	NOUN
cet-14418	4	12	bed	bed	NOUN
cet-14418	4	13	are	be	AUX
cet-14418	4	14	treated	treat	VERB
cet-14418	4	15	as	as	ADP
cet-14418	4	16	a	a	DET
cet-14418	4	17	homogeneous	homogeneous	ADJ
cet-14418	4	18	body	body	NOUN
cet-14418	4	19	,	,	PUNCT
cet-14418	4	20	in	in	ADP
cet-14418	4	21	which	which	PRON
cet-14418	4	22	permeability	permeability	NOUN
cet-14418	4	23	,	,	PUNCT
cet-14418	4	24	diffusion	diffusion	NOUN
cet-14418	4	25	coefficient	coefficient	NOUN
cet-14418	4	26	,	,	PUNCT
cet-14418	4	27	and	and	CCONJ
cet-14418	4	28	thermal	thermal	ADJ
cet-14418	4	29	conductivity	conductivity	NOUN
cet-14418	4	30	are	be	AUX
cet-14418	4	31	estimated	estimate	VERB
cet-14418	4	32	by	by	ADP
cet-14418	4	33	simplified	simplified	ADJ
cet-14418	4	34	estimation	estimation	NOUN
cet-14418	4	35	formula	formula	NOUN
cet-14418	4	36	,	,	PUNCT
cet-14418	4	37	making	make	VERB
cet-14418	4	38	it	it	PRON
cet-14418	4	39	difficult	difficult	ADJ
cet-14418	4	40	to	to	PART
cet-14418	4	41	evaluate	evaluate	VERB
cet-14418	4	42	the	the	DET
cet-14418	4	43	effects	effect	NOUN
cet-14418	4	44	of	of	ADP
cet-14418	4	45	the	the	DET
cet-14418	4	46	differences	difference	NOUN
cet-14418	4	47	in	in	ADP
cet-14418	4	48	pellet	pellet	NOUN
cet-14418	4	49	shapes	shape	NOUN
cet-14418	4	50	.	.	PUNCT
cet-14418	5	1	in	in	ADP
cet-14418	5	2	this	this	DET
cet-14418	5	3	study	study	NOUN
cet-14418	5	4	,	,	PUNCT
cet-14418	5	5	we	we	PRON
cet-14418	5	6	developed	develop	VERB
cet-14418	5	7	a	a	DET
cet-14418	5	8	macroscopic	macroscopic	ADJ
cet-14418	5	9	homogenization	homogenization	NOUN
cet-14418	5	10	model	model	NOUN
cet-14418	5	11	combined	combine	VERB
cet-14418	5	12	with	with	ADP
cet-14418	5	13	a	a	DET
cet-14418	5	14	three	three	NUM
cet-14418	5	15	-	-	PUNCT
cet-14418	5	16	dimensional	dimensional	ADJ
cet-14418	5	17	microstructure	microstructure	NOUN
cet-14418	5	18	in	in	ADP
cet-14418	5	19	the	the	DET
cet-14418	5	20	catalyst	catalyst	NOUN
cet-14418	5	21	bed	bed	NOUN
cet-14418	5	22	in	in	ADP
cet-14418	5	23	order	order	NOUN
cet-14418	5	24	to	to	PART
cet-14418	5	25	predict	predict	VERB
cet-14418	5	26	complex	complex	ADJ
cet-14418	5	27	phenomena	phenomenon	NOUN
cet-14418	5	28	in	in	ADP
cet-14418	5	29	the	the	DET
cet-14418	5	30	reactor	reactor	NOUN
cet-14418	5	31	.	.	PUNCT
cet-14418	6	1	the	the	DET
cet-14418	6	2	model	model	NOUN
cet-14418	6	3	validation	validation	NOUN
cet-14418	6	4	was	be	AUX
cet-14418	6	5	also	also	ADV
cet-14418	6	6	performed	perform	VERB
cet-14418	6	7	with	with	ADP
cet-14418	6	8	the	the	DET
cet-14418	6	9	actual	actual	ADJ
cet-14418	6	10	experiments	experiment	NOUN
cet-14418	6	11	of	of	ADP
cet-14418	6	12	catalytic	catalytic	ADJ
cet-14418	6	13	reactions	reaction	NOUN
cet-14418	6	14	.	.	PUNCT
cet-14418	7	1	furthermore	furthermore	ADV
cet-14418	7	2	,	,	PUNCT
cet-14418	7	3	the	the	DET
cet-14418	7	4	effects	effect	NOUN
cet-14418	7	5	of	of	ADP
cet-14418	7	6	different	different	ADJ
cet-14418	7	7	pellet	pellet	NOUN
cet-14418	7	8	shapes	shape	NOUN
cet-14418	7	9	on	on	ADP
cet-14418	7	10	the	the	DET
cet-14418	7	11	temperature	temperature	NOUN
cet-14418	7	12	,	,	PUNCT
cet-14418	7	13	flow	flow	NOUN
cet-14418	7	14	field	field	NOUN
cet-14418	7	15	,	,	PUNCT
cet-14418	7	16	and	and	CCONJ
cet-14418	7	17	reaction	reaction	NOUN
cet-14418	7	18	field	field	NOUN
cet-14418	7	19	in	in	ADP
cet-14418	7	20	the	the	DET
cet-14418	7	21	reactor	reactor	NOUN
cet-14418	7	22	were	be	AUX
cet-14418	7	23	compared	compare	VERB
cet-14418	7	24	.	.	PUNCT
cet-14418	8	1	1	1	X
cet-14418	8	2	.	.	X
cet-14418	8	3	introduction	introduction	NOUN
cet-14418	8	4	co2	co2	NOUN
cet-14418	8	5	methanation	methanation	NOUN
cet-14418	8	6	through	through	ADP
cet-14418	8	7	conversion	conversion	NOUN
cet-14418	8	8	into	into	ADP
cet-14418	8	9	fuels	fuel	NOUN
cet-14418	8	10	and	and	CCONJ
cet-14418	8	11	chemicals	chemical	NOUN
cet-14418	8	12	such	such	ADJ
cet-14418	8	13	as	as	ADP
cet-14418	8	14	methane	methane	NOUN
cet-14418	8	15	or	or	CCONJ
cet-14418	8	16	methanol	methanol	NOUN
cet-14418	8	17	is	be	AUX
cet-14418	8	18	recognized	recognize	VERB
cet-14418	8	19	as	as	ADP
cet-14418	8	20	a	a	DET
cet-14418	8	21	key	key	ADJ
cet-14418	8	22	technology	technology	NOUN
cet-14418	8	23	for	for	ADP
cet-14418	8	24	“	"	PUNCT
cet-14418	8	25	carbon	carbon	NOUN
cet-14418	8	26	recycling	recycling	NOUN
cet-14418	8	27	”	"	PUNCT
cet-14418	8	28	(	(	PUNCT
cet-14418	8	29	kato	kato	PROPN
cet-14418	8	30	et	et	PROPN
cet-14418	8	31	al	al	PROPN
cet-14418	8	32	.	.	PROPN
cet-14418	8	33	,	,	PUNCT
cet-14418	8	34	2010	2010	NUM
cet-14418	8	35	)	)	PUNCT
cet-14418	8	36	.	.	PUNCT
cet-14418	9	1	the	the	DET
cet-14418	9	2	efficiency	efficiency	NOUN
cet-14418	9	3	of	of	ADP
cet-14418	9	4	the	the	DET
cet-14418	9	5	conversion	conversion	NOUN
cet-14418	9	6	reactions	reaction	NOUN
cet-14418	9	7	strongly	strongly	ADV
cet-14418	9	8	depends	depend	VERB
cet-14418	9	9	on	on	ADP
cet-14418	9	10	both	both	PRON
cet-14418	9	11	macro	macro	NOUN
cet-14418	9	12	and	and	CCONJ
cet-14418	9	13	microscopic	microscopic	ADJ
cet-14418	9	14	factors	factor	NOUN
cet-14418	9	15	.	.	PUNCT
cet-14418	10	1	the	the	DET
cet-14418	10	2	former	former	ADJ
cet-14418	10	3	includes	include	VERB
cet-14418	10	4	the	the	DET
cet-14418	10	5	catalytic	catalytic	ADJ
cet-14418	10	6	performance	performance	NOUN
cet-14418	10	7	and	and	CCONJ
cet-14418	10	8	pellet	pellet	NOUN
cet-14418	10	9	shape	shape	NOUN
cet-14418	10	10	,	,	PUNCT
cet-14418	10	11	etc	etc	X
cet-14418	10	12	.	.	X
cet-14418	10	13	,	,	PUNCT
cet-14418	10	14	and	and	CCONJ
cet-14418	10	15	the	the	DET
cet-14418	10	16	latter	latter	ADJ
cet-14418	10	17	includes	include	VERB
cet-14418	10	18	reactor	reactor	NOUN
cet-14418	10	19	geometry	geometry	NOUN
cet-14418	10	20	,	,	PUNCT
cet-14418	10	21	heating	heating	NOUN
cet-14418	10	22	conditions	condition	NOUN
cet-14418	10	23	,	,	PUNCT
cet-14418	10	24	inward	inward	ADP
cet-14418	10	25	gas	gas	NOUN
cet-14418	10	26	pressure	pressure	NOUN
cet-14418	10	27	etc	etc	X
cet-14418	10	28	.	.	X
cet-14418	11	1	(	(	PUNCT
cet-14418	11	2	zhang	zhang	PROPN
cet-14418	11	3	,	,	PUNCT
cet-14418	11	4	2021	2021	NUM
cet-14418	11	5	)	)	PUNCT
cet-14418	11	6	.	.	PUNCT
cet-14418	12	1	computational	computational	ADJ
cet-14418	12	2	fluid	fluid	ADJ
cet-14418	12	3	dynamics	dynamic	NOUN
cet-14418	12	4	(	(	PUNCT
cet-14418	12	5	cfd	cfd	NOUN
cet-14418	12	6	)	)	PUNCT
cet-14418	12	7	have	have	AUX
cet-14418	12	8	been	be	AUX
cet-14418	12	9	adopted	adopt	VERB
cet-14418	12	10	widely	widely	ADV
cet-14418	12	11	for	for	ADP
cet-14418	12	12	use	use	NOUN
cet-14418	12	13	in	in	ADP
cet-14418	12	14	macroscopic	macroscopic	ADJ
cet-14418	12	15	simulations	simulation	NOUN
cet-14418	12	16	,	,	PUNCT
cet-14418	12	17	which	which	PRON
cet-14418	12	18	provide	provide	VERB
cet-14418	12	19	various	various	ADJ
cet-14418	12	20	information	information	NOUN
cet-14418	12	21	regarding	regard	VERB
cet-14418	12	22	gas	gas	NOUN
cet-14418	12	23	flow	flow	NOUN
cet-14418	12	24	velocity	velocity	NOUN
cet-14418	12	25	components	component	NOUN
cet-14418	12	26	,	,	PUNCT
cet-14418	12	27	pressure	pressure	NOUN
cet-14418	12	28	,	,	PUNCT
cet-14418	12	29	temperature	temperature	NOUN
cet-14418	12	30	,	,	PUNCT
cet-14418	12	31	and	and	CCONJ
cet-14418	12	32	chemical	chemical	NOUN
cet-14418	12	33	species	specie	NOUN
cet-14418	12	34	concentration	concentration	NOUN
cet-14418	12	35	in	in	ADP
cet-14418	12	36	a	a	DET
cet-14418	12	37	reactor	reactor	NOUN
cet-14418	12	38	.	.	PUNCT
cet-14418	13	1	the	the	DET
cet-14418	13	2	most	most	ADV
cet-14418	13	3	used	use	VERB
cet-14418	13	4	models	model	NOUN
cet-14418	13	5	assume	assume	VERB
cet-14418	13	6	the	the	DET
cet-14418	13	7	fixed	fix	VERB
cet-14418	13	8	bed	bed	NOUN
cet-14418	13	9	to	to	PART
cet-14418	13	10	be	be	AUX
cet-14418	13	11	the	the	DET
cet-14418	13	12	homogeneous	homogeneous	ADJ
cet-14418	13	13	media	medium	NOUN
cet-14418	13	14	,	,	PUNCT
cet-14418	13	15	represented	represent	VERB
cet-14418	13	16	by	by	ADP
cet-14418	13	17	porosity	porosity	NOUN
cet-14418	13	18	,	,	PUNCT
cet-14418	13	19	specific	specific	ADJ
cet-14418	13	20	surface	surface	NOUN
cet-14418	13	21	area	area	NOUN
cet-14418	13	22	,	,	PUNCT
cet-14418	13	23	and	and	CCONJ
cet-14418	13	24	effective	effective	ADJ
cet-14418	13	25	material	material	NOUN
cet-14418	13	26	properties	property	NOUN
cet-14418	13	27	,	,	PUNCT
cet-14418	13	28	including	include	VERB
cet-14418	13	29	permeability	permeability	NOUN
cet-14418	13	30	and	and	CCONJ
cet-14418	13	31	thermal	thermal	ADJ
cet-14418	13	32	conductivity	conductivity	NOUN
cet-14418	13	33	.	.	PUNCT
cet-14418	14	1	in	in	ADP
cet-14418	14	2	addition	addition	NOUN
cet-14418	14	3	to	to	ADP
cet-14418	14	4	simple	simple	ADJ
cet-14418	14	5	one	one	NUM
cet-14418	14	6	-	-	PUNCT
cet-14418	14	7	dimensional	dimensional	ADJ
cet-14418	14	8	models	model	NOUN
cet-14418	14	9	(	(	PUNCT
cet-14418	14	10	an	an	PRON
cet-14418	14	11	,	,	PUNCT
cet-14418	14	12	2017	2017	NUM
cet-14418	14	13	)	)	PUNCT
cet-14418	14	14	,	,	PUNCT
cet-14418	14	15	two(adji	two(adji	PROPN
cet-14418	14	16	et	et	NOUN
cet-14418	14	17	al	al	PROPN
cet-14418	14	18	.	.	PROPN
cet-14418	14	19	,	,	PUNCT
cet-14418	14	20	2019	2019	NUM
cet-14418	14	21	)	)	PUNCT
cet-14418	14	22	,	,	PUNCT
cet-14418	14	23	and	and	CCONJ
cet-14418	14	24	threedimensional	threedimensional	ADJ
cet-14418	14	25	models	model	NOUN
cet-14418	14	26	(	(	PUNCT
cet-14418	14	27	son	son	NOUN
cet-14418	14	28	et	et	PROPN
cet-14418	14	29	al	al	PROPN
cet-14418	14	30	.	.	PROPN
cet-14418	14	31	,	,	PUNCT
cet-14418	14	32	2019	2019	NUM
cet-14418	14	33	)	)	PUNCT
cet-14418	14	34	have	have	AUX
cet-14418	14	35	been	be	AUX
cet-14418	14	36	developed	develop	VERB
cet-14418	14	37	with	with	ADP
cet-14418	14	38	the	the	DET
cet-14418	14	39	various	various	ADJ
cet-14418	14	40	kinetic	kinetic	ADJ
cet-14418	14	41	reaction	reaction	NOUN
cet-14418	14	42	models	model	NOUN
cet-14418	14	43	.	.	PUNCT
cet-14418	15	1	although	although	SCONJ
cet-14418	15	2	these	these	DET
cet-14418	15	3	models	model	NOUN
cet-14418	15	4	have	have	VERB
cet-14418	15	5	advantages	advantage	NOUN
cet-14418	15	6	in	in	ADP
cet-14418	15	7	computation	computation	NOUN
cet-14418	15	8	efficiency	efficiency	NOUN
cet-14418	15	9	,	,	PUNCT
cet-14418	15	10	they	they	PRON
cet-14418	15	11	present	present	VERB
cet-14418	15	12	some	some	DET
cet-14418	15	13	difficulties	difficulty	NOUN
cet-14418	15	14	when	when	SCONJ
cet-14418	15	15	considering	consider	VERB
cet-14418	15	16	the	the	DET
cet-14418	15	17	effect	effect	NOUN
cet-14418	15	18	of	of	ADP
cet-14418	15	19	the	the	DET
cet-14418	15	20	actual	actual	ADJ
cet-14418	15	21	non	non	NOUN
cet-14418	15	22	-	-	NOUN
cet-14418	15	23	uniformity	uniformity	NOUN
cet-14418	15	24	of	of	ADP
cet-14418	15	25	a	a	DET
cet-14418	15	26	packed	packed	ADJ
cet-14418	15	27	bed	bed	NOUN
cet-14418	15	28	.	.	PUNCT
cet-14418	16	1	recently	recently	ADV
cet-14418	16	2	,	,	PUNCT
cet-14418	16	3	particle	particle	NOUN
cet-14418	16	4	-	-	PUNCT
cet-14418	16	5	resolved	resolve	VERB
cet-14418	16	6	cfd	cfd	NOUN
cet-14418	16	7	simulations	simulation	NOUN
cet-14418	16	8	,	,	PUNCT
cet-14418	16	9	which	which	PRON
cet-14418	16	10	consider	consider	VERB
cet-14418	16	11	the	the	DET
cet-14418	16	12	3d	3d	ADV
cet-14418	16	13	-	-	PUNCT
cet-14418	16	14	packed	pack	VERB
cet-14418	16	15	structure	structure	NOUN
cet-14418	16	16	of	of	ADP
cet-14418	16	17	the	the	DET
cet-14418	16	18	catalyst	catalyst	NOUN
cet-14418	16	19	pellets	pellet	NOUN
cet-14418	16	20	,	,	PUNCT
cet-14418	16	21	have	have	AUX
cet-14418	16	22	been	be	AUX
cet-14418	16	23	reported	report	VERB
cet-14418	16	24	(	(	PUNCT
cet-14418	16	25	maestri	maestri	PROPN
cet-14418	16	26	et	et	PROPN
cet-14418	16	27	al	al	PROPN
cet-14418	16	28	.	.	PROPN
cet-14418	16	29	,	,	PUNCT
cet-14418	16	30	2013	2013	NUM
cet-14418	16	31	;	;	PUNCT
cet-14418	16	32	dixon	dixon	PROPN
cet-14418	16	33	et	et	PROPN
cet-14418	16	34	al	al	PROPN
cet-14418	16	35	.	.	PROPN
cet-14418	16	36	,	,	PUNCT
cet-14418	16	37	2019	2019	NUM
cet-14418	16	38	)	)	PUNCT
cet-14418	16	39	.	.	PUNCT
cet-14418	17	1	nevertheless	nevertheless	ADV
cet-14418	17	2	,	,	PUNCT
cet-14418	17	3	such	such	ADJ
cet-14418	17	4	realistic	realistic	ADJ
cet-14418	17	5	3d	3d	NOUN
cet-14418	17	6	models	model	NOUN
cet-14418	17	7	require	require	VERB
cet-14418	17	8	large	large	ADJ
cet-14418	17	9	-	-	PUNCT
cet-14418	17	10	scale	scale	NOUN
cet-14418	17	11	calculation	calculation	NOUN
cet-14418	17	12	costs	cost	NOUN
cet-14418	17	13	.	.	PUNCT
cet-14418	18	1	in	in	ADP
cet-14418	18	2	this	this	DET
cet-14418	18	3	study	study	NOUN
cet-14418	18	4	,	,	PUNCT
cet-14418	18	5	a	a	DET
cet-14418	18	6	stepwise	stepwise	NOUN
cet-14418	18	7	multiscale	multiscale	NOUN
cet-14418	18	8	model	model	NOUN
cet-14418	18	9	of	of	ADP
cet-14418	18	10	a	a	DET
cet-14418	18	11	fixed	fix	VERB
cet-14418	18	12	-	-	PUNCT
cet-14418	18	13	bed	bed	NOUN
cet-14418	18	14	co2	co2	NOUN
cet-14418	18	15	methanation	methanation	NOUN
cet-14418	18	16	reactor	reactor	NOUN
cet-14418	18	17	was	be	AUX
cet-14418	18	18	developed	develop	VERB
cet-14418	18	19	considering	consider	VERB
cet-14418	18	20	the	the	DET
cet-14418	18	21	effect	effect	NOUN
cet-14418	18	22	of	of	ADP
cet-14418	18	23	3d	3d	NOUN
cet-14418	18	24	-	-	PUNCT
cet-14418	18	25	packed	pack	VERB
cet-14418	18	26	pellet	pellet	NOUN
cet-14418	18	27	geometry	geometry	NOUN
cet-14418	18	28	.	.	PUNCT
cet-14418	19	1	the	the	DET
cet-14418	19	2	key	key	ADJ
cet-14418	19	3	idea	idea	NOUN
cet-14418	19	4	of	of	ADP
cet-14418	19	5	this	this	DET
cet-14418	19	6	approach	approach	NOUN
cet-14418	19	7	is	be	AUX
cet-14418	19	8	that	that	SCONJ
cet-14418	19	9	the	the	DET
cet-14418	19	10	effective	effective	ADJ
cet-14418	19	11	properties	property	NOUN
cet-14418	19	12	,	,	PUNCT
cet-14418	19	13	including	include	VERB
cet-14418	19	14	porosity	porosity	NOUN
cet-14418	19	15	,	,	PUNCT
cet-14418	19	16	specific	specific	ADJ
cet-14418	19	17	surface	surface	NOUN
cet-14418	19	18	area	area	NOUN
cet-14418	19	19	,	,	PUNCT
cet-14418	19	20	etc	etc	X
cet-14418	19	21	.	.	X
cet-14418	19	22	,	,	PUNCT
cet-14418	19	23	are	be	AUX
cet-14418	19	24	evaluated	evaluate	VERB
cet-14418	19	25	by	by	ADP
cet-14418	19	26	the	the	DET
cet-14418	19	27	particle	particle	NOUN
cet-14418	19	28	-	-	PUNCT
cet-14418	19	29	resolved	resolve	VERB
cet-14418	19	30	model	model	NOUN
cet-14418	19	31	and	and	CCONJ
cet-14418	19	32	used	use	VERB
cet-14418	19	33	for	for	ADP
cet-14418	19	34	the	the	DET
cet-14418	19	35	homogeneous	homogeneous	ADJ
cet-14418	19	36	reactor	reactor	NOUN
cet-14418	19	37	model	model	NOUN
cet-14418	19	38	.	.	PUNCT
cet-14418	20	1	the	the	DET
cet-14418	20	2	model	model	NOUN
cet-14418	20	3	validation	validation	NOUN
cet-14418	20	4	was	be	AUX
cet-14418	20	5	conducted	conduct	VERB
cet-14418	20	6	with	with	ADP
cet-14418	20	7	the	the	DET
cet-14418	20	8	methanol	methanol	NOUN
cet-14418	20	9	synthesis	synthesis	NOUN
cet-14418	20	10	experiment	experiment	NOUN
cet-14418	20	11	for	for	ADP
cet-14418	20	12	cylindrical	cylindrical	ADJ
cet-14418	20	13	pellets	pellet	NOUN
cet-14418	20	14	of	of	ADP
cet-14418	20	15	zn.al2o3	zn.al2o3	NUM
cet-14418	20	16	.	.	PUNCT
cet-14418	21	1	moreover	moreover	ADV
cet-14418	21	2	,	,	PUNCT
cet-14418	21	3	the	the	DET
cet-14418	21	4	effects	effect	NOUN
cet-14418	21	5	of	of	ADP
cet-14418	21	6	pellet	pellet	NOUN
cet-14418	21	7	shapes	shape	NOUN
cet-14418	21	8	on	on	ADP
cet-14418	21	9	the	the	DET
cet-14418	21	10	reactor	reactor	NOUN
cet-14418	21	11	’s	’s	PART
cet-14418	21	12	performance	performance	NOUN
cet-14418	21	13	were	be	AUX
cet-14418	21	14	discussed	discuss	VERB
cet-14418	21	15	.	.	PUNCT
cet-14418	22	1	2	2	X
cet-14418	22	2	.	.	X
cet-14418	22	3	model	model	NOUN
cet-14418	22	4	development	development	NOUN
cet-14418	22	5	2.1	2.1	NUM
cet-14418	22	6	flow	flow	NOUN
cet-14418	22	7	of	of	ADP
cet-14418	22	8	stepwise	stepwise	ADJ
cet-14418	22	9	multi	multi	ADJ
cet-14418	22	10	-	-	ADJ
cet-14418	22	11	scale	scale	ADJ
cet-14418	22	12	simulations	simulation	NOUN
cet-14418	22	13	the	the	DET
cet-14418	22	14	flow	flow	NOUN
cet-14418	22	15	of	of	ADP
cet-14418	22	16	this	this	DET
cet-14418	22	17	study	study	NOUN
cet-14418	22	18	is	be	AUX
cet-14418	22	19	as	as	SCONJ
cet-14418	22	20	follows	follow	VERB
cet-14418	22	21	(	(	PUNCT
cet-14418	22	22	fig.1	fig.1	PROPN
cet-14418	22	23	)	)	PUNCT
cet-14418	22	24	.	.	PUNCT
cet-14418	23	1	firstly	firstly	ADV
cet-14418	23	2	,	,	PUNCT
cet-14418	23	3	a	a	DET
cet-14418	23	4	particle	particle	NOUN
cet-14418	23	5	-	-	PUNCT
cet-14418	23	6	resolved	resolve	VERB
cet-14418	23	7	3d	3d	NOUN
cet-14418	23	8	-	-	PUNCT
cet-14418	23	9	packed	pack	VERB
cet-14418	23	10	structure	structure	NOUN
cet-14418	23	11	of	of	ADP
cet-14418	23	12	the	the	DET
cet-14418	23	13	catalyst	catalyst	NOUN
cet-14418	23	14	pellets	pellet	NOUN
cet-14418	23	15	(	(	PUNCT
cet-14418	23	16	micro	micro	ADJ
cet-14418	23	17	-	-	NOUN
cet-14418	23	18	scale	scale	ADJ
cet-14418	23	19	model	model	NOUN
cet-14418	23	20	)	)	PUNCT
cet-14418	23	21	was	be	AUX
cet-14418	23	22	developed	develop	VERB
cet-14418	23	23	,	,	PUNCT
cet-14418	23	24	and	and	CCONJ
cet-14418	23	25	the	the	DET
cet-14418	23	26	effective	effective	ADJ
cet-14418	23	27	properties	property	NOUN
cet-14418	23	28	,	,	PUNCT
cet-14418	23	29	including	include	VERB
cet-14418	23	30	porosity	porosity	NOUN
cet-14418	23	31	,	,	PUNCT
cet-14418	23	32	specific	specific	ADJ
cet-14418	23	33	surface	surface	NOUN
cet-14418	23	34	area	area	NOUN
cet-14418	23	35	,	,	PUNCT
cet-14418	23	36	permeability	permeability	NOUN
cet-14418	23	37	,	,	PUNCT
cet-14418	23	38	and	and	CCONJ
cet-14418	23	39	thermal	thermal	ADJ
cet-14418	23	40	conductivity	conductivity	NOUN
cet-14418	23	41	,	,	PUNCT
cet-14418	23	42	were	be	AUX
cet-14418	23	43	evaluated	evaluate	VERB
cet-14418	23	44	.	.	PUNCT
cet-14418	24	1	next	next	ADV
cet-14418	24	2	,	,	PUNCT
cet-14418	24	3	a	a	DET
cet-14418	24	4	2d	2d	NUM
cet-14418	24	5	axial	axial	ADJ
cet-14418	24	6	symmetric	symmetric	ADJ
cet-14418	24	7	homogeneous	homogeneous	ADJ
cet-14418	24	8	multi	multi	ADJ
cet-14418	24	9	-	-	ADJ
cet-14418	24	10	physics	physics	ADJ
cet-14418	24	11	model	model	NOUN
cet-14418	24	12	(	(	PUNCT
cet-14418	24	13	macro	macro	ADJ
cet-14418	24	14	-	-	NOUN
cet-14418	24	15	scale	scale	NOUN
cet-14418	24	16	model	model	NOUN
cet-14418	24	17	)	)	PUNCT
cet-14418	24	18	was	be	AUX
cet-14418	24	19	constructed	construct	VERB
cet-14418	24	20	,	,	PUNCT
cet-14418	24	21	in	in	ADP
cet-14418	24	22	which	which	PRON
cet-14418	24	23	the	the	DET
cet-14418	24	24	effective	effective	ADJ
cet-14418	24	25	properties	property	NOUN
cet-14418	24	26	in	in	ADP
cet-14418	24	27	the	the	DET
cet-14418	24	28	catalyst	catalyst	NOUN
cet-14418	24	29	bed	bed	NOUN
cet-14418	24	30	were	be	AUX
cet-14418	24	31	the	the	DET
cet-14418	24	32	values	value	NOUN
cet-14418	24	33	43	43	NUM
cet-14418	24	34	obtained	obtain	VERB
cet-14418	24	35	from	from	ADP
cet-14418	24	36	the	the	DET
cet-14418	24	37	above	above	ADJ
cet-14418	24	38	model	model	NOUN
cet-14418	24	39	,	,	PUNCT
cet-14418	24	40	in	in	ADP
cet-14418	24	41	order	order	NOUN
cet-14418	24	42	to	to	PART
cet-14418	24	43	simulate	simulate	VERB
cet-14418	24	44	the	the	DET
cet-14418	24	45	reaction	reaction	NOUN
cet-14418	24	46	,	,	PUNCT
cet-14418	24	47	gas	gas	NOUN
cet-14418	24	48	flow	flow	NOUN
cet-14418	24	49	,	,	PUNCT
cet-14418	24	50	pressure	pressure	NOUN
cet-14418	24	51	,	,	PUNCT
cet-14418	24	52	and	and	CCONJ
cet-14418	24	53	temperature	temperature	NOUN
cet-14418	24	54	fields	field	NOUN
cet-14418	24	55	in	in	ADP
cet-14418	24	56	the	the	DET
cet-14418	24	57	reactor	reactor	NOUN
cet-14418	24	58	.	.	PUNCT
cet-14418	25	1	next	next	ADV
cet-14418	25	2	,	,	PUNCT
cet-14418	25	3	a	a	DET
cet-14418	25	4	methanol	methanol	NOUN
cet-14418	25	5	synthesis	synthesis	NOUN
cet-14418	25	6	experiment	experiment	NOUN
cet-14418	25	7	was	be	AUX
cet-14418	25	8	conducted	conduct	VERB
cet-14418	25	9	,	,	PUNCT
cet-14418	25	10	and	and	CCONJ
cet-14418	25	11	the	the	DET
cet-14418	25	12	micro	micro	ADJ
cet-14418	25	13	-	-	NOUN
cet-14418	25	14	scale	scale	ADJ
cet-14418	25	15	model	model	NOUN
cet-14418	25	16	was	be	AUX
cet-14418	25	17	validated	validate	VERB
cet-14418	25	18	.	.	PUNCT
cet-14418	26	1	finally	finally	ADV
cet-14418	26	2	,	,	PUNCT
cet-14418	26	3	micro	micro	ADJ
cet-14418	26	4	-	-	NOUN
cet-14418	26	5	scale	scale	ADJ
cet-14418	26	6	simulations	simulation	NOUN
cet-14418	26	7	with	with	ADP
cet-14418	26	8	different	different	ADJ
cet-14418	26	9	pellet	pellet	NOUN
cet-14418	26	10	shapes	shape	NOUN
cet-14418	26	11	were	be	AUX
cet-14418	26	12	also	also	ADV
cet-14418	26	13	carried	carry	VERB
cet-14418	26	14	out	out	ADP
cet-14418	26	15	,	,	PUNCT
cet-14418	26	16	and	and	CCONJ
cet-14418	26	17	the	the	DET
cet-14418	26	18	reactor	reactor	NOUN
cet-14418	26	19	’s	’s	PART
cet-14418	26	20	performance	performance	NOUN
cet-14418	26	21	was	be	AUX
cet-14418	26	22	predicted	predict	VERB
cet-14418	26	23	by	by	ADP
cet-14418	26	24	the	the	DET
cet-14418	26	25	macro	macro	ADJ
cet-14418	26	26	-	-	NOUN
cet-14418	26	27	scale	scale	NOUN
cet-14418	26	28	model	model	NOUN
cet-14418	26	29	.	.	PUNCT
cet-14418	27	1	geodict	geodict	PROPN
cet-14418	27	2	2020	2020	NUM
cet-14418	27	3	and	and	CCONJ
cet-14418	27	4	comsol	comsol	NOUN
cet-14418	27	5	multiphysics	multiphysic	NOUN
cet-14418	27	6	™	™	VERB
cet-14418	27	7	ver.5.6	ver.5.6	PROPN
cet-14418	27	8	were	be	AUX
cet-14418	27	9	adopted	adopt	VERB
cet-14418	27	10	for	for	ADP
cet-14418	27	11	the	the	DET
cet-14418	27	12	micro	micro	ADJ
cet-14418	27	13	-	-	NOUN
cet-14418	27	14	scale	scale	ADJ
cet-14418	27	15	simulation	simulation	NOUN
cet-14418	27	16	and	and	CCONJ
cet-14418	27	17	the	the	DET
cet-14418	27	18	macro	macro	ADJ
cet-14418	27	19	-	-	NOUN
cet-14418	27	20	scale	scale	NOUN
cet-14418	27	21	simulation	simulation	NOUN
cet-14418	27	22	,	,	PUNCT
cet-14418	27	23	respectively	respectively	ADV
cet-14418	27	24	.	.	PUNCT
cet-14418	28	1	figure	figure	NOUN
cet-14418	28	2	1	1	NUM
cet-14418	28	3	.	.	PUNCT
cet-14418	28	4	flow	flow	NOUN
cet-14418	28	5	of	of	ADP
cet-14418	28	6	model	model	NOUN
cet-14418	28	7	development	development	NOUN
cet-14418	28	8	and	and	CCONJ
cet-14418	28	9	validation	validation	NOUN
cet-14418	28	10	.	.	PUNCT
cet-14418	29	1	2.2	2.2	NUM
cet-14418	29	2	simulation	simulation	NOUN
cet-14418	29	3	method	method	NOUN
cet-14418	29	4	of	of	ADP
cet-14418	29	5	micro	micro	ADJ
cet-14418	29	6	-	-	NOUN
cet-14418	29	7	scale	scale	ADJ
cet-14418	29	8	model	model	NOUN
cet-14418	29	9	in	in	ADP
cet-14418	29	10	the	the	DET
cet-14418	29	11	micro	micro	ADJ
cet-14418	29	12	-	-	NOUN
cet-14418	29	13	scale	scale	ADJ
cet-14418	29	14	model	model	NOUN
cet-14418	29	15	,	,	PUNCT
cet-14418	29	16	the	the	DET
cet-14418	29	17	3d	3d	NUM
cet-14418	29	18	random	random	ADV
cet-14418	29	19	-	-	PUNCT
cet-14418	29	20	packed	pack	VERB
cet-14418	29	21	structure	structure	NOUN
cet-14418	29	22	of	of	ADP
cet-14418	29	23	the	the	DET
cet-14418	29	24	catalyst	catalyst	NOUN
cet-14418	29	25	pellets	pellet	NOUN
cet-14418	29	26	is	be	AUX
cet-14418	29	27	constructed	construct	VERB
cet-14418	29	28	first	first	ADV
cet-14418	29	29	,	,	PUNCT
cet-14418	29	30	and	and	CCONJ
cet-14418	29	31	the	the	DET
cet-14418	29	32	porosity	porosity	NOUN
cet-14418	29	33	and	and	CCONJ
cet-14418	29	34	the	the	DET
cet-14418	29	35	specific	specific	ADJ
cet-14418	29	36	surface	surface	NOUN
cet-14418	29	37	area	area	NOUN
cet-14418	29	38	are	be	AUX
cet-14418	29	39	estimated	estimate	VERB
cet-14418	29	40	.	.	PUNCT
cet-14418	30	1	herein	herein	NOUN
cet-14418	30	2	,	,	PUNCT
cet-14418	30	3	the	the	DET
cet-14418	30	4	cylinder	cylinder	NOUN
cet-14418	30	5	,	,	PUNCT
cet-14418	30	6	sphere	sphere	NOUN
cet-14418	30	7	and	and	CCONJ
cet-14418	30	8	hollow	hollow	ADJ
cet-14418	30	9	cylinder	cylinder	NOUN
cet-14418	30	10	were	be	AUX
cet-14418	30	11	adopted	adopt	VERB
cet-14418	30	12	as	as	ADP
cet-14418	30	13	typical	typical	ADJ
cet-14418	30	14	pellet	pellet	NOUN
cet-14418	30	15	shapes	shape	NOUN
cet-14418	30	16	(	(	PUNCT
cet-14418	30	17	table.1	table.1	NOUN
cet-14418	30	18	)	)	PUNCT
cet-14418	30	19	.	.	PUNCT
cet-14418	31	1	the	the	DET
cet-14418	31	2	pellets	pellet	NOUN
cet-14418	31	3	were	be	AUX
cet-14418	31	4	piled	pile	VERB
cet-14418	31	5	randomly	randomly	ADV
cet-14418	31	6	in	in	ADP
cet-14418	31	7	the	the	DET
cet-14418	31	8	larger	large	ADJ
cet-14418	31	9	simulation	simulation	NOUN
cet-14418	31	10	box	box	PROPN
cet-14418	31	11	with	with	ADP
cet-14418	31	12	the	the	DET
cet-14418	31	13	point	point	NOUN
cet-14418	31	14	contact	contact	NOUN
cet-14418	31	15	condition	condition	NOUN
cet-14418	31	16	,	,	PUNCT
cet-14418	31	17	and	and	CCONJ
cet-14418	31	18	the	the	DET
cet-14418	31	19	edge	edge	NOUN
cet-14418	31	20	regions	region	NOUN
cet-14418	31	21	within	within	ADP
cet-14418	31	22	the	the	DET
cet-14418	31	23	pellet	pellet	NOUN
cet-14418	31	24	size	size	NOUN
cet-14418	31	25	were	be	AUX
cet-14418	31	26	cropped	crop	VERB
cet-14418	31	27	.	.	PUNCT
cet-14418	32	1	next	next	ADV
cet-14418	32	2	,	,	PUNCT
cet-14418	32	3	the	the	DET
cet-14418	32	4	gas	gas	NOUN
cet-14418	32	5	flow	flow	NOUN
cet-14418	32	6	,	,	PUNCT
cet-14418	32	7	the	the	DET
cet-14418	32	8	diffusion	diffusion	NOUN
cet-14418	32	9	of	of	ADP
cet-14418	32	10	the	the	DET
cet-14418	32	11	chemical	chemical	NOUN
cet-14418	32	12	species	specie	NOUN
cet-14418	32	13	,	,	PUNCT
cet-14418	32	14	and	and	CCONJ
cet-14418	32	15	the	the	DET
cet-14418	32	16	heat	heat	NOUN
cet-14418	32	17	transfer	transfer	NOUN
cet-14418	32	18	simulations	simulation	NOUN
cet-14418	32	19	were	be	AUX
cet-14418	32	20	conducted	conduct	VERB
cet-14418	32	21	separately	separately	ADV
cet-14418	32	22	for	for	ADP
cet-14418	32	23	evaluation	evaluation	NOUN
cet-14418	32	24	of	of	ADP
cet-14418	32	25	the	the	DET
cet-14418	32	26	permeability	permeability	NOUN
cet-14418	32	27	and	and	CCONJ
cet-14418	32	28	the	the	DET
cet-14418	32	29	effective	effective	ADJ
cet-14418	32	30	thermal	thermal	ADJ
cet-14418	32	31	conductivity	conductivity	NOUN
cet-14418	32	32	,	,	PUNCT
cet-14418	32	33	respectively	respectively	ADV
cet-14418	32	34	.	.	PUNCT
cet-14418	33	1	navier	navier	PROPN
cet-14418	33	2	–	–	PUNCT
cet-14418	33	3	stokes	stoke	NOUN
cet-14418	33	4	and	and	CCONJ
cet-14418	33	5	mass	mass	ADJ
cet-14418	33	6	conservation	conservation	NOUN
cet-14418	33	7	equations	equation	NOUN
cet-14418	33	8	were	be	AUX
cet-14418	33	9	used	use	VERB
cet-14418	33	10	for	for	ADP
cet-14418	33	11	the	the	DET
cet-14418	33	12	evaluation	evaluation	NOUN
cet-14418	33	13	of	of	ADP
cet-14418	33	14	the	the	DET
cet-14418	33	15	gas	gas	NOUN
cet-14418	33	16	flow	flow	NOUN
cet-14418	33	17	field	field	NOUN
cet-14418	33	18	and	and	CCONJ
cet-14418	33	19	the	the	DET
cet-14418	33	20	pressure	pressure	NOUN
cet-14418	33	21	in	in	ADP
cet-14418	33	22	the	the	DET
cet-14418	33	23	reactor	reactor	NOUN
cet-14418	33	24	.	.	PUNCT
cet-14418	34	1	the	the	DET
cet-14418	34	2	constant	constant	ADJ
cet-14418	34	3	gas	gas	NOUN
cet-14418	34	4	pressure	pressure	NOUN
cet-14418	34	5	1	1	NUM
cet-14418	34	6	pa	pa	NOUN
cet-14418	34	7	was	be	AUX
cet-14418	34	8	applied	apply	VERB
cet-14418	34	9	to	to	ADP
cet-14418	34	10	the	the	DET
cet-14418	34	11	inlet	inlet	NOUN
cet-14418	34	12	boundary	boundary	NOUN
cet-14418	34	13	and	and	CCONJ
cet-14418	34	14	the	the	DET
cet-14418	34	15	zero	zero	NUM
cet-14418	34	16	-	-	PUNCT
cet-14418	34	17	pressure	pressure	NOUN
cet-14418	34	18	condition	condition	NOUN
cet-14418	34	19	was	be	AUX
cet-14418	34	20	used	use	VERB
cet-14418	34	21	in	in	ADP
cet-14418	34	22	the	the	DET
cet-14418	34	23	outlet	outlet	NOUN
cet-14418	34	24	boundary	boundary	PROPN
cet-14418	34	25	opposite	opposite	ADV
cet-14418	34	26	to	to	ADP
cet-14418	34	27	the	the	DET
cet-14418	34	28	inlet	inlet	NOUN
cet-14418	34	29	boundary	boundary	NOUN
cet-14418	34	30	.	.	PUNCT
cet-14418	35	1	the	the	DET
cet-14418	35	2	permeability	permeability	NOUN
cet-14418	35	3	κmicro	κmicro	NOUN
cet-14418	35	4	of	of	ADP
cet-14418	35	5	the	the	DET
cet-14418	35	6	gas	gas	NOUN
cet-14418	35	7	flow	flow	NOUN
cet-14418	35	8	in	in	ADP
cet-14418	35	9	the	the	DET
cet-14418	35	10	micro	micro	NOUN
cet-14418	35	11	-	-	NOUN
cet-14418	35	12	scale	scale	NOUN
cet-14418	35	13	is	be	AUX
cet-14418	35	14	estimated	estimate	VERB
cet-14418	35	15	by	by	ADP
cet-14418	35	16	𝜅𝜅	𝜅𝜅	ADJ
cet-14418	35	17	=	=	PUNCT
cet-14418	35	18	𝜇𝜇𝑢𝑢𝑎𝑎𝑎𝑎𝑎𝑎(𝑑𝑑𝑑𝑑	𝜇𝜇𝑢𝑢𝑎𝑎𝑎𝑎𝑎𝑎(𝑑𝑑𝑑𝑑	PROPN
cet-14418	35	19	𝑑𝑑𝑑𝑑⁄	𝑑𝑑𝑑𝑑⁄	PART
cet-14418	35	20	)	)	PUNCT
cet-14418	35	21	−1	−1	NOUN
cet-14418	35	22	(	(	PUNCT
cet-14418	35	23	1	1	NUM
cet-14418	35	24	)	)	PUNCT
cet-14418	35	25	where	where	SCONJ
cet-14418	35	26	μ	μ	NOUN
cet-14418	35	27	,	,	PUNCT
cet-14418	35	28	uave	uave	VERB
cet-14418	35	29	,	,	PUNCT
cet-14418	35	30	and	and	CCONJ
cet-14418	35	31	x	x	AUX
cet-14418	35	32	represent	represent	VERB
cet-14418	35	33	the	the	DET
cet-14418	35	34	viscosity	viscosity	NOUN
cet-14418	35	35	,	,	PUNCT
cet-14418	35	36	the	the	DET
cet-14418	35	37	average	average	ADJ
cet-14418	35	38	flow	flow	NOUN
cet-14418	35	39	velocity	velocity	NOUN
cet-14418	35	40	,	,	PUNCT
cet-14418	35	41	and	and	CCONJ
cet-14418	35	42	the	the	DET
cet-14418	35	43	position	position	NOUN
cet-14418	35	44	of	of	ADP
cet-14418	35	45	the	the	DET
cet-14418	35	46	main	main	ADJ
cet-14418	35	47	flow	flow	NOUN
cet-14418	35	48	direction	direction	NOUN
cet-14418	35	49	,	,	PUNCT
cet-14418	35	50	respectively	respectively	ADV
cet-14418	35	51	.	.	PUNCT
cet-14418	36	1	the	the	DET
cet-14418	36	2	effective	effective	ADJ
cet-14418	36	3	diffusion	diffusion	NOUN
cet-14418	36	4	coefficient	coefficient	NOUN
cet-14418	36	5	of	of	ADP
cet-14418	36	6	the	the	DET
cet-14418	36	7	species	specie	NOUN
cet-14418	36	8	was	be	AUX
cet-14418	36	9	evaluated	evaluate	VERB
cet-14418	36	10	based	base	VERB
cet-14418	36	11	on	on	ADP
cet-14418	36	12	mass	mass	ADJ
cet-14418	36	13	conservation	conservation	NOUN
cet-14418	36	14	law	law	NOUN
cet-14418	36	15	,	,	PUNCT
cet-14418	36	16	𝛻𝛻	𝛻𝛻	ADJ
cet-14418	36	17	∙	∙	PROPN
cet-14418	36	18	(	(	PUNCT
cet-14418	36	19	𝐷𝐷𝑖𝑖𝛻𝛻𝑐𝑐𝑖𝑖	𝐷𝐷𝑖𝑖𝛻𝛻𝑐𝑐𝑖𝑖	PROPN
cet-14418	36	20	)	)	PUNCT
cet-14418	36	21	=	=	SYM
cet-14418	36	22	0	0	NUM
cet-14418	36	23	,	,	PUNCT
cet-14418	36	24	𝐷𝐷𝑎𝑎𝑒𝑒𝑒𝑒,𝑖𝑖	𝐷𝐷𝑎𝑎𝑒𝑒𝑒𝑒,𝑖𝑖	X
cet-14418	36	25	=	=	SYM
cet-14418	36	26	−𝑗𝑗𝑎𝑎𝑎𝑎𝑎𝑎,𝑖𝑖(𝑑𝑑𝑐𝑐	−𝑗𝑗𝑎𝑎𝑎𝑎𝑎𝑎,𝑖𝑖(𝑑𝑑𝑐𝑐	NOUN
cet-14418	36	27	𝑑𝑑𝑑𝑑⁄	𝑑𝑑𝑑𝑑⁄	PROPN
cet-14418	36	28	)	)	PUNCT
cet-14418	36	29	−1	−1	NOUN
cet-14418	36	30	(	(	PUNCT
cet-14418	36	31	2	2	NUM
cet-14418	36	32	)	)	PUNCT
cet-14418	36	33	where	where	SCONJ
cet-14418	36	34	c	c	NOUN
cet-14418	36	35	and	and	CCONJ
cet-14418	36	36	d	d	PROPN
cet-14418	36	37	represent	represent	VERB
cet-14418	36	38	the	the	DET
cet-14418	36	39	concentration	concentration	NOUN
cet-14418	36	40	and	and	CCONJ
cet-14418	36	41	the	the	DET
cet-14418	36	42	diffusion	diffusion	NOUN
cet-14418	36	43	coefficient	coefficient	NOUN
cet-14418	36	44	,	,	PUNCT
cet-14418	36	45	respectively	respectively	ADV
cet-14418	36	46	.	.	PUNCT
cet-14418	37	1	the	the	DET
cet-14418	37	2	suffix	suffix	PROPN
cet-14418	37	3	i	i	PRON
cet-14418	37	4	indicates	indicate	VERB
cet-14418	37	5	the	the	DET
cet-14418	37	6	species	species	NOUN
cet-14418	37	7	number	number	NOUN
cet-14418	37	8	(	(	PUNCT
cet-14418	37	9	i=1	i=1	PROPN
cet-14418	37	10	,	,	PUNCT
cet-14418	37	11	2	2	NUM
cet-14418	37	12	,	,	PUNCT
cet-14418	37	13	3	3	NUM
cet-14418	37	14	correspond	correspond	NOUN
cet-14418	37	15	to	to	ADP
cet-14418	37	16	co2	co2	NOUN
cet-14418	37	17	,	,	PUNCT
cet-14418	37	18	h2	h2	NOUN
cet-14418	37	19	,	,	PUNCT
cet-14418	37	20	and	and	CCONJ
cet-14418	37	21	ch3oh	ch3oh	ADV
cet-14418	37	22	,	,	PUNCT
cet-14418	37	23	respectively	respectively	ADV
cet-14418	37	24	)	)	PUNCT
cet-14418	37	25	.	.	PUNCT
cet-14418	38	1	jave	jave	PROPN
cet-14418	38	2	,	,	PUNCT
cet-14418	38	3	i	i	PRON
cet-14418	38	4	is	be	AUX
cet-14418	38	5	the	the	DET
cet-14418	38	6	average	average	ADJ
cet-14418	38	7	heat	heat	NOUN
cet-14418	38	8	flux	flux	NOUN
cet-14418	38	9	for	for	ADP
cet-14418	38	10	the	the	DET
cet-14418	38	11	direction	direction	NOUN
cet-14418	38	12	from	from	ADP
cet-14418	38	13	the	the	DET
cet-14418	38	14	inlet	inlet	NOUN
cet-14418	38	15	to	to	ADP
cet-14418	38	16	the	the	DET
cet-14418	38	17	outlet	outlet	NOUN
cet-14418	38	18	boundary	boundary	NOUN
cet-14418	38	19	.	.	PUNCT
cet-14418	39	1	note	note	VERB
cet-14418	39	2	that	that	SCONJ
cet-14418	39	3	the	the	DET
cet-14418	39	4	diffusion	diffusion	NOUN
cet-14418	39	5	simulation	simulation	NOUN
cet-14418	39	6	was	be	AUX
cet-14418	39	7	conducted	conduct	VERB
cet-14418	39	8	in	in	ADP
cet-14418	39	9	the	the	DET
cet-14418	39	10	pore	pore	ADJ
cet-14418	39	11	(	(	PUNCT
cet-14418	39	12	gas	gas	NOUN
cet-14418	39	13	)	)	PUNCT
cet-14418	39	14	region	region	NOUN
cet-14418	39	15	of	of	ADP
cet-14418	39	16	the	the	DET
cet-14418	39	17	micro	micro	ADJ
cet-14418	39	18	-	-	NOUN
cet-14418	39	19	scale	scale	ADJ
cet-14418	39	20	model	model	NOUN
cet-14418	39	21	.	.	PUNCT
cet-14418	40	1	table	table	NOUN
cet-14418	40	2	1	1	NUM
cet-14418	40	3	.	.	PUNCT
cet-14418	41	1	properties	property	NOUN
cet-14418	41	2	of	of	ADP
cet-14418	41	3	the	the	DET
cet-14418	41	4	gas	gas	NOUN
cet-14418	41	5	and	and	CCONJ
cet-14418	41	6	catalyst	catalyst	NOUN
cet-14418	41	7	bed	bed	NOUN
cet-14418	41	8	used	use	VERB
cet-14418	41	9	in	in	ADP
cet-14418	41	10	this	this	DET
cet-14418	41	11	study	study	NOUN
cet-14418	41	12	pellet	pellet	NOUN
cet-14418	41	13	catalyst	catalyst	NOUN
cet-14418	41	14	co2	co2	NOUN
cet-14418	41	15	h2	h2	NOUN
cet-14418	41	16	density	density	NOUN
cet-14418	41	17	(	(	PUNCT
cet-14418	41	18	kg	kg	NOUN
cet-14418	41	19	/	/	SYM
cet-14418	41	20	m3	m3	PROPN
cet-14418	41	21	]	]	SYM
cet-14418	41	22	)	)	PUNCT
cet-14418	41	23	2781	2781	NUM
cet-14418	41	24	1.42	1.42	NUM
cet-14418	41	25	0.063	0.063	NUM
cet-14418	41	26	viscosity	viscosity	NOUN
cet-14418	41	27	(	(	PUNCT
cet-14418	41	28	pa*s	pa*s	NOUN
cet-14418	41	29	)	)	PUNCT
cet-14418	41	30	2.15×10	2.15×10	NUM
cet-14418	41	31	-	-	SYM
cet-14418	41	32	5	5	NUM
cet-14418	41	33	2.15×10	2.15×10	NUM
cet-14418	41	34	-	-	SYM
cet-14418	41	35	5	5	NUM
cet-14418	41	36	specific	specific	ADJ
cet-14418	41	37	heat	heat	NOUN
cet-14418	41	38	(	(	PUNCT
cet-14418	41	39	j	j	PROPN
cet-14418	41	40	/	/	SYM
cet-14418	41	41	kg	kg	PROPN
cet-14418	41	42	)	)	PUNCT
cet-14418	42	1	1000	1000	NUM
cet-14418	42	2	919	919	NUM
cet-14418	42	3	14470	14470	NUM
cet-14418	42	4	thermal	thermal	ADJ
cet-14418	42	5	conductivity	conductivity	NOUN
cet-14418	42	6	(	(	PUNCT
cet-14418	42	7	w/(m2*k	w/(m2*k	ADV
cet-14418	42	8	)	)	PUNCT
cet-14418	42	9	)	)	PUNCT
cet-14418	43	1	1.0	1.0	NUM
cet-14418	43	2	0.022	0.022	NUM
cet-14418	43	3	0.23	0.23	NUM
cet-14418	43	4	2.3	2.3	NUM
cet-14418	43	5	simulation	simulation	NOUN
cet-14418	43	6	method	method	NOUN
cet-14418	43	7	of	of	ADP
cet-14418	43	8	macro	macro	ADJ
cet-14418	43	9	-	-	NOUN
cet-14418	43	10	scale	scale	NOUN
cet-14418	43	11	model	model	NOUN
cet-14418	43	12	the	the	DET
cet-14418	43	13	macro	macro	ADJ
cet-14418	43	14	-	-	NOUN
cet-14418	43	15	scale	scale	ADJ
cet-14418	43	16	2d	2d	NUM
cet-14418	43	17	axial	axial	ADJ
cet-14418	43	18	symmetric	symmetric	ADJ
cet-14418	43	19	homogeneous	homogeneous	ADJ
cet-14418	43	20	models	model	NOUN
cet-14418	43	21	were	be	AUX
cet-14418	43	22	constructed	construct	VERB
cet-14418	43	23	in	in	ADP
cet-14418	43	24	order	order	NOUN
cet-14418	43	25	to	to	PART
cet-14418	43	26	simulate	simulate	VERB
cet-14418	43	27	the	the	DET
cet-14418	43	28	reaction	reaction	NOUN
cet-14418	43	29	,	,	PUNCT
cet-14418	43	30	gas	gas	NOUN
cet-14418	43	31	flow	flow	NOUN
cet-14418	43	32	,	,	PUNCT
cet-14418	43	33	pressure	pressure	NOUN
cet-14418	43	34	,	,	PUNCT
cet-14418	43	35	and	and	CCONJ
cet-14418	43	36	temperature	temperature	NOUN
cet-14418	43	37	fields	field	NOUN
cet-14418	43	38	in	in	ADP
cet-14418	43	39	the	the	DET
cet-14418	43	40	reactor	reactor	NOUN
cet-14418	43	41	.	.	PUNCT
cet-14418	44	1	the	the	DET
cet-14418	44	2	parameters	parameter	NOUN
cet-14418	44	3	,	,	PUNCT
cet-14418	44	4	including	include	VERB
cet-14418	44	5	the	the	DET
cet-14418	44	6	effective	effective	ADJ
cet-14418	44	7	properties	property	NOUN
cet-14418	44	8	in	in	ADP
cet-14418	44	9	the	the	DET
cet-14418	44	10	catalyst	catalyst	NOUN
cet-14418	44	11	bed	bed	NOUN
cet-14418	44	12	,	,	PUNCT
cet-14418	44	13	were	be	AUX
cet-14418	44	14	based	base	VERB
cet-14418	44	15	on	on	ADP
cet-14418	44	16	the	the	DET
cet-14418	44	17	values	value	NOUN
cet-14418	44	18	obtained	obtain	VERB
cet-14418	44	19	by	by	ADP
cet-14418	44	20	the	the	DET
cet-14418	44	21	micro	micro	ADJ
cet-14418	44	22	-	-	NOUN
cet-14418	44	23	scale	scale	ADJ
cet-14418	44	24	model	model	NOUN
cet-14418	44	25	described	describe	VERB
cet-14418	44	26	in	in	ADP
cet-14418	44	27	2.2	2.2	NUM
cet-14418	44	28	.	.	PUNCT
cet-14418	45	1	the	the	DET
cet-14418	45	2	dimensions	dimension	NOUN
cet-14418	45	3	of	of	ADP
cet-14418	45	4	the	the	DET
cet-14418	45	5	reactor	reactor	NOUN
cet-14418	45	6	and	and	CCONJ
cet-14418	45	7	the	the	DET
cet-14418	45	8	catalyst	catalyst	NOUN
cet-14418	45	9	bed	bed	NOUN
cet-14418	45	10	layer	layer	NOUN
cet-14418	45	11	were	be	AUX
cet-14418	45	12	set	set	VERB
cet-14418	45	13	to	to	ADP
cet-14418	45	14	the	the	DET
cet-14418	45	15	same	same	ADJ
cet-14418	45	16	values	value	NOUN
cet-14418	45	17	as	as	ADP
cet-14418	45	18	in	in	ADP
cet-14418	45	19	the	the	DET
cet-14418	45	20	actual	actual	ADJ
cet-14418	45	21	experiment	experiment	NOUN
cet-14418	45	22	(	(	PUNCT
cet-14418	45	23	see	see	VERB
cet-14418	45	24	in	in	ADP
cet-14418	45	25	2.4	2.4	NUM
cet-14418	45	26	)	)	PUNCT
cet-14418	45	27	.	.	PUNCT
cet-14418	46	1	the	the	DET
cet-14418	46	2	boundary	boundary	ADJ
cet-14418	46	3	conditions	condition	NOUN
cet-14418	46	4	of	of	ADP
cet-14418	46	5	the	the	DET
cet-14418	46	6	reactor	reactor	NOUN
cet-14418	46	7	are	be	AUX
cet-14418	46	8	also	also	ADV
cet-14418	46	9	shown	show	VERB
cet-14418	46	10	in	in	ADP
cet-14418	46	11	fig.1	fig.1	PROPN
cet-14418	46	12	.	.	PUNCT
cet-14418	47	1	as	as	ADP
cet-14418	47	2	the	the	DET
cet-14418	47	3	governing	govern	VERB
cet-14418	47	4	equations	equation	NOUN
cet-14418	47	5	for	for	ADP
cet-14418	47	6	the	the	DET
cet-14418	47	7	gas	gas	NOUN
cet-14418	47	8	phase	phase	NOUN
cet-14418	47	9	in	in	ADP
cet-14418	47	10	the	the	DET
cet-14418	47	11	reactor	reactor	NOUN
cet-14418	47	12	,	,	PUNCT
cet-14418	47	13	the	the	DET
cet-14418	47	14	momentum	momentum	NOUN
cet-14418	47	15	conservation	conservation	NOUN
cet-14418	47	16	law	law	NOUN
cet-14418	47	17	,	,	PUNCT
cet-14418	47	18	mass	mass	ADJ
cet-14418	47	19	conservation	conservation	NOUN
cet-14418	47	20	law	law	NOUN
cet-14418	47	21	,	,	PUNCT
cet-14418	47	22	reaction	reaction	NOUN
cet-14418	47	23	equations	equation	NOUN
cet-14418	47	24	,	,	PUNCT
cet-14418	47	25	and	and	CCONJ
cet-14418	47	26	heat	heat	NOUN
cet-14418	47	27	transfer	transfer	NOUN
cet-14418	47	28	equation	equation	NOUN
cet-14418	47	29	were	be	AUX
cet-14418	47	30	used	use	VERB
cet-14418	47	31	.	.	PUNCT
cet-14418	48	1	the	the	DET
cet-14418	48	2	brinkman	brinkman	PROPN
cet-14418	48	3	equation	equation	NOUN
cet-14418	48	4	based	base	VERB
cet-14418	48	5	on	on	ADP
cet-14418	48	6	the	the	DET
cet-14418	48	7	darcy	darcy	PROPN
cet-14418	48	8	velocity	velocity	NOUN
cet-14418	48	9	and	and	CCONJ
cet-14418	48	10	pressure	pressure	NOUN
cet-14418	48	11	,	,	PUNCT
cet-14418	48	12	and	and	CCONJ
cet-14418	48	13	the	the	DET
cet-14418	48	14	mass	mass	ADJ
cet-14418	48	15	conservation	conservation	NOUN
cet-14418	48	16	law	law	NOUN
cet-14418	48	17	in	in	ADP
cet-14418	48	18	the	the	DET
cet-14418	48	19	porous	porous	ADJ
cet-14418	48	20	material	material	NOUN
cet-14418	48	21	were	be	AUX
cet-14418	48	22	adopted	adopt	VERB
cet-14418	48	23	(	(	PUNCT
cet-14418	48	24	alarcon	alarcon	PROPN
cet-14418	48	25	et	et	PROPN
cet-14418	48	26	al	al	PROPN
cet-14418	48	27	.	.	PROPN
cet-14418	48	28	,	,	PUNCT
cet-14418	48	29	2022	2022	NUM
cet-14418	48	30	)	)	PUNCT
cet-14418	48	31	using	use	VERB
cet-14418	48	32	the	the	DET
cet-14418	48	33	estimated	estimate	VERB
cet-14418	48	34	effective	effective	ADJ
cet-14418	48	35	permeability	permeability	NOUN
cet-14418	48	36	and	and	CCONJ
cet-14418	48	37	the	the	DET
cet-14418	48	38	porosity	porosity	NOUN
cet-14418	48	39	in	in	ADP
cet-14418	48	40	the	the	DET
cet-14418	48	41	micro	micro	ADJ
cet-14418	48	42	-	-	NOUN
cet-14418	48	43	scale	scale	ADJ
cet-14418	48	44	model	model	NOUN
cet-14418	48	45	.	.	PUNCT
cet-14418	48	46	44	44	NUM
cet-14418	48	47	although	although	SCONJ
cet-14418	48	48	the	the	DET
cet-14418	48	49	following	follow	VERB
cet-14418	48	50	overall	overall	ADJ
cet-14418	48	51	reactions	reaction	NOUN
cet-14418	48	52	of	of	ADP
cet-14418	48	53	co2	co2	NOUN
cet-14418	48	54	methanation	methanation	NOUN
cet-14418	48	55	(	(	PUNCT
cet-14418	48	56	3)-(5	3)-(5	NUM
cet-14418	48	57	)	)	PUNCT
cet-14418	48	58	were	be	AUX
cet-14418	48	59	proposed	propose	VERB
cet-14418	48	60	typically	typically	ADV
cet-14418	48	61	,	,	PUNCT
cet-14418	48	62	the	the	DET
cet-14418	48	63	reactions	reaction	NOUN
cet-14418	48	64	related	relate	VERB
cet-14418	48	65	to	to	PART
cet-14418	48	66	co	co	VERB
cet-14418	48	67	(	(	PUNCT
cet-14418	48	68	eq.(4	eq.(4	PROPN
cet-14418	48	69	)	)	PUNCT
cet-14418	48	70	)	)	PUNCT
cet-14418	48	71	are	be	AUX
cet-14418	48	72	omitted	omit	VERB
cet-14418	48	73	for	for	ADP
cet-14418	48	74	simplicity	simplicity	NOUN
cet-14418	48	75	(	(	PUNCT
cet-14418	48	76	taco	taco	PROPN
cet-14418	48	77	-	-	PUNCT
cet-14418	48	78	vasquez	vasquez	PROPN
cet-14418	48	79	et	et	PROPN
cet-14418	48	80	al	al	PROPN
cet-14418	48	81	.	.	PROPN
cet-14418	48	82	,	,	PUNCT
cet-14418	48	83	2022	2022	NUM
cet-14418	48	84	)	)	PUNCT
cet-14418	48	85	in	in	ADP
cet-14418	48	86	this	this	DET
cet-14418	48	87	study	study	NOUN
cet-14418	48	88	.	.	PUNCT
cet-14418	49	1	co2	co2	NOUN
cet-14418	49	2	+	+	CCONJ
cet-14418	49	3	3h2	3h2	NUM
cet-14418	49	4	⇄	⇄	ADJ
cet-14418	49	5	ch3oh	ch3oh	NOUN
cet-14418	49	6	+	+	NUM
cet-14418	49	7	h2o	h2o	PROPN
cet-14418	49	8	co	co	NOUN
cet-14418	49	9	+	+	CCONJ
cet-14418	49	10	2h2	2h2	NUM
cet-14418	49	11	⇄	⇄	ADJ
cet-14418	49	12	ch3oh	ch3oh	NOUN
cet-14418	49	13	co2	co2	NOUN
cet-14418	49	14	+	+	CCONJ
cet-14418	49	15	h2	h2	NOUN
cet-14418	49	16	⇄	⇄	ADJ
cet-14418	49	17	co	co	NOUN
cet-14418	49	18	+	+	PROPN
cet-14418	49	19	h2o	h2o	PROPN
cet-14418	49	20	(	(	PUNCT
cet-14418	49	21	3	3	NUM
cet-14418	49	22	)	)	PUNCT
cet-14418	49	23	(	(	PUNCT
cet-14418	49	24	4	4	NUM
cet-14418	49	25	)	)	PUNCT
cet-14418	49	26	(	(	PUNCT
cet-14418	49	27	5	5	X
cet-14418	49	28	)	)	PUNCT
cet-14418	49	29	the	the	DET
cet-14418	49	30	simplified	simplify	VERB
cet-14418	49	31	kinetic	kinetic	ADJ
cet-14418	49	32	model	model	NOUN
cet-14418	49	33	of	of	ADP
cet-14418	49	34	methanol	methanol	NOUN
cet-14418	49	35	synthesis	synthesis	NOUN
cet-14418	49	36	can	can	AUX
cet-14418	49	37	be	be	AUX
cet-14418	49	38	described	describe	VERB
cet-14418	49	39	as	as	ADP
cet-14418	49	40	𝑟𝑟	𝑟𝑟	ADP
cet-14418	49	41	=	=	NOUN
cet-14418	50	1	𝑘𝑘𝑒𝑒[co2][h2]3	𝑘𝑘𝑒𝑒[co2][h2]3	NOUN
cet-14418	50	2	−	−	PROPN
cet-14418	50	3	𝑘𝑘𝑟𝑟[ch3oh	𝑘𝑘𝑟𝑟[ch3oh	NOUN
cet-14418	50	4	]	]	X
cet-14418	50	5	(	(	PUNCT
cet-14418	50	6	6	6	NUM
cet-14418	50	7	)	)	PUNCT
cet-14418	50	8	where	where	SCONJ
cet-14418	50	9	kf	kf	PROPN
cet-14418	50	10	,	,	PUNCT
cet-14418	50	11	kr	kr	PROPN
cet-14418	50	12	indicate	indicate	VERB
cet-14418	50	13	the	the	DET
cet-14418	50	14	reaction	reaction	NOUN
cet-14418	50	15	rate	rate	NOUN
cet-14418	50	16	constant	constant	ADJ
cet-14418	50	17	for	for	ADP
cet-14418	50	18	ch3oh	ch3oh	NOUN
cet-14418	50	19	generation	generation	NOUN
cet-14418	50	20	and	and	CCONJ
cet-14418	50	21	decomposition	decomposition	NOUN
cet-14418	50	22	,	,	PUNCT
cet-14418	50	23	respectively	respectively	ADV
cet-14418	50	24	.	.	PUNCT
cet-14418	51	1	both	both	DET
cet-14418	51	2	rate	rate	NOUN
cet-14418	51	3	constants	constant	NOUN
cet-14418	51	4	are	be	AUX
cet-14418	51	5	assumed	assume	VERB
cet-14418	51	6	to	to	PART
cet-14418	51	7	follow	follow	VERB
cet-14418	51	8	the	the	DET
cet-14418	51	9	arrhenius	arrhenius	NOUN
cet-14418	51	10	form	form	NOUN
cet-14418	51	11	.	.	PUNCT
cet-14418	52	1	𝑘𝑘𝑒𝑒	𝑘𝑘𝑒𝑒	X
cet-14418	52	2	=	=	PUNCT
cet-14418	53	1	𝐴𝐴𝑒𝑒	𝐴𝐴𝑒𝑒	PROPN
cet-14418	53	2	�	�	NOUN
cet-14418	53	3	𝑇𝑇	𝑇𝑇	PROPN
cet-14418	53	4	𝑇𝑇𝑟𝑟𝑎𝑎𝑒𝑒⁄	𝑇𝑇𝑟𝑟𝑎𝑎𝑒𝑒⁄	PROPN
cet-14418	53	5	�	�	PROPN
cet-14418	53	6	exp	exp	NOUN
cet-14418	53	7	�	�	PROPN
cet-14418	53	8	−𝐸𝐸𝑒𝑒	−𝐸𝐸𝑒𝑒	ADJ
cet-14418	53	9	𝑅𝑅𝑔𝑔𝑇𝑇	𝑅𝑅𝑔𝑔𝑇𝑇	NUM
cet-14418	53	10	�	�	PROPN
cet-14418	53	11	�	�	PROPN
cet-14418	53	12	,	,	PUNCT
cet-14418	53	13	𝑘𝑘𝑟𝑟	𝑘𝑘𝑟𝑟	NOUN
cet-14418	53	14	=	=	PUNCT
cet-14418	54	1	𝐴𝐴𝑟𝑟	𝐴𝐴𝑟𝑟	PROPN
cet-14418	54	2	�	�	PROPN
cet-14418	54	3	𝑇𝑇	𝑇𝑇	PROPN
cet-14418	54	4	𝑇𝑇𝑟𝑟𝑎𝑎𝑒𝑒⁄	𝑇𝑇𝑟𝑟𝑎𝑎𝑒𝑒⁄	PROPN
cet-14418	54	5	�	�	PROPN
cet-14418	54	6	exp	exp	NOUN
cet-14418	54	7	�	�	PROPN
cet-14418	54	8	−𝐸𝐸𝑟𝑟	−𝐸𝐸𝑟𝑟	ADJ
cet-14418	54	9	𝑅𝑅𝑔𝑔𝑇𝑇⁄	𝑅𝑅𝑔𝑔𝑇𝑇⁄	PROPN
cet-14418	54	10	�	�	PROPN
cet-14418	54	11	(	(	PUNCT
cet-14418	54	12	7	7	NUM
cet-14418	54	13	)	)	PUNCT
cet-14418	54	14	where	where	SCONJ
cet-14418	54	15	t	t	NOUN
cet-14418	54	16	and	and	CCONJ
cet-14418	54	17	tref	tref	PROPN
cet-14418	54	18	indicate	indicate	VERB
cet-14418	54	19	the	the	DET
cet-14418	54	20	temperature	temperature	NOUN
cet-14418	54	21	in	in	ADP
cet-14418	54	22	the	the	DET
cet-14418	54	23	reactor	reactor	NOUN
cet-14418	54	24	and	and	CCONJ
cet-14418	54	25	the	the	DET
cet-14418	54	26	reference	reference	NOUN
cet-14418	54	27	temperature	temperature	NOUN
cet-14418	54	28	,	,	PUNCT
cet-14418	54	29	respectively	respectively	ADV
cet-14418	54	30	.	.	PUNCT
cet-14418	54	31	herein	herein	NOUN
cet-14418	54	32	,	,	PUNCT
cet-14418	54	33	the	the	DET
cet-14418	54	34	pre	pre	ADJ
cet-14418	54	35	-	-	ADJ
cet-14418	54	36	factor	factor	ADJ
cet-14418	54	37	value	value	NOUN
cet-14418	54	38	of	of	ADP
cet-14418	54	39	af	af	PROPN
cet-14418	54	40	,	,	PUNCT
cet-14418	54	41	and	and	CCONJ
cet-14418	54	42	ar	ar	NOUN
cet-14418	54	43	is	be	AUX
cet-14418	54	44	adopted	adopt	VERB
cet-14418	54	45	as	as	ADP
cet-14418	54	46	35	35	NUM
cet-14418	54	47	(	(	PUNCT
cet-14418	54	48	mol4	mol4	NOUN
cet-14418	54	49	s)-1	s)-1	PROPN
cet-14418	54	50	and	and	CCONJ
cet-14418	54	51	0.0035	0.0035	NUM
cet-14418	54	52	(	(	PUNCT
cet-14418	54	53	mol	mol	ADP
cet-14418	54	54	s	s	PROPN
cet-14418	54	55	)	)	PUNCT
cet-14418	54	56	-1	-1	ADJ
cet-14418	54	57	,	,	PUNCT
cet-14418	54	58	and	and	CCONJ
cet-14418	54	59	58700	58700	NUM
cet-14418	54	60	j	j	NOUN
cet-14418	54	61	/	/	SYM
cet-14418	54	62	mol	mol	PROPN
cet-14418	54	63	was	be	AUX
cet-14418	54	64	used	use	VERB
cet-14418	54	65	for	for	ADP
cet-14418	54	66	the	the	DET
cet-14418	54	67	activation	activation	NOUN
cet-14418	54	68	energy	energy	NOUN
cet-14418	54	69	both	both	CCONJ
cet-14418	54	70	ef	ef	PROPN
cet-14418	54	71	and	and	CCONJ
cet-14418	54	72	er	er	INTJ
cet-14418	54	73	.	.	PUNCT
cet-14418	55	1	due	due	ADP
cet-14418	55	2	to	to	ADP
cet-14418	55	3	the	the	DET
cet-14418	55	4	simplicity	simplicity	NOUN
cet-14418	55	5	of	of	ADP
cet-14418	55	6	this	this	DET
cet-14418	55	7	model	model	NOUN
cet-14418	55	8	,	,	PUNCT
cet-14418	55	9	direct	direct	ADJ
cet-14418	55	10	comparison	comparison	NOUN
cet-14418	55	11	with	with	ADP
cet-14418	55	12	previously	previously	ADV
cet-14418	55	13	studies	study	NOUN
cet-14418	55	14	using	use	VERB
cet-14418	55	15	the	the	DET
cet-14418	55	16	typical	typical	ADJ
cet-14418	55	17	vanden	vanden	PROPN
cet-14418	55	18	bussche	bussche	NOUN
cet-14418	55	19	and	and	CCONJ
cet-14418	55	20	froment	froment	PROPN
cet-14418	55	21	model	model	NOUN
cet-14418	55	22	(	(	PUNCT
cet-14418	55	23	shahrokhi	shahrokhi	INTJ
cet-14418	55	24	et	et	PROPN
cet-14418	55	25	al	al	PROPN
cet-14418	55	26	.	.	PROPN
cet-14418	55	27	,	,	PUNCT
cet-14418	55	28	2005	2005	NUM
cet-14418	55	29	)	)	PUNCT
cet-14418	55	30	is	be	AUX
cet-14418	55	31	not	not	PART
cet-14418	55	32	feasible	feasible	ADJ
cet-14418	55	33	.	.	PUNCT
cet-14418	56	1	however	however	ADV
cet-14418	56	2	,	,	PUNCT
cet-14418	56	3	the	the	DET
cet-14418	56	4	values	value	NOUN
cet-14418	56	5	of	of	ADP
cet-14418	56	6	the	the	DET
cet-14418	56	7	activation	activation	NOUN
cet-14418	56	8	energies	energy	NOUN
cet-14418	56	9	are	be	AUX
cet-14418	56	10	similar	similar	ADJ
cet-14418	56	11	.	.	PUNCT
cet-14418	57	1	the	the	DET
cet-14418	57	2	species	specie	NOUN
cet-14418	57	3	of	of	ADP
cet-14418	57	4	co2	co2	NOUN
cet-14418	57	5	,	,	PUNCT
cet-14418	57	6	h2	h2	NOUN
cet-14418	57	7	and	and	CCONJ
cet-14418	57	8	ch3oh	ch3oh	NUM
cet-14418	57	9	concentrations	concentration	NOUN
cet-14418	57	10	in	in	ADP
cet-14418	57	11	each	each	DET
cet-14418	57	12	time	time	NOUN
cet-14418	57	13	were	be	AUX
cet-14418	57	14	simulated	simulate	VERB
cet-14418	57	15	based	base	VERB
cet-14418	57	16	on	on	ADP
cet-14418	57	17	the	the	DET
cet-14418	57	18	time	time	NOUN
cet-14418	57	19	-	-	PUNCT
cet-14418	57	20	dependent	dependent	ADJ
cet-14418	57	21	mass	mass	NOUN
cet-14418	57	22	transportation	transportation	NOUN
cet-14418	57	23	equation	equation	NOUN
cet-14418	57	24	with	with	ADP
cet-14418	57	25	the	the	DET
cet-14418	57	26	convection	convection	NOUN
cet-14418	57	27	term	term	NOUN
cet-14418	57	28	𝜕𝜕𝑐𝑐𝑖𝑖	𝜕𝜕𝑐𝑐𝑖𝑖	ADJ
cet-14418	57	29	𝜕𝜕𝜕𝜕	𝜕𝜕𝜕𝜕	NOUN
cet-14418	57	30	=	=	PUNCT
cet-14418	57	31	𝛻𝛻	𝛻𝛻	PROPN
cet-14418	57	32	∙	∙	PROPN
cet-14418	57	33	(	(	PUNCT
cet-14418	57	34	𝐷𝐷𝑖𝑖𝛻𝛻𝑐𝑐𝑖𝑖	𝐷𝐷𝑖𝑖𝛻𝛻𝑐𝑐𝑖𝑖	PROPN
cet-14418	57	35	)	)	PUNCT
cet-14418	58	1	+	+	CCONJ
cet-14418	58	2	𝑢𝑢	𝑢𝑢	NUM
cet-14418	58	3	∙	∙	ADJ
cet-14418	58	4	𝛻𝛻𝑐𝑐𝑖𝑖	𝛻𝛻𝑐𝑐𝑖𝑖	NOUN
cet-14418	58	5	+	+	CCONJ
cet-14418	58	6	𝑅𝑅𝑖𝑖	𝑅𝑅𝑖𝑖	ADJ
cet-14418	58	7	,	,	PUNCT
cet-14418	58	8	𝜌𝜌𝐶𝐶𝑝𝑝	𝜌𝜌𝐶𝐶𝑝𝑝	PROPN
cet-14418	58	9	𝜕𝜕𝑇𝑇	𝜕𝜕𝑇𝑇	PROPN
cet-14418	58	10	𝜕𝜕𝜕𝜕	𝜕𝜕𝜕𝜕	PROPN
cet-14418	58	11	=	=	PUNCT
cet-14418	58	12	𝛻𝛻	𝛻𝛻	PROPN
cet-14418	58	13	∙	∙	PROPN
cet-14418	58	14	(	(	PUNCT
cet-14418	58	15	𝑘𝑘𝛻𝛻𝑇𝑇	𝑘𝑘𝛻𝛻𝑇𝑇	NOUN
cet-14418	58	16	)	)	PUNCT
cet-14418	59	1	+	+	CCONJ
cet-14418	59	2	𝑢𝑢	𝑢𝑢	ADP
cet-14418	59	3	∙	∙	PROPN
cet-14418	59	4	𝑘𝑘𝛻𝛻𝑇𝑇	𝑘𝑘𝛻𝛻𝑇𝑇	NOUN
cet-14418	59	5	(	(	PUNCT
cet-14418	59	6	8)	8)	NUM
cet-14418	59	7	where	where	SCONJ
cet-14418	59	8	ri	ri	PROPN
cet-14418	59	9	represents	represent	VERB
cet-14418	59	10	the	the	DET
cet-14418	59	11	reaction	reaction	NOUN
cet-14418	59	12	rate	rate	NOUN
cet-14418	59	13	.	.	PUNCT
cet-14418	60	1	the	the	DET
cet-14418	60	2	temperature	temperature	NOUN
cet-14418	60	3	in	in	ADP
cet-14418	60	4	the	the	DET
cet-14418	60	5	gas	gas	NOUN
cet-14418	60	6	phase	phase	NOUN
cet-14418	60	7	and	and	CCONJ
cet-14418	60	8	the	the	DET
cet-14418	60	9	catalyst	catalyst	NOUN
cet-14418	60	10	bed	bed	NOUN
cet-14418	60	11	were	be	AUX
cet-14418	60	12	evaluated	evaluate	VERB
cet-14418	60	13	by	by	ADP
cet-14418	60	14	the	the	DET
cet-14418	60	15	heat	heat	NOUN
cet-14418	60	16	transfer	transfer	NOUN
cet-14418	60	17	equation	equation	NOUN
cet-14418	60	18	.	.	PUNCT
cet-14418	61	1	2.4	2.4	NUM
cet-14418	61	2	experimental	experimental	ADJ
cet-14418	61	3	method	method	NOUN
cet-14418	61	4	of	of	ADP
cet-14418	61	5	methanol	methanol	NOUN
cet-14418	61	6	synthesis	synthesis	NOUN
cet-14418	61	7	the	the	DET
cet-14418	61	8	methanol	methanol	NOUN
cet-14418	61	9	synthesis	synthesis	NOUN
cet-14418	61	10	experiments	experiment	NOUN
cet-14418	61	11	with	with	ADP
cet-14418	61	12	a	a	DET
cet-14418	61	13	fixed	fix	VERB
cet-14418	61	14	catalyst	catalyst	NOUN
cet-14418	61	15	bed	bed	NOUN
cet-14418	61	16	were	be	AUX
cet-14418	61	17	conducted	conduct	VERB
cet-14418	61	18	in	in	ADP
cet-14418	61	19	order	order	NOUN
cet-14418	61	20	to	to	PART
cet-14418	61	21	validate	validate	VERB
cet-14418	61	22	the	the	DET
cet-14418	61	23	macroscale	macroscale	PROPN
cet-14418	61	24	model	model	NOUN
cet-14418	61	25	.	.	PUNCT
cet-14418	62	1	figure	figure	NOUN
cet-14418	62	2	2	2	NUM
cet-14418	62	3	illustrates	illustrate	VERB
cet-14418	62	4	the	the	DET
cet-14418	62	5	experimental	experimental	ADJ
cet-14418	62	6	set	set	VERB
cet-14418	62	7	up	up	ADP
cet-14418	62	8	.	.	PUNCT
cet-14418	63	1	a	a	DET
cet-14418	63	2	quartz	quartz	NOUN
cet-14418	63	3	tube	tube	NOUN
cet-14418	63	4	reactor	reactor	NOUN
cet-14418	63	5	with	with	ADP
cet-14418	63	6	an	an	DET
cet-14418	63	7	internal	internal	ADJ
cet-14418	63	8	diameter	diameter	NOUN
cet-14418	63	9	of	of	ADP
cet-14418	63	10	26	26	NUM
cet-14418	63	11	mm	mm	NOUN
cet-14418	63	12	and	and	CCONJ
cet-14418	63	13	4.25	4.25	NUM
cet-14418	63	14	mm	mm	NOUN
cet-14418	63	15	thickness	thickness	NOUN
cet-14418	63	16	was	be	AUX
cet-14418	63	17	used	use	VERB
cet-14418	63	18	,	,	PUNCT
cet-14418	63	19	and	and	CCONJ
cet-14418	63	20	zn.al2o3	zn.al2o3	NUM
cet-14418	63	21	tablet	tablet	NOUN
cet-14418	63	22	catalysts	catalyst	NOUN
cet-14418	63	23	were	be	AUX
cet-14418	63	24	placed	place	VERB
cet-14418	63	25	in	in	ADP
cet-14418	63	26	the	the	DET
cet-14418	63	27	middle	middle	NOUN
cet-14418	63	28	of	of	ADP
cet-14418	63	29	the	the	DET
cet-14418	63	30	reactor	reactor	NOUN
cet-14418	63	31	tube	tube	NOUN
cet-14418	63	32	.	.	PUNCT
cet-14418	64	1	the	the	DET
cet-14418	64	2	dry	dry	ADJ
cet-14418	64	3	co2	co2	NOUN
cet-14418	64	4	and	and	CCONJ
cet-14418	64	5	h2	h2	NOUN
cet-14418	64	6	gases	gas	NOUN
cet-14418	64	7	were	be	AUX
cet-14418	64	8	fed	feed	VERB
cet-14418	64	9	by	by	ADP
cet-14418	64	10	two	two	NUM
cet-14418	64	11	mass	mass	NOUN
cet-14418	64	12	flow	flow	NOUN
cet-14418	64	13	controllers	controller	NOUN
cet-14418	64	14	(	(	PUNCT
cet-14418	64	15	mfc	mfc	PROPN
cet-14418	64	16	)	)	PUNCT
cet-14418	64	17	with	with	ADP
cet-14418	64	18	the	the	DET
cet-14418	64	19	ratio	ratio	NOUN
cet-14418	64	20	of	of	ADP
cet-14418	64	21	co2	co2	NOUN
cet-14418	64	22	:	:	PUNCT
cet-14418	64	23	h2	h2	NOUN
cet-14418	64	24	=	=	SYM
cet-14418	64	25	8:2	8:2	NUM
cet-14418	64	26	,	,	PUNCT
cet-14418	64	27	and	and	CCONJ
cet-14418	64	28	the	the	DET
cet-14418	64	29	pressure	pressure	NOUN
cet-14418	64	30	in	in	ADP
cet-14418	64	31	the	the	DET
cet-14418	64	32	reactor	reactor	NOUN
cet-14418	64	33	was	be	AUX
cet-14418	64	34	maintained	maintain	VERB
cet-14418	64	35	at	at	ADP
cet-14418	64	36	0.4	0.4	NUM
cet-14418	64	37	mpa	mpa	PROPN
cet-14418	64	38	-	-	PUNCT
cet-14418	64	39	g.	g.	NOUN
cet-14418	64	40	the	the	DET
cet-14418	64	41	reactor	reactor	NOUN
cet-14418	64	42	was	be	AUX
cet-14418	64	43	heated	heat	VERB
cet-14418	64	44	to	to	ADP
cet-14418	64	45	210	210	NUM
cet-14418	64	46	℃	℃	PROPN
cet-14418	64	47	from	from	ADP
cet-14418	64	48	the	the	DET
cet-14418	64	49	periphery	periphery	NOUN
cet-14418	64	50	by	by	ADP
cet-14418	64	51	the	the	DET
cet-14418	64	52	electrical	electrical	ADJ
cet-14418	64	53	heating	heating	NOUN
cet-14418	64	54	wires	wire	NOUN
cet-14418	64	55	.	.	PUNCT
cet-14418	65	1	the	the	DET
cet-14418	65	2	gas	gas	NOUN
cet-14418	65	3	temperature	temperature	NOUN
cet-14418	65	4	was	be	AUX
cet-14418	65	5	monitored	monitor	VERB
cet-14418	65	6	at	at	ADP
cet-14418	65	7	the	the	DET
cet-14418	65	8	upper	upper	ADJ
cet-14418	65	9	surface	surface	NOUN
cet-14418	65	10	,	,	PUNCT
cet-14418	65	11	the	the	DET
cet-14418	65	12	middle	middle	NOUN
cet-14418	65	13	of	of	ADP
cet-14418	65	14	the	the	DET
cet-14418	65	15	catalyst	catalyst	NOUN
cet-14418	65	16	layer	layer	NOUN
cet-14418	65	17	,	,	PUNCT
cet-14418	65	18	and	and	CCONJ
cet-14418	65	19	the	the	DET
cet-14418	65	20	lower	low	ADJ
cet-14418	65	21	position	position	NOUN
cet-14418	65	22	in	in	ADP
cet-14418	65	23	the	the	DET
cet-14418	65	24	reaction	reaction	NOUN
cet-14418	65	25	tube	tube	NOUN
cet-14418	65	26	(	(	PUNCT
cet-14418	65	27	below	below	ADP
cet-14418	65	28	the	the	DET
cet-14418	65	29	catalyst	catalyst	NOUN
cet-14418	65	30	layer	layer	NOUN
cet-14418	65	31	)	)	PUNCT
cet-14418	65	32	.	.	PUNCT
cet-14418	66	1	after	after	ADP
cet-14418	66	2	passing	pass	VERB
cet-14418	66	3	through	through	ADP
cet-14418	66	4	the	the	DET
cet-14418	66	5	catalyst	catalyst	NOUN
cet-14418	66	6	layer	layer	NOUN
cet-14418	66	7	,	,	PUNCT
cet-14418	66	8	the	the	DET
cet-14418	66	9	gas	gas	NOUN
cet-14418	66	10	was	be	AUX
cet-14418	66	11	recovered	recover	VERB
cet-14418	66	12	and	and	CCONJ
cet-14418	66	13	the	the	DET
cet-14418	66	14	ch3oh	ch3oh	NUM
cet-14418	66	15	concentration	concentration	NOUN
cet-14418	66	16	was	be	AUX
cet-14418	66	17	analysed	analyse	VERB
cet-14418	66	18	.	.	PUNCT
cet-14418	67	1	the	the	DET
cet-14418	67	2	experiments	experiment	NOUN
cet-14418	67	3	consisted	consist	VERB
cet-14418	67	4	of	of	ADP
cet-14418	67	5	the	the	DET
cet-14418	67	6	following	follow	VERB
cet-14418	67	7	steps	step	NOUN
cet-14418	67	8	:	:	PUNCT
cet-14418	67	9	as	as	ADP
cet-14418	67	10	the	the	DET
cet-14418	67	11	first	first	ADJ
cet-14418	67	12	step	step	NOUN
cet-14418	67	13	,	,	PUNCT
cet-14418	67	14	a	a	DET
cet-14418	67	15	cold	cold	ADJ
cet-14418	67	16	-	-	PUNCT
cet-14418	67	17	case	case	NOUN
cet-14418	67	18	experiment	experiment	NOUN
cet-14418	67	19	(	(	PUNCT
cet-14418	67	20	without	without	ADP
cet-14418	67	21	reaction	reaction	NOUN
cet-14418	67	22	)	)	PUNCT
cet-14418	67	23	was	be	AUX
cet-14418	67	24	conducted	conduct	VERB
cet-14418	67	25	in	in	ADP
cet-14418	67	26	order	order	NOUN
cet-14418	67	27	to	to	PART
cet-14418	67	28	validate	validate	VERB
cet-14418	67	29	the	the	DET
cet-14418	67	30	micro	micro	ADJ
cet-14418	67	31	-	-	NOUN
cet-14418	67	32	scale	scale	ADJ
cet-14418	67	33	parameters	parameter	NOUN
cet-14418	67	34	estimated	estimate	VERB
cet-14418	67	35	in	in	ADP
cet-14418	67	36	the	the	DET
cet-14418	67	37	micro	micro	ADJ
cet-14418	67	38	-	-	NOUN
cet-14418	67	39	scale	scale	ADJ
cet-14418	67	40	simulation	simulation	NOUN
cet-14418	67	41	,	,	PUNCT
cet-14418	67	42	and	and	CCONJ
cet-14418	67	43	the	the	DET
cet-14418	67	44	methanol	methanol	NOUN
cet-14418	67	45	synthesis	synthesis	NOUN
cet-14418	67	46	experiments	experiment	NOUN
cet-14418	67	47	were	be	AUX
cet-14418	67	48	carried	carry	VERB
cet-14418	67	49	out	out	ADP
cet-14418	67	50	to	to	PART
cet-14418	67	51	validate	validate	VERB
cet-14418	67	52	the	the	DET
cet-14418	67	53	macro	macro	ADJ
cet-14418	67	54	-	-	NOUN
cet-14418	67	55	scale	scale	NOUN
cet-14418	67	56	model	model	NOUN
cet-14418	67	57	.	.	PUNCT
cet-14418	68	1	figure	figure	NOUN
cet-14418	68	2	2	2	NUM
cet-14418	68	3	.	.	PUNCT
cet-14418	68	4	experimental	experimental	ADJ
cet-14418	68	5	set	set	VERB
cet-14418	68	6	up	up	ADP
cet-14418	68	7	in	in	ADP
cet-14418	68	8	this	this	DET
cet-14418	68	9	study	study	NOUN
cet-14418	68	10	.	.	PUNCT
cet-14418	69	1	3	3	X
cet-14418	69	2	.	.	NOUN
cet-14418	69	3	results	result	VERB
cet-14418	69	4	3.1	3.1	NUM
cet-14418	69	5	model	model	NOUN
cet-14418	69	6	validation	validation	NOUN
cet-14418	69	7	the	the	DET
cet-14418	69	8	permeability	permeability	NOUN
cet-14418	69	9	,	,	PUNCT
cet-14418	69	10	effective	effective	ADJ
cet-14418	69	11	diffusion	diffusion	NOUN
cet-14418	69	12	coefficient	coefficient	NOUN
cet-14418	69	13	,	,	PUNCT
cet-14418	69	14	and	and	CCONJ
cet-14418	69	15	effective	effective	ADJ
cet-14418	69	16	thermal	thermal	ADJ
cet-14418	69	17	conductivity	conductivity	NOUN
cet-14418	69	18	of	of	ADP
cet-14418	69	19	the	the	DET
cet-14418	69	20	catalyst	catalyst	NOUN
cet-14418	69	21	beds	bed	NOUN
cet-14418	69	22	with	with	ADP
cet-14418	69	23	cylindrical	cylindrical	ADJ
cet-14418	69	24	pellet	pellet	NOUN
cet-14418	69	25	geometries	geometry	NOUN
cet-14418	69	26	were	be	AUX
cet-14418	69	27	estimated	estimate	VERB
cet-14418	69	28	using	use	VERB
cet-14418	69	29	the	the	DET
cet-14418	69	30	particle	particle	NOUN
cet-14418	69	31	-	-	PUNCT
cet-14418	69	32	resolved	resolve	VERB
cet-14418	69	33	micro	micro	ADJ
cet-14418	69	34	-	-	NOUN
cet-14418	69	35	scale	scale	ADJ
cet-14418	69	36	model	model	NOUN
cet-14418	69	37	.	.	PUNCT
cet-14418	70	1	figure	figure	NOUN
cet-14418	70	2	3	3	NUM
cet-14418	70	3	shows	show	VERB
cet-14418	70	4	the	the	DET
cet-14418	70	5	steady	steady	ADJ
cet-14418	70	6	-	-	PUNCT
cet-14418	70	7	state	state	NOUN
cet-14418	70	8	pressure	pressure	NOUN
cet-14418	70	9	,	,	PUNCT
cet-14418	70	10	concentration	concentration	NOUN
cet-14418	70	11	distribution	distribution	NOUN
cet-14418	70	12	of	of	ADP
cet-14418	70	13	the	the	DET
cet-14418	70	14	gas	gas	NOUN
cet-14418	70	15	phase	phase	NOUN
cet-14418	70	16	,	,	PUNCT
cet-14418	70	17	and	and	CCONJ
cet-14418	70	18	the	the	DET
cet-14418	70	19	temperature	temperature	NOUN
cet-14418	70	20	distribution	distribution	NOUN
cet-14418	70	21	.	.	PUNCT
cet-14418	71	1	each	each	DET
cet-14418	71	2	gradient	gradient	NOUN
cet-14418	71	3	is	be	AUX
cet-14418	71	4	formed	form	VERB
cet-14418	71	5	from	from	ADP
cet-14418	71	6	the	the	DET
cet-14418	71	7	inlet	inlet	NOUN
cet-14418	71	8	to	to	PART
cet-14418	71	9	outlet	outlet	NOUN
cet-14418	71	10	boundary	boundary	ADJ
cet-14418	71	11	through	through	ADP
cet-14418	71	12	the	the	DET
cet-14418	71	13	pore	pore	ADJ
cet-14418	71	14	region	region	NOUN
cet-14418	71	15	.	.	PUNCT
cet-14418	72	1	the	the	DET
cet-14418	72	2	volume	volume	NOUN
cet-14418	72	3	fraction	fraction	NOUN
cet-14418	72	4	of	of	ADP
cet-14418	72	5	the	the	DET
cet-14418	72	6	pellets	pellet	NOUN
cet-14418	72	7	,	,	PUNCT
cet-14418	72	8	the	the	DET
cet-14418	72	9	specific	specific	ADJ
cet-14418	72	10	surface	surface	NOUN
cet-14418	72	11	area	area	NOUN
cet-14418	72	12	,	,	PUNCT
cet-14418	72	13	and	and	CCONJ
cet-14418	72	14	the	the	DET
cet-14418	72	15	estimated	estimate	VERB
cet-14418	72	16	permeability	permeability	NOUN
cet-14418	72	17	by	by	ADP
cet-14418	72	18	eq.(1	eq.(1	ADJ
cet-14418	72	19	)	)	PUNCT
cet-14418	72	20	are	be	AUX
cet-14418	72	21	listed	list	VERB
cet-14418	72	22	in	in	ADP
cet-14418	72	23	table	table	NOUN
cet-14418	72	24	2	2	NUM
cet-14418	72	25	.	.	PUNCT
cet-14418	73	1	in	in	ADP
cet-14418	73	2	addition	addition	NOUN
cet-14418	73	3	,	,	PUNCT
cet-14418	73	4	the	the	DET
cet-14418	73	5	permeability	permeability	NOUN
cet-14418	73	6	was	be	AUX
cet-14418	73	7	compared	compare	VERB
cet-14418	73	8	with	with	ADP
cet-14418	73	9	the	the	DET
cet-14418	73	10	value	value	NOUN
cet-14418	73	11	estimated	estimate	VERB
cet-14418	73	12	by	by	ADP
cet-14418	73	13	the	the	DET
cet-14418	73	14	kozeny	kozeny	PROPN
cet-14418	73	15	–	–	PUNCT
cet-14418	73	16	carman	carman	NOUN
cet-14418	73	17	equation	equation	NOUN
cet-14418	73	18	,	,	PUNCT
cet-14418	73	19	assuming	assume	VERB
cet-14418	73	20	laminar	laminar	ADJ
cet-14418	73	21	flow	flow	NOUN
cet-14418	73	22	,	,	PUNCT
cet-14418	73	23	45	45	NUM
cet-14418	73	24	𝜅𝜅	𝜅𝜅	ADJ
cet-14418	73	25	=	=	PUNCT
cet-14418	73	26	�	�	PROPN
cet-14418	73	27	φ2𝐷𝐷𝑝𝑝2	φ2𝐷𝐷𝑝𝑝2	PROPN
cet-14418	73	28	180⁄	180⁄	NUM
cet-14418	73	29	�	�	PROPN
cet-14418	73	30	(	(	PUNCT
cet-14418	73	31	𝜀𝜀3	𝜀𝜀3	NOUN
cet-14418	73	32	(	(	PUNCT
cet-14418	73	33	1−	1−	NUM
cet-14418	73	34	𝜀𝜀)2⁄	𝜀𝜀)2⁄	NOUN
cet-14418	73	35	)	)	PUNCT
cet-14418	73	36	(	(	PUNCT
cet-14418	73	37	9	9	X
cet-14418	73	38	)	)	PUNCT
cet-14418	73	39	where	where	SCONJ
cet-14418	73	40	dp	dp	NOUN
cet-14418	73	41	,	,	PUNCT
cet-14418	73	42	ε	ε	PROPN
cet-14418	73	43	,	,	PUNCT
cet-14418	73	44	and	and	CCONJ
cet-14418	73	45	φ	φ	PROPN
cet-14418	73	46	indicate	indicate	VERB
cet-14418	73	47	the	the	DET
cet-14418	73	48	particle	particle	NOUN
cet-14418	73	49	diameter	diameter	NOUN
cet-14418	73	50	,	,	PUNCT
cet-14418	73	51	porosity	porosity	NOUN
cet-14418	73	52	,	,	PUNCT
cet-14418	73	53	and	and	CCONJ
cet-14418	73	54	sphericity	sphericity	NOUN
cet-14418	73	55	,	,	PUNCT
cet-14418	73	56	respectively	respectively	ADV
cet-14418	73	57	.	.	PUNCT
cet-14418	74	1	the	the	DET
cet-14418	74	2	sphericity	sphericity	PROPN
cet-14418	74	3	φ	φ	PROPN
cet-14418	74	4	is	be	AUX
cet-14418	74	5	defined	define	VERB
cet-14418	74	6	as	as	ADP
cet-14418	74	7	φ	φ	PROPN
cet-14418	74	8	=	=	SYM
cet-14418	74	9	ss	ss	PROPN
cet-14418	74	10	/	/	SYM
cet-14418	74	11	sp	sp	NOUN
cet-14418	74	12	,	,	PUNCT
cet-14418	74	13	where	where	SCONJ
cet-14418	74	14	sp	sp	NOUN
cet-14418	75	1	and	and	CCONJ
cet-14418	75	2	ss	ss	PROPN
cet-14418	75	3	represent	represent	VERB
cet-14418	75	4	the	the	DET
cet-14418	75	5	surface	surface	NOUN
cet-14418	75	6	area	area	NOUN
cet-14418	75	7	of	of	ADP
cet-14418	75	8	the	the	DET
cet-14418	75	9	particle	particle	NOUN
cet-14418	75	10	(	(	PUNCT
cet-14418	75	11	cylinder	cylinder	NOUN
cet-14418	75	12	)	)	PUNCT
cet-14418	75	13	and	and	CCONJ
cet-14418	75	14	those	those	PRON
cet-14418	75	15	of	of	ADP
cet-14418	75	16	a	a	DET
cet-14418	75	17	sphere	sphere	NOUN
cet-14418	75	18	which	which	PRON
cet-14418	75	19	has	have	VERB
cet-14418	75	20	the	the	DET
cet-14418	75	21	same	same	ADJ
cet-14418	75	22	volume	volume	NOUN
cet-14418	75	23	as	as	ADP
cet-14418	75	24	the	the	DET
cet-14418	75	25	particle	particle	NOUN
cet-14418	75	26	,	,	PUNCT
cet-14418	75	27	respectively	respectively	ADV
cet-14418	75	28	.	.	PUNCT
cet-14418	76	1	both	both	DET
cet-14418	76	2	permeability	permeability	NOUN
cet-14418	76	3	values	value	NOUN
cet-14418	76	4	agree	agree	VERB
cet-14418	76	5	well	well	ADV
cet-14418	76	6	,	,	PUNCT
cet-14418	76	7	indicating	indicate	VERB
cet-14418	76	8	that	that	SCONJ
cet-14418	76	9	the	the	DET
cet-14418	76	10	conditions	condition	NOUN
cet-14418	76	11	including	include	VERB
cet-14418	76	12	the	the	DET
cet-14418	76	13	cell	cell	NOUN
cet-14418	76	14	size	size	NOUN
cet-14418	76	15	and	and	CCONJ
cet-14418	76	16	mesh	mesh	NOUN
cet-14418	76	17	density	density	NOUN
cet-14418	76	18	in	in	ADP
cet-14418	76	19	the	the	DET
cet-14418	76	20	micro	micro	ADJ
cet-14418	76	21	-	-	NOUN
cet-14418	76	22	scale	scale	ADJ
cet-14418	76	23	model	model	NOUN
cet-14418	76	24	are	be	AUX
cet-14418	76	25	valid	valid	ADJ
cet-14418	76	26	for	for	ADP
cet-14418	76	27	estimating	estimate	VERB
cet-14418	76	28	permeability	permeability	NOUN
cet-14418	76	29	.	.	PUNCT
cet-14418	77	1	figure	figure	NOUN
cet-14418	77	2	3	3	NUM
cet-14418	77	3	.	.	PUNCT
cet-14418	78	1	(	(	PUNCT
cet-14418	78	2	a	a	X
cet-14418	78	3	)	)	PUNCT
cet-14418	78	4	pressure	pressure	NOUN
cet-14418	78	5	,	,	PUNCT
cet-14418	78	6	(	(	PUNCT
cet-14418	78	7	b	b	NOUN
cet-14418	78	8	)	)	PUNCT
cet-14418	78	9	concentration	concentration	NOUN
cet-14418	78	10	and	and	CCONJ
cet-14418	78	11	(	(	PUNCT
cet-14418	78	12	c	c	NOUN
cet-14418	78	13	)	)	PUNCT
cet-14418	78	14	temperature	temperature	NOUN
cet-14418	78	15	distributions	distribution	NOUN
cet-14418	78	16	in	in	ADP
cet-14418	78	17	sphere	sphere	NOUN
cet-14418	78	18	-	-	PUNCT
cet-14418	78	19	packed	pack	VERB
cet-14418	78	20	micro	micro	ADJ
cet-14418	78	21	-	-	NOUN
cet-14418	78	22	scale	scale	ADJ
cet-14418	78	23	model	model	NOUN
cet-14418	78	24	.	.	PUNCT
cet-14418	79	1	table	table	NOUN
cet-14418	79	2	2	2	NUM
cet-14418	79	3	.	.	PUNCT
cet-14418	79	4	geometry	geometry	NOUN
cet-14418	79	5	parameters	parameter	NOUN
cet-14418	79	6	and	and	CCONJ
cet-14418	79	7	estimated	estimate	VERB
cet-14418	79	8	permeability	permeability	NOUN
cet-14418	79	9	in	in	ADP
cet-14418	79	10	cylinder	cylinder	NOUN
cet-14418	79	11	-	-	PUNCT
cet-14418	79	12	packed	pack	VERB
cet-14418	79	13	structure	structure	NOUN
cet-14418	79	14	.	.	PUNCT
cet-14418	80	1	volume	volume	NOUN
cet-14418	80	2	fraction	fraction	NOUN
cet-14418	80	3	(	(	PUNCT
cet-14418	80	4	-	-	PUNCT
cet-14418	80	5	)	)	PUNCT
cet-14418	80	6	specific	specific	ADJ
cet-14418	80	7	surface	surface	NOUN
cet-14418	80	8	area	area	NOUN
cet-14418	80	9	(	(	PUNCT
cet-14418	80	10	1	1	NUM
cet-14418	80	11	/	/	SYM
cet-14418	80	12	m	m	NOUN
cet-14418	80	13	)	)	PUNCT
cet-14418	80	14	permeability	permeability	NOUN
cet-14418	80	15	(	(	PUNCT
cet-14418	80	16	m2	m2	PROPN
cet-14418	80	17	)	)	PUNCT
cet-14418	80	18	micro	micro	ADJ
cet-14418	80	19	-	-	NOUN
cet-14418	80	20	scale	scale	ADJ
cet-14418	80	21	model	model	NOUN
cet-14418	80	22	0.498	0.498	NUM
cet-14418	80	23	838	838	NUM
cet-14418	80	24	1.13×10	1.13×10	NUM
cet-14418	80	25	-	-	SYM
cet-14418	80	26	8	8	NUM
cet-14418	80	27	kozeny	kozeny	NOUN
cet-14418	80	28	–	–	PUNCT
cet-14418	80	29	carman	carman	NOUN
cet-14418	80	30	eq	eq	PROPN
cet-14418	80	31	.	.	PROPN
cet-14418	80	32	1.19×10	1.19×10	NUM
cet-14418	80	33	-	-	SYM
cet-14418	80	34	8	8	NUM
cet-14418	80	35	the	the	DET
cet-14418	80	36	effective	effective	ADJ
cet-14418	80	37	thermal	thermal	ADJ
cet-14418	80	38	conductivity	conductivity	NOUN
cet-14418	80	39	and	and	CCONJ
cet-14418	80	40	the	the	DET
cet-14418	80	41	effective	effective	ADJ
cet-14418	80	42	diffusion	diffusion	NOUN
cet-14418	80	43	coefficient	coefficient	NOUN
cet-14418	80	44	in	in	ADP
cet-14418	80	45	each	each	DET
cet-14418	80	46	gas	gas	NOUN
cet-14418	80	47	species	specie	NOUN
cet-14418	80	48	,	,	PUNCT
cet-14418	80	49	are	be	AUX
cet-14418	80	50	shown	show	VERB
cet-14418	80	51	in	in	ADP
cet-14418	80	52	table	table	NOUN
cet-14418	80	53	3	3	NUM
cet-14418	80	54	.	.	PUNCT
cet-14418	81	1	for	for	ADP
cet-14418	81	2	comparison	comparison	NOUN
cet-14418	81	3	,	,	PUNCT
cet-14418	81	4	we	we	PRON
cet-14418	81	5	also	also	ADV
cet-14418	81	6	estimated	estimate	VERB
cet-14418	81	7	both	both	DET
cet-14418	81	8	values	value	NOUN
cet-14418	81	9	based	base	VERB
cet-14418	81	10	on	on	ADP
cet-14418	81	11	bruggeman	bruggeman	PROPN
cet-14418	81	12	’s	’s	PART
cet-14418	81	13	equation	equation	NOUN
cet-14418	81	14	𝑘𝑘𝑎𝑎𝑒𝑒𝑒𝑒	𝑘𝑘𝑎𝑎𝑒𝑒𝑒𝑒	NOUN
cet-14418	81	15	=	=	PRON
cet-14418	81	16	𝑘𝑘1𝜀𝜀𝑛𝑛	𝑘𝑘1𝜀𝜀𝑛𝑛	X
cet-14418	81	17	,	,	PUNCT
cet-14418	81	18	𝐷𝐷𝑎𝑎𝑒𝑒𝑒𝑒,𝑖𝑖	𝐷𝐷𝑎𝑎𝑒𝑒𝑒𝑒,𝑖𝑖	PROPN
cet-14418	81	19	=	=	SYM
cet-14418	81	20	𝐷𝐷0,𝑖𝑖𝜀𝜀𝑛𝑛	𝐷𝐷0,𝑖𝑖𝜀𝜀𝑛𝑛	PROPN
cet-14418	81	21	(	(	PUNCT
cet-14418	81	22	10	10	NUM
cet-14418	81	23	)	)	PUNCT
cet-14418	81	24	where	where	SCONJ
cet-14418	81	25	k1	k1	NOUN
cet-14418	81	26	and	and	CCONJ
cet-14418	81	27	d0	d0	NOUN
cet-14418	81	28	indicate	indicate	VERB
cet-14418	81	29	the	the	DET
cet-14418	81	30	bulk	bulk	ADJ
cet-14418	81	31	thermal	thermal	ADJ
cet-14418	81	32	conductivity	conductivity	NOUN
cet-14418	81	33	and	and	CCONJ
cet-14418	81	34	diffusion	diffusion	NOUN
cet-14418	81	35	coefficient	coefficient	NOUN
cet-14418	81	36	,	,	PUNCT
cet-14418	81	37	and	and	CCONJ
cet-14418	81	38	n	n	PRON
cet-14418	81	39	means	mean	VERB
cet-14418	81	40	the	the	DET
cet-14418	81	41	constant	constant	ADJ
cet-14418	81	42	(	(	PUNCT
cet-14418	81	43	1.5	1.5	NUM
cet-14418	81	44	was	be	AUX
cet-14418	81	45	assumed	assume	VERB
cet-14418	81	46	in	in	ADP
cet-14418	81	47	this	this	DET
cet-14418	81	48	study	study	NOUN
cet-14418	81	49	)	)	PUNCT
cet-14418	81	50	.	.	PUNCT
cet-14418	82	1	the	the	DET
cet-14418	82	2	values	value	NOUN
cet-14418	82	3	estimated	estimate	VERB
cet-14418	82	4	by	by	ADP
cet-14418	82	5	the	the	DET
cet-14418	82	6	micro	micro	ADJ
cet-14418	82	7	-	-	NOUN
cet-14418	82	8	scale	scale	ADJ
cet-14418	82	9	model	model	NOUN
cet-14418	82	10	are	be	AUX
cet-14418	82	11	close	close	ADJ
cet-14418	82	12	to	to	ADP
cet-14418	82	13	those	those	PRON
cet-14418	82	14	estimated	estimate	VERB
cet-14418	82	15	by	by	ADP
cet-14418	82	16	eq	eq	PROPN
cet-14418	82	17	.	.	PUNCT
cet-14418	83	1	(	(	PUNCT
cet-14418	83	2	10	10	NUM
cet-14418	83	3	)	)	PUNCT
cet-14418	83	4	,	,	PUNCT
cet-14418	83	5	whereas	whereas	SCONJ
cet-14418	83	6	the	the	DET
cet-14418	83	7	effective	effective	ADJ
cet-14418	83	8	thermal	thermal	ADJ
cet-14418	83	9	conductivity	conductivity	NOUN
cet-14418	83	10	of	of	ADP
cet-14418	83	11	the	the	DET
cet-14418	83	12	micro	micro	ADJ
cet-14418	83	13	-	-	NOUN
cet-14418	83	14	scale	scale	ADJ
cet-14418	83	15	model	model	NOUN
cet-14418	83	16	is	be	AUX
cet-14418	83	17	slightly	slightly	ADV
cet-14418	83	18	larger	large	ADJ
cet-14418	83	19	.	.	PUNCT
cet-14418	84	1	this	this	PRON
cet-14418	84	2	indicates	indicate	VERB
cet-14418	84	3	that	that	SCONJ
cet-14418	84	4	the	the	DET
cet-14418	84	5	conditions	condition	NOUN
cet-14418	84	6	in	in	ADP
cet-14418	84	7	the	the	DET
cet-14418	84	8	micro	micro	ADJ
cet-14418	84	9	-	-	NOUN
cet-14418	84	10	scale	scale	ADJ
cet-14418	84	11	model	model	NOUN
cet-14418	84	12	are	be	AUX
cet-14418	84	13	valid	valid	ADJ
cet-14418	84	14	not	not	PART
cet-14418	84	15	only	only	ADV
cet-14418	84	16	for	for	ADP
cet-14418	84	17	the	the	DET
cet-14418	84	18	permeability	permeability	NOUN
cet-14418	84	19	but	but	CCONJ
cet-14418	84	20	also	also	ADV
cet-14418	84	21	the	the	DET
cet-14418	84	22	effective	effective	ADJ
cet-14418	84	23	thermal	thermal	ADJ
cet-14418	84	24	conductivity	conductivity	NOUN
cet-14418	84	25	and	and	CCONJ
cet-14418	84	26	diffusion	diffusion	NOUN
cet-14418	84	27	coefficients	coefficient	NOUN
cet-14418	84	28	.	.	PUNCT
cet-14418	85	1	table	table	NOUN
cet-14418	85	2	3	3	NUM
cet-14418	85	3	.	.	PUNCT
cet-14418	86	1	estimated	estimate	VERB
cet-14418	86	2	effective	effective	ADJ
cet-14418	86	3	thermal	thermal	ADJ
cet-14418	86	4	conductivities	conductivity	NOUN
cet-14418	86	5	and	and	CCONJ
cet-14418	86	6	diffusion	diffusion	NOUN
cet-14418	86	7	coefficients	coefficient	NOUN
cet-14418	86	8	.	.	PUNCT
cet-14418	87	1	𝑘𝑘𝑎𝑎𝑒𝑒𝑒𝑒	𝑘𝑘𝑎𝑎𝑒𝑒𝑒𝑒	PROPN
cet-14418	88	1	[	[	X
cet-14418	88	2	w/(m2s	w/(m2s	X
cet-14418	88	3	)	)	PUNCT
cet-14418	88	4	]	]	PUNCT
cet-14418	88	5	𝐷𝐷𝑎𝑎𝑒𝑒𝑒𝑒,𝑖𝑖	𝐷𝐷𝑎𝑎𝑒𝑒𝑒𝑒,𝑖𝑖	VERB
cet-14418	89	1	[	[	X
cet-14418	89	2	m2	m2	PROPN
cet-14418	89	3	/	/	SYM
cet-14418	89	4	s	s	PROPN
cet-14418	89	5	]	]	X
cet-14418	89	6	h2	h2	PROPN
cet-14418	89	7	o2	o2	PROPN
cet-14418	89	8	ch3oh	ch3oh	PROPN
cet-14418	89	9	micro	micro	NOUN
cet-14418	89	10	-	-	NOUN
cet-14418	89	11	scale	scale	ADJ
cet-14418	89	12	model	model	NOUN
cet-14418	89	13	0.133	0.133	NUM
cet-14418	89	14	4.91×10	4.91×10	NUM
cet-14418	89	15	-	-	SYM
cet-14418	89	16	5	5	NUM
cet-14418	89	17	1.09×10	1.09×10	NUM
cet-14418	89	18	-	-	SYM
cet-14418	89	19	5	5	NUM
cet-14418	89	20	4.67×10	4.67×10	NUM
cet-14418	89	21	-	-	PUNCT
cet-14418	89	22	6	6	NUM
cet-14418	89	23	bruggeman	bruggeman	NOUN
cet-14418	89	24	0.165	0.165	NUM
cet-14418	89	25	5.35×10	5.35×10	NUM
cet-14418	89	26	-	-	SYM
cet-14418	89	27	5	5	NUM
cet-14418	89	28	1.19×10	1.19×10	NUM
cet-14418	89	29	-	-	SYM
cet-14418	89	30	5	5	NUM
cet-14418	89	31	5.09×10	5.09×10	NUM
cet-14418	89	32	-	-	SYM
cet-14418	89	33	6	6	NUM
cet-14418	89	34	figure	figure	NOUN
cet-14418	89	35	4	4	NUM
cet-14418	89	36	.	.	NOUN
cet-14418	89	37	comparison	comparison	NOUN
cet-14418	89	38	of	of	ADP
cet-14418	89	39	temperature	temperature	NOUN
cet-14418	89	40	distribution	distribution	NOUN
cet-14418	89	41	in	in	ADP
cet-14418	89	42	(	(	PUNCT
cet-14418	89	43	a	a	PRON
cet-14418	89	44	)	)	PUNCT
cet-14418	89	45	cold	cold	ADJ
cet-14418	89	46	case	case	NOUN
cet-14418	89	47	and	and	CCONJ
cet-14418	89	48	(	(	PUNCT
cet-14418	89	49	b	b	NOUN
cet-14418	89	50	)	)	PUNCT
cet-14418	89	51	methanol	methanol	NOUN
cet-14418	89	52	synthesis	synthesis	NOUN
cet-14418	89	53	,	,	PUNCT
cet-14418	89	54	(	(	PUNCT
cet-14418	89	55	c	c	NOUN
cet-14418	89	56	)	)	PUNCT
cet-14418	89	57	simulated	simulated	ADJ
cet-14418	89	58	temperature	temperature	NOUN
cet-14418	89	59	,	,	PUNCT
cet-14418	89	60	(	(	PUNCT
cet-14418	89	61	d	d	NOUN
cet-14418	89	62	)	)	PUNCT
cet-14418	89	63	ch3oh	ch3oh	NOUN
cet-14418	90	1	concentration	concentration	NOUN
cet-14418	90	2	.	.	PUNCT
cet-14418	91	1	the	the	DET
cet-14418	91	2	2d	2d	PROPN
cet-14418	91	3	axial	axial	ADJ
cet-14418	91	4	symmetric	symmetric	ADJ
cet-14418	91	5	homogeneous	homogeneous	ADJ
cet-14418	91	6	model	model	NOUN
cet-14418	91	7	(	(	PUNCT
cet-14418	91	8	macro	macro	ADJ
cet-14418	91	9	-	-	NOUN
cet-14418	91	10	scale	scale	NOUN
cet-14418	91	11	model	model	NOUN
cet-14418	91	12	)	)	PUNCT
cet-14418	91	13	was	be	AUX
cet-14418	91	14	validated	validate	VERB
cet-14418	91	15	to	to	ADP
cet-14418	91	16	the	the	DET
cet-14418	91	17	experimental	experimental	ADJ
cet-14418	91	18	results	result	NOUN
cet-14418	91	19	of	of	ADP
cet-14418	91	20	the	the	DET
cet-14418	91	21	cold	cold	ADJ
cet-14418	91	22	case	case	NOUN
cet-14418	91	23	(	(	PUNCT
cet-14418	91	24	without	without	ADP
cet-14418	91	25	reaction	reaction	NOUN
cet-14418	91	26	)	)	PUNCT
cet-14418	91	27	and	and	CCONJ
cet-14418	91	28	the	the	DET
cet-14418	91	29	methanol	methanol	NOUN
cet-14418	91	30	synthesis	synthesis	NOUN
cet-14418	91	31	.	.	PUNCT
cet-14418	92	1	in	in	ADP
cet-14418	92	2	the	the	DET
cet-14418	92	3	simulation	simulation	NOUN
cet-14418	92	4	,	,	PUNCT
cet-14418	92	5	the	the	DET
cet-14418	92	6	micro	micro	ADJ
cet-14418	92	7	-	-	NOUN
cet-14418	92	8	scale	scale	ADJ
cet-14418	92	9	parameters	parameter	NOUN
cet-14418	92	10	(	(	PUNCT
cet-14418	92	11	the	the	DET
cet-14418	92	12	effective	effective	ADJ
cet-14418	92	13	thermal	thermal	ADJ
cet-14418	92	14	conductivity	conductivity	NOUN
cet-14418	92	15	,	,	PUNCT
cet-14418	92	16	permeability	permeability	NOUN
cet-14418	92	17	,	,	PUNCT
cet-14418	92	18	and	and	CCONJ
cet-14418	92	19	effective	effective	ADJ
cet-14418	92	20	diffusion	diffusion	NOUN
cet-14418	92	21	coefficient	coefficient	NOUN
cet-14418	92	22	)	)	PUNCT
cet-14418	92	23	of	of	ADP
cet-14418	92	24	the	the	DET
cet-14418	92	25	cylinder	cylinder	NOUN
cet-14418	92	26	shape	shape	NOUN
cet-14418	92	27	pellet	pellet	NOUN
cet-14418	92	28	estimated	estimate	VERB
cet-14418	92	29	in	in	ADP
cet-14418	92	30	the	the	DET
cet-14418	92	31	previous	previous	ADJ
cet-14418	92	32	section	section	NOUN
cet-14418	92	33	were	be	AUX
cet-14418	92	34	adopted	adopt	VERB
cet-14418	92	35	.	.	PUNCT
cet-14418	93	1	figure	figure	NOUN
cet-14418	93	2	4a	4a	NOUN
cet-14418	93	3	and	and	CCONJ
cet-14418	93	4	b	b	NOUN
cet-14418	93	5	describes	describe	VERB
cet-14418	93	6	the	the	DET
cet-14418	93	7	comparison	comparison	NOUN
cet-14418	93	8	of	of	ADP
cet-14418	93	9	temperature	temperature	NOUN
cet-14418	93	10	between	between	ADP
cet-14418	93	11	the	the	DET
cet-14418	93	12	experiment	experiment	NOUN
cet-14418	93	13	and	and	CCONJ
cet-14418	93	14	the	the	DET
cet-14418	93	15	simulation	simulation	NOUN
cet-14418	93	16	in	in	ADP
cet-14418	93	17	the	the	DET
cet-14418	93	18	cold	cold	ADJ
cet-14418	93	19	case	case	NOUN
cet-14418	93	20	and	and	CCONJ
cet-14418	93	21	the	the	DET
cet-14418	93	22	case	case	NOUN
cet-14418	93	23	with	with	ADP
cet-14418	93	24	methanol	methanol	NOUN
cet-14418	93	25	synthesis	synthesis	NOUN
cet-14418	93	26	,	,	PUNCT
cet-14418	93	27	respectively	respectively	ADV
cet-14418	93	28	.	.	PUNCT
cet-14418	94	1	the	the	DET
cet-14418	94	2	simulated	simulated	ADJ
cet-14418	94	3	values	value	NOUN
cet-14418	94	4	agree	agree	VERB
cet-14418	94	5	well	well	ADV
cet-14418	94	6	with	with	ADP
cet-14418	94	7	the	the	DET
cet-14418	94	8	experimental	experimental	ADJ
cet-14418	94	9	ones	one	NOUN
cet-14418	94	10	,	,	PUNCT
cet-14418	94	11	indicating	indicate	VERB
cet-14418	94	12	that	that	SCONJ
cet-14418	94	13	the	the	DET
cet-14418	94	14	macro	macro	ADJ
cet-14418	94	15	-	-	NOUN
cet-14418	94	16	scale	scale	NOUN
cet-14418	94	17	model	model	NOUN
cet-14418	94	18	reproduces	reproduce	VERB
cet-14418	94	19	not	not	PART
cet-14418	94	20	only	only	ADV
cet-14418	94	21	the	the	DET
cet-14418	94	22	cold	cold	ADJ
cet-14418	94	23	case	case	NOUN
cet-14418	94	24	but	but	CCONJ
cet-14418	94	25	also	also	ADV
cet-14418	94	26	the	the	DET
cet-14418	94	27	methanol	methanol	NOUN
cet-14418	94	28	synthesis	synthesis	NOUN
cet-14418	94	29	results	result	NOUN
cet-14418	94	30	.	.	PUNCT
cet-14418	95	1	in	in	ADP
cet-14418	95	2	addition	addition	NOUN
cet-14418	95	3	,	,	PUNCT
cet-14418	95	4	the	the	DET
cet-14418	95	5	ch3oh	ch3oh	NUM
cet-14418	95	6	concentration	concentration	NOUN
cet-14418	95	7	was	be	AUX
cet-14418	95	8	measured	measure	VERB
cet-14418	95	9	,	,	PUNCT
cet-14418	95	10	and	and	CCONJ
cet-14418	95	11	the	the	DET
cet-14418	95	12	value	value	NOUN
cet-14418	95	13	agreed	agree	VERB
cet-14418	95	14	well	well	ADV
cet-14418	95	15	with	with	ADP
cet-14418	95	16	the	the	DET
cet-14418	95	17	simulated	simulate	VERB
cet-14418	95	18	one	one	NOUN
cet-14418	95	19	(	(	PUNCT
cet-14418	95	20	simulation:5.94	simulation:5.94	PROPN
cet-14418	95	21	x10	x10	PROPN
cet-14418	95	22	-	-	SYM
cet-14418	95	23	4	4	NUM
cet-14418	95	24	mol	mol	NOUN
cet-14418	95	25	/	/	SYM
cet-14418	95	26	m3	m3	PROPN
cet-14418	95	27	,	,	PUNCT
cet-14418	95	28	experiment:6.0x10(a	experiment:6.0x10(a	PROPN
cet-14418	95	29	)	)	PUNCT
cet-14418	95	30	(	(	PUNCT
cet-14418	95	31	b	b	NOUN
cet-14418	95	32	)	)	PUNCT
cet-14418	95	33	(	(	PUNCT
cet-14418	95	34	c	c	X
cet-14418	95	35	)	)	PUNCT
cet-14418	95	36	(	(	PUNCT
cet-14418	95	37	d	d	X
cet-14418	95	38	)	)	PUNCT
cet-14418	95	39	46	46	NUM
cet-14418	95	40	4	4	NUM
cet-14418	95	41	mol	mol	NOUN
cet-14418	95	42	/	/	SYM
cet-14418	95	43	m3	m3	PROPN
cet-14418	95	44	)	)	PUNCT
cet-14418	95	45	.	.	PUNCT
cet-14418	96	1	figure	figure	VERB
cet-14418	96	2	4c	4c	NOUN
cet-14418	96	3	and	and	CCONJ
cet-14418	96	4	d	d	PROPN
cet-14418	96	5	shows	show	VERB
cet-14418	96	6	the	the	DET
cet-14418	96	7	simulated	simulate	VERB
cet-14418	96	8	steady	steady	ADJ
cet-14418	96	9	-	-	PUNCT
cet-14418	96	10	state	state	NOUN
cet-14418	96	11	temperature	temperature	NOUN
cet-14418	96	12	and	and	CCONJ
cet-14418	96	13	ch3oh	ch3oh	NOUN
cet-14418	96	14	concentration	concentration	NOUN
cet-14418	96	15	distribution	distribution	NOUN
cet-14418	96	16	in	in	ADP
cet-14418	96	17	the	the	DET
cet-14418	96	18	reactor	reactor	NOUN
cet-14418	96	19	.	.	PUNCT
cet-14418	97	1	the	the	DET
cet-14418	97	2	temperature	temperature	NOUN
cet-14418	97	3	increases	increase	VERB
cet-14418	97	4	from	from	ADP
cet-14418	97	5	the	the	DET
cet-14418	97	6	reactor	reactor	NOUN
cet-14418	97	7	inlet	inlet	NOUN
cet-14418	97	8	to	to	ADP
cet-14418	97	9	the	the	DET
cet-14418	97	10	catalyst	catalyst	NOUN
cet-14418	97	11	layer	layer	NOUN
cet-14418	97	12	due	due	ADP
cet-14418	97	13	to	to	ADP
cet-14418	97	14	the	the	DET
cet-14418	97	15	heater	heater	NOUN
cet-14418	97	16	around	around	ADP
cet-14418	97	17	the	the	DET
cet-14418	97	18	reactor	reactor	NOUN
cet-14418	97	19	and	and	CCONJ
cet-14418	97	20	the	the	DET
cet-14418	97	21	heat	heat	NOUN
cet-14418	97	22	generation	generation	NOUN
cet-14418	97	23	of	of	ADP
cet-14418	97	24	the	the	DET
cet-14418	97	25	catalyst	catalyst	NOUN
cet-14418	97	26	layer	layer	NOUN
cet-14418	97	27	.	.	PUNCT
cet-14418	98	1	the	the	DET
cet-14418	98	2	concentration	concentration	NOUN
cet-14418	98	3	increases	increase	VERB
cet-14418	98	4	downstream	downstream	ADV
cet-14418	98	5	of	of	ADP
cet-14418	98	6	the	the	DET
cet-14418	98	7	catalyst	catalyst	NOUN
cet-14418	98	8	layer	layer	NOUN
cet-14418	98	9	.	.	PUNCT
cet-14418	99	1	note	note	VERB
cet-14418	99	2	that	that	SCONJ
cet-14418	99	3	the	the	DET
cet-14418	99	4	concentration	concentration	NOUN
cet-14418	99	5	is	be	AUX
cet-14418	99	6	higher	high	ADJ
cet-14418	99	7	in	in	ADP
cet-14418	99	8	the	the	DET
cet-14418	99	9	centre	centre	NOUN
cet-14418	99	10	than	than	ADP
cet-14418	99	11	near	near	ADP
cet-14418	99	12	the	the	DET
cet-14418	99	13	wall	wall	NOUN
cet-14418	99	14	.	.	PUNCT
cet-14418	100	1	this	this	PRON
cet-14418	100	2	indicates	indicate	VERB
cet-14418	100	3	that	that	SCONJ
cet-14418	100	4	the	the	DET
cet-14418	100	5	higher	high	ADJ
cet-14418	100	6	flow	flow	NOUN
cet-14418	100	7	velocity	velocity	NOUN
cet-14418	100	8	induces	induce	VERB
cet-14418	100	9	the	the	DET
cet-14418	100	10	reaction	reaction	NOUN
cet-14418	100	11	of	of	ADP
cet-14418	100	12	methanol	methanol	NOUN
cet-14418	100	13	synthesis	synthesis	NOUN
cet-14418	100	14	in	in	ADP
cet-14418	100	15	this	this	DET
cet-14418	100	16	region	region	NOUN
cet-14418	100	17	.	.	PUNCT
cet-14418	101	1	these	these	DET
cet-14418	101	2	results	result	NOUN
cet-14418	101	3	are	be	AUX
cet-14418	101	4	similar	similar	ADJ
cet-14418	101	5	to	to	ADP
cet-14418	101	6	the	the	DET
cet-14418	101	7	trends	trend	NOUN
cet-14418	101	8	of	of	ADP
cet-14418	101	9	previously	previously	ADV
cet-14418	101	10	reported	report	VERB
cet-14418	101	11	2	2	NUM
cet-14418	101	12	-	-	PUNCT
cet-14418	101	13	d	d	NOUN
cet-14418	101	14	homogenization	homogenization	NOUN
cet-14418	101	15	models	model	NOUN
cet-14418	101	16	(	(	PUNCT
cet-14418	101	17	adji	adji	PROPN
cet-14418	101	18	et	et	PROPN
cet-14418	101	19	al	al	PROPN
cet-14418	101	20	.	.	PROPN
cet-14418	101	21	,	,	PUNCT
cet-14418	101	22	2019	2019	NUM
cet-14418	101	23	)	)	PUNCT
cet-14418	101	24	.	.	PUNCT
cet-14418	102	1	3.2	3.2	NUM
cet-14418	102	2	effects	effect	NOUN
cet-14418	102	3	of	of	ADP
cet-14418	102	4	pellet	pellet	NOUN
cet-14418	102	5	shape	shape	NOUN
cet-14418	102	6	on	on	ADP
cet-14418	102	7	conversion	conversion	NOUN
cet-14418	102	8	in	in	ADP
cet-14418	102	9	order	order	NOUN
cet-14418	102	10	to	to	PART
cet-14418	102	11	clarify	clarify	VERB
cet-14418	102	12	the	the	DET
cet-14418	102	13	effects	effect	NOUN
cet-14418	102	14	of	of	ADP
cet-14418	102	15	the	the	DET
cet-14418	102	16	pellet	pellet	NOUN
cet-14418	102	17	shape	shape	NOUN
cet-14418	102	18	on	on	ADP
cet-14418	102	19	the	the	DET
cet-14418	102	20	micro	micro	ADJ
cet-14418	102	21	-	-	NOUN
cet-14418	102	22	scale	scale	ADJ
cet-14418	102	23	parameters	parameter	NOUN
cet-14418	102	24	with	with	ADP
cet-14418	102	25	the	the	DET
cet-14418	102	26	random	random	ADJ
cet-14418	102	27	packed	pack	VERB
cet-14418	102	28	sphere	sphere	NOUN
cet-14418	102	29	and	and	CCONJ
cet-14418	102	30	hollow	hollow	ADJ
cet-14418	102	31	cylinder	cylinder	NOUN
cet-14418	102	32	structures	structure	NOUN
cet-14418	102	33	were	be	AUX
cet-14418	102	34	carried	carry	VERB
cet-14418	102	35	out	out	ADP
cet-14418	102	36	.	.	PUNCT
cet-14418	103	1	the	the	DET
cet-14418	103	2	estimated	estimate	VERB
cet-14418	103	3	values	value	NOUN
cet-14418	103	4	of	of	ADP
cet-14418	103	5	volume	volume	NOUN
cet-14418	103	6	fraction	fraction	NOUN
cet-14418	103	7	,	,	PUNCT
cet-14418	103	8	surface	surface	NOUN
cet-14418	103	9	area	area	NOUN
cet-14418	103	10	,	,	PUNCT
cet-14418	103	11	permeability	permeability	NOUN
cet-14418	103	12	is	be	AUX
cet-14418	103	13	shown	show	VERB
cet-14418	103	14	in	in	ADP
cet-14418	103	15	table	table	NOUN
cet-14418	103	16	4	4	NUM
cet-14418	103	17	.	.	PUNCT
cet-14418	104	1	the	the	DET
cet-14418	104	2	volume	volume	NOUN
cet-14418	104	3	fractions	fraction	NOUN
cet-14418	104	4	of	of	ADP
cet-14418	104	5	the	the	DET
cet-14418	104	6	cylinder	cylinder	NOUN
cet-14418	104	7	and	and	CCONJ
cet-14418	104	8	sphere	sphere	NOUN
cet-14418	104	9	pellets	pellet	NOUN
cet-14418	104	10	are	be	AUX
cet-14418	104	11	almost	almost	ADV
cet-14418	104	12	50	50	NUM
cet-14418	104	13	%	%	NOUN
cet-14418	104	14	,	,	PUNCT
cet-14418	104	15	whereas	whereas	SCONJ
cet-14418	104	16	that	that	PRON
cet-14418	104	17	of	of	ADP
cet-14418	104	18	the	the	DET
cet-14418	104	19	hollow	hollow	ADJ
cet-14418	104	20	cylinder	cylinder	NOUN
cet-14418	104	21	reduces	reduce	VERB
cet-14418	104	22	to	to	ADP
cet-14418	104	23	39	39	NUM
cet-14418	104	24	%	%	NOUN
cet-14418	104	25	due	due	ADP
cet-14418	104	26	to	to	ADP
cet-14418	104	27	the	the	DET
cet-14418	104	28	hollow	hollow	ADJ
cet-14418	104	29	space	space	NOUN
cet-14418	104	30	in	in	ADP
cet-14418	104	31	the	the	DET
cet-14418	104	32	cylinder	cylinder	NOUN
cet-14418	104	33	.	.	PUNCT
cet-14418	105	1	the	the	DET
cet-14418	105	2	specific	specific	ADJ
cet-14418	105	3	surface	surface	NOUN
cet-14418	105	4	area	area	NOUN
cet-14418	105	5	of	of	ADP
cet-14418	105	6	the	the	DET
cet-14418	105	7	hollow	hollow	ADJ
cet-14418	105	8	cylinder	cylinder	NOUN
cet-14418	105	9	is	be	AUX
cet-14418	105	10	about	about	ADV
cet-14418	105	11	50	50	NUM
cet-14418	105	12	%	%	NOUN
cet-14418	105	13	larger	large	ADJ
cet-14418	105	14	than	than	ADP
cet-14418	105	15	those	those	PRON
cet-14418	105	16	of	of	ADP
cet-14418	105	17	the	the	DET
cet-14418	105	18	cylinder	cylinder	NOUN
cet-14418	105	19	and	and	CCONJ
cet-14418	105	20	sphere	sphere	NOUN
cet-14418	105	21	for	for	ADP
cet-14418	105	22	this	this	DET
cet-14418	105	23	reason	reason	NOUN
cet-14418	105	24	.	.	PUNCT
cet-14418	106	1	it	it	PRON
cet-14418	106	2	should	should	AUX
cet-14418	106	3	be	be	AUX
cet-14418	106	4	noted	note	VERB
cet-14418	106	5	that	that	SCONJ
cet-14418	106	6	the	the	DET
cet-14418	106	7	sphere	sphere	NOUN
cet-14418	106	8	structure	structure	NOUN
cet-14418	106	9	estimated	estimate	VERB
cet-14418	106	10	from	from	ADP
cet-14418	106	11	the	the	DET
cet-14418	106	12	micro	micro	ADJ
cet-14418	106	13	-	-	NOUN
cet-14418	106	14	scale	scale	ADJ
cet-14418	106	15	model	model	NOUN
cet-14418	106	16	had	have	VERB
cet-14418	106	17	the	the	DET
cet-14418	106	18	highest	high	ADJ
cet-14418	106	19	permeability	permeability	NOUN
cet-14418	106	20	,	,	PUNCT
cet-14418	106	21	although	although	SCONJ
cet-14418	106	22	those	those	PRON
cet-14418	106	23	estimated	estimate	VERB
cet-14418	106	24	from	from	ADP
cet-14418	106	25	the	the	DET
cet-14418	106	26	kozeny	kozeny	NOUN
cet-14418	106	27	–	–	PUNCT
cet-14418	106	28	carman	carman	PROPN
cet-14418	106	29	eq	eq	ADP
cet-14418	106	30	.	.	PROPN
cet-14418	106	31	ranked	rank	VERB
cet-14418	106	32	between	between	ADP
cet-14418	106	33	the	the	DET
cet-14418	106	34	cylinder	cylinder	NOUN
cet-14418	106	35	and	and	CCONJ
cet-14418	106	36	the	the	DET
cet-14418	106	37	hollow	hollow	ADJ
cet-14418	106	38	cylinder	cylinder	NOUN
cet-14418	106	39	.	.	PUNCT
cet-14418	107	1	this	this	PRON
cet-14418	107	2	could	could	AUX
cet-14418	107	3	be	be	AUX
cet-14418	107	4	attributed	attribute	VERB
cet-14418	107	5	to	to	ADP
cet-14418	107	6	the	the	DET
cet-14418	107	7	sphere	sphere	NOUN
cet-14418	107	8	-	-	PUNCT
cet-14418	107	9	packed	pack	VERB
cet-14418	107	10	structure	structure	NOUN
cet-14418	107	11	having	have	VERB
cet-14418	107	12	a	a	DET
cet-14418	107	13	larger	large	ADJ
cet-14418	107	14	average	average	ADJ
cet-14418	107	15	pore	pore	ADJ
cet-14418	107	16	size	size	NOUN
cet-14418	107	17	and	and	CCONJ
cet-14418	107	18	smaller	small	ADJ
cet-14418	107	19	tortuosity	tortuosity	NOUN
cet-14418	107	20	than	than	ADP
cet-14418	107	21	other	other	ADJ
cet-14418	107	22	structures	structure	NOUN
cet-14418	107	23	(	(	PUNCT
cet-14418	107	24	fu	fu	NOUN
cet-14418	107	25	et	et	PROPN
cet-14418	107	26	al	al	PROPN
cet-14418	107	27	.	.	PROPN
cet-14418	107	28	,	,	PUNCT
cet-14418	107	29	2021	2021	NUM
cet-14418	107	30	;	;	PUNCT
cet-14418	107	31	ahn	ahn	PROPN
cet-14418	107	32	et	et	PROPN
cet-14418	107	33	al	al	PROPN
cet-14418	107	34	.	.	PROPN
cet-14418	107	35	,	,	PUNCT
cet-14418	107	36	2021	2021	NUM
cet-14418	107	37	)	)	PUNCT
cet-14418	107	38	.	.	PUNCT
cet-14418	108	1	table	table	NOUN
cet-14418	108	2	5	5	NUM
cet-14418	108	3	shows	show	VERB
cet-14418	108	4	the	the	DET
cet-14418	108	5	effective	effective	ADJ
cet-14418	108	6	thermal	thermal	ADJ
cet-14418	108	7	conductivity	conductivity	NOUN
cet-14418	108	8	in	in	ADP
cet-14418	108	9	the	the	DET
cet-14418	108	10	gas	gas	NOUN
cet-14418	108	11	phase	phase	NOUN
cet-14418	108	12	and	and	CCONJ
cet-14418	108	13	pellet	pellet	NOUN
cet-14418	108	14	layer	layer	NOUN
cet-14418	108	15	,	,	PUNCT
cet-14418	108	16	and	and	CCONJ
cet-14418	108	17	the	the	DET
cet-14418	108	18	effective	effective	ADJ
cet-14418	108	19	diffusion	diffusion	NOUN
cet-14418	108	20	coefficient	coefficient	NOUN
cet-14418	108	21	in	in	ADP
cet-14418	108	22	each	each	DET
cet-14418	108	23	gas	gas	NOUN
cet-14418	108	24	species	specie	NOUN
cet-14418	108	25	estimated	estimate	VERB
cet-14418	108	26	from	from	ADP
cet-14418	108	27	the	the	DET
cet-14418	108	28	micro	micro	ADJ
cet-14418	108	29	-	-	NOUN
cet-14418	108	30	scale	scale	ADJ
cet-14418	108	31	model	model	NOUN
cet-14418	108	32	.	.	PUNCT
cet-14418	109	1	in	in	ADP
cet-14418	109	2	contrast	contrast	NOUN
cet-14418	109	3	to	to	ADP
cet-14418	109	4	the	the	DET
cet-14418	109	5	permeability	permeability	NOUN
cet-14418	109	6	,	,	PUNCT
cet-14418	109	7	the	the	DET
cet-14418	109	8	values	value	NOUN
cet-14418	109	9	of	of	ADP
cet-14418	109	10	the	the	DET
cet-14418	109	11	hollow	hollow	ADJ
cet-14418	109	12	cylinder	cylinder	NOUN
cet-14418	109	13	are	be	AUX
cet-14418	109	14	higher	high	ADJ
cet-14418	109	15	than	than	ADP
cet-14418	109	16	those	those	PRON
cet-14418	109	17	of	of	ADP
cet-14418	109	18	the	the	DET
cet-14418	109	19	cylinder	cylinder	NOUN
cet-14418	109	20	and	and	CCONJ
cet-14418	109	21	sphere	sphere	NOUN
cet-14418	109	22	.	.	PUNCT
cet-14418	110	1	the	the	DET
cet-14418	110	2	effective	effective	ADJ
cet-14418	110	3	values	value	NOUN
cet-14418	110	4	estimated	estimate	VERB
cet-14418	110	5	by	by	ADP
cet-14418	110	6	bruggeman	bruggeman	PROPN
cet-14418	110	7	’s	’s	PART
cet-14418	110	8	eq	eq	NOUN
cet-14418	110	9	.	.	PUNCT
cet-14418	110	10	show	show	VERB
cet-14418	110	11	the	the	DET
cet-14418	110	12	same	same	ADJ
cet-14418	110	13	tendency	tendency	NOUN
cet-14418	110	14	as	as	ADP
cet-14418	110	15	those	those	PRON
cet-14418	110	16	of	of	ADP
cet-14418	110	17	the	the	DET
cet-14418	110	18	micro	micro	ADJ
cet-14418	110	19	-	-	NOUN
cet-14418	110	20	scale	scale	ADJ
cet-14418	110	21	model	model	NOUN
cet-14418	110	22	.	.	PUNCT
cet-14418	111	1	this	this	PRON
cet-14418	111	2	suggests	suggest	VERB
cet-14418	111	3	that	that	SCONJ
cet-14418	111	4	the	the	DET
cet-14418	111	5	porosity	porosity	NOUN
cet-14418	111	6	of	of	ADP
cet-14418	111	7	the	the	DET
cet-14418	111	8	pellet	pellet	NOUN
cet-14418	111	9	region	region	NOUN
cet-14418	111	10	could	could	AUX
cet-14418	111	11	be	be	AUX
cet-14418	111	12	a	a	DET
cet-14418	111	13	dominant	dominant	ADJ
cet-14418	111	14	factor	factor	NOUN
cet-14418	111	15	regardless	regardless	ADV
cet-14418	111	16	of	of	ADP
cet-14418	111	17	the	the	DET
cet-14418	111	18	pellet	pellet	NOUN
cet-14418	111	19	shape	shape	NOUN
cet-14418	111	20	.	.	PUNCT
cet-14418	112	1	table	table	NOUN
cet-14418	112	2	4	4	NUM
cet-14418	112	3	.	.	PUNCT
cet-14418	112	4	geometry	geometry	NOUN
cet-14418	112	5	parameters	parameter	NOUN
cet-14418	112	6	and	and	CCONJ
cet-14418	112	7	estimated	estimate	VERB
cet-14418	112	8	micro	micro	ADJ
cet-14418	112	9	-	-	NOUN
cet-14418	112	10	scale	scale	ADJ
cet-14418	112	11	parameters	parameter	NOUN
cet-14418	112	12	in	in	ADP
cet-14418	112	13	each	each	DET
cet-14418	112	14	structure	structure	NOUN
cet-14418	112	15	.	.	PUNCT
cet-14418	113	1	volume	volume	NOUN
cet-14418	113	2	fraction	fraction	NOUN
cet-14418	113	3	(	(	PUNCT
cet-14418	113	4	-	-	PUNCT
cet-14418	113	5	)	)	PUNCT
cet-14418	113	6	specific	specific	ADJ
cet-14418	113	7	surface	surface	NOUN
cet-14418	113	8	area	area	NOUN
cet-14418	113	9	(	(	PUNCT
cet-14418	113	10	1	1	NUM
cet-14418	113	11	/	/	SYM
cet-14418	113	12	m	m	NOUN
cet-14418	113	13	)	)	PUNCT
cet-14418	113	14	permeability	permeability	NOUN
cet-14418	113	15	[	[	X
cet-14418	113	16	(	(	PUNCT
cet-14418	113	17	m2	m2	PROPN
cet-14418	113	18	)	)	PUNCT
cet-14418	113	19	cylinder	cylinder	NOUN
cet-14418	113	20	(	(	PUNCT
cet-14418	113	21	reshown	reshown	ADJ
cet-14418	113	22	)	)	PUNCT
cet-14418	113	23	micro	micro	ADJ
cet-14418	113	24	-	-	NOUN
cet-14418	113	25	scale	scale	ADJ
cet-14418	113	26	model	model	NOUN
cet-14418	113	27	kozeny	kozeny	PROPN
cet-14418	113	28	–	–	PUNCT
cet-14418	113	29	carman	carman	NOUN
cet-14418	113	30	0.518	0.518	NUM
cet-14418	113	31	943	943	NUM
cet-14418	113	32	1.13×10	1.13×10	NUM
cet-14418	113	33	-	-	SYM
cet-14418	113	34	8	8	NUM
cet-14418	113	35	1.19×10	1.19×10	NUM
cet-14418	113	36	-	-	SYM
cet-14418	113	37	8	8	NUM
cet-14418	113	38	sphere	sphere	NOUN
cet-14418	113	39	micro	micro	ADJ
cet-14418	113	40	-	-	NOUN
cet-14418	113	41	scale	scale	ADJ
cet-14418	113	42	model	model	NOUN
cet-14418	113	43	kozeny	kozeny	PROPN
cet-14418	113	44	–	–	PUNCT
cet-14418	113	45	carman	carman	PROPN
cet-14418	113	46	0.498	0.498	NUM
cet-14418	113	47	838	838	NUM
cet-14418	113	48	1.36×10	1.36×10	NUM
cet-14418	113	49	-	-	SYM
cet-14418	113	50	8	8	NUM
cet-14418	113	51	9.80×10	9.80×10	NUM
cet-14418	113	52	-	-	SYM
cet-14418	113	53	9	9	NUM
cet-14418	113	54	hollow	hollow	ADJ
cet-14418	113	55	cylinder	cylinder	NOUN
cet-14418	113	56	micro	micro	NOUN
cet-14418	113	57	-	-	NOUN
cet-14418	113	58	scale	scale	ADJ
cet-14418	113	59	model	model	NOUN
cet-14418	113	60	kozeny	kozeny	PROPN
cet-14418	113	61	–	–	PUNCT
cet-14418	113	62	carman	carman	NOUN
cet-14418	113	63	0.386	0.386	NUM
cet-14418	113	64	1260	1260	NUM
cet-14418	113	65	1.28×10	1.28×10	NUM
cet-14418	113	66	-	-	SYM
cet-14418	113	67	8	8	NUM
cet-14418	113	68	5.05×10	5.05×10	NUM
cet-14418	113	69	-	-	SYM
cet-14418	113	70	9	9	NUM
cet-14418	113	71	table	table	NOUN
cet-14418	113	72	5	5	NUM
cet-14418	113	73	.	.	PUNCT
cet-14418	113	74	estimated	estimate	VERB
cet-14418	113	75	effective	effective	ADJ
cet-14418	113	76	thermal	thermal	ADJ
cet-14418	113	77	conductivities	conductivity	NOUN
cet-14418	113	78	and	and	CCONJ
cet-14418	113	79	diffusion	diffusion	NOUN
cet-14418	113	80	coefficients	coefficient	NOUN
cet-14418	113	81	in	in	ADP
cet-14418	113	82	each	each	DET
cet-14418	113	83	structure	structure	NOUN
cet-14418	113	84	.	.	PUNCT
cet-14418	114	1	𝑘𝑘𝑎𝑎𝑒𝑒𝑒𝑒	𝑘𝑘𝑎𝑎𝑒𝑒𝑒𝑒	NOUN
cet-14418	114	2	(	(	PUNCT
cet-14418	114	3	w/(m2s	w/(m2s	PROPN
cet-14418	114	4	)	)	PUNCT
cet-14418	114	5	)	)	PUNCT
cet-14418	114	6	𝐷𝐷𝑎𝑎𝑒𝑒𝑒𝑒,𝑖𝑖	𝐷𝐷𝑎𝑎𝑒𝑒𝑒𝑒,𝑖𝑖	PROPN
cet-14418	114	7	(	(	PUNCT
cet-14418	114	8	m2	m2	PROPN
cet-14418	114	9	/	/	SYM
cet-14418	114	10	s	s	PROPN
cet-14418	114	11	)	)	PUNCT
cet-14418	114	12	gas	gas	NOUN
cet-14418	114	13	h2	h2	NOUN
cet-14418	114	14	o2	o2	PROPN
cet-14418	114	15	ch3oh	ch3oh	NOUN
cet-14418	114	16	cylinder	cylinder	NOUN
cet-14418	114	17	(	(	PUNCT
cet-14418	114	18	reshown	reshown	ADJ
cet-14418	114	19	)	)	PUNCT
cet-14418	114	20	micro	micro	ADJ
cet-14418	114	21	-	-	NOUN
cet-14418	114	22	scale	scale	ADJ
cet-14418	114	23	model	model	NOUN
cet-14418	114	24	0.133	0.133	NUM
cet-14418	114	25	4.91×10	4.91×10	NUM
cet-14418	114	26	-	-	SYM
cet-14418	114	27	5	5	NUM
cet-14418	114	28	1.09×10	1.09×10	NUM
cet-14418	114	29	-	-	SYM
cet-14418	114	30	5	5	NUM
cet-14418	114	31	4.67×10	4.67×10	NUM
cet-14418	114	32	-	-	PUNCT
cet-14418	114	33	6	6	NUM
cet-14418	114	34	bruggeman	bruggeman	NOUN
cet-14418	114	35	0.165	0.165	NUM
cet-14418	114	36	5.35×10	5.35×10	NUM
cet-14418	114	37	-	-	SYM
cet-14418	114	38	5	5	NUM
cet-14418	114	39	1.19×10	1.19×10	NUM
cet-14418	114	40	-	-	SYM
cet-14418	114	41	5	5	NUM
cet-14418	114	42	5.09×10	5.09×10	NUM
cet-14418	114	43	-	-	SYM
cet-14418	114	44	6	6	NUM
cet-14418	114	45	sphere	sphere	NOUN
cet-14418	114	46	micro	micro	ADJ
cet-14418	114	47	-	-	NOUN
cet-14418	114	48	scale	scale	ADJ
cet-14418	114	49	model	model	NOUN
cet-14418	114	50	0.138	0.138	NUM
cet-14418	114	51	5.47×10	5.47×10	NUM
cet-14418	114	52	-	-	SYM
cet-14418	114	53	5	5	NUM
cet-14418	114	54	1.22×10	1.22×10	NUM
cet-14418	114	55	-	-	SYM
cet-14418	114	56	5	5	NUM
cet-14418	114	57	5.20×10	5.20×10	NUM
cet-14418	114	58	-	-	SYM
cet-14418	114	59	6	6	NUM
cet-14418	114	60	bruggeman	bruggeman	NOUN
cet-14418	114	61	0.144	0.144	NUM
cet-14418	114	62	5.69×10	5.69×10	NUM
cet-14418	114	63	-	-	SYM
cet-14418	114	64	5	5	NUM
cet-14418	114	65	1.27×10	1.27×10	NUM
cet-14418	114	66	-	-	SYM
cet-14418	114	67	5	5	NUM
cet-14418	114	68	5.41×10	5.41×10	NUM
cet-14418	114	69	-	-	SYM
cet-14418	114	70	6	6	NUM
cet-14418	114	71	hollow	hollow	ADJ
cet-14418	114	72	cylinder	cylinder	NOUN
cet-14418	114	73	micro	micro	NOUN
cet-14418	114	74	-	-	NOUN
cet-14418	114	75	scale	scale	ADJ
cet-14418	114	76	model	model	NOUN
cet-14418	114	77	0.151	0.151	NUM
cet-14418	114	78	5.50×10	5.50×10	NUM
cet-14418	114	79	-	-	SYM
cet-14418	114	80	5	5	NUM
cet-14418	114	81	1.22×10	1.22×10	NUM
cet-14418	114	82	-	-	SYM
cet-14418	114	83	5	5	NUM
cet-14418	114	84	5.23×10	5.23×10	NUM
cet-14418	114	85	-	-	SYM
cet-14418	114	86	6	6	NUM
cet-14418	114	87	bruggeman	bruggeman	NOUN
cet-14418	114	88	0.211	0.211	NUM
cet-14418	114	89	7.70×10	7.70×10	NUM
cet-14418	114	90	-	-	SYM
cet-14418	114	91	5	5	NUM
cet-14418	114	92	1.71×10	1.71×10	NUM
cet-14418	114	93	-	-	SYM
cet-14418	114	94	5	5	NUM
cet-14418	114	95	7.31×10	7.31×10	NUM
cet-14418	114	96	-	-	SYM
cet-14418	114	97	6	6	NUM
cet-14418	114	98	the	the	DET
cet-14418	114	99	2d	2d	NUM
cet-14418	114	100	axial	axial	PROPN
cet-14418	114	101	symmetric	symmetric	ADJ
cet-14418	114	102	micro	micro	ADJ
cet-14418	114	103	-	-	NOUN
cet-14418	114	104	scale	scale	ADJ
cet-14418	114	105	simulations	simulation	NOUN
cet-14418	114	106	with	with	ADP
cet-14418	114	107	various	various	ADJ
cet-14418	114	108	pellet	pellet	NOUN
cet-14418	114	109	shapes	shape	NOUN
cet-14418	114	110	,	,	PUNCT
cet-14418	114	111	including	include	VERB
cet-14418	114	112	spheres	sphere	NOUN
cet-14418	114	113	,	,	PUNCT
cet-14418	114	114	cylinders	cylinder	NOUN
cet-14418	114	115	,	,	PUNCT
cet-14418	114	116	and	and	CCONJ
cet-14418	114	117	hollow	hollow	ADJ
cet-14418	114	118	cylinders	cylinder	NOUN
cet-14418	114	119	,	,	PUNCT
cet-14418	114	120	have	have	AUX
cet-14418	114	121	been	be	AUX
cet-14418	114	122	carried	carry	VERB
cet-14418	114	123	out	out	ADP
cet-14418	114	124	and	and	CCONJ
cet-14418	114	125	their	their	PRON
cet-14418	114	126	performances	performance	NOUN
cet-14418	114	127	were	be	AUX
cet-14418	114	128	compared	compare	VERB
cet-14418	114	129	.	.	PUNCT
cet-14418	115	1	the	the	DET
cet-14418	115	2	simulation	simulation	NOUN
cet-14418	115	3	conditions	condition	NOUN
cet-14418	115	4	,	,	PUNCT
cet-14418	115	5	including	include	VERB
cet-14418	115	6	inlet	inlet	NOUN
cet-14418	115	7	pressure	pressure	NOUN
cet-14418	115	8	and	and	CCONJ
cet-14418	115	9	gas	gas	NOUN
cet-14418	115	10	concentration	concentration	NOUN
cet-14418	115	11	,	,	PUNCT
cet-14418	115	12	were	be	AUX
cet-14418	115	13	the	the	DET
cet-14418	115	14	same	same	ADJ
cet-14418	115	15	as	as	ADP
cet-14418	115	16	in	in	ADP
cet-14418	115	17	the	the	DET
cet-14418	115	18	actual	actual	ADJ
cet-14418	115	19	experiment	experiment	NOUN
cet-14418	115	20	described	describe	VERB
cet-14418	115	21	in	in	ADP
cet-14418	115	22	3.1	3.1	NUM
cet-14418	115	23	.	.	PUNCT
cet-14418	116	1	figure	figure	NOUN
cet-14418	116	2	5a	5a	NUM
cet-14418	116	3	shows	show	VERB
cet-14418	116	4	the	the	DET
cet-14418	116	5	profile	profile	NOUN
cet-14418	116	6	of	of	ADP
cet-14418	116	7	the	the	DET
cet-14418	116	8	gas	gas	NOUN
cet-14418	116	9	velocity	velocity	NOUN
cet-14418	116	10	magnitude	magnitude	NOUN
cet-14418	116	11	on	on	ADP
cet-14418	116	12	the	the	DET
cet-14418	116	13	axial	axial	ADJ
cet-14418	116	14	lines	line	NOUN
cet-14418	116	15	in	in	ADP
cet-14418	116	16	each	each	DET
cet-14418	116	17	structure	structure	NOUN
cet-14418	116	18	.	.	PUNCT
cet-14418	117	1	the	the	DET
cet-14418	117	2	difference	difference	NOUN
cet-14418	117	3	of	of	ADP
cet-14418	117	4	the	the	DET
cet-14418	117	5	gas	gas	NOUN
cet-14418	117	6	velocity	velocity	NOUN
cet-14418	117	7	in	in	ADP
cet-14418	117	8	each	each	DET
cet-14418	117	9	pellet	pellet	NOUN
cet-14418	117	10	shape	shape	NOUN
cet-14418	117	11	in	in	ADP
cet-14418	117	12	the	the	DET
cet-14418	117	13	catalyst	catalyst	NOUN
cet-14418	117	14	bed	bed	NOUN
cet-14418	117	15	layer	layer	NOUN
cet-14418	117	16	was	be	AUX
cet-14418	117	17	only	only	ADV
cet-14418	117	18	within	within	ADP
cet-14418	117	19	1	1	NUM
cet-14418	117	20	%	%	NOUN
cet-14418	117	21	,	,	PUNCT
cet-14418	117	22	indicating	indicate	VERB
cet-14418	117	23	that	that	SCONJ
cet-14418	117	24	the	the	DET
cet-14418	117	25	outlet	outlet	NOUN
cet-14418	117	26	pressure	pressure	NOUN
cet-14418	117	27	loss	loss	NOUN
cet-14418	117	28	could	could	AUX
cet-14418	117	29	determine	determine	VERB
cet-14418	117	30	the	the	DET
cet-14418	117	31	velocity	velocity	NOUN
cet-14418	117	32	field	field	NOUN
cet-14418	117	33	in	in	ADP
cet-14418	117	34	the	the	DET
cet-14418	117	35	reactor	reactor	NOUN
cet-14418	117	36	.	.	PUNCT
cet-14418	118	1	figure	figure	NOUN
cet-14418	118	2	5b	5b	NOUN
cet-14418	118	3	show	show	VERB
cet-14418	118	4	the	the	DET
cet-14418	118	5	simulated	simulate	VERB
cet-14418	118	6	temperature	temperature	NOUN
cet-14418	118	7	on	on	ADP
cet-14418	118	8	the	the	DET
cet-14418	118	9	axial	axial	ADJ
cet-14418	118	10	lines	line	NOUN
cet-14418	118	11	.	.	PUNCT
cet-14418	119	1	in	in	ADP
cet-14418	119	2	all	all	DET
cet-14418	119	3	structures	structure	NOUN
cet-14418	119	4	,	,	PUNCT
cet-14418	119	5	the	the	DET
cet-14418	119	6	temperature	temperature	NOUN
cet-14418	119	7	rises	rise	VERB
cet-14418	119	8	from	from	ADP
cet-14418	119	9	the	the	DET
cet-14418	119	10	periphery	periphery	NOUN
cet-14418	119	11	from	from	ADP
cet-14418	119	12	the	the	DET
cet-14418	119	13	inlet	inlet	NOUN
cet-14418	119	14	to	to	ADP
cet-14418	119	15	the	the	DET
cet-14418	119	16	catalyst	catalyst	NOUN
cet-14418	119	17	bed	bed	NOUN
cet-14418	119	18	region	region	NOUN
cet-14418	119	19	and	and	CCONJ
cet-14418	119	20	slightly	slightly	ADV
cet-14418	119	21	decreases	decrease	VERB
cet-14418	119	22	beyond	beyond	ADP
cet-14418	119	23	the	the	DET
cet-14418	119	24	catalyst	catalyst	NOUN
cet-14418	119	25	bed	bed	NOUN
cet-14418	119	26	region	region	NOUN
cet-14418	119	27	.	.	PUNCT
cet-14418	120	1	the	the	DET
cet-14418	120	2	temperature	temperature	NOUN
cet-14418	120	3	distribution	distribution	NOUN
cet-14418	120	4	of	of	ADP
cet-14418	120	5	the	the	DET
cet-14418	120	6	cylinder	cylinder	NOUN
cet-14418	120	7	pellet	pellet	NOUN
cet-14418	120	8	structure	structure	NOUN
cet-14418	120	9	is	be	AUX
cet-14418	120	10	higher	high	ADJ
cet-14418	120	11	than	than	ADP
cet-14418	120	12	that	that	PRON
cet-14418	120	13	of	of	ADP
cet-14418	120	14	the	the	DET
cet-14418	120	15	other	other	ADJ
cet-14418	120	16	structures	structure	NOUN
cet-14418	120	17	,	,	PUNCT
cet-14418	120	18	with	with	ADP
cet-14418	120	19	a	a	DET
cet-14418	120	20	maximum	maximum	ADJ
cet-14418	120	21	difference	difference	NOUN
cet-14418	120	22	of	of	ADP
cet-14418	120	23	about	about	ADV
cet-14418	120	24	5	5	NUM
cet-14418	120	25	°	°	SYM
cet-14418	120	26	c	c	NOUN
cet-14418	120	27	in	in	ADP
cet-14418	120	28	the	the	DET
cet-14418	120	29	catalyst	catalyst	NOUN
cet-14418	120	30	bed	bed	NOUN
cet-14418	120	31	region	region	NOUN
cet-14418	120	32	.	.	PUNCT
cet-14418	121	1	it	it	PRON
cet-14418	121	2	is	be	AUX
cet-14418	121	3	natural	natural	ADJ
cet-14418	121	4	to	to	PART
cet-14418	121	5	assume	assume	VERB
cet-14418	121	6	that	that	SCONJ
cet-14418	121	7	this	this	PRON
cet-14418	121	8	is	be	AUX
cet-14418	121	9	due	due	ADJ
cet-14418	121	10	to	to	ADP
cet-14418	121	11	the	the	DET
cet-14418	121	12	effect	effect	NOUN
cet-14418	121	13	of	of	ADP
cet-14418	121	14	effective	effective	ADJ
cet-14418	121	15	thermal	thermal	ADJ
cet-14418	121	16	conductivity	conductivity	NOUN
cet-14418	121	17	evaluated	evaluate	VERB
cet-14418	121	18	in	in	ADP
cet-14418	121	19	section	section	NOUN
cet-14418	121	20	3.1	3.1	NUM
cet-14418	121	21	.	.	PUNCT
cet-14418	122	1	the	the	DET
cet-14418	122	2	steady	steady	ADJ
cet-14418	122	3	-	-	PUNCT
cet-14418	122	4	state	state	NOUN
cet-14418	122	5	ch3oh	ch3oh	NOUN
cet-14418	122	6	concentration	concentration	NOUN
cet-14418	122	7	on	on	ADP
cet-14418	122	8	the	the	DET
cet-14418	122	9	central	central	ADJ
cet-14418	122	10	axial	axial	NOUN
cet-14418	122	11	are	be	AUX
cet-14418	122	12	described	describe	VERB
cet-14418	122	13	in	in	ADP
cet-14418	122	14	fig5c	fig5c	PROPN
cet-14418	122	15	.	.	PUNCT
cet-14418	123	1	the	the	DET
cet-14418	123	2	concentration	concentration	NOUN
cet-14418	123	3	is	be	AUX
cet-14418	123	4	higher	high	ADJ
cet-14418	123	5	near	near	ADP
cet-14418	123	6	the	the	DET
cet-14418	123	7	central	central	ADJ
cet-14418	123	8	axis	axis	NOUN
cet-14418	123	9	,	,	PUNCT
cet-14418	123	10	and	and	CCONJ
cet-14418	123	11	it	it	PRON
cet-14418	123	12	increases	increase	VERB
cet-14418	123	13	with	with	ADP
cet-14418	123	14	the	the	DET
cet-14418	123	15	distance	distance	NOUN
cet-14418	123	16	from	from	ADP
cet-14418	123	17	the	the	DET
cet-14418	123	18	inlet	inlet	NOUN
cet-14418	123	19	.	.	PUNCT
cet-14418	124	1	in	in	ADP
cet-14418	124	2	this	this	DET
cet-14418	124	3	simulation	simulation	NOUN
cet-14418	124	4	condition	condition	NOUN
cet-14418	124	5	,	,	PUNCT
cet-14418	124	6	the	the	DET
cet-14418	124	7	generation	generation	NOUN
cet-14418	124	8	of	of	ADP
cet-14418	124	9	ch3oh	ch3oh	PROPN
cet-14418	124	10	is	be	AUX
cet-14418	124	11	largest	large	ADJ
cet-14418	124	12	in	in	ADP
cet-14418	124	13	the	the	DET
cet-14418	124	14	hollow	hollow	ADJ
cet-14418	124	15	-	-	PUNCT
cet-14418	124	16	cylinder	cylinder	NOUN
cet-14418	124	17	-	-	PUNCT
cet-14418	124	18	shaped	shape	VERB
cet-14418	124	19	pellets	pellet	NOUN
cet-14418	124	20	,	,	PUNCT
cet-14418	124	21	followed	follow	VERB
cet-14418	124	22	by	by	ADP
cet-14418	124	23	the	the	DET
cet-14418	124	24	cylinderand	cylinderand	NOUN
cet-14418	124	25	the	the	DET
cet-14418	124	26	sphereshaped	sphereshape	VERB
cet-14418	124	27	ones	one	NOUN
cet-14418	124	28	.	.	PUNCT
cet-14418	125	1	this	this	DET
cet-14418	125	2	order	order	NOUN
cet-14418	125	3	agrees	agree	VERB
cet-14418	125	4	with	with	ADP
cet-14418	125	5	that	that	PRON
cet-14418	125	6	of	of	ADP
cet-14418	125	7	the	the	DET
cet-14418	125	8	specific	specific	ADJ
cet-14418	125	9	surface	surface	NOUN
cet-14418	125	10	area	area	NOUN
cet-14418	125	11	of	of	ADP
cet-14418	125	12	the	the	DET
cet-14418	125	13	pellets	pellet	NOUN
cet-14418	125	14	(	(	PUNCT
cet-14418	125	15	table	table	NOUN
cet-14418	125	16	4	4	NUM
cet-14418	125	17	)	)	PUNCT
cet-14418	125	18	,	,	PUNCT
cet-14418	125	19	suggesting	suggest	VERB
cet-14418	125	20	that	that	SCONJ
cet-14418	125	21	the	the	DET
cet-14418	125	22	pellet	pellet	NOUN
cet-14418	125	23	surface	surface	NOUN
cet-14418	125	24	area	area	NOUN
cet-14418	125	25	in	in	ADP
cet-14418	125	26	the	the	DET
cet-14418	125	27	catalyst	catalyst	NOUN
cet-14418	125	28	bed	bed	NOUN
cet-14418	125	29	layer	layer	NOUN
cet-14418	125	30	is	be	AUX
cet-14418	125	31	the	the	DET
cet-14418	125	32	dominant	dominant	ADJ
cet-14418	125	33	factor	factor	NOUN
cet-14418	125	34	of	of	ADP
cet-14418	125	35	ch3oh	ch3oh	NOUN
cet-14418	125	36	generation	generation	NOUN
cet-14418	125	37	in	in	ADP
cet-14418	125	38	the	the	DET
cet-14418	125	39	conditions	condition	NOUN
cet-14418	125	40	,	,	PUNCT
cet-14418	125	41	compared	compare	VERB
cet-14418	125	42	to	to	ADP
cet-14418	125	43	permeability	permeability	NOUN
cet-14418	125	44	,	,	PUNCT
cet-14418	125	45	thermal	thermal	ADJ
cet-14418	125	46	conductivity	conductivity	NOUN
cet-14418	125	47	,	,	PUNCT
cet-14418	125	48	and	and	CCONJ
cet-14418	125	49	diffusion	diffusion	NOUN
cet-14418	125	50	coefficient	coefficient	NOUN
cet-14418	125	51	.	.	PUNCT
cet-14418	126	1	it	it	PRON
cet-14418	126	2	should	should	AUX
cet-14418	126	3	be	be	AUX
cet-14418	126	4	noted	note	VERB
cet-14418	126	5	that	that	SCONJ
cet-14418	126	6	these	these	DET
cet-14418	126	7	results	result	NOUN
cet-14418	126	8	47	47	NUM
cet-14418	126	9	can	can	AUX
cet-14418	126	10	vary	vary	VERB
cet-14418	126	11	greatly	greatly	ADV
cet-14418	126	12	depending	depend	VERB
cet-14418	126	13	on	on	ADP
cet-14418	126	14	conditions	condition	NOUN
cet-14418	126	15	such	such	ADJ
cet-14418	126	16	as	as	ADP
cet-14418	126	17	temperature	temperature	NOUN
cet-14418	126	18	,	,	PUNCT
cet-14418	126	19	pressure	pressure	NOUN
cet-14418	126	20	,	,	PUNCT
cet-14418	126	21	and	and	CCONJ
cet-14418	126	22	reactor	reactor	NOUN
cet-14418	126	23	geometry	geometry	NOUN
cet-14418	126	24	.	.	PUNCT
cet-14418	127	1	however	however	ADV
cet-14418	127	2	,	,	PUNCT
cet-14418	127	3	the	the	DET
cet-14418	127	4	present	present	ADJ
cet-14418	127	5	model	model	NOUN
cet-14418	127	6	is	be	AUX
cet-14418	127	7	significant	significant	ADJ
cet-14418	127	8	in	in	SCONJ
cet-14418	127	9	that	that	SCONJ
cet-14418	127	10	they	they	PRON
cet-14418	127	11	enable	enable	VERB
cet-14418	127	12	prediction	prediction	NOUN
cet-14418	127	13	of	of	ADP
cet-14418	127	14	macroscopic	macroscopic	ADJ
cet-14418	127	15	information	information	NOUN
cet-14418	127	16	such	such	ADJ
cet-14418	127	17	as	as	ADP
cet-14418	127	18	temperature	temperature	NOUN
cet-14418	127	19	,	,	PUNCT
cet-14418	127	20	flow	flow	NOUN
cet-14418	127	21	velocity	velocity	NOUN
cet-14418	127	22	,	,	PUNCT
cet-14418	127	23	and	and	CCONJ
cet-14418	127	24	methanol	methanol	NOUN
cet-14418	127	25	concentration	concentration	NOUN
cet-14418	127	26	in	in	ADP
cet-14418	127	27	the	the	DET
cet-14418	127	28	reactor	reactor	NOUN
cet-14418	127	29	from	from	ADP
cet-14418	127	30	microscopic	microscopic	ADJ
cet-14418	127	31	information	information	NOUN
cet-14418	127	32	such	such	ADJ
cet-14418	127	33	as	as	ADP
cet-14418	127	34	pellet	pellet	NOUN
cet-14418	127	35	shape	shape	NOUN
cet-14418	127	36	.	.	PUNCT
cet-14418	128	1	figure	figure	NOUN
cet-14418	128	2	5	5	NUM
cet-14418	128	3	.	.	PUNCT
cet-14418	129	1	(	(	PUNCT
cet-14418	129	2	a	a	X
cet-14418	129	3	)	)	PUNCT
cet-14418	129	4	gas	gas	NOUN
cet-14418	129	5	velocity	velocity	NOUN
cet-14418	129	6	,	,	PUNCT
cet-14418	129	7	(	(	PUNCT
cet-14418	129	8	b	b	NOUN
cet-14418	129	9	)	)	PUNCT
cet-14418	129	10	temperature	temperature	NOUN
cet-14418	129	11	,	,	PUNCT
cet-14418	129	12	(	(	PUNCT
cet-14418	129	13	c	c	NOUN
cet-14418	129	14	)	)	PUNCT
cet-14418	129	15	ch3oh	ch3oh	NOUN
cet-14418	129	16	concentration	concentration	NOUN
cet-14418	129	17	in	in	ADP
cet-14418	129	18	each	each	DET
cet-14418	129	19	pellet	pellet	NOUN
cet-14418	129	20	shape	shape	NOUN
cet-14418	129	21	.	.	PUNCT
cet-14418	130	1	4	4	X
cet-14418	130	2	.	.	X
cet-14418	130	3	conclusions	conclusion	NOUN
cet-14418	130	4	a	a	DET
cet-14418	130	5	stepwise	stepwise	PROPN
cet-14418	130	6	multiscale	multiscale	NOUN
cet-14418	130	7	model	model	NOUN
cet-14418	130	8	was	be	AUX
cet-14418	130	9	developed	develop	VERB
cet-14418	130	10	in	in	ADP
cet-14418	130	11	order	order	NOUN
cet-14418	130	12	to	to	PART
cet-14418	130	13	perform	perform	VERB
cet-14418	130	14	the	the	DET
cet-14418	130	15	homogeneous	homogeneous	ADJ
cet-14418	130	16	simulation	simulation	NOUN
cet-14418	130	17	of	of	ADP
cet-14418	130	18	the	the	DET
cet-14418	130	19	fixed	fix	VERB
cet-14418	130	20	-	-	PUNCT
cet-14418	130	21	bed	bed	NOUN
cet-14418	130	22	reactor	reactor	NOUN
cet-14418	130	23	of	of	ADP
cet-14418	130	24	co2	co2	NOUN
cet-14418	130	25	methanation	methanation	NOUN
cet-14418	130	26	considering	consider	VERB
cet-14418	130	27	the	the	DET
cet-14418	130	28	effect	effect	NOUN
cet-14418	130	29	of	of	ADP
cet-14418	130	30	3d	3d	NUM
cet-14418	130	31	packed	pack	VERB
cet-14418	130	32	pellet	pellet	NOUN
cet-14418	130	33	geometry	geometry	NOUN
cet-14418	130	34	.	.	PUNCT
cet-14418	131	1	the	the	DET
cet-14418	131	2	microscopic	microscopic	ADJ
cet-14418	131	3	parameters	parameter	NOUN
cet-14418	131	4	including	include	VERB
cet-14418	131	5	permeability	permeability	NOUN
cet-14418	131	6	,	,	PUNCT
cet-14418	131	7	effective	effective	ADJ
cet-14418	131	8	thermal	thermal	ADJ
cet-14418	131	9	conductivity	conductivity	NOUN
cet-14418	131	10	,	,	PUNCT
cet-14418	131	11	and	and	CCONJ
cet-14418	131	12	effective	effective	ADJ
cet-14418	131	13	diffusion	diffusion	NOUN
cet-14418	131	14	coefficient	coefficient	NOUN
cet-14418	131	15	were	be	AUX
cet-14418	131	16	found	find	VERB
cet-14418	131	17	to	to	PART
cet-14418	131	18	be	be	AUX
cet-14418	131	19	in	in	ADP
cet-14418	131	20	good	good	ADJ
cet-14418	131	21	agreement	agreement	NOUN
cet-14418	131	22	with	with	ADP
cet-14418	131	23	the	the	DET
cet-14418	131	24	values	value	NOUN
cet-14418	131	25	estimated	estimate	VERB
cet-14418	131	26	by	by	ADP
cet-14418	131	27	the	the	DET
cet-14418	131	28	deductive	deductive	ADJ
cet-14418	131	29	equations	equation	NOUN
cet-14418	131	30	.	.	PUNCT
cet-14418	132	1	a	a	DET
cet-14418	132	2	macro	macro	ADJ
cet-14418	132	3	-	-	ADJ
cet-14418	132	4	scale	scale	NOUN
cet-14418	132	5	model	model	NOUN
cet-14418	132	6	for	for	ADP
cet-14418	132	7	methanol	methanol	NOUN
cet-14418	132	8	synthesis	synthesis	NOUN
cet-14418	132	9	in	in	ADP
cet-14418	132	10	a	a	DET
cet-14418	132	11	fixed	fix	VERB
cet-14418	132	12	-	-	PUNCT
cet-14418	132	13	bed	bed	NOUN
cet-14418	132	14	reactor	reactor	NOUN
cet-14418	132	15	was	be	AUX
cet-14418	132	16	validated	validate	VERB
cet-14418	132	17	using	use	VERB
cet-14418	132	18	the	the	DET
cet-14418	132	19	condition	condition	NOUN
cet-14418	132	20	of	of	ADP
cet-14418	132	21	the	the	DET
cet-14418	132	22	cylindrical	cylindrical	ADJ
cet-14418	132	23	pellets	pellet	NOUN
cet-14418	132	24	of	of	ADP
cet-14418	132	25	zn.al2o3	zn.al2o3	NUM
cet-14418	132	26	with	with	ADP
cet-14418	132	27	the	the	DET
cet-14418	132	28	actual	actual	ADJ
cet-14418	132	29	experiment	experiment	NOUN
cet-14418	132	30	.	.	PUNCT
cet-14418	133	1	the	the	DET
cet-14418	133	2	effects	effect	NOUN
cet-14418	133	3	of	of	ADP
cet-14418	133	4	pellet	pellet	NOUN
cet-14418	133	5	shapes	shape	NOUN
cet-14418	133	6	,	,	PUNCT
cet-14418	133	7	including	include	VERB
cet-14418	133	8	spheres	sphere	NOUN
cet-14418	133	9	and	and	CCONJ
cet-14418	133	10	hollow	hollow	ADJ
cet-14418	133	11	cylinders	cylinder	NOUN
cet-14418	133	12	,	,	PUNCT
cet-14418	133	13	on	on	ADP
cet-14418	133	14	the	the	DET
cet-14418	133	15	reactor	reactor	NOUN
cet-14418	133	16	performance	performance	NOUN
cet-14418	133	17	were	be	AUX
cet-14418	133	18	studied	study	VERB
cet-14418	133	19	,	,	PUNCT
cet-14418	133	20	and	and	CCONJ
cet-14418	133	21	the	the	DET
cet-14418	133	22	results	result	NOUN
cet-14418	133	23	showed	show	VERB
cet-14418	133	24	that	that	SCONJ
cet-14418	133	25	the	the	DET
cet-14418	133	26	highest	high	ADJ
cet-14418	133	27	methanol	methanol	NOUN
cet-14418	133	28	reactivity	reactivity	NOUN
cet-14418	133	29	was	be	AUX
cet-14418	133	30	obtained	obtain	VERB
cet-14418	133	31	for	for	ADP
cet-14418	133	32	the	the	DET
cet-14418	133	33	hollow	hollow	ADJ
cet-14418	133	34	cylinder	cylinder	NOUN
cet-14418	133	35	pellets	pellet	NOUN
cet-14418	133	36	,	,	PUNCT
cet-14418	133	37	which	which	PRON
cet-14418	133	38	have	have	VERB
cet-14418	133	39	the	the	DET
cet-14418	133	40	largest	large	ADJ
cet-14418	133	41	surface	surface	NOUN
cet-14418	133	42	area	area	NOUN
cet-14418	133	43	,	,	PUNCT
cet-14418	133	44	rather	rather	ADV
cet-14418	133	45	than	than	ADP
cet-14418	133	46	the	the	DET
cet-14418	133	47	cylindrical	cylindrical	ADJ
cet-14418	133	48	pellets	pellet	NOUN
cet-14418	133	49	,	,	PUNCT
cet-14418	133	50	which	which	PRON
cet-14418	133	51	have	have	VERB
cet-14418	133	52	the	the	DET
cet-14418	133	53	highest	high	ADJ
cet-14418	133	54	permeability	permeability	NOUN
cet-14418	133	55	and	and	CCONJ
cet-14418	133	56	thermal	thermal	ADJ
cet-14418	133	57	conductivity	conductivity	NOUN
cet-14418	133	58	.	.	PUNCT
cet-14418	134	1	while	while	SCONJ
cet-14418	134	2	the	the	DET
cet-14418	134	3	results	result	NOUN
cet-14418	134	4	may	may	AUX
cet-14418	134	5	be	be	AUX
cet-14418	134	6	influenced	influence	VERB
cet-14418	134	7	by	by	ADP
cet-14418	134	8	factors	factor	NOUN
cet-14418	134	9	including	include	VERB
cet-14418	134	10	temperature	temperature	NOUN
cet-14418	134	11	,	,	PUNCT
cet-14418	134	12	pressure	pressure	NOUN
cet-14418	134	13	,	,	PUNCT
cet-14418	134	14	and	and	CCONJ
cet-14418	134	15	the	the	DET
cet-14418	134	16	reactor	reactor	NOUN
cet-14418	134	17	design	design	NOUN
cet-14418	134	18	,	,	PUNCT
cet-14418	134	19	the	the	DET
cet-14418	134	20	importance	importance	NOUN
cet-14418	134	21	of	of	ADP
cet-14418	134	22	the	the	DET
cet-14418	134	23	present	present	ADJ
cet-14418	134	24	model	model	NOUN
cet-14418	134	25	lies	lie	VERB
cet-14418	134	26	in	in	ADP
cet-14418	134	27	its	its	PRON
cet-14418	134	28	ability	ability	NOUN
cet-14418	134	29	to	to	PART
cet-14418	134	30	predict	predict	VERB
cet-14418	134	31	the	the	DET
cet-14418	134	32	reactions	reaction	NOUN
cet-14418	134	33	based	base	VERB
cet-14418	134	34	on	on	ADP
cet-14418	134	35	the	the	DET
cet-14418	134	36	pellet	pellet	NOUN
cet-14418	134	37	geometry	geometry	NOUN
cet-14418	134	38	.	.	PUNCT
cet-14418	135	1	as	as	ADP
cet-14418	135	2	a	a	DET
cet-14418	135	3	future	future	ADJ
cet-14418	135	4	research	research	NOUN
cet-14418	135	5	,	,	PUNCT
cet-14418	135	6	it	it	PRON
cet-14418	135	7	is	be	AUX
cet-14418	135	8	proposed	propose	VERB
cet-14418	135	9	to	to	PART
cet-14418	135	10	extend	extend	VERB
cet-14418	135	11	and	and	CCONJ
cet-14418	135	12	apply	apply	VERB
cet-14418	135	13	this	this	DET
cet-14418	135	14	model	model	NOUN
cet-14418	135	15	to	to	ADP
cet-14418	135	16	other	other	ADJ
cet-14418	135	17	pellet	pellet	NOUN
cet-14418	135	18	shapes	shape	NOUN
cet-14418	135	19	such	such	ADJ
cet-14418	135	20	as	as	ADP
cet-14418	135	21	cubes	cube	NOUN
cet-14418	135	22	and	and	CCONJ
cet-14418	135	23	cross	cross	NOUN
cet-14418	135	24	webs	webs	NOUN
cet-14418	135	25	,	,	PUNCT
cet-14418	135	26	and	and	CCONJ
cet-14418	135	27	to	to	PART
cet-14418	135	28	conduct	conduct	VERB
cet-14418	135	29	prediction	prediction	NOUN
cet-14418	135	30	and	and	CCONJ
cet-14418	135	31	verification	verification	NOUN
cet-14418	135	32	of	of	ADP
cet-14418	135	33	their	their	PRON
cet-14418	135	34	characteristics	characteristic	NOUN
cet-14418	135	35	.	.	PUNCT
cet-14418	136	1	references	reference	NOUN
cet-14418	136	2	adji	adji	VERB
cet-14418	136	3	b.s	b.s	PROPN
cet-14418	136	4	.	.	PROPN
cet-14418	136	5	,	,	PUNCT
cet-14418	136	6	muharam	muharam	PROPN
cet-14418	136	7	y.	y.	PROPN
cet-14418	136	8	,	,	PUNCT
cet-14418	136	9	kartohardjono	kartohardjono	NOUN
cet-14418	136	10	,	,	PUNCT
cet-14418	136	11	2019	2019	NUM
cet-14418	136	12	,	,	PUNCT
cet-14418	136	13	s.	s.	PROPN
cet-14418	136	14	simulation	simulation	PROPN
cet-14418	136	15	of	of	ADP
cet-14418	136	16	methanol	methanol	NOUN
cet-14418	136	17	synthesis	synthesis	NOUN
cet-14418	136	18	from	from	ADP
cet-14418	136	19	co2	co2	NOUN
cet-14418	136	20	hydrogenation	hydrogenation	NOUN
cet-14418	136	21	in	in	ADP
cet-14418	136	22	a	a	DET
cet-14418	136	23	packed	packed	ADJ
cet-14418	136	24	bed	bed	NOUN
cet-14418	136	25	reactor	reactor	NOUN
cet-14418	136	26	using	use	VERB
cet-14418	136	27	comsol	comsol	NOUN
cet-14418	136	28	multiphysics	multiphysic	NOUN
cet-14418	136	29	,	,	PUNCT
cet-14418	136	30	international	international	ADJ
cet-14418	136	31	journal	journal	NOUN
cet-14418	136	32	of	of	ADP
cet-14418	136	33	engineering	engineering	NOUN
cet-14418	136	34	research	research	NOUN
cet-14418	136	35	and	and	CCONJ
cet-14418	136	36	technology,12	technology,12	NOUN
cet-14418	136	37	,	,	PUNCT
cet-14418	136	38	12	12	NUM
cet-14418	136	39	,	,	PUNCT
cet-14418	136	40	2592	2592	NUM
cet-14418	136	41	-	-	SYM
cet-14418	136	42	2599	2599	NUM
cet-14418	136	43	.	.	PUNCT
cet-14418	137	1	ahn	ahn	PROPN
cet-14418	137	2	j.	j.	PROPN
cet-14418	137	3	,	,	PUNCT
cet-14418	137	4	kim	kim	PROPN
cet-14418	137	5	h.	h.	PROPN
cet-14418	137	6	,	,	PUNCT
cet-14418	137	7	ro	ro	PROPN
cet-14418	137	8	y.	y.	PROPN
cet-14418	137	9	,	,	PUNCT
cet-14418	137	10	kim	kim	PROPN
cet-14418	137	11	j.	j.	PROPN
cet-14418	137	12	,	,	PUNCT
cet-14418	137	13	chung	chung	PROPN
cet-14418	137	14	w.	w.	PROPN
cet-14418	137	15	,	,	PUNCT
cet-14418	137	16	chang	chang	PROPN
cet-14418	137	17	s.	s.	PROPN
cet-14418	137	18	,	,	PUNCT
cet-14418	137	19	2021	2021	NUM
cet-14418	137	20	,	,	PUNCT
cet-14418	137	21	development	development	NOUN
cet-14418	137	22	of	of	ADP
cet-14418	137	23	pilot	pilot	NOUN
cet-14418	137	24	-	-	PUNCT
cet-14418	137	25	scale	scale	NOUN
cet-14418	137	26	co2	co2	NOUN
cet-14418	137	27	methanation	methanation	NOUN
cet-14418	137	28	using	use	VERB
cet-14418	137	29	pellet	pellet	NOUN
cet-14418	137	30	-	-	PUNCT
cet-14418	137	31	type	type	NOUN
cet-14418	137	32	catalysts	catalyst	NOUN
cet-14418	137	33	for	for	ADP
cet-14418	137	34	co2	co2	NOUN
cet-14418	137	35	recycling	recycling	NOUN
cet-14418	137	36	in	in	ADP
cet-14418	137	37	sewage	sewage	NOUN
cet-14418	137	38	treatment	treatment	NOUN
cet-14418	137	39	plants	plant	NOUN
cet-14418	137	40	and	and	CCONJ
cet-14418	137	41	its	its	PRON
cet-14418	137	42	validation	validation	NOUN
cet-14418	137	43	through	through	ADP
cet-14418	137	44	computational	computational	ADJ
cet-14418	137	45	fluid	fluid	ADJ
cet-14418	137	46	dynamics	dynamic	NOUN
cet-14418	137	47	(	(	PUNCT
cet-14418	137	48	cfd	cfd	NOUN
cet-14418	137	49	)	)	PUNCT
cet-14418	137	50	modeling	modeling	NOUN
cet-14418	137	51	.	.	PUNCT
cet-14418	138	1	catalysts	catalyst	NOUN
cet-14418	138	2	11	11	NUM
cet-14418	138	3	,	,	PUNCT
cet-14418	138	4	1005	1005	NUM
cet-14418	138	5	.	.	PUNCT
cet-14418	139	1	alarcón	alarcón	PROPN
cet-14418	139	2	a.	a.	PROPN
cet-14418	139	3	,	,	PUNCT
cet-14418	139	4	busqué	busqué	PROPN
cet-14418	139	5	r.	r.	PROPN
cet-14418	139	6	,	,	PUNCT
cet-14418	139	7	andreu	andreu	PROPN
cet-14418	139	8	t.	t.	PROPN
cet-14418	139	9	,	,	PUNCT
cet-14418	139	10	guilera	guilera	PROPN
cet-14418	139	11	j.	j.	PROPN
cet-14418	139	12	,	,	PUNCT
cet-14418	139	13	2022	2022	NUM
cet-14418	139	14	,	,	PUNCT
cet-14418	139	15	design	design	NOUN
cet-14418	139	16	of	of	ADP
cet-14418	139	17	a	a	DET
cet-14418	139	18	multi	multi	ADJ
cet-14418	139	19	-	-	ADJ
cet-14418	139	20	tubular	tubular	ADJ
cet-14418	139	21	catalytic	catalytic	ADJ
cet-14418	139	22	reactor	reactor	NOUN
cet-14418	139	23	assisted	assist	VERB
cet-14418	139	24	by	by	ADP
cet-14418	139	25	cfd	cfd	NOUN
cet-14418	139	26	based	base	VERB
cet-14418	139	27	on	on	ADP
cet-14418	139	28	free	free	ADJ
cet-14418	139	29	-	-	PUNCT
cet-14418	139	30	convection	convection	NOUN
cet-14418	139	31	heat	heat	NOUN
cet-14418	139	32	-	-	PUNCT
cet-14418	139	33	management	management	NOUN
cet-14418	139	34	for	for	ADP
cet-14418	139	35	decentralised	decentralised	ADJ
cet-14418	139	36	synthetic	synthetic	ADJ
cet-14418	139	37	methane	methane	NOUN
cet-14418	139	38	production	production	NOUN
cet-14418	139	39	.	.	PUNCT
cet-14418	140	1	catalysts	catalyst	NOUN
cet-14418	140	2	,	,	PUNCT
cet-14418	140	3	12	12	NUM
cet-14418	140	4	,	,	PUNCT
cet-14418	140	5	1053	1053	NUM
cet-14418	140	6	.	.	PUNCT
cet-14418	141	1	an	an	DET
cet-14418	141	2	q.	q.	NOUN
cet-14418	141	3	,	,	PUNCT
cet-14418	141	4	on	on	ADP
cet-14418	141	5	application	application	NOUN
cet-14418	141	6	of	of	ADP
cet-14418	141	7	computer	computer	NOUN
cet-14418	141	8	simulation	simulation	NOUN
cet-14418	141	9	technology	technology	NOUN
cet-14418	141	10	in	in	ADP
cet-14418	141	11	methanol	methanol	NOUN
cet-14418	141	12	synthesis	synthesis	NOUN
cet-14418	141	13	in	in	ADP
cet-14418	141	14	the	the	DET
cet-14418	141	15	coal	coal	NOUN
cet-14418	141	16	chemical	chemical	NOUN
cet-14418	141	17	industry	industry	NOUN
cet-14418	141	18	,	,	PUNCT
cet-14418	141	19	2017	2017	NUM
cet-14418	141	20	,	,	PUNCT
cet-14418	141	21	chemical	chemical	NOUN
cet-14418	141	22	engineering	engineering	NOUN
cet-14418	141	23	transactions	transaction	NOUN
cet-14418	141	24	59	59	NUM
cet-14418	141	25	,	,	PUNCT
cet-14418	141	26	607	607	NUM
cet-14418	141	27	-	-	PUNCT
cet-14418	141	28	612	612	NUM
cet-14418	141	29	.	.	PUNCT
cet-14418	142	1	fu	fu	PROPN
cet-14418	142	2	j.	j.	PROPN
cet-14418	142	3	,	,	PUNCT
cet-14418	142	4	hywel	hywel	PROPN
cet-14418	142	5	r.	r.	PROPN
cet-14418	142	6	t.	t.	PROPN
cet-14418	142	7	,	,	PUNCT
cet-14418	142	8	li	li	PROPN
cet-14418	142	9	c.	c.	PROPN
cet-14418	142	10	,	,	PUNCT
cet-14418	142	11	2021	2021	NUM
cet-14418	142	12	,	,	PUNCT
cet-14418	142	13	tortuosity	tortuosity	NOUN
cet-14418	142	14	of	of	ADP
cet-14418	142	15	porous	porous	ADJ
cet-14418	142	16	media	medium	NOUN
cet-14418	142	17	:	:	PUNCT
cet-14418	142	18	image	image	NOUN
cet-14418	142	19	analysis	analysis	NOUN
cet-14418	142	20	and	and	CCONJ
cet-14418	142	21	physical	physical	ADJ
cet-14418	142	22	simulation	simulation	NOUN
cet-14418	142	23	.	.	PUNCT
cet-14418	143	1	earthscience	earthscience	NOUN
cet-14418	143	2	reviews	review	NOUN
cet-14418	143	3	2021	2021	NUM
cet-14418	143	4	,	,	PUNCT
cet-14418	143	5	212	212	NUM
cet-14418	143	6	,	,	PUNCT
cet-14418	143	7	103439	103439	NUM
cet-14418	143	8	.	.	PUNCT
cet-14418	144	1	kato	kato	PROPN
cet-14418	144	2	y.	y.	PROPN
cet-14418	144	3	,	,	PUNCT
cet-14418	144	4	2010	2010	NUM
cet-14418	144	5	,	,	PUNCT
cet-14418	144	6	carbon	carbon	NOUN
cet-14418	144	7	recycling	recycling	NOUN
cet-14418	144	8	for	for	ADP
cet-14418	144	9	reduction	reduction	NOUN
cet-14418	144	10	of	of	ADP
cet-14418	144	11	carbon	carbon	NOUN
cet-14418	144	12	dioxide	dioxide	NOUN
cet-14418	144	13	emission	emission	NOUN
cet-14418	144	14	from	from	ADP
cet-14418	144	15	iron	iron	NOUN
cet-14418	144	16	-	-	PUNCT
cet-14418	144	17	making	make	VERB
cet-14418	144	18	process	process	NOUN
cet-14418	144	19	.	.	PUNCT
cet-14418	145	1	isij	isij	PROPN
cet-14418	145	2	international	international	PROPN
cet-14418	145	3	,	,	PUNCT
cet-14418	145	4	50	50	NUM
cet-14418	145	5	,	,	PUNCT
cet-14418	145	6	181–185	181–185	NUM
cet-14418	145	7	.	.	PUNCT
cet-14418	146	1	maestri	maestri	PROPN
cet-14418	146	2	m.	m.	PROPN
cet-14418	146	3	,	,	PUNCT
cet-14418	146	4	cuoci	cuoci	PROPN
cet-14418	146	5	a.	a.	NOUN
cet-14418	146	6	,	,	PUNCT
cet-14418	146	7	2013	2013	NUM
cet-14418	146	8	,	,	PUNCT
cet-14418	146	9	coupling	couple	VERB
cet-14418	146	10	cfd	cfd	NOUN
cet-14418	146	11	with	with	ADP
cet-14418	146	12	detailed	detailed	ADJ
cet-14418	146	13	microkinetic	microkinetic	ADJ
cet-14418	146	14	modelling	modelling	NOUN
cet-14418	146	15	in	in	ADP
cet-14418	146	16	heterogeneous	heterogeneous	ADJ
cet-14418	146	17	catalysis	catalysis	NOUN
cet-14418	146	18	,	,	PUNCT
cet-14418	146	19	chemical	chemical	NOUN
cet-14418	146	20	engineering	engineering	NOUN
cet-14418	146	21	science	science	NOUN
cet-14418	146	22	96	96	NUM
cet-14418	146	23	,	,	PUNCT
cet-14418	146	24	106	106	NUM
cet-14418	146	25	.	.	PUNCT
cet-14418	147	1	shahrokhi	shahrokhi	PROPN
cet-14418	147	2	m.	m.	NOUN
cet-14418	147	3	and	and	CCONJ
cet-14418	147	4	baghmisheh	baghmisheh	PROPN
cet-14418	147	5	g.r	g.r	PROPN
cet-14418	147	6	.	.	PROPN
cet-14418	147	7	,	,	PUNCT
cet-14418	147	8	2005	2005	NUM
cet-14418	147	9	,	,	PUNCT
cet-14418	147	10	modeling	modeling	NOUN
cet-14418	147	11	,	,	PUNCT
cet-14418	147	12	simulation	simulation	NOUN
cet-14418	147	13	and	and	CCONJ
cet-14418	147	14	control	control	NOUN
cet-14418	147	15	of	of	ADP
cet-14418	147	16	a	a	DET
cet-14418	147	17	methanol	methanol	NOUN
cet-14418	147	18	synthesisfixed	synthesisfixe	VERB
cet-14418	147	19	-	-	PUNCT
cet-14418	147	20	bed	bed	NOUN
cet-14418	147	21	reactor	reactor	NOUN
cet-14418	147	22	,	,	PUNCT
cet-14418	147	23	chemical	chemical	NOUN
cet-14418	147	24	engineering	engineering	NOUN
cet-14418	147	25	science	science	NOUN
cet-14418	147	26	60	60	NUM
cet-14418	147	27	,	,	PUNCT
cet-14418	147	28	4275	4275	NUM
cet-14418	147	29	.	.	PUNCT
cet-14418	148	1	son	son	PROPN
cet-14418	148	2	m.	m.	NOUN
cet-14418	148	3	,	,	PUNCT
cet-14418	148	4	woo	woo	VERB
cet-14418	148	5	y.	y.	PROPN
cet-14418	148	6	,	,	PUNCT
cet-14418	148	7	kwak	kwak	PROPN
cet-14418	148	8	g.	g.	PROPN
cet-14418	148	9	,	,	PUNCT
cet-14418	148	10	lee	lee	PROPN
cet-14418	148	11	y.	y.	PROPN
cet-14418	148	12	j.	j.	PROPN
cet-14418	148	13	,	,	PUNCT
cet-14418	148	14	park	park	PROPN
cet-14418	148	15	m.	m.	PROPN
cet-14418	148	16	j.	j.	PROPN
cet-14418	148	17	,	,	PUNCT
cet-14418	148	18	2019	2019	NUM
cet-14418	148	19	,	,	PUNCT
cet-14418	148	20	cfd	cfd	NOUN
cet-14418	148	21	modeling	modeling	NOUN
cet-14418	148	22	of	of	ADP
cet-14418	148	23	a	a	DET
cet-14418	148	24	compact	compact	ADJ
cet-14418	148	25	reactor	reactor	NOUN
cet-14418	148	26	for	for	ADP
cet-14418	148	27	methanol	methanol	NOUN
cet-14418	148	28	synthesis	synthesis	NOUN
cet-14418	148	29	:	:	PUNCT
cet-14418	148	30	maximizing	maximize	VERB
cet-14418	148	31	productivity	productivity	NOUN
cet-14418	148	32	with	with	ADP
cet-14418	148	33	increased	increase	VERB
cet-14418	148	34	thermal	thermal	ADJ
cet-14418	148	35	controllability	controllability	NOUN
cet-14418	148	36	,	,	PUNCT
cet-14418	148	37	international	international	ADJ
cet-14418	148	38	journal	journal	NOUN
cet-14418	148	39	of	of	ADP
cet-14418	148	40	heat	heat	NOUN
cet-14418	148	41	and	and	CCONJ
cet-14418	148	42	mass	mass	NOUN
cet-14418	148	43	transfer	transfer	NOUN
cet-14418	148	44	145	145	NUM
cet-14418	148	45	,	,	PUNCT
cet-14418	148	46	118776	118776	NUM
cet-14418	148	47	.	.	PUNCT
cet-14418	149	1	taco	taco	PROPN
cet-14418	149	2	-	-	PUNCT
cet-14418	149	3	vasquez	vasquez	PROPN
cet-14418	149	4	s.	s.	PROPN
cet-14418	149	5	,	,	PUNCT
cet-14418	149	6	ron	ron	PROPN
cet-14418	149	7	c.a	c.a	PROPN
cet-14418	149	8	.	.	PROPN
cet-14418	149	9	,	,	PUNCT
cet-14418	149	10	murillo	murillo	PROPN
cet-14418	149	11	h.a	h.a	PROPN
cet-14418	149	12	.	.	PROPN
cet-14418	149	13	,	,	PUNCT
cet-14418	149	14	chico	chico	PROPN
cet-14418	149	15	a.	a.	PROPN
cet-14418	149	16	,	,	PUNCT
cet-14418	149	17	arauz	arauz	PROPN
cet-14418	149	18	p.g	p.g	PROPN
cet-14418	149	19	.	.	PROPN
cet-14418	149	20	,	,	PUNCT
cet-14418	149	21	2022	2022	NUM
cet-14418	149	22	,	,	PUNCT
cet-14418	149	23	thermochemical	thermochemical	ADJ
cet-14418	149	24	analysis	analysis	NOUN
cet-14418	149	25	of	of	ADP
cet-14418	149	26	a	a	DET
cet-14418	149	27	packedbed	packedbe	VERB
cet-14418	149	28	reactor	reactor	NOUN
cet-14418	149	29	using	use	VERB
cet-14418	149	30	finite	finite	ADJ
cet-14418	149	31	elements	element	NOUN
cet-14418	149	32	with	with	ADP
cet-14418	149	33	flexpde	flexpde	NOUN
cet-14418	149	34	and	and	CCONJ
cet-14418	149	35	comsol	comsol	NOUN
cet-14418	149	36	multiphysics	multiphysic	NOUN
cet-14418	149	37	.	.	PUNCT
cet-14418	150	1	processes	process	NOUN
cet-14418	150	2	,	,	PUNCT
cet-14418	150	3	10	10	NUM
cet-14418	150	4	,	,	PUNCT
cet-14418	150	5	1144	1144	NUM
cet-14418	150	6	.	.	PUNCT
cet-14418	151	1	zhang	zhang	PROPN
cet-14418	151	2	x.	x.	PROPN
cet-14418	151	3	,	,	PUNCT
cet-14418	151	4	zhang	zhang	PROPN
cet-14418	151	5	g	g	PROPN
cet-14418	151	6	,	,	PUNCT
cet-14418	151	7	song	song	PROPN
cet-14418	151	8	c.	c.	PROPN
cet-14418	151	9	,	,	PUNCT
cet-14418	151	10	guo	guo	PROPN
cet-14418	151	11	x.	x.	PROPN
cet-14418	151	12	,	,	PUNCT
cet-14418	151	13	2021	2021	NUM
cet-14418	151	14	,	,	PUNCT
cet-14418	151	15	catalytic	catalytic	ADJ
cet-14418	151	16	conversion	conversion	NOUN
cet-14418	151	17	of	of	ADP
cet-14418	151	18	carbon	carbon	NOUN
cet-14418	151	19	dioxide	dioxide	NOUN
cet-14418	151	20	to	to	PART
cet-14418	151	21	methanol	methanol	VERB
cet-14418	151	22	:	:	PUNCT
cet-14418	151	23	current	current	ADJ
cet-14418	151	24	status	status	NOUN
cet-14418	151	25	and	and	CCONJ
cet-14418	151	26	future	future	ADJ
cet-14418	151	27	perspective	perspective	NOUN
cet-14418	151	28	.	.	PUNCT
cet-14418	152	1	frontiers	frontier	NOUN
cet-14418	152	2	in	in	ADP
cet-14418	152	3	energy	energy	NOUN
cet-14418	152	4	research	research	NOUN
cet-14418	152	5	8	8	NUM
cet-14418	152	6	,	,	PUNCT
cet-14418	152	7	621119	621119	NUM
cet-14418	152	8	.	.	PUNCT
cet-14418	153	1	48	48	NUM
cet-14418	153	2	296takagishi-pagato.pdf	296takagishi-pagato.pdf	NUM
cet-14418	153	3	multi	multi	ADJ
cet-14418	153	4	-	-	ADJ
cet-14418	153	5	scale	scale	ADJ
cet-14418	153	6	simulations	simulation	NOUN
cet-14418	153	7	in	in	ADP
cet-14418	153	8	a	a	DET
cet-14418	153	9	catalytic	catalytic	ADJ
cet-14418	153	10	reactor	reactor	NOUN
cet-14418	153	11	considering	consider	VERB
cet-14418	153	12	three	three	NUM
cet-14418	153	13	-	-	PUNCT
cet-14418	153	14	dimensional	dimensional	ADJ
cet-14418	153	15	pellet	pellet	NOUN
cet-14418	153	16	geometry	geometry	NOUN
