id	sid	tid	token	lemma	pos
cet-15373	1	1	doi	doi	NOUN
cet-15373	1	2	:	:	PUNCT
cet-15373	1	3	10.3303	10.3303	NUM
cet-15373	1	4	/	/	SYM
cet-15373	1	5	cet25117123	cet25117123	PROPN
cet-15373	1	6	paper	paper	NOUN
cet-15373	1	7	received	receive	VERB
cet-15373	1	8	:	:	PUNCT
cet-15373	1	9	11	11	NUM
cet-15373	1	10	january	january	NOUN
cet-15373	1	11	2025	2025	NUM
cet-15373	1	12	;	;	PUNCT
cet-15373	1	13	revised	revise	VERB
cet-15373	1	14	:	:	PUNCT
cet-15373	1	15	10	10	NUM
cet-15373	1	16	april	april	PROPN
cet-15373	1	17	2025	2025	NUM
cet-15373	1	18	;	;	PUNCT
cet-15373	1	19	accepted	accept	VERB
cet-15373	1	20	:	:	PUNCT
cet-15373	1	21	11	11	NUM
cet-15373	1	22	may	may	AUX
cet-15373	1	23	2025	2025	NUM
cet-15373	1	24	please	please	INTJ
cet-15373	1	25	cite	cite	VERB
cet-15373	1	26	this	this	DET
cet-15373	1	27	article	article	NOUN
cet-15373	1	28	as	as	ADP
cet-15373	1	29	:	:	PUNCT
cet-15373	1	30	miceli	miceli	PROPN
cet-15373	1	31	m.	m.	NOUN
cet-15373	1	32	,	,	PUNCT
cet-15373	1	33	tavella	tavella	PROPN
cet-15373	1	34	f.	f.	PROPN
cet-15373	1	35	,	,	PUNCT
cet-15373	1	36	giusi	giusi	PROPN
cet-15373	1	37	d.	d.	PROPN
cet-15373	1	38	,	,	PUNCT
cet-15373	1	39	tefera	tefera	NOUN
cet-15373	1	40	m.e	m.e	PROPN
cet-15373	1	41	.	.	PROPN
cet-15373	1	42	,	,	PUNCT
cet-15373	1	43	torre	torre	PROPN
cet-15373	1	44	m.f	m.f	PROPN
cet-15373	1	45	.	.	PROPN
cet-15373	1	46	,	,	PUNCT
cet-15373	1	47	perathoner	perathoner	PROPN
cet-15373	1	48	s.	s.	PROPN
cet-15373	1	49	,	,	PUNCT
cet-15373	1	50	centi	centi	PROPN
cet-15373	1	51	g.	g.	PROPN
cet-15373	1	52	,	,	PUNCT
cet-15373	1	53	ampelli	ampelli	PROPN
cet-15373	1	54	c.	c.	PROPN
cet-15373	1	55	,	,	PUNCT
cet-15373	1	56	2025	2025	NUM
cet-15373	1	57	,	,	PUNCT
cet-15373	1	58	activation	activation	NOUN
cet-15373	1	59	of	of	ADP
cet-15373	1	60	dinitrogen	dinitrogen	NOUN
cet-15373	1	61	molecule	molecule	NOUN
cet-15373	1	62	(	(	PUNCT
cet-15373	1	63	n2	n2	NOUN
cet-15373	1	64	)	)	PUNCT
cet-15373	1	65	in	in	ADP
cet-15373	1	66	unconventional	unconventional	ADJ
cet-15373	1	67	electrochemical	electrochemical	ADJ
cet-15373	1	68	reactors	reactor	NOUN
cet-15373	1	69	for	for	ADP
cet-15373	1	70	ammonia	ammonia	NOUN
cet-15373	1	71	production	production	NOUN
cet-15373	1	72	,	,	PUNCT
cet-15373	1	73	chemical	chemical	NOUN
cet-15373	1	74	engineering	engineering	NOUN
cet-15373	1	75	transactions	transaction	NOUN
cet-15373	1	76	,	,	PUNCT
cet-15373	1	77	117	117	NUM
cet-15373	1	78	,	,	PUNCT
cet-15373	1	79	733738	733738	NUM
cet-15373	1	80	doi:10.3303	doi:10.3303	X
cet-15373	1	81	/	/	SYM
cet-15373	1	82	cet25117123	cet25117123	VERB
cet-15373	1	83	chemical	chemical	PROPN
cet-15373	1	84	engineering	engineering	NOUN
cet-15373	1	85	transactions	transaction	NOUN
cet-15373	1	86	vol	vol	NOUN
cet-15373	1	87	.	.	PROPN
cet-15373	1	88	117	117	NUM
cet-15373	1	89	,	,	PUNCT
cet-15373	1	90	2025	2025	NUM
cet-15373	1	91	a	a	DET
cet-15373	1	92	publication	publication	NOUN
cet-15373	1	93	of	of	ADP
cet-15373	1	94	the	the	DET
cet-15373	1	95	italian	italian	ADJ
cet-15373	1	96	association	association	NOUN
cet-15373	1	97	of	of	ADP
cet-15373	1	98	chemical	chemical	PROPN
cet-15373	1	99	engineering	engineering	NOUN
cet-15373	1	100	online	online	ADV
cet-15373	1	101	at	at	ADP
cet-15373	1	102	www.cetjournal.it	www.cetjournal.it	PROPN
cet-15373	1	103	guest	guest	NOUN
cet-15373	1	104	editors	editor	NOUN
cet-15373	1	105	:	:	PUNCT
cet-15373	1	106	fabrizio	fabrizio	PROPN
cet-15373	1	107	bezzo	bezzo	PROPN
cet-15373	1	108	,	,	PUNCT
cet-15373	1	109	flavio	flavio	PROPN
cet-15373	1	110	manenti	manenti	PROPN
cet-15373	1	111	,	,	PUNCT
cet-15373	1	112	gabriele	gabriele	PROPN
cet-15373	1	113	pannocchia	pannocchia	PROPN
cet-15373	1	114	,	,	PUNCT
cet-15373	1	115	almerinda	almerinda	PROPN
cet-15373	1	116	di	di	PROPN
cet-15373	1	117	benedetto	benedetto	PROPN
cet-15373	1	118	copyright	copyright	PROPN
cet-15373	1	119	©	©	PROPN
cet-15373	1	120	2025	2025	NUM
cet-15373	1	121	,	,	PUNCT
cet-15373	1	122	aidic	aidic	ADJ
cet-15373	1	123	servizi	servizi	PROPN
cet-15373	1	124	s.r.l	s.r.l	NOUN
cet-15373	1	125	.	.	PUNCT
cet-15373	2	1	isbn	isbn	PROPN
cet-15373	2	2	979	979	NUM
cet-15373	2	3	-	-	SYM
cet-15373	2	4	12	12	NUM
cet-15373	2	5	-	-	PUNCT
cet-15373	2	6	81206	81206	NUM
cet-15373	2	7	-	-	SYM
cet-15373	2	8	17	17	NUM
cet-15373	2	9	-	-	SYM
cet-15373	2	10	5	5	NUM
cet-15373	2	11	;	;	PUNCT
cet-15373	2	12	issn	issn	PROPN
cet-15373	2	13	2283	2283	NUM
cet-15373	2	14	-	-	SYM
cet-15373	2	15	9216	9216	NUM
cet-15373	2	16	activation	activation	NOUN
cet-15373	2	17	of	of	ADP
cet-15373	2	18	dinitrogen	dinitrogen	NOUN
cet-15373	2	19	molecule	molecule	NOUN
cet-15373	2	20	(	(	PUNCT
cet-15373	2	21	n2	n2	NOUN
cet-15373	2	22	)	)	PUNCT
cet-15373	2	23	in	in	ADP
cet-15373	2	24	unconventional	unconventional	ADJ
cet-15373	2	25	electrochemical	electrochemical	ADJ
cet-15373	2	26	reactors	reactor	NOUN
cet-15373	2	27	for	for	ADP
cet-15373	2	28	ammonia	ammonia	NOUN
cet-15373	2	29	production	production	NOUN
cet-15373	2	30	matteo	matteo	PROPN
cet-15373	2	31	miceli	miceli	PROPN
cet-15373	2	32	*	*	PROPN
cet-15373	2	33	,	,	PUNCT
cet-15373	2	34	francesco	francesco	PROPN
cet-15373	2	35	tavella	tavella	PROPN
cet-15373	2	36	,	,	PUNCT
cet-15373	2	37	daniele	daniele	PROPN
cet-15373	2	38	giusi	giusi	PROPN
cet-15373	2	39	,	,	PUNCT
cet-15373	2	40	muluken	muluken	PROPN
cet-15373	2	41	eshetu	eshetu	PROPN
cet-15373	2	42	tefera	tefera	PROPN
cet-15373	2	43	,	,	PUNCT
cet-15373	2	44	marco	marco	PROPN
cet-15373	2	45	francesco	francesco	PROPN
cet-15373	2	46	torre	torre	PROPN
cet-15373	2	47	,	,	PUNCT
cet-15373	2	48	siglinda	siglinda	NOUN
cet-15373	2	49	perathoner	perathoner	NOUN
cet-15373	2	50	,	,	PUNCT
cet-15373	2	51	gabriele	gabriele	PROPN
cet-15373	2	52	centi	centi	PROPN
cet-15373	2	53	,	,	PUNCT
cet-15373	2	54	claudio	claudio	PROPN
cet-15373	2	55	ampelli	ampelli	PROPN
cet-15373	2	56	department	department	PROPN
cet-15373	2	57	of	of	ADP
cet-15373	2	58	chemical	chemical	PROPN
cet-15373	2	59	,	,	PUNCT
cet-15373	2	60	biological	biological	ADJ
cet-15373	2	61	,	,	PUNCT
cet-15373	2	62	pharmaceutical	pharmaceutical	ADJ
cet-15373	2	63	and	and	CCONJ
cet-15373	2	64	environmental	environmental	ADJ
cet-15373	2	65	sciences	sciences	PROPN
cet-15373	2	66	(	(	PUNCT
cet-15373	2	67	chibiofaram	chibiofaram	PROPN
cet-15373	2	68	)	)	PUNCT
cet-15373	2	69	–	–	PUNCT
cet-15373	2	70	university	university	NOUN
cet-15373	2	71	of	of	ADP
cet-15373	2	72	messina	messina	PROPN
cet-15373	2	73	,	,	PUNCT
cet-15373	2	74	eric	eric	PROPN
cet-15373	2	75	aisbl	aisbl	PROPN
cet-15373	2	76	and	and	CCONJ
cet-15373	2	77	caspe	caspe	PROPN
cet-15373	2	78	/	/	SYM
cet-15373	2	79	instm	instm	PROPN
cet-15373	2	80	,	,	PUNCT
cet-15373	2	81	v.le	v.le	PROPN
cet-15373	2	82	f.	f.	PROPN
cet-15373	2	83	stagno	stagno	PROPN
cet-15373	2	84	d'alcontres	d'alcontres	PROPN
cet-15373	2	85	,	,	PUNCT
cet-15373	2	86	31	31	NUM
cet-15373	2	87	–	–	SYM
cet-15373	2	88	98166	98166	NUM
cet-15373	2	89	messina	messina	PROPN
cet-15373	2	90	,	,	PUNCT
cet-15373	2	91	italy	italy	PROPN
cet-15373	2	92	matmiceli@unime.it	matmiceli@unime.it	X
cet-15373	2	93	in	in	ADP
cet-15373	2	94	this	this	DET
cet-15373	2	95	study	study	NOUN
cet-15373	2	96	,	,	PUNCT
cet-15373	2	97	we	we	PRON
cet-15373	2	98	present	present	VERB
cet-15373	2	99	the	the	DET
cet-15373	2	100	development	development	NOUN
cet-15373	2	101	of	of	ADP
cet-15373	2	102	a	a	DET
cet-15373	2	103	novel	novel	ADJ
cet-15373	2	104	electrochemical	electrochemical	ADJ
cet-15373	2	105	device	device	NOUN
cet-15373	2	106	designed	design	VERB
cet-15373	2	107	for	for	ADP
cet-15373	2	108	the	the	DET
cet-15373	2	109	nitrogen	nitrogen	NOUN
cet-15373	2	110	reduction	reduction	NOUN
cet-15373	2	111	reaction	reaction	NOUN
cet-15373	2	112	(	(	PUNCT
cet-15373	2	113	nrr	nrr	PROPN
cet-15373	2	114	)	)	PUNCT
cet-15373	2	115	process	process	NOUN
cet-15373	2	116	,	,	PUNCT
cet-15373	2	117	which	which	PRON
cet-15373	2	118	operates	operate	VERB
cet-15373	2	119	under	under	ADP
cet-15373	2	120	unconventional	unconventional	ADJ
cet-15373	2	121	conditions	condition	NOUN
cet-15373	2	122	.	.	PUNCT
cet-15373	3	1	this	this	DET
cet-15373	3	2	zero	zero	NUM
cet-15373	3	3	-	-	PUNCT
cet-15373	3	4	gap	gap	NOUN
cet-15373	3	5	flow	flow	NOUN
cet-15373	3	6	cell	cell	NOUN
cet-15373	3	7	works	work	VERB
cet-15373	3	8	without	without	ADP
cet-15373	3	9	a	a	DET
cet-15373	3	10	liquid	liquid	ADJ
cet-15373	3	11	electrolyte	electrolyte	NOUN
cet-15373	3	12	in	in	ADP
cet-15373	3	13	the	the	DET
cet-15373	3	14	cathodic	cathodic	NOUN
cet-15373	3	15	section	section	NOUN
cet-15373	3	16	and	and	CCONJ
cet-15373	3	17	incorporates	incorporate	VERB
cet-15373	3	18	novel	novel	ADJ
cet-15373	3	19	electrocatalysts	electrocatalyst	NOUN
cet-15373	3	20	integrated	integrate	VERB
cet-15373	3	21	into	into	ADP
cet-15373	3	22	gas	gas	NOUN
cet-15373	3	23	diffusion	diffusion	NOUN
cet-15373	3	24	electrodes	electrode	NOUN
cet-15373	3	25	(	(	PUNCT
cet-15373	3	26	gdes	gde	NOUN
cet-15373	3	27	)	)	PUNCT
cet-15373	3	28	.	.	PUNCT
cet-15373	4	1	specifically	specifically	ADV
cet-15373	4	2	,	,	PUNCT
cet-15373	4	3	the	the	DET
cet-15373	4	4	electrocatalysts	electrocatalyst	NOUN
cet-15373	4	5	are	be	AUX
cet-15373	4	6	based	base	VERB
cet-15373	4	7	on	on	ADP
cet-15373	4	8	ruthenium	ruthenium	NOUN
cet-15373	4	9	(	(	PUNCT
cet-15373	4	10	ru	ru	PROPN
cet-15373	4	11	)	)	PUNCT
cet-15373	4	12	,	,	PUNCT
cet-15373	4	13	deposited	deposit	VERB
cet-15373	4	14	on	on	ADP
cet-15373	4	15	alumina	alumina	NOUN
cet-15373	4	16	(	(	PUNCT
cet-15373	4	17	al2o3	al2o3	NOUN
cet-15373	4	18	)	)	PUNCT
cet-15373	4	19	or	or	CCONJ
cet-15373	4	20	carbon	carbon	NOUN
cet-15373	4	21	nanotubes	nanotube	NOUN
cet-15373	4	22	(	(	PUNCT
cet-15373	4	23	cnts	cnts	PROPN
cet-15373	4	24	)	)	PUNCT
cet-15373	4	25	.	.	PUNCT
cet-15373	5	1	a	a	DET
cet-15373	5	2	key	key	ADJ
cet-15373	5	3	objective	objective	NOUN
cet-15373	5	4	of	of	ADP
cet-15373	5	5	this	this	DET
cet-15373	5	6	study	study	NOUN
cet-15373	5	7	is	be	AUX
cet-15373	5	8	to	to	PART
cet-15373	5	9	evaluate	evaluate	VERB
cet-15373	5	10	the	the	DET
cet-15373	5	11	partial	partial	ADJ
cet-15373	5	12	or	or	CCONJ
cet-15373	5	13	total	total	ADJ
cet-15373	5	14	replacement	replacement	NOUN
cet-15373	5	15	of	of	ADP
cet-15373	5	16	ru	ru	PROPN
cet-15373	5	17	with	with	ADP
cet-15373	5	18	a	a	DET
cet-15373	5	19	more	more	ADV
cet-15373	5	20	abundant	abundant	ADJ
cet-15373	5	21	and	and	CCONJ
cet-15373	5	22	cost	cost	NOUN
cet-15373	5	23	-	-	PUNCT
cet-15373	5	24	effective	effective	ADJ
cet-15373	5	25	material	material	NOUN
cet-15373	5	26	,	,	PUNCT
cet-15373	5	27	such	such	ADJ
cet-15373	5	28	as	as	ADP
cet-15373	5	29	iron	iron	NOUN
cet-15373	5	30	(	(	PUNCT
cet-15373	5	31	fe	fe	NOUN
cet-15373	5	32	)	)	PUNCT
cet-15373	5	33	.	.	PUNCT
cet-15373	6	1	the	the	DET
cet-15373	6	2	productivity	productivity	NOUN
cet-15373	6	3	of	of	ADP
cet-15373	6	4	the	the	DET
cet-15373	6	5	produced	produce	VERB
cet-15373	6	6	nh3	nh3	NOUN
cet-15373	6	7	(	(	PUNCT
cet-15373	6	8	in	in	ADP
cet-15373	6	9	g	g	PROPN
cet-15373	6	10	mgcat	mgcat	PROPN
cet-15373	6	11	-1	-1	PUNCT
cet-15373	6	12	h-1	h-1	PROPN
cet-15373	6	13	)	)	PUNCT
cet-15373	6	14	and	and	CCONJ
cet-15373	6	15	the	the	DET
cet-15373	6	16	faradaic	faradaic	ADJ
cet-15373	6	17	efficiency	efficiency	NOUN
cet-15373	6	18	(	(	PUNCT
cet-15373	6	19	fe	fe	NOUN
cet-15373	6	20	)	)	PUNCT
cet-15373	6	21	are	be	AUX
cet-15373	6	22	provided	provide	VERB
cet-15373	6	23	and	and	CCONJ
cet-15373	6	24	discussed	discuss	VERB
cet-15373	6	25	.	.	PUNCT
cet-15373	7	1	another	another	DET
cet-15373	7	2	important	important	ADJ
cet-15373	7	3	aspect	aspect	NOUN
cet-15373	7	4	of	of	ADP
cet-15373	7	5	this	this	DET
cet-15373	7	6	work	work	NOUN
cet-15373	7	7	is	be	AUX
cet-15373	7	8	how	how	SCONJ
cet-15373	7	9	ammonia	ammonia	ADJ
cet-15373	7	10	contamination	contamination	NOUN
cet-15373	7	11	is	be	AUX
cet-15373	7	12	addressed	address	VERB
cet-15373	7	13	,	,	PUNCT
cet-15373	7	14	using	use	VERB
cet-15373	7	15	a	a	DET
cet-15373	7	16	cheaper	cheap	ADJ
cet-15373	7	17	but	but	CCONJ
cet-15373	7	18	still	still	ADV
cet-15373	7	19	rigorous	rigorous	ADJ
cet-15373	7	20	protocol	protocol	NOUN
cet-15373	7	21	than	than	ADP
cet-15373	7	22	the	the	DET
cet-15373	7	23	one	one	NOUN
cet-15373	7	24	reported	report	VERB
cet-15373	7	25	in	in	ADP
cet-15373	7	26	the	the	DET
cet-15373	7	27	literature	literature	NOUN
cet-15373	7	28	using	use	VERB
cet-15373	7	29	expensive	expensive	ADJ
cet-15373	7	30	labelled	label	VERB
cet-15373	7	31	nitrogen	nitrogen	NOUN
cet-15373	7	32	(	(	PUNCT
cet-15373	7	33	n15	n15	PROPN
cet-15373	7	34	)	)	PUNCT
cet-15373	7	35	.	.	PUNCT
cet-15373	8	1	results	result	NOUN
cet-15373	8	2	show	show	VERB
cet-15373	8	3	that	that	SCONJ
cet-15373	8	4	cell	cell	NOUN
cet-15373	8	5	design	design	NOUN
cet-15373	8	6	plays	play	VERB
cet-15373	8	7	a	a	DET
cet-15373	8	8	key	key	ADJ
cet-15373	8	9	role	role	NOUN
cet-15373	8	10	,	,	PUNCT
cet-15373	8	11	and	and	CCONJ
cet-15373	8	12	the	the	DET
cet-15373	8	13	partial	partial	ADJ
cet-15373	8	14	substitution	substitution	NOUN
cet-15373	8	15	of	of	ADP
cet-15373	8	16	an	an	DET
cet-15373	8	17	abundant	abundant	ADJ
cet-15373	8	18	material	material	NOUN
cet-15373	8	19	(	(	PUNCT
cet-15373	8	20	fe	fe	NOUN
cet-15373	8	21	)	)	PUNCT
cet-15373	8	22	brings	bring	VERB
cet-15373	8	23	benefits	benefit	NOUN
cet-15373	8	24	,	,	PUNCT
cet-15373	8	25	compared	compare	VERB
cet-15373	8	26	with	with	ADP
cet-15373	8	27	the	the	DET
cet-15373	8	28	common	common	ADJ
cet-15373	8	29	noble	noble	ADJ
cet-15373	8	30	metals	metal	NOUN
cet-15373	8	31	reported	report	VERB
cet-15373	8	32	in	in	ADP
cet-15373	8	33	the	the	DET
cet-15373	8	34	literature	literature	NOUN
cet-15373	8	35	.	.	PUNCT
cet-15373	9	1	furthermore	furthermore	ADV
cet-15373	9	2	,	,	PUNCT
cet-15373	9	3	this	this	DET
cet-15373	9	4	contribution	contribution	NOUN
cet-15373	9	5	identifies	identify	VERB
cet-15373	9	6	the	the	DET
cet-15373	9	7	critical	critical	ADJ
cet-15373	9	8	aspects	aspect	NOUN
cet-15373	9	9	to	to	PART
cet-15373	9	10	be	be	AUX
cet-15373	9	11	addressed	address	VERB
cet-15373	9	12	,	,	PUNCT
cet-15373	9	13	emphasizing	emphasize	VERB
cet-15373	9	14	the	the	DET
cet-15373	9	15	need	need	NOUN
cet-15373	9	16	for	for	SCONJ
cet-15373	9	17	breakthroughs	breakthrough	NOUN
cet-15373	9	18	to	to	PART
cet-15373	9	19	enhance	enhance	VERB
cet-15373	9	20	performance	performance	NOUN
cet-15373	9	21	in	in	ADP
cet-15373	9	22	this	this	DET
cet-15373	9	23	highly	highly	ADV
cet-15373	9	24	challenging	challenging	ADJ
cet-15373	9	25	process	process	NOUN
cet-15373	9	26	.	.	PUNCT
cet-15373	10	1	1	1	X
cet-15373	10	2	.	.	X
cet-15373	10	3	introduction	introduction	NOUN
cet-15373	10	4	nitrogen	nitrogen	NOUN
cet-15373	10	5	reduction	reduction	NOUN
cet-15373	10	6	reaction	reaction	NOUN
cet-15373	10	7	(	(	PUNCT
cet-15373	10	8	nrr	nrr	PROPN
cet-15373	10	9	)	)	PUNCT
cet-15373	10	10	is	be	AUX
cet-15373	10	11	a	a	DET
cet-15373	10	12	today	today	NOUN
cet-15373	10	13	’s	’s	PART
cet-15373	10	14	challenge	challenge	NOUN
cet-15373	10	15	to	to	PART
cet-15373	10	16	meet	meet	VERB
cet-15373	10	17	the	the	DET
cet-15373	10	18	growing	grow	VERB
cet-15373	10	19	demand	demand	NOUN
cet-15373	10	20	for	for	ADP
cet-15373	10	21	ammonia	ammonia	NOUN
cet-15373	10	22	.	.	PUNCT
cet-15373	11	1	the	the	DET
cet-15373	11	2	haber	haber	PROPN
cet-15373	11	3	bosh	bosh	PROPN
cet-15373	11	4	process	process	NOUN
cet-15373	11	5	is	be	AUX
cet-15373	11	6	the	the	DET
cet-15373	11	7	only	only	ADJ
cet-15373	11	8	current	current	ADJ
cet-15373	11	9	industrial	industrial	ADJ
cet-15373	11	10	-	-	PUNCT
cet-15373	11	11	scale	scale	NOUN
cet-15373	11	12	ammonia	ammonia	NOUN
cet-15373	11	13	production	production	NOUN
cet-15373	11	14	system	system	NOUN
cet-15373	11	15	,	,	PUNCT
cet-15373	11	16	operating	operate	VERB
cet-15373	11	17	at	at	ADP
cet-15373	11	18	high	high	ADJ
cet-15373	11	19	pressures	pressure	NOUN
cet-15373	11	20	and	and	CCONJ
cet-15373	11	21	temperatures	temperature	NOUN
cet-15373	11	22	(	(	PUNCT
cet-15373	11	23	20−40	20−40	PROPN
cet-15373	11	24	mpa	mpa	PROPN
cet-15373	11	25	,	,	PUNCT
cet-15373	11	26	400−600	400−600	PROPN
cet-15373	11	27	°	°	NOUN
cet-15373	11	28	c	c	NOUN
cet-15373	11	29	)	)	PUNCT
cet-15373	11	30	.	.	PUNCT
cet-15373	12	1	this	this	DET
cet-15373	12	2	process	process	NOUN
cet-15373	12	3	is	be	AUX
cet-15373	12	4	highly	highly	ADV
cet-15373	12	5	energy	energy	NOUN
cet-15373	12	6	intensive	intensive	ADJ
cet-15373	12	7	as	as	SCONJ
cet-15373	12	8	it	it	PRON
cet-15373	12	9	consumes	consume	VERB
cet-15373	12	10	1	1	NUM
cet-15373	12	11	%	%	NOUN
cet-15373	12	12	of	of	ADP
cet-15373	12	13	global	global	ADJ
cet-15373	12	14	energy	energy	NOUN
cet-15373	12	15	production	production	NOUN
cet-15373	12	16	(	(	PUNCT
cet-15373	12	17	schrock	schrock	NOUN
cet-15373	12	18	,	,	PUNCT
cet-15373	12	19	2006	2006	NUM
cet-15373	12	20	)	)	PUNCT
cet-15373	12	21	and	and	CCONJ
cet-15373	12	22	emits	emit	VERB
cet-15373	12	23	millions	million	NOUN
cet-15373	12	24	of	of	ADP
cet-15373	12	25	tons	ton	NOUN
cet-15373	12	26	of	of	ADP
cet-15373	12	27	co2	co2	NOUN
cet-15373	12	28	into	into	ADP
cet-15373	12	29	the	the	DET
cet-15373	12	30	atmosphere	atmosphere	NOUN
cet-15373	12	31	(	(	PUNCT
cet-15373	12	32	rafiqul	rafiqul	VERB
cet-15373	12	33	et	et	PROPN
cet-15373	12	34	al	al	PROPN
cet-15373	12	35	.	.	PROPN
cet-15373	12	36	,	,	PUNCT
cet-15373	12	37	2005	2005	NUM
cet-15373	12	38	)	)	PUNCT
cet-15373	12	39	despite	despite	SCONJ
cet-15373	12	40	the	the	DET
cet-15373	12	41	haber	haber	PROPN
cet-15373	12	42	bosh	bosh	PROPN
cet-15373	12	43	reactor	reactor	NOUN
cet-15373	12	44	and	and	CCONJ
cet-15373	12	45	the	the	DET
cet-15373	12	46	process	process	NOUN
cet-15373	12	47	itself	itself	PRON
cet-15373	12	48	being	be	AUX
cet-15373	12	49	highly	highly	ADV
cet-15373	12	50	engineered	engineer	VERB
cet-15373	12	51	and	and	CCONJ
cet-15373	12	52	optimized	optimize	VERB
cet-15373	12	53	(	(	PUNCT
cet-15373	12	54	rowenhorst	rowenhorst	ADV
cet-15373	12	55	et	et	PROPN
cet-15373	12	56	al	al	PROPN
cet-15373	12	57	.	.	PROPN
cet-15373	12	58	,	,	PUNCT
cet-15373	12	59	2021	2021	NUM
cet-15373	12	60	)	)	PUNCT
cet-15373	12	61	.	.	PUNCT
cet-15373	13	1	for	for	ADP
cet-15373	13	2	this	this	DET
cet-15373	13	3	reason	reason	NOUN
cet-15373	13	4	,	,	PUNCT
cet-15373	13	5	the	the	DET
cet-15373	13	6	challenge	challenge	NOUN
cet-15373	13	7	is	be	AUX
cet-15373	13	8	to	to	PART
cet-15373	13	9	find	find	VERB
cet-15373	13	10	an	an	DET
cet-15373	13	11	emerging	emerge	VERB
cet-15373	13	12	technology	technology	NOUN
cet-15373	13	13	that	that	PRON
cet-15373	13	14	allows	allow	VERB
cet-15373	13	15	ammonia	ammonia	NOUN
cet-15373	13	16	to	to	PART
cet-15373	13	17	be	be	AUX
cet-15373	13	18	obtained	obtain	VERB
cet-15373	13	19	in	in	ADP
cet-15373	13	20	a	a	DET
cet-15373	13	21	more	more	ADV
cet-15373	13	22	sustainable	sustainable	ADJ
cet-15373	13	23	and	and	CCONJ
cet-15373	13	24	decentralized	decentralized	ADJ
cet-15373	13	25	way	way	NOUN
cet-15373	13	26	.	.	PUNCT
cet-15373	14	1	among	among	ADP
cet-15373	14	2	the	the	DET
cet-15373	14	3	various	various	ADJ
cet-15373	14	4	innovative	innovative	ADJ
cet-15373	14	5	approaches	approach	NOUN
cet-15373	14	6	to	to	ADP
cet-15373	14	7	ammonia	ammonia	NOUN
cet-15373	14	8	production	production	NOUN
cet-15373	14	9	,	,	PUNCT
cet-15373	14	10	there	there	PRON
cet-15373	14	11	are	be	VERB
cet-15373	14	12	electrocatalytic	electrocatalytic	ADJ
cet-15373	14	13	processes	process	NOUN
cet-15373	14	14	that	that	PRON
cet-15373	14	15	exploit	exploit	VERB
cet-15373	14	16	electrical	electrical	ADJ
cet-15373	14	17	energy	energy	NOUN
cet-15373	14	18	to	to	PART
cet-15373	14	19	drive	drive	VERB
cet-15373	14	20	the	the	DET
cet-15373	14	21	reactions	reaction	NOUN
cet-15373	14	22	and	and	CCONJ
cet-15373	14	23	can	can	AUX
cet-15373	14	24	be	be	AUX
cet-15373	14	25	perfectly	perfectly	ADV
cet-15373	14	26	integrated	integrate	VERB
cet-15373	14	27	with	with	ADP
cet-15373	14	28	the	the	DET
cet-15373	14	29	current	current	ADJ
cet-15373	14	30	energy	energy	NOUN
cet-15373	14	31	transition	transition	NOUN
cet-15373	14	32	,	,	PUNCT
cet-15373	14	33	although	although	SCONJ
cet-15373	14	34	the	the	DET
cet-15373	14	35	electrocatalysis	electrocatalysis	NOUN
cet-15373	14	36	remains	remain	VERB
cet-15373	14	37	far	far	ADV
cet-15373	14	38	from	from	ADP
cet-15373	14	39	industrial	industrial	ADJ
cet-15373	14	40	standards	standard	NOUN
cet-15373	14	41	(	(	PUNCT
cet-15373	14	42	tavella	tavella	NOUN
cet-15373	14	43	et	et	PROPN
cet-15373	14	44	al	al	PROPN
cet-15373	14	45	.	.	PROPN
cet-15373	14	46	,	,	PUNCT
cet-15373	14	47	2022	2022	NUM
cet-15373	14	48	)	)	PUNCT
cet-15373	14	49	.	.	PUNCT
cet-15373	15	1	the	the	DET
cet-15373	15	2	main	main	ADJ
cet-15373	15	3	problems	problem	NOUN
cet-15373	15	4	of	of	ADP
cet-15373	15	5	electrochemical	electrochemical	ADJ
cet-15373	15	6	nrr	nrr	PROPN
cet-15373	15	7	are	be	AUX
cet-15373	15	8	the	the	DET
cet-15373	15	9	low	low	ADJ
cet-15373	15	10	solubility	solubility	NOUN
cet-15373	15	11	of	of	ADP
cet-15373	15	12	nitrogen	nitrogen	NOUN
cet-15373	15	13	in	in	ADP
cet-15373	15	14	the	the	DET
cet-15373	15	15	aqueous	aqueous	ADJ
cet-15373	15	16	medium	medium	NOUN
cet-15373	15	17	and	and	CCONJ
cet-15373	15	18	the	the	DET
cet-15373	15	19	concurrent	concurrent	ADJ
cet-15373	15	20	hydrogen	hydrogen	NOUN
cet-15373	15	21	evolution	evolution	NOUN
cet-15373	15	22	reaction	reaction	NOUN
cet-15373	15	23	(	(	PUNCT
cet-15373	15	24	her	her	NOUN
cet-15373	15	25	)	)	PUNCT
cet-15373	15	26	.	.	PUNCT
cet-15373	16	1	reactors	reactor	NOUN
cet-15373	16	2	that	that	PRON
cet-15373	16	3	operate	operate	VERB
cet-15373	16	4	without	without	ADP
cet-15373	16	5	electrolyte	electrolyte	NOUN
cet-15373	16	6	have	have	AUX
cet-15373	16	7	recently	recently	ADV
cet-15373	16	8	attracted	attract	VERB
cet-15373	16	9	attention	attention	NOUN
cet-15373	16	10	.	.	PUNCT
cet-15373	17	1	this	this	DET
cet-15373	17	2	work	work	NOUN
cet-15373	17	3	aims	aim	VERB
cet-15373	17	4	to	to	PART
cet-15373	17	5	compare	compare	VERB
cet-15373	17	6	the	the	DET
cet-15373	17	7	performance	performance	NOUN
cet-15373	17	8	of	of	ADP
cet-15373	17	9	noble	noble	ADJ
cet-15373	17	10	and	and	CCONJ
cet-15373	17	11	non	non	ADJ
cet-15373	17	12	-	-	ADJ
cet-15373	17	13	noble	noble	ADJ
cet-15373	17	14	metals	metal	NOUN
cet-15373	17	15	when	when	SCONJ
cet-15373	17	16	processed	process	VERB
cet-15373	17	17	in	in	ADP
cet-15373	17	18	these	these	DET
cet-15373	17	19	innovative	innovative	ADJ
cet-15373	17	20	gas	gas	NOUN
cet-15373	17	21	-	-	PUNCT
cet-15373	17	22	phase	phase	NOUN
cet-15373	17	23	electrochemical	electrochemical	ADJ
cet-15373	17	24	devices	device	NOUN
cet-15373	17	25	.	.	PUNCT
cet-15373	18	1	ruthenium	ruthenium	NOUN
cet-15373	18	2	(	(	PUNCT
cet-15373	18	3	ru	ru	PROPN
cet-15373	18	4	)	)	PUNCT
cet-15373	18	5	and	and	CCONJ
cet-15373	18	6	iron	iron	NOUN
cet-15373	18	7	(	(	PUNCT
cet-15373	18	8	fe	fe	NOUN
cet-15373	18	9	)	)	PUNCT
cet-15373	18	10	are	be	AUX
cet-15373	18	11	found	find	VERB
cet-15373	18	12	at	at	ADP
cet-15373	18	13	the	the	DET
cet-15373	18	14	top	top	NOUN
cet-15373	18	15	of	of	ADP
cet-15373	18	16	the	the	DET
cet-15373	18	17	volcano	volcano	NOUN
cet-15373	18	18	plot	plot	NOUN
cet-15373	18	19	(	(	PUNCT
cet-15373	18	20	guo	guo	PROPN
cet-15373	18	21	et	et	PROPN
cet-15373	18	22	al	al	PROPN
cet-15373	18	23	.	.	PROPN
cet-15373	18	24	,	,	PUNCT
cet-15373	18	25	2019	2019	NUM
cet-15373	18	26	)	)	PUNCT
cet-15373	18	27	and	and	CCONJ
cet-15373	18	28	therefore	therefore	ADV
cet-15373	18	29	have	have	VERB
cet-15373	18	30	a	a	DET
cet-15373	18	31	greater	great	ADJ
cet-15373	18	32	affinity	affinity	NOUN
cet-15373	18	33	for	for	ADP
cet-15373	18	34	the	the	DET
cet-15373	18	35	dinitrogen	dinitrogen	NOUN
cet-15373	18	36	molecule	molecule	NOUN
cet-15373	18	37	,	,	PUNCT
cet-15373	18	38	whose	whose	DET
cet-15373	18	39	triple	triple	ADJ
cet-15373	18	40	bond	bond	NOUN
cet-15373	18	41	(	(	PUNCT
cet-15373	18	42	945	945	NUM
cet-15373	18	43	kj	kj	PROPN
cet-15373	18	44	mol-1	mol-1	NOUN
cet-15373	18	45	)	)	PUNCT
cet-15373	18	46	is	be	AUX
cet-15373	18	47	difficult	difficult	ADJ
cet-15373	18	48	to	to	PART
cet-15373	18	49	break	break	VERB
cet-15373	18	50	(	(	PUNCT
cet-15373	18	51	li	li	PROPN
cet-15373	18	52	et	et	PROPN
cet-15373	18	53	al	al	PROPN
cet-15373	18	54	.	.	PROPN
cet-15373	18	55	,	,	PUNCT
cet-15373	18	56	2022	2022	NUM
cet-15373	18	57	)	)	PUNCT
cet-15373	18	58	.	.	PUNCT
cet-15373	19	1	in	in	ADP
cet-15373	19	2	the	the	DET
cet-15373	19	3	literature	literature	NOUN
cet-15373	19	4	,	,	PUNCT
cet-15373	19	5	many	many	ADJ
cet-15373	19	6	works	work	VERB
cet-15373	19	7	use	use	VERB
cet-15373	19	8	cnts	cnt	NOUN
cet-15373	19	9	as	as	ADP
cet-15373	19	10	conductive	conductive	ADJ
cet-15373	19	11	supports	support	NOUN
cet-15373	19	12	specially	specially	ADV
cet-15373	19	13	doped	dope	VERB
cet-15373	19	14	with	with	ADP
cet-15373	19	15	nanoparticles	nanoparticle	NOUN
cet-15373	19	16	(	(	PUNCT
cet-15373	19	17	chen	chen	PROPN
cet-15373	19	18	et	et	PROPN
cet-15373	19	19	al	al	PROPN
cet-15373	19	20	.	.	PROPN
cet-15373	19	21	,	,	PUNCT
cet-15373	19	22	2017	2017	NUM
cet-15373	19	23	)	)	PUNCT
cet-15373	19	24	,	,	PUNCT
cet-15373	19	25	such	such	ADJ
cet-15373	19	26	as	as	ADP
cet-15373	19	27	fe2o3	fe2o3	PROPN
cet-15373	19	28	or	or	CCONJ
cet-15373	19	29	ru	ru	NOUN
cet-15373	19	30	,	,	PUNCT
cet-15373	19	31	while	while	SCONJ
cet-15373	19	32	metal	metal	NOUN
cet-15373	19	33	doped	dope	VERB
cet-15373	19	34	-alumina	-alumina	PROPN
cet-15373	19	35	has	have	AUX
cet-15373	19	36	been	be	AUX
cet-15373	19	37	mainly	mainly	ADV
cet-15373	19	38	reported	report	VERB
cet-15373	19	39	for	for	ADP
cet-15373	19	40	thermal	thermal	ADJ
cet-15373	19	41	catalysis	catalysis	NOUN
cet-15373	19	42	and	and	CCONJ
cet-15373	19	43	plasma	plasma	NOUN
cet-15373	19	44	catalysis	catalysis	NOUN
cet-15373	19	45	,	,	PUNCT
cet-15373	19	46	but	but	CCONJ
cet-15373	19	47	less	less	ADJ
cet-15373	19	48	for	for	ADP
cet-15373	19	49	electrocatalysis	electrocatalysis	NOUN
cet-15373	19	50	.	.	PUNCT
cet-15373	20	1	numerous	numerous	ADJ
cet-15373	20	2	studies	study	NOUN
cet-15373	20	3	highlight	highlight	VERB
cet-15373	20	4	how	how	SCONJ
cet-15373	20	5	the	the	DET
cet-15373	20	6	analysis	analysis	NOUN
cet-15373	20	7	protocol	protocol	NOUN
cet-15373	20	8	is	be	AUX
cet-15373	20	9	important	important	ADJ
cet-15373	20	10	to	to	PART
cet-15373	20	11	avoid	avoid	VERB
cet-15373	20	12	false	false	ADJ
cet-15373	20	13	positives	positive	NOUN
cet-15373	20	14	in	in	ADP
cet-15373	20	15	the	the	DET
cet-15373	20	16	detection	detection	NOUN
cet-15373	20	17	of	of	ADP
cet-15373	20	18	ammonium	ammonium	NOUN
cet-15373	20	19	ion	ion	NOUN
cet-15373	20	20	in	in	ADP
cet-15373	20	21	relation	relation	NOUN
cet-15373	20	22	to	to	ADP
cet-15373	20	23	the	the	DET
cet-15373	20	24	low	low	ADJ
cet-15373	20	25	productivity	productivity	NOUN
cet-15373	20	26	in	in	ADP
cet-15373	20	27	water	water	NOUN
cet-15373	20	28	and	and	CCONJ
cet-15373	20	29	the	the	DET
cet-15373	20	30	numerous	numerous	ADJ
cet-15373	20	31	sources	source	NOUN
cet-15373	20	32	of	of	ADP
cet-15373	20	33	contamination	contamination	NOUN
cet-15373	20	34	.	.	PUNCT
cet-15373	21	1	for	for	ADP
cet-15373	21	2	this	this	DET
cet-15373	21	3	reason	reason	NOUN
cet-15373	21	4	,	,	PUNCT
cet-15373	21	5	the	the	DET
cet-15373	21	6	most	most	ADV
cet-15373	21	7	rigorous	rigorous	ADJ
cet-15373	21	8	protocols	protocol	NOUN
cet-15373	21	9	foresee	foresee	VERB
cet-15373	21	10	high	high	ADJ
cet-15373	21	11	analysis	analysis	NOUN
cet-15373	21	12	costs	cost	NOUN
cet-15373	21	13	for	for	ADP
cet-15373	21	14	the	the	DET
cet-15373	21	15	use	use	NOUN
cet-15373	21	16	of	of	ADP
cet-15373	21	17	labelled	label	VERB
cet-15373	21	18	nitrogen	nitrogen	NOUN
cet-15373	21	19	,	,	PUNCT
cet-15373	21	20	but	but	CCONJ
cet-15373	21	21	this	this	PRON
cet-15373	21	22	is	be	AUX
cet-15373	21	23	733	733	NUM
cet-15373	21	24	unsustainable	unsustainable	ADJ
cet-15373	21	25	for	for	ADP
cet-15373	21	26	research	research	NOUN
cet-15373	21	27	purposes	purpose	NOUN
cet-15373	21	28	.	.	PUNCT
cet-15373	22	1	a	a	DET
cet-15373	22	2	new	new	ADJ
cet-15373	22	3	protocol	protocol	NOUN
cet-15373	22	4	is	be	AUX
cet-15373	22	5	also	also	ADV
cet-15373	22	6	discussed	discuss	VERB
cet-15373	22	7	,	,	PUNCT
cet-15373	22	8	offering	offer	VERB
cet-15373	22	9	improved	improve	VERB
cet-15373	22	10	cost	cost	NOUN
cet-15373	22	11	-	-	PUNCT
cet-15373	22	12	effectiveness	effectiveness	NOUN
cet-15373	22	13	and	and	CCONJ
cet-15373	22	14	ease	ease	NOUN
cet-15373	22	15	of	of	ADP
cet-15373	22	16	use	use	NOUN
cet-15373	22	17	while	while	SCONJ
cet-15373	22	18	maintaining	maintain	VERB
cet-15373	22	19	a	a	DET
cet-15373	22	20	high	high	ADJ
cet-15373	22	21	degree	degree	NOUN
cet-15373	22	22	of	of	ADP
cet-15373	22	23	rigor	rigor	NOUN
cet-15373	22	24	.	.	PUNCT
cet-15373	23	1	to	to	PART
cet-15373	23	2	achieve	achieve	VERB
cet-15373	23	3	gas	gas	NOUN
cet-15373	23	4	-	-	PUNCT
cet-15373	23	5	phase	phase	NOUN
cet-15373	23	6	conditions	condition	NOUN
cet-15373	23	7	(	(	PUNCT
cet-15373	23	8	also	also	ADV
cet-15373	23	9	known	know	VERB
cet-15373	23	10	as	as	ADP
cet-15373	23	11	electrolyte	electrolyte	NOUN
cet-15373	23	12	-	-	PUNCT
cet-15373	23	13	less	less	ADJ
cet-15373	23	14	or	or	CCONJ
cet-15373	23	15	zero	zero	NUM
cet-15373	23	16	-	-	PUNCT
cet-15373	23	17	gap	gap	NOUN
cet-15373	23	18	conditions	condition	NOUN
cet-15373	23	19	)	)	PUNCT
cet-15373	23	20	,	,	PUNCT
cet-15373	23	21	a	a	DET
cet-15373	23	22	membrane	membrane	NOUN
cet-15373	23	23	electrode	electrode	NOUN
cet-15373	23	24	assembly	assembly	NOUN
cet-15373	23	25	(	(	PUNCT
cet-15373	23	26	mea	mea	NOUN
cet-15373	23	27	)	)	PUNCT
cet-15373	23	28	can	can	AUX
cet-15373	23	29	be	be	AUX
cet-15373	23	30	used	use	VERB
cet-15373	23	31	,	,	PUNCT
cet-15373	23	32	similar	similar	ADJ
cet-15373	23	33	to	to	ADP
cet-15373	23	34	fuel	fuel	NOUN
cet-15373	23	35	cell	cell	NOUN
cet-15373	23	36	technology	technology	NOUN
cet-15373	23	37	(	(	PUNCT
cet-15373	23	38	ampelli	ampelli	ADV
cet-15373	23	39	,	,	PUNCT
cet-15373	23	40	2020	2020	NUM
cet-15373	23	41	)	)	PUNCT
cet-15373	23	42	.	.	PUNCT
cet-15373	24	1	the	the	DET
cet-15373	24	2	mea	mea	NOUN
cet-15373	24	3	involves	involve	VERB
cet-15373	24	4	coupling	couple	VERB
cet-15373	24	5	the	the	DET
cet-15373	24	6	catalyst	catalyst	NOUN
cet-15373	24	7	with	with	ADP
cet-15373	24	8	an	an	DET
cet-15373	24	9	ion	ion	NOUN
cet-15373	24	10	-	-	PUNCT
cet-15373	24	11	exchange	exchange	NOUN
cet-15373	24	12	membrane	membrane	NOUN
cet-15373	24	13	to	to	PART
cet-15373	24	14	create	create	VERB
cet-15373	24	15	a	a	DET
cet-15373	24	16	solid	solid	ADJ
cet-15373	24	17	electrolyte	electrolyte	NOUN
cet-15373	24	18	,	,	PUNCT
cet-15373	24	19	replacing	replace	VERB
cet-15373	24	20	the	the	DET
cet-15373	24	21	liquid	liquid	ADJ
cet-15373	24	22	cathodic	cathodic	NOUN
cet-15373	24	23	compartment	compartment	NOUN
cet-15373	24	24	(	(	PUNCT
cet-15373	24	25	park	park	NOUN
cet-15373	24	26	et	et	NOUN
cet-15373	24	27	al	al	PROPN
cet-15373	24	28	.	.	PROPN
cet-15373	24	29	,	,	PUNCT
cet-15373	24	30	2023	2023	NUM
cet-15373	24	31	)	)	PUNCT
cet-15373	24	32	.	.	PUNCT
cet-15373	25	1	factors	factor	NOUN
cet-15373	25	2	such	such	ADJ
cet-15373	25	3	as	as	ADP
cet-15373	25	4	i	i	PROPN
cet-15373	25	5	)	)	PUNCT
cet-15373	25	6	increased	increase	VERB
cet-15373	25	7	n2	n2	ADJ
cet-15373	25	8	concentration	concentration	NOUN
cet-15373	25	9	on	on	ADP
cet-15373	25	10	the	the	DET
cet-15373	25	11	electrode	electrode	NOUN
cet-15373	25	12	surface	surface	NOUN
cet-15373	25	13	and	and	CCONJ
cet-15373	25	14	ii	ii	NOUN
cet-15373	25	15	)	)	PUNCT
cet-15373	25	16	regulated	regulate	VERB
cet-15373	25	17	proton	proton	NOUN
cet-15373	25	18	mobility	mobility	NOUN
cet-15373	25	19	in	in	ADP
cet-15373	25	20	the	the	DET
cet-15373	25	21	catalyst	catalyst	NOUN
cet-15373	25	22	/	/	SYM
cet-15373	25	23	membrane	membrane	NOUN
cet-15373	25	24	interface	interface	NOUN
cet-15373	25	25	enable	enable	VERB
cet-15373	25	26	catalytic	catalytic	ADJ
cet-15373	25	27	surface	surface	NOUN
cet-15373	25	28	reactions	reaction	NOUN
cet-15373	25	29	to	to	PART
cet-15373	25	30	form	form	VERB
cet-15373	25	31	ammonia	ammonia	NOUN
cet-15373	25	32	while	while	SCONJ
cet-15373	25	33	limiting	limit	VERB
cet-15373	25	34	hydrogen	hydrogen	NOUN
cet-15373	25	35	(	(	PUNCT
cet-15373	25	36	h2	h2	NOUN
cet-15373	25	37	)	)	PUNCT
cet-15373	25	38	generation	generation	NOUN
cet-15373	25	39	.	.	PUNCT
cet-15373	26	1	engineering	engineer	VERB
cet-15373	26	2	the	the	DET
cet-15373	26	3	electrochemical	electrochemical	ADJ
cet-15373	26	4	reactor	reactor	NOUN
cet-15373	26	5	and	and	CCONJ
cet-15373	26	6	related	related	ADJ
cet-15373	26	7	electrodes	electrode	NOUN
cet-15373	26	8	can	can	AUX
cet-15373	26	9	lead	lead	VERB
cet-15373	26	10	to	to	ADP
cet-15373	26	11	drastic	drastic	ADJ
cet-15373	26	12	changes	change	NOUN
cet-15373	26	13	in	in	ADP
cet-15373	26	14	selectivity	selectivity	NOUN
cet-15373	26	15	and	and	CCONJ
cet-15373	26	16	a	a	DET
cet-15373	26	17	decrease	decrease	NOUN
cet-15373	26	18	of	of	ADP
cet-15373	26	19	h2	h2	NOUN
cet-15373	26	20	production	production	NOUN
cet-15373	26	21	as	as	ADP
cet-15373	26	22	a	a	DET
cet-15373	26	23	side	side	NOUN
cet-15373	26	24	reaction	reaction	NOUN
cet-15373	26	25	.	.	PUNCT
cet-15373	27	1	specifically	specifically	ADV
cet-15373	27	2	,	,	PUNCT
cet-15373	27	3	this	this	PRON
cet-15373	27	4	depends	depend	VERB
cet-15373	27	5	on	on	ADP
cet-15373	27	6	mass	mass	NOUN
cet-15373	27	7	and	and	CCONJ
cet-15373	27	8	charge	charge	NOUN
cet-15373	27	9	transfer	transfer	NOUN
cet-15373	27	10	phenomena	phenomenon	NOUN
cet-15373	27	11	at	at	ADP
cet-15373	27	12	the	the	DET
cet-15373	27	13	electrode	electrode	NOUN
cet-15373	27	14	interface	interface	NOUN
cet-15373	27	15	.	.	PUNCT
cet-15373	28	1	in	in	ADP
cet-15373	28	2	this	this	DET
cet-15373	28	3	view	view	NOUN
cet-15373	28	4	,	,	PUNCT
cet-15373	28	5	the	the	DET
cet-15373	28	6	performance	performance	NOUN
cet-15373	28	7	of	of	ADP
cet-15373	28	8	different	different	ADJ
cet-15373	28	9	catalysts	catalyst	NOUN
cet-15373	28	10	doped	dope	VERB
cet-15373	28	11	with	with	ADP
cet-15373	28	12	noble	noble	ADJ
cet-15373	28	13	metals	metal	NOUN
cet-15373	28	14	are	be	AUX
cet-15373	28	15	compared	compare	VERB
cet-15373	28	16	and	and	CCONJ
cet-15373	28	17	the	the	DET
cet-15373	28	18	total	total	ADJ
cet-15373	28	19	or	or	CCONJ
cet-15373	28	20	partial	partial	ADJ
cet-15373	28	21	replacement	replacement	NOUN
cet-15373	28	22	with	with	ADP
cet-15373	28	23	more	more	ADV
cet-15373	28	24	abundant	abundant	ADJ
cet-15373	28	25	metals	metal	NOUN
cet-15373	28	26	will	will	AUX
cet-15373	28	27	be	be	AUX
cet-15373	28	28	compared	compare	VERB
cet-15373	28	29	.	.	PUNCT
cet-15373	29	1	this	this	DET
cet-15373	29	2	configuration	configuration	NOUN
cet-15373	29	3	,	,	PUNCT
cet-15373	29	4	in	in	ADP
cet-15373	29	5	addition	addition	NOUN
cet-15373	29	6	to	to	ADP
cet-15373	29	7	allowing	allow	VERB
cet-15373	29	8	a	a	DET
cet-15373	29	9	continuous	continuous	ADJ
cet-15373	29	10	supply	supply	NOUN
cet-15373	29	11	of	of	ADP
cet-15373	29	12	nitrogen	nitrogen	NOUN
cet-15373	29	13	species	specie	NOUN
cet-15373	29	14	onto	onto	ADP
cet-15373	29	15	the	the	DET
cet-15373	29	16	electrocatalytic	electrocatalytic	ADJ
cet-15373	29	17	surface	surface	NOUN
cet-15373	29	18	,	,	PUNCT
cet-15373	29	19	has	have	VERB
cet-15373	29	20	the	the	DET
cet-15373	29	21	advantage	advantage	NOUN
cet-15373	29	22	of	of	ADP
cet-15373	29	23	i	i	PROPN
cet-15373	29	24	)	)	PUNCT
cet-15373	29	25	allowing	allow	VERB
cet-15373	29	26	to	to	PART
cet-15373	29	27	design	design	VERB
cet-15373	29	28	compact	compact	ADJ
cet-15373	29	29	and	and	CCONJ
cet-15373	29	30	scalable	scalable	ADJ
cet-15373	29	31	systems	system	NOUN
cet-15373	29	32	to	to	ADP
cet-15373	29	33	an	an	DET
cet-15373	29	34	industrial	industrial	ADJ
cet-15373	29	35	level	level	NOUN
cet-15373	29	36	;	;	PUNCT
cet-15373	29	37	ii	ii	X
cet-15373	29	38	)	)	PUNCT
cet-15373	29	39	limiting	limit	VERB
cet-15373	29	40	the	the	DET
cet-15373	29	41	diffusion	diffusion	NOUN
cet-15373	29	42	processes	process	NOUN
cet-15373	29	43	present	present	ADJ
cet-15373	29	44	in	in	ADP
cet-15373	29	45	the	the	DET
cet-15373	29	46	liquid	liquid	ADJ
cet-15373	29	47	phase	phase	NOUN
cet-15373	29	48	and	and	CCONJ
cet-15373	29	49	iii	iii	NOUN
cet-15373	29	50	)	)	PUNCT
cet-15373	29	51	easy	easy	ADJ
cet-15373	29	52	recovery	recovery	NOUN
cet-15373	29	53	of	of	ADP
cet-15373	29	54	the	the	DET
cet-15373	29	55	liquid	liquid	ADJ
cet-15373	29	56	products	product	NOUN
cet-15373	29	57	.	.	PUNCT
cet-15373	30	1	2	2	X
cet-15373	30	2	.	.	X
cet-15373	30	3	experimental	experimental	ADJ
cet-15373	30	4	2.1	2.1	NUM
cet-15373	30	5	al2o3	al2o3	NOUN
cet-15373	30	6	-	-	PUNCT
cet-15373	30	7	based	base	VERB
cet-15373	30	8	catalysts	catalyst	NOUN
cet-15373	30	9	preparation	preparation	NOUN
cet-15373	30	10	blank	blank	ADP
cet-15373	30	11	-alumina	-alumina	PROPN
cet-15373	30	12	pellets	pellet	NOUN
cet-15373	30	13	(	(	PUNCT
cet-15373	30	14	mateck	mateck	NOUN
cet-15373	30	15	)	)	PUNCT
cet-15373	30	16	with	with	ADP
cet-15373	30	17	a	a	DET
cet-15373	30	18	surface	surface	NOUN
cet-15373	30	19	area	area	NOUN
cet-15373	30	20	of	of	ADP
cet-15373	30	21	0.18	0.18	NUM
cet-15373	30	22	m2	m2	PROPN
cet-15373	30	23	g-1	g-1	PROPN
cet-15373	30	24	were	be	AUX
cet-15373	30	25	purchased	purchase	VERB
cet-15373	30	26	,	,	PUNCT
cet-15373	30	27	smashed	smash	VERB
cet-15373	30	28	,	,	PUNCT
cet-15373	30	29	and	and	CCONJ
cet-15373	30	30	separated	separate	VERB
cet-15373	30	31	by	by	ADP
cet-15373	30	32	mechanical	mechanical	ADJ
cet-15373	30	33	milling	milling	NOUN
cet-15373	30	34	and	and	CCONJ
cet-15373	30	35	sieving	sieving	NOUN
cet-15373	30	36	in	in	ADP
cet-15373	30	37	the	the	DET
cet-15373	30	38	range	range	NOUN
cet-15373	30	39	of	of	ADP
cet-15373	30	40	250	250	NUM
cet-15373	30	41	-	-	SYM
cet-15373	30	42	355	355	NUM
cet-15373	30	43	m	m	PROPN
cet-15373	30	44	.	.	PUNCT
cet-15373	31	1	2.1.1	2.1.1	NUM
cet-15373	31	2	ru	ru	NOUN
cet-15373	31	3	/	/	SYM
cet-15373	31	4	al2o3	al2o3	PROPN
cet-15373	31	5	the	the	DET
cet-15373	31	6	-alumina	-alumina	PROPN
cet-15373	31	7	(	(	PUNCT
cet-15373	31	8	0.95	0.95	NUM
cet-15373	31	9	g	g	NOUN
cet-15373	31	10	)	)	PUNCT
cet-15373	31	11	and	and	CCONJ
cet-15373	31	12	ruthenium(iii	ruthenium(iii	ADJ
cet-15373	31	13	)	)	PUNCT
cet-15373	31	14	chloride	chloride	NOUN
cet-15373	31	15	hydrate	hydrate	NOUN
cet-15373	31	16	(	(	PUNCT
cet-15373	31	17	0.1316	0.1316	NUM
cet-15373	31	18	g	g	NOUN
cet-15373	31	19	,	,	PUNCT
cet-15373	31	20	rucl3⸱xh2o	rucl3⸱xh2o	NOUN
cet-15373	31	21	,	,	PUNCT
cet-15373	31	22	ru	ru	NOUN
cet-15373	31	23	basis	basis	NOUN
cet-15373	31	24	,	,	PUNCT
cet-15373	31	25	38.0	38.0	NUM
cet-15373	31	26	-	-	SYM
cet-15373	31	27	42.0	42.0	NUM
cet-15373	31	28	%	%	NOUN
cet-15373	31	29	)	)	PUNCT
cet-15373	31	30	were	be	AUX
cet-15373	31	31	used	use	VERB
cet-15373	31	32	to	to	PART
cet-15373	31	33	make	make	VERB
cet-15373	31	34	an	an	DET
cet-15373	31	35	aqueous	aqueous	ADJ
cet-15373	31	36	suspension	suspension	NOUN
cet-15373	31	37	(	(	PUNCT
cet-15373	31	38	25	25	NUM
cet-15373	31	39	ml	ml	NOUN
cet-15373	31	40	ultrapure	ultrapure	ADJ
cet-15373	31	41	h2o	h2o	PROPN
cet-15373	31	42	)	)	PUNCT
cet-15373	31	43	for	for	ADP
cet-15373	31	44	the	the	DET
cet-15373	31	45	wet	wet	ADJ
cet-15373	31	46	impregnation	impregnation	NOUN
cet-15373	31	47	process	process	NOUN
cet-15373	31	48	.	.	PUNCT
cet-15373	32	1	after	after	ADP
cet-15373	32	2	one	one	NUM
cet-15373	32	3	hour	hour	NOUN
cet-15373	32	4	of	of	ADP
cet-15373	32	5	impregnation	impregnation	NOUN
cet-15373	32	6	,	,	PUNCT
cet-15373	32	7	the	the	DET
cet-15373	32	8	sample	sample	NOUN
cet-15373	32	9	was	be	AUX
cet-15373	32	10	dried	dry	VERB
cet-15373	32	11	overnight	overnight	ADV
cet-15373	32	12	and	and	CCONJ
cet-15373	32	13	then	then	ADV
cet-15373	32	14	calcined	calcine	VERB
cet-15373	32	15	in	in	ADP
cet-15373	32	16	air	air	NOUN
cet-15373	32	17	at	at	ADP
cet-15373	32	18	400	400	NUM
cet-15373	32	19	°	°	ADP
cet-15373	32	20	c	c	NOUN
cet-15373	32	21	for	for	ADP
cet-15373	32	22	4	4	NUM
cet-15373	32	23	h	h	NOUN
cet-15373	32	24	,	,	PUNCT
cet-15373	32	25	and	and	CCONJ
cet-15373	32	26	finally	finally	ADV
cet-15373	32	27	reduced	reduce	VERB
cet-15373	32	28	at	at	ADP
cet-15373	32	29	400	400	NUM
cet-15373	32	30	°	°	ADP
cet-15373	32	31	c	c	NOUN
cet-15373	32	32	in	in	ADP
cet-15373	32	33	a	a	DET
cet-15373	32	34	tubular	tubular	ADJ
cet-15373	32	35	furnace	furnace	NOUN
cet-15373	32	36	under	under	ADP
cet-15373	32	37	h2	h2	NOUN
cet-15373	32	38	and	and	CCONJ
cet-15373	32	39	ar	ar	NOUN
cet-15373	32	40	flow	flow	NOUN
cet-15373	32	41	for	for	ADP
cet-15373	32	42	4	4	NUM
cet-15373	32	43	h.	h.	NOUN
cet-15373	32	44	a	a	DET
cet-15373	32	45	metal	metal	NOUN
cet-15373	32	46	loading	loading	NOUN
cet-15373	32	47	of	of	ADP
cet-15373	32	48	5	5	NUM
cet-15373	32	49	wt.%	wt.%	PROPN
cet-15373	32	50	ru	ru	PROPN
cet-15373	32	51	/	/	SYM
cet-15373	32	52	al2o3	al2o3	PROPN
cet-15373	32	53	was	be	AUX
cet-15373	32	54	obtained	obtain	VERB
cet-15373	32	55	.	.	PUNCT
cet-15373	33	1	2.1.2	2.1.2	NUM
cet-15373	33	2	ru	ru	PROPN
cet-15373	33	3	-	-	PUNCT
cet-15373	33	4	fe	fe	NOUN
cet-15373	33	5	/	/	SYM
cet-15373	33	6	al2o3	al2o3	PROPN
cet-15373	33	7	the	the	DET
cet-15373	33	8	-alumina	-alumina	PROPN
cet-15373	33	9	(	(	PUNCT
cet-15373	33	10	1.90	1.90	NUM
cet-15373	33	11	g	g	NOUN
cet-15373	33	12	)	)	PUNCT
cet-15373	33	13	,	,	PUNCT
cet-15373	33	14	ruthenium(iii	ruthenium(iii	PROPN
cet-15373	33	15	)	)	PUNCT
cet-15373	33	16	chloride	chloride	NOUN
cet-15373	33	17	hydrate	hydrate	NOUN
cet-15373	33	18	(	(	PUNCT
cet-15373	33	19	0.256	0.256	NUM
cet-15373	33	20	g	g	NOUN
cet-15373	33	21	,	,	PUNCT
cet-15373	33	22	rucl3⸱xh2o	rucl3⸱xh2o	NOUN
cet-15373	33	23	,	,	PUNCT
cet-15373	33	24	ru	ru	NOUN
cet-15373	33	25	basis	basis	NOUN
cet-15373	33	26	,	,	PUNCT
cet-15373	33	27	38.0	38.0	NUM
cet-15373	33	28	-	-	SYM
cet-15373	33	29	42.0	42.0	NUM
cet-15373	33	30	%	%	NOUN
cet-15373	33	31	)	)	PUNCT
cet-15373	33	32	and	and	CCONJ
cet-15373	33	33	iron(iii	iron(iii	NOUN
cet-15373	33	34	)	)	PUNCT
cet-15373	33	35	nitrate	nitrate	NOUN
cet-15373	33	36	nonahydrate	nonahydrate	NOUN
cet-15373	33	37	(	(	PUNCT
cet-15373	33	38	0.361	0.361	NUM
cet-15373	33	39	g	g	NOUN
cet-15373	33	40	,	,	PUNCT
cet-15373	33	41	fe(no3)3⸱9h2o	fe(no3)3⸱9h2o	PROPN
cet-15373	33	42	,	,	PUNCT
cet-15373	33	43	≥	≥	NUM
cet-15373	33	44	99.95	99.95	NUM
cet-15373	33	45	%	%	NOUN
cet-15373	33	46	trace	trace	NOUN
cet-15373	33	47	metals	metal	NOUN
cet-15373	33	48	basis	basis	NOUN
cet-15373	33	49	)	)	PUNCT
cet-15373	33	50	were	be	AUX
cet-15373	33	51	used	use	VERB
cet-15373	33	52	to	to	PART
cet-15373	33	53	make	make	VERB
cet-15373	33	54	an	an	DET
cet-15373	33	55	aqueous	aqueous	ADJ
cet-15373	33	56	suspension	suspension	NOUN
cet-15373	33	57	(	(	PUNCT
cet-15373	33	58	25	25	NUM
cet-15373	33	59	ml	ml	NOUN
cet-15373	33	60	ultrapure	ultrapure	ADJ
cet-15373	33	61	h2o	h2o	PROPN
cet-15373	33	62	)	)	PUNCT
cet-15373	33	63	for	for	ADP
cet-15373	33	64	the	the	DET
cet-15373	33	65	wet	wet	ADJ
cet-15373	33	66	impregnation	impregnation	NOUN
cet-15373	33	67	process	process	NOUN
cet-15373	33	68	.	.	PUNCT
cet-15373	34	1	after	after	ADP
cet-15373	34	2	one	one	NUM
cet-15373	34	3	hour	hour	NOUN
cet-15373	34	4	of	of	ADP
cet-15373	34	5	impregnation	impregnation	NOUN
cet-15373	34	6	,	,	PUNCT
cet-15373	34	7	the	the	DET
cet-15373	34	8	sample	sample	NOUN
cet-15373	34	9	was	be	AUX
cet-15373	34	10	dried	dry	VERB
cet-15373	34	11	overnight	overnight	ADV
cet-15373	34	12	,	,	PUNCT
cet-15373	34	13	then	then	ADV
cet-15373	34	14	calcined	calcine	VERB
cet-15373	34	15	in	in	ADP
cet-15373	34	16	air	air	NOUN
cet-15373	34	17	at	at	ADP
cet-15373	34	18	400	400	NUM
cet-15373	34	19	°	°	ADP
cet-15373	34	20	c	c	NOUN
cet-15373	34	21	for	for	ADP
cet-15373	34	22	4	4	NUM
cet-15373	34	23	h	h	NOUN
cet-15373	34	24	,	,	PUNCT
cet-15373	34	25	and	and	CCONJ
cet-15373	34	26	finally	finally	ADV
cet-15373	34	27	reduced	reduce	VERB
cet-15373	34	28	at	at	ADP
cet-15373	34	29	400	400	NUM
cet-15373	34	30	°	°	ADP
cet-15373	34	31	c	c	NOUN
cet-15373	34	32	in	in	ADP
cet-15373	34	33	a	a	DET
cet-15373	34	34	tubular	tubular	ADJ
cet-15373	34	35	furnace	furnace	NOUN
cet-15373	34	36	under	under	ADP
cet-15373	34	37	h2	h2	NOUN
cet-15373	34	38	and	and	CCONJ
cet-15373	34	39	ar	ar	NOUN
cet-15373	34	40	flow	flow	NOUN
cet-15373	34	41	for	for	ADP
cet-15373	34	42	4	4	NUM
cet-15373	34	43	h.	h.	NOUN
cet-15373	34	44	the	the	DET
cet-15373	34	45	final	final	ADJ
cet-15373	34	46	metal	metal	NOUN
cet-15373	34	47	loading	loading	NOUN
cet-15373	34	48	of	of	ADP
cet-15373	34	49	ru	ru	PROPN
cet-15373	34	50	-	-	PUNCT
cet-15373	34	51	fe	fe	NOUN
cet-15373	34	52	/	/	SYM
cet-15373	34	53	al2o3	al2o3	PROPN
cet-15373	34	54	was	be	AUX
cet-15373	34	55	2.5	2.5	NUM
cet-15373	34	56	wt.%	wt.%	ADJ
cet-15373	34	57	for	for	ADP
cet-15373	34	58	iron	iron	NOUN
cet-15373	34	59	and	and	CCONJ
cet-15373	34	60	2.5	2.5	NUM
cet-15373	34	61	wt.%	wt.%	NOUN
cet-15373	34	62	for	for	ADP
cet-15373	34	63	ruthenium	ruthenium	NOUN
cet-15373	34	64	.	.	PUNCT
cet-15373	35	1	2.1.3	2.1.3	NUM
cet-15373	35	2	fe2o3	fe2o3	PROPN
cet-15373	35	3	/	/	SYM
cet-15373	35	4	al2o3	al2o3	PROPN
cet-15373	35	5	the	the	DET
cet-15373	35	6	-alumina	-alumina	PROPN
cet-15373	35	7	(	(	PUNCT
cet-15373	35	8	0.903	0.903	NUM
cet-15373	35	9	g	g	NOUN
cet-15373	35	10	)	)	PUNCT
cet-15373	35	11	and	and	CCONJ
cet-15373	35	12	fe	fe	NOUN
cet-15373	35	13	-	-	NOUN
cet-15373	35	14	precursor	precursor	NOUN
cet-15373	35	15	,	,	PUNCT
cet-15373	35	16	iron(iii	iron(iii	NOUN
cet-15373	35	17	)	)	PUNCT
cet-15373	35	18	nitrate	nitrate	NOUN
cet-15373	35	19	nonahydrate	nonahydrate	NOUN
cet-15373	35	20	(	(	PUNCT
cet-15373	35	21	0.253	0.253	NUM
cet-15373	35	22	g	g	NOUN
cet-15373	35	23	,	,	PUNCT
cet-15373	35	24	fe(no3)3⸱9h2o	fe(no3)3⸱9h2o	PROPN
cet-15373	35	25	,	,	PUNCT
cet-15373	35	26	≥	≥	NUM
cet-15373	35	27	99.95	99.95	NUM
cet-15373	35	28	%	%	NOUN
cet-15373	35	29	trace	trace	NOUN
cet-15373	35	30	metals	metal	NOUN
cet-15373	35	31	basis	basis	NOUN
cet-15373	35	32	)	)	PUNCT
cet-15373	35	33	,	,	PUNCT
cet-15373	35	34	were	be	AUX
cet-15373	35	35	suspended	suspend	VERB
cet-15373	35	36	in	in	ADP
cet-15373	35	37	25	25	NUM
cet-15373	35	38	ml	ml	NOUN
cet-15373	35	39	of	of	ADP
cet-15373	35	40	deionized	deionize	VERB
cet-15373	35	41	water	water	NOUN
cet-15373	35	42	with	with	ADP
cet-15373	35	43	1	1	NUM
cet-15373	35	44	ml	ml	NOUN
cet-15373	35	45	of	of	ADP
cet-15373	35	46	ethylene	ethylene	NOUN
cet-15373	35	47	glycol	glycol	NOUN
cet-15373	35	48	;	;	PUNCT
cet-15373	35	49	then	then	ADV
cet-15373	35	50	,	,	PUNCT
cet-15373	35	51	the	the	DET
cet-15373	35	52	mixture	mixture	NOUN
cet-15373	35	53	was	be	AUX
cet-15373	35	54	sonicated	sonicate	VERB
cet-15373	35	55	for	for	ADP
cet-15373	35	56	30	30	NUM
cet-15373	35	57	minutes	minute	NOUN
cet-15373	35	58	,	,	PUNCT
cet-15373	35	59	and	and	CCONJ
cet-15373	35	60	the	the	DET
cet-15373	35	61	ph	ph	NOUN
cet-15373	35	62	was	be	AUX
cet-15373	35	63	adjusted	adjust	VERB
cet-15373	35	64	to	to	ADP
cet-15373	35	65	8	8	NUM
cet-15373	35	66	with	with	ADP
cet-15373	35	67	a	a	DET
cet-15373	35	68	5	5	NUM
cet-15373	35	69	%	%	NOUN
cet-15373	35	70	ammonium	ammonium	NOUN
cet-15373	35	71	hydroxide	hydroxide	NOUN
cet-15373	35	72	solution	solution	NOUN
cet-15373	35	73	.	.	PUNCT
cet-15373	36	1	afterwards	afterwards	ADV
cet-15373	36	2	,	,	PUNCT
cet-15373	36	3	the	the	DET
cet-15373	36	4	solvent	solvent	NOUN
cet-15373	36	5	was	be	AUX
cet-15373	36	6	eliminated	eliminate	VERB
cet-15373	36	7	by	by	ADP
cet-15373	36	8	drying	dry	VERB
cet-15373	36	9	at	at	ADP
cet-15373	36	10	120	120	NUM
cet-15373	36	11	°	°	NOUN
cet-15373	36	12	c	c	NOUN
cet-15373	36	13	overnight	overnight	ADV
cet-15373	36	14	.	.	PUNCT
cet-15373	37	1	the	the	DET
cet-15373	37	2	obtained	obtain	VERB
cet-15373	37	3	powder	powder	NOUN
cet-15373	37	4	was	be	AUX
cet-15373	37	5	calcined	calcine	VERB
cet-15373	37	6	for	for	ADP
cet-15373	37	7	2	2	NUM
cet-15373	37	8	h	h	NOUN
cet-15373	37	9	at	at	ADP
cet-15373	37	10	400	400	NUM
cet-15373	37	11	°	°	ADP
cet-15373	37	12	c	c	NOUN
cet-15373	37	13	in	in	ADP
cet-15373	37	14	a	a	DET
cet-15373	37	15	horizontal	horizontal	ADJ
cet-15373	37	16	tubular	tubular	ADJ
cet-15373	37	17	furnace	furnace	NOUN
cet-15373	37	18	under	under	ADP
cet-15373	37	19	ar	ar	NOUN
cet-15373	37	20	flow	flow	NOUN
cet-15373	37	21	.	.	PUNCT
cet-15373	38	1	a	a	DET
cet-15373	38	2	metal	metal	NOUN
cet-15373	38	3	loading	loading	NOUN
cet-15373	38	4	of	of	ADP
cet-15373	38	5	5	5	NUM
cet-15373	38	6	wt.%	wt.%	NOUN
cet-15373	38	7	was	be	AUX
cet-15373	38	8	finally	finally	ADV
cet-15373	38	9	obtained	obtain	VERB
cet-15373	38	10	.	.	PUNCT
cet-15373	39	1	2.2	2.2	NUM
cet-15373	39	2	cnts	cnt	NOUN
cet-15373	39	3	-	-	PUNCT
cet-15373	39	4	based	base	VERB
cet-15373	39	5	catalysts	catalyst	NOUN
cet-15373	39	6	preparation	preparation	VERB
cet-15373	39	7	the	the	DET
cet-15373	39	8	functionalization	functionalization	NOUN
cet-15373	39	9	of	of	ADP
cet-15373	39	10	cnts	cnts	PROPN
cet-15373	39	11	consists	consist	VERB
cet-15373	39	12	of	of	ADP
cet-15373	39	13	a	a	DET
cet-15373	39	14	pre	pre	NOUN
cet-15373	39	15	-	-	NOUN
cet-15373	39	16	treatment	treatment	NOUN
cet-15373	39	17	of	of	ADP
cet-15373	39	18	commercial	commercial	ADJ
cet-15373	39	19	cnts	cnt	NOUN
cet-15373	39	20	(	(	PUNCT
cet-15373	39	21	pyrograph	pyrograph	NOUN
cet-15373	39	22	-	-	PUNCT
cet-15373	39	23	iii	iii	NOUN
cet-15373	39	24	,	,	PUNCT
cet-15373	39	25	pr-24xt	pr-24xt	PROPN
cet-15373	39	26	)	)	PUNCT
cet-15373	39	27	with	with	ADP
cet-15373	39	28	nitric	nitric	ADJ
cet-15373	39	29	acid	acid	NOUN
cet-15373	39	30	(	(	PUNCT
cet-15373	39	31	conc	conc	NOUN
cet-15373	39	32	.	.	PUNCT
cet-15373	40	1	65	65	NUM
cet-15373	40	2	%	%	NOUN
cet-15373	40	3	)	)	PUNCT
cet-15373	40	4	,	,	PUNCT
cet-15373	40	5	50	50	NUM
cet-15373	40	6	ml	ml	NOUN
cet-15373	40	7	for	for	ADP
cet-15373	40	8	1	1	NUM
cet-15373	40	9	g	g	NOUN
cet-15373	40	10	of	of	ADP
cet-15373	40	11	cnts	cnt	NOUN
cet-15373	40	12	,	,	PUNCT
cet-15373	40	13	in	in	ADP
cet-15373	40	14	order	order	NOUN
cet-15373	40	15	to	to	PART
cet-15373	40	16	create	create	VERB
cet-15373	40	17	oxygen	oxygen	NOUN
cet-15373	40	18	functionalities	functionality	NOUN
cet-15373	40	19	as	as	SCONJ
cet-15373	40	20	reported	report	VERB
cet-15373	40	21	by	by	ADP
cet-15373	40	22	hirsh	hirsh	NOUN
cet-15373	40	23	,	,	PUNCT
cet-15373	40	24	a.	a.	NOUN
cet-15373	40	25	and	and	CCONJ
cet-15373	40	26	volstrowsky	volstrowsky	ADJ
cet-15373	40	27	,	,	PUNCT
cet-15373	40	28	o.	o.	PROPN
cet-15373	40	29	(	(	PUNCT
cet-15373	40	30	2005	2005	NUM
cet-15373	40	31	)	)	PUNCT
cet-15373	40	32	,	,	PUNCT
cet-15373	40	33	hereafter	hereafter	ADV
cet-15373	40	34	called	call	VERB
cet-15373	40	35	cnts	cnt	NOUN
cet-15373	40	36	for	for	ADP
cet-15373	40	37	simplicity	simplicity	NOUN
cet-15373	40	38	,	,	PUNCT
cet-15373	40	39	then	then	ADV
cet-15373	40	40	treated	treat	VERB
cet-15373	40	41	at	at	ADP
cet-15373	40	42	120	120	NUM
cet-15373	40	43	°	°	NOUN
cet-15373	40	44	c	c	NOUN
cet-15373	40	45	for	for	ADP
cet-15373	40	46	2	2	NUM
cet-15373	40	47	h	h	NOUN
cet-15373	40	48	in	in	ADP
cet-15373	40	49	a	a	DET
cet-15373	40	50	reflux	reflux	NOUN
cet-15373	40	51	apparatus	apparatus	NOUN
cet-15373	40	52	(	(	PUNCT
cet-15373	40	53	chen	chen	PROPN
cet-15373	40	54	et	et	PROPN
cet-15373	40	55	al	al	PROPN
cet-15373	40	56	.	.	PROPN
cet-15373	40	57	,	,	PUNCT
cet-15373	40	58	2020	2020	NUM
cet-15373	40	59	)	)	PUNCT
cet-15373	40	60	.	.	PUNCT
cet-15373	41	1	the	the	DET
cet-15373	41	2	suspension	suspension	NOUN
cet-15373	41	3	was	be	AUX
cet-15373	41	4	filtered	filter	VERB
cet-15373	41	5	and	and	CCONJ
cet-15373	41	6	washed	wash	VERB
cet-15373	41	7	with	with	ADP
cet-15373	41	8	deionized	deionize	VERB
cet-15373	41	9	water	water	NOUN
cet-15373	41	10	until	until	ADP
cet-15373	41	11	neutral	neutral	ADJ
cet-15373	41	12	ph	ph	PROPN
cet-15373	41	13	.	.	PUNCT
cet-15373	42	1	the	the	DET
cet-15373	42	2	sample	sample	NOUN
cet-15373	42	3	was	be	AUX
cet-15373	42	4	dried	dry	VERB
cet-15373	42	5	at	at	ADP
cet-15373	42	6	80	80	NUM
cet-15373	42	7	°	°	NOUN
cet-15373	42	8	c	c	NOUN
cet-15373	42	9	overnight	overnight	ADV
cet-15373	42	10	.	.	PUNCT
cet-15373	43	1	2.2.1	2.2.1	NUM
cet-15373	43	2	ru	ru	NOUN
cet-15373	43	3	/	/	SYM
cet-15373	43	4	cnts	cnts	PROPN
cet-15373	43	5	the	the	DET
cet-15373	43	6	cnts	cnts	PROPN
cet-15373	43	7	(	(	PUNCT
cet-15373	43	8	0.425	0.425	NUM
cet-15373	43	9	g	g	NOUN
cet-15373	43	10	)	)	PUNCT
cet-15373	43	11	and	and	CCONJ
cet-15373	43	12	ru	ru	NOUN
cet-15373	43	13	-	-	NOUN
cet-15373	43	14	precursor	precursor	NOUN
cet-15373	43	15	,	,	PUNCT
cet-15373	43	16	ruthenium(iii	ruthenium(iii	PROPN
cet-15373	43	17	)	)	PUNCT
cet-15373	43	18	chloride	chloride	NOUN
cet-15373	43	19	hydrate	hydrate	NOUN
cet-15373	43	20	(	(	PUNCT
cet-15373	43	21	0.128	0.128	NUM
cet-15373	43	22	g	g	NOUN
cet-15373	43	23	,	,	PUNCT
cet-15373	43	24	rucl3⸱xh2o	rucl3⸱xh2o	NOUN
cet-15373	43	25	,	,	PUNCT
cet-15373	43	26	ru	ru	NOUN
cet-15373	43	27	basis	basis	NOUN
cet-15373	43	28	,	,	PUNCT
cet-15373	43	29	38.042.0	38.042.0	NUM
cet-15373	43	30	%	%	NOUN
cet-15373	43	31	)	)	PUNCT
cet-15373	43	32	were	be	AUX
cet-15373	43	33	dissolved	dissolve	VERB
cet-15373	43	34	in	in	ADP
cet-15373	43	35	25	25	NUM
cet-15373	43	36	ml	ml	NOUN
cet-15373	43	37	of	of	ADP
cet-15373	43	38	deionized	deionize	VERB
cet-15373	43	39	water	water	NOUN
cet-15373	43	40	,	,	PUNCT
cet-15373	43	41	then	then	ADV
cet-15373	43	42	the	the	DET
cet-15373	43	43	mixture	mixture	NOUN
cet-15373	43	44	was	be	AUX
cet-15373	43	45	stirred	stir	VERB
cet-15373	43	46	for	for	ADP
cet-15373	43	47	1.5h	1.5h	NUM
cet-15373	43	48	.	.	PUNCT
cet-15373	44	1	afterwards	afterwards	ADV
cet-15373	44	2	,	,	PUNCT
cet-15373	44	3	the	the	DET
cet-15373	44	4	solvent	solvent	NOUN
cet-15373	44	5	was	be	AUX
cet-15373	44	6	eliminated	eliminate	VERB
cet-15373	44	7	by	by	ADP
cet-15373	44	8	drying	dry	VERB
cet-15373	44	9	at	at	ADP
cet-15373	44	10	120	120	NUM
cet-15373	44	11	°	°	NOUN
cet-15373	44	12	c	c	NOUN
cet-15373	44	13	overnight	overnight	ADV
cet-15373	44	14	.	.	PUNCT
cet-15373	45	1	the	the	DET
cet-15373	45	2	obtained	obtain	VERB
cet-15373	45	3	powder	powder	NOUN
cet-15373	45	4	was	be	AUX
cet-15373	45	5	calcined	calcine	VERB
cet-15373	45	6	for	for	ADP
cet-15373	45	7	4	4	NUM
cet-15373	45	8	h	h	NOUN
cet-15373	45	9	at	at	ADP
cet-15373	45	10	400	400	NUM
cet-15373	45	11	°	°	ADP
cet-15373	45	12	c	c	NOUN
cet-15373	45	13	in	in	ADP
cet-15373	45	14	a	a	DET
cet-15373	45	15	horizontal	horizontal	ADJ
cet-15373	45	16	tubular	tubular	ADJ
cet-15373	45	17	furnace	furnace	NOUN
cet-15373	45	18	under	under	ADP
cet-15373	45	19	h2	h2	NOUN
cet-15373	45	20	and	and	CCONJ
cet-15373	45	21	ar	ar	NOUN
cet-15373	45	22	flows	flow	NOUN
cet-15373	45	23	.	.	PUNCT
cet-15373	46	1	the	the	DET
cet-15373	46	2	ru	ru	PROPN
cet-15373	46	3	-	-	PUNCT
cet-15373	46	4	cnts	cnts	PROPN
cet-15373	46	5	sample	sample	NOUN
cet-15373	46	6	was	be	AUX
cet-15373	46	7	obtained	obtain	VERB
cet-15373	46	8	with	with	ADP
cet-15373	46	9	a	a	DET
cet-15373	46	10	final	final	ADJ
cet-15373	46	11	metal	metal	NOUN
cet-15373	46	12	loading	loading	NOUN
cet-15373	46	13	of	of	ADP
cet-15373	46	14	5	5	NUM
cet-15373	46	15	wt.%	wt.%	ADJ
cet-15373	46	16	.	.	PUNCT
cet-15373	47	1	734	734	NUM
cet-15373	47	2	2.2.2	2.2.2	NUM
cet-15373	47	3	ru	ru	NOUN
cet-15373	47	4	-	-	PUNCT
cet-15373	47	5	fe	fe	NOUN
cet-15373	47	6	/	/	SYM
cet-15373	47	7	cnts	cnts	PROPN
cet-15373	47	8	the	the	DET
cet-15373	47	9	cnts	cnts	PROPN
cet-15373	47	10	(	(	PUNCT
cet-15373	47	11	0.95	0.95	NUM
cet-15373	47	12	g	g	NOUN
cet-15373	47	13	)	)	PUNCT
cet-15373	47	14	and	and	CCONJ
cet-15373	47	15	ru	ru	NOUN
cet-15373	47	16	-	-	NOUN
cet-15373	47	17	precursor	precursor	NOUN
cet-15373	47	18	,	,	PUNCT
cet-15373	47	19	ruthenium(iii	ruthenium(iii	PROPN
cet-15373	47	20	)	)	PUNCT
cet-15373	47	21	chloride	chloride	NOUN
cet-15373	47	22	hydrate	hydrate	NOUN
cet-15373	47	23	(	(	PUNCT
cet-15373	47	24	0.180	0.180	NUM
cet-15373	47	25	g	g	NOUN
cet-15373	47	26	,	,	PUNCT
cet-15373	47	27	rucl3⸱xh2o	rucl3⸱xh2o	NOUN
cet-15373	47	28	,	,	PUNCT
cet-15373	47	29	ru	ru	NOUN
cet-15373	47	30	basis	basis	NOUN
cet-15373	47	31	,	,	PUNCT
cet-15373	47	32	35.040.0	35.040.0	NUM
cet-15373	47	33	%	%	NOUN
cet-15373	47	34	)	)	PUNCT
cet-15373	47	35	and	and	CCONJ
cet-15373	47	36	iron(iii	iron(iii	NOUN
cet-15373	47	37	)	)	PUNCT
cet-15373	47	38	chloride	chloride	NOUN
cet-15373	47	39	hexahydrate	hexahydrate	NOUN
cet-15373	47	40	(	(	PUNCT
cet-15373	47	41	0.121	0.121	NUM
cet-15373	47	42	g	g	NOUN
cet-15373	47	43	,	,	PUNCT
cet-15373	47	44	fecl3⸱6h2o	fecl3⸱6h2o	NOUN
cet-15373	47	45	)	)	PUNCT
cet-15373	47	46	were	be	AUX
cet-15373	47	47	dissolved	dissolve	VERB
cet-15373	47	48	in	in	ADP
cet-15373	47	49	25	25	NUM
cet-15373	47	50	ml	ml	NOUN
cet-15373	47	51	of	of	ADP
cet-15373	47	52	deionized	deionize	VERB
cet-15373	47	53	water	water	NOUN
cet-15373	47	54	,	,	PUNCT
cet-15373	47	55	then	then	ADV
cet-15373	47	56	the	the	DET
cet-15373	47	57	mixture	mixture	NOUN
cet-15373	47	58	was	be	AUX
cet-15373	47	59	stirred	stir	VERB
cet-15373	47	60	for	for	ADP
cet-15373	47	61	1.5	1.5	NUM
cet-15373	47	62	h.	h.	NOUN
cet-15373	47	63	afterwards	afterwards	ADV
cet-15373	47	64	,	,	PUNCT
cet-15373	47	65	the	the	DET
cet-15373	47	66	solvent	solvent	NOUN
cet-15373	47	67	was	be	AUX
cet-15373	47	68	eliminated	eliminate	VERB
cet-15373	47	69	by	by	ADP
cet-15373	47	70	drying	dry	VERB
cet-15373	47	71	at	at	ADP
cet-15373	47	72	120	120	NUM
cet-15373	47	73	°	°	NOUN
cet-15373	47	74	c	c	NOUN
cet-15373	47	75	overnight	overnight	ADV
cet-15373	47	76	.	.	PUNCT
cet-15373	48	1	the	the	DET
cet-15373	48	2	obtained	obtain	VERB
cet-15373	48	3	powder	powder	NOUN
cet-15373	48	4	was	be	AUX
cet-15373	48	5	calcined	calcine	VERB
cet-15373	48	6	for	for	ADP
cet-15373	48	7	4	4	NUM
cet-15373	48	8	h	h	NOUN
cet-15373	48	9	at	at	ADP
cet-15373	48	10	400	400	NUM
cet-15373	48	11	°	°	ADP
cet-15373	48	12	c	c	NOUN
cet-15373	48	13	in	in	ADP
cet-15373	48	14	a	a	DET
cet-15373	48	15	horizontal	horizontal	ADJ
cet-15373	48	16	tubular	tubular	ADJ
cet-15373	48	17	furnace	furnace	NOUN
cet-15373	48	18	under	under	ADP
cet-15373	48	19	h2	h2	NOUN
cet-15373	48	20	and	and	CCONJ
cet-15373	48	21	ar	ar	NOUN
cet-15373	48	22	flows	flow	NOUN
cet-15373	48	23	.	.	PUNCT
cet-15373	49	1	the	the	DET
cet-15373	49	2	rufe	rufe	NOUN
cet-15373	49	3	/	/	SYM
cet-15373	49	4	cnts	cnts	PROPN
cet-15373	49	5	was	be	AUX
cet-15373	49	6	finally	finally	ADV
cet-15373	49	7	obtained	obtain	VERB
cet-15373	49	8	with	with	ADP
cet-15373	49	9	2.5	2.5	NUM
cet-15373	49	10	wt.%	wt.%	ADJ
cet-15373	49	11	iron	iron	NOUN
cet-15373	49	12	and	and	CCONJ
cet-15373	49	13	2.5	2.5	NUM
cet-15373	49	14	wt.%	wt.%	PROPN
cet-15373	49	15	ruthenium	ruthenium	NOUN
cet-15373	49	16	.	.	PUNCT
cet-15373	50	1	2.2.3	2.2.3	NUM
cet-15373	50	2	fe2o3	fe2o3	PROPN
cet-15373	50	3	/	/	SYM
cet-15373	50	4	cnts	cnt	NOUN
cet-15373	50	5	the	the	DET
cet-15373	50	6	cnts	cnts	PROPN
cet-15373	50	7	(	(	PUNCT
cet-15373	50	8	0.7	0.7	NUM
cet-15373	50	9	g	g	NOUN
cet-15373	50	10	)	)	PUNCT
cet-15373	50	11	and	and	CCONJ
cet-15373	50	12	fe	fe	NOUN
cet-15373	50	13	-	-	NOUN
cet-15373	50	14	precursor	precursor	NOUN
cet-15373	50	15	,	,	PUNCT
cet-15373	50	16	iron(iii	iron(iii	NOUN
cet-15373	50	17	)	)	PUNCT
cet-15373	50	18	nitrate	nitrate	NOUN
cet-15373	50	19	nonahydrate	nonahydrate	NOUN
cet-15373	50	20	(	(	PUNCT
cet-15373	50	21	1.515	1.515	NUM
cet-15373	50	22	g	g	NOUN
cet-15373	50	23	,	,	PUNCT
cet-15373	50	24	fe(no3)3⸱9h2o	fe(no3)3⸱9h2o	PROPN
cet-15373	50	25	,	,	PUNCT
cet-15373	50	26	≥	≥	NUM
cet-15373	50	27	99.95	99.95	NUM
cet-15373	50	28	%	%	NOUN
cet-15373	50	29	trace	trace	NOUN
cet-15373	50	30	metals	metal	NOUN
cet-15373	50	31	basis	basis	NOUN
cet-15373	50	32	)	)	PUNCT
cet-15373	50	33	,	,	PUNCT
cet-15373	50	34	were	be	AUX
cet-15373	50	35	dissolved	dissolve	VERB
cet-15373	50	36	in	in	ADP
cet-15373	50	37	25	25	NUM
cet-15373	50	38	ml	ml	NOUN
cet-15373	50	39	of	of	ADP
cet-15373	50	40	deionized	deionize	VERB
cet-15373	50	41	water	water	NOUN
cet-15373	50	42	with	with	ADP
cet-15373	50	43	1	1	NUM
cet-15373	50	44	ml	ml	NOUN
cet-15373	50	45	of	of	ADP
cet-15373	50	46	ethylene	ethylene	NOUN
cet-15373	50	47	glycol	glycol	NOUN
cet-15373	50	48	,	,	PUNCT
cet-15373	50	49	then	then	ADV
cet-15373	50	50	the	the	DET
cet-15373	50	51	mixture	mixture	NOUN
cet-15373	50	52	was	be	AUX
cet-15373	50	53	sonicated	sonicate	VERB
cet-15373	50	54	for	for	ADP
cet-15373	50	55	30	30	NUM
cet-15373	50	56	minutes	minute	NOUN
cet-15373	50	57	,	,	PUNCT
cet-15373	50	58	and	and	CCONJ
cet-15373	50	59	the	the	DET
cet-15373	50	60	ph	ph	NOUN
cet-15373	50	61	was	be	AUX
cet-15373	50	62	adjusted	adjust	VERB
cet-15373	50	63	to	to	ADP
cet-15373	50	64	8	8	NUM
cet-15373	50	65	with	with	ADP
cet-15373	50	66	a	a	DET
cet-15373	50	67	5	5	NUM
cet-15373	50	68	%	%	NOUN
cet-15373	50	69	ammonium	ammonium	NOUN
cet-15373	50	70	hydroxide	hydroxide	NOUN
cet-15373	50	71	solution	solution	NOUN
cet-15373	50	72	.	.	PUNCT
cet-15373	51	1	afterward	afterward	ADV
cet-15373	51	2	,	,	PUNCT
cet-15373	51	3	the	the	DET
cet-15373	51	4	solvent	solvent	NOUN
cet-15373	51	5	was	be	AUX
cet-15373	51	6	eliminated	eliminate	VERB
cet-15373	51	7	by	by	ADP
cet-15373	51	8	drying	dry	VERB
cet-15373	51	9	at	at	ADP
cet-15373	51	10	120	120	NUM
cet-15373	51	11	°	°	NOUN
cet-15373	51	12	c	c	NOUN
cet-15373	51	13	overnight	overnight	ADV
cet-15373	51	14	.	.	PUNCT
cet-15373	52	1	the	the	DET
cet-15373	52	2	obtained	obtain	VERB
cet-15373	52	3	powder	powder	NOUN
cet-15373	52	4	was	be	AUX
cet-15373	52	5	calcined	calcine	VERB
cet-15373	52	6	for	for	ADP
cet-15373	52	7	2	2	NUM
cet-15373	52	8	h	h	NOUN
cet-15373	52	9	at	at	ADP
cet-15373	52	10	400	400	NUM
cet-15373	52	11	°	°	ADP
cet-15373	52	12	c	c	NOUN
cet-15373	52	13	in	in	ADP
cet-15373	52	14	a	a	DET
cet-15373	52	15	horizontal	horizontal	ADJ
cet-15373	52	16	tubular	tubular	ADJ
cet-15373	52	17	furnace	furnace	NOUN
cet-15373	52	18	under	under	SCONJ
cet-15373	52	19	he	he	PRON
cet-15373	52	20	flows	flow	VERB
cet-15373	52	21	.	.	PUNCT
cet-15373	53	1	the	the	DET
cet-15373	53	2	fe2o3	fe2o3	PROPN
cet-15373	53	3	-	-	PUNCT
cet-15373	53	4	cnts	cnts	PROPN
cet-15373	53	5	was	be	AUX
cet-15373	53	6	finally	finally	ADV
cet-15373	53	7	obtained	obtain	VERB
cet-15373	53	8	with	with	ADP
cet-15373	53	9	30	30	NUM
cet-15373	53	10	wt.%	wt.%	ADJ
cet-15373	53	11	metal	metal	NOUN
cet-15373	53	12	loading	loading	NOUN
cet-15373	53	13	.	.	PUNCT
cet-15373	54	1	2.3	2.3	NUM
cet-15373	54	2	electrode	electrode	NOUN
cet-15373	54	3	preparation	preparation	NOUN
cet-15373	54	4	in	in	ADP
cet-15373	54	5	the	the	DET
cet-15373	54	6	electrode	electrode	NOUN
cet-15373	54	7	fabrication	fabrication	NOUN
cet-15373	54	8	process	process	NOUN
cet-15373	54	9	,	,	PUNCT
cet-15373	54	10	a	a	DET
cet-15373	54	11	commercial	commercial	ADJ
cet-15373	54	12	gas	gas	NOUN
cet-15373	54	13	-	-	PUNCT
cet-15373	54	14	diffusion	diffusion	NOUN
cet-15373	54	15	layer	layer	NOUN
cet-15373	54	16	(	(	PUNCT
cet-15373	54	17	gdl	gdl	NOUN
cet-15373	54	18	)	)	PUNCT
cet-15373	54	19	,	,	PUNCT
cet-15373	54	20	specifically	specifically	ADV
cet-15373	54	21	the	the	DET
cet-15373	54	22	sigracet	sigracet	ADJ
cet-15373	54	23	gdl	gdl	NOUN
cet-15373	54	24	39bb	39bb	NOUN
cet-15373	54	25	,	,	PUNCT
cet-15373	54	26	and	and	CCONJ
cet-15373	54	27	a	a	DET
cet-15373	54	28	nafion	nafion	NOUN
cet-15373	54	29	®	®	NOUN
cet-15373	54	30	membrane	membrane	NOUN
cet-15373	54	31	n115	n115	PROPN
cet-15373	54	32	were	be	AUX
cet-15373	54	33	provided	provide	VERB
cet-15373	54	34	by	by	ADP
cet-15373	54	35	sgl	sgl	PROPN
cet-15373	54	36	group	group	NOUN
cet-15373	54	37	,	,	PUNCT
cet-15373	54	38	and	and	CCONJ
cet-15373	54	39	a	a	DET
cet-15373	54	40	10	10	NUM
cet-15373	54	41	wt.%	wt.%	ADJ
cet-15373	54	42	weight	weight	NOUN
cet-15373	54	43	nafion	nafion	NOUN
cet-15373	54	44	solution	solution	NOUN
cet-15373	54	45	used	use	VERB
cet-15373	54	46	.	.	PUNCT
cet-15373	55	1	the	the	DET
cet-15373	55	2	ink	ink	NOUN
cet-15373	55	3	preparation	preparation	NOUN
cet-15373	55	4	consisted	consist	VERB
cet-15373	55	5	in	in	ADP
cet-15373	55	6	a	a	DET
cet-15373	55	7	sonication	sonication	NOUN
cet-15373	55	8	of	of	ADP
cet-15373	55	9	50	50	NUM
cet-15373	55	10	mg	mg	NOUN
cet-15373	55	11	of	of	ADP
cet-15373	55	12	catalyst	catalyst	NOUN
cet-15373	55	13	,	,	PUNCT
cet-15373	55	14	8	8	NUM
cet-15373	55	15	ml	ml	NOUN
cet-15373	55	16	of	of	ADP
cet-15373	55	17	isopropanol	isopropanol	NOUN
cet-15373	55	18	,	,	PUNCT
cet-15373	55	19	and	and	CCONJ
cet-15373	55	20	50	50	NUM
cet-15373	55	21	l	l	NOUN
cet-15373	55	22	of	of	ADP
cet-15373	55	23	a	a	DET
cet-15373	55	24	perfluorinated	perfluorinate	VERB
cet-15373	55	25	(	(	PUNCT
cet-15373	55	26	10	10	NUM
cet-15373	55	27	wt.%	wt.%	ADJ
cet-15373	55	28	)	)	PUNCT
cet-15373	55	29	nafion	nafion	NOUN
cet-15373	55	30	solution	solution	NOUN
cet-15373	55	31	,	,	PUNCT
cet-15373	55	32	for	for	ADP
cet-15373	55	33	30	30	NUM
cet-15373	55	34	minutes	minute	NOUN
cet-15373	55	35	until	until	SCONJ
cet-15373	55	36	a	a	DET
cet-15373	55	37	uniform	uniform	ADJ
cet-15373	55	38	and	and	CCONJ
cet-15373	55	39	homogeneous	homogeneous	ADJ
cet-15373	55	40	mixture	mixture	NOUN
cet-15373	55	41	was	be	AUX
cet-15373	55	42	attained	attain	VERB
cet-15373	55	43	.	.	PUNCT
cet-15373	56	1	subsequently	subsequently	ADV
cet-15373	56	2	,	,	PUNCT
cet-15373	56	3	the	the	DET
cet-15373	56	4	prepared	prepare	VERB
cet-15373	56	5	ink	ink	NOUN
cet-15373	56	6	was	be	AUX
cet-15373	56	7	applied	apply	VERB
cet-15373	56	8	via	via	ADP
cet-15373	56	9	spray	spray	NOUN
cet-15373	56	10	coating	coating	NOUN
cet-15373	56	11	and	and	CCONJ
cet-15373	56	12	deposited	deposit	VERB
cet-15373	56	13	across	across	ADP
cet-15373	56	14	a	a	DET
cet-15373	56	15	25	25	NUM
cet-15373	56	16	cm2	cm2	NOUN
cet-15373	56	17	area	area	NOUN
cet-15373	56	18	.	.	PUNCT
cet-15373	57	1	once	once	ADV
cet-15373	57	2	the	the	DET
cet-15373	57	3	load	load	NOUN
cet-15373	57	4	is	be	AUX
cet-15373	57	5	reached	reach	VERB
cet-15373	57	6	,	,	PUNCT
cet-15373	57	7	the	the	DET
cet-15373	57	8	catalyst	catalyst	NOUN
cet-15373	57	9	is	be	AUX
cet-15373	57	10	cut	cut	VERB
cet-15373	57	11	into	into	ADP
cet-15373	57	12	a	a	DET
cet-15373	57	13	round	round	ADJ
cet-15373	57	14	shape	shape	NOUN
cet-15373	57	15	(	(	PUNCT
cet-15373	57	16	20	20	NUM
cet-15373	57	17	mm	mm	PROPN
cet-15373	57	18	diameter	diameter	NOUN
cet-15373	57	19	)	)	PUNCT
cet-15373	57	20	and	and	CCONJ
cet-15373	57	21	hot	hot	ADV
cet-15373	57	22	-	-	PUNCT
cet-15373	57	23	pressed	press	VERB
cet-15373	57	24	for	for	ADP
cet-15373	57	25	15	15	NUM
cet-15373	57	26	s	s	NOUN
cet-15373	57	27	at	at	ADP
cet-15373	57	28	130	130	NUM
cet-15373	57	29	°	°	ADP
cet-15373	57	30	c	c	NOUN
cet-15373	57	31	with	with	ADP
cet-15373	57	32	a	a	DET
cet-15373	57	33	purified	purify	VERB
cet-15373	57	34	nafion	nafion	NOUN
cet-15373	57	35	membrane	membrane	NOUN
cet-15373	57	36	(	(	PUNCT
cet-15373	57	37	membrane	membrane	NOUN
cet-15373	57	38	electrode	electrode	NOUN
cet-15373	57	39	assembly	assembly	NOUN
cet-15373	57	40	mea	mea	PROPN
cet-15373	57	41	)	)	PUNCT
cet-15373	57	42	.	.	PUNCT
cet-15373	58	1	all	all	DET
cet-15373	58	2	the	the	DET
cet-15373	58	3	chemical	chemical	ADJ
cet-15373	58	4	reagents	reagent	NOUN
cet-15373	58	5	used	use	VERB
cet-15373	58	6	in	in	ADP
cet-15373	58	7	this	this	DET
cet-15373	58	8	study	study	NOUN
cet-15373	58	9	were	be	AUX
cet-15373	58	10	of	of	ADP
cet-15373	58	11	analytical	analytical	ADJ
cet-15373	58	12	grade	grade	NOUN
cet-15373	58	13	without	without	ADP
cet-15373	58	14	any	any	DET
cet-15373	58	15	purification	purification	NOUN
cet-15373	58	16	.	.	PUNCT
cet-15373	59	1	2.4	2.4	NUM
cet-15373	59	2	electrochemical	electrochemical	ADJ
cet-15373	59	3	device	device	NOUN
cet-15373	59	4	the	the	DET
cet-15373	59	5	electrocatalytic	electrocatalytic	ADJ
cet-15373	59	6	tests	test	NOUN
cet-15373	59	7	were	be	AUX
cet-15373	59	8	conducted	conduct	VERB
cet-15373	59	9	using	use	VERB
cet-15373	59	10	a	a	DET
cet-15373	59	11	gas	gas	NOUN
cet-15373	59	12	-	-	PUNCT
cet-15373	59	13	phase	phase	NOUN
cet-15373	59	14	cell	cell	NOUN
cet-15373	59	15	reactor	reactor	NOUN
cet-15373	59	16	(	(	PUNCT
cet-15373	59	17	refer	refer	VERB
cet-15373	59	18	to	to	PART
cet-15373	59	19	figure	figure	VERB
cet-15373	59	20	1	1	NUM
cet-15373	59	21	)	)	PUNCT
cet-15373	59	22	.	.	PUNCT
cet-15373	60	1	the	the	DET
cet-15373	60	2	flow	flow	NOUN
cet-15373	60	3	reactor	reactor	NOUN
cet-15373	60	4	operates	operate	VERB
cet-15373	60	5	under	under	ADP
cet-15373	60	6	room	room	NOUN
cet-15373	60	7	temperature	temperature	NOUN
cet-15373	60	8	and	and	CCONJ
cet-15373	60	9	atmospheric	atmospheric	ADJ
cet-15373	60	10	pressure	pressure	NOUN
cet-15373	60	11	.	.	PUNCT
cet-15373	61	1	the	the	DET
cet-15373	61	2	gas	gas	NOUN
cet-15373	61	3	-	-	PUNCT
cet-15373	61	4	phase	phase	NOUN
cet-15373	61	5	reactor	reactor	NOUN
cet-15373	61	6	consists	consist	VERB
cet-15373	61	7	of	of	ADP
cet-15373	61	8	i	i	PRON
cet-15373	61	9	)	)	PUNCT
cet-15373	61	10	a	a	DET
cet-15373	61	11	cathode	cathode	NOUN
cet-15373	61	12	compartment	compartment	NOUN
cet-15373	61	13	made	make	VERB
cet-15373	61	14	of	of	ADP
cet-15373	61	15	a	a	DET
cet-15373	61	16	gas	gas	NOUN
cet-15373	61	17	-	-	PUNCT
cet-15373	61	18	chamber	chamber	NOUN
cet-15373	61	19	in	in	ADP
cet-15373	61	20	which	which	PRON
cet-15373	61	21	the	the	DET
cet-15373	61	22	n2	n2	NOUN
cet-15373	61	23	flows	flow	VERB
cet-15373	61	24	through	through	ADP
cet-15373	61	25	the	the	DET
cet-15373	61	26	gdl	gdl	NOUN
cet-15373	61	27	,	,	PUNCT
cet-15373	61	28	ii	ii	PROPN
cet-15373	61	29	)	)	PUNCT
cet-15373	61	30	the	the	DET
cet-15373	61	31	deposited	deposit	VERB
cet-15373	61	32	catalyst	catalyst	NOUN
cet-15373	61	33	and	and	CCONJ
cet-15373	61	34	iii	iii	X
cet-15373	61	35	)	)	PUNCT
cet-15373	61	36	the	the	DET
cet-15373	61	37	proton	proton	NOUN
cet-15373	61	38	-	-	PUNCT
cet-15373	61	39	exchange	exchange	NOUN
cet-15373	61	40	membrane	membrane	NOUN
cet-15373	61	41	(	(	PUNCT
cet-15373	61	42	nafion	nafion	NOUN
cet-15373	61	43	®	®	NOUN
cet-15373	61	44	115	115	NUM
cet-15373	61	45	)	)	PUNCT
cet-15373	61	46	,	,	PUNCT
cet-15373	61	47	assembled	assemble	VERB
cet-15373	61	48	to	to	PART
cet-15373	61	49	form	form	VERB
cet-15373	61	50	the	the	DET
cet-15373	61	51	mea	mea	NOUN
cet-15373	61	52	(	(	PUNCT
cet-15373	61	53	see	see	VERB
cet-15373	61	54	figure	figure	NOUN
cet-15373	61	55	1	1	NUM
cet-15373	61	56	)	)	PUNCT
cet-15373	61	57	to	to	PART
cet-15373	61	58	form	form	VERB
cet-15373	61	59	the	the	DET
cet-15373	61	60	working	work	VERB
cet-15373	61	61	electrode	electrode	NOUN
cet-15373	61	62	(	(	PUNCT
cet-15373	61	63	we	we	PRON
cet-15373	61	64	)	)	PUNCT
cet-15373	61	65	.	.	PUNCT
cet-15373	62	1	the	the	DET
cet-15373	62	2	n2	n2	NOUN
cet-15373	62	3	adsorbs	adsorb	VERB
cet-15373	62	4	on	on	ADP
cet-15373	62	5	the	the	DET
cet-15373	62	6	catalyst	catalyst	NOUN
cet-15373	62	7	surface	surface	NOUN
cet-15373	62	8	and	and	CCONJ
cet-15373	62	9	reacts	react	VERB
cet-15373	62	10	with	with	ADP
cet-15373	62	11	the	the	DET
cet-15373	62	12	protons	proton	NOUN
cet-15373	62	13	diffusing	diffuse	VERB
cet-15373	62	14	from	from	ADP
cet-15373	62	15	the	the	DET
cet-15373	62	16	protonexchange	protonexchange	ADJ
cet-15373	62	17	membrane	membrane	NOUN
cet-15373	62	18	(	(	PUNCT
cet-15373	62	19	tavella	tavella	NOUN
cet-15373	62	20	et	et	PROPN
cet-15373	62	21	al	al	PROPN
cet-15373	62	22	.	.	PROPN
cet-15373	62	23	,	,	PUNCT
cet-15373	62	24	2022	2022	NUM
cet-15373	62	25	)	)	PUNCT
cet-15373	62	26	.	.	PUNCT
cet-15373	63	1	the	the	DET
cet-15373	63	2	membrane	membrane	NOUN
cet-15373	63	3	guarantees	guarantee	VERB
cet-15373	63	4	separation	separation	NOUN
cet-15373	63	5	with	with	ADP
cet-15373	63	6	the	the	DET
cet-15373	63	7	anodic	anodic	ADJ
cet-15373	63	8	compartment	compartment	NOUN
cet-15373	63	9	filled	fill	VERB
cet-15373	63	10	with	with	ADP
cet-15373	63	11	n2	n2	ADJ
cet-15373	63	12	-	-	PUNCT
cet-15373	63	13	saturated	saturate	VERB
cet-15373	63	14	na2so4	na2so4	NOUN
cet-15373	63	15	aqueous	aqueous	ADJ
cet-15373	63	16	solution	solution	NOUN
cet-15373	63	17	,	,	PUNCT
cet-15373	63	18	in	in	ADP
cet-15373	63	19	which	which	PRON
cet-15373	63	20	a	a	DET
cet-15373	63	21	commercial	commercial	ADJ
cet-15373	63	22	pt	pt	NOUN
cet-15373	63	23	electrode	electrode	NOUN
cet-15373	63	24	acts	act	VERB
cet-15373	63	25	as	as	ADP
cet-15373	63	26	a	a	DET
cet-15373	63	27	counter	counter	ADJ
cet-15373	63	28	electrode	electrode	NOUN
cet-15373	63	29	(	(	PUNCT
cet-15373	63	30	ce	ce	PROPN
cet-15373	63	31	)	)	PUNCT
cet-15373	63	32	and	and	CCONJ
cet-15373	63	33	ag	ag	PROPN
cet-15373	63	34	/	/	SYM
cet-15373	63	35	agcl	agcl	NOUN
cet-15373	63	36	(	(	PUNCT
cet-15373	63	37	3.0	3.0	NUM
cet-15373	63	38	m	m	NOUN
cet-15373	63	39	kcl	kcl	NOUN
cet-15373	63	40	)	)	PUNCT
cet-15373	63	41	electrode	electrode	NOUN
cet-15373	63	42	as	as	ADP
cet-15373	63	43	the	the	DET
cet-15373	63	44	reference	reference	NOUN
cet-15373	63	45	(	(	PUNCT
cet-15373	63	46	re	re	NOUN
cet-15373	63	47	)	)	PUNCT
cet-15373	63	48	.	.	PUNCT
cet-15373	64	1	the	the	DET
cet-15373	64	2	gas	gas	NOUN
cet-15373	64	3	products	product	NOUN
cet-15373	64	4	diffuse	diffuse	VERB
cet-15373	64	5	back	back	ADV
cet-15373	64	6	into	into	ADP
cet-15373	64	7	the	the	DET
cet-15373	64	8	gas	gas	NOUN
cet-15373	64	9	chamber	chamber	NOUN
cet-15373	64	10	and	and	CCONJ
cet-15373	64	11	are	be	AUX
cet-15373	64	12	absorbed	absorb	VERB
cet-15373	64	13	in	in	ADP
cet-15373	64	14	a	a	DET
cet-15373	64	15	dilute	dilute	NOUN
cet-15373	64	16	solution	solution	NOUN
cet-15373	64	17	of	of	ADP
cet-15373	64	18	sulfuric	sulfuric	ADJ
cet-15373	64	19	acid	acid	NOUN
cet-15373	64	20	(	(	PUNCT
cet-15373	64	21	0.001	0.001	NUM
cet-15373	64	22	m	m	NOUN
cet-15373	64	23	)	)	PUNCT
cet-15373	64	24	that	that	PRON
cet-15373	64	25	acts	act	VERB
cet-15373	64	26	as	as	ADP
cet-15373	64	27	a	a	DET
cet-15373	64	28	trap	trap	NOUN
cet-15373	64	29	for	for	ADP
cet-15373	64	30	the	the	DET
cet-15373	64	31	produced	produce	VERB
cet-15373	64	32	nh3	nh3	NOUN
cet-15373	64	33	.	.	PUNCT
cet-15373	65	1	at	at	ADP
cet-15373	65	2	the	the	DET
cet-15373	65	3	end	end	NOUN
cet-15373	65	4	of	of	ADP
cet-15373	65	5	the	the	DET
cet-15373	65	6	test	test	NOUN
cet-15373	65	7	,	,	PUNCT
cet-15373	65	8	the	the	DET
cet-15373	65	9	trap	trap	NOUN
cet-15373	65	10	solution	solution	NOUN
cet-15373	65	11	was	be	AUX
cet-15373	65	12	analysed	analyse	VERB
cet-15373	65	13	using	use	VERB
cet-15373	65	14	the	the	DET
cet-15373	65	15	ion	ion	NOUN
cet-15373	65	16	chromatography	chromatography	NOUN
cet-15373	65	17	(	(	PUNCT
cet-15373	65	18	ic	ic	PROPN
cet-15373	65	19	,	,	PUNCT
cet-15373	65	20	cationic	cationic	ADJ
cet-15373	65	21	column	column	NOUN
cet-15373	65	22	)	)	PUNCT
cet-15373	65	23	,	,	PUNCT
cet-15373	65	24	and	and	CCONJ
cet-15373	65	25	the	the	DET
cet-15373	65	26	electrolyte	electrolyte	NOUN
cet-15373	65	27	was	be	AUX
cet-15373	65	28	analysed	analyse	VERB
cet-15373	65	29	using	use	VERB
cet-15373	65	30	the	the	DET
cet-15373	65	31	salicylic	salicylic	ADJ
cet-15373	65	32	method	method	NOUN
cet-15373	65	33	(	(	PUNCT
cet-15373	65	34	uv	uv	NOUN
cet-15373	65	35	-	-	PUNCT
cet-15373	65	36	vis	vis	X
cet-15373	65	37	,	,	PUNCT
cet-15373	65	38	jasco	jasco	PROPN
cet-15373	65	39	570	570	NUM
cet-15373	65	40	)	)	PUNCT
cet-15373	65	41	.	.	PUNCT
cet-15373	66	1	a	a	DET
cet-15373	66	2	)	)	PUNCT
cet-15373	66	3	b	b	NOUN
cet-15373	66	4	)	)	PUNCT
cet-15373	66	5	figure	figure	NOUN
cet-15373	66	6	1	1	NUM
cet-15373	66	7	:	:	PUNCT
cet-15373	66	8	a	a	X
cet-15373	66	9	)	)	PUNCT
cet-15373	66	10	gas	gas	NOUN
cet-15373	66	11	-	-	PUNCT
cet-15373	66	12	phase	phase	NOUN
cet-15373	66	13	assembly	assembly	NOUN
cet-15373	66	14	.	.	PUNCT
cet-15373	67	1	black	black	ADJ
cet-15373	67	2	,	,	PUNCT
cet-15373	67	3	orange	orange	ADJ
cet-15373	67	4	,	,	PUNCT
cet-15373	67	5	and	and	CCONJ
cet-15373	67	6	yellow	yellow	ADJ
cet-15373	67	7	circles	circle	NOUN
cet-15373	67	8	refer	refer	VERB
cet-15373	67	9	to	to	ADP
cet-15373	67	10	gdl	gdl	NOUN
cet-15373	67	11	,	,	PUNCT
cet-15373	67	12	catalyst	catalyst	NOUN
cet-15373	67	13	,	,	PUNCT
cet-15373	67	14	and	and	CCONJ
cet-15373	67	15	membrane	membrane	NOUN
cet-15373	67	16	,	,	PUNCT
cet-15373	67	17	respectively	respectively	ADV
cet-15373	67	18	,	,	PUNCT
cet-15373	67	19	and	and	CCONJ
cet-15373	67	20	b	b	X
cet-15373	67	21	)	)	PUNCT
cet-15373	67	22	exploded	explode	VERB
cet-15373	67	23	depiction	depiction	NOUN
cet-15373	67	24	of	of	ADP
cet-15373	67	25	the	the	DET
cet-15373	67	26	cell	cell	NOUN
cet-15373	67	27	.	.	PUNCT
cet-15373	68	1	735	735	NUM
cet-15373	68	2	3	3	NUM
cet-15373	68	3	.	.	NOUN
cet-15373	68	4	results	result	NOUN
cet-15373	68	5	and	and	CCONJ
cet-15373	68	6	discussion	discussion	NOUN
cet-15373	68	7	3.1	3.1	NUM
cet-15373	68	8	x	x	NOUN
cet-15373	68	9	-	-	NOUN
cet-15373	68	10	ray	ray	NOUN
cet-15373	68	11	diffraction	diffraction	NOUN
cet-15373	68	12	(	(	PUNCT
cet-15373	68	13	xrd	xrd	NOUN
cet-15373	68	14	)	)	PUNCT
cet-15373	68	15	analysis	analysis	NOUN
cet-15373	68	16	figure	figure	NOUN
cet-15373	68	17	2	2	NUM
cet-15373	68	18	:	:	PUNCT
cet-15373	68	19	xrd	xrd	NOUN
cet-15373	68	20	patterns	pattern	NOUN
cet-15373	68	21	for	for	ADP
cet-15373	68	22	a	a	DET
cet-15373	68	23	)	)	PUNCT
cet-15373	68	24	al2o3	al2o3	NOUN
cet-15373	68	25	-	-	PUNCT
cet-15373	68	26	based	base	VERB
cet-15373	68	27	catalysts	catalyst	NOUN
cet-15373	68	28	and	and	CCONJ
cet-15373	68	29	b	b	X
cet-15373	68	30	)	)	PUNCT
cet-15373	68	31	cnts	cnts	PROPN
cet-15373	68	32	-	-	PUNCT
cet-15373	68	33	based	base	VERB
cet-15373	68	34	catalysts	catalyst	NOUN
cet-15373	68	35	.	.	PUNCT
cet-15373	69	1	in	in	ADP
cet-15373	69	2	figure	figure	NOUN
cet-15373	69	3	(	(	PUNCT
cet-15373	69	4	■	■	NOUN
cet-15373	69	5	)	)	PUNCT
cet-15373	69	6	ruthenium	ruthenium	NOUN
cet-15373	69	7	,	,	PUNCT
cet-15373	69	8	(	(	PUNCT
cet-15373	69	9	●	●	NOUN
cet-15373	69	10	)	)	PUNCT
cet-15373	69	11	fe2o3	fe2o3	PROPN
cet-15373	69	12	,	,	PUNCT
cet-15373	69	13	(	(	PUNCT
cet-15373	69	14	▲	▲	PUNCT
cet-15373	69	15	)	)	PUNCT
cet-15373	69	16	al2o3	al2o3	PROPN
cet-15373	69	17	and	and	CCONJ
cet-15373	69	18	(	(	PUNCT
cet-15373	69	19	▼	▼	NOUN
cet-15373	69	20	)	)	PUNCT
cet-15373	69	21	cnts	cnt	NOUN
cet-15373	69	22	respectively	respectively	ADV
cet-15373	69	23	.	.	PUNCT
cet-15373	70	1	figure	figure	NOUN
cet-15373	70	2	2a	2a	PROPN
cet-15373	70	3	shows	show	VERB
cet-15373	70	4	the	the	DET
cet-15373	70	5	alumina	alumina	NOUN
cet-15373	70	6	-	-	PUNCT
cet-15373	70	7	based	base	VERB
cet-15373	70	8	catalysts	catalyst	NOUN
cet-15373	70	9	.	.	PUNCT
cet-15373	71	1	the	the	DET
cet-15373	71	2	diffraction	diffraction	NOUN
cet-15373	71	3	peaks	peak	NOUN
cet-15373	71	4	at	at	ADP
cet-15373	71	5	2θ	2θ	NUM
cet-15373	71	6	=	=	SYM
cet-15373	71	7	25.58	25.58	NUM
cet-15373	71	8	,	,	PUNCT
cet-15373	71	9	35.16	35.16	NUM
cet-15373	71	10	,	,	PUNCT
cet-15373	71	11	37.78	37.78	NUM
cet-15373	71	12	,	,	PUNCT
cet-15373	71	13	43.36	43.36	NUM
cet-15373	71	14	,	,	PUNCT
cet-15373	71	15	52.56	52.56	NUM
cet-15373	71	16	,	,	PUNCT
cet-15373	71	17	57.51	57.51	NUM
cet-15373	71	18	,	,	PUNCT
cet-15373	71	19	59.75	59.75	NUM
cet-15373	71	20	,	,	PUNCT
cet-15373	71	21	61.32	61.32	NUM
cet-15373	71	22	,	,	PUNCT
cet-15373	71	23	66.53	66.53	NUM
cet-15373	71	24	,	,	PUNCT
cet-15373	71	25	68.22	68.22	NUM
cet-15373	71	26	,	,	PUNCT
cet-15373	71	27	70.43	70.43	NUM
cet-15373	71	28	,	,	PUNCT
cet-15373	71	29	74.32	74.32	NUM
cet-15373	71	30	,	,	PUNCT
cet-15373	71	31	76.89	76.89	NUM
cet-15373	71	32	,	,	PUNCT
cet-15373	71	33	77.25	77.25	NUM
cet-15373	71	34	are	be	AUX
cet-15373	71	35	related	relate	VERB
cet-15373	71	36	to	to	ADP
cet-15373	71	37	-al2o3	-al2o3	PROPN
cet-15373	71	38	(	(	PUNCT
cet-15373	71	39	international	international	ADJ
cet-15373	71	40	center	center	NOUN
cet-15373	71	41	of	of	ADP
cet-15373	71	42	diffraction	diffraction	NOUN
cet-15373	71	43	data	datum	NOUN
cet-15373	71	44	-icddof	-icddof	PROPN
cet-15373	71	45	card	card	NOUN
cet-15373	71	46	number	number	NOUN
cet-15373	71	47	00–010–0173	00–010–0173	PROPN
cet-15373	71	48	of	of	ADP
cet-15373	71	49	αal2o3	αal2o3	PROPN
cet-15373	71	50	)	)	PUNCT
cet-15373	71	51	corresponding	correspond	VERB
cet-15373	71	52	to	to	ADP
cet-15373	71	53	the	the	DET
cet-15373	71	54	(	(	PUNCT
cet-15373	71	55	0	0	NUM
cet-15373	71	56	1	1	NUM
cet-15373	71	57	2	2	NUM
cet-15373	71	58	)	)	PUNCT
cet-15373	71	59	,	,	PUNCT
cet-15373	71	60	(	(	PUNCT
cet-15373	71	61	1	1	NUM
cet-15373	71	62	0	0	NUM
cet-15373	71	63	4	4	NUM
cet-15373	71	64	)	)	PUNCT
cet-15373	71	65	,	,	PUNCT
cet-15373	71	66	(	(	PUNCT
cet-15373	71	67	1	1	NUM
cet-15373	71	68	1	1	NUM
cet-15373	71	69	0	0	NUM
cet-15373	71	70	)	)	PUNCT
cet-15373	71	71	,	,	PUNCT
cet-15373	71	72	(	(	PUNCT
cet-15373	71	73	1	1	NUM
cet-15373	71	74	1	1	NUM
cet-15373	71	75	3	3	NUM
cet-15373	71	76	)	)	PUNCT
cet-15373	71	77	,	,	PUNCT
cet-15373	71	78	(	(	PUNCT
cet-15373	71	79	0	0	NUM
cet-15373	71	80	2	2	NUM
cet-15373	71	81	4	4	NUM
cet-15373	71	82	)	)	PUNCT
cet-15373	71	83	,	,	PUNCT
cet-15373	71	84	(	(	PUNCT
cet-15373	71	85	1	1	NUM
cet-15373	71	86	1	1	NUM
cet-15373	71	87	6	6	NUM
cet-15373	71	88	)	)	PUNCT
cet-15373	71	89	,	,	PUNCT
cet-15373	71	90	(	(	PUNCT
cet-15373	71	91	2	2	NUM
cet-15373	71	92	1	1	NUM
cet-15373	71	93	1	1	NUM
cet-15373	71	94	)	)	PUNCT
cet-15373	71	95	,	,	PUNCT
cet-15373	71	96	(	(	PUNCT
cet-15373	71	97	0	0	NUM
cet-15373	71	98	1	1	NUM
cet-15373	71	99	8)	8)	NUM
cet-15373	71	100	,	,	PUNCT
cet-15373	71	101	(	(	PUNCT
cet-15373	71	102	2	2	NUM
cet-15373	71	103	1	1	NUM
cet-15373	71	104	4	4	NUM
cet-15373	71	105	)	)	PUNCT
cet-15373	71	106	,	,	PUNCT
cet-15373	71	107	(	(	PUNCT
cet-15373	71	108	3	3	NUM
cet-15373	71	109	0	0	NUM
cet-15373	71	110	0	0	NUM
cet-15373	71	111	)	)	PUNCT
cet-15373	71	112	,	,	PUNCT
cet-15373	71	113	(	(	PUNCT
cet-15373	71	114	1	1	NUM
cet-15373	71	115	2	2	NUM
cet-15373	71	116	5	5	NUM
cet-15373	71	117	)	)	PUNCT
cet-15373	71	118	,	,	PUNCT
cet-15373	71	119	(	(	PUNCT
cet-15373	71	120	2	2	NUM
cet-15373	71	121	0	0	NUM
cet-15373	71	122	8)	8)	NUM
cet-15373	71	123	,	,	PUNCT
cet-15373	71	124	(	(	PUNCT
cet-15373	71	125	1	1	NUM
cet-15373	71	126	0	0	NUM
cet-15373	71	127	10	10	NUM
cet-15373	71	128	)	)	PUNCT
cet-15373	71	129	and	and	CCONJ
cet-15373	71	130	(	(	PUNCT
cet-15373	71	131	1	1	NUM
cet-15373	71	132	1	1	NUM
cet-15373	71	133	9	9	NUM
cet-15373	71	134	)	)	PUNCT
cet-15373	71	135	planes	plane	NOUN
cet-15373	71	136	,	,	PUNCT
cet-15373	71	137	respectively	respectively	ADV
cet-15373	71	138	(	(	PUNCT
cet-15373	71	139	green	green	ADJ
cet-15373	71	140	line	line	NOUN
cet-15373	71	141	in	in	ADP
cet-15373	71	142	figure	figure	NOUN
cet-15373	71	143	2a	2a	NUM
cet-15373	71	144	)	)	PUNCT
cet-15373	71	145	.	.	PUNCT
cet-15373	72	1	diffraction	diffraction	NOUN
cet-15373	72	2	peaks	peak	NOUN
cet-15373	72	3	at	at	ADP
cet-15373	72	4	2θ	2θ	NUM
cet-15373	72	5	=	=	SYM
cet-15373	72	6	38.41	38.41	NUM
cet-15373	72	7	,	,	PUNCT
cet-15373	72	8	42.18	42.18	NUM
cet-15373	72	9	,	,	PUNCT
cet-15373	72	10	44.04	44.04	NUM
cet-15373	72	11	,	,	PUNCT
cet-15373	72	12	58.36	58.36	NUM
cet-15373	72	13	,	,	PUNCT
cet-15373	72	14	69.47	69.47	NUM
cet-15373	72	15	,	,	PUNCT
cet-15373	72	16	78.41	78.41	NUM
cet-15373	72	17	,	,	PUNCT
cet-15373	72	18	for	for	ADP
cet-15373	72	19	ruthenium	ruthenium	NOUN
cet-15373	72	20	(	(	PUNCT
cet-15373	72	21	jcpds	jcpds	PROPN
cet-15373	72	22	card	card	NOUN
cet-15373	72	23	no	no	INTJ
cet-15373	72	24	.	.	NOUN
cet-15373	72	25	89	89	NUM
cet-15373	72	26	-	-	SYM
cet-15373	72	27	3942	3942	NUM
cet-15373	72	28	)	)	PUNCT
cet-15373	72	29	correspond	correspond	VERB
cet-15373	72	30	to	to	ADP
cet-15373	72	31	the	the	DET
cet-15373	72	32	(	(	PUNCT
cet-15373	72	33	1	1	NUM
cet-15373	72	34	0	0	NUM
cet-15373	72	35	0	0	NUM
cet-15373	72	36	)	)	PUNCT
cet-15373	72	37	,	,	PUNCT
cet-15373	72	38	(	(	PUNCT
cet-15373	72	39	0	0	NUM
cet-15373	72	40	0	0	NUM
cet-15373	72	41	2	2	NUM
cet-15373	72	42	)	)	PUNCT
cet-15373	72	43	,	,	PUNCT
cet-15373	72	44	(	(	PUNCT
cet-15373	72	45	1	1	NUM
cet-15373	72	46	0	0	NUM
cet-15373	72	47	1	1	NUM
cet-15373	72	48	)	)	PUNCT
cet-15373	72	49	,	,	PUNCT
cet-15373	72	50	(	(	PUNCT
cet-15373	72	51	1	1	NUM
cet-15373	72	52	0	0	NUM
cet-15373	72	53	2	2	NUM
cet-15373	72	54	)	)	PUNCT
cet-15373	72	55	,	,	PUNCT
cet-15373	72	56	(	(	PUNCT
cet-15373	72	57	1	1	NUM
cet-15373	72	58	1	1	NUM
cet-15373	72	59	0	0	NUM
cet-15373	72	60	)	)	PUNCT
cet-15373	72	61	and	and	CCONJ
cet-15373	72	62	(	(	PUNCT
cet-15373	72	63	1	1	NUM
cet-15373	72	64	0	0	NUM
cet-15373	72	65	3	3	NUM
cet-15373	72	66	)	)	PUNCT
cet-15373	72	67	planes	plane	NOUN
cet-15373	72	68	,	,	PUNCT
cet-15373	72	69	respectively	respectively	ADV
cet-15373	72	70	(	(	PUNCT
cet-15373	72	71	black	black	ADJ
cet-15373	72	72	line	line	NOUN
cet-15373	72	73	in	in	ADP
cet-15373	72	74	figure	figure	NOUN
cet-15373	72	75	2a	2a	NUM
cet-15373	72	76	)	)	PUNCT
cet-15373	72	77	.	.	PUNCT
cet-15373	73	1	fe2o3	fe2o3	PROPN
cet-15373	73	2	and	and	CCONJ
cet-15373	73	3	ru	ru	PROPN
cet-15373	73	4	-	-	PUNCT
cet-15373	73	5	fe	fe	NOUN
cet-15373	73	6	are	be	AUX
cet-15373	73	7	not	not	PART
cet-15373	73	8	detectable	detectable	ADJ
cet-15373	73	9	from	from	ADP
cet-15373	73	10	xrd	xrd	NOUN
cet-15373	73	11	but	but	CCONJ
cet-15373	73	12	are	be	AUX
cet-15373	73	13	confirmed	confirm	VERB
cet-15373	73	14	by	by	ADP
cet-15373	73	15	energy	energy	NOUN
cet-15373	73	16	dispersive	dispersive	ADJ
cet-15373	73	17	x	x	NOUN
cet-15373	73	18	-	-	NOUN
cet-15373	73	19	ray	ray	NOUN
cet-15373	73	20	(	(	PUNCT
cet-15373	73	21	edx	edx	PROPN
cet-15373	73	22	)	)	PUNCT
cet-15373	73	23	analysis	analysis	NOUN
cet-15373	73	24	.	.	PUNCT
cet-15373	74	1	figure	figure	NOUN
cet-15373	74	2	2b	2b	NOUN
cet-15373	74	3	,	,	PUNCT
cet-15373	74	4	shows	show	VERB
cet-15373	74	5	the	the	DET
cet-15373	74	6	cnts	cnts	PROPN
cet-15373	74	7	-	-	PUNCT
cet-15373	74	8	based	base	VERB
cet-15373	74	9	catalyst	catalyst	NOUN
cet-15373	74	10	.	.	PUNCT
cet-15373	75	1	cnts	cnts	PROPN
cet-15373	75	2	characteristic	characteristic	ADJ
cet-15373	75	3	peaks	peak	NOUN
cet-15373	75	4	at	at	ADP
cet-15373	75	5	2θ	2θ	NUM
cet-15373	75	6	=	=	SYM
cet-15373	75	7	26	26	NUM
cet-15373	75	8	,	,	PUNCT
cet-15373	75	9	42	42	NUM
cet-15373	75	10	,	,	PUNCT
cet-15373	75	11	and	and	CCONJ
cet-15373	75	12	48	48	NUM
cet-15373	75	13	are	be	AUX
cet-15373	75	14	related	relate	VERB
cet-15373	75	15	to	to	ADP
cet-15373	75	16	(	(	PUNCT
cet-15373	75	17	0	0	NUM
cet-15373	75	18	0	0	NUM
cet-15373	75	19	2	2	NUM
cet-15373	75	20	)	)	PUNCT
cet-15373	75	21	,	,	PUNCT
cet-15373	75	22	(	(	PUNCT
cet-15373	75	23	1	1	NUM
cet-15373	75	24	0	0	NUM
cet-15373	75	25	0	0	NUM
cet-15373	75	26	)	)	PUNCT
cet-15373	75	27	,	,	PUNCT
cet-15373	75	28	and	and	CCONJ
cet-15373	75	29	(	(	PUNCT
cet-15373	75	30	1	1	NUM
cet-15373	75	31	0	0	NUM
cet-15373	75	32	1	1	NUM
cet-15373	75	33	)	)	PUNCT
cet-15373	75	34	planes	plane	NOUN
cet-15373	75	35	,	,	PUNCT
cet-15373	75	36	respectively	respectively	ADV
cet-15373	75	37	.	.	PUNCT
cet-15373	76	1	for	for	ADP
cet-15373	76	2	fe2o3	fe2o3	PROPN
cet-15373	76	3	,	,	PUNCT
cet-15373	76	4	it	it	PRON
cet-15373	76	5	can	can	AUX
cet-15373	76	6	be	be	AUX
cet-15373	76	7	observed	observe	VERB
cet-15373	76	8	the	the	DET
cet-15373	76	9	peaks	peak	NOUN
cet-15373	76	10	at	at	ADP
cet-15373	76	11	2θ	2θ	NUM
cet-15373	76	12	=	=	NUM
cet-15373	76	13	30.3	30.3	NUM
cet-15373	76	14	,	,	PUNCT
cet-15373	76	15	35.6	35.6	NUM
cet-15373	76	16	,	,	PUNCT
cet-15373	76	17	43.3	43.3	NUM
cet-15373	76	18	,	,	PUNCT
cet-15373	76	19	53.8	53.8	NUM
cet-15373	76	20	,	,	PUNCT
cet-15373	76	21	57.1	57.1	NUM
cet-15373	76	22	and	and	CCONJ
cet-15373	76	23	62.8	62.8	NUM
cet-15373	76	24	,	,	PUNCT
cet-15373	76	25	corresponding	correspond	VERB
cet-15373	76	26	to	to	ADP
cet-15373	76	27	(	(	PUNCT
cet-15373	76	28	2	2	NUM
cet-15373	76	29	2	2	NUM
cet-15373	76	30	0	0	NUM
cet-15373	76	31	)	)	PUNCT
cet-15373	76	32	,	,	PUNCT
cet-15373	76	33	(	(	PUNCT
cet-15373	76	34	3	3	NUM
cet-15373	76	35	1	1	NUM
cet-15373	76	36	1	1	NUM
cet-15373	76	37	)	)	PUNCT
cet-15373	76	38	,	,	PUNCT
cet-15373	76	39	(	(	PUNCT
cet-15373	76	40	4	4	NUM
cet-15373	76	41	0	0	NUM
cet-15373	76	42	0	0	NUM
cet-15373	76	43	)	)	PUNCT
cet-15373	76	44	,	,	PUNCT
cet-15373	76	45	(	(	PUNCT
cet-15373	76	46	4	4	NUM
cet-15373	76	47	2	2	NUM
cet-15373	76	48	2	2	NUM
cet-15373	76	49	)	)	PUNCT
cet-15373	76	50	,	,	PUNCT
cet-15373	76	51	(	(	PUNCT
cet-15373	76	52	5	5	NUM
cet-15373	76	53	1	1	NUM
cet-15373	76	54	1	1	NUM
cet-15373	76	55	)	)	PUNCT
cet-15373	76	56	and	and	CCONJ
cet-15373	76	57	(	(	PUNCT
cet-15373	76	58	4	4	NUM
cet-15373	76	59	4	4	NUM
cet-15373	76	60	0	0	NUM
cet-15373	76	61	)	)	PUNCT
cet-15373	76	62	planes	plane	NOUN
cet-15373	76	63	(	(	PUNCT
cet-15373	76	64	blue	blue	ADJ
cet-15373	76	65	line	line	NOUN
cet-15373	76	66	in	in	ADP
cet-15373	76	67	figure	figure	NOUN
cet-15373	76	68	2b	2b	NOUN
cet-15373	76	69	)	)	PUNCT
cet-15373	76	70	,	,	PUNCT
cet-15373	76	71	confirming	confirm	VERB
cet-15373	76	72	the	the	DET
cet-15373	76	73	presence	presence	NOUN
cet-15373	76	74	of	of	ADP
cet-15373	76	75	γfe2o3	γfe2o3	NOUN
cet-15373	76	76	phase	phase	NOUN
cet-15373	76	77	(	(	PUNCT
cet-15373	76	78	shaoo	shaoo	VERB
cet-15373	76	79	et	et	PROPN
cet-15373	76	80	al	al	PROPN
cet-15373	76	81	.	.	PROPN
cet-15373	76	82	,	,	PUNCT
cet-15373	76	83	2010	2010	NUM
cet-15373	76	84	)	)	PUNCT
cet-15373	76	85	.	.	PUNCT
cet-15373	77	1	in	in	ADP
cet-15373	77	2	addition	addition	NOUN
cet-15373	77	3	to	to	ADP
cet-15373	77	4	the	the	DET
cet-15373	77	5	ruthenium	ruthenium	NOUN
cet-15373	77	6	spectra	spectra	NOUN
cet-15373	77	7	already	already	ADV
cet-15373	77	8	mentioned	mention	VERB
cet-15373	77	9	above	above	ADV
cet-15373	77	10	,	,	PUNCT
cet-15373	77	11	three	three	NUM
cet-15373	77	12	extra	extra	ADJ
cet-15373	77	13	peaks	peak	NOUN
cet-15373	77	14	exist	exist	VERB
cet-15373	77	15	at	at	ADP
cet-15373	77	16	2θ	2θ	NUM
cet-15373	77	17	=	=	SYM
cet-15373	77	18	82.28	82.28	NUM
cet-15373	77	19	,	,	PUNCT
cet-15373	77	20	84.73	84.73	NUM
cet-15373	77	21	and	and	CCONJ
cet-15373	77	22	86.01	86.01	NUM
cet-15373	77	23	,	,	PUNCT
cet-15373	77	24	corresponding	correspond	VERB
cet-15373	77	25	to	to	ADP
cet-15373	77	26	(	(	PUNCT
cet-15373	77	27	2	2	NUM
cet-15373	77	28	0	0	NUM
cet-15373	77	29	0	0	NUM
cet-15373	77	30	)	)	PUNCT
cet-15373	77	31	,	,	PUNCT
cet-15373	77	32	(	(	PUNCT
cet-15373	77	33	1	1	NUM
cet-15373	77	34	1	1	NUM
cet-15373	77	35	2	2	NUM
cet-15373	77	36	)	)	PUNCT
cet-15373	77	37	and	and	CCONJ
cet-15373	77	38	(	(	PUNCT
cet-15373	77	39	2	2	NUM
cet-15373	77	40	0	0	NUM
cet-15373	77	41	1	1	NUM
cet-15373	77	42	)	)	PUNCT
cet-15373	77	43	planes	plane	NOUN
cet-15373	77	44	,	,	PUNCT
cet-15373	77	45	respectively	respectively	ADV
cet-15373	77	46	(	(	PUNCT
cet-15373	77	47	black	black	ADJ
cet-15373	77	48	line	line	NOUN
cet-15373	77	49	in	in	ADP
cet-15373	77	50	figure	figure	NOUN
cet-15373	77	51	2b	2b	NOUN
cet-15373	77	52	)	)	PUNCT
cet-15373	77	53	.	.	PUNCT
cet-15373	78	1	ru	ru	PROPN
cet-15373	78	2	-	-	PUNCT
cet-15373	78	3	fe	fe	NOUN
cet-15373	78	4	was	be	AUX
cet-15373	78	5	not	not	PART
cet-15373	78	6	detected	detect	VERB
cet-15373	78	7	by	by	ADP
cet-15373	78	8	xrd	xrd	NOUN
cet-15373	78	9	but	but	CCONJ
cet-15373	78	10	was	be	AUX
cet-15373	78	11	confirmed	confirm	VERB
cet-15373	78	12	through	through	ADP
cet-15373	78	13	energy	energy	NOUN
cet-15373	78	14	dispersive	dispersive	ADJ
cet-15373	78	15	x	x	NOUN
cet-15373	78	16	-	-	NOUN
cet-15373	78	17	ray	ray	NOUN
cet-15373	78	18	(	(	PUNCT
cet-15373	78	19	edx	edx	PROPN
cet-15373	78	20	)	)	PUNCT
cet-15373	78	21	analysis	analysis	NOUN
cet-15373	78	22	on	on	ADP
cet-15373	78	23	both	both	CCONJ
cet-15373	78	24	al2o3	al2o3	PROPN
cet-15373	78	25	and	and	CCONJ
cet-15373	78	26	cnts	cnts	PROPN
cet-15373	78	27	supports	support	VERB
cet-15373	78	28	as	as	SCONJ
cet-15373	78	29	shown	show	VERB
cet-15373	78	30	in	in	ADP
cet-15373	78	31	figure	figure	NOUN
cet-15373	78	32	3a	3a	NUM
cet-15373	78	33	and	and	CCONJ
cet-15373	78	34	3b	3b	NUM
cet-15373	78	35	,	,	PUNCT
cet-15373	78	36	respectively	respectively	ADV
cet-15373	78	37	.	.	PUNCT
cet-15373	79	1	figure	figure	NOUN
cet-15373	79	2	3	3	NUM
cet-15373	79	3	:	:	PUNCT
cet-15373	79	4	edx	edx	NOUN
cet-15373	79	5	pattern	pattern	NOUN
cet-15373	79	6	for	for	ADP
cet-15373	79	7	ruthenium	ruthenium	NOUN
cet-15373	79	8	-	-	PUNCT
cet-15373	79	9	iron	iron	NOUN
cet-15373	79	10	on	on	ADP
cet-15373	79	11	a	a	DET
cet-15373	79	12	)	)	PUNCT
cet-15373	79	13	al2o3	al2o3	PROPN
cet-15373	79	14	and	and	CCONJ
cet-15373	79	15	b	b	NOUN
cet-15373	79	16	)	)	PUNCT
cet-15373	79	17	cnts	cnt	NOUN
cet-15373	79	18	with	with	ADP
cet-15373	79	19	atomic	atomic	ADJ
cet-15373	79	20	percentage	percentage	NOUN
cet-15373	79	21	of	of	ADP
cet-15373	79	22	metals	metal	NOUN
cet-15373	79	23	.	.	PUNCT
cet-15373	80	1	3.2	3.2	NUM
cet-15373	80	2	n2	n2	ADJ
cet-15373	80	3	reduction	reduction	NOUN
cet-15373	80	4	tests	test	VERB
cet-15373	80	5	the	the	DET
cet-15373	80	6	al2o3	al2o3	PROPN
cet-15373	80	7	and	and	CCONJ
cet-15373	80	8	cnts	cnts	PROPN
cet-15373	80	9	-	-	PUNCT
cet-15373	80	10	based	base	VERB
cet-15373	80	11	electrodes	electrode	NOUN
cet-15373	80	12	were	be	AUX
cet-15373	80	13	tested	test	VERB
cet-15373	80	14	in	in	ADP
cet-15373	80	15	the	the	DET
cet-15373	80	16	gas	gas	NOUN
cet-15373	80	17	-	-	PUNCT
cet-15373	80	18	phase	phase	NOUN
cet-15373	80	19	system	system	NOUN
cet-15373	80	20	.	.	PUNCT
cet-15373	81	1	before	before	ADP
cet-15373	81	2	testing	testing	NOUN
cet-15373	81	3	,	,	PUNCT
cet-15373	81	4	a	a	DET
cet-15373	81	5	rigid	rigid	ADJ
cet-15373	81	6	electrochemical	electrochemical	ADJ
cet-15373	81	7	protocol	protocol	NOUN
cet-15373	81	8	was	be	AUX
cet-15373	81	9	performed	perform	VERB
cet-15373	81	10	,	,	PUNCT
cet-15373	81	11	consisting	consist	VERB
cet-15373	81	12	of	of	ADP
cet-15373	81	13	i	i	NOUN
cet-15373	81	14	)	)	PUNCT
cet-15373	81	15	decontamination	decontamination	NOUN
cet-15373	81	16	process	process	NOUN
cet-15373	81	17	and	and	CCONJ
cet-15373	81	18	ii	ii	NOUN
cet-15373	81	19	)	)	PUNCT
cet-15373	81	20	a	a	DET
cet-15373	81	21	chrono	chrono	NOUN
cet-15373	81	22	-	-	PUNCT
cet-15373	81	23	amperometry	amperometry	NOUN
cet-15373	81	24	(	(	PUNCT
cet-15373	81	25	ca	ca	NOUN
cet-15373	81	26	)	)	PUNCT
cet-15373	81	27	at	at	ADP
cet-15373	81	28	the	the	DET
cet-15373	81	29	desired	desire	VERB
cet-15373	81	30	set	set	NOUN
cet-15373	81	31	potential	potential	NOUN
cet-15373	81	32	.	.	PUNCT
cet-15373	82	1	the	the	DET
cet-15373	82	2	investigated	investigate	VERB
cet-15373	82	3	potentials	potential	NOUN
cet-15373	82	4	range	range	VERB
cet-15373	82	5	from	from	ADP
cet-15373	82	6	-0.1	-0.1	PROPN
cet-15373	82	7	to	to	ADP
cet-15373	82	8	-0.8	-0.8	PROPN
cet-15373	82	9	v	v	NOUN
cet-15373	82	10	vs.	vs.	ADP
cet-15373	82	11	rhe	rhe	NOUN
cet-15373	82	12	.	.	PUNCT
cet-15373	83	1	the	the	DET
cet-15373	83	2	selection	selection	NOUN
cet-15373	83	3	of	of	ADP
cet-15373	83	4	potential	potential	ADJ
cet-15373	83	5	increments	increment	NOUN
cet-15373	83	6	was	be	AUX
cet-15373	83	7	based	base	VERB
cet-15373	83	8	on	on	ADP
cet-15373	83	9	preliminary	preliminary	ADJ
cet-15373	83	10	tests	test	NOUN
cet-15373	83	11	,	,	PUNCT
cet-15373	83	12	in	in	ADP
cet-15373	83	13	order	order	NOUN
cet-15373	83	14	to	to	PART
cet-15373	83	15	operate	operate	VERB
cet-15373	83	16	at	at	ADP
cet-15373	83	17	optimal	optimal	ADJ
cet-15373	83	18	current	current	ADJ
cet-15373	83	19	densities	density	NOUN
cet-15373	83	20	from	from	ADP
cet-15373	83	21	100	100	NUM
cet-15373	83	22	to	to	ADP
cet-15373	83	23	-400	-400	PROPN
cet-15373	83	24	a	a	PROPN
cet-15373	83	25	cm-2	cm-2	NOUN
cet-15373	83	26	,	,	PUNCT
cet-15373	83	27	which	which	PRON
cet-15373	83	28	is	be	AUX
cet-15373	83	29	the	the	DET
cet-15373	83	30	range	range	NOUN
cet-15373	83	31	where	where	SCONJ
cet-15373	83	32	the	the	DET
cet-15373	83	33	onset	onset	NOUN
cet-15373	83	34	potential	potential	NOUN
cet-15373	83	35	of	of	ADP
cet-15373	83	36	the	the	DET
cet-15373	83	37	reaction	reaction	NOUN
cet-15373	83	38	occurs	occur	VERB
cet-15373	83	39	,	,	PUNCT
cet-15373	83	40	just	just	ADV
cet-15373	83	41	before	before	SCONJ
cet-15373	83	42	the	the	DET
cet-15373	83	43	hydrogen	hydrogen	NOUN
cet-15373	83	44	evolution	evolution	NOUN
cet-15373	83	45	reaction	reaction	NOUN
cet-15373	83	46	(	(	PUNCT
cet-15373	83	47	her	her	PRON
cet-15373	83	48	)	)	PUNCT
cet-15373	83	49	becomes	become	VERB
cet-15373	83	50	predominant	predominant	ADJ
cet-15373	83	51	.	.	PUNCT
cet-15373	84	1	the	the	DET
cet-15373	84	2	decontamination	decontamination	NOUN
cet-15373	84	3	process	process	NOUN
cet-15373	84	4	was	be	AUX
cet-15373	84	5	conducted	conduct	VERB
cet-15373	84	6	by	by	ADP
cet-15373	84	7	applying	apply	VERB
cet-15373	84	8	a	a	DET
cet-15373	84	9	low	low	ADJ
cet-15373	84	10	potential	potential	NOUN
cet-15373	84	11	(	(	PUNCT
cet-15373	84	12	-0.1	-0.1	PROPN
cet-15373	84	13	v	v	NOUN
cet-15373	84	14	vs	vs	ADP
cet-15373	84	15	rhe	rhe	NOUN
cet-15373	84	16	)	)	PUNCT
cet-15373	84	17	for	for	ADP
cet-15373	84	18	a	a	DET
cet-15373	84	19	duration	duration	NOUN
cet-15373	84	20	of	of	ADP
cet-15373	84	21	60	60	NUM
cet-15373	84	22	minutes	minute	NOUN
cet-15373	84	23	.	.	PUNCT
cet-15373	85	1	this	this	DET
cet-15373	85	2	procedure	procedure	NOUN
cet-15373	85	3	was	be	AUX
cet-15373	85	4	essential	essential	ADJ
cet-15373	85	5	for	for	ADP
cet-15373	85	6	the	the	DET
cet-15373	85	7	removal	removal	NOUN
cet-15373	85	8	of	of	ADP
cet-15373	85	9	any	any	DET
cet-15373	85	10	nitrogen	nitrogen	NOUN
cet-15373	85	11	contamination	contamination	NOUN
cet-15373	85	12	(	(	PUNCT
cet-15373	85	13	e.g.	e.g.	ADV
cet-15373	85	14	,	,	PUNCT
cet-15373	85	15	ammonia	ammonia	NOUN
cet-15373	85	16	or	or	CCONJ
cet-15373	85	17	other	other	ADJ
cet-15373	85	18	n	n	CCONJ
cet-15373	85	19	-	-	PUNCT
cet-15373	85	20	compounds	compound	NOUN
cet-15373	85	21	adhered	adhere	VERB
cet-15373	85	22	to	to	ADP
cet-15373	85	23	the	the	DET
cet-15373	85	24	electrode	electrode	NOUN
cet-15373	85	25	surface	surface	NOUN
cet-15373	85	26	during	during	ADP
cet-15373	85	27	deposition	deposition	NOUN
cet-15373	85	28	or	or	CCONJ
cet-15373	85	29	adsorbed	adsorb	VERB
cet-15373	85	30	to	to	ADP
cet-15373	85	31	the	the	DET
cet-15373	85	32	nafion	nafion	NOUN
cet-15373	85	33	membrane	membrane	NOUN
cet-15373	85	34	)	)	PUNCT
cet-15373	85	35	not	not	PART
cet-15373	85	36	originating	originate	VERB
cet-15373	85	37	from	from	ADP
cet-15373	85	38	the	the	DET
cet-15373	85	39	nitrogen	nitrogen	NOUN
cet-15373	85	40	present	present	NOUN
cet-15373	85	41	in	in	ADP
cet-15373	85	42	the	the	DET
cet-15373	85	43	reactant	reactant	NOUN
cet-15373	85	44	gas	gas	NOUN
cet-15373	85	45	.	.	PUNCT
cet-15373	86	1	furthermore	furthermore	ADV
cet-15373	86	2	,	,	PUNCT
cet-15373	86	3	before	before	ADP
cet-15373	86	4	testing	testing	NOUN
cet-15373	86	5	,	,	PUNCT
cet-15373	86	6	the	the	DET
cet-15373	86	7	electrolyte	electrolyte	NOUN
cet-15373	86	8	and	and	CCONJ
cet-15373	86	9	the	the	DET
cet-15373	86	10	sulphuric	sulphuric	PROPN
cet-15373	86	11	acid	acid	PROPN
cet-15373	86	12	trap	trap	NOUN
cet-15373	86	13	were	be	AUX
cet-15373	86	14	subjected	subject	VERB
cet-15373	86	15	to	to	ADP
cet-15373	86	16	analysis	analysis	NOUN
cet-15373	86	17	using	use	VERB
cet-15373	86	18	the	the	DET
cet-15373	86	19	spectrophotometric	spectrophotometric	ADJ
cet-15373	86	20	method	method	NOUN
cet-15373	86	21	and	and	CCONJ
cet-15373	86	22	the	the	DET
cet-15373	86	23	ion	ion	NOUN
cet-15373	86	24	chromatograph	chromatograph	NOUN
cet-15373	86	25	,	,	PUNCT
cet-15373	86	26	respectively	respectively	ADV
cet-15373	86	27	.	.	PUNCT
cet-15373	87	1	these	these	DET
cet-15373	87	2	analyses	analysis	NOUN
cet-15373	87	3	were	be	AUX
cet-15373	87	4	performed	perform	VERB
cet-15373	87	5	to	to	PART
cet-15373	87	6	ensure	ensure	VERB
cet-15373	87	7	the	the	DET
cet-15373	87	8	absence	absence	NOUN
cet-15373	87	9	of	of	ADP
cet-15373	87	10	ammonium	ammonium	NOUN
cet-15373	87	11	.	.	PUNCT
cet-15373	88	1	the	the	DET
cet-15373	88	2	entire	entire	ADJ
cet-15373	88	3	apparatus	apparatus	NOUN
cet-15373	88	4	employed	employ	VERB
cet-15373	88	5	for	for	ADP
cet-15373	88	6	the	the	DET
cet-15373	88	7	experiment	experiment	NOUN
cet-15373	88	8	maintained	maintain	VERB
cet-15373	88	9	a	a	DET
cet-15373	88	10	gas	gas	NOUN
cet-15373	88	11	-	-	PUNCT
cet-15373	88	12	tight	tight	NOUN
cet-15373	88	13	10	10	NUM
cet-15373	88	14	20	20	NUM
cet-15373	88	15	30	30	NUM
cet-15373	88	16	40	40	NUM
cet-15373	88	17	50	50	NUM
cet-15373	88	18	60	60	NUM
cet-15373	88	19	70	70	NUM
cet-15373	88	20	80	80	NUM
cet-15373	88	21	90	90	NUM
cet-15373	88	22	a	a	PRON
cet-15373	88	23	)	)	PUNCT
cet-15373	88	24	theta	theta	NOUN
cet-15373	88	25	(	(	PUNCT
cet-15373	88	26	°	°	PROPN
cet-15373	88	27	)	)	PUNCT
cet-15373	88	28	-al2o3	-al2o3	NOUN
cet-15373	88	29	in	in	ADP
cet-15373	88	30	te	te	PROPN
cet-15373	88	31	n	n	PROPN
cet-15373	88	32	s	s	VERB
cet-15373	88	33	it	it	PRON
cet-15373	88	34	y	y	PROPN
cet-15373	88	35	(	(	PUNCT
cet-15373	88	36	a	a	DET
cet-15373	88	37	.u	.u	NOUN
cet-15373	88	38	.	.	PUNCT
cet-15373	88	39	)	)	PUNCT
cet-15373	89	1	fe2o3	fe2o3	ADJ
cet-15373	89	2	/	/	SYM
cet-15373	89	3	al2o3	al2o3	PROPN
cet-15373	89	4	rufe	rufe	NOUN
cet-15373	89	5	/	/	SYM
cet-15373	89	6	al2o3	al2o3	PROPN
cet-15373	89	7	ru	ru	PROPN
cet-15373	89	8	/	/	SYM
cet-15373	89	9	al2o3	al2o3	PROPN
cet-15373	89	10	10	10	NUM
cet-15373	89	11	20	20	NUM
cet-15373	89	12	30	30	NUM
cet-15373	89	13	40	40	NUM
cet-15373	89	14	50	50	NUM
cet-15373	89	15	60	60	NUM
cet-15373	89	16	70	70	NUM
cet-15373	89	17	80	80	NUM
cet-15373	89	18	90	90	NUM
cet-15373	89	19	theta	theta	NOUN
cet-15373	89	20	(	(	PUNCT
cet-15373	89	21	°	°	NOUN
cet-15373	89	22	)	)	PUNCT
cet-15373	89	23	cnts	cnt	NOUN
cet-15373	89	24	in	in	ADP
cet-15373	89	25	te	te	PROPN
cet-15373	89	26	n	n	PROPN
cet-15373	89	27	s	s	VERB
cet-15373	89	28	it	it	PRON
cet-15373	89	29	y	y	PROPN
cet-15373	89	30	(	(	PUNCT
cet-15373	89	31	a	a	DET
cet-15373	89	32	.u	.u	NOUN
cet-15373	89	33	)	)	PUNCT
cet-15373	90	1	fe2o3	fe2o3	PROPN
cet-15373	90	2	/	/	SYM
cet-15373	90	3	cnts	cnts	PROPN
cet-15373	90	4	rufe	rufe	PROPN
cet-15373	90	5	/	/	SYM
cet-15373	90	6	cnts	cnts	PROPN
cet-15373	90	7	ru	ru	PROPN
cet-15373	90	8	/	/	SYM
cet-15373	90	9	cnts	cnts	PROPN
cet-15373	90	10	b	b	PROPN
cet-15373	90	11	)	)	PUNCT
cet-15373	90	12	a	a	DET
cet-15373	90	13	)	)	PUNCT
cet-15373	90	14	b	b	NOUN
cet-15373	90	15	)	)	PUNCT
cet-15373	90	16	736	736	NUM
cet-15373	90	17	environment	environment	NOUN
cet-15373	90	18	and	and	CCONJ
cet-15373	90	19	the	the	DET
cet-15373	90	20	decontamination	decontamination	NOUN
cet-15373	90	21	values	value	NOUN
cet-15373	90	22	have	have	AUX
cet-15373	90	23	been	be	AUX
cet-15373	90	24	voluntarily	voluntarily	ADV
cet-15373	90	25	omitted	omit	VERB
cet-15373	90	26	for	for	ADP
cet-15373	90	27	simplicity	simplicity	NOUN
cet-15373	90	28	.	.	PUNCT
cet-15373	91	1	the	the	DET
cet-15373	91	2	purpose	purpose	NOUN
cet-15373	91	3	of	of	ADP
cet-15373	91	4	this	this	DET
cet-15373	91	5	work	work	NOUN
cet-15373	91	6	is	be	AUX
cet-15373	91	7	to	to	PART
cet-15373	91	8	evaluate	evaluate	VERB
cet-15373	91	9	the	the	DET
cet-15373	91	10	option	option	NOUN
cet-15373	91	11	of	of	ADP
cet-15373	91	12	partial	partial	ADJ
cet-15373	91	13	or	or	CCONJ
cet-15373	91	14	total	total	ADJ
cet-15373	91	15	replacement	replacement	NOUN
cet-15373	91	16	of	of	ADP
cet-15373	91	17	noble	noble	ADJ
cet-15373	91	18	metals	metal	NOUN
cet-15373	91	19	with	with	ADP
cet-15373	91	20	more	more	ADJ
cet-15373	91	21	earth	earth	NOUN
cet-15373	91	22	-	-	PUNCT
cet-15373	91	23	abundant	abundant	ADJ
cet-15373	91	24	materials	material	NOUN
cet-15373	91	25	.	.	PUNCT
cet-15373	92	1	figures	figure	NOUN
cet-15373	92	2	4a	4a	NOUN
cet-15373	92	3	and	and	CCONJ
cet-15373	92	4	4b	4b	PROPN
cet-15373	92	5	show	show	VERB
cet-15373	92	6	the	the	DET
cet-15373	92	7	production	production	NOUN
cet-15373	92	8	of	of	ADP
cet-15373	92	9	ammonia	ammonia	NOUN
cet-15373	92	10	expressed	express	VERB
cet-15373	92	11	in	in	ADP
cet-15373	92	12	g	g	PROPN
cet-15373	92	13	mgcat	mgcat	PROPN
cet-15373	92	14	-1	-1	PUNCT
cet-15373	92	15	h-1	h-1	PROPN
cet-15373	92	16	for	for	ADP
cet-15373	92	17	al2o3	al2o3	PROPN
cet-15373	92	18	and	and	CCONJ
cet-15373	92	19	cnts	cnts	PROPN
cet-15373	92	20	-	-	PUNCT
cet-15373	92	21	based	base	VERB
cet-15373	92	22	electrodes	electrode	NOUN
cet-15373	92	23	,	,	PUNCT
cet-15373	92	24	respectively	respectively	ADV
cet-15373	92	25	,	,	PUNCT
cet-15373	92	26	at	at	ADP
cet-15373	92	27	different	different	ADJ
cet-15373	92	28	applied	applied	ADJ
cet-15373	92	29	potentials	potential	NOUN
cet-15373	92	30	.	.	PUNCT
cet-15373	93	1	during	during	ADP
cet-15373	93	2	the	the	DET
cet-15373	93	3	tests	test	NOUN
cet-15373	93	4	no	no	DET
cet-15373	93	5	ammonia	ammonia	NOUN
cet-15373	93	6	was	be	AUX
cet-15373	93	7	detected	detect	VERB
cet-15373	93	8	in	in	ADP
cet-15373	93	9	liquid	liquid	ADJ
cet-15373	93	10	phase	phase	NOUN
cet-15373	93	11	(	(	PUNCT
cet-15373	93	12	anodic	anodic	ADJ
cet-15373	93	13	compartment	compartment	NOUN
cet-15373	93	14	)	)	PUNCT
cet-15373	93	15	,	,	PUNCT
cet-15373	93	16	and	and	CCONJ
cet-15373	93	17	the	the	DET
cet-15373	93	18	totality	totality	NOUN
cet-15373	93	19	of	of	ADP
cet-15373	93	20	reduced	reduce	VERB
cet-15373	93	21	nitrogen	nitrogen	NOUN
cet-15373	93	22	was	be	AUX
cet-15373	93	23	detected	detect	VERB
cet-15373	93	24	in	in	ADP
cet-15373	93	25	the	the	DET
cet-15373	93	26	gas	gas	NOUN
cet-15373	93	27	phase	phase	NOUN
cet-15373	93	28	trap	trap	NOUN
cet-15373	93	29	(	(	PUNCT
cet-15373	93	30	cathode	cathode	NOUN
cet-15373	93	31	)	)	PUNCT
cet-15373	93	32	.	.	PUNCT
cet-15373	94	1	figure	figure	VERB
cet-15373	94	2	4	4	NUM
cet-15373	94	3	:	:	PUNCT
cet-15373	94	4	ammonia	ammonia	NOUN
cet-15373	94	5	production	production	NOUN
cet-15373	94	6	for	for	ADP
cet-15373	94	7	a	a	DET
cet-15373	94	8	)	)	PUNCT
cet-15373	94	9	al2o3	al2o3	NOUN
cet-15373	94	10	-	-	PUNCT
cet-15373	94	11	based	base	VERB
cet-15373	94	12	catalysts	catalyst	NOUN
cet-15373	94	13	and	and	CCONJ
cet-15373	94	14	b	b	NOUN
cet-15373	94	15	)	)	PUNCT
cet-15373	94	16	for	for	ADP
cet-15373	94	17	cnts	cnts	PROPN
cet-15373	94	18	-	-	PUNCT
cet-15373	94	19	based	base	VERB
cet-15373	94	20	catalysts	catalyst	NOUN
cet-15373	94	21	.	.	PUNCT
cet-15373	95	1	the	the	DET
cet-15373	95	2	results	result	NOUN
cet-15373	95	3	shown	show	VERB
cet-15373	95	4	in	in	ADP
cet-15373	95	5	figure	figure	NOUN
cet-15373	95	6	4a	4a	NOUN
cet-15373	95	7	for	for	ADP
cet-15373	95	8	alumina	alumina	NOUN
cet-15373	95	9	-	-	PUNCT
cet-15373	95	10	based	base	VERB
cet-15373	95	11	catalysts	catalyst	NOUN
cet-15373	95	12	denote	denote	VERB
cet-15373	95	13	a	a	DET
cet-15373	95	14	predominantly	predominantly	ADV
cet-15373	95	15	best	good	ADJ
cet-15373	95	16	performance	performance	NOUN
cet-15373	95	17	in	in	ADP
cet-15373	95	18	gasphase	gasphase	NOUN
cet-15373	95	19	,	,	PUNCT
cet-15373	95	20	in	in	ADP
cet-15373	95	21	terms	term	NOUN
cet-15373	95	22	of	of	ADP
cet-15373	95	23	ammonia	ammonia	NOUN
cet-15373	95	24	productivity	productivity	NOUN
cet-15373	95	25	at	at	ADP
cet-15373	95	26	-0.3	-0.3	PROPN
cet-15373	95	27	v	v	NOUN
cet-15373	95	28	vs.	vs.	ADP
cet-15373	95	29	rhe	rhe	NOUN
cet-15373	95	30	with	with	ADP
cet-15373	95	31	the	the	DET
cet-15373	95	32	co	co	ADJ
cet-15373	95	33	-	-	ADJ
cet-15373	95	34	doped	doped	ADJ
cet-15373	95	35	catalyst	catalyst	NOUN
cet-15373	95	36	ru	ru	PROPN
cet-15373	95	37	-	-	PUNCT
cet-15373	95	38	fe	fe	NOUN
cet-15373	95	39	/	/	SYM
cet-15373	95	40	al2o3	al2o3	PROPN
cet-15373	95	41	,	,	PUNCT
cet-15373	95	42	yielded	yield	VERB
cet-15373	95	43	the	the	DET
cet-15373	95	44	highest	high	ADJ
cet-15373	95	45	observed	observed	ADJ
cet-15373	95	46	catalytic	catalytic	ADJ
cet-15373	95	47	performance	performance	NOUN
cet-15373	95	48	(	(	PUNCT
cet-15373	95	49	1.16	1.16	NUM
cet-15373	95	50	g	g	PROPN
cet-15373	95	51	mgcat	mgcat	PROPN
cet-15373	95	52	-1	-1	PUNCT
cet-15373	95	53	h-1	h-1	PROPN
cet-15373	95	54	)	)	PUNCT
cet-15373	95	55	with	with	ADP
cet-15373	95	56	a	a	DET
cet-15373	95	57	faradaic	faradaic	ADJ
cet-15373	95	58	efficiency	efficiency	NOUN
cet-15373	95	59	(	(	PUNCT
cet-15373	95	60	fe	fe	NOUN
cet-15373	95	61	)	)	PUNCT
cet-15373	95	62	of	of	ADP
cet-15373	95	63	0.55	0.55	NUM
cet-15373	95	64	%	%	NOUN
cet-15373	95	65	and	and	CCONJ
cet-15373	95	66	a	a	DET
cet-15373	95	67	current	current	ADJ
cet-15373	95	68	density	density	NOUN
cet-15373	95	69	of	of	ADP
cet-15373	95	70	-294	-294	PROPN
cet-15373	95	71	a	a	PROPN
cet-15373	95	72	cm-2	cm-2	NOUN
cet-15373	95	73	at	at	ADP
cet-15373	95	74	-0.3	-0.3	PROPN
cet-15373	95	75	v	v	NOUN
cet-15373	95	76	vs.	vs.	ADP
cet-15373	95	77	rhe	rhe	NOUN
cet-15373	95	78	.	.	PUNCT
cet-15373	96	1	in	in	ADP
cet-15373	96	2	figure	figure	NOUN
cet-15373	96	3	4b	4b	PROPN
cet-15373	96	4	for	for	ADP
cet-15373	96	5	functionalized	functionalize	VERB
cet-15373	96	6	-	-	PUNCT
cet-15373	96	7	cnts	cnt	NOUN
cet-15373	96	8	-	-	PUNCT
cet-15373	96	9	based	base	VERB
cet-15373	96	10	catalysts	catalyst	NOUN
cet-15373	96	11	,	,	PUNCT
cet-15373	96	12	fe2o3	fe2o3	PROPN
cet-15373	96	13	/	/	SYM
cet-15373	96	14	cnts	cnts	PROPN
cet-15373	96	15	shows	show	VERB
cet-15373	96	16	the	the	DET
cet-15373	96	17	best	good	ADJ
cet-15373	96	18	performance	performance	NOUN
cet-15373	96	19	of	of	ADP
cet-15373	96	20	0.62	0.62	NUM
cet-15373	96	21	g	g	PROPN
cet-15373	96	22	mgcat	mgcat	PROPN
cet-15373	96	23	-1	-1	PUNCT
cet-15373	96	24	h-1	h-1	PROPN
cet-15373	96	25	with	with	ADP
cet-15373	96	26	a	a	DET
cet-15373	96	27	fe	fe	NOUN
cet-15373	96	28	of	of	ADP
cet-15373	96	29	1.5	1.5	NUM
cet-15373	96	30	%	%	NOUN
cet-15373	96	31	and	and	CCONJ
cet-15373	96	32	a	a	DET
cet-15373	96	33	current	current	ADJ
cet-15373	96	34	density	density	NOUN
cet-15373	96	35	of	of	ADP
cet-15373	96	36	-40	-40	PROPN
cet-15373	96	37	a	a	PROPN
cet-15373	96	38	cm-2	cm-2	NOUN
cet-15373	96	39	at	at	ADP
cet-15373	96	40	-0.3	-0.3	PROPN
cet-15373	96	41	v	v	NOUN
cet-15373	96	42	vs.	vs.	ADP
cet-15373	96	43	rhe	rhe	NOUN
cet-15373	96	44	.	.	PUNCT
cet-15373	97	1	productivity	productivity	NOUN
cet-15373	97	2	in	in	ADP
cet-15373	97	3	ru	ru	PROPN
cet-15373	97	4	-	-	PUNCT
cet-15373	97	5	fe	fe	NOUN
cet-15373	97	6	co	co	ADJ
cet-15373	97	7	-	-	ADJ
cet-15373	97	8	doped	doped	ADJ
cet-15373	97	9	alumina	alumina	NOUN
cet-15373	97	10	catalyst	catalyst	NOUN
cet-15373	97	11	is	be	AUX
cet-15373	97	12	1.87	1.87	NUM
cet-15373	97	13	times	time	NOUN
cet-15373	97	14	more	more	ADJ
cet-15373	97	15	than	than	ADP
cet-15373	97	16	iron	iron	NOUN
cet-15373	97	17	(	(	PUNCT
cet-15373	97	18	iii	iii	NOUN
cet-15373	97	19	)	)	PUNCT
cet-15373	97	20	oxide	oxide	NOUN
cet-15373	97	21	on	on	ADP
cet-15373	97	22	cnts	cnts	PROPN
cet-15373	97	23	.	.	PUNCT
cet-15373	98	1	the	the	DET
cet-15373	98	2	presence	presence	NOUN
cet-15373	98	3	of	of	ADP
cet-15373	98	4	ruthenium	ruthenium	NOUN
cet-15373	98	5	reduces	reduce	VERB
cet-15373	98	6	the	the	DET
cet-15373	98	7	onset	onset	NOUN
cet-15373	98	8	potential	potential	NOUN
cet-15373	98	9	,	,	PUNCT
cet-15373	98	10	while	while	SCONJ
cet-15373	98	11	iron	iron	NOUN
cet-15373	98	12	enhances	enhance	VERB
cet-15373	98	13	productivity	productivity	NOUN
cet-15373	98	14	.	.	PUNCT
cet-15373	99	1	in	in	ADP
cet-15373	99	2	the	the	DET
cet-15373	99	3	case	case	NOUN
cet-15373	99	4	of	of	ADP
cet-15373	99	5	alumina	alumina	NOUN
cet-15373	99	6	,	,	PUNCT
cet-15373	99	7	the	the	DET
cet-15373	99	8	partial	partial	ADJ
cet-15373	99	9	substitution	substitution	NOUN
cet-15373	99	10	results	result	NOUN
cet-15373	99	11	in	in	ADP
cet-15373	99	12	beneficial	beneficial	ADJ
cet-15373	99	13	effects	effect	NOUN
cet-15373	99	14	on	on	ADP
cet-15373	99	15	productivity	productivity	NOUN
cet-15373	99	16	and	and	CCONJ
cet-15373	99	17	the	the	DET
cet-15373	99	18	main	main	ADJ
cet-15373	99	19	values	value	NOUN
cet-15373	99	20	for	for	ADP
cet-15373	99	21	produced	produce	VERB
cet-15373	99	22	ammonia	ammonia	NOUN
cet-15373	99	23	are	be	AUX
cet-15373	99	24	reported	report	VERB
cet-15373	99	25	in	in	ADP
cet-15373	99	26	table	table	NOUN
cet-15373	99	27	1	1	NUM
cet-15373	99	28	.	.	PUNCT
cet-15373	99	29	table	table	NOUN
cet-15373	99	30	1	1	NUM
cet-15373	99	31	:	:	PUNCT
cet-15373	99	32	comparison	comparison	NOUN
cet-15373	99	33	of	of	ADP
cet-15373	99	34	the	the	DET
cet-15373	99	35	best	good	ADJ
cet-15373	99	36	catalyst	catalyst	NOUN
cet-15373	99	37	results	result	NOUN
cet-15373	99	38	for	for	ADP
cet-15373	99	39	electrochemical	electrochemical	ADJ
cet-15373	99	40	approach	approach	NOUN
cet-15373	99	41	as	as	SCONJ
cet-15373	99	42	reported	report	VERB
cet-15373	99	43	by	by	ADP
cet-15373	99	44	chen	chen	PROPN
cet-15373	99	45	et	et	PROPN
cet-15373	99	46	al	al	PROPN
cet-15373	99	47	.	.	PROPN
cet-15373	100	1	(	(	PUNCT
cet-15373	100	2	2020	2020	NUM
cet-15373	100	3	)	)	PUNCT
cet-15373	100	4	,	,	PUNCT
cet-15373	100	5	the	the	DET
cet-15373	100	6	application	application	NOUN
cet-15373	100	7	of	of	ADP
cet-15373	100	8	a	a	DET
cet-15373	100	9	low	low	ADJ
cet-15373	100	10	potential	potential	NOUN
cet-15373	100	11	can	can	AUX
cet-15373	100	12	change	change	VERB
cet-15373	100	13	the	the	DET
cet-15373	100	14	structure	structure	NOUN
cet-15373	100	15	of	of	ADP
cet-15373	100	16	the	the	DET
cet-15373	100	17	active	active	ADJ
cet-15373	100	18	site	site	NOUN
cet-15373	100	19	by	by	ADP
cet-15373	100	20	forming	form	VERB
cet-15373	100	21	the	the	DET
cet-15373	100	22	active	active	ADJ
cet-15373	100	23	species	specie	NOUN
cet-15373	100	24	-feooh	-feooh	PUNCT
cet-15373	100	25	(	(	PUNCT
cet-15373	100	26	lepidocrocite	lepidocrocite	NOUN
cet-15373	100	27	)	)	PUNCT
cet-15373	100	28	from	from	ADP
cet-15373	100	29	γ	γ	PROPN
cet-15373	100	30	-	-	PUNCT
cet-15373	100	31	fe2o3	fe2o3	ADJ
cet-15373	100	32	phase	phase	NOUN
cet-15373	100	33	found	find	VERB
cet-15373	100	34	in	in	ADP
cet-15373	100	35	xrd	xrd	NOUN
cet-15373	100	36	characterization	characterization	NOUN
cet-15373	100	37	.	.	PUNCT
cet-15373	101	1	the	the	DET
cet-15373	101	2	active	active	ADJ
cet-15373	101	3	-feooh	-feooh	PUNCT
cet-15373	101	4	is	be	AUX
cet-15373	101	5	able	able	ADJ
cet-15373	101	6	to	to	PART
cet-15373	101	7	promote	promote	VERB
cet-15373	101	8	the	the	DET
cet-15373	101	9	reaction	reaction	NOUN
cet-15373	101	10	in	in	ADP
cet-15373	101	11	agreement	agreement	NOUN
cet-15373	101	12	also	also	ADV
cet-15373	101	13	with	with	ADP
cet-15373	101	14	the	the	DET
cet-15373	101	15	example	example	NOUN
cet-15373	101	16	found	find	VERB
cet-15373	101	17	in	in	ADP
cet-15373	101	18	nature	nature	NOUN
cet-15373	101	19	with	with	ADP
cet-15373	101	20	nitrogenase	nitrogenase	NOUN
cet-15373	101	21	femo	femo	NOUN
cet-15373	101	22	-	-	PUNCT
cet-15373	101	23	cofactor	cofactor	NOUN
cet-15373	101	24	(	(	PUNCT
cet-15373	101	25	einsle	einsle	NOUN
cet-15373	101	26	,	,	PUNCT
cet-15373	101	27	2014	2014	NUM
cet-15373	101	28	)	)	PUNCT
cet-15373	101	29	.	.	PUNCT
cet-15373	102	1	moreover	moreover	ADV
cet-15373	102	2	liu	liu	PROPN
cet-15373	102	3	et	et	PROPN
cet-15373	102	4	al	al	PROPN
cet-15373	102	5	.	.	PROPN
cet-15373	103	1	(	(	PUNCT
cet-15373	103	2	2023	2023	NUM
cet-15373	103	3	)	)	PUNCT
cet-15373	103	4	observed	observe	VERB
cet-15373	103	5	a	a	DET
cet-15373	103	6	similar	similar	ADJ
cet-15373	103	7	behaviour	behaviour	NOUN
cet-15373	103	8	with	with	ADP
cet-15373	103	9	fe	fe	ADJ
cet-15373	103	10	-	-	ADJ
cet-15373	103	11	ru	ru	PROPN
cet-15373	103	12	bimetallic	bimetallic	PROPN
cet-15373	103	13	catalyst	catalyst	NOUN
cet-15373	103	14	prepared	prepare	VERB
cet-15373	103	15	by	by	ADP
cet-15373	103	16	atomically	atomically	ADV
cet-15373	103	17	dispersing	disperse	VERB
cet-15373	103	18	the	the	DET
cet-15373	103	19	metals	metal	NOUN
cet-15373	103	20	on	on	ADP
cet-15373	103	21	metal	metal	NOUN
cet-15373	103	22	organic	organic	ADJ
cet-15373	103	23	frameworks	framework	NOUN
cet-15373	103	24	(	(	PUNCT
cet-15373	103	25	mofs	mof	NOUN
cet-15373	103	26	)	)	PUNCT
cet-15373	103	27	by	by	ADP
cet-15373	103	28	wetness	wetness	ADJ
cet-15373	103	29	incipient	incipient	ADJ
cet-15373	103	30	impregnation	impregnation	NOUN
cet-15373	103	31	.	.	PUNCT
cet-15373	104	1	when	when	SCONJ
cet-15373	104	2	comparing	compare	VERB
cet-15373	104	3	the	the	DET
cet-15373	104	4	adsorption	adsorption	NOUN
cet-15373	104	5	and	and	CCONJ
cet-15373	104	6	desorption	desorption	NOUN
cet-15373	104	7	energies	energy	NOUN
cet-15373	104	8	by	by	ADP
cet-15373	104	9	dft	dft	PROPN
cet-15373	104	10	calculations	calculation	NOUN
cet-15373	104	11	,	,	PUNCT
cet-15373	104	12	the	the	DET
cet-15373	104	13	presence	presence	NOUN
cet-15373	104	14	of	of	ADP
cet-15373	104	15	atomically	atomically	ADV
cet-15373	104	16	dispersed	disperse	VERB
cet-15373	104	17	fe	fe	NOUN
cet-15373	104	18	and	and	CCONJ
cet-15373	104	19	ru	ru	PROPN
cet-15373	104	20	reduces	reduce	VERB
cet-15373	104	21	the	the	DET
cet-15373	104	22	n2	n2	ADJ
cet-15373	104	23	-	-	PUNCT
cet-15373	104	24	fe	fe	NOUN
cet-15373	104	25	reaction	reaction	NOUN
cet-15373	104	26	path	path	NOUN
cet-15373	104	27	by	by	ADP
cet-15373	104	28	reducing	reduce	VERB
cet-15373	104	29	the	the	DET
cet-15373	104	30	adsorption	adsorption	NOUN
cet-15373	104	31	/	/	SYM
cet-15373	104	32	desorption	desorption	NOUN
cet-15373	104	33	energies	energy	NOUN
cet-15373	104	34	without	without	ADP
cet-15373	104	35	being	be	AUX
cet-15373	104	36	detected	detect	VERB
cet-15373	104	37	by	by	ADP
cet-15373	104	38	xrd	xrd	NOUN
cet-15373	104	39	analysis	analysis	NOUN
cet-15373	104	40	.	.	PUNCT
cet-15373	105	1	these	these	DET
cet-15373	105	2	results	result	NOUN
cet-15373	105	3	emphasize	emphasize	VERB
cet-15373	105	4	the	the	DET
cet-15373	105	5	need	need	NOUN
cet-15373	105	6	for	for	ADP
cet-15373	105	7	further	further	ADJ
cet-15373	105	8	research	research	NOUN
cet-15373	105	9	to	to	PART
cet-15373	105	10	reach	reach	VERB
cet-15373	105	11	industrial	industrial	ADJ
cet-15373	105	12	competitiveness	competitiveness	NOUN
cet-15373	105	13	and	and	CCONJ
cet-15373	105	14	highlight	highlight	VERB
cet-15373	105	15	the	the	DET
cet-15373	105	16	key	key	ADJ
cet-15373	105	17	role	role	NOUN
cet-15373	105	18	of	of	ADP
cet-15373	105	19	electrode	electrode	NOUN
cet-15373	105	20	and	and	CCONJ
cet-15373	105	21	reactor	reactor	NOUN
cet-15373	105	22	engineering	engineering	NOUN
cet-15373	105	23	in	in	ADP
cet-15373	105	24	this	this	DET
cet-15373	105	25	advancement	advancement	NOUN
cet-15373	105	26	(	(	PUNCT
cet-15373	105	27	rouwenhorst	rouwenhorst	PROPN
cet-15373	105	28	et	et	PROPN
cet-15373	105	29	al	al	PROPN
cet-15373	105	30	.	.	PROPN
cet-15373	105	31	,	,	PUNCT
cet-15373	105	32	2021	2021	NUM
cet-15373	105	33	)	)	PUNCT
cet-15373	105	34	.	.	PUNCT
cet-15373	106	1	the	the	DET
cet-15373	106	2	electrochemical	electrochemical	ADJ
cet-15373	106	3	nrr	nrr	PROPN
cet-15373	106	4	future	future	ADJ
cet-15373	106	5	efforts	effort	NOUN
cet-15373	106	6	should	should	AUX
cet-15373	106	7	be	be	AUX
cet-15373	106	8	addressed	address	VERB
cet-15373	106	9	to	to	ADP
cet-15373	106	10	i	i	PRON
cet-15373	106	11	)	)	PUNCT
cet-15373	106	12	increase	increase	VERB
cet-15373	106	13	the	the	DET
cet-15373	106	14	maximum	maximum	ADJ
cet-15373	106	15	productivity	productivity	NOUN
cet-15373	106	16	compared	compare	VERB
cet-15373	106	17	to	to	ADP
cet-15373	106	18	the	the	DET
cet-15373	106	19	state	state	NOUN
cet-15373	106	20	of	of	ADP
cet-15373	106	21	the	the	DET
cet-15373	106	22	art	art	NOUN
cet-15373	106	23	,	,	PUNCT
cet-15373	106	24	ii	ii	NOUN
cet-15373	106	25	)	)	PUNCT
cet-15373	106	26	increase	increase	VERB
cet-15373	106	27	the	the	DET
cet-15373	106	28	mechanical	mechanical	ADJ
cet-15373	106	29	and	and	CCONJ
cet-15373	106	30	chemical	chemical	ADJ
cet-15373	106	31	stability	stability	NOUN
cet-15373	106	32	of	of	ADP
cet-15373	106	33	the	the	DET
cet-15373	106	34	catalysts	catalyst	NOUN
cet-15373	106	35	over	over	ADP
cet-15373	106	36	time	time	NOUN
cet-15373	106	37	,	,	PUNCT
cet-15373	106	38	iii	iii	X
cet-15373	106	39	)	)	PUNCT
cet-15373	106	40	increase	increase	VERB
cet-15373	106	41	the	the	DET
cet-15373	106	42	energy	energy	NOUN
cet-15373	106	43	efficiency	efficiency	NOUN
cet-15373	106	44	of	of	ADP
cet-15373	106	45	the	the	DET
cet-15373	106	46	process	process	NOUN
cet-15373	106	47	,	,	PUNCT
cet-15373	106	48	vi	vi	X
cet-15373	106	49	)	)	PUNCT
cet-15373	106	50	reduce	reduce	VERB
cet-15373	106	51	the	the	DET
cet-15373	106	52	use	use	NOUN
cet-15373	106	53	of	of	ADP
cet-15373	106	54	critical	critical	ADJ
cet-15373	106	55	materials	material	NOUN
cet-15373	106	56	having	have	VERB
cet-15373	106	57	priority	priority	NOUN
cet-15373	106	58	for	for	ADP
cet-15373	106	59	sustainability	sustainability	NOUN
cet-15373	106	60	.	.	PUNCT
cet-15373	107	1	also	also	ADV
cet-15373	107	2	,	,	PUNCT
cet-15373	107	3	the	the	DET
cet-15373	107	4	use	use	NOUN
cet-15373	107	5	of	of	ADP
cet-15373	107	6	a	a	DET
cet-15373	107	7	different	different	ADJ
cet-15373	107	8	reaction	reaction	NOUN
cet-15373	107	9	media	medium	NOUN
cet-15373	107	10	such	such	ADJ
cet-15373	107	11	as	as	ADP
cet-15373	107	12	organic	organic	ADJ
cet-15373	107	13	environment	environment	NOUN
cet-15373	107	14	(	(	PUNCT
cet-15373	107	15	ampelli	ampelli	NOUN
cet-15373	107	16	,	,	PUNCT
cet-15373	107	17	2020	2020	NUM
cet-15373	107	18	)	)	PUNCT
cet-15373	107	19	or	or	CCONJ
cet-15373	107	20	ionic	ionic	ADJ
cet-15373	107	21	liquid	liquid	NOUN
cet-15373	107	22	(	(	PUNCT
cet-15373	107	23	tian	tian	PROPN
cet-15373	107	24	et	et	PROPN
cet-15373	107	25	al	al	PROPN
cet-15373	107	26	.	.	PROPN
cet-15373	107	27	,	,	PUNCT
cet-15373	107	28	2022	2022	NUM
cet-15373	107	29	)	)	PUNCT
cet-15373	107	30	minimizing	minimize	VERB
cet-15373	107	31	the	the	DET
cet-15373	107	32	proton	proton	NOUN
cet-15373	107	33	activity	activity	NOUN
cet-15373	107	34	respect	respect	NOUN
cet-15373	107	35	to	to	ADP
cet-15373	107	36	aqueous	aqueous	ADJ
cet-15373	107	37	media	medium	NOUN
cet-15373	107	38	,	,	PUNCT
cet-15373	107	39	could	could	AUX
cet-15373	107	40	reduce	reduce	VERB
cet-15373	107	41	the	the	DET
cet-15373	107	42	side	side	NOUN
cet-15373	107	43	reaction	reaction	NOUN
cet-15373	107	44	of	of	ADP
cet-15373	107	45	her	she	PRON
cet-15373	107	46	.	.	PUNCT
cet-15373	108	1	only	only	ADV
cet-15373	108	2	by	by	ADP
cet-15373	108	3	incorporating	incorporate	VERB
cet-15373	108	4	innovative	innovative	ADJ
cet-15373	108	5	technologies	technology	NOUN
cet-15373	108	6	and	and	CCONJ
cet-15373	108	7	methodologies	methodology	NOUN
cet-15373	108	8	,	,	PUNCT
cet-15373	108	9	new	new	ADJ
cet-15373	108	10	paths	path	NOUN
cet-15373	108	11	can	can	AUX
cet-15373	108	12	be	be	AUX
cet-15373	108	13	opened	open	VERB
cet-15373	108	14	for	for	ADP
cet-15373	108	15	substantial	substantial	ADJ
cet-15373	108	16	improvements	improvement	NOUN
cet-15373	108	17	in	in	ADP
cet-15373	108	18	the	the	DET
cet-15373	108	19	nrr	nrr	PROPN
cet-15373	108	20	driven	drive	VERB
cet-15373	108	21	by	by	ADP
cet-15373	108	22	renewable	renewable	ADJ
cet-15373	108	23	electricity	electricity	NOUN
cet-15373	108	24	.	.	PUNCT
cet-15373	109	1	-0.1	-0.1	PROPN
cet-15373	109	2	-0.2	-0.2	PROPN
cet-15373	109	3	-0.3	-0.3	PROPN
cet-15373	109	4	-0.4	-0.4	PROPN
cet-15373	109	5	-0.5	-0.5	PROPN
cet-15373	109	6	-0.6	-0.6	PROPN
cet-15373	109	7	-0.7	-0.7	PROPN
cet-15373	109	8	-0.8	-0.8	PROPN
cet-15373	109	9	0.0	0.0	NUM
cet-15373	109	10	0.2	0.2	NUM
cet-15373	109	11	0.4	0.4	NUM
cet-15373	109	12	0.6	0.6	NUM
cet-15373	109	13	0.8	0.8	NUM
cet-15373	109	14	1.0	1.0	NUM
cet-15373	109	15	1.2	1.2	NUM
cet-15373	109	16	n	n	NOUN
cet-15373	109	17	h	h	NOUN
cet-15373	109	18	3	3	NUM
cet-15373	109	19	p	p	NOUN
cet-15373	109	20	ro	ro	X
cet-15373	109	21	d	d	X
cet-15373	109	22	u	u	X
cet-15373	109	23	c	c	NOUN
cet-15373	109	24	ti	ti	X
cet-15373	109	25	v	v	ADP
cet-15373	109	26	it	it	PRON
cet-15373	109	27	y	y	NOUN
cet-15373	109	28	(	(	PUNCT
cet-15373	109	29			NOUN
cet-15373	109	30	g	g	NOUN
cet-15373	109	31	m	m	NOUN
cet-15373	109	32	g	g	NOUN
cet-15373	109	33	-1	-1	INTJ
cet-15373	109	34	c	c	PROPN
cet-15373	109	35	a	a	DET
cet-15373	109	36	t	t	PROPN
cet-15373	109	37	h	h	NOUN
cet-15373	109	38	-1	-1	PUNCT
cet-15373	109	39	)	)	PUNCT
cet-15373	110	1	potential	potential	NOUN
cet-15373	110	2	(	(	PUNCT
cet-15373	110	3	v	v	NOUN
cet-15373	110	4	vs	vs	ADP
cet-15373	110	5	rhe	rhe	NOUN
cet-15373	110	6	)	)	PUNCT
cet-15373	110	7	ru	ru	PROPN
cet-15373	110	8	/	/	SYM
cet-15373	110	9	al2o3	al2o3	PROPN
cet-15373	110	10	ru	ru	PROPN
cet-15373	110	11	-	-	PUNCT
cet-15373	110	12	fe	fe	NOUN
cet-15373	110	13	/	/	SYM
cet-15373	110	14	al2o3	al2o3	PROPN
cet-15373	110	15	fe2o3	fe2o3	PROPN
cet-15373	110	16	/	/	SYM
cet-15373	110	17	al2o3	al2o3	PROPN
cet-15373	110	18	al2o3	al2o3	PROPN
cet-15373	110	19	fe	fe	PROPN
cet-15373	110	20	:	:	PUNCT
cet-15373	110	21	0.55	0.55	NUM
cet-15373	110	22	%	%	NOUN
cet-15373	110	23	-0.1	-0.1	PROPN
cet-15373	110	24	-0.2	-0.2	PROPN
cet-15373	110	25	-0.3	-0.3	PROPN
cet-15373	110	26	-0.4	-0.4	PROPN
cet-15373	110	27	-0.5	-0.5	PROPN
cet-15373	110	28	-0.6	-0.6	PROPN
cet-15373	110	29	-0.7	-0.7	PROPN
cet-15373	110	30	-0.8	-0.8	PROPN
cet-15373	110	31	-0.1	-0.1	PROPN
cet-15373	110	32	-0.2	-0.2	PROPN
cet-15373	110	33	-0.3	-0.3	PROPN
cet-15373	110	34	-0.4	-0.4	PROPN
cet-15373	110	35	-0.5	-0.5	PROPN
cet-15373	110	36	-0.6	-0.6	PROPN
cet-15373	110	37	-0.7	-0.7	PROPN
cet-15373	110	38	-0.8	-0.8	PROPN
cet-15373	110	39	0.0	0.0	NUM
cet-15373	110	40	0.2	0.2	NUM
cet-15373	110	41	0.4	0.4	NUM
cet-15373	110	42	0.6	0.6	NUM
cet-15373	110	43	0.8	0.8	NUM
cet-15373	110	44	1.0	1.0	NUM
cet-15373	110	45	1.2	1.2	NUM
cet-15373	110	46	n	n	NOUN
cet-15373	110	47	h	h	NOUN
cet-15373	110	48	3	3	NUM
cet-15373	110	49	p	p	NOUN
cet-15373	110	50	ro	ro	X
cet-15373	111	1	d	d	X
cet-15373	111	2	u	u	X
cet-15373	111	3	c	c	NOUN
cet-15373	111	4	ti	ti	X
cet-15373	111	5	v	v	ADP
cet-15373	111	6	it	it	PRON
cet-15373	111	7	y	y	NOUN
cet-15373	111	8	(	(	PUNCT
cet-15373	111	9			NOUN
cet-15373	111	10	g	g	NOUN
cet-15373	111	11	m	m	NOUN
cet-15373	111	12	g	g	NOUN
cet-15373	111	13	-1	-1	INTJ
cet-15373	111	14	c	c	PROPN
cet-15373	111	15	a	a	DET
cet-15373	111	16	t	t	PROPN
cet-15373	111	17	h	h	NOUN
cet-15373	111	18	-1	-1	PUNCT
cet-15373	111	19	)	)	PUNCT
cet-15373	112	1	potential	potential	NOUN
cet-15373	112	2	(	(	PUNCT
cet-15373	112	3	v	v	NOUN
cet-15373	112	4	vs	vs	ADP
cet-15373	112	5	rhe	rhe	NOUN
cet-15373	112	6	)	)	PUNCT
cet-15373	112	7	ru	ru	PROPN
cet-15373	112	8	/	/	SYM
cet-15373	112	9	cnts	cnts	PROPN
cet-15373	112	10	ru	ru	PROPN
cet-15373	112	11	-	-	PUNCT
cet-15373	112	12	fe	fe	PROPN
cet-15373	112	13	/	/	SYM
cet-15373	112	14	cnts	cnts	PROPN
cet-15373	112	15	fe2o3	fe2o3	PROPN
cet-15373	112	16	/	/	SYM
cet-15373	112	17	cnts	cnts	PROPN
cet-15373	112	18	cnts	cnts	PROPN
cet-15373	112	19	fe	fe	PROPN
cet-15373	112	20	:	:	PUNCT
cet-15373	112	21	1.85	1.85	NUM
cet-15373	112	22	%	%	NOUN
cet-15373	112	23	catalysts	catalyst	NOUN
cet-15373	112	24	nh3	nh3	NOUN
cet-15373	112	25	productivity	productivity	NOUN
cet-15373	112	26	(	(	PUNCT
cet-15373	112	27	g	g	PROPN
cet-15373	112	28	mgcat	mgcat	PROPN
cet-15373	112	29	-1	-1	PUNCT
cet-15373	112	30	h-1	h-1	PROPN
cet-15373	112	31	)	)	PUNCT
cet-15373	112	32	faradaic	faradaic	ADJ
cet-15373	112	33	efficiency	efficiency	NOUN
cet-15373	112	34	(	(	PUNCT
cet-15373	112	35	%	%	INTJ
cet-15373	112	36	)	)	PUNCT
cet-15373	112	37	ru	ru	PROPN
cet-15373	112	38	-	-	PUNCT
cet-15373	112	39	fe	fe	NOUN
cet-15373	112	40	/	/	SYM
cet-15373	112	41	al2o3	al2o3	PROPN
cet-15373	112	42	1.16	1.16	NUM
cet-15373	112	43	0.55	0.55	NUM
cet-15373	112	44	fe2o3	fe2o3	PROPN
cet-15373	112	45	/	/	SYM
cet-15373	112	46	cnts	cnts	PROPN
cet-15373	112	47	0.62	0.62	NUM
cet-15373	112	48	1.85	1.85	NUM
cet-15373	112	49	a	a	DET
cet-15373	112	50	)	)	PUNCT
cet-15373	112	51	b	b	NOUN
cet-15373	112	52	)	)	PUNCT
cet-15373	112	53	737	737	NUM
cet-15373	112	54	4	4	NUM
cet-15373	112	55	.	.	PUNCT
cet-15373	112	56	conclusions	conclusion	NOUN
cet-15373	112	57	the	the	DET
cet-15373	112	58	electrocatalytic	electrocatalytic	ADJ
cet-15373	112	59	behaviour	behaviour	NOUN
cet-15373	112	60	of	of	ADP
cet-15373	112	61	ru	ru	PROPN
cet-15373	112	62	and/or	and/or	CCONJ
cet-15373	112	63	fe	fe	NOUN
cet-15373	112	64	-	-	PUNCT
cet-15373	112	65	doped	doped	ADJ
cet-15373	112	66	alumina	alumina	NOUN
cet-15373	112	67	(	(	PUNCT
cet-15373	112	68	al2o3	al2o3	NOUN
cet-15373	112	69	)	)	PUNCT
cet-15373	112	70	or	or	CCONJ
cet-15373	112	71	carbon	carbon	NOUN
cet-15373	112	72	nanotubes	nanotube	NOUN
cet-15373	112	73	(	(	PUNCT
cet-15373	112	74	cnts	cnts	PROPN
cet-15373	112	75	)	)	PUNCT
cet-15373	112	76	was	be	AUX
cet-15373	112	77	evaluated	evaluate	VERB
cet-15373	112	78	in	in	ADP
cet-15373	112	79	the	the	DET
cet-15373	112	80	nitrogen	nitrogen	NOUN
cet-15373	112	81	reduction	reduction	NOUN
cet-15373	112	82	reaction	reaction	NOUN
cet-15373	112	83	(	(	PUNCT
cet-15373	112	84	nrr	nrr	PROPN
cet-15373	112	85	)	)	PUNCT
cet-15373	112	86	in	in	ADP
cet-15373	112	87	combination	combination	NOUN
cet-15373	112	88	with	with	ADP
cet-15373	112	89	a	a	DET
cet-15373	112	90	gas	gas	NOUN
cet-15373	112	91	-	-	PUNCT
cet-15373	112	92	diffusion	diffusion	NOUN
cet-15373	112	93	layer	layer	NOUN
cet-15373	112	94	(	(	PUNCT
cet-15373	112	95	gdl	gdl	NOUN
cet-15373	112	96	)	)	PUNCT
cet-15373	112	97	to	to	PART
cet-15373	112	98	form	form	VERB
cet-15373	112	99	novel	novel	ADJ
cet-15373	112	100	gas	gas	NOUN
cet-15373	112	101	-	-	PUNCT
cet-15373	112	102	diffusion	diffusion	NOUN
cet-15373	112	103	electrodes	electrode	NOUN
cet-15373	112	104	,	,	PUNCT
cet-15373	112	105	using	use	VERB
cet-15373	112	106	custom	custom	NOUN
cet-15373	112	107	reactors	reactor	NOUN
cet-15373	112	108	of	of	ADP
cet-15373	112	109	advanced	advanced	ADJ
cet-15373	112	110	design	design	NOUN
cet-15373	112	111	,	,	PUNCT
cet-15373	112	112	working	work	VERB
cet-15373	112	113	in	in	ADP
cet-15373	112	114	gas	gas	NOUN
cet-15373	112	115	phase	phase	NOUN
cet-15373	112	116	(	(	PUNCT
cet-15373	112	117	i.e.	i.e.	X
cet-15373	112	118	electrolyteless	electrolyteless	NOUN
cet-15373	112	119	conditions	condition	NOUN
cet-15373	112	120	)	)	PUNCT
cet-15373	112	121	to	to	PART
cet-15373	112	122	overcome	overcome	VERB
cet-15373	112	123	the	the	DET
cet-15373	112	124	low	low	ADJ
cet-15373	112	125	solubility	solubility	NOUN
cet-15373	112	126	of	of	ADP
cet-15373	112	127	nitrogen	nitrogen	NOUN
cet-15373	112	128	in	in	ADP
cet-15373	112	129	aqueous	aqueous	ADJ
cet-15373	112	130	media	medium	NOUN
cet-15373	112	131	.	.	PUNCT
cet-15373	113	1	in	in	ADP
cet-15373	113	2	the	the	DET
cet-15373	113	3	case	case	NOUN
cet-15373	113	4	of	of	ADP
cet-15373	113	5	catalysts	catalyst	NOUN
cet-15373	113	6	based	base	VERB
cet-15373	113	7	on	on	ADP
cet-15373	113	8	carbon	carbon	NOUN
cet-15373	113	9	nanotubes	nanotube	NOUN
cet-15373	113	10	(	(	PUNCT
cet-15373	113	11	cnts	cnts	PROPN
cet-15373	113	12	)	)	PUNCT
cet-15373	113	13	,	,	PUNCT
cet-15373	113	14	they	they	PRON
cet-15373	113	15	showed	show	VERB
cet-15373	113	16	similar	similar	ADJ
cet-15373	113	17	activity	activity	NOUN
cet-15373	113	18	,	,	PUNCT
cet-15373	113	19	such	such	ADJ
cet-15373	113	20	as	as	ADP
cet-15373	113	21	fe2o3	fe2o3	PROPN
cet-15373	113	22	in	in	ADP
cet-15373	113	23	comparison	comparison	NOUN
cet-15373	113	24	to	to	ADP
cet-15373	113	25	ru	ru	PROPN
cet-15373	113	26	and	and	CCONJ
cet-15373	113	27	ru	ru	PROPN
cet-15373	113	28	-	-	PUNCT
cet-15373	113	29	fe	fe	NOUN
cet-15373	113	30	codoped	codope	VERB
cet-15373	113	31	variants	variant	NOUN
cet-15373	113	32	.	.	PUNCT
cet-15373	114	1	on	on	ADP
cet-15373	114	2	the	the	DET
cet-15373	114	3	contrary	contrary	ADJ
cet-15373	114	4	,	,	PUNCT
cet-15373	114	5	alumina	alumina	NOUN
cet-15373	114	6	-	-	PUNCT
cet-15373	114	7	based	base	VERB
cet-15373	114	8	catalysts	catalyst	NOUN
cet-15373	114	9	showcased	showcase	VERB
cet-15373	114	10	distinctive	distinctive	ADJ
cet-15373	114	11	trends	trend	NOUN
cet-15373	114	12	.	.	PUNCT
cet-15373	115	1	specifically	specifically	ADV
cet-15373	115	2	,	,	PUNCT
cet-15373	115	3	doping	dope	VERB
cet-15373	115	4	with	with	ADP
cet-15373	115	5	ru	ru	PROPN
cet-15373	115	6	provided	provide	VERB
cet-15373	115	7	higher	high	ADJ
cet-15373	115	8	catalytic	catalytic	ADJ
cet-15373	115	9	performance	performance	NOUN
cet-15373	115	10	compared	compare	VERB
cet-15373	115	11	to	to	ADP
cet-15373	115	12	fe2o3	fe2o3	PROPN
cet-15373	115	13	,	,	PUNCT
cet-15373	115	14	while	while	SCONJ
cet-15373	115	15	the	the	DET
cet-15373	115	16	substitution	substitution	NOUN
cet-15373	115	17	of	of	ADP
cet-15373	115	18	fe	fe	NOUN
cet-15373	115	19	with	with	ADP
cet-15373	115	20	ru	ru	PROPN
cet-15373	115	21	in	in	ADP
cet-15373	115	22	a	a	DET
cet-15373	115	23	co	co	ADJ
cet-15373	115	24	-	-	ADJ
cet-15373	115	25	doped	doped	ADJ
cet-15373	115	26	configuration	configuration	NOUN
cet-15373	115	27	(	(	PUNCT
cet-15373	115	28	ru	ru	NOUN
cet-15373	115	29	-	-	PUNCT
cet-15373	115	30	fe	fe	NOUN
cet-15373	115	31	/	/	SYM
cet-15373	115	32	al2o3	al2o3	PROPN
cet-15373	115	33	)	)	PUNCT
cet-15373	115	34	yielded	yield	VERB
cet-15373	115	35	the	the	DET
cet-15373	115	36	highest	high	ADJ
cet-15373	115	37	observed	observed	ADJ
cet-15373	115	38	catalytic	catalytic	ADJ
cet-15373	115	39	performance	performance	NOUN
cet-15373	115	40	of	of	ADP
cet-15373	115	41	1.16	1.16	NUM
cet-15373	115	42	g	g	PROPN
cet-15373	115	43	mgcat	mgcat	PROPN
cet-15373	115	44	-1	-1	PUNCT
cet-15373	115	45	h-1	h-1	PROPN
cet-15373	115	46	,	,	PUNCT
cet-15373	115	47	and	and	CCONJ
cet-15373	115	48	a	a	DET
cet-15373	115	49	current	current	ADJ
cet-15373	115	50	density	density	NOUN
cet-15373	115	51	of	of	ADP
cet-15373	115	52	-294	-294	PROPN
cet-15373	115	53	a	a	PROPN
cet-15373	115	54	cm-2	cm-2	NOUN
cet-15373	115	55	at	at	ADP
cet-15373	115	56	-0.3	-0.3	PROPN
cet-15373	115	57	v	v	NOUN
cet-15373	115	58	vs	vs	ADP
cet-15373	115	59	rhe	rhe	NOUN
cet-15373	115	60	.	.	PUNCT
cet-15373	116	1	it	it	PRON
cet-15373	116	2	is	be	AUX
cet-15373	116	3	evident	evident	ADJ
cet-15373	116	4	that	that	SCONJ
cet-15373	116	5	,	,	PUNCT
cet-15373	116	6	partially	partially	ADV
cet-15373	116	7	replacing	replace	VERB
cet-15373	116	8	an	an	DET
cet-15373	116	9	expensive	expensive	ADJ
cet-15373	116	10	metal	metal	NOUN
cet-15373	116	11	(	(	PUNCT
cet-15373	116	12	such	such	ADJ
cet-15373	116	13	as	as	ADP
cet-15373	116	14	ru	ru	NOUN
cet-15373	116	15	)	)	PUNCT
cet-15373	116	16	with	with	ADP
cet-15373	116	17	a	a	DET
cet-15373	116	18	less	less	ADV
cet-15373	116	19	expensive	expensive	ADJ
cet-15373	116	20	one	one	NUM
cet-15373	116	21	(	(	PUNCT
cet-15373	116	22	fe	fe	NOUN
cet-15373	116	23	)	)	PUNCT
cet-15373	116	24	brings	bring	VERB
cet-15373	116	25	benefits	benefit	NOUN
cet-15373	116	26	.	.	PUNCT
cet-15373	117	1	among	among	ADP
cet-15373	117	2	all	all	DET
cet-15373	117	3	the	the	DET
cet-15373	117	4	samples	sample	NOUN
cet-15373	117	5	,	,	PUNCT
cet-15373	117	6	fe2o3	fe2o3	PROPN
cet-15373	117	7	/	/	SYM
cet-15373	117	8	cnts	cnts	PROPN
cet-15373	117	9	showed	show	VERB
cet-15373	117	10	the	the	DET
cet-15373	117	11	best	good	ADJ
cet-15373	117	12	performance	performance	NOUN
cet-15373	117	13	of	of	ADP
cet-15373	117	14	0.62	0.62	NUM
cet-15373	117	15	g	g	PROPN
cet-15373	117	16	mgcat	mgcat	PROPN
cet-15373	117	17	-1	-1	PUNCT
cet-15373	118	1	h-1	h-1	PROPN
cet-15373	118	2	and	and	CCONJ
cet-15373	118	3	a	a	DET
cet-15373	118	4	current	current	ADJ
cet-15373	118	5	density	density	NOUN
cet-15373	118	6	of	of	ADP
cet-15373	118	7	-40	-40	PROPN
cet-15373	118	8	a	a	PROPN
cet-15373	118	9	cm-2	cm-2	NOUN
cet-15373	118	10	at	at	ADP
cet-15373	118	11	-0.3	-0.3	PROPN
cet-15373	118	12	v	v	NOUN
cet-15373	118	13	vs	vs	ADP
cet-15373	118	14	rhe	rhe	NOUN
cet-15373	118	15	.	.	PUNCT
cet-15373	119	1	although	although	SCONJ
cet-15373	119	2	h₂	h₂	PROPN
cet-15373	119	3	is	be	AUX
cet-15373	119	4	the	the	DET
cet-15373	119	5	predominant	predominant	ADJ
cet-15373	119	6	product	product	NOUN
cet-15373	119	7	observed	observe	VERB
cet-15373	119	8	in	in	ADP
cet-15373	119	9	these	these	DET
cet-15373	119	10	experiments	experiment	NOUN
cet-15373	119	11	,	,	PUNCT
cet-15373	119	12	this	this	DET
cet-15373	119	13	study	study	NOUN
cet-15373	119	14	has	have	AUX
cet-15373	119	15	provided	provide	VERB
cet-15373	119	16	insights	insight	NOUN
cet-15373	119	17	into	into	ADP
cet-15373	119	18	the	the	DET
cet-15373	119	19	potential	potential	ADJ
cet-15373	119	20	range	range	NOUN
cet-15373	119	21	in	in	ADP
cet-15373	119	22	which	which	PRON
cet-15373	119	23	nrr	nrr	PROPN
cet-15373	119	24	occurs	occur	VERB
cet-15373	119	25	in	in	ADP
cet-15373	119	26	relation	relation	NOUN
cet-15373	119	27	to	to	ADP
cet-15373	119	28	the	the	DET
cet-15373	119	29	electrocatalyst	electrocatalyst	NOUN
cet-15373	119	30	used	use	VERB
cet-15373	119	31	.	.	PUNCT
cet-15373	120	1	ongoing	ongoing	ADJ
cet-15373	120	2	research	research	NOUN
cet-15373	120	3	aims	aim	VERB
cet-15373	120	4	to	to	PART
cet-15373	120	5	reduce	reduce	VERB
cet-15373	120	6	h₂	h₂	PROPN
cet-15373	120	7	production	production	NOUN
cet-15373	120	8	in	in	ADP
cet-15373	120	9	favour	favour	NOUN
cet-15373	120	10	of	of	ADP
cet-15373	120	11	nrr	nrr	PROPN
cet-15373	120	12	by	by	ADP
cet-15373	120	13	engineering	engineer	VERB
cet-15373	120	14	the	the	DET
cet-15373	120	15	electrode	electrode	NOUN
cet-15373	120	16	to	to	PART
cet-15373	120	17	modulate	modulate	VERB
cet-15373	120	18	wettability	wettability	NOUN
cet-15373	120	19	properties	property	NOUN
cet-15373	120	20	,	,	PUNCT
cet-15373	120	21	thereby	thereby	ADV
cet-15373	120	22	controlling	control	VERB
cet-15373	120	23	proton	proton	NOUN
cet-15373	120	24	accessibility	accessibility	NOUN
cet-15373	120	25	to	to	ADP
cet-15373	120	26	the	the	DET
cet-15373	120	27	catalytic	catalytic	ADJ
cet-15373	120	28	active	active	ADJ
cet-15373	120	29	sites	site	NOUN
cet-15373	120	30	.	.	PUNCT
cet-15373	121	1	acknowledgments	acknowledgment	NOUN
cet-15373	121	2	this	this	DET
cet-15373	121	3	work	work	NOUN
cet-15373	121	4	was	be	AUX
cet-15373	121	5	funded	fund	VERB
cet-15373	121	6	by	by	ADP
cet-15373	121	7	the	the	DET
cet-15373	121	8	european	european	PROPN
cet-15373	121	9	union	union	PROPN
cet-15373	121	10	next	next	ADJ
cet-15373	121	11	generation	generation	NOUN
cet-15373	121	12	eu	eu	PROPN
cet-15373	121	13	,	,	PUNCT
cet-15373	121	14	mission	mission	NOUN
cet-15373	121	15	4	4	NUM
cet-15373	121	16	component	component	NOUN
cet-15373	121	17	1	1	NUM
cet-15373	121	18	cup	cup	NOUN
cet-15373	121	19	j53d23007700006	j53d23007700006	NOUN
cet-15373	121	20	through	through	ADP
cet-15373	121	21	the	the	DET
cet-15373	121	22	prin	prin	NOUN
cet-15373	121	23	2022	2022	NUM
cet-15373	121	24	project	project	NOUN
cet-15373	121	25	hydream	hydream	NOUN
cet-15373	121	26	(	(	PUNCT
cet-15373	121	27	i	i	NOUN
cet-15373	121	28	d	d	PROPN
cet-15373	121	29	:	:	PUNCT
cet-15373	121	30	2022yxhxh5	2022yxhxh5	NUM
cet-15373	121	31	)	)	PUNCT
cet-15373	121	32	,	,	PUNCT
cet-15373	121	33	which	which	PRON
cet-15373	121	34	is	be	AUX
cet-15373	121	35	gratefully	gratefully	ADV
cet-15373	121	36	acknowledged	acknowledge	VERB
cet-15373	121	37	.	.	PUNCT
cet-15373	122	1	references	reference	NOUN
cet-15373	122	2	ampelli	ampelli	PROPN
cet-15373	122	3	,	,	PUNCT
cet-15373	122	4	c.	c.	PROPN
cet-15373	122	5	,	,	PUNCT
cet-15373	122	6	2020	2020	NUM
cet-15373	122	7	,	,	PUNCT
cet-15373	122	8	electrode	electrode	NOUN
cet-15373	122	9	design	design	NOUN
cet-15373	122	10	for	for	ADP
cet-15373	122	11	ammonia	ammonia	NOUN
cet-15373	122	12	synthesis	synthesis	NOUN
cet-15373	122	13	,	,	PUNCT
cet-15373	122	14	nature	nature	NOUN
cet-15373	122	15	catalysis	catalysis	NOUN
cet-15373	122	16	,	,	PUNCT
cet-15373	122	17	3(5	3(5	NUM
cet-15373	122	18	)	)	PUNCT
cet-15373	122	19	,	,	PUNCT
cet-15373	122	20	420–421	420–421	NUM
cet-15373	122	21	.	.	PUNCT
cet-15373	123	1	chen	chen	PROPN
cet-15373	123	2	,	,	PUNCT
cet-15373	123	3	s.	s.	PROPN
cet-15373	123	4	,	,	PUNCT
cet-15373	123	5	perathoner	perathoner	NOUN
cet-15373	123	6	,	,	PUNCT
cet-15373	123	7	s.	s.	PROPN
cet-15373	123	8	,	,	PUNCT
cet-15373	123	9	ampelli	ampelli	PROPN
cet-15373	123	10	,	,	PUNCT
cet-15373	123	11	c.	c.	PROPN
cet-15373	123	12	,	,	PUNCT
cet-15373	123	13	mebrahtu	mebrahtu	PROPN
cet-15373	123	14	,	,	PUNCT
cet-15373	123	15	c.	c.	PROPN
cet-15373	123	16	,	,	PUNCT
cet-15373	123	17	su	su	PROPN
cet-15373	123	18	,	,	PUNCT
cet-15373	123	19	d.	d.	PROPN
cet-15373	123	20	and	and	CCONJ
cet-15373	123	21	centi	centi	PROPN
cet-15373	123	22	,	,	PUNCT
cet-15373	123	23	g.	g.	PROPN
cet-15373	123	24	,	,	PUNCT
cet-15373	123	25	2017	2017	NUM
cet-15373	123	26	,	,	PUNCT
cet-15373	123	27	room	room	NOUN
cet-15373	123	28	-	-	PUNCT
cet-15373	123	29	temperature	temperature	NOUN
cet-15373	123	30	electrocatalytic	electrocatalytic	ADJ
cet-15373	123	31	synthesis	synthesis	NOUN
cet-15373	123	32	of	of	ADP
cet-15373	123	33	nh3	nh3	NOUN
cet-15373	123	34	from	from	ADP
cet-15373	123	35	h2o	h2o	PROPN
cet-15373	123	36	and	and	CCONJ
cet-15373	123	37	n2	n2	NOUN
cet-15373	123	38	in	in	ADP
cet-15373	123	39	a	a	DET
cet-15373	123	40	gas	gas	NOUN
cet-15373	123	41	–	–	PUNCT
cet-15373	123	42	liquid	liquid	ADJ
cet-15373	123	43	–	–	PUNCT
cet-15373	123	44	solid	solid	ADJ
cet-15373	123	45	three	three	NUM
cet-15373	123	46	-	-	PUNCT
cet-15373	123	47	phase	phase	NOUN
cet-15373	123	48	reactor	reactor	NOUN
cet-15373	123	49	,	,	PUNCT
cet-15373	123	50	acs	acs	PROPN
cet-15373	123	51	sustainable	sustainable	ADJ
cet-15373	123	52	chemistry	chemistry	NOUN
cet-15373	123	53	&	&	CCONJ
cet-15373	123	54	engineering	engineering	PROPN
cet-15373	123	55	,	,	PUNCT
cet-15373	123	56	5(8	5(8	NUM
cet-15373	123	57	)	)	PUNCT
cet-15373	123	58	,	,	PUNCT
cet-15373	123	59	7393–7400	7393–7400	NOUN
cet-15373	123	60	.	.	PUNCT
cet-15373	124	1	chen	chen	PROPN
cet-15373	124	2	,	,	PUNCT
cet-15373	124	3	s.	s.	PROPN
cet-15373	124	4	,	,	PUNCT
cet-15373	124	5	perathoner	perathoner	NOUN
cet-15373	124	6	,	,	PUNCT
cet-15373	124	7	s.	s.	PROPN
cet-15373	124	8	,	,	PUNCT
cet-15373	124	9	ampelli	ampelli	PROPN
cet-15373	124	10	,	,	PUNCT
cet-15373	124	11	c.	c.	PROPN
cet-15373	124	12	,	,	PUNCT
cet-15373	124	13	wei	wei	PROPN
cet-15373	124	14	,	,	PUNCT
cet-15373	124	15	h.	h.	PROPN
cet-15373	124	16	,	,	PUNCT
cet-15373	124	17	abate	abate	VERB
cet-15373	124	18	,	,	PUNCT
cet-15373	124	19	s.	s.	PROPN
cet-15373	124	20	,	,	PUNCT
cet-15373	124	21	zhang	zhang	PROPN
cet-15373	124	22	,	,	PUNCT
cet-15373	124	23	b.	b.	PROPN
cet-15373	124	24	and	and	CCONJ
cet-15373	124	25	centi	centi	PROPN
cet-15373	124	26	,	,	PUNCT
cet-15373	124	27	g.	g.	PROPN
cet-15373	124	28	,	,	PUNCT
cet-15373	124	29	2020	2020	NUM
cet-15373	124	30	,	,	PUNCT
cet-15373	124	31	enhanced	enhance	VERB
cet-15373	124	32	performance	performance	NOUN
cet-15373	124	33	in	in	ADP
cet-15373	124	34	the	the	DET
cet-15373	124	35	direct	direct	ADJ
cet-15373	124	36	electrocatalytic	electrocatalytic	ADJ
cet-15373	124	37	synthesis	synthesis	NOUN
cet-15373	124	38	of	of	ADP
cet-15373	124	39	ammonia	ammonia	NOUN
cet-15373	124	40	from	from	ADP
cet-15373	124	41	n2	n2	NOUN
cet-15373	124	42	and	and	CCONJ
cet-15373	124	43	h2o	h2o	NOUN
cet-15373	124	44	by	by	ADP
cet-15373	124	45	an	an	DET
cet-15373	124	46	in	in	ADP
cet-15373	124	47	-	-	PUNCT
cet-15373	124	48	situ	situ	ADJ
cet-15373	124	49	electrochemical	electrochemical	ADJ
cet-15373	124	50	activation	activation	NOUN
cet-15373	124	51	of	of	ADP
cet-15373	124	52	cnt	cnt	ADV
cet-15373	124	53	-	-	PUNCT
cet-15373	124	54	supported	support	VERB
cet-15373	124	55	iron	iron	NOUN
cet-15373	124	56	oxide	oxide	NOUN
cet-15373	124	57	nanoparticles	nanoparticle	NOUN
cet-15373	124	58	,	,	PUNCT
cet-15373	124	59	journal	journal	NOUN
cet-15373	124	60	of	of	ADP
cet-15373	124	61	energy	energy	NOUN
cet-15373	124	62	chemistry	chemistry	NOUN
cet-15373	124	63	,	,	PUNCT
cet-15373	124	64	49	49	NUM
cet-15373	124	65	,	,	PUNCT
cet-15373	124	66	22–32	22–32	NUM
cet-15373	124	67	.	.	PUNCT
cet-15373	125	1	einsle	einsle	PROPN
cet-15373	125	2	,	,	PUNCT
cet-15373	125	3	o.	o.	PROPN
cet-15373	125	4	,	,	PUNCT
cet-15373	125	5	2014	2014	NUM
cet-15373	125	6	,	,	PUNCT
cet-15373	125	7	nitrogenase	nitrogenase	NOUN
cet-15373	125	8	femo	femo	NOUN
cet-15373	125	9	cofactor	cofactor	NOUN
cet-15373	125	10	:	:	PUNCT
cet-15373	125	11	an	an	DET
cet-15373	125	12	atomic	atomic	ADJ
cet-15373	125	13	structure	structure	NOUN
cet-15373	125	14	in	in	ADP
cet-15373	125	15	three	three	NUM
cet-15373	125	16	simple	simple	ADJ
cet-15373	125	17	steps	step	NOUN
cet-15373	125	18	,	,	PUNCT
cet-15373	125	19	jbic	jbic	ADJ
cet-15373	125	20	journal	journal	NOUN
cet-15373	125	21	of	of	ADP
cet-15373	125	22	biological	biological	ADJ
cet-15373	125	23	inorganic	inorganic	ADJ
cet-15373	125	24	chemistry	chemistry	NOUN
cet-15373	125	25	,	,	PUNCT
cet-15373	125	26	19(6	19(6	NUM
cet-15373	125	27	)	)	PUNCT
cet-15373	125	28	,	,	PUNCT
cet-15373	125	29	737–745	737–745	NUM
cet-15373	125	30	.	.	PUNCT
cet-15373	126	1	giusi	giusi	PROPN
cet-15373	126	2	,	,	PUNCT
cet-15373	126	3	d.	d.	PROPN
cet-15373	126	4	,	,	PUNCT
cet-15373	126	5	miceli	miceli	PROPN
cet-15373	126	6	,	,	PUNCT
cet-15373	126	7	m.	m.	NOUN
cet-15373	126	8	,	,	PUNCT
cet-15373	126	9	genovese	genovese	NOUN
cet-15373	126	10	,	,	PUNCT
cet-15373	126	11	c.	c.	PROPN
cet-15373	126	12	,	,	PUNCT
cet-15373	126	13	centi	centi	PROPN
cet-15373	126	14	,	,	PUNCT
cet-15373	126	15	g.	g.	PROPN
cet-15373	126	16	,	,	PUNCT
cet-15373	126	17	perathoner	perathoner	NOUN
cet-15373	126	18	,	,	PUNCT
cet-15373	126	19	s.	s.	PROPN
cet-15373	126	20	and	and	CCONJ
cet-15373	126	21	ampelli	ampelli	PROPN
cet-15373	126	22	,	,	PUNCT
cet-15373	126	23	c.	c.	NOUN
cet-15373	126	24	,	,	PUNCT
cet-15373	126	25	2022	2022	NUM
cet-15373	126	26	,	,	PUNCT
cet-15373	126	27	,	,	PUNCT
cet-15373	126	28	in	in	ADP
cet-15373	126	29	situ	situ	ADJ
cet-15373	126	30	electrochemical	electrochemical	ADJ
cet-15373	126	31	characterization	characterization	NOUN
cet-15373	126	32	of	of	ADP
cet-15373	126	33	cuxo	cuxo	NOUN
cet-15373	126	34	-	-	PUNCT
cet-15373	126	35	based	base	VERB
cet-15373	126	36	gas	gas	NOUN
cet-15373	126	37	-	-	PUNCT
cet-15373	126	38	diffusion	diffusion	NOUN
cet-15373	126	39	electrodes	electrode	NOUN
cet-15373	126	40	(	(	PUNCT
cet-15373	126	41	gdes	gde	NOUN
cet-15373	126	42	)	)	PUNCT
cet-15373	126	43	for	for	ADP
cet-15373	126	44	co2	co2	VERB
cet-15373	126	45	electrocatalytic	electrocatalytic	ADJ
cet-15373	126	46	reduction	reduction	NOUN
cet-15373	126	47	in	in	ADP
cet-15373	126	48	presence	presence	NOUN
cet-15373	126	49	and	and	CCONJ
cet-15373	126	50	absence	absence	NOUN
cet-15373	126	51	of	of	ADP
cet-15373	126	52	liquid	liquid	ADJ
cet-15373	126	53	electrolyte	electrolyte	NOUN
cet-15373	126	54	and	and	CCONJ
cet-15373	126	55	relationship	relationship	NOUN
cet-15373	126	56	with	with	ADP
cet-15373	126	57	c2	c2	PROPN
cet-15373	126	58	+	+	CCONJ
cet-15373	126	59	products	product	NOUN
cet-15373	126	60	formation	formation	NOUN
cet-15373	126	61	,	,	PUNCT
cet-15373	126	62	applied	apply	VERB
cet-15373	126	63	catalysis	catalysis	NOUN
cet-15373	126	64	b	b	NOUN
cet-15373	126	65	:	:	PUNCT
cet-15373	126	66	environmental	environmental	ADJ
cet-15373	126	67	,	,	PUNCT
cet-15373	126	68	318	318	NUM
cet-15373	126	69	,	,	PUNCT
cet-15373	126	70	121845	121845	NUM
cet-15373	126	71	.	.	PUNCT
cet-15373	127	1	guo	guo	PROPN
cet-15373	127	2	,	,	PUNCT
cet-15373	127	3	x.-x	x.-x	PROPN
cet-15373	127	4	.	.	PROPN
cet-15373	127	5	,	,	PUNCT
cet-15373	127	6	du	du	PROPN
cet-15373	127	7	,	,	PUNCT
cet-15373	127	8	h.	h.	PROPN
cet-15373	127	9	,	,	PUNCT
cet-15373	127	10	qu	qu	PROPN
cet-15373	127	11	,	,	PUNCT
cet-15373	127	12	f.	f.	PROPN
cet-15373	127	13	and	and	CCONJ
cet-15373	127	14	li	li	PROPN
cet-15373	127	15	,	,	PUNCT
cet-15373	127	16	j.	j.	PROPN
cet-15373	127	17	,	,	PUNCT
cet-15373	127	18	2019	2019	NUM
cet-15373	127	19	,	,	PUNCT
cet-15373	127	20	recent	recent	ADJ
cet-15373	127	21	progress	progress	NOUN
cet-15373	127	22	in	in	ADP
cet-15373	127	23	electrocatalytic	electrocatalytic	ADJ
cet-15373	127	24	nitrogen	nitrogen	NOUN
cet-15373	127	25	reduction	reduction	NOUN
cet-15373	127	26	,	,	PUNCT
cet-15373	127	27	journal	journal	NOUN
cet-15373	127	28	of	of	ADP
cet-15373	127	29	materials	material	NOUN
cet-15373	127	30	chemistry	chemistry	NOUN
cet-15373	127	31	.	.	PUNCT
cet-15373	128	1	a	a	PRON
cet-15373	128	2	,	,	PUNCT
cet-15373	128	3	materials	material	NOUN
cet-15373	128	4	for	for	ADP
cet-15373	128	5	energy	energy	NOUN
cet-15373	128	6	and	and	CCONJ
cet-15373	128	7	sustainability	sustainability	NOUN
cet-15373	128	8	,	,	PUNCT
cet-15373	128	9	7(8	7(8	NUM
cet-15373	128	10	)	)	PUNCT
cet-15373	128	11	,	,	PUNCT
cet-15373	128	12	3531–3543	3531–3543	NUM
cet-15373	128	13	.	.	PUNCT
cet-15373	129	1	hirsch	hirsch	PROPN
cet-15373	129	2	,	,	PUNCT
cet-15373	129	3	a.	a.	NOUN
cet-15373	129	4	and	and	CCONJ
cet-15373	129	5	vostrowsky	vostrowsky	NOUN
cet-15373	129	6	,	,	PUNCT
cet-15373	129	7	o.	o.	PROPN
cet-15373	129	8	,	,	PUNCT
cet-15373	129	9	2005	2005	NUM
cet-15373	129	10	,	,	PUNCT
cet-15373	129	11	functionalization	functionalization	NOUN
cet-15373	129	12	of	of	ADP
cet-15373	129	13	carbon	carbon	NOUN
cet-15373	129	14	nanotubes	nanotube	NOUN
cet-15373	129	15	,	,	PUNCT
cet-15373	129	16	topics	topic	NOUN
cet-15373	129	17	in	in	ADP
cet-15373	129	18	current	current	ADJ
cet-15373	129	19	chemistry	chemistry	NOUN
cet-15373	129	20	,	,	PUNCT
cet-15373	129	21	193	193	NUM
cet-15373	129	22	–	–	SYM
cet-15373	129	23	237	237	NUM
cet-15373	129	24	.	.	PUNCT
cet-15373	130	1	li	li	PROPN
cet-15373	130	2	,	,	PUNCT
cet-15373	130	3	d.	d.	PROPN
cet-15373	130	4	,	,	PUNCT
cet-15373	130	5	zan	zan	PROPN
cet-15373	130	6	,	,	PUNCT
cet-15373	130	7	l.	l.	PROPN
cet-15373	130	8	,	,	PUNCT
cet-15373	130	9	chen	chen	PROPN
cet-15373	130	10	,	,	PUNCT
cet-15373	130	11	s.	s.	PROPN
cet-15373	130	12	,	,	PUNCT
cet-15373	130	13	shi	shi	PROPN
cet-15373	130	14	,	,	PUNCT
cet-15373	130	15	z.-j	z.-j	PROPN
cet-15373	130	16	.	.	PROPN
cet-15373	130	17	,	,	PUNCT
cet-15373	130	18	chen	chen	PROPN
cet-15373	130	19	,	,	PUNCT
cet-15373	130	20	p.	p.	PROPN
cet-15373	130	21	,	,	PUNCT
cet-15373	130	22	xi	xi	PROPN
cet-15373	130	23	,	,	PUNCT
cet-15373	130	24	z.	z.	PROPN
cet-15373	130	25	and	and	CCONJ
cet-15373	130	26	deng	deng	PROPN
cet-15373	130	27	,	,	PUNCT
cet-15373	130	28	d.	d.	PROPN
cet-15373	130	29	,	,	PUNCT
cet-15373	130	30	2022	2022	NUM
cet-15373	130	31	,	,	PUNCT
cet-15373	130	32	direct	direct	ADJ
cet-15373	130	33	conversion	conversion	NOUN
cet-15373	130	34	of	of	ADP
cet-15373	130	35	n2	n2	ADJ
cet-15373	130	36	and	and	CCONJ
cet-15373	130	37	o2	o2	PROPN
cet-15373	130	38	:	:	PUNCT
cet-15373	130	39	status	status	NOUN
cet-15373	130	40	,	,	PUNCT
cet-15373	130	41	challenge	challenge	NOUN
cet-15373	130	42	,	,	PUNCT
cet-15373	130	43	and	and	CCONJ
cet-15373	130	44	perspective	perspective	NOUN
cet-15373	130	45	,	,	PUNCT
cet-15373	130	46	national	national	ADJ
cet-15373	130	47	science	science	PROPN
cet-15373	130	48	review	review	PROPN
cet-15373	130	49	,	,	PUNCT
cet-15373	130	50	9(12	9(12	NUM
cet-15373	130	51	)	)	PUNCT
cet-15373	130	52	,	,	PUNCT
cet-15373	130	53	2095	2095	NUM
cet-15373	130	54	-	-	SYM
cet-15373	130	55	5138	5138	NUM
cet-15373	130	56	.	.	PUNCT
cet-15373	131	1	liu	liu	PROPN
cet-15373	131	2	,	,	PUNCT
cet-15373	131	3	m.	m.	NOUN
cet-15373	131	4	,	,	PUNCT
cet-15373	131	5	zhang	zhang	PROPN
cet-15373	131	6	,	,	PUNCT
cet-15373	131	7	s.	s.	PROPN
cet-15373	131	8	,	,	PUNCT
cet-15373	131	9	chen	chen	PROPN
cet-15373	131	10	,	,	PUNCT
cet-15373	131	11	m.	m.	NOUN
cet-15373	131	12	,	,	PUNCT
cet-15373	131	13	zhou	zhou	PROPN
cet-15373	131	14	,	,	PUNCT
cet-15373	131	15	s.	s.	PROPN
cet-15373	131	16	and	and	CCONJ
cet-15373	131	17	wu	wu	PROPN
cet-15373	131	18	,	,	PUNCT
cet-15373	131	19	l.	l.	PROPN
cet-15373	131	20	,	,	PUNCT
cet-15373	131	21	2023	2023	NUM
cet-15373	131	22	,	,	PUNCT
cet-15373	131	23	an	an	DET
cet-15373	131	24	isolated	isolated	ADJ
cet-15373	131	25	bimetallic	bimetallic	ADJ
cet-15373	131	26	fe	fe	X
cet-15373	131	27	–	–	PUNCT
cet-15373	131	28	ru	ru	PROPN
cet-15373	131	29	single	single	ADJ
cet-15373	131	30	-	-	PUNCT
cet-15373	131	31	atom	atom	NOUN
cet-15373	131	32	catalyst	catalyst	NOUN
cet-15373	131	33	for	for	ADP
cet-15373	131	34	efficient	efficient	ADJ
cet-15373	131	35	electrochemical	electrochemical	ADJ
cet-15373	131	36	nitrogen	nitrogen	NOUN
cet-15373	131	37	reduction	reduction	NOUN
cet-15373	131	38	,	,	PUNCT
cet-15373	131	39	journal	journal	NOUN
cet-15373	131	40	of	of	ADP
cet-15373	131	41	materials	material	NOUN
cet-15373	131	42	chemistry	chemistry	NOUN
cet-15373	131	43	a	a	PRON
cet-15373	131	44	,	,	PUNCT
cet-15373	131	45	11(27	11(27	NUM
cet-15373	131	46	)	)	PUNCT
cet-15373	131	47	,	,	PUNCT
cet-15373	131	48	14900–14910	14900–14910	NUM
cet-15373	131	49	.	.	PUNCT
cet-15373	131	50	park	park	PROPN
cet-15373	131	51	,	,	PUNCT
cet-15373	131	52	j.	j.	PROPN
cet-15373	131	53	,	,	PUNCT
cet-15373	131	54	ko	ko	PROPN
cet-15373	131	55	,	,	PUNCT
cet-15373	131	56	y.	y.	PROPN
cet-15373	131	57	j.	j.	PROPN
cet-15373	131	58	,	,	PUNCT
cet-15373	131	59	lim	lim	PROPN
cet-15373	131	60	,	,	PUNCT
cet-15373	131	61	c.	c.	PROPN
cet-15373	131	62	,	,	PUNCT
cet-15373	131	63	kim	kim	PROPN
cet-15373	131	64	,	,	PUNCT
cet-15373	131	65	h.	h.	PROPN
cet-15373	131	66	,	,	PUNCT
cet-15373	131	67	min	min	PROPN
cet-15373	131	68	,	,	PUNCT
cet-15373	131	69	b.	b.	PROPN
cet-15373	131	70	k.	k.	PROPN
cet-15373	131	71	,	,	PUNCT
cet-15373	131	72	lee	lee	PROPN
cet-15373	131	73	,	,	PUNCT
cet-15373	131	74	k.	k.	PROPN
cet-15373	131	75	y.	y.	PROPN
cet-15373	131	76	,	,	PUNCT
cet-15373	131	77	koh	koh	PROPN
cet-15373	131	78	,	,	PUNCT
cet-15373	131	79	j.	j.	PROPN
cet-15373	131	80	h.	h.	PROPN
cet-15373	131	81	,	,	PUNCT
cet-15373	131	82	oh	oh	INTJ
cet-15373	131	83	,	,	PUNCT
cet-15373	131	84	h.	h.	PROPN
cet-15373	131	85	s.	s.	PROPN
cet-15373	131	86	,	,	PUNCT
cet-15373	131	87	&	&	CCONJ
cet-15373	131	88	lee	lee	PROPN
cet-15373	131	89	,	,	PUNCT
cet-15373	131	90	w.	w.	PROPN
cet-15373	131	91	h.	h.	PROPN
cet-15373	131	92	,	,	PUNCT
cet-15373	131	93	2023	2023	NUM
cet-15373	131	94	,	,	PUNCT
cet-15373	131	95	strategies	strategy	NOUN
cet-15373	131	96	for	for	ADP
cet-15373	131	97	co2	co2	NOUN
cet-15373	131	98	electroreduction	electroreduction	NOUN
cet-15373	131	99	in	in	ADP
cet-15373	131	100	cation	cation	NOUN
cet-15373	131	101	exchange	exchange	NOUN
cet-15373	131	102	membrane	membrane	NOUN
cet-15373	131	103	electrode	electrode	NOUN
cet-15373	131	104	assembly	assembly	NOUN
cet-15373	131	105	,	,	PUNCT
cet-15373	131	106	chemical	chemical	ADJ
cet-15373	131	107	engineering	engineering	NOUN
cet-15373	131	108	journal	journal	NOUN
cet-15373	131	109	,	,	PUNCT
cet-15373	131	110	453	453	NUM
cet-15373	131	111	,	,	PUNCT
cet-15373	131	112	139826–139826	139826–139826	NUM
cet-15373	131	113	.	.	PUNCT
cet-15373	132	1	rafiqul	rafiqul	PROPN
cet-15373	132	2	,	,	PUNCT
cet-15373	132	3	i.	i.	PROPN
cet-15373	132	4	,	,	PUNCT
cet-15373	132	5	weber	weber	PROPN
cet-15373	132	6	,	,	PUNCT
cet-15373	132	7	c.	c.	PROPN
cet-15373	132	8	,	,	PUNCT
cet-15373	132	9	lehmann	lehmann	PROPN
cet-15373	132	10	,	,	PUNCT
cet-15373	132	11	b.	b.	PROPN
cet-15373	132	12	and	and	CCONJ
cet-15373	132	13	voss	voss	PROPN
cet-15373	132	14	,	,	PUNCT
cet-15373	132	15	a.	a.	PROPN
cet-15373	132	16	,	,	PUNCT
cet-15373	132	17	2005	2005	NUM
cet-15373	132	18	,	,	PUNCT
cet-15373	132	19	energy	energy	NOUN
cet-15373	132	20	efficiency	efficiency	NOUN
cet-15373	132	21	improvements	improvement	NOUN
cet-15373	132	22	in	in	ADP
cet-15373	132	23	ammonia	ammonia	NOUN
cet-15373	132	24	production	production	NOUN
cet-15373	132	25	—	—	PUNCT
cet-15373	132	26	perspectives	perspective	NOUN
cet-15373	132	27	and	and	CCONJ
cet-15373	132	28	uncertainties	uncertainty	NOUN
cet-15373	132	29	,	,	PUNCT
cet-15373	132	30	energy	energy	NOUN
cet-15373	132	31	,	,	PUNCT
cet-15373	132	32	30(13	30(13	NUM
cet-15373	132	33	)	)	PUNCT
cet-15373	132	34	,	,	PUNCT
cet-15373	132	35	2487–2504	2487–2504	NUM
cet-15373	132	36	.	.	PUNCT
cet-15373	133	1	rouwenhorst	rouwenhorst	PROPN
cet-15373	133	2	,	,	PUNCT
cet-15373	133	3	k.h.r	k.h.r	PROPN
cet-15373	133	4	.	.	PROPN
cet-15373	133	5	,	,	PUNCT
cet-15373	133	6	krzywda	krzywda	PROPN
cet-15373	133	7	,	,	PUNCT
cet-15373	133	8	p.m.	p.m.	NOUN
cet-15373	133	9	,	,	PUNCT
cet-15373	133	10	benes	benes	PROPN
cet-15373	133	11	,	,	PUNCT
cet-15373	133	12	n.e	n.e	PROPN
cet-15373	133	13	.	.	PROPN
cet-15373	133	14	,	,	PUNCT
cet-15373	133	15	mul	mul	PROPN
cet-15373	133	16	,	,	PUNCT
cet-15373	133	17	g.	g.	PROPN
cet-15373	133	18	and	and	CCONJ
cet-15373	133	19	lefferts	leffert	NOUN
cet-15373	133	20	,	,	PUNCT
cet-15373	133	21	l.	l.	PROPN
cet-15373	133	22	,	,	PUNCT
cet-15373	133	23	2021	2021	NUM
cet-15373	133	24	,	,	PUNCT
cet-15373	133	25	ammonia	ammonia	NOUN
cet-15373	133	26	production	production	NOUN
cet-15373	133	27	technologies	technology	NOUN
cet-15373	133	28	,	,	PUNCT
cet-15373	133	29	 	 	SPACE
cet-15373	133	30	techno	techno	NOUN
cet-15373	133	31	-	-	PUNCT
cet-15373	133	32	economic	economic	ADJ
cet-15373	133	33	challenges	challenge	NOUN
cet-15373	133	34	of	of	ADP
cet-15373	133	35	green	green	ADJ
cet-15373	133	36	ammonia	ammonia	NOUN
cet-15373	133	37	as	as	ADP
cet-15373	133	38	an	an	DET
cet-15373	133	39	energy	energy	NOUN
cet-15373	133	40	vector	vector	NOUN
cet-15373	133	41	,	,	PUNCT
cet-15373	133	42	41–83	41–83	NUM
cet-15373	133	43	.	.	PUNCT
cet-15373	134	1	sahoo	sahoo	PROPN
cet-15373	134	2	,	,	PUNCT
cet-15373	134	3	s.	s.	PROPN
cet-15373	134	4	k.	k.	PROPN
cet-15373	134	5	,	,	PUNCT
cet-15373	134	6	agarwal	agarwal	PROPN
cet-15373	134	7	,	,	PUNCT
cet-15373	134	8	k.	k.	PROPN
cet-15373	134	9	,	,	PUNCT
cet-15373	134	10	singh	singh	PROPN
cet-15373	134	11	,	,	PUNCT
cet-15373	134	12	a.	a.	PROPN
cet-15373	134	13	k.	k.	PROPN
cet-15373	134	14	,	,	PUNCT
cet-15373	134	15	polke	polke	ADV
cet-15373	134	16	,	,	PUNCT
cet-15373	134	17	b.	b.	PROPN
cet-15373	134	18	g.	g.	PROPN
cet-15373	134	19	,	,	PUNCT
cet-15373	134	20	and	and	CCONJ
cet-15373	134	21	raha	raha	PROPN
cet-15373	134	22	,	,	PUNCT
cet-15373	134	23	k.	k.	PROPN
cet-15373	134	24	c.	c.	PROPN
cet-15373	134	25	,	,	PUNCT
cet-15373	134	26	2011	2011	NUM
cet-15373	134	27	,	,	PUNCT
cet-15373	134	28	characterization	characterization	NOUN
cet-15373	134	29	of	of	ADP
cet-15373	134	30	γ	γ	PROPN
cet-15373	134	31	and	and	CCONJ
cet-15373	134	32	αfe2o3	αfe2o3	NOUN
cet-15373	134	33	nano	nano	NOUN
cet-15373	134	34	powders	powder	NOUN
cet-15373	134	35	synthesized	synthesize	VERB
cet-15373	134	36	by	by	ADP
cet-15373	134	37	emulsion	emulsion	NOUN
cet-15373	134	38	precipitation	precipitation	NOUN
cet-15373	134	39	-	-	PUNCT
cet-15373	134	40	calcination	calcination	NOUN
cet-15373	134	41	route	route	NOUN
cet-15373	134	42	and	and	CCONJ
cet-15373	134	43	rheological	rheological	ADJ
cet-15373	134	44	behaviour	behaviour	NOUN
cet-15373	134	45	of	of	ADP
cet-15373	134	46	α	α	PROPN
cet-15373	134	47	-	-	PUNCT
cet-15373	134	48	fe2o3	fe2o3	ADJ
cet-15373	134	49	,	,	PUNCT
cet-15373	134	50	international	international	ADJ
cet-15373	134	51	journal	journal	NOUN
cet-15373	134	52	of	of	ADP
cet-15373	134	53	engineering	engineering	NOUN
cet-15373	134	54	,	,	PUNCT
cet-15373	134	55	science	science	NOUN
cet-15373	134	56	and	and	CCONJ
cet-15373	134	57	technology	technology	NOUN
cet-15373	134	58	,	,	PUNCT
cet-15373	134	59	2(8	2(8	NUM
cet-15373	134	60	)	)	PUNCT
cet-15373	134	61	.	.	PUNCT
cet-15373	135	1	schrock	schrock	PROPN
cet-15373	135	2	,	,	PUNCT
cet-15373	135	3	r.r	r.r	PROPN
cet-15373	135	4	.	.	PROPN
cet-15373	135	5	,	,	PUNCT
cet-15373	135	6	2006	2006	NUM
cet-15373	135	7	,	,	PUNCT
cet-15373	135	8	reduction	reduction	NOUN
cet-15373	135	9	of	of	ADP
cet-15373	135	10	dinitrogen	dinitrogen	NOUN
cet-15373	135	11	,	,	PUNCT
cet-15373	135	12	proceedings	proceeding	NOUN
cet-15373	135	13	of	of	ADP
cet-15373	135	14	the	the	DET
cet-15373	135	15	national	national	PROPN
cet-15373	135	16	academy	academy	PROPN
cet-15373	135	17	of	of	ADP
cet-15373	135	18	sciences	sciences	PROPN
cet-15373	135	19	,	,	PUNCT
cet-15373	135	20	103(46	103(46	NUM
cet-15373	135	21	)	)	PUNCT
cet-15373	135	22	,	,	PUNCT
cet-15373	135	23	17087–17087	17087–17087	NUM
cet-15373	135	24	tavella	tavella	NOUN
cet-15373	135	25	,	,	PUNCT
cet-15373	135	26	f.	f.	PROPN
cet-15373	135	27	,	,	PUNCT
cet-15373	135	28	giusi	giusi	PROPN
cet-15373	135	29	,	,	PUNCT
cet-15373	135	30	d.	d.	PROPN
cet-15373	135	31	and	and	CCONJ
cet-15373	135	32	ampelli	ampelli	PROPN
cet-15373	135	33	,	,	PUNCT
cet-15373	135	34	c.	c.	NOUN
cet-15373	135	35	,	,	PUNCT
cet-15373	135	36	2022	2022	NUM
cet-15373	135	37	,	,	PUNCT
cet-15373	135	38	nitrogen	nitrogen	NOUN
cet-15373	135	39	reduction	reduction	NOUN
cet-15373	135	40	reaction	reaction	NOUN
cet-15373	135	41	to	to	ADP
cet-15373	135	42	ammonia	ammonia	NOUN
cet-15373	135	43	at	at	ADP
cet-15373	135	44	ambient	ambient	ADJ
cet-15373	135	45	conditions	condition	NOUN
cet-15373	135	46	:	:	PUNCT
cet-15373	135	47	a	a	DET
cet-15373	135	48	short	short	ADJ
cet-15373	135	49	review	review	NOUN
cet-15373	135	50	analysis	analysis	NOUN
cet-15373	135	51	of	of	ADP
cet-15373	135	52	the	the	DET
cet-15373	135	53	critical	critical	ADJ
cet-15373	135	54	factors	factor	NOUN
cet-15373	135	55	limiting	limit	VERB
cet-15373	135	56	electrocatalytic	electrocatalytic	ADJ
cet-15373	135	57	performance	performance	NOUN
cet-15373	135	58	,	,	PUNCT
cet-15373	135	59	current	current	ADJ
cet-15373	135	60	opinion	opinion	NOUN
cet-15373	135	61	in	in	ADP
cet-15373	135	62	green	green	ADJ
cet-15373	135	63	and	and	CCONJ
cet-15373	135	64	sustainable	sustainable	ADJ
cet-15373	135	65	chemistry	chemistry	NOUN
cet-15373	135	66	,	,	PUNCT
cet-15373	135	67	35	35	NUM
cet-15373	135	68	,	,	PUNCT
cet-15373	135	69	100604	100604	NUM
cet-15373	135	70	.	.	PUNCT
cet-15373	136	1	tian	tian	ADJ
cet-15373	136	2	,	,	PUNCT
cet-15373	136	3	y.	y.	PROPN
cet-15373	136	4	,	,	PUNCT
cet-15373	136	5	liu	liu	PROPN
cet-15373	136	6	,	,	PUNCT
cet-15373	136	7	y.	y.	PROPN
cet-15373	136	8	,	,	PUNCT
cet-15373	136	9	wang	wang	PROPN
cet-15373	136	10	,	,	PUNCT
cet-15373	136	11	h.	h.	PROPN
cet-15373	136	12	,	,	PUNCT
cet-15373	136	13	liu	liu	PROPN
cet-15373	136	14	,	,	PUNCT
cet-15373	136	15	l.	l.	PROPN
cet-15373	136	16	and	and	CCONJ
cet-15373	136	17	hu	hu	PROPN
cet-15373	136	18	,	,	PUNCT
cet-15373	136	19	w.	w.	PROPN
cet-15373	136	20	,	,	PUNCT
cet-15373	136	21	2022	2022	NUM
cet-15373	136	22	,	,	PUNCT
cet-15373	136	23	electrocatalytic	electrocatalytic	ADJ
cet-15373	136	24	reduction	reduction	NOUN
cet-15373	136	25	of	of	ADP
cet-15373	136	26	nitrogen	nitrogen	NOUN
cet-15373	136	27	to	to	ADP
cet-15373	136	28	ammonia	ammonia	NOUN
cet-15373	136	29	in	in	ADP
cet-15373	136	30	ionic	ionic	ADJ
cet-15373	136	31	liquids	liquid	NOUN
cet-15373	136	32	,	,	PUNCT
cet-15373	136	33	acs	acs	PROPN
cet-15373	136	34	sustainable	sustainable	ADJ
cet-15373	136	35	chemistry	chemistry	NOUN
cet-15373	136	36	&	&	CCONJ
cet-15373	136	37	engineering	engineering	PROPN
cet-15373	136	38	,	,	PUNCT
cet-15373	136	39	10(14	10(14	NUM
cet-15373	136	40	)	)	PUNCT
cet-15373	136	41	,	,	PUNCT
cet-15373	136	42	4345–4358	4345–4358	NOUN
cet-15373	136	43	.	.	PUNCT
cet-15373	137	1	738	738	NUM
cet-15373	137	2	cet-vol117-b.pdf	cet-vol117-b.pdf	NUM
cet-15373	137	3	147miceli.pdf	147miceli.pdf	NUM
cet-15373	137	4	activation	activation	NOUN
cet-15373	137	5	of	of	ADP
cet-15373	137	6	dinitrogen	dinitrogen	NOUN
cet-15373	137	7	molecule	molecule	NOUN
cet-15373	137	8	(	(	PUNCT
cet-15373	137	9	n2	n2	NOUN
cet-15373	137	10	)	)	PUNCT
cet-15373	137	11	in	in	ADP
cet-15373	137	12	unconventional	unconventional	ADJ
cet-15373	137	13	electrochemical	electrochemical	ADJ
cet-15373	137	14	reactors	reactor	NOUN
cet-15373	137	15	for	for	ADP
cet-15373	137	16	ammonia	ammonia	ADJ
cet-15373	137	17	production	production	NOUN
