id	sid	tid	token	lemma	pos
cet-15688	1	1	doi	doi	NOUN
cet-15688	1	2	:	:	PUNCT
cet-15688	1	3	10.3303	10.3303	NUM
cet-15688	1	4	/	/	SYM
cet-15688	1	5	cet25120063	cet25120063	ADJ
cet-15688	1	6	paper	paper	NOUN
cet-15688	1	7	received	receive	VERB
cet-15688	1	8	:	:	PUNCT
cet-15688	1	9	13/04/2025	13/04/2025	NUM
cet-15688	1	10	;	;	PUNCT
cet-15688	1	11	revised	revise	VERB
cet-15688	1	12	:	:	PUNCT
cet-15688	1	13	17	17	NUM
cet-15688	1	14	july	july	PROPN
cet-15688	1	15	2025	2025	NUM
cet-15688	1	16	;	;	PUNCT
cet-15688	1	17	accepted	accept	VERB
cet-15688	1	18	:	:	PUNCT
cet-15688	1	19	2	2	NUM
cet-15688	1	20	september	september	PROPN
cet-15688	1	21	2025	2025	NUM
cet-15688	1	22	please	please	INTJ
cet-15688	1	23	cite	cite	VERB
cet-15688	1	24	this	this	DET
cet-15688	1	25	article	article	NOUN
cet-15688	1	26	as	as	ADP
cet-15688	1	27	:	:	PUNCT
cet-15688	1	28	tscvetkov	tscvetkov	X
cet-15688	2	1	d.y	d.y	PROPN
cet-15688	2	2	.	.	PROPN
cet-15688	2	3	,	,	PUNCT
cet-15688	2	4	kuragin	kuragin	PROPN
cet-15688	2	5	a.a	a.a	PROPN
cet-15688	2	6	.	.	PROPN
cet-15688	2	7	,	,	PUNCT
cet-15688	2	8	markova	markova	X
cet-15688	3	1	m.e	m.e	PROPN
cet-15688	3	2	.	.	PROPN
cet-15688	3	3	,	,	PUNCT
cet-15688	3	4	bahvalova	bahvalova	PROPN
cet-15688	3	5	e.s	e.s	PROPN
cet-15688	3	6	.	.	PROPN
cet-15688	3	7	,	,	PUNCT
cet-15688	3	8	sidorov	sidorov	PROPN
cet-15688	3	9	a.i	a.i	PROPN
cet-15688	3	10	.	.	PROPN
cet-15688	3	11	,	,	PUNCT
cet-15688	3	12	lakina	lakina	PROPN
cet-15688	3	13	n.v	n.v	PROPN
cet-15688	3	14	.	.	PROPN
cet-15688	3	15	,	,	PUNCT
cet-15688	3	16	sulman	sulman	ADJ
cet-15688	3	17	m.	m.	NOUN
cet-15688	3	18	,	,	PUNCT
cet-15688	3	19	doluda	doluda	NOUN
cet-15688	3	20	v.y	v.y	PROPN
cet-15688	3	21	.	.	PROPN
cet-15688	3	22	,	,	PUNCT
cet-15688	3	23	2025	2025	NUM
cet-15688	3	24	,	,	PUNCT
cet-15688	3	25	cu	cu	PROPN
cet-15688	3	26	,	,	PUNCT
cet-15688	3	27	ni	ni	PROPN
cet-15688	3	28	,	,	PUNCT
cet-15688	3	29	pt	pt	PROPN
cet-15688	3	30	bimetallic	bimetallic	PROPN
cet-15688	3	31	microporous	microporous	ADJ
cet-15688	3	32	supported	support	VERB
cet-15688	3	33	silica	silica	NOUN
cet-15688	3	34	catalysts	catalyst	NOUN
cet-15688	3	35	for	for	ADP
cet-15688	3	36	direct	direct	ADJ
cet-15688	3	37	formaldehyde	formaldehyde	NOUN
cet-15688	3	38	synthesis	synthesis	NOUN
cet-15688	3	39	from	from	ADP
cet-15688	3	40	carbon	carbon	NOUN
cet-15688	3	41	dioxide	dioxide	NOUN
cet-15688	3	42	and	and	CCONJ
cet-15688	3	43	hydrogen	hydrogen	NOUN
cet-15688	3	44	,	,	PUNCT
cet-15688	3	45	chemical	chemical	ADJ
cet-15688	3	46	engineering	engineering	NOUN
cet-15688	3	47	transactions	transaction	NOUN
cet-15688	3	48	,	,	PUNCT
cet-15688	3	49	120	120	NUM
cet-15688	3	50	,	,	PUNCT
cet-15688	3	51	373	373	NUM
cet-15688	3	52	-	-	SYM
cet-15688	3	53	378	378	NUM
cet-15688	3	54	doi:10.3303	doi:10.3303	NOUN
cet-15688	3	55	/	/	SYM
cet-15688	3	56	cet25120063	cet25120063	NOUN
cet-15688	3	57	chemical	chemical	PROPN
cet-15688	3	58	engineering	engineering	NOUN
cet-15688	3	59	transactions	transaction	NOUN
cet-15688	3	60	vol	vol	NOUN
cet-15688	3	61	.	.	PUNCT
cet-15688	4	1	120	120	NUM
cet-15688	4	2	,	,	PUNCT
cet-15688	4	3	2025	2025	NUM
cet-15688	4	4	a	a	DET
cet-15688	4	5	publication	publication	NOUN
cet-15688	4	6	of	of	ADP
cet-15688	4	7	the	the	DET
cet-15688	4	8	italian	italian	ADJ
cet-15688	4	9	association	association	NOUN
cet-15688	4	10	of	of	ADP
cet-15688	4	11	chemical	chemical	PROPN
cet-15688	4	12	engineering	engineering	NOUN
cet-15688	4	13	online	online	ADV
cet-15688	4	14	at	at	ADP
cet-15688	4	15	www.cetjournal.it	www.cetjournal.it	PROPN
cet-15688	4	16	guest	guest	NOUN
cet-15688	4	17	editors	editor	NOUN
cet-15688	4	18	:	:	PUNCT
cet-15688	4	19	bing	bing	NOUN
cet-15688	4	20	shen	shen	NOUN
cet-15688	5	1	how	how	SCONJ
cet-15688	5	2	,	,	PUNCT
cet-15688	5	3	viknesh	viknesh	ADJ
cet-15688	5	4	andiappan	andiappan	NOUN
cet-15688	5	5	,	,	PUNCT
cet-15688	5	6	denny	denny	PROPN
cet-15688	5	7	k.s	k.s	PROPN
cet-15688	5	8	.	.	PROPN
cet-15688	5	9	ng	ng	PROPN
cet-15688	5	10	,	,	PUNCT
cet-15688	5	11	hon	hon	PROPN
cet-15688	5	12	loong	loong	PROPN
cet-15688	5	13	lam	lam	PROPN
cet-15688	5	14	,	,	PUNCT
cet-15688	5	15	petar	petar	PROPN
cet-15688	5	16	s.	s.	PROPN
cet-15688	5	17	varbanov	varbanov	PROPN
cet-15688	5	18	copyright	copyright	NOUN
cet-15688	5	19	©	©	PROPN
cet-15688	5	20	2025	2025	NUM
cet-15688	5	21	,	,	PUNCT
cet-15688	5	22	aidic	aidic	ADJ
cet-15688	5	23	servizi	servizi	PROPN
cet-15688	5	24	s.r.l	s.r.l	NOUN
cet-15688	5	25	.	.	PUNCT
cet-15688	6	1	isbn	isbn	PROPN
cet-15688	6	2	979	979	NUM
cet-15688	6	3	-	-	SYM
cet-15688	6	4	12	12	NUM
cet-15688	6	5	-	-	PUNCT
cet-15688	6	6	81206	81206	NUM
cet-15688	6	7	-	-	PUNCT
cet-15688	6	8	21	21	NUM
cet-15688	6	9	-	-	SYM
cet-15688	6	10	2	2	NUM
cet-15688	6	11	;	;	PUNCT
cet-15688	6	12	issn	issn	PROPN
cet-15688	6	13	2283	2283	NUM
cet-15688	6	14	-	-	SYM
cet-15688	6	15	9216	9216	NUM
cet-15688	6	16	cu	cu	PROPN
cet-15688	6	17	,	,	PUNCT
cet-15688	6	18	ni	ni	PROPN
cet-15688	6	19	,	,	PUNCT
cet-15688	6	20	pt	pt	PROPN
cet-15688	6	21	bimetallic	bimetallic	PROPN
cet-15688	6	22	microporous	microporous	ADJ
cet-15688	6	23	supported	support	VERB
cet-15688	6	24	silica	silica	NOUN
cet-15688	6	25	catalysts	catalyst	NOUN
cet-15688	6	26	for	for	ADP
cet-15688	6	27	direct	direct	ADJ
cet-15688	6	28	formaldehyde	formaldehyde	NOUN
cet-15688	6	29	synthesis	synthesis	NOUN
cet-15688	6	30	from	from	ADP
cet-15688	6	31	carbon	carbon	NOUN
cet-15688	6	32	dioxide	dioxide	NOUN
cet-15688	6	33	and	and	CCONJ
cet-15688	6	34	hydrogen	hydrogen	NOUN
cet-15688	6	35	dmitrii	dmitrii	PROPN
cet-15688	6	36	y.	y.	PROPN
cet-15688	6	37	tscvetkov	tscvetkov	PROPN
cet-15688	6	38	,	,	PUNCT
cet-15688	6	39	alexey	alexey	PROPN
cet-15688	6	40	a.	a.	PROPN
cet-15688	6	41	kuragin	kuragin	PROPN
cet-15688	6	42	,	,	PUNCT
cet-15688	6	43	mariia	mariia	PROPN
cet-15688	6	44	e.	e.	PROPN
cet-15688	6	45	markova	markova	PROPN
cet-15688	6	46	,	,	PUNCT
cet-15688	6	47	elena	elena	PROPN
cet-15688	6	48	s.	s.	PROPN
cet-15688	6	49	bahvalova	bahvalova	PROPN
cet-15688	6	50	,	,	PUNCT
cet-15688	6	51	alexander	alexander	PROPN
cet-15688	6	52	i.	i.	PROPN
cet-15688	6	53	sidorov	sidorov	PROPN
cet-15688	6	54	,	,	PUNCT
cet-15688	6	55	natalia	natalia	PROPN
cet-15688	6	56	v.	v.	PROPN
cet-15688	6	57	lakina	lakina	PROPN
cet-15688	6	58	,	,	PUNCT
cet-15688	6	59	mikhail	mikhail	PROPN
cet-15688	6	60	g.	g.	PROPN
cet-15688	6	61	sulman	sulman	PROPN
cet-15688	6	62	,	,	PUNCT
cet-15688	6	63	valentin	valentin	PROPN
cet-15688	6	64	y.	y.	PROPN
cet-15688	6	65	doluda	doluda	PROPN
cet-15688	6	66	*	*	PUNCT
cet-15688	6	67	tver	tver	PROPN
cet-15688	6	68	state	state	PROPN
cet-15688	6	69	technical	technical	PROPN
cet-15688	6	70	university	university	PROPN
cet-15688	6	71	,	,	PUNCT
cet-15688	6	72	170026	170026	NUM
cet-15688	6	73	,	,	PUNCT
cet-15688	6	74	a.nikitina	a.nikitina	ADP
cet-15688	6	75	str	str	PROPN
cet-15688	6	76	.	.	PUNCT
cet-15688	6	77	,	,	PUNCT
cet-15688	6	78	22	22	NUM
cet-15688	6	79	,	,	PUNCT
cet-15688	6	80	tver	tver	PROPN
cet-15688	6	81	,	,	PUNCT
cet-15688	6	82	russia	russia	PROPN
cet-15688	6	83	,	,	PUNCT
cet-15688	6	84	doludav@yandex.ru	doludav@yandex.ru	VERB
cet-15688	6	85	an	an	DET
cet-15688	6	86	increase	increase	NOUN
cet-15688	6	87	in	in	ADP
cet-15688	6	88	world	world	NOUN
cet-15688	6	89	greenhouse	greenhouse	NOUN
cet-15688	6	90	gas	gas	NOUN
cet-15688	6	91	emissions	emission	NOUN
cet-15688	6	92	requires	require	VERB
cet-15688	6	93	the	the	DET
cet-15688	6	94	development	development	NOUN
cet-15688	6	95	of	of	ADP
cet-15688	6	96	modern	modern	ADJ
cet-15688	6	97	technologies	technology	NOUN
cet-15688	6	98	for	for	ADP
cet-15688	6	99	converting	convert	VERB
cet-15688	6	100	them	they	PRON
cet-15688	6	101	into	into	ADP
cet-15688	6	102	valuable	valuable	ADJ
cet-15688	6	103	substances	substance	NOUN
cet-15688	6	104	and	and	CCONJ
cet-15688	6	105	eliminating	eliminate	VERB
cet-15688	6	106	their	their	PRON
cet-15688	6	107	formation	formation	NOUN
cet-15688	6	108	during	during	ADP
cet-15688	6	109	various	various	ADJ
cet-15688	6	110	technological	technological	ADJ
cet-15688	6	111	and	and	CCONJ
cet-15688	6	112	economic	economic	ADJ
cet-15688	6	113	processes	process	NOUN
cet-15688	6	114	.	.	PUNCT
cet-15688	7	1	one	one	NUM
cet-15688	7	2	of	of	ADP
cet-15688	7	3	the	the	DET
cet-15688	7	4	possible	possible	ADJ
cet-15688	7	5	ways	way	NOUN
cet-15688	7	6	to	to	PART
cet-15688	7	7	solve	solve	VERB
cet-15688	7	8	this	this	DET
cet-15688	7	9	problem	problem	NOUN
cet-15688	7	10	is	be	AUX
cet-15688	7	11	the	the	DET
cet-15688	7	12	development	development	NOUN
cet-15688	7	13	of	of	ADP
cet-15688	7	14	sustainable	sustainable	ADJ
cet-15688	7	15	methods	method	NOUN
cet-15688	7	16	for	for	ADP
cet-15688	7	17	producing	produce	VERB
cet-15688	7	18	widely	widely	ADV
cet-15688	7	19	used	use	VERB
cet-15688	7	20	products	product	NOUN
cet-15688	7	21	that	that	PRON
cet-15688	7	22	can	can	AUX
cet-15688	7	23	be	be	AUX
cet-15688	7	24	applied	apply	VERB
cet-15688	7	25	in	in	ADP
cet-15688	7	26	different	different	ADJ
cet-15688	7	27	sectors	sector	NOUN
cet-15688	7	28	of	of	ADP
cet-15688	7	29	the	the	DET
cet-15688	7	30	modern	modern	ADJ
cet-15688	7	31	economy	economy	NOUN
cet-15688	7	32	.	.	PUNCT
cet-15688	8	1	formaldehyde	formaldehyde	NOUN
cet-15688	8	2	is	be	AUX
cet-15688	8	3	one	one	NUM
cet-15688	8	4	of	of	ADP
cet-15688	8	5	the	the	DET
cet-15688	8	6	largest	large	ADJ
cet-15688	8	7	-	-	PUNCT
cet-15688	8	8	scale	scale	NOUN
cet-15688	8	9	chemicals	chemical	NOUN
cet-15688	8	10	used	use	VERB
cet-15688	8	11	in	in	ADP
cet-15688	8	12	chemical	chemical	NOUN
cet-15688	8	13	processes	process	NOUN
cet-15688	8	14	.	.	PUNCT
cet-15688	9	1	modern	modern	ADJ
cet-15688	9	2	industrial	industrial	ADJ
cet-15688	9	3	methods	method	NOUN
cet-15688	9	4	rely	rely	VERB
cet-15688	9	5	on	on	ADP
cet-15688	9	6	the	the	DET
cet-15688	9	7	oxidation	oxidation	NOUN
cet-15688	9	8	of	of	ADP
cet-15688	9	9	methanol	methanol	NOUN
cet-15688	9	10	using	use	VERB
cet-15688	9	11	industrial	industrial	ADJ
cet-15688	9	12	catalysts	catalyst	NOUN
cet-15688	9	13	.	.	PUNCT
cet-15688	10	1	this	this	DET
cet-15688	10	2	process	process	NOUN
cet-15688	10	3	can	can	AUX
cet-15688	10	4	be	be	AUX
cet-15688	10	5	adapted	adapt	VERB
cet-15688	10	6	to	to	PART
cet-15688	10	7	utilize	utilize	VERB
cet-15688	10	8	carbon	carbon	NOUN
cet-15688	10	9	dioxide	dioxide	NOUN
cet-15688	10	10	for	for	ADP
cet-15688	10	11	the	the	DET
cet-15688	10	12	direct	direct	ADJ
cet-15688	10	13	production	production	NOUN
cet-15688	10	14	of	of	ADP
cet-15688	10	15	formaldehyde	formaldehyde	NOUN
cet-15688	10	16	.	.	PUNCT
cet-15688	11	1	however	however	ADV
cet-15688	11	2	,	,	PUNCT
cet-15688	11	3	some	some	DET
cet-15688	11	4	thermodynamic	thermodynamic	ADJ
cet-15688	11	5	and	and	CCONJ
cet-15688	11	6	technical	technical	ADJ
cet-15688	11	7	issues	issue	NOUN
cet-15688	11	8	prevent	prevent	VERB
cet-15688	11	9	the	the	DET
cet-15688	11	10	implementation	implementation	NOUN
cet-15688	11	11	of	of	ADP
cet-15688	11	12	this	this	DET
cet-15688	11	13	process	process	NOUN
cet-15688	11	14	.	.	PUNCT
cet-15688	12	1	the	the	DET
cet-15688	12	2	current	current	ADJ
cet-15688	12	3	study	study	NOUN
cet-15688	12	4	focuses	focus	VERB
cet-15688	12	5	on	on	ADP
cet-15688	12	6	the	the	DET
cet-15688	12	7	synthesis	synthesis	NOUN
cet-15688	12	8	of	of	ADP
cet-15688	12	9	bimetallic	bimetallic	ADJ
cet-15688	12	10	catalysts	catalyst	NOUN
cet-15688	12	11	based	base	VERB
cet-15688	12	12	on	on	ADP
cet-15688	12	13	cu	cu	PROPN
cet-15688	12	14	,	,	PUNCT
cet-15688	12	15	ni	ni	PROPN
cet-15688	12	16	and	and	CCONJ
cet-15688	12	17	pt	pt	NOUN
cet-15688	12	18	using	use	VERB
cet-15688	12	19	microporous	microporous	ADJ
cet-15688	12	20	silica	silica	NOUN
cet-15688	12	21	to	to	PART
cet-15688	12	22	provide	provide	VERB
cet-15688	12	23	a	a	DET
cet-15688	12	24	high	high	ADJ
cet-15688	12	25	concentration	concentration	NOUN
cet-15688	12	26	of	of	ADP
cet-15688	12	27	active	active	ADJ
cet-15688	12	28	sites	site	NOUN
cet-15688	12	29	.	.	PUNCT
cet-15688	13	1	the	the	DET
cet-15688	13	2	catalysts	catalyst	NOUN
cet-15688	13	3	were	be	AUX
cet-15688	13	4	characterized	characterize	VERB
cet-15688	13	5	using	use	VERB
cet-15688	13	6	nitrogen	nitrogen	NOUN
cet-15688	13	7	physisorption	physisorption	NOUN
cet-15688	13	8	,	,	PUNCT
cet-15688	13	9	hydrogen	hydrogen	NOUN
cet-15688	13	10	and	and	CCONJ
cet-15688	13	11	carbon	carbon	NOUN
cet-15688	13	12	dioxide	dioxide	NOUN
cet-15688	13	13	chemisorption	chemisorption	NOUN
cet-15688	13	14	,	,	PUNCT
cet-15688	13	15	as	as	ADV
cet-15688	13	16	well	well	ADV
cet-15688	13	17	as	as	ADP
cet-15688	13	18	x	x	NOUN
cet-15688	13	19	-	-	NOUN
cet-15688	13	20	ray	ray	NOUN
cet-15688	13	21	fluorescence	fluorescence	NOUN
cet-15688	13	22	analysis	analysis	NOUN
cet-15688	13	23	.	.	PUNCT
cet-15688	14	1	the	the	DET
cet-15688	14	2	synthesis	synthesis	NOUN
cet-15688	14	3	of	of	ADP
cet-15688	14	4	formaldehyde	formaldehyde	NOUN
cet-15688	14	5	was	be	AUX
cet-15688	14	6	carried	carry	VERB
cet-15688	14	7	out	out	ADP
cet-15688	14	8	in	in	ADP
cet-15688	14	9	a	a	DET
cet-15688	14	10	high	high	ADJ
cet-15688	14	11	-	-	PUNCT
cet-15688	14	12	pressure	pressure	NOUN
cet-15688	14	13	parr	parr	NOUN
cet-15688	14	14	instrument	instrument	NOUN
cet-15688	14	15	reactor	reactor	NOUN
cet-15688	14	16	.	.	PUNCT
cet-15688	15	1	providing	provide	VERB
cet-15688	15	2	catalysts	catalyst	NOUN
cet-15688	15	3	synthesis	synthesis	NOUN
cet-15688	15	4	using	use	VERB
cet-15688	15	5	micro	micro	ADJ
cet-15688	15	6	-	-	ADJ
cet-15688	15	7	mesoporous	mesoporous	ADJ
cet-15688	15	8	silica	silica	NOUN
cet-15688	15	9	results	result	NOUN
cet-15688	15	10	in	in	ADP
cet-15688	15	11	the	the	DET
cet-15688	15	12	formation	formation	NOUN
cet-15688	15	13	of	of	ADP
cet-15688	15	14	metallic	metallic	ADJ
cet-15688	15	15	species	specie	NOUN
cet-15688	15	16	within	within	ADP
cet-15688	15	17	the	the	DET
cet-15688	15	18	microand	microand	ADJ
cet-15688	15	19	mesoporous	mesoporous	ADJ
cet-15688	15	20	areas	area	NOUN
cet-15688	15	21	of	of	ADP
cet-15688	15	22	the	the	DET
cet-15688	15	23	silica	silica	NOUN
cet-15688	15	24	,	,	PUNCT
cet-15688	15	25	and	and	CCONJ
cet-15688	15	26	in	in	ADP
cet-15688	15	27	an	an	DET
cet-15688	15	28	increase	increase	NOUN
cet-15688	15	29	in	in	ADP
cet-15688	15	30	the	the	DET
cet-15688	15	31	formaldehyde	formaldehyde	NOUN
cet-15688	15	32	yield	yield	NOUN
cet-15688	15	33	by	by	ADP
cet-15688	15	34	15	15	NUM
cet-15688	15	35	-	-	SYM
cet-15688	15	36	20	20	NUM
cet-15688	15	37	%	%	NOUN
cet-15688	15	38	compared	compare	VERB
cet-15688	15	39	to	to	ADP
cet-15688	15	40	the	the	DET
cet-15688	15	41	catalysts	catalyst	NOUN
cet-15688	15	42	described	describe	VERB
cet-15688	15	43	in	in	ADP
cet-15688	15	44	literature	literature	NOUN
cet-15688	15	45	.	.	PUNCT
cet-15688	16	1	1	1	X
cet-15688	16	2	.	.	X
cet-15688	16	3	introduction	introduction	NOUN
cet-15688	16	4	an	an	DET
cet-15688	16	5	increase	increase	NOUN
cet-15688	16	6	in	in	ADP
cet-15688	16	7	carbon	carbon	NOUN
cet-15688	16	8	dioxide	dioxide	NOUN
cet-15688	16	9	concentrations	concentration	NOUN
cet-15688	16	10	in	in	ADP
cet-15688	16	11	the	the	DET
cet-15688	16	12	atmosphere	atmosphere	NOUN
cet-15688	16	13	(	(	PUNCT
cet-15688	16	14	hepburn	hepburn	NOUN
cet-15688	16	15	et	et	PROPN
cet-15688	16	16	al	al	PROPN
cet-15688	16	17	.	.	PROPN
cet-15688	16	18	,	,	PUNCT
cet-15688	16	19	2019	2019	NUM
cet-15688	16	20	)	)	PUNCT
cet-15688	16	21	declares	declare	VERB
cet-15688	16	22	the	the	DET
cet-15688	16	23	need	need	NOUN
cet-15688	16	24	for	for	ADP
cet-15688	16	25	new	new	ADJ
cet-15688	16	26	technologies	technology	NOUN
cet-15688	16	27	to	to	PART
cet-15688	16	28	be	be	AUX
cet-15688	16	29	developed	develop	VERB
cet-15688	16	30	for	for	ADP
cet-15688	16	31	its	its	PRON
cet-15688	16	32	use	use	NOUN
cet-15688	16	33	in	in	ADP
cet-15688	16	34	sustainable	sustainable	ADJ
cet-15688	16	35	development	development	NOUN
cet-15688	16	36	of	of	ADP
cet-15688	16	37	modern	modern	ADJ
cet-15688	16	38	industry	industry	NOUN
cet-15688	16	39	and	and	CCONJ
cet-15688	16	40	society	society	NOUN
cet-15688	16	41	(	(	PUNCT
cet-15688	16	42	rauch	rauch	VERB
cet-15688	16	43	et	et	PROPN
cet-15688	16	44	al	al	PROPN
cet-15688	16	45	.	.	PROPN
cet-15688	16	46	,	,	PUNCT
cet-15688	16	47	2019	2019	NUM
cet-15688	16	48	)	)	PUNCT
cet-15688	16	49	.	.	PUNCT
cet-15688	17	1	possible	possible	ADJ
cet-15688	17	2	methods	method	NOUN
cet-15688	17	3	for	for	ADP
cet-15688	17	4	utilizing	utilize	VERB
cet-15688	17	5	carbon	carbon	NOUN
cet-15688	17	6	dioxide	dioxide	NOUN
cet-15688	17	7	include	include	VERB
cet-15688	17	8	the	the	DET
cet-15688	17	9	production	production	NOUN
cet-15688	17	10	of	of	ADP
cet-15688	17	11	fuels	fuel	NOUN
cet-15688	17	12	(	(	PUNCT
cet-15688	17	13	leclerc	leclerc	PROPN
cet-15688	17	14	et	et	PROPN
cet-15688	17	15	al	al	PROPN
cet-15688	17	16	.	.	PROPN
cet-15688	17	17	,	,	PUNCT
cet-15688	17	18	2024	2024	NUM
cet-15688	17	19	)	)	PUNCT
cet-15688	17	20	and	and	CCONJ
cet-15688	17	21	valuable	valuable	ADJ
cet-15688	17	22	chemicals	chemical	NOUN
cet-15688	17	23	(	(	PUNCT
cet-15688	17	24	banerjee	banerjee	PROPN
cet-15688	17	25	et	et	PROPN
cet-15688	17	26	al	al	PROPN
cet-15688	17	27	.	.	PROPN
cet-15688	17	28	,	,	PUNCT
cet-15688	17	29	2016	2016	NUM
cet-15688	17	30	)	)	PUNCT
cet-15688	17	31	.	.	PUNCT
cet-15688	18	1	the	the	DET
cet-15688	18	2	highest	high	ADJ
cet-15688	18	3	impact	impact	NOUN
cet-15688	18	4	of	of	ADP
cet-15688	18	5	carbon	carbon	NOUN
cet-15688	18	6	dioxide	dioxide	NOUN
cet-15688	18	7	incorporation	incorporation	NOUN
cet-15688	18	8	in	in	ADP
cet-15688	18	9	industrial	industrial	ADJ
cet-15688	18	10	processes	process	NOUN
cet-15688	18	11	can	can	AUX
cet-15688	18	12	be	be	AUX
cet-15688	18	13	achieved	achieve	VERB
cet-15688	18	14	through	through	ADP
cet-15688	18	15	a	a	DET
cet-15688	18	16	partial	partial	ADJ
cet-15688	18	17	or	or	CCONJ
cet-15688	18	18	full	full	ADJ
cet-15688	18	19	substitution	substitution	NOUN
cet-15688	18	20	of	of	ADP
cet-15688	18	21	typical	typical	ADJ
cet-15688	18	22	petrochemical	petrochemical	NOUN
cet-15688	18	23	processes	process	NOUN
cet-15688	18	24	such	such	ADJ
cet-15688	18	25	as	as	ADP
cet-15688	18	26	the	the	DET
cet-15688	18	27	production	production	NOUN
cet-15688	18	28	of	of	ADP
cet-15688	18	29	hydrocarbons	hydrocarbon	NOUN
cet-15688	18	30	,	,	PUNCT
cet-15688	18	31	methanol	methanol	NOUN
cet-15688	18	32	,	,	PUNCT
cet-15688	18	33	and	and	CCONJ
cet-15688	18	34	formaldehyde	formaldehyde	NOUN
cet-15688	18	35	(	(	PUNCT
cet-15688	18	36	leclerc	leclerc	PROPN
cet-15688	18	37	et	et	PROPN
cet-15688	18	38	al	al	PROPN
cet-15688	18	39	.	.	PROPN
cet-15688	18	40	,	,	PUNCT
cet-15688	18	41	2024	2024	NUM
cet-15688	18	42	)	)	PUNCT
cet-15688	18	43	.	.	PUNCT
cet-15688	19	1	formaldehyde	formaldehyde	NOUN
cet-15688	19	2	is	be	AUX
cet-15688	19	3	one	one	NUM
cet-15688	19	4	of	of	ADP
cet-15688	19	5	the	the	DET
cet-15688	19	6	most	most	ADV
cet-15688	19	7	widely	widely	ADV
cet-15688	19	8	used	use	VERB
cet-15688	19	9	feedstocks	feedstock	NOUN
cet-15688	19	10	for	for	ADP
cet-15688	19	11	industrial	industrial	ADJ
cet-15688	19	12	chemicals	chemical	NOUN
cet-15688	19	13	and	and	CCONJ
cet-15688	19	14	polymers	polymer	NOUN
cet-15688	19	15	production	production	NOUN
cet-15688	19	16	.	.	PUNCT
cet-15688	20	1	it	it	PRON
cet-15688	20	2	is	be	AUX
cet-15688	20	3	typically	typically	ADV
cet-15688	20	4	produced	produce	VERB
cet-15688	20	5	by	by	ADP
cet-15688	20	6	the	the	DET
cet-15688	20	7	consecutive	consecutive	ADJ
cet-15688	20	8	methane	methane	NOUN
cet-15688	20	9	oxidation	oxidation	NOUN
cet-15688	20	10	to	to	ADP
cet-15688	20	11	syngas	syngas	NOUN
cet-15688	20	12	,	,	PUNCT
cet-15688	20	13	syngas	syngas	NOUN
cet-15688	20	14	transformation	transformation	NOUN
cet-15688	20	15	to	to	PART
cet-15688	20	16	methanol	methanol	VERB
cet-15688	20	17	and	and	CCONJ
cet-15688	20	18	methanol	methanol	NOUN
cet-15688	20	19	catalytical	catalytical	ADJ
cet-15688	20	20	oxidation	oxidation	NOUN
cet-15688	20	21	over	over	ADP
cet-15688	20	22	a	a	DET
cet-15688	20	23	silver	silver	NOUN
cet-15688	20	24	or	or	CCONJ
cet-15688	20	25	mixed	mixed	ADJ
cet-15688	20	26	catalyst	catalyst	NOUN
cet-15688	20	27	(	(	PUNCT
cet-15688	20	28	chan	chan	PROPN
cet-15688	20	29	et	et	PROPN
cet-15688	20	30	al	al	PROPN
cet-15688	20	31	.	.	PROPN
cet-15688	20	32	,	,	PUNCT
cet-15688	20	33	2018	2018	NUM
cet-15688	20	34	)	)	PUNCT
cet-15688	20	35	.	.	PUNCT
cet-15688	21	1	the	the	DET
cet-15688	21	2	direct	direct	ADJ
cet-15688	21	3	formation	formation	NOUN
cet-15688	21	4	of	of	ADP
cet-15688	21	5	formaldehyde	formaldehyde	NOUN
cet-15688	21	6	from	from	ADP
cet-15688	21	7	carbon	carbon	NOUN
cet-15688	21	8	dioxide	dioxide	NOUN
cet-15688	21	9	can	can	AUX
cet-15688	21	10	possibly	possibly	ADV
cet-15688	21	11	exclude	exclude	VERB
cet-15688	21	12	methane	methane	NOUN
cet-15688	21	13	application	application	NOUN
cet-15688	21	14	for	for	ADP
cet-15688	21	15	formaldehyde	formaldehyde	NOUN
cet-15688	21	16	synthesis	synthesis	NOUN
cet-15688	21	17	,	,	PUNCT
cet-15688	21	18	that	that	PRON
cet-15688	21	19	can	can	AUX
cet-15688	21	20	play	play	VERB
cet-15688	21	21	a	a	DET
cet-15688	21	22	positive	positive	ADJ
cet-15688	21	23	role	role	NOUN
cet-15688	21	24	for	for	ADP
cet-15688	21	25	carbon	carbon	NOUN
cet-15688	21	26	dioxide	dioxide	NOUN
cet-15688	21	27	concentration	concentration	NOUN
cet-15688	21	28	decrease	decrease	NOUN
cet-15688	21	29	in	in	ADP
cet-15688	21	30	the	the	DET
cet-15688	21	31	atmosphere	atmosphere	NOUN
cet-15688	21	32	(	(	PUNCT
cet-15688	21	33	siebert	siebert	PROPN
cet-15688	21	34	et	et	PROPN
cet-15688	21	35	al	al	PROPN
cet-15688	21	36	.	.	PROPN
cet-15688	21	37	,	,	PUNCT
cet-15688	21	38	2019	2019	NUM
cet-15688	21	39	)	)	PUNCT
cet-15688	21	40	.	.	PUNCT
cet-15688	22	1	the	the	DET
cet-15688	22	2	other	other	ADJ
cet-15688	22	3	possible	possible	ADJ
cet-15688	22	4	way	way	NOUN
cet-15688	22	5	for	for	ADP
cet-15688	22	6	formaldehyde	formaldehyde	NOUN
cet-15688	22	7	synthesis	synthesis	NOUN
cet-15688	22	8	is	be	AUX
cet-15688	22	9	hydrogenation	hydrogenation	NOUN
cet-15688	22	10	of	of	ADP
cet-15688	22	11	formic	formic	ADJ
cet-15688	22	12	acid	acid	NOUN
cet-15688	22	13	produced	produce	VERB
cet-15688	22	14	by	by	ADP
cet-15688	22	15	carbon	carbon	NOUN
cet-15688	22	16	dioxide	dioxide	NOUN
cet-15688	22	17	hydrogenation	hydrogenation	NOUN
cet-15688	22	18	.	.	PUNCT
cet-15688	23	1	however	however	ADV
cet-15688	23	2	,	,	PUNCT
cet-15688	23	3	an	an	DET
cet-15688	23	4	addition	addition	NOUN
cet-15688	23	5	of	of	ADP
cet-15688	23	6	a	a	DET
cet-15688	23	7	second	second	ADJ
cet-15688	23	8	step	step	NOUN
cet-15688	23	9	in	in	ADP
cet-15688	23	10	carbon	carbon	NOUN
cet-15688	23	11	dioxide	dioxide	NOUN
cet-15688	23	12	transformation	transformation	NOUN
cet-15688	23	13	is	be	AUX
cet-15688	23	14	not	not	PART
cet-15688	23	15	technologically	technologically	ADV
cet-15688	23	16	and	and	CCONJ
cet-15688	23	17	economically	economically	ADV
cet-15688	23	18	favourable	favourable	ADJ
cet-15688	23	19	(	(	PUNCT
cet-15688	23	20	singh	singh	PROPN
cet-15688	23	21	et	et	PROPN
cet-15688	23	22	al	al	PROPN
cet-15688	23	23	.	.	PROPN
cet-15688	23	24	,	,	PUNCT
cet-15688	23	25	2021	2021	NUM
cet-15688	23	26	)	)	PUNCT
cet-15688	23	27	.	.	PUNCT
cet-15688	24	1	therefore	therefore	ADV
cet-15688	24	2	,	,	PUNCT
cet-15688	24	3	the	the	DET
cet-15688	24	4	study	study	NOUN
cet-15688	24	5	of	of	ADP
cet-15688	24	6	direct	direct	ADJ
cet-15688	24	7	carbon	carbon	NOUN
cet-15688	24	8	dioxide	dioxide	NOUN
cet-15688	24	9	transformation	transformation	NOUN
cet-15688	24	10	into	into	ADP
cet-15688	24	11	formaldehyde	formaldehyde	NOUN
cet-15688	24	12	is	be	AUX
cet-15688	24	13	of	of	ADP
cet-15688	24	14	special	special	ADJ
cet-15688	24	15	interest	interest	NOUN
cet-15688	24	16	for	for	ADP
cet-15688	24	17	the	the	DET
cet-15688	24	18	sustainable	sustainable	ADJ
cet-15688	24	19	development	development	NOUN
cet-15688	24	20	of	of	ADP
cet-15688	24	21	modern	modern	ADJ
cet-15688	24	22	society	society	NOUN
cet-15688	24	23	toward	toward	ADP
cet-15688	24	24	carbon	carbon	NOUN
cet-15688	24	25	dioxide	dioxide	NOUN
cet-15688	24	26	zero	zero	NUM
cet-15688	24	27	emission	emission	NOUN
cet-15688	24	28	.	.	PUNCT
cet-15688	25	1	formaldehyde	formaldehyde	NOUN
cet-15688	25	2	direct	direct	ADJ
cet-15688	25	3	synthesis	synthesis	NOUN
cet-15688	25	4	from	from	ADP
cet-15688	25	5	carbon	carbon	NOUN
cet-15688	25	6	dioxide	dioxide	NOUN
cet-15688	25	7	has	have	VERB
cet-15688	25	8	several	several	ADJ
cet-15688	25	9	reactions	reaction	NOUN
cet-15688	25	10	that	that	PRON
cet-15688	25	11	can	can	AUX
cet-15688	25	12	take	take	VERB
cet-15688	25	13	place	place	NOUN
cet-15688	25	14	in	in	ADP
cet-15688	25	15	the	the	DET
cet-15688	25	16	reaction	reaction	NOUN
cet-15688	25	17	medium	medium	NOUN
cet-15688	25	18	,	,	PUNCT
cet-15688	25	19	and	and	CCONJ
cet-15688	25	20	the	the	DET
cet-15688	25	21	possible	possible	ADJ
cet-15688	25	22	reaction	reaction	NOUN
cet-15688	25	23	pathway	pathway	NOUN
cet-15688	25	24	is	be	AUX
cet-15688	25	25	shown	show	VERB
cet-15688	25	26	in	in	ADP
cet-15688	25	27	figure	figure	NOUN
cet-15688	25	28	1	1	NUM
cet-15688	25	29	(	(	PUNCT
cet-15688	25	30	lee	lee	PROPN
cet-15688	25	31	et	et	PROPN
cet-15688	25	32	al	al	PROPN
cet-15688	25	33	.	.	PROPN
cet-15688	25	34	,	,	PUNCT
cet-15688	25	35	2001	2001	NUM
cet-15688	25	36	)	)	PUNCT
cet-15688	25	37	.	.	PUNCT
cet-15688	26	1	373	373	NUM
cet-15688	26	2	co2	co2	NOUN
cet-15688	26	3	+	+	X
cet-15688	26	4	h2	h2	NOUN
cet-15688	26	5	co	co	NOUN
cet-15688	26	6	+	+	PROPN
cet-15688	26	7	h2o	h2o	PROPN
cet-15688	26	8	co	co	PROPN
cet-15688	26	9	+	+	ADJ
cet-15688	26	10	h2	h2	NOUN
cet-15688	26	11	hcoh	hcoh	NOUN
cet-15688	26	12	ch3oh+	ch3oh+	NOUN
cet-15688	26	13	h2hcoh	h2hcoh	ADJ
cet-15688	26	14	carbon	carbon	NOUN
cet-15688	26	15	dioxide	dioxide	NOUN
cet-15688	26	16	carbone	carbone	NOUN
cet-15688	26	17	monoxide	monoxide	NOUN
cet-15688	26	18	hydrogen	hydrogen	PROPN
cet-15688	26	19	water	water	NOUN
cet-15688	26	20	methanol	methanol	NOUN
cet-15688	26	21	carbone	carbone	NOUN
cet-15688	26	22	monoxide	monoxide	NOUN
cet-15688	26	23	hydrogen	hydrogen	PROPN
cet-15688	26	24	formaldehyde	formaldehyde	NOUN
cet-15688	26	25	formaldehyde	formaldehyde	NOUN
cet-15688	26	26	hydrogen	hydrogen	NOUN
cet-15688	26	27	figure	figure	NOUN
cet-15688	26	28	1	1	NUM
cet-15688	26	29	:	:	PUNCT
cet-15688	26	30	scheme	scheme	NOUN
cet-15688	26	31	of	of	ADP
cet-15688	26	32	the	the	DET
cet-15688	26	33	reaction	reaction	NOUN
cet-15688	26	34	pathway	pathway	NOUN
cet-15688	26	35	of	of	ADP
cet-15688	26	36	formaldehyde	formaldehyde	NOUN
cet-15688	26	37	synthesis	synthesis	NOUN
cet-15688	26	38	from	from	ADP
cet-15688	26	39	carbon	carbon	NOUN
cet-15688	26	40	dioxide	dioxide	NOUN
cet-15688	26	41	the	the	DET
cet-15688	26	42	first	first	ADJ
cet-15688	26	43	step	step	NOUN
cet-15688	26	44	in	in	ADP
cet-15688	26	45	the	the	DET
cet-15688	26	46	consecutive	consecutive	ADJ
cet-15688	26	47	reactions	reaction	NOUN
cet-15688	26	48	can	can	AUX
cet-15688	26	49	be	be	AUX
cet-15688	26	50	the	the	DET
cet-15688	26	51	conversion	conversion	NOUN
cet-15688	26	52	of	of	ADP
cet-15688	26	53	carbon	carbon	NOUN
cet-15688	26	54	dioxide	dioxide	NOUN
cet-15688	26	55	into	into	ADP
cet-15688	26	56	carbon	carbon	NOUN
cet-15688	26	57	monoxide	monoxide	NOUN
cet-15688	26	58	and	and	CCONJ
cet-15688	26	59	water	water	NOUN
cet-15688	26	60	.	.	PUNCT
cet-15688	27	1	therefore	therefore	ADV
cet-15688	27	2	,	,	PUNCT
cet-15688	27	3	a	a	DET
cet-15688	27	4	decrease	decrease	NOUN
cet-15688	27	5	in	in	ADP
cet-15688	27	6	the	the	DET
cet-15688	27	7	water	water	NOUN
cet-15688	27	8	content	content	NOUN
cet-15688	27	9	of	of	ADP
cet-15688	27	10	the	the	DET
cet-15688	27	11	reaction	reaction	NOUN
cet-15688	27	12	medium	medium	NOUN
cet-15688	27	13	can	can	AUX
cet-15688	27	14	play	play	VERB
cet-15688	27	15	positive	positive	ADJ
cet-15688	27	16	role	role	NOUN
cet-15688	27	17	in	in	ADP
cet-15688	27	18	the	the	DET
cet-15688	27	19	rate	rate	NOUN
cet-15688	27	20	of	of	ADP
cet-15688	27	21	carbon	carbon	NOUN
cet-15688	27	22	monoxide	monoxide	NOUN
cet-15688	27	23	production	production	NOUN
cet-15688	27	24	.	.	PUNCT
cet-15688	28	1	the	the	DET
cet-15688	28	2	second	second	ADJ
cet-15688	28	3	stage	stage	NOUN
cet-15688	28	4	of	of	ADP
cet-15688	28	5	this	this	DET
cet-15688	28	6	process	process	NOUN
cet-15688	28	7	is	be	AUX
cet-15688	28	8	the	the	DET
cet-15688	28	9	formation	formation	NOUN
cet-15688	28	10	of	of	ADP
cet-15688	28	11	formaldehyde	formaldehyde	NOUN
cet-15688	28	12	by	by	ADP
cet-15688	28	13	hydrogenation	hydrogenation	NOUN
cet-15688	28	14	of	of	ADP
cet-15688	28	15	carbon	carbon	NOUN
cet-15688	28	16	monoxide	monoxide	NOUN
cet-15688	28	17	.	.	PUNCT
cet-15688	29	1	however	however	ADV
cet-15688	29	2	,	,	PUNCT
cet-15688	29	3	formaldehyde	formaldehyde	NOUN
cet-15688	29	4	is	be	AUX
cet-15688	29	5	immediately	immediately	ADV
cet-15688	29	6	converted	convert	VERB
cet-15688	29	7	into	into	ADP
cet-15688	29	8	methanol	methanol	NOUN
cet-15688	29	9	,	,	PUNCT
cet-15688	29	10	so	so	ADV
cet-15688	29	11	methanol	methanol	NOUN
cet-15688	29	12	formation	formation	NOUN
cet-15688	29	13	must	must	AUX
cet-15688	29	14	be	be	AUX
cet-15688	29	15	suppressed	suppress	VERB
cet-15688	29	16	in	in	ADP
cet-15688	29	17	the	the	DET
cet-15688	29	18	reaction	reaction	NOUN
cet-15688	29	19	medium	medium	NOUN
cet-15688	29	20	to	to	PART
cet-15688	29	21	obtain	obtain	VERB
cet-15688	29	22	a	a	DET
cet-15688	29	23	high	high	ADJ
cet-15688	29	24	yield	yield	NOUN
cet-15688	29	25	of	of	ADP
cet-15688	29	26	formaldehyde	formaldehyde	NOUN
cet-15688	29	27	.	.	PUNCT
cet-15688	30	1	here	here	ADV
cet-15688	30	2	,	,	PUNCT
cet-15688	30	3	the	the	DET
cet-15688	30	4	catalytic	catalytic	ADJ
cet-15688	30	5	route	route	NOUN
cet-15688	30	6	of	of	ADP
cet-15688	30	7	formaldehyde	formaldehyde	NOUN
cet-15688	30	8	formation	formation	NOUN
cet-15688	30	9	on	on	ADP
cet-15688	30	10	bimetallic	bimetallic	PROPN
cet-15688	30	11	cu	cu	PROPN
cet-15688	30	12	,	,	PUNCT
cet-15688	30	13	ni	ni	PROPN
cet-15688	30	14	,	,	PUNCT
cet-15688	30	15	and	and	CCONJ
cet-15688	30	16	pt	pt	NOUN
cet-15688	30	17	catalysts	catalyst	NOUN
cet-15688	30	18	is	be	AUX
cet-15688	30	19	studied	study	VERB
cet-15688	30	20	and	and	CCONJ
cet-15688	30	21	discussed	discuss	VERB
cet-15688	30	22	.	.	PUNCT
cet-15688	31	1	2	2	X
cet-15688	31	2	.	.	X
cet-15688	31	3	materials	material	NOUN
cet-15688	31	4	and	and	CCONJ
cet-15688	31	5	methods	method	NOUN
cet-15688	31	6	2.1	2.1	NUM
cet-15688	31	7	materials	material	NOUN
cet-15688	31	8	for	for	ADP
cet-15688	31	9	catalyst	catalyst	NOUN
cet-15688	31	10	synthesis	synthesis	NOUN
cet-15688	31	11	,	,	PUNCT
cet-15688	31	12	reagent	reagent	ADJ
cet-15688	31	13	-	-	PUNCT
cet-15688	31	14	grade	grade	NOUN
cet-15688	31	15	platinic	platinic	ADJ
cet-15688	31	16	acid	acid	NOUN
cet-15688	31	17	,	,	PUNCT
cet-15688	31	18	copper	copper	NOUN
cet-15688	31	19	nitrate	nitrate	NOUN
cet-15688	31	20	,	,	PUNCT
cet-15688	31	21	nickel	nickel	NOUN
cet-15688	31	22	nitrate	nitrate	NOUN
cet-15688	31	23	,	,	PUNCT
cet-15688	31	24	ultra	ultra	ADJ
cet-15688	31	25	-	-	ADJ
cet-15688	31	26	fine	fine	ADJ
cet-15688	31	27	silica	silica	NOUN
cet-15688	31	28	,	,	PUNCT
cet-15688	31	29	hydrogen	hydrogen	NOUN
cet-15688	31	30	,	,	PUNCT
cet-15688	31	31	and	and	CCONJ
cet-15688	31	32	carbon	carbon	NOUN
cet-15688	31	33	dioxide	dioxide	NOUN
cet-15688	31	34	(	(	PUNCT
cet-15688	31	35	grade	grade	NOUN
cet-15688	31	36	a	a	NOUN
cet-15688	31	37	,	,	PUNCT
cet-15688	31	38	99.99	99.99	NUM
cet-15688	31	39	%	%	NOUN
cet-15688	31	40	vol	vol	NOUN
cet-15688	31	41	.	.	PUNCT
cet-15688	31	42	)	)	PUNCT
cet-15688	31	43	were	be	AUX
cet-15688	31	44	purchased	purchase	VERB
cet-15688	31	45	from	from	ADP
cet-15688	31	46	a	a	DET
cet-15688	31	47	local	local	ADJ
cet-15688	31	48	supplier	supplier	NOUN
cet-15688	31	49	and	and	CCONJ
cet-15688	31	50	used	use	VERB
cet-15688	31	51	as	as	SCONJ
cet-15688	31	52	received	receive	VERB
cet-15688	31	53	.	.	PUNCT
cet-15688	32	1	distilled	distil	VERB
cet-15688	32	2	water	water	NOUN
cet-15688	32	3	was	be	AUX
cet-15688	32	4	purified	purify	VERB
cet-15688	32	5	using	use	VERB
cet-15688	32	6	an	an	DET
cet-15688	32	7	aqua	aqua	NOUN
cet-15688	32	8	post	post	NOUN
cet-15688	32	9	water	water	NOUN
cet-15688	32	10	purifier	purifier	NOUN
cet-15688	32	11	.	.	PUNCT
cet-15688	33	1	2.2	2.2	NUM
cet-15688	33	2	catalyst	catalyst	NOUN
cet-15688	33	3	synthesis	synthesis	NOUN
cet-15688	33	4	for	for	ADP
cet-15688	33	5	catalyst	catalyst	NOUN
cet-15688	33	6	synthesis	synthesis	NOUN
cet-15688	33	7	,	,	PUNCT
cet-15688	33	8	a	a	DET
cet-15688	33	9	sample	sample	NOUN
cet-15688	33	10	of	of	ADP
cet-15688	33	11	silica	silica	NOUN
cet-15688	33	12	was	be	AUX
cet-15688	33	13	suspended	suspend	VERB
cet-15688	33	14	in	in	ADP
cet-15688	33	15	water	water	NOUN
cet-15688	33	16	.	.	PUNCT
cet-15688	34	1	a	a	DET
cet-15688	34	2	solution	solution	NOUN
cet-15688	34	3	of	of	ADP
cet-15688	34	4	precursor	precursor	NOUN
cet-15688	34	5	was	be	AUX
cet-15688	34	6	then	then	ADV
cet-15688	34	7	added	add	VERB
cet-15688	34	8	to	to	ADP
cet-15688	34	9	the	the	DET
cet-15688	34	10	suspension	suspension	NOUN
cet-15688	34	11	,	,	PUNCT
cet-15688	34	12	and	and	CCONJ
cet-15688	34	13	the	the	DET
cet-15688	34	14	suspension	suspension	NOUN
cet-15688	34	15	was	be	AUX
cet-15688	34	16	transferred	transfer	VERB
cet-15688	34	17	into	into	ADP
cet-15688	34	18	an	an	DET
cet-15688	34	19	evaporation	evaporation	NOUN
cet-15688	34	20	cup	cup	NOUN
cet-15688	34	21	,	,	PUNCT
cet-15688	34	22	where	where	SCONJ
cet-15688	34	23	the	the	DET
cet-15688	34	24	water	water	NOUN
cet-15688	34	25	was	be	AUX
cet-15688	34	26	evaporated	evaporate	VERB
cet-15688	34	27	.	.	PUNCT
cet-15688	35	1	the	the	DET
cet-15688	35	2	sample	sample	NOUN
cet-15688	35	3	was	be	AUX
cet-15688	35	4	then	then	ADV
cet-15688	35	5	reduced	reduce	VERB
cet-15688	35	6	in	in	ADP
cet-15688	35	7	a	a	DET
cet-15688	35	8	tube	tube	NOUN
cet-15688	35	9	furnace	furnace	NOUN
cet-15688	35	10	at	at	ADP
cet-15688	35	11	500	500	NUM
cet-15688	35	12	°	°	NOUN
cet-15688	35	13	c	c	NOUN
cet-15688	35	14	for	for	ADP
cet-15688	35	15	3	3	NUM
cet-15688	35	16	h	h	NOUN
cet-15688	35	17	in	in	ADP
cet-15688	35	18	a	a	DET
cet-15688	35	19	hydrogen	hydrogen	NOUN
cet-15688	35	20	atmosphere	atmosphere	NOUN
cet-15688	35	21	.	.	PUNCT
cet-15688	36	1	if	if	SCONJ
cet-15688	36	2	a	a	DET
cet-15688	36	3	second	second	ADJ
cet-15688	36	4	metal	metal	NOUN
cet-15688	36	5	was	be	AUX
cet-15688	36	6	introduced	introduce	VERB
cet-15688	36	7	into	into	ADP
cet-15688	36	8	the	the	DET
cet-15688	36	9	sample	sample	NOUN
cet-15688	36	10	,	,	PUNCT
cet-15688	36	11	the	the	DET
cet-15688	36	12	procedure	procedure	NOUN
cet-15688	36	13	was	be	AUX
cet-15688	36	14	then	then	ADV
cet-15688	36	15	repeated	repeat	VERB
cet-15688	36	16	twice	twice	ADV
cet-15688	36	17	,	,	PUNCT
cet-15688	36	18	with	with	ADP
cet-15688	36	19	different	different	ADJ
cet-15688	36	20	metals	metal	NOUN
cet-15688	36	21	each	each	DET
cet-15688	36	22	time	time	NOUN
cet-15688	36	23	.	.	PUNCT
cet-15688	37	1	2.3	2.3	NUM
cet-15688	37	2	formaldehyde	formaldehyde	NOUN
cet-15688	37	3	synthesis	synthesis	NOUN
cet-15688	37	4	procedure	procedure	NOUN
cet-15688	37	5	for	for	ADP
cet-15688	37	6	formaldehyde	formaldehyde	NOUN
cet-15688	37	7	synthesis	synthesis	NOUN
cet-15688	37	8	,	,	PUNCT
cet-15688	37	9	100	100	NUM
cet-15688	37	10	mg	mg	NOUN
cet-15688	37	11	of	of	ADP
cet-15688	37	12	a	a	DET
cet-15688	37	13	catalyst	catalyst	NOUN
cet-15688	37	14	was	be	AUX
cet-15688	37	15	placed	place	VERB
cet-15688	37	16	into	into	ADP
cet-15688	37	17	a	a	DET
cet-15688	37	18	reactor	reactor	NOUN
cet-15688	37	19	vessel	vessel	NOUN
cet-15688	37	20	(	(	PUNCT
cet-15688	37	21	a	a	DET
cet-15688	37	22	parr	parr	NOUN
cet-15688	37	23	instruments	instrument	NOUN
cet-15688	37	24	4820	4820	NUM
cet-15688	37	25	high	high	ADJ
cet-15688	37	26	-	-	PUNCT
cet-15688	37	27	pressure	pressure	NOUN
cet-15688	37	28	reactor	reactor	NOUN
cet-15688	37	29	apparatus	apparatus	NOUN
cet-15688	37	30	)	)	PUNCT
cet-15688	37	31	filled	fill	VERB
cet-15688	37	32	with	with	ADP
cet-15688	37	33	30	30	NUM
cet-15688	37	34	ml	ml	NOUN
cet-15688	37	35	of	of	ADP
cet-15688	37	36	methanol	methanol	NOUN
cet-15688	37	37	.	.	PUNCT
cet-15688	38	1	the	the	DET
cet-15688	38	2	reactor	reactor	NOUN
cet-15688	38	3	was	be	AUX
cet-15688	38	4	purged	purge	VERB
cet-15688	38	5	three	three	NUM
cet-15688	38	6	times	time	NOUN
cet-15688	38	7	with	with	ADP
cet-15688	38	8	hydrogen	hydrogen	NOUN
cet-15688	38	9	,	,	PUNCT
cet-15688	38	10	the	the	DET
cet-15688	38	11	hydrogen	hydrogen	NOUN
cet-15688	38	12	pressure	pressure	NOUN
cet-15688	38	13	was	be	AUX
cet-15688	38	14	set	set	VERB
cet-15688	38	15	to	to	ADP
cet-15688	38	16	10	10	NUM
cet-15688	38	17	bars	bar	NOUN
cet-15688	38	18	,	,	PUNCT
cet-15688	38	19	and	and	CCONJ
cet-15688	38	20	the	the	DET
cet-15688	38	21	reactor	reactor	NOUN
cet-15688	38	22	vessel	vessel	NOUN
cet-15688	38	23	was	be	AUX
cet-15688	38	24	then	then	ADV
cet-15688	38	25	heated	heated	ADJ
cet-15688	38	26	to	to	ADP
cet-15688	38	27	250	250	NUM
cet-15688	38	28	°	°	NOUN
cet-15688	38	29	c	c	NOUN
cet-15688	38	30	and	and	CCONJ
cet-15688	38	31	maintained	maintain	VERB
cet-15688	38	32	at	at	ADP
cet-15688	38	33	that	that	DET
cet-15688	38	34	pressure	pressure	NOUN
cet-15688	38	35	for	for	ADP
cet-15688	38	36	two	two	NUM
cet-15688	38	37	hours	hour	NOUN
cet-15688	38	38	.	.	PUNCT
cet-15688	39	1	after	after	SCONJ
cet-15688	39	2	the	the	DET
cet-15688	39	3	reactor	reactor	NOUN
cet-15688	39	4	had	have	AUX
cet-15688	39	5	cooled	cool	VERB
cet-15688	39	6	to	to	ADP
cet-15688	39	7	room	room	NOUN
cet-15688	39	8	temperature	temperature	NOUN
cet-15688	39	9	,	,	PUNCT
cet-15688	39	10	it	it	PRON
cet-15688	39	11	was	be	AUX
cet-15688	39	12	flushed	flush	VERB
cet-15688	39	13	with	with	ADP
cet-15688	39	14	a	a	DET
cet-15688	39	15	mixture	mixture	NOUN
cet-15688	39	16	of	of	ADP
cet-15688	39	17	carbon	carbon	NOUN
cet-15688	39	18	dioxide	dioxide	NOUN
cet-15688	39	19	and	and	CCONJ
cet-15688	39	20	hydrogen	hydrogen	NOUN
cet-15688	39	21	with	with	ADP
cet-15688	39	22	a	a	DET
cet-15688	39	23	carbon	carbon	NOUN
cet-15688	39	24	dioxide	dioxide	NOUN
cet-15688	39	25	-	-	PUNCT
cet-15688	39	26	to	to	ADP
cet-15688	39	27	-	-	PUNCT
cet-15688	39	28	hydrogen	hydrogen	NOUN
cet-15688	39	29	ratio	ratio	NOUN
cet-15688	39	30	of	of	ADP
cet-15688	39	31	1:10	1:10	NUM
cet-15688	39	32	three	three	NUM
cet-15688	39	33	times	time	NOUN
cet-15688	39	34	.	.	PUNCT
cet-15688	40	1	the	the	DET
cet-15688	40	2	gas	gas	NOUN
cet-15688	40	3	mixture	mixture	NOUN
cet-15688	40	4	pressure	pressure	NOUN
cet-15688	40	5	was	be	AUX
cet-15688	40	6	set	set	VERB
cet-15688	40	7	at	at	ADP
cet-15688	40	8	70	70	NUM
cet-15688	40	9	bars	bar	NOUN
cet-15688	40	10	and	and	CCONJ
cet-15688	40	11	the	the	DET
cet-15688	40	12	reactor	reactor	NOUN
cet-15688	40	13	was	be	AUX
cet-15688	40	14	heated	heat	VERB
cet-15688	40	15	up	up	ADP
cet-15688	40	16	to	to	ADP
cet-15688	40	17	a	a	DET
cet-15688	40	18	temperature	temperature	NOUN
cet-15688	40	19	of	of	ADP
cet-15688	40	20	180	180	NUM
cet-15688	40	21	°	°	NOUN
cet-15688	40	22	c	c	NOUN
cet-15688	40	23	.	.	PUNCT
cet-15688	41	1	samples	sample	NOUN
cet-15688	41	2	from	from	ADP
cet-15688	41	3	the	the	DET
cet-15688	41	4	reaction	reaction	NOUN
cet-15688	41	5	medium	medium	NOUN
cet-15688	41	6	were	be	AUX
cet-15688	41	7	collected	collect	VERB
cet-15688	41	8	hourly	hourly	ADV
cet-15688	41	9	and	and	CCONJ
cet-15688	41	10	analyzed	analyze	VERB
cet-15688	41	11	using	use	VERB
cet-15688	41	12	gas	gas	NOUN
cet-15688	41	13	chromatography	chromatography	NOUN
cet-15688	41	14	and	and	CCONJ
cet-15688	41	15	mass	mass	ADJ
cet-15688	41	16	spectrometry	spectrometry	NOUN
cet-15688	41	17	.	.	PUNCT
cet-15688	42	1	figure	figure	NOUN
cet-15688	42	2	2	2	NUM
cet-15688	42	3	:	:	PUNCT
cet-15688	42	4	experimental	experimental	ADJ
cet-15688	42	5	setup	setup	NOUN
cet-15688	42	6	for	for	ADP
cet-15688	42	7	formaldehyde	formaldehyde	NOUN
cet-15688	42	8	synthesis	synthesis	NOUN
cet-15688	42	9	(	(	PUNCT
cet-15688	42	10	1	1	NUM
cet-15688	42	11	–	–	PUNCT
cet-15688	42	12	tank	tank	NOUN
cet-15688	42	13	with	with	ADP
cet-15688	42	14	reaction	reaction	NOUN
cet-15688	42	15	mixture	mixture	NOUN
cet-15688	42	16	,	,	PUNCT
cet-15688	42	17	2	2	NUM
cet-15688	42	18	–	–	PUNCT
cet-15688	42	19	tank	tank	NOUN
cet-15688	42	20	with	with	ADP
cet-15688	42	21	hydrogen	hydrogen	NOUN
cet-15688	42	22	,	,	PUNCT
cet-15688	42	23	3	3	NUM
cet-15688	42	24	–	–	PUNCT
cet-15688	42	25	reactor	reactor	NOUN
cet-15688	42	26	,	,	PUNCT
cet-15688	42	27	4	4	NUM
cet-15688	42	28	–	–	PUNCT
cet-15688	42	29	mixer	mixer	NOUN
cet-15688	42	30	,	,	PUNCT
cet-15688	42	31	5	5	NUM
cet-15688	42	32	–	–	PUNCT
cet-15688	42	33	electric	electric	ADJ
cet-15688	42	34	heater	heater	NOUN
cet-15688	42	35	,	,	PUNCT
cet-15688	42	36	6	6	NUM
cet-15688	42	37	–	–	PUNCT
cet-15688	42	38	online	online	ADJ
cet-15688	42	39	gas	gas	NOUN
cet-15688	42	40	chromatograph	chromatograph	NOUN
cet-15688	42	41	)	)	PUNCT
cet-15688	42	42	374	374	NUM
cet-15688	42	43	2.4	2.4	NUM
cet-15688	42	44	analysis	analysis	NOUN
cet-15688	42	45	gc	gc	PROPN
cet-15688	42	46	and	and	CCONJ
cet-15688	42	47	mass	mass	ADJ
cet-15688	42	48	-	-	PUNCT
cet-15688	42	49	spectroscopic	spectroscopic	NOUN
cet-15688	42	50	analysis	analysis	NOUN
cet-15688	42	51	.	.	PUNCT
cet-15688	43	1	the	the	DET
cet-15688	43	2	reactor	reactor	NOUN
cet-15688	43	3	was	be	AUX
cet-15688	43	4	connected	connect	VERB
cet-15688	43	5	to	to	ADP
cet-15688	43	6	a	a	DET
cet-15688	43	7	gas	gas	NOUN
cet-15688	43	8	chromatograph	chromatograph	NOUN
cet-15688	43	9	,	,	PUNCT
cet-15688	43	10	kristall	kristall	PROPN
cet-15688	43	11	2000	2000	NUM
cet-15688	43	12	m	m	PROPN
cet-15688	43	13	,	,	PUNCT
cet-15688	43	14	equipped	equip	VERB
cet-15688	43	15	with	with	ADP
cet-15688	43	16	the	the	DET
cet-15688	43	17	chromatographic	chromatographic	ADJ
cet-15688	43	18	column	column	NOUN
cet-15688	43	19	,	,	PUNCT
cet-15688	43	20	hayesep	hayesep	NOUN
cet-15688	43	21	q80/100	q80/100	PROPN
cet-15688	43	22	(	(	PUNCT
cet-15688	43	23	l	l	NOUN
cet-15688	43	24	=	=	SYM
cet-15688	43	25	3	3	NUM
cet-15688	43	26	m	m	NOUN
cet-15688	43	27	,	,	PUNCT
cet-15688	43	28	d	d	NOUN
cet-15688	43	29	=	=	SYM
cet-15688	43	30	2	2	NUM
cet-15688	43	31	mm	mm	NOUN
cet-15688	43	32	,	,	PUNCT
cet-15688	43	33	the	the	DET
cet-15688	43	34	maximum	maximum	ADJ
cet-15688	43	35	column	column	NOUN
cet-15688	43	36	temperature	temperature	NOUN
cet-15688	43	37	is	be	AUX
cet-15688	43	38	275	275	NUM
cet-15688	43	39	°	°	NOUN
cet-15688	43	40	c	c	NOUN
cet-15688	43	41	)	)	PUNCT
cet-15688	43	42	.	.	PUNCT
cet-15688	44	1	the	the	DET
cet-15688	44	2	transport	transport	NOUN
cet-15688	44	3	line	line	NOUN
cet-15688	44	4	temperature	temperature	NOUN
cet-15688	44	5	was	be	AUX
cet-15688	44	6	maintained	maintain	VERB
cet-15688	44	7	at	at	ADP
cet-15688	44	8	80	80	NUM
cet-15688	44	9	°	°	NOUN
cet-15688	44	10	c	c	NOUN
cet-15688	44	11	,	,	PUNCT
cet-15688	44	12	the	the	DET
cet-15688	44	13	analysis	analysis	NOUN
cet-15688	44	14	valve	valve	NOUN
cet-15688	44	15	temperature	temperature	NOUN
cet-15688	44	16	was	be	AUX
cet-15688	44	17	150	150	NUM
cet-15688	44	18	°	°	NOUN
cet-15688	44	19	c	c	NOUN
cet-15688	44	20	,	,	PUNCT
cet-15688	44	21	the	the	DET
cet-15688	44	22	evaporator	evaporator	NOUN
cet-15688	44	23	temperature	temperature	NOUN
cet-15688	44	24	was	be	AUX
cet-15688	44	25	230	230	NUM
cet-15688	44	26	°	°	NOUN
cet-15688	44	27	c	c	NOUN
cet-15688	44	28	,	,	PUNCT
cet-15688	44	29	the	the	DET
cet-15688	44	30	temperature	temperature	NOUN
cet-15688	44	31	of	of	ADP
cet-15688	44	32	flame	flame	NOUN
cet-15688	44	33	ionization	ionization	NOUN
cet-15688	44	34	detector	detector	NOUN
cet-15688	44	35	was	be	AUX
cet-15688	44	36	250	250	NUM
cet-15688	44	37	°	°	NOUN
cet-15688	44	38	c	c	NOUN
cet-15688	44	39	.	.	PUNCT
cet-15688	45	1	the	the	DET
cet-15688	45	2	column	column	NOUN
cet-15688	45	3	temperature	temperature	NOUN
cet-15688	45	4	was	be	AUX
cet-15688	45	5	maintained	maintain	VERB
cet-15688	45	6	at	at	ADP
cet-15688	45	7	40	40	NUM
cet-15688	45	8	°	°	NOUN
cet-15688	45	9	c	c	NOUN
cet-15688	45	10	for	for	ADP
cet-15688	45	11	the	the	DET
cet-15688	45	12	first	first	ADJ
cet-15688	45	13	5	5	NUM
cet-15688	45	14	minutes	minute	NOUN
cet-15688	45	15	of	of	ADP
cet-15688	45	16	analysis	analysis	NOUN
cet-15688	45	17	,	,	PUNCT
cet-15688	45	18	then	then	ADV
cet-15688	45	19	it	it	PRON
cet-15688	45	20	increased	increase	VERB
cet-15688	45	21	to	to	ADP
cet-15688	45	22	245	245	NUM
cet-15688	45	23	°	°	NOUN
cet-15688	45	24	c	c	NOUN
cet-15688	45	25	with	with	ADP
cet-15688	45	26	a	a	DET
cet-15688	45	27	rate	rate	NOUN
cet-15688	45	28	of	of	ADP
cet-15688	45	29	10	10	NUM
cet-15688	45	30	°	°	NOUN
cet-15688	45	31	c	c	NOUN
cet-15688	45	32	/	/	SYM
cet-15688	45	33	min	min	NOUN
cet-15688	45	34	.	.	PUNCT
cet-15688	45	35	the	the	DET
cet-15688	45	36	gas	gas	NOUN
cet-15688	45	37	phase	phase	NOUN
cet-15688	45	38	feed	feed	NOUN
cet-15688	45	39	rate	rate	NOUN
cet-15688	45	40	was	be	AUX
cet-15688	45	41	20	20	NUM
cet-15688	45	42	ml	ml	NOUN
cet-15688	45	43	/	/	SYM
cet-15688	45	44	min	min	NOUN
cet-15688	45	45	,	,	PUNCT
cet-15688	45	46	the	the	DET
cet-15688	45	47	hydrogen	hydrogen	NOUN
cet-15688	45	48	feed	feed	NOUN
cet-15688	45	49	rate	rate	NOUN
cet-15688	45	50	was	be	AUX
cet-15688	45	51	25	25	NUM
cet-15688	45	52	ml	ml	NOUN
cet-15688	45	53	/	/	SYM
cet-15688	45	54	min	min	NOUN
cet-15688	45	55	,	,	PUNCT
cet-15688	45	56	and	and	CCONJ
cet-15688	45	57	the	the	DET
cet-15688	45	58	air	air	NOUN
cet-15688	45	59	feed	feed	NOUN
cet-15688	45	60	rate	rate	NOUN
cet-15688	45	61	was	be	AUX
cet-15688	45	62	250	250	NUM
cet-15688	45	63	ml	ml	NOUN
cet-15688	45	64	/	/	SYM
cet-15688	45	65	min	min	NOUN
cet-15688	45	66	.	.	PROPN
cet-15688	45	67	for	for	ADP
cet-15688	45	68	liquid	liquid	ADJ
cet-15688	45	69	phase	phase	NOUN
cet-15688	45	70	analysis	analysis	NOUN
cet-15688	45	71	,	,	PUNCT
cet-15688	45	72	a	a	DET
cet-15688	45	73	shimadzu	shimadzu	ADJ
cet-15688	45	74	hpmsqp2010	hpmsqp2010	PROPN
cet-15688	45	75	gc	gc	PROPN
cet-15688	45	76	-	-	PUNCT
cet-15688	45	77	ms	ms	PROPN
cet-15688	45	78	spectrometer	spectrometer	NOUN
cet-15688	45	79	was	be	AUX
cet-15688	45	80	used	use	VERB
cet-15688	45	81	to	to	PART
cet-15688	45	82	analyze	analyze	VERB
cet-15688	45	83	samples	sample	NOUN
cet-15688	45	84	.	.	PUNCT
cet-15688	46	1	the	the	DET
cet-15688	46	2	sample	sample	NOUN
cet-15688	46	3	was	be	AUX
cet-15688	46	4	analyzed	analyze	VERB
cet-15688	46	5	using	use	VERB
cet-15688	46	6	a	a	DET
cet-15688	46	7	capillary	capillary	ADJ
cet-15688	46	8	column	column	NOUN
cet-15688	46	9	(	(	PUNCT
cet-15688	46	10	ms-1	ms-1	NOUN
cet-15688	46	11	)	)	PUNCT
cet-15688	46	12	,	,	PUNCT
cet-15688	46	13	with	with	ADP
cet-15688	46	14	a	a	DET
cet-15688	46	15	length	length	NOUN
cet-15688	46	16	of	of	ADP
cet-15688	46	17	100	100	NUM
cet-15688	46	18	m	m	NOUN
cet-15688	46	19	and	and	CCONJ
cet-15688	46	20	a	a	DET
cet-15688	46	21	diameter	diameter	NOUN
cet-15688	46	22	of	of	ADP
cet-15688	46	23	0.32	0.32	NUM
cet-15688	46	24	mm	mm	NOUN
cet-15688	46	25	.	.	PUNCT
cet-15688	47	1	the	the	DET
cet-15688	47	2	maximum	maximum	ADJ
cet-15688	47	3	column	column	NOUN
cet-15688	47	4	temperature	temperature	NOUN
cet-15688	47	5	was	be	AUX
cet-15688	47	6	set	set	VERB
cet-15688	47	7	to	to	ADP
cet-15688	47	8	310	310	NUM
cet-15688	47	9	°	°	NOUN
cet-15688	47	10	c	c	NOUN
cet-15688	47	11	.	.	PUNCT
cet-15688	48	1	the	the	DET
cet-15688	48	2	initial	initial	ADJ
cet-15688	48	3	thermostat	thermostat	NOUN
cet-15688	48	4	temperature	temperature	NOUN
cet-15688	48	5	was	be	AUX
cet-15688	48	6	set	set	VERB
cet-15688	48	7	at	at	ADP
cet-15688	48	8	50	50	NUM
cet-15688	48	9	°	°	NOUN
cet-15688	48	10	c	c	NOUN
cet-15688	48	11	,	,	PUNCT
cet-15688	48	12	the	the	DET
cet-15688	48	13	evaporator	evaporator	NOUN
cet-15688	48	14	temperature	temperature	NOUN
cet-15688	48	15	set	set	VERB
cet-15688	48	16	at	at	ADP
cet-15688	48	17	300	300	NUM
cet-15688	48	18	°	°	NOUN
cet-15688	48	19	c	c	NOUN
cet-15688	48	20	,	,	PUNCT
cet-15688	48	21	and	and	CCONJ
cet-15688	48	22	the	the	DET
cet-15688	48	23	gas	gas	NOUN
cet-15688	48	24	pressure	pressure	NOUN
cet-15688	48	25	set	set	VERB
cet-15688	48	26	at	at	ADP
cet-15688	48	27	182.9	182.9	NUM
cet-15688	48	28	kpa	kpa	NOUN
cet-15688	48	29	.	.	PUNCT
cet-15688	49	1	the	the	DET
cet-15688	49	2	helium	helium	NOUN
cet-15688	49	3	flow	flow	NOUN
cet-15688	49	4	rate	rate	NOUN
cet-15688	49	5	was	be	AUX
cet-15688	49	6	set	set	VERB
cet-15688	49	7	at	at	ADP
cet-15688	49	8	81.5	81.5	NUM
cet-15688	49	9	ml	ml	NOUN
cet-15688	49	10	/	/	SYM
cet-15688	49	11	min	min	NOUN
cet-15688	49	12	,	,	PUNCT
cet-15688	49	13	and	and	CCONJ
cet-15688	49	14	the	the	DET
cet-15688	49	15	carrier	carrier	NOUN
cet-15688	49	16	gas	gas	NOUN
cet-15688	49	17	flow	flow	NOUN
cet-15688	49	18	rate	rate	NOUN
cet-15688	49	19	was	be	AUX
cet-15688	49	20	set	set	VERB
cet-15688	49	21	at	at	ADP
cet-15688	49	22	1	1	NUM
cet-15688	49	23	ml	ml	NOUN
cet-15688	49	24	/	/	SYM
cet-15688	49	25	min	min	NOUN
cet-15688	49	26	.	.	PUNCT
cet-15688	50	1	the	the	DET
cet-15688	50	2	gas	gas	NOUN
cet-15688	50	3	velocity	velocity	NOUN
cet-15688	50	4	was	be	AUX
cet-15688	50	5	19.9	19.9	NUM
cet-15688	50	6	cm	cm	NOUN
cet-15688	50	7	/	/	SYM
cet-15688	50	8	s	s	PROPN
cet-15688	50	9	,	,	PUNCT
cet-15688	50	10	and	and	CCONJ
cet-15688	50	11	the	the	DET
cet-15688	50	12	purge	purge	NOUN
cet-15688	50	13	gas	gas	NOUN
cet-15688	50	14	flow	flow	NOUN
cet-15688	50	15	rate	rate	NOUN
cet-15688	50	16	was	be	AUX
cet-15688	50	17	5	5	NUM
cet-15688	50	18	ml	ml	NOUN
cet-15688	50	19	/	/	SYM
cet-15688	50	20	min	min	NOUN
cet-15688	50	21	.	.	PROPN
cet-15688	50	22	gas	gas	NOUN
cet-15688	50	23	split	split	NOUN
cet-15688	50	24	ratio	ratio	NOUN
cet-15688	50	25	was	be	AUX
cet-15688	50	26	set	set	VERB
cet-15688	50	27	at	at	ADP
cet-15688	50	28	1:1	1:1	NUM
cet-15688	50	29	,	,	PUNCT
cet-15688	50	30	evaporator	evaporator	NOUN
cet-15688	50	31	pressure	pressure	NOUN
cet-15688	50	32	was	be	AUX
cet-15688	50	33	set	set	VERB
cet-15688	50	34	at	at	ADP
cet-15688	50	35	200	200	NUM
cet-15688	50	36	kpa	kpa	NOUN
cet-15688	50	37	,	,	PUNCT
cet-15688	50	38	and	and	CCONJ
cet-15688	50	39	sampling	sample	VERB
cet-15688	50	40	time	time	NOUN
cet-15688	50	41	was	be	AUX
cet-15688	50	42	set	set	VERB
cet-15688	50	43	at	at	ADP
cet-15688	50	44	5	5	NUM
cet-15688	50	45	s.	s.	PROPN
cet-15688	50	46	the	the	DET
cet-15688	50	47	column	column	NOUN
cet-15688	50	48	temperature	temperature	NOUN
cet-15688	50	49	was	be	AUX
cet-15688	50	50	maintained	maintain	VERB
cet-15688	50	51	at	at	ADP
cet-15688	50	52	50	50	NUM
cet-15688	50	53	°	°	NOUN
cet-15688	50	54	c	c	NOUN
cet-15688	50	55	for	for	ADP
cet-15688	50	56	10	10	NUM
cet-15688	50	57	min	min	NOUN
cet-15688	50	58	,	,	PUNCT
cet-15688	50	59	then	then	ADV
cet-15688	50	60	it	it	PRON
cet-15688	50	61	was	be	AUX
cet-15688	50	62	increased	increase	VERB
cet-15688	50	63	to	to	ADP
cet-15688	50	64	310	310	NUM
cet-15688	50	65	°	°	NOUN
cet-15688	50	66	c	c	NOUN
cet-15688	50	67	at	at	ADP
cet-15688	50	68	a	a	DET
cet-15688	50	69	rate	rate	NOUN
cet-15688	50	70	of	of	ADP
cet-15688	50	71	10	10	NUM
cet-15688	50	72	°	°	NOUN
cet-15688	50	73	c	c	PROPN
cet-15688	50	74	/	/	SYM
cet-15688	50	75	min	min	PROPN
cet-15688	50	76	.	.	PROPN
cet-15688	50	77	ion	ion	NOUN
cet-15688	50	78	source	source	NOUN
cet-15688	50	79	and	and	CCONJ
cet-15688	50	80	interface	interface	NOUN
cet-15688	50	81	temperatures	temperature	NOUN
cet-15688	50	82	were	be	AUX
cet-15688	50	83	set	set	VERB
cet-15688	50	84	at	at	ADP
cet-15688	50	85	260	260	NUM
cet-15688	50	86	°	°	ADP
cet-15688	50	87	c	c	NOUN
cet-15688	50	88	and	and	CCONJ
cet-15688	50	89	280	280	NUM
cet-15688	50	90	°	°	NOUN
cet-15688	50	91	c	c	NOUN
cet-15688	50	92	respectively	respectively	ADV
cet-15688	50	93	.	.	PUNCT
cet-15688	51	1	the	the	DET
cet-15688	51	2	initial	initial	ADJ
cet-15688	51	3	measured	measure	VERB
cet-15688	51	4	mass	mass	NOUN
cet-15688	51	5	was	be	AUX
cet-15688	51	6	10	10	NUM
cet-15688	51	7	amu	amu	NOUN
cet-15688	51	8	,	,	PUNCT
cet-15688	51	9	and	and	CCONJ
cet-15688	51	10	the	the	DET
cet-15688	51	11	final	final	ADJ
cet-15688	51	12	mass	mass	NOUN
cet-15688	51	13	was	be	AUX
cet-15688	51	14	100	100	NUM
cet-15688	51	15	amu	amu	PROPN
cet-15688	51	16	.	.	PUNCT
cet-15688	52	1	peak	peak	PROPN
cet-15688	52	2	identification	identification	NOUN
cet-15688	52	3	was	be	AUX
cet-15688	52	4	made	make	VERB
cet-15688	52	5	using	use	VERB
cet-15688	52	6	the	the	DET
cet-15688	52	7	nist	nist	NOUN
cet-15688	52	8	library	library	NOUN
cet-15688	52	9	,	,	PUNCT
cet-15688	52	10	and	and	CCONJ
cet-15688	52	11	concentration	concentration	NOUN
cet-15688	52	12	of	of	ADP
cet-15688	52	13	reaction	reaction	NOUN
cet-15688	52	14	products	product	NOUN
cet-15688	52	15	was	be	AUX
cet-15688	52	16	made	make	VERB
cet-15688	52	17	using	use	VERB
cet-15688	52	18	the	the	DET
cet-15688	52	19	calibration	calibration	NOUN
cet-15688	52	20	curves	curve	NOUN
cet-15688	52	21	.	.	PUNCT
cet-15688	53	1	x	x	X
cet-15688	53	2	-	-	PUNCT
cet-15688	53	3	ray	ray	NOUN
cet-15688	53	4	fluorescence	fluorescence	NOUN
cet-15688	53	5	analysis	analysis	NOUN
cet-15688	53	6	was	be	AUX
cet-15688	53	7	made	make	VERB
cet-15688	53	8	using	use	VERB
cet-15688	53	9	a	a	DET
cet-15688	53	10	spectroscan	spectroscan	ADJ
cet-15688	53	11	-	-	PUNCT
cet-15688	53	12	maks	mak	NOUN
cet-15688	53	13	-	-	PUNCT
cet-15688	53	14	gf1e	gf1e	PROPN
cet-15688	53	15	spectrometer	spectrometer	NOUN
cet-15688	53	16	equipped	equip	VERB
cet-15688	53	17	with	with	ADP
cet-15688	53	18	a	a	DET
cet-15688	53	19	mo	mo	NOUN
cet-15688	53	20	anode	anode	NOUN
cet-15688	53	21	and	and	CCONJ
cet-15688	53	22	lif	lif	PROPN
cet-15688	53	23	crystal	crystal	PROPN
cet-15688	53	24	analyzer	analyzer	PROPN
cet-15688	53	25	and	and	CCONJ
cet-15688	53	26	sz	sz	NOUN
cet-15688	53	27	detectors	detector	NOUN
cet-15688	53	28	.	.	PUNCT
cet-15688	54	1	the	the	DET
cet-15688	54	2	analysis	analysis	NOUN
cet-15688	54	3	was	be	AUX
cet-15688	54	4	based	base	VERB
cet-15688	54	5	on	on	ADP
cet-15688	54	6	the	the	DET
cet-15688	54	7	co	co	PROPN
cet-15688	54	8	ka	ka	PROPN
cet-15688	54	9	line	line	PROPN
cet-15688	54	10	.	.	PUNCT
cet-15688	55	1	a	a	DET
cet-15688	55	2	series	series	NOUN
cet-15688	55	3	of	of	ADP
cet-15688	55	4	standards	standard	NOUN
cet-15688	55	5	containing	contain	VERB
cet-15688	55	6	metals	metal	NOUN
cet-15688	55	7	was	be	AUX
cet-15688	55	8	prepared	prepare	VERB
cet-15688	55	9	by	by	ADP
cet-15688	55	10	mixing	mix	VERB
cet-15688	55	11	0.1–0.2	0.1–0.2	NOUN
cet-15688	56	1	g	g	NOUN
cet-15688	56	2	of	of	ADP
cet-15688	56	3	matrix	matrix	NOUN
cet-15688	56	4	with	with	ADP
cet-15688	56	5	10–20	10–20	NUM
cet-15688	56	6	mg	mg	NOUN
cet-15688	56	7	of	of	ADP
cet-15688	56	8	standard	standard	ADJ
cet-15688	56	9	metal	metal	NOUN
cet-15688	56	10	compound	compound	NOUN
cet-15688	56	11	.	.	PUNCT
cet-15688	57	1	liquid	liquid	ADJ
cet-15688	57	2	nitrogen	nitrogen	NOUN
cet-15688	57	3	physisorption	physisorption	NOUN
cet-15688	57	4	was	be	AUX
cet-15688	57	5	made	make	VERB
cet-15688	57	6	at	at	ADP
cet-15688	57	7	the	the	DET
cet-15688	57	8	normal	normal	ADJ
cet-15688	57	9	boiling	boiling	NOUN
cet-15688	57	10	point	point	NOUN
cet-15688	57	11	of	of	ADP
cet-15688	57	12	liquid	liquid	ADJ
cet-15688	57	13	nitrogen	nitrogen	NOUN
cet-15688	57	14	,	,	PUNCT
cet-15688	57	15	using	use	VERB
cet-15688	57	16	a	a	DET
cet-15688	57	17	beckman	beckman	PROPN
cet-15688	57	18	coulter	coulter	PROPN
cet-15688	57	19	sa3100	sa3100	PROPN
cet-15688	57	20	instrument	instrument	NOUN
cet-15688	57	21	.	.	PUNCT
cet-15688	58	1	before	before	ADP
cet-15688	58	2	the	the	DET
cet-15688	58	3	analysis	analysis	NOUN
cet-15688	58	4	,	,	PUNCT
cet-15688	58	5	the	the	DET
cet-15688	58	6	samples	sample	NOUN
cet-15688	58	7	were	be	AUX
cet-15688	58	8	degassed	degas	VERB
cet-15688	58	9	using	use	VERB
cet-15688	58	10	a	a	DET
cet-15688	58	11	beckman	beckman	PROPN
cet-15688	58	12	sa	sa	PROPN
cet-15688	58	13	-	-	PUNCT
cet-15688	58	14	prep	prep	NOUN
cet-15688	58	15	instrument	instrument	NOUN
cet-15688	58	16	for	for	ADP
cet-15688	58	17	sample	sample	NOUN
cet-15688	58	18	preparation	preparation	NOUN
cet-15688	58	19	at	at	ADP
cet-15688	58	20	120	120	NUM
cet-15688	58	21	°	°	NOUN
cet-15688	58	22	c	c	NOUN
cet-15688	58	23	in	in	ADP
cet-15688	58	24	a	a	DET
cet-15688	58	25	vacuum	vacuum	NOUN
cet-15688	58	26	for	for	ADP
cet-15688	58	27	1	1	NUM
cet-15688	58	28	h.	h.	PROPN
cet-15688	58	29	hydrogen	hydrogen	PROPN
cet-15688	58	30	and	and	CCONJ
cet-15688	58	31	carbon	carbon	NOUN
cet-15688	58	32	dioxide	dioxide	NOUN
cet-15688	58	33	chemisorption	chemisorption	NOUN
cet-15688	58	34	was	be	AUX
cet-15688	58	35	performed	perform	VERB
cet-15688	58	36	using	use	VERB
cet-15688	58	37	the	the	DET
cet-15688	58	38	micromeritics	micromeritic	NOUN
cet-15688	58	39	autochem	autochem	NOUN
cet-15688	58	40	2910	2910	NUM
cet-15688	58	41	.	.	PUNCT
cet-15688	59	1	prior	prior	ADV
cet-15688	59	2	to	to	ADP
cet-15688	59	3	analysis	analysis	NOUN
cet-15688	59	4	,	,	PUNCT
cet-15688	59	5	the	the	DET
cet-15688	59	6	samples	sample	NOUN
cet-15688	59	7	were	be	AUX
cet-15688	59	8	purified	purify	VERB
cet-15688	59	9	in	in	ADP
cet-15688	59	10	-	-	PUNCT
cet-15688	59	11	situ	situ	NOUN
cet-15688	59	12	at	at	ADP
cet-15688	59	13	500	500	NUM
cet-15688	59	14	°	°	NOUN
cet-15688	59	15	c	c	NOUN
cet-15688	59	16	for	for	ADP
cet-15688	59	17	2	2	NUM
cet-15688	59	18	hours	hour	NOUN
cet-15688	59	19	in	in	ADP
cet-15688	59	20	a	a	DET
cet-15688	59	21	continuous	continuous	ADJ
cet-15688	59	22	stream	stream	NOUN
cet-15688	59	23	of	of	ADP
cet-15688	59	24	ar	ar	NOUN
cet-15688	59	25	and	and	CCONJ
cet-15688	59	26	he	he	PRON
cet-15688	59	27	,	,	PUNCT
cet-15688	59	28	then	then	ADV
cet-15688	59	29	the	the	DET
cet-15688	59	30	temperature	temperature	NOUN
cet-15688	59	31	was	be	AUX
cet-15688	59	32	decreased	decrease	VERB
cet-15688	59	33	to	to	ADP
cet-15688	59	34	105	105	NUM
cet-15688	59	35	°	°	NOUN
cet-15688	59	36	c	c	NOUN
cet-15688	59	37	and	and	CCONJ
cet-15688	59	38	the	the	DET
cet-15688	59	39	samples	sample	NOUN
cet-15688	59	40	were	be	AUX
cet-15688	59	41	flushed	flush	VERB
cet-15688	59	42	with	with	ADP
cet-15688	59	43	active	active	ADJ
cet-15688	59	44	gases	gas	NOUN
cet-15688	59	45	for	for	ADP
cet-15688	59	46	an	an	DET
cet-15688	59	47	hour	hour	NOUN
cet-15688	59	48	.	.	PUNCT
cet-15688	60	1	after	after	ADP
cet-15688	60	2	that	that	PRON
cet-15688	60	3	,	,	PUNCT
cet-15688	60	4	the	the	DET
cet-15688	60	5	samples	sample	NOUN
cet-15688	60	6	were	be	AUX
cet-15688	60	7	again	again	ADV
cet-15688	60	8	flushed	flush	VERB
cet-15688	60	9	with	with	ADP
cet-15688	60	10	ar	ar	NOUN
cet-15688	60	11	or	or	CCONJ
cet-15688	60	12	he	he	PRON
cet-15688	60	13	in	in	ADP
cet-15688	60	14	order	order	NOUN
cet-15688	60	15	to	to	PART
cet-15688	60	16	reduce	reduce	VERB
cet-15688	60	17	the	the	DET
cet-15688	60	18	amount	amount	NOUN
cet-15688	60	19	of	of	ADP
cet-15688	60	20	physically	physically	ADV
cet-15688	60	21	adsorbed	adsorb	VERB
cet-15688	60	22	gases	gas	NOUN
cet-15688	60	23	,	,	PUNCT
cet-15688	60	24	and	and	CCONJ
cet-15688	60	25	then	then	ADV
cet-15688	60	26	the	the	DET
cet-15688	60	27	temperature	temperature	NOUN
cet-15688	60	28	was	be	AUX
cet-15688	60	29	increased	increase	VERB
cet-15688	60	30	to	to	ADP
cet-15688	60	31	500	500	NUM
cet-15688	60	32	°	°	NOUN
cet-15688	60	33	c	c	NOUN
cet-15688	60	34	at	at	ADP
cet-15688	60	35	a	a	DET
cet-15688	60	36	rate	rate	NOUN
cet-15688	60	37	of	of	ADP
cet-15688	60	38	10	10	NUM
cet-15688	60	39	°	°	NOUN
cet-15688	60	40	c	c	NOUN
cet-15688	60	41	/	/	SYM
cet-15688	60	42	min	min	NOUN
cet-15688	60	43	,	,	PUNCT
cet-15688	60	44	and	and	CCONJ
cet-15688	60	45	gas	gas	NOUN
cet-15688	60	46	adsorption	adsorption	NOUN
cet-15688	60	47	curves	curve	NOUN
cet-15688	60	48	were	be	AUX
cet-15688	60	49	recorded	record	VERB
cet-15688	60	50	.	.	PUNCT
cet-15688	61	1	3	3	X
cet-15688	61	2	.	.	X
cet-15688	61	3	results	result	NOUN
cet-15688	61	4	and	and	CCONJ
cet-15688	61	5	discussion	discussion	VERB
cet-15688	61	6	the	the	DET
cet-15688	61	7	initial	initial	ADJ
cet-15688	61	8	sample	sample	NOUN
cet-15688	61	9	of	of	ADP
cet-15688	61	10	silica	silica	NOUN
cet-15688	61	11	was	be	AUX
cet-15688	61	12	characterized	characterize	VERB
cet-15688	61	13	by	by	ADP
cet-15688	61	14	a	a	DET
cet-15688	61	15	nitrogen	nitrogen	NOUN
cet-15688	61	16	physisorption	physisorption	NOUN
cet-15688	61	17	isotherm	isotherm	NOUN
cet-15688	61	18	(	(	PUNCT
cet-15688	61	19	figure	figure	NOUN
cet-15688	61	20	3	3	NUM
cet-15688	61	21	)	)	PUNCT
cet-15688	61	22	,	,	PUNCT
cet-15688	61	23	the	the	PRON
cet-15688	61	24	obtained	obtain	VERB
cet-15688	61	25	isotherm	isotherm	NOUN
cet-15688	61	26	curve	curve	NOUN
cet-15688	61	27	is	be	AUX
cet-15688	61	28	typical	typical	ADJ
cet-15688	61	29	for	for	ADP
cet-15688	61	30	micro	micro	ADJ
cet-15688	61	31	-	-	NOUN
cet-15688	61	32	mesopores	mesopore	NOUN
cet-15688	61	33	samples	sample	NOUN
cet-15688	61	34	.	.	PUNCT
cet-15688	62	1	the	the	DET
cet-15688	62	2	incorporation	incorporation	NOUN
cet-15688	62	3	of	of	ADP
cet-15688	62	4	metal	metal	NOUN
cet-15688	62	5	over	over	ADP
cet-15688	62	6	silica	silica	NOUN
cet-15688	62	7	surface	surface	NOUN
cet-15688	62	8	results	result	NOUN
cet-15688	62	9	in	in	ADP
cet-15688	62	10	some	some	DET
cet-15688	62	11	decrease	decrease	NOUN
cet-15688	62	12	of	of	ADP
cet-15688	62	13	hysteresis	hysteresis	NOUN
cet-15688	62	14	loop	loop	NOUN
cet-15688	62	15	,	,	PUNCT
cet-15688	62	16	from	from	ADP
cet-15688	62	17	the	the	DET
cet-15688	62	18	other	other	ADJ
cet-15688	62	19	side	side	NOUN
cet-15688	62	20	,	,	PUNCT
cet-15688	62	21	micropore	micropore	NOUN
cet-15688	62	22	region	region	NOUN
cet-15688	62	23	remains	remain	VERB
cet-15688	62	24	unchanged	unchanged	ADJ
cet-15688	62	25	.	.	PUNCT
cet-15688	63	1	figure	figure	VERB
cet-15688	63	2	3	3	NUM
cet-15688	63	3	:	:	PUNCT
cet-15688	63	4	nitrogen	nitrogen	NOUN
cet-15688	63	5	physisorption	physisorption	NOUN
cet-15688	63	6	isotherms	isotherm	NOUN
cet-15688	63	7	for	for	ADP
cet-15688	63	8	a	a	DET
cet-15688	63	9	)	)	PUNCT
cet-15688	63	10	monometallic	monometallic	NOUN
cet-15688	63	11	and	and	CCONJ
cet-15688	63	12	b	b	NOUN
cet-15688	63	13	)	)	PUNCT
cet-15688	63	14	bimetallic	bimetallic	NOUN
cet-15688	63	15	samples	sample	NOUN
cet-15688	63	16	in	in	ADP
cet-15688	63	17	the	the	DET
cet-15688	63	18	case	case	NOUN
cet-15688	63	19	of	of	ADP
cet-15688	63	20	bimetallic	bimetallic	ADJ
cet-15688	63	21	samples	sample	NOUN
cet-15688	63	22	,	,	PUNCT
cet-15688	63	23	ni	ni	PROPN
cet-15688	63	24	-	-	PROPN
cet-15688	63	25	cu	cu	PROPN
cet-15688	63	26	-	-	PUNCT
cet-15688	63	27	sio2	sio2	PROPN
cet-15688	63	28	and	and	CCONJ
cet-15688	63	29	cu	cu	PROPN
cet-15688	63	30	-	-	PUNCT
cet-15688	63	31	ni	ni	PROPN
cet-15688	63	32	-	-	NOUN
cet-15688	63	33	sio2	sio2	NOUN
cet-15688	63	34	a	a	DET
cet-15688	63	35	decrease	decrease	NOUN
cet-15688	63	36	in	in	ADP
cet-15688	63	37	mesopore	mesopore	NOUN
cet-15688	63	38	loop	loop	NOUN
cet-15688	63	39	is	be	AUX
cet-15688	63	40	rather	rather	ADV
cet-15688	63	41	noticeable	noticeable	ADJ
cet-15688	63	42	.	.	PUNCT
cet-15688	64	1	in	in	ADP
cet-15688	64	2	the	the	DET
cet-15688	64	3	case	case	NOUN
cet-15688	64	4	of	of	ADP
cet-15688	64	5	platinum	platinum	NOUN
cet-15688	64	6	containing	contain	VERB
cet-15688	64	7	pt	pt	PROPN
cet-15688	64	8	-	-	PUNCT
cet-15688	64	9	cu	cu	PROPN
cet-15688	64	10	-	-	PUNCT
cet-15688	64	11	sio2	sio2	PROPN
cet-15688	64	12	sample	sample	NOUN
cet-15688	64	13	,	,	PUNCT
cet-15688	64	14	some	some	DET
cet-15688	64	15	decrease	decrease	NOUN
cet-15688	64	16	in	in	ADP
cet-15688	64	17	the	the	DET
cet-15688	64	18	micropore	micropore	NOUN
cet-15688	64	19	slope	slope	NOUN
cet-15688	64	20	region	region	NOUN
cet-15688	64	21	can	can	AUX
cet-15688	64	22	be	be	AUX
cet-15688	64	23	determined	determine	VERB
cet-15688	64	24	.	.	PUNCT
cet-15688	65	1	introduction	introduction	NOUN
cet-15688	65	2	of	of	ADP
cet-15688	65	3	cu	cu	PROPN
cet-15688	65	4	on	on	ADP
cet-15688	65	5	silica	silica	NOUN
cet-15688	65	6	support	support	NOUN
cet-15688	65	7	results	result	NOUN
cet-15688	65	8	in	in	ADP
cet-15688	65	9	some	some	DET
cet-15688	65	10	shift	shift	NOUN
cet-15688	65	11	in	in	ADP
cet-15688	65	12	the	the	DET
cet-15688	65	13	pore	pore	ADJ
cet-15688	65	14	diameter	diameter	NOUN
cet-15688	65	15	dispersion	dispersion	NOUN
cet-15688	65	16	from	from	ADP
cet-15688	65	17	5	5	NUM
cet-15688	65	18	nm	nm	NOUN
cet-15688	65	19	to	to	ADP
cet-15688	65	20	7	7	NUM
cet-15688	65	21	nm	nm	NOUN
cet-15688	65	22	(	(	PUNCT
cet-15688	65	23	figure	figure	NOUN
cet-15688	65	24	4a	4a	NUM
cet-15688	65	25	)	)	PUNCT
cet-15688	65	26	,	,	PUNCT
cet-15688	65	27	that	that	PRON
cet-15688	65	28	can	can	AUX
cet-15688	65	29	be	be	AUX
cet-15688	65	30	subscribed	subscribe	VERB
cet-15688	65	31	to	to	ADP
cet-15688	65	32	the	the	DET
cet-15688	65	33	cu	cu	PROPN
cet-15688	65	34	species	specie	NOUN
cet-15688	65	35	formation	formation	NOUN
cet-15688	65	36	in	in	ADP
cet-15688	65	37	the	the	DET
cet-15688	65	38	pores	pore	NOUN
cet-15688	65	39	with	with	ADP
cet-15688	65	40	a	a	DET
cet-15688	65	41	diameter	diameter	NOUN
cet-15688	65	42	of	of	ADP
cet-15688	65	43	3	3	NUM
cet-15688	65	44	-	-	SYM
cet-15688	65	45	4	4	NUM
cet-15688	65	46	nm	nm	NOUN
cet-15688	65	47	.	.	PUNCT
cet-15688	66	1	while	while	SCONJ
cet-15688	66	2	ni	ni	PROPN
cet-15688	66	3	incorporation	incorporation	NOUN
cet-15688	66	4	over	over	ADP
cet-15688	66	5	silica	silica	NOUN
cet-15688	66	6	results	result	NOUN
cet-15688	66	7	in	in	ADP
cet-15688	66	8	a	a	DET
cet-15688	66	9	drastic	drastic	ADJ
cet-15688	66	10	shift	shift	NOUN
cet-15688	66	11	of	of	ADP
cet-15688	66	12	the	the	DET
cet-15688	66	13	pore	pore	ADJ
cet-15688	66	14	dispersion	dispersion	NOUN
cet-15688	66	15	to	to	ADP
cet-15688	66	16	10	10	NUM
cet-15688	66	17	nm	nm	NOUN
cet-15688	66	18	,	,	PUNCT
cet-15688	66	19	that	that	PRON
cet-15688	66	20	can	can	AUX
cet-15688	66	21	be	be	AUX
cet-15688	66	22	explained	explain	VERB
cet-15688	66	23	0	0	NUM
cet-15688	66	24	50	50	NUM
cet-15688	66	25	100	100	NUM
cet-15688	66	26	150	150	NUM
cet-15688	66	27	200	200	NUM
cet-15688	66	28	250	250	NUM
cet-15688	66	29	300	300	NUM
cet-15688	66	30	350	350	NUM
cet-15688	66	31	400	400	NUM
cet-15688	66	32	450	450	NUM
cet-15688	66	33	500	500	NUM
cet-15688	66	34	0	0	NUM
cet-15688	66	35	0.2	0.2	NUM
cet-15688	66	36	0.4	0.4	NUM
cet-15688	66	37	0.6	0.6	NUM
cet-15688	66	38	0.8	0.8	NUM
cet-15688	66	39	1	1	NUM
cet-15688	66	40	v	v	ADP
cet-15688	66	41	a	a	DET
cet-15688	66	42	d	d	X
cet-15688	66	43	s	s	PROPN
cet-15688	66	44	,	,	PUNCT
cet-15688	66	45	c	c	PROPN
cet-15688	66	46	c	c	X
cet-15688	66	47	(	(	PUNCT
cet-15688	66	48	st	st	PROPN
cet-15688	66	49	p	p	PROPN
cet-15688	66	50	)	)	PUNCT
cet-15688	66	51	/	/	SYM
cet-15688	66	52	g	g	PROPN
cet-15688	66	53	ps	ps	PROPN
cet-15688	66	54	/	/	SYM
cet-15688	66	55	p0	p0	PROPN
cet-15688	66	56	sio2	sio2	PROPN
cet-15688	66	57	cu	cu	PROPN
cet-15688	66	58	-	-	PUNCT
cet-15688	66	59	sio2	sio2	PROPN
cet-15688	66	60	ni	ni	PROPN
cet-15688	66	61	-	-	PUNCT
cet-15688	66	62	sio2	sio2	PROPN
cet-15688	66	63	pt	pt	PROPN
cet-15688	66	64	-	-	PUNCT
cet-15688	66	65	sio2	sio2	PROPN
cet-15688	66	66	a	a	PRON
cet-15688	66	67	)	)	PUNCT
cet-15688	66	68	0	0	NUM
cet-15688	67	1	50	50	NUM
cet-15688	67	2	100	100	NUM
cet-15688	67	3	150	150	NUM
cet-15688	67	4	200	200	NUM
cet-15688	67	5	250	250	NUM
cet-15688	67	6	300	300	NUM
cet-15688	67	7	350	350	NUM
cet-15688	67	8	400	400	NUM
cet-15688	67	9	450	450	NUM
cet-15688	67	10	500	500	NUM
cet-15688	67	11	0	0	NUM
cet-15688	67	12	0.2	0.2	NUM
cet-15688	67	13	0.4	0.4	NUM
cet-15688	67	14	0.6	0.6	NUM
cet-15688	67	15	0.8	0.8	NUM
cet-15688	67	16	1	1	NUM
cet-15688	67	17	v	v	ADP
cet-15688	67	18	a	a	DET
cet-15688	67	19	d	d	X
cet-15688	67	20	s	s	PROPN
cet-15688	67	21	,	,	PUNCT
cet-15688	67	22	c	c	PROPN
cet-15688	67	23	c	c	X
cet-15688	67	24	(	(	PUNCT
cet-15688	67	25	st	st	PROPN
cet-15688	67	26	p	p	PROPN
cet-15688	67	27	)	)	PUNCT
cet-15688	67	28	/	/	SYM
cet-15688	67	29	g	g	PROPN
cet-15688	67	30	ps	ps	PROPN
cet-15688	67	31	/	/	SYM
cet-15688	67	32	p0	p0	PROPN
cet-15688	67	33	sio2	sio2	PROPN
cet-15688	67	34	ni	ni	PROPN
cet-15688	67	35	-	-	PROPN
cet-15688	67	36	cu	cu	PROPN
cet-15688	67	37	-	-	PUNCT
cet-15688	67	38	sio2	sio2	PROPN
cet-15688	67	39	cu	cu	PROPN
cet-15688	67	40	-	-	PUNCT
cet-15688	67	41	ni	ni	PROPN
cet-15688	67	42	-	-	PUNCT
cet-15688	67	43	sio2	sio2	PROPN
cet-15688	67	44	pt	pt	PROPN
cet-15688	67	45	-	-	PUNCT
cet-15688	67	46	cu	cu	PROPN
cet-15688	67	47	-	-	PUNCT
cet-15688	67	48	sio2	sio2	PROPN
cet-15688	67	49	b	b	PROPN
cet-15688	67	50	)	)	PUNCT
cet-15688	67	51	375	375	NUM
cet-15688	67	52	by	by	ADP
cet-15688	67	53	ni	ni	PROPN
cet-15688	67	54	species	specie	NOUN
cet-15688	67	55	formation	formation	NOUN
cet-15688	67	56	in	in	ADP
cet-15688	67	57	the	the	DET
cet-15688	67	58	pores	pore	NOUN
cet-15688	67	59	with	with	ADP
cet-15688	67	60	a	a	DET
cet-15688	67	61	diameter	diameter	NOUN
cet-15688	67	62	from	from	ADP
cet-15688	67	63	3	3	NUM
cet-15688	67	64	to	to	PART
cet-15688	67	65	10	10	NUM
cet-15688	67	66	nm	nm	NOUN
cet-15688	67	67	.	.	PUNCT
cet-15688	68	1	from	from	ADP
cet-15688	68	2	the	the	DET
cet-15688	68	3	other	other	ADJ
cet-15688	68	4	side	side	NOUN
cet-15688	68	5	,	,	PUNCT
cet-15688	68	6	pt	pt	X
cet-15688	68	7	incorporation	incorporation	NOUN
cet-15688	68	8	over	over	ADP
cet-15688	68	9	support	support	NOUN
cet-15688	68	10	results	result	NOUN
cet-15688	68	11	only	only	ADV
cet-15688	68	12	in	in	ADP
cet-15688	68	13	a	a	DET
cet-15688	68	14	small	small	ADJ
cet-15688	68	15	decrease	decrease	NOUN
cet-15688	68	16	in	in	ADP
cet-15688	68	17	the	the	DET
cet-15688	68	18	pore	pore	ADJ
cet-15688	68	19	volume	volume	NOUN
cet-15688	68	20	in	in	ADP
cet-15688	68	21	the	the	DET
cet-15688	68	22	4	4	NUM
cet-15688	68	23	-	-	SYM
cet-15688	68	24	6	6	NUM
cet-15688	68	25	nm	nm	NOUN
cet-15688	68	26	region	region	NOUN
cet-15688	68	27	that	that	PRON
cet-15688	68	28	can	can	AUX
cet-15688	68	29	be	be	AUX
cet-15688	68	30	subscribed	subscribe	VERB
cet-15688	68	31	to	to	ADP
cet-15688	68	32	pt	pt	VERB
cet-15688	68	33	species	specie	NOUN
cet-15688	68	34	formation	formation	NOUN
cet-15688	68	35	in	in	ADP
cet-15688	68	36	these	these	DET
cet-15688	68	37	pores	pore	NOUN
cet-15688	68	38	.	.	PUNCT
cet-15688	69	1	incorporation	incorporation	NOUN
cet-15688	69	2	of	of	ADP
cet-15688	69	3	a	a	DET
cet-15688	69	4	second	second	ADJ
cet-15688	69	5	metal	metal	NOUN
cet-15688	69	6	onto	onto	ADP
cet-15688	69	7	a	a	DET
cet-15688	69	8	silica	silica	NOUN
cet-15688	69	9	support	support	NOUN
cet-15688	69	10	results	result	NOUN
cet-15688	69	11	in	in	ADP
cet-15688	69	12	a	a	DET
cet-15688	69	13	drastic	drastic	ADJ
cet-15688	69	14	change	change	NOUN
cet-15688	69	15	in	in	ADP
cet-15688	69	16	the	the	DET
cet-15688	69	17	distribution	distribution	NOUN
cet-15688	69	18	of	of	ADP
cet-15688	69	19	pore	pore	ADJ
cet-15688	69	20	volumes	volume	NOUN
cet-15688	69	21	(	(	PUNCT
cet-15688	69	22	figure	figure	NOUN
cet-15688	69	23	4b	4b	PROPN
cet-15688	69	24	)	)	PUNCT
cet-15688	69	25	.	.	PUNCT
cet-15688	70	1	in	in	ADP
cet-15688	70	2	the	the	DET
cet-15688	70	3	case	case	NOUN
cet-15688	70	4	of	of	ADP
cet-15688	70	5	the	the	DET
cet-15688	70	6	ni	ni	PROPN
cet-15688	70	7	-	-	PROPN
cet-15688	70	8	cu	cu	PROPN
cet-15688	70	9	sample	sample	NOUN
cet-15688	70	10	,	,	PUNCT
cet-15688	70	11	there	there	PRON
cet-15688	70	12	is	be	VERB
cet-15688	70	13	a	a	DET
cet-15688	70	14	decrease	decrease	NOUN
cet-15688	70	15	in	in	ADP
cet-15688	70	16	pore	pore	ADJ
cet-15688	70	17	volumes	volume	NOUN
cet-15688	70	18	in	in	ADP
cet-15688	70	19	the	the	DET
cet-15688	70	20	3	3	NUM
cet-15688	70	21	-	-	SYM
cet-15688	70	22	7	7	NUM
cet-15688	70	23	nm	nm	NOUN
cet-15688	70	24	range	range	NOUN
cet-15688	70	25	and	and	CCONJ
cet-15688	70	26	the	the	DET
cet-15688	70	27	appearance	appearance	NOUN
cet-15688	70	28	of	of	ADP
cet-15688	70	29	additional	additional	ADJ
cet-15688	70	30	pore	pore	ADJ
cet-15688	70	31	volumes	volume	NOUN
cet-15688	70	32	in	in	ADP
cet-15688	70	33	the	the	DET
cet-15688	70	34	range	range	NOUN
cet-15688	70	35	of	of	ADP
cet-15688	70	36	7	7	NUM
cet-15688	70	37	-	-	SYM
cet-15688	70	38	15	15	NUM
cet-15688	70	39	nm	nm	NOUN
cet-15688	70	40	,	,	PUNCT
cet-15688	70	41	which	which	PRON
cet-15688	70	42	can	can	AUX
cet-15688	70	43	be	be	AUX
cet-15688	70	44	explained	explain	VERB
cet-15688	70	45	by	by	ADP
cet-15688	70	46	the	the	DET
cet-15688	70	47	partial	partial	ADJ
cet-15688	70	48	formation	formation	NOUN
cet-15688	70	49	of	of	ADP
cet-15688	70	50	ni	ni	PROPN
cet-15688	70	51	-	-	PROPN
cet-15688	70	52	cu	cu	PROPN
cet-15688	70	53	species	specie	NOUN
cet-15688	70	54	in	in	ADP
cet-15688	70	55	the	the	DET
cet-15688	70	56	pores	pore	NOUN
cet-15688	70	57	of	of	ADP
cet-15688	70	58	3	3	NUM
cet-15688	70	59	-	-	SYM
cet-15688	70	60	7	7	NUM
cet-15688	70	61	nm	nm	NOUN
cet-15688	70	62	in	in	ADP
cet-15688	70	63	diameter	diameter	NOUN
cet-15688	70	64	and	and	CCONJ
cet-15688	70	65	on	on	ADP
cet-15688	70	66	the	the	DET
cet-15688	70	67	external	external	ADJ
cet-15688	70	68	surface	surface	NOUN
cet-15688	70	69	of	of	ADP
cet-15688	70	70	silica	silica	NOUN
cet-15688	70	71	.	.	PUNCT
cet-15688	71	1	for	for	ADP
cet-15688	71	2	the	the	DET
cet-15688	71	3	cuni	cuni	ADJ
cet-15688	71	4	species	specie	NOUN
cet-15688	71	5	,	,	PUNCT
cet-15688	71	6	there	there	PRON
cet-15688	71	7	is	be	VERB
cet-15688	71	8	some	some	DET
cet-15688	71	9	shift	shift	NOUN
cet-15688	71	10	in	in	ADP
cet-15688	71	11	pore	pore	ADJ
cet-15688	71	12	volumes	volume	NOUN
cet-15688	71	13	from	from	ADP
cet-15688	71	14	the	the	DET
cet-15688	71	15	4	4	NUM
cet-15688	71	16	-	-	SYM
cet-15688	71	17	5	5	NUM
cet-15688	71	18	nm	nm	NOUN
cet-15688	71	19	range	range	NOUN
cet-15688	71	20	to	to	ADP
cet-15688	71	21	the	the	DET
cet-15688	71	22	7	7	NUM
cet-15688	71	23	-	-	SYM
cet-15688	71	24	8	8	NUM
cet-15688	71	25	nm	nm	NOUN
cet-15688	71	26	region	region	NOUN
cet-15688	71	27	,	,	PUNCT
cet-15688	71	28	which	which	PRON
cet-15688	71	29	can	can	AUX
cet-15688	71	30	also	also	ADV
cet-15688	71	31	be	be	AUX
cet-15688	71	32	explained	explain	VERB
cet-15688	71	33	by	by	ADP
cet-15688	71	34	cu	cu	PROPN
cet-15688	71	35	-	-	PUNCT
cet-15688	71	36	ni	ni	PROPN
cet-15688	71	37	species	species	NOUN
cet-15688	71	38	formation	formation	NOUN
cet-15688	71	39	in	in	ADP
cet-15688	71	40	the	the	DET
cet-15688	71	41	pores	pore	NOUN
cet-15688	71	42	of	of	ADP
cet-15688	71	43	4	4	NUM
cet-15688	71	44	-	-	SYM
cet-15688	71	45	5	5	NUM
cet-15688	71	46	nm	nm	NOUN
cet-15688	71	47	in	in	ADP
cet-15688	71	48	diameter	diameter	NOUN
cet-15688	71	49	.	.	PUNCT
cet-15688	72	1	in	in	ADP
cet-15688	72	2	the	the	DET
cet-15688	72	3	presence	presence	NOUN
cet-15688	72	4	of	of	ADP
cet-15688	72	5	pt	pt	PROPN
cet-15688	72	6	-	-	PUNCT
cet-15688	72	7	cu	cu	NOUN
cet-15688	72	8	species	specie	NOUN
cet-15688	72	9	,	,	PUNCT
cet-15688	72	10	there	there	PRON
cet-15688	72	11	is	be	VERB
cet-15688	72	12	an	an	DET
cet-15688	72	13	even	even	ADV
cet-15688	72	14	more	more	ADV
cet-15688	72	15	drastic	drastic	ADJ
cet-15688	72	16	reduction	reduction	NOUN
cet-15688	72	17	in	in	ADP
cet-15688	72	18	the	the	DET
cet-15688	72	19	pore	pore	ADJ
cet-15688	72	20	volumes	volume	NOUN
cet-15688	72	21	between	between	ADP
cet-15688	72	22	3	3	NUM
cet-15688	72	23	and	and	CCONJ
cet-15688	72	24	9	9	NUM
cet-15688	72	25	nm	nm	NOUN
cet-15688	72	26	,	,	PUNCT
cet-15688	72	27	as	as	ADV
cet-15688	72	28	well	well	ADV
cet-15688	72	29	as	as	ADP
cet-15688	72	30	the	the	DET
cet-15688	72	31	addition	addition	NOUN
cet-15688	72	32	of	of	ADP
cet-15688	72	33	new	new	ADJ
cet-15688	72	34	mesopores	mesopore	NOUN
cet-15688	72	35	in	in	ADP
cet-15688	72	36	the	the	DET
cet-15688	72	37	10	10	NUM
cet-15688	72	38	-	-	SYM
cet-15688	72	39	20	20	NUM
cet-15688	72	40	nm	nm	NOUN
cet-15688	72	41	region	region	NOUN
cet-15688	72	42	.	.	PUNCT
cet-15688	73	1	this	this	PRON
cet-15688	73	2	can	can	AUX
cet-15688	73	3	be	be	AUX
cet-15688	73	4	attributed	attribute	VERB
cet-15688	73	5	to	to	ADP
cet-15688	73	6	pt	pt	PROPN
cet-15688	73	7	-	-	PUNCT
cet-15688	73	8	cu	cu	NOUN
cet-15688	73	9	species	specie	NOUN
cet-15688	73	10	formation	formation	NOUN
cet-15688	73	11	in	in	ADP
cet-15688	73	12	small	small	ADJ
cet-15688	73	13	pores	pore	NOUN
cet-15688	73	14	of	of	ADP
cet-15688	73	15	silica	silica	NOUN
cet-15688	73	16	with	with	ADP
cet-15688	73	17	a	a	DET
cet-15688	73	18	diameter	diameter	NOUN
cet-15688	73	19	of	of	ADP
cet-15688	73	20	3	3	NUM
cet-15688	73	21	-	-	SYM
cet-15688	73	22	9	9	NUM
cet-15688	73	23	nm	nm	NOUN
cet-15688	73	24	and	and	CCONJ
cet-15688	73	25	over	over	ADP
cet-15688	73	26	the	the	DET
cet-15688	73	27	silica	silica	NOUN
cet-15688	73	28	surface	surface	NOUN
cet-15688	73	29	,	,	PUNCT
cet-15688	73	30	forming	form	VERB
cet-15688	73	31	additional	additional	ADJ
cet-15688	73	32	pores	pore	NOUN
cet-15688	73	33	in	in	ADP
cet-15688	73	34	the	the	DET
cet-15688	73	35	10	10	NUM
cet-15688	73	36	-	-	SYM
cet-15688	73	37	20	20	NUM
cet-15688	73	38	nm	nm	NOUN
cet-15688	73	39	region	region	NOUN
cet-15688	73	40	.	.	PUNCT
cet-15688	74	1	figure	figure	VERB
cet-15688	74	2	4	4	NUM
cet-15688	74	3	:	:	PUNCT
cet-15688	74	4	pore	pore	VERB
cet-15688	74	5	volume	volume	NOUN
cet-15688	74	6	distribution	distribution	NOUN
cet-15688	74	7	for	for	ADP
cet-15688	74	8	a	a	DET
cet-15688	74	9	)	)	PUNCT
cet-15688	74	10	monometallic	monometallic	NOUN
cet-15688	74	11	and	and	CCONJ
cet-15688	74	12	b	b	NOUN
cet-15688	74	13	)	)	PUNCT
cet-15688	74	14	bimetallic	bimetallic	NOUN
cet-15688	74	15	samples	sample	NOUN
cet-15688	74	16	bet	bet	VERB
cet-15688	74	17	surface	surface	NOUN
cet-15688	74	18	area	area	NOUN
cet-15688	74	19	values	value	NOUN
cet-15688	74	20	for	for	ADP
cet-15688	74	21	monometallic	monometallic	ADJ
cet-15688	74	22	samples	sample	NOUN
cet-15688	74	23	(	(	PUNCT
cet-15688	74	24	table	table	NOUN
cet-15688	74	25	1	1	NUM
cet-15688	74	26	)	)	PUNCT
cet-15688	74	27	are	be	AUX
cet-15688	74	28	slightly	slightly	ADV
cet-15688	74	29	lower	low	ADJ
cet-15688	74	30	compared	compare	VERB
cet-15688	74	31	to	to	ADP
cet-15688	74	32	pure	pure	ADJ
cet-15688	74	33	silica	silica	NOUN
cet-15688	74	34	,	,	PUNCT
cet-15688	74	35	with	with	ADP
cet-15688	74	36	the	the	DET
cet-15688	74	37	lowest	low	ADJ
cet-15688	74	38	value	value	NOUN
cet-15688	74	39	being	be	AUX
cet-15688	74	40	332	332	NUM
cet-15688	74	41	m²/g	m²/g	NOUN
cet-15688	74	42	for	for	ADP
cet-15688	74	43	a	a	DET
cet-15688	74	44	platinum	platinum	NOUN
cet-15688	74	45	monometallic	monometallic	NOUN
cet-15688	74	46	sample	sample	NOUN
cet-15688	74	47	.	.	PUNCT
cet-15688	75	1	the	the	DET
cet-15688	75	2	addition	addition	NOUN
cet-15688	75	3	of	of	ADP
cet-15688	75	4	a	a	DET
cet-15688	75	5	second	second	ADJ
cet-15688	75	6	metal	metal	NOUN
cet-15688	75	7	leads	lead	VERB
cet-15688	75	8	to	to	ADP
cet-15688	75	9	a	a	DET
cet-15688	75	10	further	further	ADJ
cet-15688	75	11	decrease	decrease	NOUN
cet-15688	75	12	in	in	ADP
cet-15688	75	13	bet	bet	PROPN
cet-15688	75	14	surface	surface	NOUN
cet-15688	75	15	area	area	NOUN
cet-15688	75	16	compared	compare	VERB
cet-15688	75	17	to	to	ADP
cet-15688	75	18	monometallic	monometallic	ADJ
cet-15688	75	19	ones	one	NOUN
cet-15688	75	20	.	.	PUNCT
cet-15688	76	1	a	a	DET
cet-15688	76	2	bimetallic	bimetallic	ADJ
cet-15688	76	3	platinum	platinum	NOUN
cet-15688	76	4	-	-	PUNCT
cet-15688	76	5	copper	copper	NOUN
cet-15688	76	6	sample	sample	NOUN
cet-15688	76	7	has	have	VERB
cet-15688	76	8	the	the	DET
cet-15688	76	9	lowest	low	ADJ
cet-15688	76	10	bet	bet	NOUN
cet-15688	76	11	area	area	NOUN
cet-15688	76	12	of	of	ADP
cet-15688	76	13	173	173	NUM
cet-15688	76	14	m²/g	m²/g	NOUN
cet-15688	76	15	,	,	PUNCT
cet-15688	76	16	which	which	PRON
cet-15688	76	17	can	can	AUX
cet-15688	76	18	be	be	AUX
cet-15688	76	19	attributed	attribute	VERB
cet-15688	76	20	to	to	ADP
cet-15688	76	21	the	the	DET
cet-15688	76	22	formation	formation	NOUN
cet-15688	76	23	of	of	ADP
cet-15688	76	24	platinum	platinum	NOUN
cet-15688	76	25	and	and	CCONJ
cet-15688	76	26	copper	copper	NOUN
cet-15688	76	27	species	specie	NOUN
cet-15688	76	28	in	in	ADP
cet-15688	76	29	the	the	DET
cet-15688	76	30	mesopores	mesopore	NOUN
cet-15688	76	31	,	,	PUNCT
cet-15688	76	32	resulting	result	VERB
cet-15688	76	33	in	in	ADP
cet-15688	76	34	a	a	DET
cet-15688	76	35	decrease	decrease	NOUN
cet-15688	76	36	in	in	ADP
cet-15688	76	37	catalyst	catalyst	NOUN
cet-15688	76	38	surface	surface	NOUN
cet-15688	76	39	area	area	NOUN
cet-15688	76	40	.	.	PUNCT
cet-15688	77	1	the	the	DET
cet-15688	77	2	active	active	ADJ
cet-15688	77	3	metal	metal	NOUN
cet-15688	77	4	concentration	concentration	NOUN
cet-15688	77	5	(	(	PUNCT
cet-15688	77	6	see	see	VERB
cet-15688	77	7	table	table	NOUN
cet-15688	77	8	1	1	NUM
cet-15688	77	9	)	)	PUNCT
cet-15688	77	10	ranges	range	VERB
cet-15688	77	11	from	from	ADP
cet-15688	77	12	0.72	0.72	NUM
cet-15688	77	13	to	to	ADP
cet-15688	77	14	0.98	0.98	NUM
cet-15688	77	15	wt	wt	NOUN
cet-15688	77	16	.	.	NOUN
cet-15688	78	1	%	%	INTJ
cet-15688	78	2	.	.	PUNCT
cet-15688	79	1	table	table	NOUN
cet-15688	79	2	1	1	NUM
cet-15688	79	3	:	:	PUNCT
cet-15688	79	4	initial	initial	ADJ
cet-15688	79	5	catalysts	catalyst	NOUN
cet-15688	79	6	characteristics	characteristics	PROPN
cet-15688	79	7	sample	sample	NOUN
cet-15688	79	8	bet	bet	PROPN
cet-15688	79	9	*	*	PROPN
cet-15688	79	10	surface	surface	NOUN
cet-15688	79	11	area	area	NOUN
cet-15688	79	12	,	,	PUNCT
cet-15688	79	13	m2	m2	PROPN
cet-15688	79	14	/	/	SYM
cet-15688	79	15	g	g	PROPN
cet-15688	79	16	metal	metal	NOUN
cet-15688	79	17	concentration	concentration	NOUN
cet-15688	79	18	*	*	PUNCT
cet-15688	79	19	*	*	NOUN
cet-15688	79	20	,	,	PUNCT
cet-15688	79	21	wt	wt	PROPN
cet-15688	79	22	.	.	PUNCT
cet-15688	79	23	%	%	PROPN
cet-15688	79	24	sio2	sio2	PROPN
cet-15688	79	25	360	360	NUM
cet-15688	79	26	cu	cu	PROPN
cet-15688	79	27	-	-	PUNCT
cet-15688	79	28	sio2	sio2	PROPN
cet-15688	79	29	349	349	NUM
cet-15688	79	30	0.72	0.72	NUM
cet-15688	79	31	ni	ni	PROPN
cet-15688	79	32	-	-	PROPN
cet-15688	79	33	sio2	sio2	PROPN
cet-15688	79	34	349	349	NUM
cet-15688	79	35	0.93	0.93	NUM
cet-15688	79	36	pt	pt	PROPN
cet-15688	79	37	-	-	PUNCT
cet-15688	79	38	sio2	sio2	PROPN
cet-15688	79	39	332	332	NUM
cet-15688	79	40	0.95	0.95	NUM
cet-15688	79	41	ni	ni	PROPN
cet-15688	79	42	-	-	PROPN
cet-15688	79	43	cu	cu	PROPN
cet-15688	79	44	-	-	PUNCT
cet-15688	79	45	sio2	sio2	PROPN
cet-15688	79	46	319	319	NUM
cet-15688	79	47	ni-0.83	ni-0.83	PROPN
cet-15688	79	48	cu-0.78	cu-0.78	PROPN
cet-15688	79	49	cu	cu	PROPN
cet-15688	79	50	-	-	PUNCT
cet-15688	79	51	ni	ni	PROPN
cet-15688	79	52	-	-	PUNCT
cet-15688	79	53	sio2	sio2	ADJ
cet-15688	79	54	314	314	NUM
cet-15688	79	55	cu-0.87	cu-0.87	VERB
cet-15688	79	56	ni-0.92	ni-0.92	PROPN
cet-15688	79	57	pt	pt	PROPN
cet-15688	79	58	-	-	PUNCT
cet-15688	79	59	cu	cu	NOUN
cet-15688	79	60	-	-	PUNCT
cet-15688	79	61	sio2	sio2	PROPN
cet-15688	79	62	173	173	NUM
cet-15688	79	63	pt-0.97	pt-0.97	NOUN
cet-15688	79	64	cu-0.98	cu-0.98	PROPN
cet-15688	79	65	*	*	PUNCT
cet-15688	79	66	determined	determine	VERB
cet-15688	79	67	by	by	ADP
cet-15688	79	68	the	the	DET
cet-15688	79	69	liquid	liquid	ADJ
cet-15688	79	70	nitrogen	nitrogen	NOUN
cet-15688	79	71	physisorption	physisorption	NOUN
cet-15688	79	72	,	,	PUNCT
cet-15688	79	73	*	*	PUNCT
cet-15688	79	74	*	*	PUNCT
cet-15688	79	75	determined	determine	VERB
cet-15688	79	76	using	use	VERB
cet-15688	79	77	x	x	PROPN
cet-15688	79	78	-	-	NOUN
cet-15688	79	79	ray	ray	NOUN
cet-15688	79	80	fluorescence	fluorescence	NOUN
cet-15688	79	81	analysis	analysis	NOUN
cet-15688	79	82	.	.	PUNCT
cet-15688	80	1	hydrogen	hydrogen	NOUN
cet-15688	80	2	programmed	program	VERB
cet-15688	80	3	desorption	desorption	NOUN
cet-15688	80	4	from	from	ADP
cet-15688	80	5	the	the	DET
cet-15688	80	6	silica	silica	NOUN
cet-15688	80	7	surface	surface	NOUN
cet-15688	80	8	(	(	PUNCT
cet-15688	80	9	figure	figure	NOUN
cet-15688	80	10	5a	5a	NUM
cet-15688	80	11	)	)	PUNCT
cet-15688	80	12	and	and	CCONJ
cet-15688	80	13	monometallic	monometallic	PROPN
cet-15688	80	14	catalyst	catalyst	NOUN
cet-15688	80	15	shows	show	VERB
cet-15688	80	16	desorption	desorption	NOUN
cet-15688	80	17	of	of	ADP
cet-15688	80	18	hydrogen	hydrogen	NOUN
cet-15688	80	19	at	at	ADP
cet-15688	80	20	one	one	NUM
cet-15688	80	21	type	type	NOUN
cet-15688	80	22	of	of	ADP
cet-15688	80	23	active	active	ADJ
cet-15688	80	24	site	site	NOUN
cet-15688	80	25	with	with	ADP
cet-15688	80	26	weak	weak	ADJ
cet-15688	80	27	strength	strength	NOUN
cet-15688	80	28	at	at	ADP
cet-15688	80	29	a	a	DET
cet-15688	80	30	temperature	temperature	NOUN
cet-15688	80	31	range	range	NOUN
cet-15688	80	32	of	of	ADP
cet-15688	80	33	160–180	160–180	NUM
cet-15688	80	34	°	°	PROPN
cet-15688	80	35	c	c	PROPN
cet-15688	80	36	.	.	PUNCT
cet-15688	81	1	bimetallic	bimetallic	NOUN
cet-15688	81	2	samples	sample	NOUN
cet-15688	81	3	(	(	PUNCT
cet-15688	81	4	figure	figure	NOUN
cet-15688	81	5	5b	5b	NUM
cet-15688	81	6	)	)	PUNCT
cet-15688	81	7	of	of	ADP
cet-15688	81	8	ni	ni	PROPN
cet-15688	81	9	-	-	PROPN
cet-15688	81	10	cu	cu	PROPN
cet-15688	81	11	and	and	CCONJ
cet-15688	81	12	cu	cu	PROPN
cet-15688	81	13	-	-	PROPN
cet-15688	81	14	ni	ni	PROPN
cet-15688	81	15	show	show	VERB
cet-15688	81	16	additional	additional	ADJ
cet-15688	81	17	lines	line	NOUN
cet-15688	81	18	at	at	ADP
cet-15688	81	19	temperatures	temperature	NOUN
cet-15688	81	20	of	of	ADP
cet-15688	81	21	290	290	NUM
cet-15688	81	22	°	°	NOUN
cet-15688	81	23	c	c	NOUN
cet-15688	81	24	and	and	CCONJ
cet-15688	81	25	340	340	NUM
cet-15688	81	26	°	°	NOUN
cet-15688	81	27	c	c	NOUN
cet-15688	81	28	,	,	PUNCT
cet-15688	81	29	while	while	SCONJ
cet-15688	81	30	the	the	DET
cet-15688	81	31	pt	pt	PROPN
cet-15688	81	32	-	-	PUNCT
cet-15688	81	33	cu	cu	NOUN
cet-15688	81	34	sample	sample	NOUN
cet-15688	81	35	shows	show	VERB
cet-15688	81	36	a	a	DET
cet-15688	81	37	small	small	ADJ
cet-15688	81	38	peak	peak	NOUN
cet-15688	81	39	at	at	ADP
cet-15688	81	40	280	280	NUM
cet-15688	81	41	°	°	NOUN
cet-15688	81	42	c	c	NOUN
cet-15688	81	43	.	.	PUNCT
cet-15688	82	1	the	the	DET
cet-15688	82	2	desorption	desorption	NOUN
cet-15688	82	3	of	of	ADP
cet-15688	82	4	carbon	carbon	NOUN
cet-15688	82	5	dioxide	dioxide	NOUN
cet-15688	82	6	from	from	ADP
cet-15688	82	7	the	the	DET
cet-15688	82	8	surface	surface	NOUN
cet-15688	82	9	of	of	ADP
cet-15688	82	10	silica	silica	NOUN
cet-15688	82	11	and	and	CCONJ
cet-15688	82	12	monometallic	monometallic	NOUN
cet-15688	82	13	samples	sample	NOUN
cet-15688	82	14	forms	form	VERB
cet-15688	82	15	a	a	DET
cet-15688	82	16	line	line	NOUN
cet-15688	82	17	in	in	ADP
cet-15688	82	18	the	the	DET
cet-15688	82	19	160–190	160–190	NUM
cet-15688	82	20	°	°	NOUN
cet-15688	82	21	c	c	NOUN
cet-15688	82	22	region	region	NOUN
cet-15688	82	23	(	(	PUNCT
cet-15688	82	24	figure	figure	NOUN
cet-15688	82	25	5c	5c	NUM
cet-15688	82	26	)	)	PUNCT
cet-15688	82	27	.	.	PUNCT
cet-15688	83	1	the	the	DET
cet-15688	83	2	copper	copper	NOUN
cet-15688	83	3	sample	sample	NOUN
cet-15688	83	4	additionally	additionally	ADV
cet-15688	83	5	has	have	VERB
cet-15688	83	6	a	a	DET
cet-15688	83	7	small	small	ADJ
cet-15688	83	8	reflection	reflection	NOUN
cet-15688	83	9	in	in	ADP
cet-15688	83	10	the	the	DET
cet-15688	83	11	340	340	NUM
cet-15688	83	12	°	°	PROPN
cet-15688	83	13	c	c	NOUN
cet-15688	83	14	region	region	NOUN
cet-15688	83	15	.	.	PUNCT
cet-15688	84	1	the	the	DET
cet-15688	84	2	desorption	desorption	NOUN
cet-15688	84	3	of	of	ADP
cet-15688	84	4	carbon	carbon	NOUN
cet-15688	84	5	dioxide	dioxide	NOUN
cet-15688	84	6	from	from	ADP
cet-15688	84	7	the	the	DET
cet-15688	84	8	bimetallic	bimetallic	NOUN
cet-15688	84	9	samples	sample	NOUN
cet-15688	84	10	proceeded	proceed	VERB
cet-15688	84	11	from	from	ADP
cet-15688	84	12	the	the	DET
cet-15688	84	13	sites	site	NOUN
cet-15688	84	14	in	in	ADP
cet-15688	84	15	the	the	DET
cet-15688	84	16	160–190	160–190	NUM
cet-15688	84	17	°	°	NOUN
cet-15688	84	18	c	c	NOUN
cet-15688	84	19	range	range	NOUN
cet-15688	84	20	(	(	PUNCT
cet-15688	84	21	figure	figure	NOUN
cet-15688	84	22	5d	5d	NUM
cet-15688	84	23	)	)	PUNCT
cet-15688	84	24	.	.	PUNCT
cet-15688	85	1	additionally	additionally	ADV
cet-15688	85	2	,	,	PUNCT
cet-15688	85	3	copper	copper	NOUN
cet-15688	85	4	-	-	PUNCT
cet-15688	85	5	containing	contain	VERB
cet-15688	85	6	samples	sample	NOUN
cet-15688	85	7	0	0	NUM
cet-15688	85	8	0.02	0.02	NUM
cet-15688	85	9	0.04	0.04	NUM
cet-15688	85	10	0.06	0.06	NUM
cet-15688	85	11	0.08	0.08	NUM
cet-15688	85	12	0.1	0.1	NUM
cet-15688	85	13	0.12	0.12	NUM
cet-15688	85	14	0.14	0.14	NUM
cet-15688	85	15	0.16	0.16	NUM
cet-15688	85	16	0.18	0.18	NUM
cet-15688	85	17	0.2	0.2	NUM
cet-15688	85	18	0	0	NUM
cet-15688	85	19	5	5	NUM
cet-15688	85	20	10	10	NUM
cet-15688	85	21	15	15	NUM
cet-15688	85	22	20	20	NUM
cet-15688	85	23	d	d	NOUN
cet-15688	85	24	(	(	PUNCT
cet-15688	85	25	v	v	ADP
cet-15688	85	26	p	p	NOUN
cet-15688	85	27	)	)	PUNCT
cet-15688	85	28	/	/	SYM
cet-15688	86	1	d	d	NOUN
cet-15688	86	2	(	(	PUNCT
cet-15688	86	3	d	d	X
cet-15688	86	4	p	p	NOUN
cet-15688	86	5	)	)	PUNCT
cet-15688	86	6	,	,	PUNCT
cet-15688	86	7	(	(	PUNCT
cet-15688	86	8	m	m	X
cet-15688	86	9	l/	l/	NOUN
cet-15688	86	10	g	g	PROPN
cet-15688	86	11	*	*	PROPN
cet-15688	86	12	n	n	PROPN
cet-15688	86	13	m	m	NOUN
cet-15688	86	14	)	)	PUNCT
cet-15688	86	15	pores	pore	VERB
cet-15688	86	16	average	average	ADJ
cet-15688	86	17	diameter	diameter	NOUN
cet-15688	86	18	,	,	PUNCT
cet-15688	86	19	nm	nm	PROPN
cet-15688	86	20	sio2	sio2	PROPN
cet-15688	86	21	cu	cu	PROPN
cet-15688	86	22	-	-	PUNCT
cet-15688	86	23	sio2	sio2	PROPN
cet-15688	86	24	ni	ni	PROPN
cet-15688	86	25	-	-	PUNCT
cet-15688	86	26	sio2	sio2	PROPN
cet-15688	86	27	pt	pt	PROPN
cet-15688	86	28	-	-	PUNCT
cet-15688	86	29	sio2	sio2	PROPN
cet-15688	86	30	a	a	PRON
cet-15688	86	31	)	)	PUNCT
cet-15688	86	32	0	0	NUM
cet-15688	86	33	0.02	0.02	NUM
cet-15688	86	34	0.04	0.04	NUM
cet-15688	86	35	0.06	0.06	NUM
cet-15688	86	36	0.08	0.08	NUM
cet-15688	86	37	0.1	0.1	NUM
cet-15688	86	38	0.12	0.12	NUM
cet-15688	86	39	0.14	0.14	NUM
cet-15688	86	40	0.16	0.16	NUM
cet-15688	86	41	0.18	0.18	NUM
cet-15688	86	42	0.2	0.2	NUM
cet-15688	86	43	0	0	NUM
cet-15688	86	44	5	5	NUM
cet-15688	86	45	10	10	NUM
cet-15688	86	46	15	15	NUM
cet-15688	86	47	20	20	NUM
cet-15688	86	48	d	d	NOUN
cet-15688	86	49	(	(	PUNCT
cet-15688	86	50	v	v	ADP
cet-15688	86	51	p	p	NOUN
cet-15688	86	52	)	)	PUNCT
cet-15688	86	53	/	/	SYM
cet-15688	87	1	d	d	NOUN
cet-15688	87	2	(	(	PUNCT
cet-15688	87	3	d	d	X
cet-15688	87	4	p	p	NOUN
cet-15688	87	5	)	)	PUNCT
cet-15688	87	6	,	,	PUNCT
cet-15688	87	7	(	(	PUNCT
cet-15688	87	8	m	m	X
cet-15688	87	9	l/	l/	NOUN
cet-15688	87	10	g	g	PROPN
cet-15688	87	11	*	*	PROPN
cet-15688	87	12	n	n	PROPN
cet-15688	87	13	m	m	NOUN
cet-15688	87	14	)	)	PUNCT
cet-15688	87	15	pores	pore	VERB
cet-15688	87	16	average	average	ADJ
cet-15688	87	17	diameter	diameter	NOUN
cet-15688	87	18	,	,	PUNCT
cet-15688	87	19	nm	nm	PROPN
cet-15688	87	20	sio2	sio2	PROPN
cet-15688	87	21	ni	ni	PROPN
cet-15688	87	22	-	-	PROPN
cet-15688	87	23	cu	cu	PROPN
cet-15688	87	24	-	-	PUNCT
cet-15688	87	25	sio2	sio2	PROPN
cet-15688	87	26	cu	cu	PROPN
cet-15688	87	27	-	-	PUNCT
cet-15688	87	28	ni	ni	PROPN
cet-15688	87	29	-	-	PUNCT
cet-15688	87	30	sio2	sio2	PROPN
cet-15688	87	31	pt	pt	PROPN
cet-15688	87	32	-	-	PUNCT
cet-15688	87	33	cu	cu	PROPN
cet-15688	87	34	-	-	PUNCT
cet-15688	87	35	sio2	sio2	PROPN
cet-15688	87	36	b	b	PROPN
cet-15688	87	37	)	)	PUNCT
cet-15688	87	38	376	376	NUM
cet-15688	87	39	have	have	VERB
cet-15688	87	40	a	a	DET
cet-15688	87	41	small	small	ADJ
cet-15688	87	42	reflection	reflection	NOUN
cet-15688	87	43	at	at	ADP
cet-15688	87	44	340	340	NUM
cet-15688	87	45	°	°	NOUN
cet-15688	87	46	c	c	NOUN
cet-15688	87	47	.	.	PUNCT
cet-15688	88	1	the	the	DET
cet-15688	88	2	presence	presence	NOUN
cet-15688	88	3	of	of	ADP
cet-15688	88	4	additional	additional	ADJ
cet-15688	88	5	desorption	desorption	NOUN
cet-15688	88	6	peaks	peak	NOUN
cet-15688	88	7	suggests	suggest	VERB
cet-15688	88	8	the	the	DET
cet-15688	88	9	presence	presence	NOUN
cet-15688	88	10	of	of	ADP
cet-15688	88	11	additional	additional	ADJ
cet-15688	88	12	active	active	ADJ
cet-15688	88	13	sites	site	NOUN
cet-15688	88	14	for	for	ADP
cet-15688	88	15	carbon	carbon	NOUN
cet-15688	88	16	dioxide	dioxide	NOUN
cet-15688	88	17	.	.	PUNCT
cet-15688	89	1	pure	pure	ADJ
cet-15688	89	2	silica	silica	NOUN
cet-15688	89	3	is	be	AUX
cet-15688	89	4	characterized	characterize	VERB
cet-15688	89	5	by	by	ADP
cet-15688	89	6	the	the	DET
cet-15688	89	7	highest	high	ADJ
cet-15688	89	8	value	value	NOUN
cet-15688	89	9	of	of	ADP
cet-15688	89	10	hydrogen	hydrogen	NOUN
cet-15688	89	11	desorbing	desorbing	NOUN
cet-15688	89	12	from	from	ADP
cet-15688	89	13	its	its	PRON
cet-15688	89	14	surface	surface	NOUN
cet-15688	89	15	,	,	PUNCT
cet-15688	89	16	0.004	0.004	NUM
cet-15688	89	17	mmol	mmol	NOUN
cet-15688	89	18	/	/	SYM
cet-15688	89	19	g	g	NOUN
cet-15688	89	20	(	(	PUNCT
cet-15688	89	21	table	table	NOUN
cet-15688	89	22	2	2	NUM
cet-15688	89	23	)	)	PUNCT
cet-15688	89	24	.	.	PUNCT
cet-15688	90	1	comparable	comparable	ADJ
cet-15688	90	2	values	value	NOUN
cet-15688	90	3	of	of	ADP
cet-15688	90	4	desorbing	desorb	VERB
cet-15688	90	5	hydrogen	hydrogen	NOUN
cet-15688	90	6	were	be	AUX
cet-15688	90	7	achieved	achieve	VERB
cet-15688	90	8	with	with	ADP
cet-15688	90	9	a	a	DET
cet-15688	90	10	pt	pt	NOUN
cet-15688	90	11	monometallic	monometallic	NOUN
cet-15688	90	12	and	and	CCONJ
cet-15688	90	13	cu	cu	PROPN
cet-15688	90	14	-	-	PUNCT
cet-15688	90	15	ni	ni	PROPN
cet-15688	90	16	bimetallic	bimetallic	NOUN
cet-15688	90	17	samples	sample	NOUN
cet-15688	90	18	.	.	PUNCT
cet-15688	91	1	the	the	DET
cet-15688	91	2	copper	copper	NOUN
cet-15688	91	3	-	-	PUNCT
cet-15688	91	4	containing	contain	VERB
cet-15688	91	5	monometallic	monometallic	NOUN
cet-15688	91	6	sample	sample	NOUN
cet-15688	91	7	has	have	VERB
cet-15688	91	8	the	the	DET
cet-15688	91	9	highest	high	ADJ
cet-15688	91	10	value	value	NOUN
cet-15688	91	11	of	of	ADP
cet-15688	91	12	desorbed	desorbed	ADJ
cet-15688	91	13	hydrogen	hydrogen	NOUN
cet-15688	91	14	from	from	ADP
cet-15688	91	15	its	its	PRON
cet-15688	91	16	surface	surface	NOUN
cet-15688	91	17	,	,	PUNCT
cet-15688	91	18	0.03	0.03	NUM
cet-15688	91	19	mmol	mmol	NOUN
cet-15688	91	20	/	/	SYM
cet-15688	91	21	g	g	NOUN
cet-15688	91	22	(	(	PUNCT
cet-15688	91	23	see	see	VERB
cet-15688	91	24	table	table	NOUN
cet-15688	91	25	2	2	NUM
cet-15688	91	26	)	)	PUNCT
cet-15688	91	27	.	.	PUNCT
cet-15688	92	1	desorption	desorption	NOUN
cet-15688	92	2	sites	site	NOUN
cet-15688	92	3	are	be	AUX
cet-15688	92	4	located	locate	VERB
cet-15688	92	5	in	in	ADP
cet-15688	92	6	the	the	DET
cet-15688	92	7	170–190	170–190	NUM
cet-15688	92	8	°	°	PROPN
cet-15688	92	9	c	c	NOUN
cet-15688	92	10	region	region	NOUN
cet-15688	92	11	for	for	ADP
cet-15688	92	12	all	all	DET
cet-15688	92	13	samples	sample	NOUN
cet-15688	92	14	,	,	PUNCT
cet-15688	92	15	which	which	PRON
cet-15688	92	16	suggests	suggest	VERB
cet-15688	92	17	competitive	competitive	ADJ
cet-15688	92	18	adsorption	adsorption	NOUN
cet-15688	92	19	of	of	ADP
cet-15688	92	20	both	both	DET
cet-15688	92	21	hydrogen	hydrogen	NOUN
cet-15688	92	22	and	and	CCONJ
cet-15688	92	23	carbon	carbon	NOUN
cet-15688	92	24	dioxide	dioxide	NOUN
cet-15688	92	25	.	.	PUNCT
cet-15688	93	1	the	the	DET
cet-15688	93	2	quantity	quantity	NOUN
cet-15688	93	3	of	of	ADP
cet-15688	93	4	adsorbed	adsorb	VERB
cet-15688	93	5	co2	co2	NOUN
cet-15688	93	6	is	be	AUX
cet-15688	93	7	10–15	10–15	NUM
cet-15688	93	8	times	time	NOUN
cet-15688	93	9	higher	high	ADJ
cet-15688	93	10	than	than	ADP
cet-15688	93	11	that	that	PRON
cet-15688	93	12	for	for	ADP
cet-15688	93	13	hydrogen	hydrogen	NOUN
cet-15688	93	14	,	,	PUNCT
cet-15688	93	15	resulting	result	VERB
cet-15688	93	16	in	in	ADP
cet-15688	93	17	a	a	DET
cet-15688	93	18	higher	high	ADJ
cet-15688	93	19	adsorption	adsorption	NOUN
cet-15688	93	20	of	of	ADP
cet-15688	93	21	co2	co2	NOUN
cet-15688	93	22	over	over	ADP
cet-15688	93	23	the	the	DET
cet-15688	93	24	sample	sample	NOUN
cet-15688	93	25	surface	surface	NOUN
cet-15688	93	26	compared	compare	VERB
cet-15688	93	27	to	to	ADP
cet-15688	93	28	hydrogen	hydrogen	PROPN
cet-15688	93	29	.	.	PUNCT
cet-15688	94	1	figure	figure	NOUN
cet-15688	94	2	5	5	NUM
cet-15688	94	3	:	:	PUNCT
cet-15688	94	4	hydrogen	hydrogen	NOUN
cet-15688	94	5	a	a	NOUN
cet-15688	94	6	)	)	PUNCT
cet-15688	94	7	,	,	PUNCT
cet-15688	94	8	and	and	CCONJ
cet-15688	94	9	b	b	X
cet-15688	94	10	)	)	PUNCT
cet-15688	94	11	carbon	carbon	NOUN
cet-15688	94	12	dioxide	dioxide	NOUN
cet-15688	94	13	c	c	NOUN
cet-15688	94	14	)	)	PUNCT
cet-15688	94	15	,	,	PUNCT
cet-15688	94	16	d	d	X
cet-15688	94	17	)	)	PUNCT
cet-15688	94	18	temperature	temperature	NOUN
cet-15688	94	19	programmed	program	VERB
cet-15688	94	20	desorption	desorption	NOUN
cet-15688	94	21	curves	curve	NOUN
cet-15688	94	22	for	for	ADP
cet-15688	94	23	a	a	DET
cet-15688	94	24	)	)	PUNCT
cet-15688	94	25	monometallic	monometallic	NOUN
cet-15688	94	26	and	and	CCONJ
cet-15688	94	27	b	b	NOUN
cet-15688	94	28	)	)	PUNCT
cet-15688	94	29	bimetallic	bimetallic	NOUN
cet-15688	94	30	samples	sample	NOUN
cet-15688	94	31	for	for	ADP
cet-15688	94	32	c	c	NOUN
cet-15688	94	33	)	)	PUNCT
cet-15688	94	34	monometallic	monometallic	NOUN
cet-15688	94	35	and	and	CCONJ
cet-15688	94	36	d	d	NOUN
cet-15688	94	37	)	)	PUNCT
cet-15688	94	38	bimetallic	bimetallic	NOUN
cet-15688	94	39	samples	sample	VERB
cet-15688	94	40	the	the	DET
cet-15688	94	41	partial	partial	ADJ
cet-15688	94	42	pressure	pressure	NOUN
cet-15688	94	43	of	of	ADP
cet-15688	94	44	hydrogen	hydrogen	NOUN
cet-15688	94	45	becomes	become	VERB
cet-15688	94	46	a	a	DET
cet-15688	94	47	key	key	ADJ
cet-15688	94	48	reaction	reaction	NOUN
cet-15688	94	49	parameter	parameter	NOUN
cet-15688	94	50	in	in	ADP
cet-15688	94	51	achieving	achieve	VERB
cet-15688	94	52	high	high	ADJ
cet-15688	94	53	reaction	reaction	NOUN
cet-15688	94	54	rates	rate	NOUN
cet-15688	94	55	,	,	PUNCT
cet-15688	94	56	so	so	SCONJ
cet-15688	94	57	it	it	PRON
cet-15688	94	58	needs	need	VERB
cet-15688	94	59	to	to	PART
cet-15688	94	60	be	be	AUX
cet-15688	94	61	higher	high	ADJ
cet-15688	94	62	in	in	ADP
cet-15688	94	63	magnitude	magnitude	NOUN
cet-15688	94	64	than	than	ADP
cet-15688	94	65	the	the	DET
cet-15688	94	66	partial	partial	ADJ
cet-15688	94	67	pressure	pressure	NOUN
cet-15688	94	68	of	of	ADP
cet-15688	94	69	carbon	carbon	NOUN
cet-15688	94	70	dioxide	dioxide	NOUN
cet-15688	94	71	to	to	PART
cet-15688	94	72	provide	provide	VERB
cet-15688	94	73	a	a	DET
cet-15688	94	74	high	high	ADJ
cet-15688	94	75	rate	rate	NOUN
cet-15688	94	76	of	of	ADP
cet-15688	94	77	carbon	carbon	NOUN
cet-15688	94	78	dioxide	dioxide	NOUN
cet-15688	94	79	transformation	transformation	NOUN
cet-15688	94	80	.	.	PUNCT
cet-15688	95	1	table	table	NOUN
cet-15688	95	2	2	2	NUM
cet-15688	95	3	:	:	PUNCT
cet-15688	95	4	hydrogen	hydrogen	NOUN
cet-15688	95	5	and	and	CCONJ
cet-15688	95	6	carbon	carbon	NOUN
cet-15688	95	7	dioxide	dioxide	NOUN
cet-15688	95	8	adsorption	adsorption	NOUN
cet-15688	95	9	values	value	NOUN
cet-15688	95	10	for	for	ADP
cet-15688	95	11	synthesized	synthesize	VERB
cet-15688	95	12	catalysts	catalyst	NOUN
cet-15688	95	13	sample	sample	NOUN
cet-15688	95	14	h2	h2	PROPN
cet-15688	95	15	desorption	desorption	NOUN
cet-15688	95	16	,	,	PUNCT
cet-15688	95	17	mmol	mmol	NOUN
cet-15688	95	18	/	/	SYM
cet-15688	95	19	g	g	NOUN
cet-15688	95	20	co2	co2	NOUN
cet-15688	95	21	desorption	desorption	NOUN
cet-15688	95	22	,	,	PUNCT
cet-15688	95	23	mmol	mmol	NOUN
cet-15688	95	24	/	/	SYM
cet-15688	95	25	g	g	PROPN
cet-15688	95	26	sio2	sio2	NOUN
cet-15688	95	27	0.004	0.004	NUM
cet-15688	95	28	0.01	0.01	NUM
cet-15688	95	29	cu	cu	PROPN
cet-15688	95	30	-	-	PUNCT
cet-15688	95	31	sio2	sio2	PROPN
cet-15688	95	32	0.001	0.001	NUM
cet-15688	95	33	0.03	0.03	NUM
cet-15688	95	34	ni	ni	PROPN
cet-15688	95	35	-	-	PUNCT
cet-15688	95	36	sio2	sio2	PROPN
cet-15688	95	37	0.002	0.002	NUM
cet-15688	95	38	0.01	0.01	NUM
cet-15688	95	39	pt	pt	PROPN
cet-15688	95	40	-	-	PUNCT
cet-15688	95	41	sio2	sio2	NOUN
cet-15688	95	42	0.003	0.003	NUM
cet-15688	95	43	0.007	0.007	NUM
cet-15688	95	44	ni	ni	PROPN
cet-15688	95	45	-	-	PROPN
cet-15688	95	46	cu	cu	PROPN
cet-15688	95	47	-	-	PUNCT
cet-15688	95	48	sio2	sio2	PROPN
cet-15688	95	49	0.002	0.002	NUM
cet-15688	95	50	0.021	0.021	NUM
cet-15688	95	51	cu	cu	PROPN
cet-15688	95	52	-	-	PUNCT
cet-15688	95	53	ni	ni	PROPN
cet-15688	95	54	-	-	NOUN
cet-15688	95	55	sio2	sio2	NOUN
cet-15688	95	56	0.004	0.004	NUM
cet-15688	95	57	0.022	0.022	NUM
cet-15688	95	58	pt	pt	PROPN
cet-15688	95	59	-	-	PUNCT
cet-15688	95	60	cu	cu	NOUN
cet-15688	95	61	-	-	PUNCT
cet-15688	95	62	sio2	sio2	PROPN
cet-15688	95	63	0.002	0.002	NUM
cet-15688	95	64	0.007	0.007	NUM
cet-15688	95	65	the	the	DET
cet-15688	95	66	developed	develop	VERB
cet-15688	95	67	catalysts	catalyst	NOUN
cet-15688	95	68	'	'	PART
cet-15688	95	69	testing	testing	NOUN
cet-15688	95	70	results	result	NOUN
cet-15688	95	71	(	(	PUNCT
cet-15688	95	72	see	see	VERB
cet-15688	95	73	table	table	NOUN
cet-15688	95	74	3	3	NUM
cet-15688	95	75	)	)	PUNCT
cet-15688	95	76	show	show	VERB
cet-15688	95	77	that	that	SCONJ
cet-15688	95	78	pure	pure	ADJ
cet-15688	95	79	silica	silica	NOUN
cet-15688	95	80	is	be	AUX
cet-15688	95	81	nearly	nearly	ADV
cet-15688	95	82	inactive	inactive	ADJ
cet-15688	95	83	in	in	ADP
cet-15688	95	84	the	the	DET
cet-15688	95	85	carbon	carbon	NOUN
cet-15688	95	86	dioxide	dioxide	NOUN
cet-15688	95	87	to	to	ADP
cet-15688	95	88	formaldehyde	formaldehyde	NOUN
cet-15688	95	89	transformation	transformation	NOUN
cet-15688	95	90	process	process	NOUN
cet-15688	95	91	.	.	PUNCT
cet-15688	96	1	the	the	DET
cet-15688	96	2	copper	copper	NOUN
cet-15688	96	3	-	-	PUNCT
cet-15688	96	4	containing	contain	VERB
cet-15688	96	5	sample	sample	NOUN
cet-15688	96	6	shows	show	VERB
cet-15688	96	7	only	only	ADV
cet-15688	96	8	0.002	0.002	NUM
cet-15688	96	9	mmol(hcoh)/g(cat	mmol(hcoh)/g(cat	NUM
cet-15688	96	10	)	)	PUNCT
cet-15688	96	11	,	,	PUNCT
cet-15688	96	12	the	the	DET
cet-15688	96	13	nickel	nickel	NOUN
cet-15688	96	14	-	-	PUNCT
cet-15688	96	15	containing	contain	VERB
cet-15688	96	16	sample	sample	NOUN
cet-15688	96	17	shows	show	VERB
cet-15688	96	18	0.01	0.01	NUM
cet-15688	96	19	mmol(hcoh	mmol(hcoh	NUM
cet-15688	96	20	)	)	PUNCT
cet-15688	96	21	/g(cat	/g(cat	X
cet-15688	96	22	)	)	PUNCT
cet-15688	96	23	,	,	PUNCT
cet-15688	96	24	and	and	CCONJ
cet-15688	96	25	the	the	DET
cet-15688	96	26	platinum	platinum	NOUN
cet-15688	96	27	result	result	VERB
cet-15688	96	28	0	0	NUM
cet-15688	96	29	0.005	0.005	NUM
cet-15688	96	30	0.01	0.01	NUM
cet-15688	96	31	0.015	0.015	NUM
cet-15688	96	32	0.02	0.02	NUM
cet-15688	96	33	0.025	0.025	NUM
cet-15688	96	34	100	100	NUM
cet-15688	96	35	150	150	NUM
cet-15688	96	36	200	200	NUM
cet-15688	96	37	250	250	NUM
cet-15688	96	38	300	300	NUM
cet-15688	96	39	n	n	NUM
cet-15688	96	40	o	o	NOUN
cet-15688	96	41	rm	rm	NOUN
cet-15688	97	1	al	al	PROPN
cet-15688	98	1	iz	iz	INTJ
cet-15688	98	2	ed	ed	PROPN
cet-15688	98	3	a	a	DET
cet-15688	98	4	.u	.u	NOUN
cet-15688	98	5	.	.	PUNCT
cet-15688	99	1	temperature	temperature	NOUN
cet-15688	99	2	,	,	PUNCT
cet-15688	99	3	℃	℃	PROPN
cet-15688	99	4	sio2	sio2	PROPN
cet-15688	99	5	cu	cu	PROPN
cet-15688	99	6	-	-	PUNCT
cet-15688	99	7	sio2	sio2	PROPN
cet-15688	99	8	ni	ni	PROPN
cet-15688	99	9	-	-	PUNCT
cet-15688	99	10	sio2	sio2	PROPN
cet-15688	99	11	pt	pt	PROPN
cet-15688	99	12	-	-	PUNCT
cet-15688	99	13	sio2	sio2	NOUN
cet-15688	99	14	t=170	t=170	VERB
cet-15688	99	15	℃	℃	PROPN
cet-15688	99	16	a	a	PRON
cet-15688	99	17	)	)	PUNCT
cet-15688	99	18	0	0	NUM
cet-15688	99	19	0.005	0.005	NUM
cet-15688	99	20	0.01	0.01	NUM
cet-15688	99	21	0.015	0.015	NUM
cet-15688	99	22	0.02	0.02	NUM
cet-15688	99	23	0.025	0.025	NUM
cet-15688	99	24	100	100	NUM
cet-15688	99	25	200	200	NUM
cet-15688	99	26	300	300	NUM
cet-15688	99	27	400	400	NUM
cet-15688	99	28	n	n	NUM
cet-15688	99	29	o	o	NOUN
cet-15688	99	30	rm	rm	NOUN
cet-15688	100	1	al	al	PROPN
cet-15688	101	1	iz	iz	INTJ
cet-15688	101	2	ed	ed	PROPN
cet-15688	101	3	a	a	DET
cet-15688	101	4	.u	.u	NOUN
cet-15688	101	5	.	.	PUNCT
cet-15688	102	1	temperature	temperature	NOUN
cet-15688	102	2	,	,	PUNCT
cet-15688	102	3	℃	℃	PROPN
cet-15688	102	4	sio2	sio2	VERB
cet-15688	102	5	ni	ni	PROPN
cet-15688	102	6	-	-	PROPN
cet-15688	102	7	cu	cu	PROPN
cet-15688	102	8	-	-	PUNCT
cet-15688	102	9	sio2	sio2	PROPN
cet-15688	102	10	t=170	t=170	VERB
cet-15688	102	11	℃	℃	PROPN
cet-15688	102	12	t=290	t=290	NUM
cet-15688	102	13	℃	℃	PROPN
cet-15688	102	14	t=340	t=340	PROPN
cet-15688	102	15	℃	℃	PROPN
cet-15688	102	16	b	b	PROPN
cet-15688	102	17	)	)	PUNCT
cet-15688	102	18	0	0	NUM
cet-15688	103	1	0.01	0.01	NUM
cet-15688	103	2	0.02	0.02	NUM
cet-15688	103	3	0.03	0.03	NUM
cet-15688	103	4	0.04	0.04	NUM
cet-15688	103	5	0.05	0.05	NUM
cet-15688	103	6	0.06	0.06	NUM
cet-15688	103	7	0.07	0.07	NUM
cet-15688	103	8	0.08	0.08	NUM
cet-15688	103	9	100	100	NUM
cet-15688	103	10	200	200	NUM
cet-15688	103	11	300	300	NUM
cet-15688	103	12	400	400	NUM
cet-15688	103	13	n	n	NUM
cet-15688	103	14	o	o	NOUN
cet-15688	103	15	rm	rm	NOUN
cet-15688	103	16	al	al	PROPN
cet-15688	103	17	iz	iz	INTJ
cet-15688	103	18	ed	ed	PROPN
cet-15688	103	19	a	a	DET
cet-15688	103	20	.u	.u	NOUN
cet-15688	103	21	.	.	PUNCT
cet-15688	104	1	temperature	temperature	NOUN
cet-15688	104	2	,	,	PUNCT
cet-15688	104	3	℃	℃	PROPN
cet-15688	104	4	sio2	sio2	PROPN
cet-15688	104	5	cu	cu	PROPN
cet-15688	104	6	-	-	PUNCT
cet-15688	104	7	sio2	sio2	PROPN
cet-15688	104	8	ni	ni	PROPN
cet-15688	104	9	-	-	PUNCT
cet-15688	104	10	sio2	sio2	PROPN
cet-15688	104	11	pt	pt	PROPN
cet-15688	104	12	-	-	PUNCT
cet-15688	104	13	sio2	sio2	NOUN
cet-15688	104	14	t=180	t=180	NOUN
cet-15688	104	15	℃	℃	PROPN
cet-15688	104	16	t=340	t=340	PROPN
cet-15688	104	17	℃	℃	PROPN
cet-15688	104	18	c	c	PROPN
cet-15688	104	19	)	)	PUNCT
cet-15688	104	20	0	0	NUM
cet-15688	104	21	0.01	0.01	NUM
cet-15688	104	22	0.02	0.02	NUM
cet-15688	104	23	0.03	0.03	NUM
cet-15688	104	24	0.04	0.04	NUM
cet-15688	104	25	0.05	0.05	NUM
cet-15688	104	26	0.06	0.06	NUM
cet-15688	104	27	0.07	0.07	NUM
cet-15688	104	28	0.08	0.08	NUM
cet-15688	104	29	0.09	0.09	NUM
cet-15688	104	30	100	100	NUM
cet-15688	104	31	200	200	NUM
cet-15688	104	32	300	300	NUM
cet-15688	104	33	400	400	NUM
cet-15688	104	34	n	n	NUM
cet-15688	104	35	o	o	NOUN
cet-15688	105	1	rm	rm	NOUN
cet-15688	106	1	al	al	PROPN
cet-15688	107	1	iz	iz	INTJ
cet-15688	107	2	ed	ed	PROPN
cet-15688	107	3	a	a	DET
cet-15688	107	4	.u	.u	NOUN
cet-15688	107	5	.	.	PUNCT
cet-15688	108	1	temperature	temperature	NOUN
cet-15688	108	2	,	,	PUNCT
cet-15688	108	3	℃	℃	PROPN
cet-15688	108	4	sio2	sio2	VERB
cet-15688	108	5	ni	ni	PROPN
cet-15688	108	6	-	-	PROPN
cet-15688	108	7	cu	cu	PROPN
cet-15688	108	8	-	-	PUNCT
cet-15688	108	9	sio2	sio2	PROPN
cet-15688	108	10	cu	cu	PROPN
cet-15688	108	11	-	-	PUNCT
cet-15688	108	12	ni	ni	PROPN
cet-15688	108	13	-	-	PUNCT
cet-15688	108	14	sio2	sio2	PROPN
cet-15688	108	15	pt	pt	PROPN
cet-15688	108	16	-	-	PUNCT
cet-15688	108	17	cu	cu	NOUN
cet-15688	108	18	-	-	PUNCT
cet-15688	108	19	sio2	sio2	PROPN
cet-15688	108	20	t=180	t=180	PROPN
cet-15688	108	21	℃	℃	PROPN
cet-15688	108	22	t=340	t=340	PROPN
cet-15688	108	23	℃	℃	PROPN
cet-15688	108	24	d	d	PROPN
cet-15688	108	25	)	)	PUNCT
cet-15688	108	26	377	377	NUM
cet-15688	108	27	was	be	AUX
cet-15688	108	28	slightly	slightly	ADV
cet-15688	108	29	higher	high	ADJ
cet-15688	108	30	,	,	PUNCT
cet-15688	108	31	0.2	0.2	NUM
cet-15688	108	32	mmol(hcoh)/g(cat	mmol(hcoh)/g(cat	NUM
cet-15688	108	33	)	)	PUNCT
cet-15688	108	34	.	.	PUNCT
cet-15688	109	1	it	it	PRON
cet-15688	109	2	can	can	AUX
cet-15688	109	3	be	be	AUX
cet-15688	109	4	concluded	conclude	VERB
cet-15688	109	5	that	that	SCONJ
cet-15688	109	6	monometallic	monometallic	NOUN
cet-15688	109	7	samples	sample	NOUN
cet-15688	109	8	do	do	AUX
cet-15688	109	9	not	not	PART
cet-15688	109	10	show	show	VERB
cet-15688	109	11	activity	activity	NOUN
cet-15688	109	12	in	in	ADP
cet-15688	109	13	the	the	DET
cet-15688	109	14	transformation	transformation	NOUN
cet-15688	109	15	of	of	ADP
cet-15688	109	16	carbon	carbon	NOUN
cet-15688	109	17	dioxide	dioxide	NOUN
cet-15688	109	18	into	into	ADP
cet-15688	109	19	formaldehyde	formaldehyde	NOUN
cet-15688	109	20	,	,	PUNCT
cet-15688	109	21	while	while	SCONJ
cet-15688	109	22	bimetallic	bimetallic	ADJ
cet-15688	109	23	catalyst	catalyst	NOUN
cet-15688	109	24	samples	sample	NOUN
cet-15688	109	25	have	have	VERB
cet-15688	109	26	a	a	DET
cet-15688	109	27	higher	high	ADJ
cet-15688	109	28	activity	activity	NOUN
cet-15688	109	29	.	.	PUNCT
cet-15688	110	1	nickel	nickel	NOUN
cet-15688	110	2	and	and	CCONJ
cet-15688	110	3	copper	copper	NOUN
cet-15688	110	4	-	-	PUNCT
cet-15688	110	5	containing	contain	VERB
cet-15688	110	6	samples	sample	NOUN
cet-15688	110	7	showed	show	VERB
cet-15688	110	8	a	a	DET
cet-15688	110	9	yield	yield	NOUN
cet-15688	110	10	of	of	ADP
cet-15688	110	11	1.4–1.6	1.4–1.6	NUM
cet-15688	110	12	mmol(hcoh)/g(cat	mmol(hcoh)/g(cat	NUM
cet-15688	110	13	)	)	PUNCT
cet-15688	110	14	,	,	PUNCT
cet-15688	110	15	whereas	whereas	SCONJ
cet-15688	110	16	platinum	platinum	NOUN
cet-15688	110	17	and	and	CCONJ
cet-15688	110	18	copper	copper	NOUN
cet-15688	110	19	-	-	PUNCT
cet-15688	110	20	containing	contain	VERB
cet-15688	110	21	samples	sample	NOUN
cet-15688	110	22	showed	show	VERB
cet-15688	110	23	a	a	DET
cet-15688	110	24	yield	yield	NOUN
cet-15688	110	25	of	of	ADP
cet-15688	110	26	2.4	2.4	NUM
cet-15688	110	27	mmol(hcho)/g(cat	mmol(hcho)/g(cat	NUM
cet-15688	110	28	)	)	PUNCT
cet-15688	110	29	(	(	PUNCT
cet-15688	110	30	table	table	NOUN
cet-15688	110	31	3	3	NUM
cet-15688	110	32	)	)	PUNCT
cet-15688	110	33	.	.	PUNCT
cet-15688	111	1	table	table	NOUN
cet-15688	111	2	3	3	NUM
cet-15688	111	3	:	:	PUNCT
cet-15688	111	4	catalyst	catalyst	NOUN
cet-15688	111	5	testing	testing	NOUN
cet-15688	111	6	results	result	VERB
cet-15688	111	7	sample	sample	VERB
cet-15688	111	8	hcoh	hcoh	NOUN
cet-15688	111	9	yield	yield	NOUN
cet-15688	111	10	,	,	PUNCT
cet-15688	111	11	mmol	mmol	NOUN
cet-15688	111	12	/	/	SYM
cet-15688	111	13	g	g	NOUN
cet-15688	111	14	(	(	PUNCT
cet-15688	111	15	cat	cat	NOUN
cet-15688	111	16	)	)	PUNCT
cet-15688	111	17	co2	co2	NOUN
cet-15688	111	18	conversion	conversion	NOUN
cet-15688	111	19	,	,	PUNCT
cet-15688	111	20	%	%	PROPN
cet-15688	111	21	sio2	sio2	PROPN
cet-15688	111	22	cu	cu	PROPN
cet-15688	111	23	-	-	PUNCT
cet-15688	111	24	sio2	sio2	PROPN
cet-15688	111	25	0.002	0.002	NUM
cet-15688	111	26	0.004	0.004	NUM
cet-15688	111	27	ni	ni	PROPN
cet-15688	111	28	-	-	PUNCT
cet-15688	111	29	sio2	sio2	NOUN
cet-15688	111	30	0.01	0.01	NUM
cet-15688	111	31	0.01	0.01	NUM
cet-15688	111	32	pt	pt	PROPN
cet-15688	111	33	-	-	PUNCT
cet-15688	111	34	sio2	sio2	PROPN
cet-15688	111	35	0.2	0.2	NUM
cet-15688	111	36	0.7	0.7	NUM
cet-15688	111	37	ni	ni	PROPN
cet-15688	111	38	-	-	PROPN
cet-15688	111	39	cu	cu	PROPN
cet-15688	111	40	-	-	PUNCT
cet-15688	111	41	sio2	sio2	PROPN
cet-15688	111	42	1.4	1.4	NUM
cet-15688	111	43	5.3	5.3	NUM
cet-15688	111	44	cu	cu	PROPN
cet-15688	111	45	-	-	PUNCT
cet-15688	111	46	ni	ni	PROPN
cet-15688	111	47	-	-	PUNCT
cet-15688	111	48	sio2	sio2	PROPN
cet-15688	111	49	1.6	1.6	NUM
cet-15688	111	50	6.4	6.4	NUM
cet-15688	111	51	pt	pt	PROPN
cet-15688	111	52	-	-	PUNCT
cet-15688	111	53	cu	cu	NOUN
cet-15688	111	54	-	-	PUNCT
cet-15688	111	55	sio2	sio2	PROPN
cet-15688	111	56	7.4	7.4	NUM
cet-15688	111	57	24.2	24.2	NUM
cet-15688	111	58	a	a	DET
cet-15688	111	59	comparison	comparison	NOUN
cet-15688	111	60	of	of	ADP
cet-15688	111	61	the	the	DET
cet-15688	111	62	highest	high	ADJ
cet-15688	111	63	achieved	achieve	VERB
cet-15688	111	64	yield	yield	NOUN
cet-15688	111	65	of	of	ADP
cet-15688	111	66	formaldehyde	formaldehyde	NOUN
cet-15688	111	67	formation	formation	NOUN
cet-15688	111	68	for	for	ADP
cet-15688	111	69	the	the	DET
cet-15688	111	70	platinum	platinum	NOUN
cet-15688	111	71	-	-	PUNCT
cet-15688	111	72	copper	copper	NOUN
cet-15688	111	73	sample	sample	NOUN
cet-15688	111	74	impregnated	impregnate	VERB
cet-15688	111	75	on	on	ADP
cet-15688	111	76	silica	silica	NOUN
cet-15688	111	77	showed	show	VERB
cet-15688	111	78	an	an	DET
cet-15688	111	79	increase	increase	NOUN
cet-15688	111	80	in	in	ADP
cet-15688	111	81	the	the	DET
cet-15688	111	82	yield	yield	NOUN
cet-15688	111	83	by	by	ADP
cet-15688	111	84	15–20	15–20	NUM
cet-15688	111	85	%	%	NOUN
cet-15688	111	86	compared	compare	VERB
cet-15688	111	87	to	to	ADP
cet-15688	111	88	literature	literature	NOUN
cet-15688	111	89	data	datum	NOUN
cet-15688	111	90	(	(	PUNCT
cet-15688	111	91	chan	chan	PROPN
cet-15688	111	92	et	et	PROPN
cet-15688	111	93	al	al	PROPN
cet-15688	111	94	.	.	PROPN
cet-15688	111	95	,	,	PUNCT
cet-15688	111	96	2018	2018	NUM
cet-15688	111	97	)	)	PUNCT
cet-15688	111	98	.	.	PUNCT
cet-15688	112	1	4	4	X
cet-15688	112	2	.	.	X
cet-15688	112	3	conclusions	conclusion	NOUN
cet-15688	112	4	synthesis	synthesis	NOUN
cet-15688	112	5	of	of	ADP
cet-15688	112	6	active	active	ADJ
cet-15688	112	7	nickel-	nickel-	NOUN
cet-15688	112	8	,	,	PUNCT
cet-15688	112	9	copper-	copper-	NOUN
cet-15688	112	10	,	,	PUNCT
cet-15688	112	11	and	and	CCONJ
cet-15688	112	12	platinum	platinum	NOUN
cet-15688	112	13	-	-	PUNCT
cet-15688	112	14	containing	contain	VERB
cet-15688	112	15	samples	sample	NOUN
cet-15688	112	16	of	of	ADP
cet-15688	112	17	silica	silica	NOUN
cet-15688	112	18	for	for	ADP
cet-15688	112	19	direct	direct	ADJ
cet-15688	112	20	carbon	carbon	NOUN
cet-15688	112	21	dioxide	dioxide	NOUN
cet-15688	112	22	transformation	transformation	NOUN
cet-15688	112	23	into	into	ADP
cet-15688	112	24	formaldehyde	formaldehyde	NOUN
cet-15688	112	25	was	be	AUX
cet-15688	112	26	provided	provide	VERB
cet-15688	112	27	.	.	PUNCT
cet-15688	113	1	the	the	DET
cet-15688	113	2	developed	develop	VERB
cet-15688	113	3	samples	sample	NOUN
cet-15688	113	4	were	be	AUX
cet-15688	113	5	characterized	characterize	VERB
cet-15688	113	6	by	by	ADP
cet-15688	113	7	the	the	DET
cet-15688	113	8	nitrogen	nitrogen	NOUN
cet-15688	113	9	physisorption	physisorption	NOUN
cet-15688	113	10	analysis	analysis	NOUN
cet-15688	113	11	,	,	PUNCT
cet-15688	113	12	x	x	ADJ
cet-15688	113	13	-	-	NOUN
cet-15688	113	14	ray	ray	NOUN
cet-15688	113	15	fluorescence	fluorescence	NOUN
cet-15688	113	16	spectroscopy	spectroscopy	NOUN
cet-15688	113	17	,	,	PUNCT
cet-15688	113	18	and	and	CCONJ
cet-15688	113	19	hydrogen	hydrogen	NOUN
cet-15688	113	20	and	and	CCONJ
cet-15688	113	21	carbon	carbon	NOUN
cet-15688	113	22	dioxide	dioxide	NOUN
cet-15688	113	23	programmed	program	VERB
cet-15688	113	24	desorption	desorption	NOUN
cet-15688	113	25	.	.	PUNCT
cet-15688	114	1	the	the	DET
cet-15688	114	2	temperature	temperature	NOUN
cet-15688	114	3	-	-	PUNCT
cet-15688	114	4	programmed	program	VERB
cet-15688	114	5	desorption	desorption	NOUN
cet-15688	114	6	of	of	ADP
cet-15688	114	7	hydrogen	hydrogen	NOUN
cet-15688	114	8	and	and	CCONJ
cet-15688	114	9	carbon	carbon	NOUN
cet-15688	114	10	dioxide	dioxide	NOUN
cet-15688	114	11	revealed	reveal	VERB
cet-15688	114	12	the	the	DET
cet-15688	114	13	formation	formation	NOUN
cet-15688	114	14	of	of	ADP
cet-15688	114	15	primarily	primarily	ADV
cet-15688	114	16	one	one	NUM
cet-15688	114	17	desorption	desorption	NOUN
cet-15688	114	18	site	site	NOUN
cet-15688	114	19	for	for	ADP
cet-15688	114	20	hydrogen	hydrogen	NOUN
cet-15688	114	21	and	and	CCONJ
cet-15688	114	22	carbon	carbon	NOUN
cet-15688	114	23	dioxide	dioxide	NOUN
cet-15688	114	24	at	at	ADP
cet-15688	114	25	temperatures	temperature	NOUN
cet-15688	114	26	between	between	ADP
cet-15688	114	27	160	160	NUM
cet-15688	114	28	°	°	ADP
cet-15688	114	29	c	c	NOUN
cet-15688	114	30	and	and	CCONJ
cet-15688	114	31	190	190	NUM
cet-15688	114	32	°	°	NOUN
cet-15688	114	33	c	c	NOUN
cet-15688	114	34	.	.	PUNCT
cet-15688	115	1	the	the	DET
cet-15688	115	2	application	application	NOUN
cet-15688	115	3	of	of	ADP
cet-15688	115	4	microand	microand	PROPN
cet-15688	115	5	mesoporous	mesoporous	ADJ
cet-15688	115	6	silica	silica	NOUN
cet-15688	115	7	for	for	ADP
cet-15688	115	8	the	the	DET
cet-15688	115	9	formation	formation	NOUN
cet-15688	115	10	of	of	ADP
cet-15688	115	11	active	active	ADJ
cet-15688	115	12	metal	metal	NOUN
cet-15688	115	13	species	specie	NOUN
cet-15688	115	14	results	result	VERB
cet-15688	115	15	in	in	ADP
cet-15688	115	16	the	the	DET
cet-15688	115	17	formation	formation	NOUN
cet-15688	115	18	of	of	ADP
cet-15688	115	19	metallic	metallic	ADJ
cet-15688	115	20	species	specie	NOUN
cet-15688	115	21	within	within	ADP
cet-15688	115	22	the	the	DET
cet-15688	115	23	microand	microand	ADJ
cet-15688	115	24	mesoporous	mesoporous	ADJ
cet-15688	115	25	areas	area	NOUN
cet-15688	115	26	of	of	ADP
cet-15688	115	27	the	the	DET
cet-15688	115	28	silica	silica	NOUN
cet-15688	115	29	.	.	PUNCT
cet-15688	116	1	this	this	PRON
cet-15688	116	2	leads	lead	VERB
cet-15688	116	3	to	to	ADP
cet-15688	116	4	an	an	DET
cet-15688	116	5	increase	increase	NOUN
cet-15688	116	6	in	in	ADP
cet-15688	116	7	the	the	DET
cet-15688	116	8	formaldehyde	formaldehyde	NOUN
cet-15688	116	9	yield	yield	NOUN
cet-15688	116	10	by	by	ADP
cet-15688	116	11	15–20	15–20	NUM
cet-15688	116	12	%	%	NOUN
cet-15688	116	13	compared	compare	VERB
cet-15688	116	14	to	to	ADP
cet-15688	116	15	literature	literature	NOUN
cet-15688	116	16	data	datum	NOUN
cet-15688	116	17	.	.	PUNCT
cet-15688	117	1	acknowledgments	acknowledgment	NOUN
cet-15688	117	2	the	the	DET
cet-15688	117	3	study	study	NOUN
cet-15688	117	4	was	be	AUX
cet-15688	117	5	provided	provide	VERB
cet-15688	117	6	in	in	ADP
cet-15688	117	7	frame	frame	NOUN
cet-15688	117	8	of	of	ADP
cet-15688	117	9	the	the	DET
cet-15688	117	10	russian	russian	ADJ
cet-15688	117	11	science	science	PROPN
cet-15688	117	12	foundation	foundation	PROPN
cet-15688	117	13	,	,	PUNCT
cet-15688	117	14	grant	grant	VERB
cet-15688	117	15	number	number	NOUN
cet-15688	117	16	25	25	NUM
cet-15688	117	17	-	-	SYM
cet-15688	117	18	23	23	NUM
cet-15688	117	19	-	-	PUNCT
cet-15688	117	20	00333	00333	NUM
cet-15688	117	21	.	.	PUNCT
cet-15688	118	1	references	reference	NOUN
cet-15688	118	2	banerjee	banerjee	PROPN
cet-15688	118	3	a.	a.	PROPN
cet-15688	118	4	,	,	PUNCT
cet-15688	118	5	dick	dick	PROPN
cet-15688	118	6	g.r	g.r	PROPN
cet-15688	118	7	.	.	PROPN
cet-15688	118	8	,	,	PUNCT
cet-15688	118	9	yoshino	yoshino	PROPN
cet-15688	118	10	t.	t.	PROPN
cet-15688	118	11	,	,	PUNCT
cet-15688	118	12	kanan	kanan	PROPN
cet-15688	118	13	m.w	m.w	PROPN
cet-15688	118	14	.	.	PROPN
cet-15688	118	15	,	,	PUNCT
cet-15688	118	16	2016	2016	NUM
cet-15688	118	17	,	,	PUNCT
cet-15688	118	18	carbon	carbon	NOUN
cet-15688	118	19	dioxide	dioxide	NOUN
cet-15688	118	20	utilization	utilization	NOUN
cet-15688	118	21	via	via	ADP
cet-15688	118	22	carbonate	carbonate	NOUN
cet-15688	118	23	-	-	PUNCT
cet-15688	118	24	promoted	promote	VERB
cet-15688	118	25	c	c	NOUN
cet-15688	118	26	–	–	PUNCT
cet-15688	118	27	h	h	NOUN
cet-15688	118	28	carboxylation	carboxylation	NOUN
cet-15688	118	29	.	.	PUNCT
cet-15688	119	1	nature	nature	NOUN
cet-15688	119	2	,	,	PUNCT
cet-15688	119	3	531(7593	531(7593	NUM
cet-15688	119	4	)	)	PUNCT
cet-15688	119	5	,	,	PUNCT
cet-15688	119	6	215–219	215–219	NUM
cet-15688	119	7	.	.	PUNCT
cet-15688	120	1	chan	chan	PROPN
cet-15688	120	2	f.l	f.l	PROPN
cet-15688	120	3	.	.	PROPN
cet-15688	120	4	,	,	PUNCT
cet-15688	120	5	altinkaya	altinkaya	PROPN
cet-15688	120	6	g.	g.	PROPN
cet-15688	120	7	,	,	PUNCT
cet-15688	120	8	fung	fung	PROPN
cet-15688	120	9	n.	n.	PROPN
cet-15688	120	10	,	,	PUNCT
cet-15688	120	11	tanksale	tanksale	NOUN
cet-15688	120	12	a.	a.	NOUN
cet-15688	120	13	,	,	PUNCT
cet-15688	120	14	2018	2018	NUM
cet-15688	120	15	,	,	PUNCT
cet-15688	120	16	low	low	ADJ
cet-15688	120	17	temperature	temperature	NOUN
cet-15688	120	18	hydrogenation	hydrogenation	NOUN
cet-15688	120	19	of	of	ADP
cet-15688	120	20	carbon	carbon	NOUN
cet-15688	120	21	dioxide	dioxide	NOUN
cet-15688	120	22	into	into	ADP
cet-15688	120	23	formaldehyde	formaldehyde	NOUN
cet-15688	120	24	in	in	ADP
cet-15688	120	25	liquid	liquid	ADJ
cet-15688	120	26	media	medium	NOUN
cet-15688	120	27	.	.	PUNCT
cet-15688	121	1	catalysis	catalysis	NOUN
cet-15688	121	2	today	today	NOUN
cet-15688	121	3	,	,	PUNCT
cet-15688	121	4	309	309	NUM
cet-15688	121	5	,	,	PUNCT
cet-15688	121	6	242–247	242–247	NUM
cet-15688	121	7	.	.	PUNCT
cet-15688	122	1	hepburn	hepburn	PROPN
cet-15688	122	2	c.	c.	PROPN
cet-15688	122	3	,	,	PUNCT
cet-15688	122	4	adlen	adlen	PROPN
cet-15688	122	5	e.	e.	PROPN
cet-15688	122	6	,	,	PUNCT
cet-15688	122	7	beddington	beddington	PROPN
cet-15688	122	8	j.	j.	PROPN
cet-15688	122	9	,	,	PUNCT
cet-15688	122	10	carter	carter	PROPN
cet-15688	122	11	e.a	e.a	PROPN
cet-15688	122	12	.	.	PROPN
cet-15688	122	13	,	,	PUNCT
cet-15688	122	14	fuss	fuss	PROPN
cet-15688	122	15	s.	s.	PROPN
cet-15688	122	16	,	,	PUNCT
cet-15688	122	17	mac	mac	PROPN
cet-15688	122	18	dowell	dowell	PROPN
cet-15688	122	19	n.	n.	PROPN
cet-15688	122	20	,	,	PUNCT
cet-15688	122	21	minx	minx	PROPN
cet-15688	122	22	j.c	j.c	PROPN
cet-15688	122	23	.	.	PROPN
cet-15688	122	24	,	,	PUNCT
cet-15688	122	25	smith	smith	PROPN
cet-15688	122	26	p.	p.	PROPN
cet-15688	122	27	,	,	PUNCT
cet-15688	122	28	williams	williams	PROPN
cet-15688	122	29	c.k	c.k	PROPN
cet-15688	122	30	.	.	PROPN
cet-15688	122	31	,	,	PUNCT
cet-15688	122	32	2019	2019	NUM
cet-15688	122	33	,	,	PUNCT
cet-15688	122	34	the	the	DET
cet-15688	122	35	technological	technological	ADJ
cet-15688	122	36	and	and	CCONJ
cet-15688	122	37	economic	economic	ADJ
cet-15688	122	38	prospects	prospect	NOUN
cet-15688	122	39	for	for	ADP
cet-15688	122	40	co2	co2	NOUN
cet-15688	122	41	utilization	utilization	NOUN
cet-15688	122	42	and	and	CCONJ
cet-15688	122	43	removal	removal	NOUN
cet-15688	122	44	.	.	PUNCT
cet-15688	123	1	nature	nature	NOUN
cet-15688	123	2	,	,	PUNCT
cet-15688	123	3	575(7781	575(7781	NUM
cet-15688	123	4	)	)	PUNCT
cet-15688	123	5	,	,	PUNCT
cet-15688	123	6	87	87	NUM
cet-15688	123	7	–	–	SYM
cet-15688	123	8	97	97	NUM
cet-15688	123	9	.	.	PUNCT
cet-15688	124	1	leclerc	leclerc	PROPN
cet-15688	124	2	h.o	h.o	PROPN
cet-15688	124	3	.	.	PROPN
cet-15688	124	4	,	,	PUNCT
cet-15688	124	5	erythropel	erythropel	PROPN
cet-15688	124	6	h.	h.	PROPN
cet-15688	124	7	c.	c.	PROPN
cet-15688	124	8	,	,	PUNCT
cet-15688	124	9	backhaus	backhaus	PROPN
cet-15688	124	10	a.	a.	PROPN
cet-15688	124	11	,	,	PUNCT
cet-15688	124	12	lee	lee	PROPN
cet-15688	124	13	d.s	d.s	PROPN
cet-15688	124	14	.	.	PROPN
cet-15688	124	15	,	,	PUNCT
cet-15688	124	16	judd	judd	PROPN
cet-15688	124	17	d.r	d.r	PROPN
cet-15688	124	18	.	.	PROPN
cet-15688	124	19	,	,	PUNCT
cet-15688	124	20	paulsen	paulsen	PROPN
cet-15688	124	21	m.m	m.m	PROPN
cet-15688	124	22	.	.	PROPN
cet-15688	124	23	,	,	PUNCT
cet-15688	124	24	ishii	ishii	PROPN
cet-15688	124	25	m.	m.	NOUN
cet-15688	124	26	,	,	PUNCT
cet-15688	124	27	long	long	ADJ
cet-15688	124	28	a.	a.	NOUN
cet-15688	124	29	,	,	PUNCT
cet-15688	124	30	ratjen	ratjen	PROPN
cet-15688	124	31	l.	l.	PROPN
cet-15688	124	32	,	,	PUNCT
cet-15688	124	33	gonsalves	gonsalves	PROPN
cet-15688	124	34	bertho	bertho	PROPN
cet-15688	124	35	g.	g.	PROPN
cet-15688	124	36	,	,	PUNCT
cet-15688	124	37	deetman	deetman	PROPN
cet-15688	124	38	c.	c.	PROPN
cet-15688	124	39	,	,	PUNCT
cet-15688	124	40	du	du	PROPN
cet-15688	124	41	y.	y.	PROPN
cet-15688	124	42	,	,	PUNCT
cet-15688	124	43	lane	lane	PROPN
cet-15688	124	44	m.k.m	m.k.m	NOUN
cet-15688	124	45	.	.	PUNCT
cet-15688	124	46	,	,	PUNCT
cet-15688	124	47	petrovic	petrovic	PROPN
cet-15688	124	48	p.v	p.v	PROPN
cet-15688	124	49	.	.	PROPN
cet-15688	124	50	,	,	PUNCT
cet-15688	124	51	champlin	champlin	PROPN
cet-15688	124	52	a.t	a.t	PROPN
cet-15688	124	53	.	.	PROPN
cet-15688	124	54	,	,	PUNCT
cet-15688	124	55	bordet	bordet	PROPN
cet-15688	124	56	a.	a.	PROPN
cet-15688	124	57	,	,	PUNCT
cet-15688	124	58	kaeffer	kaeffer	PROPN
cet-15688	124	59	n.	n.	PROPN
cet-15688	124	60	,	,	PUNCT
cet-15688	124	61	kemper	kemper	PROPN
cet-15688	124	62	g.	g.	PROPN
cet-15688	124	63	,	,	PUNCT
cet-15688	124	64	zimmerman	zimmerman	PROPN
cet-15688	124	65	j.b	j.b	PROPN
cet-15688	124	66	.	.	PROPN
cet-15688	124	67	,	,	PUNCT
cet-15688	124	68	anastas	anasta	VERB
cet-15688	124	69	p.t	p.t	PROPN
cet-15688	124	70	.	.	PROPN
cet-15688	124	71	,	,	PUNCT
cet-15688	124	72	2025	2025	NUM
cet-15688	124	73	,	,	PUNCT
cet-15688	124	74	the	the	DET
cet-15688	124	75	co2	co2	NOUN
cet-15688	124	76	tree	tree	NOUN
cet-15688	124	77	:	:	PUNCT
cet-15688	124	78	the	the	DET
cet-15688	124	79	potential	potential	NOUN
cet-15688	124	80	for	for	ADP
cet-15688	124	81	carbon	carbon	NOUN
cet-15688	124	82	dioxide	dioxide	NOUN
cet-15688	124	83	utilization	utilization	NOUN
cet-15688	124	84	pathways	pathway	NOUN
cet-15688	124	85	.	.	PUNCT
cet-15688	125	1	acs	acs	PROPN
cet-15688	125	2	sustainable	sustainable	ADJ
cet-15688	125	3	chemistry	chemistry	NOUN
cet-15688	125	4	and	and	CCONJ
cet-15688	125	5	engineering	engineering	NOUN
cet-15688	125	6	,	,	PUNCT
cet-15688	125	7	13	13	NUM
cet-15688	125	8	,	,	PUNCT
cet-15688	125	9	5	5	NUM
cet-15688	125	10	-	-	SYM
cet-15688	125	11	29	29	NUM
cet-15688	125	12	.	.	PUNCT
cet-15688	126	1	lee	lee	PROPN
cet-15688	126	2	d.-k	d.-k	PROPN
cet-15688	126	3	.	.	PUNCT
cet-15688	126	4	,	,	PUNCT
cet-15688	126	5	kim	kim	PROPN
cet-15688	126	6	d.-s	d.-s	PROPN
cet-15688	126	7	.	.	PUNCT
cet-15688	126	8	,	,	PUNCT
cet-15688	126	9	kim	kim	PROPN
cet-15688	126	10	s.-w	s.-w	PROPN
cet-15688	126	11	.	.	PUNCT
cet-15688	126	12	,	,	PUNCT
cet-15688	126	13	2001	2001	NUM
cet-15688	126	14	,	,	PUNCT
cet-15688	126	15	selective	selective	ADJ
cet-15688	126	16	formation	formation	NOUN
cet-15688	126	17	of	of	ADP
cet-15688	126	18	formaldehyde	formaldehyde	NOUN
cet-15688	126	19	from	from	ADP
cet-15688	126	20	carbon	carbon	NOUN
cet-15688	126	21	dioxide	dioxide	NOUN
cet-15688	126	22	and	and	CCONJ
cet-15688	126	23	hydrogen	hydrogen	NOUN
cet-15688	126	24	over	over	ADP
cet-15688	126	25	ptcu	ptcu	NOUN
cet-15688	126	26	/	/	SYM
cet-15688	126	27	sio2	sio2	PROPN
cet-15688	126	28	.	.	PUNCT
cet-15688	126	29	applied	apply	VERB
cet-15688	126	30	organometallic	organometallic	ADJ
cet-15688	126	31	chemistry	chemistry	NOUN
cet-15688	126	32	,	,	PUNCT
cet-15688	126	33	15	15	NUM
cet-15688	126	34	(	(	PUNCT
cet-15688	126	35	2	2	NUM
cet-15688	126	36	)	)	PUNCT
cet-15688	126	37	,	,	PUNCT
cet-15688	126	38	148–150	148–150	NUM
cet-15688	126	39	.	.	PUNCT
cet-15688	127	1	rauch	rauch	PROPN
cet-15688	127	2	m.	m.	PROPN
cet-15688	127	3	,	,	PUNCT
cet-15688	127	4	strater	strater	PROPN
cet-15688	127	5	z.	z.	PROPN
cet-15688	127	6	,	,	PUNCT
cet-15688	127	7	parkin	parkin	ADJ
cet-15688	127	8	g.	g.	NOUN
cet-15688	127	9	,	,	PUNCT
cet-15688	127	10	2019	2019	NUM
cet-15688	127	11	,	,	PUNCT
cet-15688	127	12	selective	selective	ADJ
cet-15688	127	13	conversion	conversion	NOUN
cet-15688	127	14	of	of	ADP
cet-15688	127	15	carbon	carbon	NOUN
cet-15688	127	16	dioxide	dioxide	NOUN
cet-15688	127	17	to	to	AUX
cet-15688	127	18	formaldehyde	formaldehyde	NOUN
cet-15688	127	19	via	via	ADP
cet-15688	127	20	a	a	DET
cet-15688	127	21	bis(silyl)acetal	bis(silyl)acetal	NUM
cet-15688	127	22	:	:	PUNCT
cet-15688	127	23	incorporation	incorporation	NOUN
cet-15688	127	24	of	of	ADP
cet-15688	127	25	isotopically	isotopically	ADV
cet-15688	127	26	labeled	label	VERB
cet-15688	127	27	c1	c1	NOUN
cet-15688	127	28	moieties	moiety	NOUN
cet-15688	127	29	derived	derive	VERB
cet-15688	127	30	from	from	ADP
cet-15688	127	31	carbon	carbon	NOUN
cet-15688	127	32	dioxide	dioxide	NOUN
cet-15688	127	33	into	into	ADP
cet-15688	127	34	organic	organic	ADJ
cet-15688	127	35	molecules	molecule	NOUN
cet-15688	127	36	.	.	PUNCT
cet-15688	128	1	journal	journal	NOUN
cet-15688	128	2	of	of	ADP
cet-15688	128	3	the	the	DET
cet-15688	128	4	american	american	PROPN
cet-15688	128	5	chemical	chemical	PROPN
cet-15688	128	6	society	society	PROPN
cet-15688	128	7	,	,	PUNCT
cet-15688	128	8	141(44	141(44	NUM
cet-15688	128	9	)	)	PUNCT
cet-15688	128	10	,	,	PUNCT
cet-15688	128	11	17754–17762	17754–17762	NUM
cet-15688	128	12	.	.	PUNCT
cet-15688	129	1	siebert	siebert	PROPN
cet-15688	129	2	m.	m.	PROPN
cet-15688	129	3	,	,	PUNCT
cet-15688	129	4	seibicke	seibicke	VERB
cet-15688	129	5	m.	m.	NOUN
cet-15688	129	6	,	,	PUNCT
cet-15688	129	7	siegle	siegle	PROPN
cet-15688	129	8	a.f	a.f	PROPN
cet-15688	129	9	.	.	PROPN
cet-15688	129	10	,	,	PUNCT
cet-15688	129	11	kräh	kräh	PROPN
cet-15688	129	12	s.	s.	PROPN
cet-15688	129	13	,	,	PUNCT
cet-15688	129	14	trapp	trapp	PROPN
cet-15688	129	15	o.	o.	PROPN
cet-15688	129	16	,	,	PUNCT
cet-15688	129	17	2019	2019	NUM
cet-15688	129	18	,	,	PUNCT
cet-15688	129	19	selective	selective	ADJ
cet-15688	129	20	ruthenium	ruthenium	NOUN
cet-15688	129	21	-	-	PUNCT
cet-15688	129	22	catalyzed	catalyze	VERB
cet-15688	129	23	transformation	transformation	NOUN
cet-15688	129	24	of	of	ADP
cet-15688	129	25	carbon	carbon	NOUN
cet-15688	129	26	dioxide	dioxide	NOUN
cet-15688	129	27	:	:	PUNCT
cet-15688	129	28	an	an	DET
cet-15688	129	29	alternative	alternative	ADJ
cet-15688	129	30	approach	approach	NOUN
cet-15688	129	31	toward	toward	ADP
cet-15688	129	32	formaldehyde	formaldehyde	NOUN
cet-15688	129	33	.	.	PUNCT
cet-15688	130	1	journal	journal	NOUN
cet-15688	130	2	of	of	ADP
cet-15688	130	3	the	the	DET
cet-15688	130	4	american	american	PROPN
cet-15688	130	5	chemical	chemical	PROPN
cet-15688	130	6	society	society	PROPN
cet-15688	130	7	,	,	PUNCT
cet-15688	130	8	141(1	141(1	NUM
cet-15688	130	9	)	)	PUNCT
cet-15688	130	10	,	,	PUNCT
cet-15688	130	11	334–341	334–341	NUM
cet-15688	130	12	.	.	PUNCT
cet-15688	131	1	singh	singh	PROPN
cet-15688	131	2	d.	d.	PROPN
cet-15688	131	3	,	,	PUNCT
cet-15688	131	4	gupta	gupta	PROPN
cet-15688	131	5	s.k	s.k	PROPN
cet-15688	131	6	.	.	PROPN
cet-15688	131	7	,	,	PUNCT
cet-15688	131	8	seriani	seriani	PROPN
cet-15688	131	9	n.	n.	PROPN
cet-15688	131	10	,	,	PUNCT
cet-15688	131	11	lukačević	lukačević	PROPN
cet-15688	131	12	i.	i.	PROPN
cet-15688	131	13	,	,	PUNCT
cet-15688	131	14	sonvane	sonvane	NOUN
cet-15688	131	15	y.	y.	PROPN
cet-15688	131	16	,	,	PUNCT
cet-15688	131	17	gajjar	gajjar	NOUN
cet-15688	131	18	p.n	p.n	PROPN
cet-15688	131	19	.	.	PROPN
cet-15688	131	20	,	,	PUNCT
cet-15688	131	21	ahuja	ahuja	PROPN
cet-15688	131	22	r.	r.	PROPN
cet-15688	131	23	,	,	PUNCT
cet-15688	131	24	2021	2021	NUM
cet-15688	131	25	,	,	PUNCT
cet-15688	131	26	mechanism	mechanism	NOUN
cet-15688	131	27	of	of	ADP
cet-15688	131	28	formaldehyde	formaldehyde	NOUN
cet-15688	131	29	and	and	CCONJ
cet-15688	131	30	formic	formic	ADJ
cet-15688	131	31	acid	acid	NOUN
cet-15688	131	32	formation	formation	NOUN
cet-15688	131	33	on	on	ADP
cet-15688	131	34	(	(	PUNCT
cet-15688	131	35	101)-tio2@cu4	101)-tio2@cu4	PROPN
cet-15688	131	36	systems	system	NOUN
cet-15688	131	37	through	through	ADP
cet-15688	131	38	co2	co2	NOUN
cet-15688	131	39	hydrogenation	hydrogenation	NOUN
cet-15688	131	40	.	.	PUNCT
cet-15688	132	1	sustainable	sustainable	ADJ
cet-15688	132	2	energy	energy	NOUN
cet-15688	132	3	fuels	fuel	NOUN
cet-15688	132	4	,	,	PUNCT
cet-15688	132	5	5	5	NUM
cet-15688	132	6	,	,	PUNCT
cet-15688	132	7	564	564	NUM
cet-15688	132	8	-	-	SYM
cet-15688	132	9	574	574	NUM
cet-15688	132	10	.	.	X
cet-15688	132	11	378	378	NUM
cet-15688	132	12	0189.pdf	0189.pdf	NOUN
cet-15688	132	13	cu	cu	PROPN
cet-15688	132	14	,	,	PUNCT
cet-15688	132	15	ni	ni	PROPN
cet-15688	132	16	,	,	PUNCT
cet-15688	132	17	pt	pt	PROPN
cet-15688	132	18	bimetallic	bimetallic	PROPN
cet-15688	132	19	microporous	microporous	ADJ
cet-15688	132	20	supported	support	VERB
cet-15688	132	21	silica	silica	NOUN
cet-15688	132	22	catalysts	catalyst	NOUN
cet-15688	132	23	for	for	ADP
cet-15688	132	24	direct	direct	ADJ
cet-15688	132	25	formaldehyde	formaldehyde	NOUN
cet-15688	132	26	synthesis	synthesis	NOUN
cet-15688	132	27	from	from	ADP
cet-15688	132	28	carbon	carbon	NOUN
cet-15688	132	29	dioxide	dioxide	NOUN
cet-15688	132	30	and	and	CCONJ
cet-15688	132	31	hydrogen	hydrogen	NOUN