id	sid	tid	token	lemma	pos
cet-2646	1	1	microsoft	microsoft	PROPN
cet-2646	1	2	word	word	PROPN
cet-2646	1	3	55castellanos.docx	55castellanos.docx	NUM
cet-2646	1	4	chemical	chemical	NOUN
cet-2646	1	5	engineering	engineering	NOUN
cet-2646	1	6	transactions	transaction	NOUN
cet-2646	1	7	vol	vol	NOUN
cet-2646	1	8	.	.	PROPN
cet-2646	1	9	64	64	NUM
cet-2646	1	10	,	,	PUNCT
cet-2646	1	11	2018	2018	NUM
cet-2646	1	12	a	a	DET
cet-2646	1	13	publication	publication	NOUN
cet-2646	1	14	of	of	ADP
cet-2646	1	15	the	the	DET
cet-2646	1	16	italian	italian	ADJ
cet-2646	1	17	association	association	NOUN
cet-2646	1	18	of	of	ADP
cet-2646	1	19	chemical	chemical	PROPN
cet-2646	1	20	engineering	engineering	NOUN
cet-2646	1	21	online	online	ADV
cet-2646	1	22	at	at	ADP
cet-2646	1	23	www.aidic.it/cet	www.aidic.it/cet	PROPN
cet-2646	1	24	guest	guest	NOUN
cet-2646	1	25	editors	editor	NOUN
cet-2646	1	26	:	:	PUNCT
cet-2646	1	27	enrico	enrico	PROPN
cet-2646	1	28	bardone	bardone	PROPN
cet-2646	1	29	,	,	PUNCT
cet-2646	1	30	antonio	antonio	NOUN
cet-2646	1	31	marzocchella	marzocchella	PROPN
cet-2646	1	32	,	,	PUNCT
cet-2646	1	33	tajalli	tajalli	PROPN
cet-2646	1	34	keshavarz	keshavarz	PROPN
cet-2646	1	35	copyright	copyright	NOUN
cet-2646	1	36	©	©	PROPN
cet-2646	1	37	2018	2018	NUM
cet-2646	1	38	,	,	PUNCT
cet-2646	1	39	aidic	aidic	ADJ
cet-2646	1	40	servizi	servizi	PROPN
cet-2646	1	41	s.r.l	s.r.l	PROPN
cet-2646	1	42	.	.	PUNCT
cet-2646	2	1	isbn	isbn	ADJ
cet-2646	2	2	978	978	NUM
cet-2646	2	3	-	-	SYM
cet-2646	2	4	88	88	NUM
cet-2646	2	5	-	-	PUNCT
cet-2646	2	6	9560856	9560856	NUM
cet-2646	2	7	-	-	SYM
cet-2646	2	8	3	3	NUM
cet-2646	2	9	;	;	PUNCT
cet-2646	2	10	issn	issn	PROPN
cet-2646	2	11	2283	2283	NUM
cet-2646	2	12	-	-	SYM
cet-2646	2	13	9216	9216	NUM
cet-2646	2	14	mechanism	mechanism	NOUN
cet-2646	2	15	and	and	CCONJ
cet-2646	2	16	application	application	NOUN
cet-2646	2	17	of	of	ADP
cet-2646	2	18	photocatalytic	photocatalytic	ADJ
cet-2646	2	19	hydrogen	hydrogen	NOUN
cet-2646	2	20	generation	generation	NOUN
cet-2646	2	21	by	by	ADP
cet-2646	2	22	cobalt	cobalt	NOUN
cet-2646	2	23	oximes	oxime	NOUN
cet-2646	2	24	shuai	shuai	PROPN
cet-2646	2	25	zhanga	zhanga	PROPN
cet-2646	2	26	,	,	PUNCT
cet-2646	2	27	lei	lei	PROPN
cet-2646	2	28	chen	chen	PROPN
cet-2646	2	29	*	*	PROPN
cet-2646	2	30	,	,	PUNCT
cet-2646	2	31	b	b	X
cet-2646	2	32	acollege	acollege	NOUN
cet-2646	2	33	of	of	ADP
cet-2646	2	34	materials	material	NOUN
cet-2646	2	35	science	science	NOUN
cet-2646	2	36	and	and	CCONJ
cet-2646	2	37	engineering	engineering	NOUN
cet-2646	2	38	,	,	PUNCT
cet-2646	2	39	jilin	jilin	PROPN
cet-2646	2	40	jian	jian	PROPN
cet-2646	2	41	zhu	zhu	PROPN
cet-2646	2	42	university	university	PROPN
cet-2646	2	43	,	,	PUNCT
cet-2646	2	44	changchun	changchun	PROPN
cet-2646	2	45	130118	130118	NUM
cet-2646	2	46	,	,	PUNCT
cet-2646	2	47	china	china	PROPN
cet-2646	2	48	bcollege	bcollege	PROPN
cet-2646	2	49	of	of	ADP
cet-2646	2	50	municipal	municipal	ADJ
cet-2646	2	51	and	and	CCONJ
cet-2646	2	52	environmental	environmental	ADJ
cet-2646	2	53	engineering	engineering	NOUN
cet-2646	2	54	,	,	PUNCT
cet-2646	2	55	jilin	jilin	PROPN
cet-2646	2	56	jian	jian	PROPN
cet-2646	2	57	zhu	zhu	PROPN
cet-2646	2	58	university	university	PROPN
cet-2646	2	59	,	,	PUNCT
cet-2646	2	60	changchun	changchun	PROPN
cet-2646	2	61	130118	130118	NUM
cet-2646	2	62	,	,	PUNCT
cet-2646	2	63	china	china	PROPN
cet-2646	2	64	chenlei@jlju.edu.cn	chenlei@jlju.edu.cn	VERB
cet-2646	2	65	in	in	ADP
cet-2646	2	66	this	this	DET
cet-2646	2	67	work	work	NOUN
cet-2646	2	68	,	,	PUNCT
cet-2646	2	69	cobaloxime	cobaloxime	ADJ
cet-2646	2	70	molecules	molecule	NOUN
cet-2646	2	71	have	have	AUX
cet-2646	2	72	been	be	AUX
cet-2646	2	73	synthesized	synthesize	VERB
cet-2646	2	74	in	in	ADP
cet-2646	2	75	our	our	PRON
cet-2646	2	76	group	group	NOUN
cet-2646	2	77	,	,	PUNCT
cet-2646	2	78	and	and	CCONJ
cet-2646	2	79	new	new	ADJ
cet-2646	2	80	photoinduced	photoinduce	VERB
cet-2646	2	81	hydrogen	hydrogen	NOUN
cet-2646	2	82	production	production	NOUN
cet-2646	2	83	systems	system	NOUN
cet-2646	2	84	have	have	AUX
cet-2646	2	85	been	be	AUX
cet-2646	2	86	constructed	construct	VERB
cet-2646	2	87	.	.	PUNCT
cet-2646	3	1	based	base	VERB
cet-2646	3	2	on	on	ADP
cet-2646	3	3	the	the	DET
cet-2646	3	4	new	new	ADJ
cet-2646	3	5	systems	system	NOUN
cet-2646	3	6	for	for	ADP
cet-2646	3	7	hydrogen	hydrogen	NOUN
cet-2646	3	8	production	production	NOUN
cet-2646	3	9	,	,	PUNCT
cet-2646	3	10	the	the	DET
cet-2646	3	11	mechanism	mechanism	NOUN
cet-2646	3	12	of	of	ADP
cet-2646	3	13	electron	electron	NOUN
cet-2646	3	14	transfer	transfer	NOUN
cet-2646	3	15	as	as	ADV
cet-2646	3	16	well	well	ADV
cet-2646	3	17	as	as	ADP
cet-2646	3	18	system	system	NOUN
cet-2646	3	19	degradation	degradation	NOUN
cet-2646	3	20	have	have	AUX
cet-2646	3	21	been	be	AUX
cet-2646	3	22	investigated	investigate	VERB
cet-2646	3	23	in	in	ADP
cet-2646	3	24	detail	detail	NOUN
cet-2646	3	25	.	.	PUNCT
cet-2646	4	1	according	accord	VERB
cet-2646	4	2	to	to	ADP
cet-2646	4	3	the	the	DET
cet-2646	4	4	simulation	simulation	NOUN
cet-2646	4	5	results	result	VERB
cet-2646	4	6	in	in	ADP
cet-2646	4	7	gaussian	gaussian	ADJ
cet-2646	4	8	03	03	NUM
cet-2646	4	9	software	software	NOUN
cet-2646	4	10	,	,	PUNCT
cet-2646	4	11	we	we	PRON
cet-2646	4	12	implement	implement	VERB
cet-2646	4	13	the	the	DET
cet-2646	4	14	ideal	ideal	ADJ
cet-2646	4	15	catalytic	catalytic	ADJ
cet-2646	4	16	process	process	NOUN
cet-2646	4	17	for	for	ADP
cet-2646	4	18	hydrogen	hydrogen	NOUN
cet-2646	4	19	production	production	NOUN
cet-2646	4	20	induced	induce	VERB
cet-2646	4	21	by	by	ADP
cet-2646	4	22	cobaloxime	cobaloxime	NOUN
cet-2646	4	23	.	.	PUNCT
cet-2646	5	1	in	in	ADP
cet-2646	5	2	cobaloxime	cobaloxime	ADJ
cet-2646	5	3	molecular	molecular	NOUN
cet-2646	5	4	,	,	PUNCT
cet-2646	5	5	co	co	X
cet-2646	5	6	is	be	AUX
cet-2646	5	7	indeed	indeed	ADV
cet-2646	5	8	the	the	DET
cet-2646	5	9	catalytic	catalytic	ADJ
cet-2646	5	10	center	center	NOUN
cet-2646	5	11	,	,	PUNCT
cet-2646	5	12	that	that	PRON
cet-2646	5	13	is	be	AUX
cet-2646	5	14	to	to	PART
cet-2646	5	15	say	say	VERB
cet-2646	5	16	,	,	PUNCT
cet-2646	5	17	it	it	PRON
cet-2646	5	18	is	be	AUX
cet-2646	5	19	the	the	DET
cet-2646	5	20	change	change	NOUN
cet-2646	5	21	of	of	ADP
cet-2646	5	22	electrovalence	electrovalence	NOUN
cet-2646	5	23	of	of	ADP
cet-2646	5	24	co	co	NOUN
cet-2646	5	25	atoms	atom	NOUN
cet-2646	5	26	from	from	ADP
cet-2646	5	27	3	3	NUM
cet-2646	5	28	to	to	ADP
cet-2646	5	29	2	2	NUM
cet-2646	5	30	and	and	CCONJ
cet-2646	5	31	1	1	NUM
cet-2646	5	32	,	,	PUNCT
cet-2646	5	33	and	and	CCONJ
cet-2646	5	34	then	then	ADV
cet-2646	5	35	from	from	ADP
cet-2646	5	36	1	1	NUM
cet-2646	5	37	to	to	ADP
cet-2646	5	38	3	3	NUM
cet-2646	5	39	,	,	PUNCT
cet-2646	5	40	implies	imply	VERB
cet-2646	5	41	the	the	DET
cet-2646	5	42	catalytic	catalytic	ADJ
cet-2646	5	43	process	process	NOUN
cet-2646	5	44	.	.	PUNCT
cet-2646	6	1	through	through	ADP
cet-2646	6	2	the	the	DET
cet-2646	6	3	simulation	simulation	NOUN
cet-2646	6	4	,	,	PUNCT
cet-2646	6	5	we	we	PRON
cet-2646	6	6	can	can	AUX
cet-2646	6	7	obtain	obtain	VERB
cet-2646	6	8	the	the	DET
cet-2646	6	9	middle	middle	ADJ
cet-2646	6	10	products	product	NOUN
cet-2646	6	11	in	in	ADP
cet-2646	6	12	the	the	DET
cet-2646	6	13	catalytic	catalytic	ADJ
cet-2646	6	14	process	process	NOUN
cet-2646	6	15	clearly	clearly	ADV
cet-2646	6	16	.	.	PUNCT
cet-2646	7	1	moreover	moreover	ADV
cet-2646	7	2	,	,	PUNCT
cet-2646	7	3	the	the	DET
cet-2646	7	4	electron	electron	NOUN
cet-2646	7	5	charge	charge	NOUN
cet-2646	7	6	of	of	ADP
cet-2646	7	7	middle	middle	ADJ
cet-2646	7	8	products	product	NOUN
cet-2646	7	9	can	can	AUX
cet-2646	7	10	be	be	AUX
cet-2646	7	11	analyzed	analyze	VERB
cet-2646	7	12	,	,	PUNCT
cet-2646	7	13	based	base	VERB
cet-2646	7	14	on	on	ADP
cet-2646	7	15	which	which	PRON
cet-2646	7	16	the	the	DET
cet-2646	7	17	catalytic	catalytic	ADJ
cet-2646	7	18	pathway	pathway	NOUN
cet-2646	7	19	predicted	predict	VERB
cet-2646	7	20	by	by	ADP
cet-2646	7	21	other	other	ADJ
cet-2646	7	22	experimental	experimental	ADJ
cet-2646	7	23	results	result	NOUN
cet-2646	7	24	is	be	AUX
cet-2646	7	25	confirmed	confirm	VERB
cet-2646	7	26	.	.	PUNCT
cet-2646	8	1	all	all	DET
cet-2646	8	2	this	this	PRON
cet-2646	8	3	provides	provide	VERB
cet-2646	8	4	the	the	DET
cet-2646	8	5	theoretical	theoretical	ADJ
cet-2646	8	6	basis	basis	NOUN
cet-2646	8	7	for	for	SCONJ
cet-2646	8	8	the	the	DET
cet-2646	8	9	hydrogen	hydrogen	NOUN
cet-2646	8	10	production	production	NOUN
cet-2646	8	11	catalyzed	catalyze	VERB
cet-2646	8	12	by	by	ADP
cet-2646	8	13	cobaloxime	cobaloxime	ADJ
cet-2646	8	14	molecular	molecular	NOUN
cet-2646	8	15	.	.	PUNCT
cet-2646	9	1	1	1	X
cet-2646	9	2	.	.	X
cet-2646	9	3	introduction	introduction	NOUN
cet-2646	9	4	how	how	SCONJ
cet-2646	9	5	to	to	PART
cet-2646	9	6	utilize	utilize	VERB
cet-2646	9	7	inexhaustible	inexhaustible	ADJ
cet-2646	9	8	solar	solar	ADJ
cet-2646	9	9	energy	energy	NOUN
cet-2646	9	10	to	to	PART
cet-2646	9	11	prepare	prepare	VERB
cet-2646	9	12	hydrogen	hydrogen	NOUN
cet-2646	9	13	from	from	ADP
cet-2646	9	14	photolysis	photolysis	NOUN
cet-2646	9	15	water	water	NOUN
cet-2646	9	16	efficiently	efficiently	ADV
cet-2646	9	17	and	and	CCONJ
cet-2646	9	18	inexpensively	inexpensively	ADV
cet-2646	9	19	is	be	AUX
cet-2646	9	20	one	one	NUM
cet-2646	9	21	of	of	ADP
cet-2646	9	22	the	the	DET
cet-2646	9	23	hotspots	hotspot	NOUN
cet-2646	9	24	in	in	ADP
cet-2646	9	25	the	the	DET
cet-2646	9	26	hydrogen	hydrogen	NOUN
cet-2646	9	27	energy	energy	NOUN
cet-2646	9	28	development	development	NOUN
cet-2646	9	29	and	and	CCONJ
cet-2646	9	30	augurs	augur	VERB
cet-2646	9	31	well	well	ADV
cet-2646	9	32	for	for	ADP
cet-2646	9	33	the	the	DET
cet-2646	9	34	future	future	ADJ
cet-2646	9	35	development	development	NOUN
cet-2646	9	36	of	of	ADP
cet-2646	9	37	new	new	ADJ
cet-2646	9	38	energy	energy	NOUN
cet-2646	9	39	in	in	ADP
cet-2646	9	40	our	our	PRON
cet-2646	9	41	country	country	NOUN
cet-2646	9	42	.	.	PUNCT
cet-2646	10	1	currently	currently	ADV
cet-2646	10	2	,	,	PUNCT
cet-2646	10	3	in	in	ADP
cet-2646	10	4	view	view	NOUN
cet-2646	10	5	of	of	ADP
cet-2646	10	6	the	the	DET
cet-2646	10	7	increasingly	increasingly	ADV
cet-2646	10	8	shortage	shortage	NOUN
cet-2646	10	9	of	of	ADP
cet-2646	10	10	energy	energy	NOUN
cet-2646	10	11	resources	resource	NOUN
cet-2646	10	12	and	and	CCONJ
cet-2646	10	13	the	the	DET
cet-2646	10	14	continuously	continuously	ADV
cet-2646	10	15	serious	serious	ADJ
cet-2646	10	16	environmental	environmental	ADJ
cet-2646	10	17	pollution	pollution	NOUN
cet-2646	10	18	,	,	PUNCT
cet-2646	10	19	the	the	DET
cet-2646	10	20	photocatalytic	photocatalytic	ADJ
cet-2646	10	21	water	water	NOUN
cet-2646	10	22	splitting	splitting	NOUN
cet-2646	10	23	for	for	ADP
cet-2646	10	24	hydrogen	hydrogen	NOUN
cet-2646	10	25	production	production	NOUN
cet-2646	10	26	by	by	ADP
cet-2646	10	27	utilizing	utilize	VERB
cet-2646	10	28	the	the	DET
cet-2646	10	29	solar	solar	ADJ
cet-2646	10	30	energy	energy	NOUN
cet-2646	10	31	is	be	AUX
cet-2646	10	32	an	an	DET
cet-2646	10	33	ultimate	ultimate	ADJ
cet-2646	10	34	method	method	NOUN
cet-2646	10	35	to	to	PART
cet-2646	10	36	resolve	resolve	VERB
cet-2646	10	37	energy	energy	NOUN
cet-2646	10	38	and	and	CCONJ
cet-2646	10	39	environmental	environmental	ADJ
cet-2646	10	40	problems	problem	NOUN
cet-2646	10	41	(	(	PUNCT
cet-2646	10	42	kudo	kudo	NOUN
cet-2646	10	43	and	and	CCONJ
cet-2646	10	44	miseki	miseki	PROPN
cet-2646	10	45	,	,	PUNCT
cet-2646	10	46	2009	2009	NUM
cet-2646	10	47	)	)	PUNCT
cet-2646	10	48	.	.	PUNCT
cet-2646	11	1	in	in	ADP
cet-2646	11	2	the	the	DET
cet-2646	11	3	process	process	NOUN
cet-2646	11	4	of	of	ADP
cet-2646	11	5	hydrogen	hydrogen	NOUN
cet-2646	11	6	production	production	NOUN
cet-2646	11	7	by	by	ADP
cet-2646	11	8	photocatalytic	photocatalytic	ADJ
cet-2646	11	9	water	water	NOUN
cet-2646	11	10	splitting	splitting	NOUN
cet-2646	11	11	,	,	PUNCT
cet-2646	11	12	the	the	DET
cet-2646	11	13	key	key	ADJ
cet-2646	11	14	challenge	challenge	NOUN
cet-2646	11	15	for	for	ADP
cet-2646	11	16	capturing	capture	VERB
cet-2646	11	17	hydrogen	hydrogen	NOUN
cet-2646	11	18	by	by	ADP
cet-2646	11	19	solar	solar	ADJ
cet-2646	11	20	energy	energy	NOUN
cet-2646	11	21	is	be	AUX
cet-2646	11	22	how	how	SCONJ
cet-2646	11	23	to	to	PART
cet-2646	11	24	develop	develop	VERB
cet-2646	11	25	the	the	DET
cet-2646	11	26	catalytic	catalytic	ADJ
cet-2646	11	27	material	material	NOUN
cet-2646	11	28	with	with	ADP
cet-2646	11	29	high	high	ADJ
cet-2646	11	30	photocatalytic	photocatalytic	ADJ
cet-2646	11	31	activity	activity	NOUN
cet-2646	11	32	and	and	CCONJ
cet-2646	11	33	hydrogen	hydrogen	NOUN
cet-2646	11	34	generation	generation	NOUN
cet-2646	11	35	efficiency	efficiency	NOUN
cet-2646	11	36	in	in	ADP
cet-2646	11	37	the	the	DET
cet-2646	11	38	visible	visible	ADJ
cet-2646	11	39	light	light	ADJ
cet-2646	11	40	range	range	NOUN
cet-2646	11	41	at	at	ADP
cet-2646	11	42	a	a	DET
cet-2646	11	43	low	low	ADJ
cet-2646	11	44	cost	cost	NOUN
cet-2646	11	45	.	.	PUNCT
cet-2646	12	1	so	so	ADV
cet-2646	12	2	far	far	ADV
cet-2646	12	3	,	,	PUNCT
cet-2646	12	4	scholars	scholar	NOUN
cet-2646	12	5	have	have	AUX
cet-2646	12	6	made	make	VERB
cet-2646	12	7	extensive	extensive	ADJ
cet-2646	12	8	studies	study	NOUN
cet-2646	12	9	on	on	ADP
cet-2646	12	10	the	the	DET
cet-2646	12	11	photocatalytic	photocatalytic	ADJ
cet-2646	12	12	materials	material	NOUN
cet-2646	12	13	,	,	PUNCT
cet-2646	12	14	especially	especially	ADV
cet-2646	12	15	on	on	ADP
cet-2646	12	16	some	some	DET
cet-2646	12	17	photocatalysts	photocatalyst	NOUN
cet-2646	12	18	about	about	ADP
cet-2646	12	19	metal	metal	NOUN
cet-2646	12	20	oxides	oxide	NOUN
cet-2646	12	21	and	and	CCONJ
cet-2646	12	22	sulfides	sulfide	NOUN
cet-2646	12	23	(	(	PUNCT
cet-2646	12	24	fujishima	fujishima	NOUN
cet-2646	12	25	and	and	CCONJ
cet-2646	12	26	honda	honda	NOUN
cet-2646	12	27	,	,	PUNCT
cet-2646	12	28	1972	1972	NUM
cet-2646	12	29	;	;	PUNCT
cet-2646	12	30	bernhard	bernhard	PROPN
cet-2646	12	31	and	and	CCONJ
cet-2646	12	32	allen	allen	PROPN
cet-2646	12	33	,	,	PUNCT
cet-2646	12	34	1978	1978	NUM
cet-2646	12	35	;	;	PUNCT
cet-2646	12	36	mark	mark	NOUN
cet-2646	12	37	and	and	CCONJ
cet-2646	12	38	mate	mate	NOUN
cet-2646	12	39	,	,	PUNCT
cet-2646	12	40	2010	2010	NUM
cet-2646	12	41	;	;	PUNCT
cet-2646	12	42	bigi	bigi	PROPN
cet-2646	12	43	et	et	PROPN
cet-2646	12	44	al	al	PROPN
cet-2646	12	45	.	.	PROPN
cet-2646	12	46	,	,	PUNCT
cet-2646	12	47	2010	2010	NUM
cet-2646	12	48	;	;	PUNCT
cet-2646	12	49	osterloh	osterloh	NOUN
cet-2646	12	50	,	,	PUNCT
cet-2646	12	51	2008	2008	NUM
cet-2646	12	52	)	)	PUNCT
cet-2646	12	53	such	such	ADJ
cet-2646	12	54	as	as	ADP
cet-2646	12	55	tio2	tio2	NOUN
cet-2646	12	56	and	and	CCONJ
cet-2646	12	57	cds	cd	NOUN
cet-2646	12	58	.	.	PUNCT
cet-2646	13	1	although	although	SCONJ
cet-2646	13	2	tio2	tio2	NOUN
cet-2646	13	3	features	feature	VERB
cet-2646	13	4	non	non	ADJ
cet-2646	13	5	-	-	NOUN
cet-2646	13	6	toxicity	toxicity	ADJ
cet-2646	13	7	,	,	PUNCT
cet-2646	13	8	low	low	ADJ
cet-2646	13	9	cost	cost	NOUN
cet-2646	13	10	,	,	PUNCT
cet-2646	13	11	chemical	chemical	NOUN
cet-2646	13	12	stability	stability	NOUN
cet-2646	13	13	and	and	CCONJ
cet-2646	13	14	other	other	ADJ
cet-2646	13	15	properties	property	NOUN
cet-2646	13	16	,	,	PUNCT
cet-2646	13	17	a	a	DET
cet-2646	13	18	larger	large	ADJ
cet-2646	13	19	energy	energy	NOUN
cet-2646	13	20	gap	gap	NOUN
cet-2646	13	21	makes	make	VERB
cet-2646	13	22	the	the	DET
cet-2646	13	23	tio2	tio2	NOUN
cet-2646	13	24	only	only	ADV
cet-2646	13	25	response	response	NOUN
cet-2646	13	26	to	to	ADP
cet-2646	13	27	the	the	DET
cet-2646	13	28	solar	solar	ADJ
cet-2646	13	29	ultraviolet	ultraviolet	ADJ
cet-2646	13	30	light	light	NOUN
cet-2646	13	31	at	at	ADP
cet-2646	13	32	a	a	DET
cet-2646	13	33	low	low	ADJ
cet-2646	13	34	utilization	utilization	NOUN
cet-2646	13	35	rate	rate	NOUN
cet-2646	13	36	;	;	PUNCT
cet-2646	13	37	the	the	DET
cet-2646	13	38	application	application	NOUN
cet-2646	13	39	of	of	ADP
cet-2646	13	40	cds	cd	NOUN
cet-2646	13	41	is	be	AUX
cet-2646	13	42	also	also	ADV
cet-2646	13	43	limited	limit	VERB
cet-2646	13	44	due	due	ADP
cet-2646	13	45	to	to	ADP
cet-2646	13	46	its	its	PRON
cet-2646	13	47	liable	liable	ADJ
cet-2646	13	48	light	light	ADJ
cet-2646	13	49	corrosion	corrosion	NOUN
cet-2646	13	50	.	.	PUNCT
cet-2646	14	1	in	in	ADP
cet-2646	14	2	this	this	DET
cet-2646	14	3	paper	paper	NOUN
cet-2646	14	4	,	,	PUNCT
cet-2646	14	5	we	we	PRON
cet-2646	14	6	mainly	mainly	ADV
cet-2646	14	7	explore	explore	VERB
cet-2646	14	8	the	the	DET
cet-2646	14	9	catalytic	catalytic	ADJ
cet-2646	14	10	hydrogen	hydrogen	NOUN
cet-2646	14	11	production	production	NOUN
cet-2646	14	12	cycle	cycle	NOUN
cet-2646	14	13	of	of	ADP
cet-2646	14	14	cobalt	cobalt	NOUN
cet-2646	14	15	oximes	oxime	NOUN
cet-2646	14	16	by	by	ADP
cet-2646	14	17	computational	computational	ADJ
cet-2646	14	18	simulation	simulation	NOUN
cet-2646	14	19	,	,	PUNCT
cet-2646	14	20	and	and	CCONJ
cet-2646	14	21	probe	probe	VERB
cet-2646	14	22	into	into	ADP
cet-2646	14	23	the	the	DET
cet-2646	14	24	internal	internal	ADJ
cet-2646	14	25	charge	charge	NOUN
cet-2646	14	26	transport	transport	NOUN
cet-2646	14	27	process	process	NOUN
cet-2646	14	28	to	to	PART
cet-2646	14	29	reveal	reveal	VERB
cet-2646	14	30	a	a	DET
cet-2646	14	31	real	real	ADJ
cet-2646	14	32	process	process	NOUN
cet-2646	14	33	about	about	ADP
cet-2646	14	34	how	how	SCONJ
cet-2646	14	35	the	the	DET
cet-2646	14	36	cobalt	cobalt	NOUN
cet-2646	14	37	oxime	oxime	NOUN
cet-2646	14	38	molecules	molecule	NOUN
cet-2646	14	39	are	be	AUX
cet-2646	14	40	catalyzed	catalyze	VERB
cet-2646	14	41	.	.	PUNCT
cet-2646	15	1	2	2	X
cet-2646	15	2	.	.	X
cet-2646	15	3	model	model	NOUN
cet-2646	15	4	the	the	DET
cet-2646	15	5	[	[	X
cet-2646	15	6	co(dmgh)2pycl	co(dmgh)2pycl	NOUN
cet-2646	15	7	]	]	X
cet-2646	15	8	molecule	molecule	NOUN
cet-2646	15	9	is	be	AUX
cet-2646	15	10	taken	take	VERB
cet-2646	15	11	as	as	ADP
cet-2646	15	12	a	a	DET
cet-2646	15	13	study	study	NOUN
cet-2646	15	14	object	object	NOUN
cet-2646	15	15	in	in	ADP
cet-2646	15	16	this	this	DET
cet-2646	15	17	paper	paper	NOUN
cet-2646	15	18	,	,	PUNCT
cet-2646	15	19	by	by	ADP
cet-2646	15	20	which	which	PRON
cet-2646	15	21	,	,	PUNCT
cet-2646	15	22	the	the	DET
cet-2646	15	23	charge	charge	NOUN
cet-2646	15	24	transport	transport	NOUN
cet-2646	15	25	during	during	ADP
cet-2646	15	26	hydrogen	hydrogen	NOUN
cet-2646	15	27	production	production	NOUN
cet-2646	15	28	is	be	AUX
cet-2646	15	29	simulated	simulate	VERB
cet-2646	15	30	using	use	VERB
cet-2646	15	31	gussian03	gussian03	NOUN
cet-2646	15	32	.	.	PUNCT
cet-2646	16	1	the	the	DET
cet-2646	16	2	cobalt	cobalt	NOUN
cet-2646	16	3	oxime	oxime	NOUN
cet-2646	16	4	[	[	X
cet-2646	16	5	co(dmgh)2pycl	co(dmgh)2pycl	NOUN
cet-2646	16	6	]	]	X
cet-2646	16	7	molecule	molecule	NOUN
cet-2646	16	8	geometry	geometry	NOUN
cet-2646	16	9	model	model	NOUN
cet-2646	16	10	is	be	AUX
cet-2646	16	11	shown	show	VERB
cet-2646	16	12	in	in	ADP
cet-2646	16	13	figure	figure	NOUN
cet-2646	16	14	1	1	NUM
cet-2646	16	15	:	:	PUNCT
cet-2646	16	16	doi	doi	NOUN
cet-2646	16	17	:	:	PUNCT
cet-2646	16	18	10.3303	10.3303	NUM
cet-2646	16	19	/	/	SYM
cet-2646	16	20	cet1864104	cet1864104	NOUN
cet-2646	16	21	please	please	INTJ
cet-2646	16	22	cite	cite	VERB
cet-2646	16	23	this	this	DET
cet-2646	16	24	article	article	NOUN
cet-2646	16	25	as	as	ADP
cet-2646	16	26	:	:	PUNCT
cet-2646	16	27	shuai	shuai	PROPN
cet-2646	16	28	zhang	zhang	PROPN
cet-2646	16	29	,	,	PUNCT
cet-2646	16	30	lei	lei	PROPN
cet-2646	16	31	chen	chen	PROPN
cet-2646	16	32	,	,	PUNCT
cet-2646	16	33	2018	2018	NUM
cet-2646	16	34	,	,	PUNCT
cet-2646	16	35	mechanism	mechanism	NOUN
cet-2646	16	36	and	and	CCONJ
cet-2646	16	37	application	application	NOUN
cet-2646	16	38	of	of	ADP
cet-2646	16	39	photocatalytic	photocatalytic	ADJ
cet-2646	16	40	hydrogen	hydrogen	NOUN
cet-2646	16	41	generation	generation	NOUN
cet-2646	16	42	by	by	ADP
cet-2646	16	43	cobalt	cobalt	NOUN
cet-2646	16	44	oximes	oxime	NOUN
cet-2646	16	45	,	,	PUNCT
cet-2646	16	46	chemical	chemical	NOUN
cet-2646	16	47	engineering	engineering	NOUN
cet-2646	16	48	transactions	transaction	NOUN
cet-2646	16	49	,	,	PUNCT
cet-2646	16	50	64	64	NUM
cet-2646	16	51	,	,	PUNCT
cet-2646	16	52	619	619	NUM
cet-2646	16	53	-	-	SYM
cet-2646	16	54	624	624	NUM
cet-2646	16	55	doi	doi	NOUN
cet-2646	16	56	:	:	PUNCT
cet-2646	16	57	10.3303	10.3303	NUM
cet-2646	16	58	/	/	SYM
cet-2646	16	59	cet1864104	cet1864104	NOUN
cet-2646	16	60	619	619	NUM
cet-2646	16	61	figure	figure	VERB
cet-2646	16	62	1	1	NUM
cet-2646	16	63	:	:	PUNCT
cet-2646	16	64	cobalt	cobalt	NOUN
cet-2646	16	65	oxime	oxime	NOUN
cet-2646	16	66	[	[	X
cet-2646	16	67	co(dmgh)2pycl	co(dmgh)2pycl	NOUN
cet-2646	16	68	]	]	X
cet-2646	16	69	molecule	molecule	NOUN
cet-2646	16	70	geometry	geometry	NOUN
cet-2646	16	71	model	model	NOUN
cet-2646	16	72	first	first	ADV
cet-2646	16	73	,	,	PUNCT
cet-2646	16	74	the	the	DET
cet-2646	16	75	molecular	molecular	ADJ
cet-2646	16	76	structure	structure	NOUN
cet-2646	16	77	model	model	NOUN
cet-2646	16	78	for	for	ADP
cet-2646	16	79	cobalt	cobalt	NOUN
cet-2646	16	80	oximes	oxime	NOUN
cet-2646	16	81	is	be	AUX
cet-2646	16	82	built	build	VERB
cet-2646	16	83	on	on	ADP
cet-2646	16	84	the	the	DET
cet-2646	16	85	gussian03	gussian03	ADJ
cet-2646	16	86	g	g	NOUN
cet-2646	16	87	-	-	PUNCT
cet-2646	16	88	view	view	NOUN
cet-2646	16	89	interface	interface	NOUN
cet-2646	16	90	.	.	PUNCT
cet-2646	17	1	then	then	ADV
cet-2646	17	2	the	the	DET
cet-2646	17	3	[	[	X
cet-2646	17	4	co	co	NOUN
cet-2646	17	5	(	(	PUNCT
cet-2646	17	6	dmgh	dmgh	NOUN
cet-2646	17	7	)	)	PUNCT
cet-2646	17	8	2pycl	2pycl	NUM
cet-2646	17	9	]	]	X
cet-2646	17	10	molecular	molecular	ADJ
cet-2646	17	11	geometry	geometry	NOUN
cet-2646	17	12	structure	structure	NOUN
cet-2646	17	13	is	be	AUX
cet-2646	17	14	optimized	optimize	VERB
cet-2646	17	15	by	by	ADP
cet-2646	17	16	using	use	VERB
cet-2646	17	17	the	the	DET
cet-2646	17	18	density	density	NOUN
cet-2646	17	19	functional	functional	ADJ
cet-2646	17	20	theory	theory	NOUN
cet-2646	17	21	(	(	PUNCT
cet-2646	17	22	dft	dft	NOUN
cet-2646	17	23	)	)	PUNCT
cet-2646	17	24	in	in	ADP
cet-2646	17	25	gussian03	gussian03	ADJ
cet-2646	17	26	quantum	quantum	ADJ
cet-2646	17	27	chemistry	chemistry	NOUN
cet-2646	17	28	calculation	calculation	NOUN
cet-2646	17	29	software	software	NOUN
cet-2646	17	30	.	.	PUNCT
cet-2646	18	1	the	the	DET
cet-2646	18	2	geometrical	geometrical	ADJ
cet-2646	18	3	parameters	parameter	NOUN
cet-2646	18	4	of	of	ADP
cet-2646	18	5	optimized	optimize	VERB
cet-2646	18	6	molecule	molecule	NOUN
cet-2646	18	7	are	be	AUX
cet-2646	18	8	shown	show	VERB
cet-2646	18	9	in	in	ADP
cet-2646	18	10	the	the	DET
cet-2646	18	11	table	table	NOUN
cet-2646	18	12	1	1	X
cet-2646	18	13	.	.	PUNCT
cet-2646	19	1	it	it	PRON
cet-2646	19	2	is	be	AUX
cet-2646	19	3	obvious	obvious	ADJ
cet-2646	19	4	that	that	SCONJ
cet-2646	19	5	the	the	DET
cet-2646	19	6	results	result	NOUN
cet-2646	19	7	of	of	ADP
cet-2646	19	8	the	the	DET
cet-2646	19	9	dft	dft	PROPN
cet-2646	19	10	computational	computational	PROPN
cet-2646	19	11	simulation	simulation	NOUN
cet-2646	19	12	coincide	coincide	NOUN
cet-2646	19	13	with	with	ADP
cet-2646	19	14	those	those	PRON
cet-2646	19	15	from	from	ADP
cet-2646	19	16	other	other	ADJ
cet-2646	19	17	scholars	scholar	NOUN
cet-2646	19	18	’	’	PART
cet-2646	19	19	experiments	experiment	NOUN
cet-2646	19	20	,	,	PUNCT
cet-2646	19	21	which	which	PRON
cet-2646	19	22	demonstrates	demonstrate	VERB
cet-2646	19	23	the	the	DET
cet-2646	19	24	rationalities	rationality	NOUN
cet-2646	19	25	of	of	ADP
cet-2646	19	26	the	the	DET
cet-2646	19	27	simulation	simulation	NOUN
cet-2646	19	28	and	and	CCONJ
cet-2646	19	29	the	the	DET
cet-2646	19	30	preferences	preference	NOUN
cet-2646	19	31	as	as	ADP
cet-2646	19	32	a	a	DET
cet-2646	19	33	reasonable	reasonable	ADJ
cet-2646	19	34	parameter	parameter	NOUN
cet-2646	19	35	setting	set	VERB
cet-2646	19	36	for	for	ADP
cet-2646	19	37	further	further	ADJ
cet-2646	19	38	charge	charge	NOUN
cet-2646	19	39	transfer	transfer	NOUN
cet-2646	19	40	computations	computation	NOUN
cet-2646	19	41	.	.	PUNCT
cet-2646	20	1	table	table	NOUN
cet-2646	20	2	1	1	NUM
cet-2646	20	3	:	:	PUNCT
cet-2646	20	4	the	the	DET
cet-2646	20	5	geometrical	geometrical	ADJ
cet-2646	20	6	parameters	parameter	NOUN
cet-2646	20	7	of	of	ADP
cet-2646	20	8	optimized	optimize	VERB
cet-2646	20	9	molecule	molecule	NOUN
cet-2646	20	10	bond	bond	NOUN
cet-2646	20	11	length(å)/angle	length(å)/angle	NOUN
cet-2646	20	12	(	(	PUNCT
cet-2646	20	13	º	º	NOUN
cet-2646	20	14	)	)	PUNCT
cet-2646	20	15	dft	dft	PROPN
cet-2646	20	16	computation	computation	NOUN
cet-2646	20	17	data	datum	NOUN
cet-2646	20	18	from	from	ADP
cet-2646	20	19	literature	literature	NOUN
cet-2646	20	20	bond	bond	NOUN
cet-2646	20	21	length(å)/angle	length(å)/angle	PROPN
cet-2646	20	22	(	(	PUNCT
cet-2646	20	23	º	º	NOUN
cet-2646	20	24	)	)	PUNCT
cet-2646	20	25	dft	dft	PROPN
cet-2646	20	26	computation	computation	NOUN
cet-2646	20	27	data	datum	NOUN
cet-2646	20	28	from	from	ADP
cet-2646	20	29	literature	literature	PROPN
cet-2646	20	30	co1	co1	PROPN
cet-2646	20	31	-	-	PROPN
cet-2646	20	32	c1	c1	PROPN
cet-2646	20	33	1.94889	1.94889	NUM
cet-2646	20	34	1.931(3	1.931(3	NUM
cet-2646	20	35	)	)	PUNCT
cet-2646	20	36	n11	n11	PROPN
cet-2646	20	37	-	-	PUNCT
cet-2646	20	38	co1	co1	PROPN
cet-2646	20	39	-	-	PROPN
cet-2646	20	40	n21	n21	PROPN
cet-2646	20	41	98.51726	98.51726	NUM
cet-2646	20	42	98.59(13	98.59(13	NUM
cet-2646	20	43	)	)	PUNCT
cet-2646	20	44	co1	co1	PROPN
cet-2646	20	45	-	-	NOUN
cet-2646	20	46	n11	n11	PROPN
cet-2646	20	47	1.91883	1.91883	NUM
cet-2646	20	48	1.883(2	1.883(2	NUM
cet-2646	20	49	)	)	PUNCT
cet-2646	20	50	n14	n14	NOUN
cet-2646	20	51	-	-	PUNCT
cet-2646	20	52	co1	co1	PROPN
cet-2646	20	53	-	-	PROPN
cet-2646	20	54	n24	n24	PROPN
cet-2646	20	55	98.57008	98.57008	NUM
cet-2646	20	56	98.19(12	98.19(12	NUM
cet-2646	20	57	)	)	PUNCT
cet-2646	20	58	co1	co1	PROPN
cet-2646	20	59	-	-	PUNCT
cet-2646	20	60	n14	n14	PROPN
cet-2646	20	61	1.92780	1.92780	NUM
cet-2646	20	62	1.891(2	1.891(2	NUM
cet-2646	20	63	)	)	PUNCT
cet-2646	20	64	n11	n11	NOUN
cet-2646	20	65	-	-	PUNCT
cet-2646	20	66	co1	co1	PROPN
cet-2646	20	67	-	-	PUNCT
cet-2646	20	68	n14	n14	X
cet-2646	20	69	81.43517	81.43517	NUM
cet-2646	20	70	81.77(12	81.77(12	NUM
cet-2646	20	71	)	)	PUNCT
cet-2646	20	72	co1	co1	PROPN
cet-2646	20	73	-	-	PROPN
cet-2646	20	74	n21	n21	PROPN
cet-2646	20	75	1.92683	1.92683	NUM
cet-2646	20	76	1.889(2	1.889(2	NUM
cet-2646	20	77	)	)	PUNCT
cet-2646	20	78	n21	n21	NOUN
cet-2646	20	79	-	-	PUNCT
cet-2646	20	80	co1	co1	PROPN
cet-2646	20	81	-	-	PROPN
cet-2646	20	82	n24	n24	PROPN
cet-2646	20	83	81.42611	81.42611	NUM
cet-2646	20	84	81.42(13	81.42(13	NUM
cet-2646	20	85	)	)	PUNCT
cet-2646	20	86	co1	co1	PROPN
cet-2646	20	87	-	-	PROPN
cet-2646	20	88	n24	n24	PROPN
cet-2646	20	89	1.92024	1.92024	NUM
cet-2646	20	90	1.885(2	1.885(2	NUM
cet-2646	20	91	)	)	PUNCT
cet-2646	20	92	n11	n11	PROPN
cet-2646	20	93	-	-	PUNCT
cet-2646	20	94	co1	co1	NOUN
cet-2646	20	95	-	-	NOUN
cet-2646	20	96	c1	c1	PROPN
cet-2646	20	97	86.68097	86.68097	NUM
cet-2646	20	98	89.91(17	89.91(17	NUM
cet-2646	20	99	)	)	PUNCT
cet-2646	20	100	co1	co1	PROPN
cet-2646	20	101	-	-	NOUN
cet-2646	20	102	n31	n31	ADJ
cet-2646	20	103	2.05502	2.05502	NUM
cet-2646	20	104	2.040(2	2.040(2	NUM
cet-2646	20	105	)	)	PUNCT
cet-2646	20	106	n11	n11	NOUN
cet-2646	20	107	-	-	PUNCT
cet-2646	20	108	co1	co1	NOUN
cet-2646	20	109	-	-	NOUN
cet-2646	20	110	n31	n31	ADJ
cet-2646	20	111	91.32890	91.32890	NUM
cet-2646	20	112	90.75(12	90.75(12	NUM
cet-2646	20	113	)	)	PUNCT
cet-2646	20	114	n11	n11	NOUN
cet-2646	20	115	-	-	PUNCT
cet-2646	20	116	o15	o15	NOUN
cet-2646	20	117	1.36514	1.36514	NUM
cet-2646	20	118	1.358(3	1.358(3	NUM
cet-2646	20	119	)	)	PUNCT
cet-2646	20	120	n14	n14	PROPN
cet-2646	20	121	-	-	PUNCT
cet-2646	20	122	co1	co1	NOUN
cet-2646	20	123	-	-	PROPN
cet-2646	20	124	c1	c1	NOUN
cet-2646	20	125	91.49525	91.49525	NUM
cet-2646	20	126	87.75(10	87.75(10	NUM
cet-2646	20	127	)	)	PUNCT
cet-2646	20	128	n24	n24	NOUN
cet-2646	20	129	-	-	PUNCT
cet-2646	20	130	o26	o26	PROPN
cet-2646	20	131	1.36485	1.36485	NUM
cet-2646	20	132	1.353(3	1.353(3	NUM
cet-2646	20	133	)	)	PUNCT
cet-2646	20	134	n14	n14	NOUN
cet-2646	20	135	-	-	PUNCT
cet-2646	20	136	co1	co1	PROPN
cet-2646	20	137	-	-	ADJ
cet-2646	20	138	n31	n31	ADJ
cet-2646	20	139	90.46430	90.46430	NUM
cet-2646	20	140	89.10(9	89.10(9	NUM
cet-2646	20	141	)	)	PUNCT
cet-2646	20	142	n14	n14	PROPN
cet-2646	20	143	-	-	PUNCT
cet-2646	20	144	o16	o16	PROPN
cet-2646	20	145	1.30531	1.30531	NUM
cet-2646	20	146	1.322(3	1.322(3	NUM
cet-2646	20	147	)	)	PUNCT
cet-2646	20	148	n21	n21	PROPN
cet-2646	20	149	-	-	PUNCT
cet-2646	20	150	co1	co1	PROPN
cet-2646	20	151	-	-	PROPN
cet-2646	20	152	c1	c1	NOUN
cet-2646	20	153	87.59563	87.59563	NUM
cet-2646	20	154	91.60(11	91.60(11	NUM
cet-2646	20	155	)	)	PUNCT
cet-2646	20	156	n21	n21	NOUN
cet-2646	20	157	-	-	PUNCT
cet-2646	20	158	o25	o25	VERB
cet-2646	20	159	1.30455	1.30455	NUM
cet-2646	20	160	1.337(4	1.337(4	NUM
cet-2646	20	161	)	)	PUNCT
cet-2646	20	162	n21	n21	NOUN
cet-2646	20	163	-	-	PUNCT
cet-2646	20	164	co1	co1	PROPN
cet-2646	20	165	-	-	ADJ
cet-2646	20	166	n31	n31	ADJ
cet-2646	20	167	90.44449	90.44449	NUM
cet-2646	20	168	91.55(8	91.55(8	NOUN
cet-2646	20	169	)	)	PUNCT
cet-2646	20	170	n11	n11	NOUN
cet-2646	20	171	-	-	PUNCT
cet-2646	20	172	co1	co1	PROPN
cet-2646	20	173	-	-	PROPN
cet-2646	20	174	n24	n24	PROPN
cet-2646	20	175	176.79654	176.79654	NUM
cet-2646	20	176	177.16(10	177.16(10	NUM
cet-2646	20	177	)	)	PUNCT
cet-2646	20	178	n24	n24	PROPN
cet-2646	20	179	-	-	PUNCT
cet-2646	20	180	co1	co1	PROPN
cet-2646	20	181	-	-	NOUN
cet-2646	20	182	c1	c1	NOUN
cet-2646	20	183	90.11695	90.11695	NUM
cet-2646	20	184	87.26(17	87.26(17	NUM
cet-2646	20	185	)	)	PUNCT
cet-2646	20	186	n14	n14	PROPN
cet-2646	20	187	-	-	PUNCT
cet-2646	20	188	co1	co1	PROPN
cet-2646	20	189	-	-	PUNCT
cet-2646	20	190	n21	n21	NOUN
cet-2646	20	191	179.09083	179.09083	NUM
cet-2646	20	192	179.25(12	179.25(12	NUM
cet-2646	20	193	)	)	PUNCT
cet-2646	20	194	n24	n24	NOUN
cet-2646	20	195	-	-	PUNCT
cet-2646	20	196	co1	co1	PROPN
cet-2646	20	197	-	-	ADJ
cet-2646	20	198	n31	n31	ADJ
cet-2646	20	199	91.87438	91.87438	NUM
cet-2646	20	200	92.09(12	92.09(12	NUM
cet-2646	20	201	)	)	PUNCT
cet-2646	20	202	the	the	DET
cet-2646	20	203	energy	energy	NOUN
cet-2646	20	204	of	of	ADP
cet-2646	20	205	geometrically	geometrically	ADV
cet-2646	20	206	optimized	optimize	VERB
cet-2646	20	207	[	[	X
cet-2646	20	208	co	co	INTJ
cet-2646	20	209	(	(	PUNCT
cet-2646	20	210	dmgh	dmgh	NOUN
cet-2646	20	211	)	)	PUNCT
cet-2646	20	212	2pycl	2pycl	NUM
cet-2646	20	213	]	]	X
cet-2646	20	214	molecule	molecule	NOUN
cet-2646	20	215	is	be	AUX
cet-2646	20	216	then	then	ADV
cet-2646	20	217	improved	improve	VERB
cet-2646	20	218	using	use	VERB
cet-2646	20	219	dft	dft	NOUN
cet-2646	20	220	.	.	PUNCT
cet-2646	21	1	by	by	ADP
cet-2646	21	2	calculating	calculate	VERB
cet-2646	21	3	the	the	DET
cet-2646	21	4	energy	energy	NOUN
cet-2646	21	5	level	level	NOUN
cet-2646	21	6	and	and	CCONJ
cet-2646	21	7	distribution	distribution	NOUN
cet-2646	21	8	at	at	ADP
cet-2646	21	9	the	the	DET
cet-2646	21	10	lumo	lumo	NOUN
cet-2646	21	11	orbit	orbit	NOUN
cet-2646	21	12	,	,	PUNCT
cet-2646	21	13	we	we	PRON
cet-2646	21	14	discovery	discovery	VERB
cet-2646	21	15	that	that	SCONJ
cet-2646	21	16	the	the	DET
cet-2646	21	17	lumo	lumo	NOUN
cet-2646	21	18	of	of	ADP
cet-2646	21	19	[	[	X
cet-2646	21	20	co	co	NOUN
cet-2646	21	21	(	(	PUNCT
cet-2646	21	22	dmgh	dmgh	NOUN
cet-2646	21	23	)	)	PUNCT
cet-2646	21	24	2pycl	2pycl	NUM
cet-2646	21	25	]	]	X
cet-2646	21	26	molecule	molecule	NOUN
cet-2646	21	27	lies	lie	VERB
cet-2646	21	28	in	in	ADP
cet-2646	21	29	the	the	DET
cet-2646	21	30	axial	axial	ADJ
cet-2646	21	31	pyridyl	pyridyl	PROPN
cet-2646	21	32	group	group	NOUN
cet-2646	21	33	,	,	PUNCT
cet-2646	21	34	as	as	SCONJ
cet-2646	21	35	shown	show	VERB
cet-2646	21	36	in	in	ADP
cet-2646	21	37	figure	figure	NOUN
cet-2646	21	38	.	.	PUNCT
cet-2646	22	1	2	2	NUM
cet-2646	22	2	:	:	PUNCT
cet-2646	22	3	figure	figure	NOUN
cet-2646	22	4	2	2	NUM
cet-2646	22	5	:	:	PUNCT
cet-2646	22	6	lumo	lumo	NOUN
cet-2646	22	7	of	of	ADP
cet-2646	22	8	[	[	X
cet-2646	22	9	co	co	NOUN
cet-2646	22	10	(	(	PUNCT
cet-2646	22	11	dmgh	dmgh	NOUN
cet-2646	22	12	)	)	PUNCT
cet-2646	22	13	2pycl	2pycl	NUM
cet-2646	22	14	]	]	X
cet-2646	22	15	molecule	molecule	NOUN
cet-2646	22	16	lies	lie	VERB
cet-2646	22	17	in	in	ADP
cet-2646	22	18	the	the	DET
cet-2646	22	19	axial	axial	ADJ
cet-2646	22	20	pyridyl	pyridyl	PROPN
cet-2646	22	21	group	group	NOUN
cet-2646	22	22	the	the	DET
cet-2646	22	23	result	result	NOUN
cet-2646	22	24	from	from	ADP
cet-2646	22	25	this	this	DET
cet-2646	22	26	calculation	calculation	NOUN
cet-2646	22	27	shows	show	VERB
cet-2646	22	28	that	that	SCONJ
cet-2646	22	29	the	the	DET
cet-2646	22	30	cobalt	cobalt	NOUN
cet-2646	22	31	oxime	oxime	NOUN
cet-2646	22	32	molecule	molecule	NOUN
cet-2646	22	33	[	[	X
cet-2646	22	34	co	co	NOUN
cet-2646	22	35	(	(	PUNCT
cet-2646	22	36	dmgh	dmgh	NOUN
cet-2646	22	37	)	)	PUNCT
cet-2646	22	38	2pycl	2pycl	NUM
cet-2646	22	39	]	]	PUNCT
cet-2646	22	40	accesses	access	VERB
cet-2646	22	41	to	to	ADP
cet-2646	22	42	the	the	DET
cet-2646	22	43	catalytic	catalytic	ADJ
cet-2646	22	44	center	center	NOUN
cet-2646	22	45	from	from	ADP
cet-2646	22	46	axial	axial	ADJ
cet-2646	22	47	orbit	orbit	NOUN
cet-2646	22	48	when	when	SCONJ
cet-2646	22	49	it	it	PRON
cet-2646	22	50	receives	receive	VERB
cet-2646	22	51	electrons	electron	NOUN
cet-2646	22	52	generated	generate	VERB
cet-2646	22	53	after	after	SCONJ
cet-2646	22	54	the	the	DET
cet-2646	22	55	sunlight	sunlight	NOUN
cet-2646	22	56	is	be	AUX
cet-2646	22	57	absorbed	absorb	VERB
cet-2646	22	58	by	by	ADP
cet-2646	22	59	the	the	DET
cet-2646	22	60	sensitizer	sensitizer	NOUN
cet-2646	22	61	.	.	PUNCT
cet-2646	23	1	620	620	NUM
cet-2646	23	2	under	under	ADP
cet-2646	23	3	the	the	DET
cet-2646	23	4	condition	condition	NOUN
cet-2646	23	5	that	that	SCONJ
cet-2646	23	6	the	the	DET
cet-2646	23	7	axial	axial	ADJ
cet-2646	23	8	ligand	ligand	NOUN
cet-2646	23	9	is	be	AUX
cet-2646	23	10	known	know	VERB
cet-2646	23	11	as	as	ADP
cet-2646	23	12	the	the	DET
cet-2646	23	13	means	mean	NOUN
cet-2646	23	14	for	for	ADP
cet-2646	23	15	[	[	PUNCT
cet-2646	23	16	co(dmgh)2pycl	co(dmgh)2pycl	ADJ
cet-2646	23	17	]	]	X
cet-2646	23	18	molecule	molecule	NOUN
cet-2646	23	19	to	to	PART
cet-2646	23	20	receive	receive	VERB
cet-2646	23	21	the	the	DET
cet-2646	23	22	electrons	electron	NOUN
cet-2646	23	23	,	,	PUNCT
cet-2646	23	24	we	we	PRON
cet-2646	23	25	have	have	AUX
cet-2646	23	26	tuned	tune	VERB
cet-2646	23	27	the	the	DET
cet-2646	23	28	axial	axial	ADJ
cet-2646	23	29	ligands	ligand	NOUN
cet-2646	23	30	of	of	ADP
cet-2646	23	31	the	the	DET
cet-2646	23	32	central	central	ADJ
cet-2646	23	33	co	co	NOUN
cet-2646	23	34	,	,	PUNCT
cet-2646	23	35	mainly	mainly	ADV
cet-2646	23	36	including	include	VERB
cet-2646	23	37	the	the	DET
cet-2646	23	38	ligand	ligand	ADJ
cet-2646	23	39	species	specie	NOUN
cet-2646	23	40	on	on	ADP
cet-2646	23	41	the	the	DET
cet-2646	23	42	pyridyl	pyridyl	PROPN
cet-2646	23	43	group	group	NOUN
cet-2646	23	44	.	.	PUNCT
cet-2646	24	1	it	it	PRON
cet-2646	24	2	is	be	AUX
cet-2646	24	3	found	find	VERB
cet-2646	24	4	that	that	SCONJ
cet-2646	24	5	when	when	SCONJ
cet-2646	24	6	the	the	DET
cet-2646	24	7	ligand	ligand	ADJ
cet-2646	24	8	groups	group	NOUN
cet-2646	24	9	on	on	ADP
cet-2646	24	10	pyridine	pyridine	NOUN
cet-2646	24	11	-ch3	-ch3	PROPN
cet-2646	24	12	,	,	PUNCT
cet-2646	24	13	-ch2ch3	-ch2ch3	ADJ
cet-2646	24	14	,	,	PUNCT
cet-2646	24	15	-oh	-oh	INTJ
cet-2646	24	16	,	,	PUNCT
cet-2646	24	17	-cn	-cn	VERB
cet-2646	24	18	and	and	CCONJ
cet-2646	24	19	-n	-n	X
cet-2646	24	20	(	(	PUNCT
cet-2646	24	21	ch3	ch3	PROPN
cet-2646	24	22	)	)	PUNCT
cet-2646	24	23	2	2	NUM
cet-2646	24	24	respectively	respectively	ADV
cet-2646	24	25	take	take	VERB
cet-2646	24	26	place	place	NOUN
cet-2646	24	27	of	of	ADP
cet-2646	24	28	the	the	DET
cet-2646	24	29	opposite	opposite	ADJ
cet-2646	24	30	group	group	NOUN
cet-2646	24	31	of	of	ADP
cet-2646	24	32	n	n	PROPN
cet-2646	24	33	on	on	ADP
cet-2646	24	34	the	the	DET
cet-2646	24	35	pyridine	pyridine	ADJ
cet-2646	24	36	ligand	ligand	NOUN
cet-2646	24	37	that	that	PRON
cet-2646	24	38	links	link	VERB
cet-2646	24	39	to	to	PART
cet-2646	24	40	co	co	VERB
cet-2646	24	41	,	,	PUNCT
cet-2646	24	42	the	the	DET
cet-2646	24	43	lumo	lumo	NOUN
cet-2646	24	44	orbit	orbit	NOUN
cet-2646	24	45	energy	energy	NOUN
cet-2646	24	46	level	level	NOUN
cet-2646	24	47	remains	remain	VERB
cet-2646	24	48	on	on	ADP
cet-2646	24	49	the	the	DET
cet-2646	24	50	pyridyl	pyridyl	PROPN
cet-2646	24	51	group	group	NOUN
cet-2646	24	52	.	.	PUNCT
cet-2646	25	1	in	in	ADP
cet-2646	25	2	this	this	DET
cet-2646	25	3	type	type	NOUN
cet-2646	25	4	of	of	ADP
cet-2646	25	5	axial	axial	ADJ
cet-2646	25	6	ligand	ligand	NOUN
cet-2646	25	7	cobalt	cobalt	NOUN
cet-2646	25	8	oxime	oxime	NOUN
cet-2646	25	9	molecule	molecule	NOUN
cet-2646	25	10	,	,	PUNCT
cet-2646	25	11	the	the	DET
cet-2646	25	12	electrons	electron	NOUN
cet-2646	25	13	enter	enter	VERB
cet-2646	25	14	the	the	DET
cet-2646	25	15	catalytic	catalytic	ADJ
cet-2646	25	16	center	center	NOUN
cet-2646	25	17	only	only	ADV
cet-2646	25	18	from	from	ADP
cet-2646	25	19	the	the	DET
cet-2646	25	20	axial	axial	ADJ
cet-2646	25	21	ligand	ligand	NOUN
cet-2646	25	22	.	.	PUNCT
cet-2646	26	1	in	in	ADP
cet-2646	26	2	the	the	DET
cet-2646	26	3	current	current	ADJ
cet-2646	26	4	studies	study	NOUN
cet-2646	26	5	on	on	ADP
cet-2646	26	6	the	the	DET
cet-2646	26	7	photocatalytic	photocatalytic	ADJ
cet-2646	26	8	water	water	NOUN
cet-2646	26	9	splitting	splitting	NOUN
cet-2646	26	10	system	system	NOUN
cet-2646	26	11	,	,	PUNCT
cet-2646	26	12	the	the	DET
cet-2646	26	13	principal	principal	ADJ
cet-2646	26	14	concerns	concern	NOUN
cet-2646	26	15	are	be	AUX
cet-2646	26	16	how	how	SCONJ
cet-2646	26	17	to	to	PART
cet-2646	26	18	improve	improve	VERB
cet-2646	26	19	the	the	DET
cet-2646	26	20	utilizations	utilization	NOUN
cet-2646	26	21	of	of	ADP
cet-2646	26	22	visible	visible	ADJ
cet-2646	26	23	light	light	NOUN
cet-2646	26	24	in	in	ADP
cet-2646	26	25	the	the	DET
cet-2646	26	26	sunlight	sunlight	NOUN
cet-2646	26	27	,	,	PUNCT
cet-2646	26	28	the	the	DET
cet-2646	26	29	rate	rate	NOUN
cet-2646	26	30	of	of	ADP
cet-2646	26	31	hydrogen	hydrogen	NOUN
cet-2646	26	32	production	production	NOUN
cet-2646	26	33	and	and	CCONJ
cet-2646	26	34	the	the	DET
cet-2646	26	35	quantum	quantum	NOUN
cet-2646	26	36	yield	yield	NOUN
cet-2646	26	37	.	.	PUNCT
cet-2646	27	1	the	the	DET
cet-2646	27	2	scholars	scholar	NOUN
cet-2646	27	3	still	still	ADV
cet-2646	27	4	resort	resort	VERB
cet-2646	27	5	to	to	ADP
cet-2646	27	6	the	the	DET
cet-2646	27	7	experimental	experimental	ADJ
cet-2646	27	8	approaches	approach	NOUN
cet-2646	27	9	in	in	ADP
cet-2646	27	10	this	this	DET
cet-2646	27	11	field	field	NOUN
cet-2646	27	12	(	(	PUNCT
cet-2646	27	13	young	young	ADJ
cet-2646	27	14	et	et	PROPN
cet-2646	27	15	al	al	PROPN
cet-2646	27	16	.	.	PROPN
cet-2646	27	17	,1975	,1975	PROPN
cet-2646	27	18	;	;	PUNCT
cet-2646	27	19	esswein	esswein	NOUN
cet-2646	27	20	and	and	CCONJ
cet-2646	27	21	nocera	nocera	PROPN
cet-2646	27	22	,	,	PUNCT
cet-2646	27	23	2007	2007	NUM
cet-2646	27	24	;	;	PUNCT
cet-2646	27	25	sun	sun	PROPN
cet-2646	27	26	et	et	PROPN
cet-2646	27	27	al	al	PROPN
cet-2646	27	28	.	.	PROPN
cet-2646	27	29	,	,	PUNCT
cet-2646	27	30	2001	2001	NUM
cet-2646	27	31	)	)	PUNCT
cet-2646	27	32	.	.	PUNCT
cet-2646	28	1	a	a	DET
cet-2646	28	2	catalysis	catalysis	NOUN
cet-2646	28	3	in	in	ADP
cet-2646	28	4	homogenous	homogenous	ADJ
cet-2646	28	5	system	system	NOUN
cet-2646	28	6	is	be	AUX
cet-2646	28	7	built	build	VERB
cet-2646	28	8	with	with	ADP
cet-2646	28	9	different	different	ADJ
cet-2646	28	10	catalyst	catalyst	NOUN
cet-2646	28	11	molecular	molecular	ADJ
cet-2646	28	12	structures	structure	NOUN
cet-2646	28	13	compatible	compatible	ADJ
cet-2646	28	14	with	with	ADP
cet-2646	28	15	different	different	ADJ
cet-2646	28	16	photosensitizers	photosensitizer	NOUN
cet-2646	28	17	,	,	PUNCT
cet-2646	28	18	sacrificial	sacrificial	ADJ
cet-2646	28	19	agents	agent	NOUN
cet-2646	28	20	and	and	CCONJ
cet-2646	28	21	solutions	solution	NOUN
cet-2646	28	22	,	,	PUNCT
cet-2646	28	23	as	as	SCONJ
cet-2646	28	24	developed	develop	VERB
cet-2646	28	25	,	,	PUNCT
cet-2646	28	26	to	to	PART
cet-2646	28	27	probe	probe	VERB
cet-2646	28	28	into	into	ADP
cet-2646	28	29	the	the	DET
cet-2646	28	30	law	law	NOUN
cet-2646	28	31	of	of	ADP
cet-2646	28	32	quantum	quantum	ADJ
cet-2646	28	33	yield	yield	NOUN
cet-2646	28	34	.	.	PUNCT
cet-2646	29	1	the	the	DET
cet-2646	29	2	most	most	ADV
cet-2646	29	3	efficient	efficient	ADJ
cet-2646	29	4	catalytic	catalytic	ADJ
cet-2646	29	5	hydrogen	hydrogen	NOUN
cet-2646	29	6	production	production	NOUN
cet-2646	29	7	system	system	NOUN
cet-2646	29	8	reported	report	VERB
cet-2646	29	9	in	in	ADP
cet-2646	29	10	the	the	DET
cet-2646	29	11	literature	literature	NOUN
cet-2646	29	12	is	be	AUX
cet-2646	29	13	:	:	PUNCT
cet-2646	29	14	[	[	X
cet-2646	29	15	co	co	INTJ
cet-2646	29	16	(	(	PUNCT
cet-2646	29	17	dmgh	dmgh	NOUN
cet-2646	29	18	)	)	PUNCT
cet-2646	30	1	2pycl	2pycl	NUM
cet-2646	30	2	]	]	X
cet-2646	30	3	as	as	ADP
cet-2646	30	4	a	a	DET
cet-2646	30	5	catalyst	catalyst	NOUN
cet-2646	30	6	,	,	PUNCT
cet-2646	30	7	pt	pt	X
cet-2646	30	8	(	(	PUNCT
cet-2646	30	9	ttpy	ttpy	NOUN
cet-2646	30	10	)	)	PUNCT
cet-2646	30	11	(	(	PUNCT
cet-2646	30	12	c≡cph	c≡cph	PROPN
cet-2646	30	13	)	)	PUNCT
cet-2646	30	14	clo4	clo4	PROPN
cet-2646	30	15	as	as	ADP
cet-2646	30	16	a	a	DET
cet-2646	30	17	dye	dye	NOUN
cet-2646	30	18	and	and	CCONJ
cet-2646	30	19	triethanolamine	triethanolamine	NOUN
cet-2646	30	20	teoa	teoa	VERB
cet-2646	30	21	(	(	PUNCT
cet-2646	30	22	0.27	0.27	NUM
cet-2646	30	23	m	m	NOUN
cet-2646	30	24	)	)	PUNCT
cet-2646	30	25	as	as	ADP
cet-2646	30	26	a	a	DET
cet-2646	30	27	cytoplasm	cytoplasm	NOUN
cet-2646	30	28	.	.	PUNCT
cet-2646	31	1	after	after	ADP
cet-2646	31	2	an	an	DET
cet-2646	31	3	irradiation	irradiation	NOUN
cet-2646	31	4	of	of	ADP
cet-2646	31	5	10	10	NUM
cet-2646	31	6	hours	hour	NOUN
cet-2646	31	7	at	at	ADP
cet-2646	31	8	λ	λ	X
cet-2646	31	9	>	>	X
cet-2646	31	10	410	410	NUM
cet-2646	31	11	nm	nm	NOUN
cet-2646	31	12	,	,	PUNCT
cet-2646	31	13	the	the	DET
cet-2646	31	14	catalytic	catalytic	ADJ
cet-2646	31	15	hydrogen	hydrogen	NOUN
cet-2646	31	16	production	production	NOUN
cet-2646	31	17	can	can	AUX
cet-2646	31	18	reach	reach	VERB
cet-2646	31	19	up	up	ADP
cet-2646	31	20	to	to	ADP
cet-2646	31	21	about	about	ADP
cet-2646	31	22	2150	2150	NUM
cet-2646	31	23	cycles	cycle	NOUN
cet-2646	31	24	.	.	PUNCT
cet-2646	32	1	however	however	ADV
cet-2646	32	2	,	,	PUNCT
cet-2646	32	3	the	the	DET
cet-2646	32	4	lack	lack	NOUN
cet-2646	32	5	of	of	ADP
cet-2646	32	6	theoretical	theoretical	ADJ
cet-2646	32	7	study	study	NOUN
cet-2646	32	8	on	on	ADP
cet-2646	32	9	the	the	DET
cet-2646	32	10	charge	charge	NOUN
cet-2646	32	11	transport	transport	NOUN
cet-2646	32	12	path	path	NOUN
cet-2646	32	13	and	and	CCONJ
cet-2646	32	14	its	its	PRON
cet-2646	32	15	mechanism	mechanism	NOUN
cet-2646	32	16	in	in	ADP
cet-2646	32	17	catalytic	catalytic	ADJ
cet-2646	32	18	hydrogen	hydrogen	NOUN
cet-2646	32	19	production	production	NOUN
cet-2646	32	20	badly	badly	ADV
cet-2646	32	21	restricts	restrict	VERB
cet-2646	32	22	the	the	DET
cet-2646	32	23	hydrogen	hydrogen	NOUN
cet-2646	32	24	production	production	NOUN
cet-2646	32	25	efficiency	efficiency	NOUN
cet-2646	32	26	.	.	PUNCT
cet-2646	33	1	in	in	ADP
cet-2646	33	2	many	many	ADJ
cet-2646	33	3	experiments	experiment	NOUN
cet-2646	33	4	,	,	PUNCT
cet-2646	33	5	it	it	PRON
cet-2646	33	6	is	be	AUX
cet-2646	33	7	proposed	propose	VERB
cet-2646	33	8	that	that	SCONJ
cet-2646	33	9	the	the	DET
cet-2646	33	10	catalytic	catalytic	ADJ
cet-2646	33	11	hydrogen	hydrogen	NOUN
cet-2646	33	12	production	production	NOUN
cet-2646	33	13	cycle	cycle	NOUN
cet-2646	33	14	of	of	ADP
cet-2646	33	15	cobalt	cobalt	NOUN
cet-2646	33	16	oxime	oxime	NOUN
cet-2646	33	17	molecules	molecule	NOUN
cet-2646	33	18	is	be	AUX
cet-2646	33	19	a	a	DET
cet-2646	33	20	process	process	NOUN
cet-2646	33	21	related	relate	VERB
cet-2646	33	22	to	to	ADP
cet-2646	33	23	the	the	DET
cet-2646	33	24	change	change	NOUN
cet-2646	33	25	of	of	ADP
cet-2646	33	26	the	the	DET
cet-2646	33	27	co	co	NOUN
cet-2646	33	28	charge	charge	NOUN
cet-2646	33	29	.	.	PUNCT
cet-2646	34	1	the	the	DET
cet-2646	34	2	change	change	NOUN
cet-2646	34	3	of	of	ADP
cet-2646	34	4	the	the	DET
cet-2646	34	5	cobalt	cobalt	NOUN
cet-2646	34	6	price	price	NOUN
cet-2646	34	7	level	level	NOUN
cet-2646	34	8	measured	measure	VERB
cet-2646	34	9	by	by	ADP
cet-2646	34	10	the	the	DET
cet-2646	34	11	cyclic	cyclic	ADJ
cet-2646	34	12	voltammetry	voltammetry	NOUN
cet-2646	34	13	is	be	AUX
cet-2646	34	14	based	base	VERB
cet-2646	34	15	on	on	ADP
cet-2646	34	16	to	to	PART
cet-2646	34	17	predict	predict	VERB
cet-2646	34	18	the	the	DET
cet-2646	34	19	results	result	NOUN
cet-2646	34	20	of	of	ADP
cet-2646	34	21	hydrogen	hydrogen	NOUN
cet-2646	34	22	production	production	NOUN
cet-2646	34	23	by	by	ADP
cet-2646	34	24	catalytic	catalytic	ADJ
cet-2646	34	25	cobalt	cobalt	NOUN
cet-2646	34	26	oximes	oxime	NOUN
cet-2646	34	27	.	.	PUNCT
cet-2646	35	1	for	for	ADP
cet-2646	35	2	the	the	DET
cet-2646	35	3	mechanism	mechanism	NOUN
cet-2646	35	4	of	of	ADP
cet-2646	35	5	photocatalytic	photocatalytic	ADJ
cet-2646	35	6	hydrogen	hydrogen	NOUN
cet-2646	35	7	production	production	NOUN
cet-2646	35	8	by	by	ADP
cet-2646	35	9	cobalt	cobalt	NOUN
cet-2646	35	10	oximes	oxime	NOUN
cet-2646	35	11	,	,	PUNCT
cet-2646	35	12	most	most	ADJ
cet-2646	35	13	of	of	ADP
cet-2646	35	14	the	the	DET
cet-2646	35	15	studies	study	NOUN
cet-2646	35	16	resort	resort	VERB
cet-2646	35	17	to	to	ADP
cet-2646	35	18	the	the	DET
cet-2646	35	19	cyclic	cyclic	ADJ
cet-2646	35	20	voltammetry	voltammetry	NOUN
cet-2646	35	21	to	to	PART
cet-2646	35	22	predict	predict	VERB
cet-2646	35	23	the	the	DET
cet-2646	35	24	catalytic	catalytic	ADJ
cet-2646	35	25	hydrogen	hydrogen	NOUN
cet-2646	35	26	production	production	NOUN
cet-2646	35	27	path	path	NOUN
cet-2646	35	28	based	base	VERB
cet-2646	35	29	on	on	ADP
cet-2646	35	30	the	the	DET
cet-2646	35	31	change	change	NOUN
cet-2646	35	32	of	of	ADP
cet-2646	35	33	metal	metal	NOUN
cet-2646	35	34	cobalt	cobalt	NOUN
cet-2646	35	35	price	price	NOUN
cet-2646	35	36	level	level	NOUN
cet-2646	35	37	in	in	ADP
cet-2646	35	38	the	the	DET
cet-2646	35	39	ligand	ligand	ADJ
cet-2646	35	40	center	center	NOUN
cet-2646	35	41	.	.	PUNCT
cet-2646	36	1	in	in	ADP
cet-2646	36	2	the	the	DET
cet-2646	36	3	process	process	NOUN
cet-2646	36	4	of	of	ADP
cet-2646	36	5	hydrogen	hydrogen	NOUN
cet-2646	36	6	reaction	reaction	NOUN
cet-2646	36	7	,	,	PUNCT
cet-2646	36	8	cobalt	cobalt	NOUN
cet-2646	36	9	coiii	coiii	NOUN
cet-2646	36	10	ligands	ligand	NOUN
cet-2646	36	11	,	,	PUNCT
cet-2646	36	12	in	in	ADP
cet-2646	36	13	turn	turn	NOUN
cet-2646	36	14	,	,	PUNCT
cet-2646	36	15	generate	generate	VERB
cet-2646	36	16	divalent	divalent	NOUN
cet-2646	36	17	and	and	CCONJ
cet-2646	36	18	monovalent	monovalent	NOUN
cet-2646	36	19	cobalt	cobalt	NOUN
cet-2646	36	20	coii	coii	NOUN
cet-2646	36	21	and	and	CCONJ
cet-2646	36	22	coi	coi	NOUN
cet-2646	36	23	midbodies	midbodie	NOUN
cet-2646	36	24	by	by	ADP
cet-2646	36	25	the	the	DET
cet-2646	36	26	reduction	reduction	NOUN
cet-2646	36	27	of	of	ADP
cet-2646	36	28	two	two	NUM
cet-2646	36	29	single	single	ADJ
cet-2646	36	30	electrons	electron	NOUN
cet-2646	36	31	,	,	PUNCT
cet-2646	36	32	where	where	SCONJ
cet-2646	36	33	the	the	DET
cet-2646	36	34	coi	coi	NOUN
cet-2646	36	35	midbody	midbody	NOUN
cet-2646	36	36	is	be	AUX
cet-2646	36	37	a	a	DET
cet-2646	36	38	key	key	ADJ
cet-2646	36	39	intermediate	intermediate	ADJ
cet-2646	36	40	product	product	NOUN
cet-2646	36	41	in	in	ADP
cet-2646	36	42	the	the	DET
cet-2646	36	43	hydrogen	hydrogen	NOUN
cet-2646	36	44	production	production	NOUN
cet-2646	36	45	process	process	NOUN
cet-2646	36	46	.	.	PUNCT
cet-2646	37	1	a	a	DET
cet-2646	37	2	nucleophilic	nucleophilic	ADJ
cet-2646	37	3	coi	coi	NOUN
cet-2646	37	4	midbody	midbody	NOUN
cet-2646	37	5	interacts	interact	VERB
cet-2646	37	6	with	with	ADP
cet-2646	37	7	protons	proton	NOUN
cet-2646	37	8	to	to	PART
cet-2646	37	9	form	form	VERB
cet-2646	37	10	hydride	hydride	NOUN
cet-2646	37	11	coiiih	coiiih	NOUN
cet-2646	37	12	,	,	PUNCT
cet-2646	37	13	namely	namely	ADV
cet-2646	37	14	:	:	PUNCT
cet-2646	37	15	coiii	coiii	X
cet-2646	37	16	+	+	CCONJ
cet-2646	37	17	e-1	e-1	PROPN
cet-2646	37	18	→	→	SYM
cet-2646	37	19	coii	coii	PROPN
cet-2646	37	20	;	;	PUNCT
cet-2646	37	21	coii	coii	PROPN
cet-2646	37	22	+	+	CCONJ
cet-2646	37	23	e-1	e-1	PROPN
cet-2646	37	24	→	→	SYM
cet-2646	37	25	coi	coi	NOUN
cet-2646	37	26	;	;	PUNCT
cet-2646	37	27	coi	coi	NOUN
cet-2646	37	28	+	+	CCONJ
cet-2646	37	29	h+	h+	X
cet-2646	37	30	→	→	SYM
cet-2646	37	31	coiiih	coiiih	NOUN
cet-2646	37	32	subsequently	subsequently	ADV
cet-2646	37	33	,	,	PUNCT
cet-2646	37	34	the	the	DET
cet-2646	37	35	path	path	NOUN
cet-2646	37	36	for	for	ADP
cet-2646	37	37	catalytic	catalytic	ADJ
cet-2646	37	38	hydrogen	hydrogen	NOUN
cet-2646	37	39	production	production	NOUN
cet-2646	37	40	is	be	AUX
cet-2646	37	41	not	not	PART
cet-2646	37	42	unique	unique	ADJ
cet-2646	37	43	.	.	PUNCT
cet-2646	38	1	currently	currently	ADV
cet-2646	38	2	,	,	PUNCT
cet-2646	38	3	there	there	PRON
cet-2646	38	4	are	be	VERB
cet-2646	38	5	two	two	NUM
cet-2646	38	6	hydrogen	hydrogen	NOUN
cet-2646	38	7	production	production	NOUN
cet-2646	38	8	mechanisms	mechanism	NOUN
cet-2646	38	9	available	available	ADJ
cet-2646	38	10	by	by	ADP
cet-2646	38	11	everyone	everyone	PRON
cet-2646	38	12	,	,	PUNCT
cet-2646	38	13	i.e.	i.e.	X
cet-2646	38	14	monometallic	monometallic	ADJ
cet-2646	38	15	and	and	CCONJ
cet-2646	38	16	bimetallic	bimetallic	ADJ
cet-2646	38	17	mechanisms	mechanism	NOUN
cet-2646	38	18	.	.	PUNCT
cet-2646	39	1	in	in	ADP
cet-2646	39	2	the	the	DET
cet-2646	39	3	first	first	ADJ
cet-2646	39	4	place	place	NOUN
cet-2646	39	5	,	,	PUNCT
cet-2646	39	6	co	co	X
cet-2646	39	7	(	(	PUNCT
cet-2646	39	8	iii	iii	NOUN
cet-2646	39	9	)	)	PUNCT
cet-2646	39	10	hydride	hydride	NOUN
cet-2646	39	11	can	can	AUX
cet-2646	39	12	produce	produce	VERB
cet-2646	39	13	hydrogen	hydrogen	NOUN
cet-2646	39	14	and	and	CCONJ
cet-2646	39	15	a	a	DET
cet-2646	39	16	co	co	X
cet-2646	39	17	(	(	PUNCT
cet-2646	39	18	iii	iii	NOUN
cet-2646	39	19	)	)	PUNCT
cet-2646	39	20	by	by	ADP
cet-2646	39	21	further	further	ADJ
cet-2646	39	22	proton	proton	NOUN
cet-2646	39	23	addition	addition	NOUN
cet-2646	39	24	,	,	PUNCT
cet-2646	39	25	or	or	CCONJ
cet-2646	39	26	co	co	ADJ
cet-2646	39	27	(	(	PUNCT
cet-2646	39	28	iii	iii	NOUN
cet-2646	39	29	)	)	PUNCT
cet-2646	39	30	hydride	hydride	NOUN
cet-2646	39	31	is	be	AUX
cet-2646	39	32	further	far	ADV
cet-2646	39	33	restored	restore	VERB
cet-2646	39	34	to	to	PART
cet-2646	39	35	co	co	PROPN
cet-2646	39	36	(	(	PUNCT
cet-2646	39	37	ii	ii	NOUN
cet-2646	39	38	)	)	PUNCT
cet-2646	39	39	and	and	CCONJ
cet-2646	39	40	produce	produce	VERB
cet-2646	39	41	hydrogen	hydrogen	NOUN
cet-2646	39	42	and	and	CCONJ
cet-2646	39	43	one	one	NUM
cet-2646	39	44	co	co	X
cet-2646	39	45	(	(	PUNCT
cet-2646	39	46	ii	ii	NOUN
cet-2646	39	47	)	)	PUNCT
cet-2646	39	48	by	by	ADP
cet-2646	39	49	proton	proton	NOUN
cet-2646	39	50	addition	addition	NOUN
cet-2646	39	51	,	,	PUNCT
cet-2646	39	52	so	so	SCONJ
cet-2646	39	53	that	that	SCONJ
cet-2646	39	54	the	the	DET
cet-2646	39	55	monometallic	monometallic	PROPN
cet-2646	39	56	catalysis	catalysis	NOUN
cet-2646	39	57	mechanism	mechanism	NOUN
cet-2646	39	58	is	be	AUX
cet-2646	39	59	achieved	achieve	VERB
cet-2646	39	60	;	;	PUNCT
cet-2646	39	61	the	the	DET
cet-2646	39	62	other	other	ADJ
cet-2646	39	63	path	path	NOUN
cet-2646	39	64	is	be	AUX
cet-2646	39	65	that	that	SCONJ
cet-2646	39	66	hydrogen	hydrogen	NOUN
cet-2646	39	67	and	and	CCONJ
cet-2646	39	68	two	two	NUM
cet-2646	39	69	co	co	X
cet-2646	39	70	(	(	PUNCT
cet-2646	39	71	ii	ii	NOUN
cet-2646	39	72	)	)	PUNCT
cet-2646	39	73	are	be	AUX
cet-2646	39	74	produced	produce	VERB
cet-2646	39	75	by	by	ADP
cet-2646	39	76	the	the	DET
cet-2646	39	77	reaction	reaction	NOUN
cet-2646	39	78	of	of	ADP
cet-2646	39	79	two	two	NUM
cet-2646	39	80	co	co	X
cet-2646	39	81	(	(	PUNCT
cet-2646	39	82	iii	iii	NOUN
cet-2646	39	83	)	)	PUNCT
cet-2646	39	84	hydrides	hydride	NOUN
cet-2646	39	85	.	.	PUNCT
cet-2646	40	1	although	although	SCONJ
cet-2646	40	2	the	the	DET
cet-2646	40	3	latter	latter	ADJ
cet-2646	40	4	path	path	NOUN
cet-2646	40	5	seems	seem	VERB
cet-2646	40	6	to	to	PART
cet-2646	40	7	be	be	AUX
cet-2646	40	8	fully	fully	ADV
cet-2646	40	9	feasible	feasible	ADJ
cet-2646	40	10	in	in	ADP
cet-2646	40	11	chemical	chemical	ADJ
cet-2646	40	12	experiments	experiment	NOUN
cet-2646	40	13	,	,	PUNCT
cet-2646	40	14	it	it	PRON
cet-2646	40	15	is	be	AUX
cet-2646	40	16	more	more	ADV
cet-2646	40	17	difficult	difficult	ADJ
cet-2646	40	18	to	to	PART
cet-2646	40	19	work	work	VERB
cet-2646	40	20	out	out	ADP
cet-2646	40	21	the	the	DET
cet-2646	40	22	computational	computational	ADJ
cet-2646	40	23	simulation	simulation	NOUN
cet-2646	40	24	and	and	CCONJ
cet-2646	40	25	get	get	VERB
cet-2646	40	26	experimentally	experimentally	ADV
cet-2646	40	27	relevant	relevant	ADJ
cet-2646	40	28	information	information	NOUN
cet-2646	40	29	.	.	PUNCT
cet-2646	41	1	in	in	ADP
cet-2646	41	2	the	the	DET
cet-2646	41	3	study	study	NOUN
cet-2646	41	4	,	,	PUNCT
cet-2646	41	5	we	we	PRON
cet-2646	41	6	mainly	mainly	ADV
cet-2646	41	7	use	use	VERB
cet-2646	41	8	the	the	DET
cet-2646	41	9	computational	computational	ADJ
cet-2646	41	10	simulation	simulation	NOUN
cet-2646	41	11	to	to	PART
cet-2646	41	12	simulate	simulate	VERB
cet-2646	41	13	and	and	CCONJ
cet-2646	41	14	calculate	calculate	VERB
cet-2646	41	15	the	the	DET
cet-2646	41	16	catalytic	catalytic	ADJ
cet-2646	41	17	mechanism	mechanism	NOUN
cet-2646	41	18	of	of	ADP
cet-2646	41	19	the	the	DET
cet-2646	41	20	monometal	monometal	ADJ
cet-2646	41	21	in	in	ADP
cet-2646	41	22	order	order	NOUN
cet-2646	41	23	to	to	PART
cet-2646	41	24	obtain	obtain	VERB
cet-2646	41	25	a	a	DET
cet-2646	41	26	series	series	NOUN
cet-2646	41	27	of	of	ADP
cet-2646	41	28	physical	physical	ADJ
cet-2646	41	29	information	information	NOUN
cet-2646	41	30	about	about	ADP
cet-2646	41	31	midbodies	midbodie	NOUN
cet-2646	41	32	in	in	ADP
cet-2646	41	33	the	the	DET
cet-2646	41	34	process	process	NOUN
cet-2646	41	35	of	of	ADP
cet-2646	41	36	catalytic	catalytic	ADJ
cet-2646	41	37	hydrogen	hydrogen	NOUN
cet-2646	41	38	production	production	NOUN
cet-2646	41	39	.	.	PUNCT
cet-2646	42	1	however	however	ADV
cet-2646	42	2	,	,	PUNCT
cet-2646	42	3	these	these	DET
cet-2646	42	4	intermediate	intermediate	ADJ
cet-2646	42	5	products	product	NOUN
cet-2646	42	6	are	be	AUX
cet-2646	42	7	hardly	hardly	ADV
cet-2646	42	8	found	find	VERB
cet-2646	42	9	and	and	CCONJ
cet-2646	42	10	recorded	record	VERB
cet-2646	42	11	in	in	ADP
cet-2646	42	12	the	the	DET
cet-2646	42	13	lab	lab	NOUN
cet-2646	42	14	.	.	PUNCT
cet-2646	43	1	in	in	ADP
cet-2646	43	2	the	the	DET
cet-2646	43	3	monometallic	monometallic	PROPN
cet-2646	43	4	catalyst	catalyst	NOUN
cet-2646	43	5	path	path	NOUN
cet-2646	43	6	,	,	PUNCT
cet-2646	43	7	the	the	DET
cet-2646	43	8	hydride	hydride	NOUN
cet-2646	43	9	coiiih	coiiih	NOUN
cet-2646	43	10	charged	charge	VERB
cet-2646	43	11	hydrogen	hydrogen	NOUN
cet-2646	43	12	production	production	NOUN
cet-2646	43	13	process	process	NOUN
cet-2646	43	14	also	also	ADV
cet-2646	43	15	has	have	VERB
cet-2646	43	16	two	two	NUM
cet-2646	43	17	ways	way	NOUN
cet-2646	43	18	,	,	PUNCT
cet-2646	43	19	namely	namely	ADV
cet-2646	43	20	:	:	PUNCT
cet-2646	43	21	monometallic	monometallic	PROPN
cet-2646	43	22	pathways	pathway	NOUN
cet-2646	44	1	a	a	DET
cet-2646	44	2	+	+	X
cet-2646	44	3	→	→	SYM
cet-2646	44	4	+	+	ADJ
cet-2646	44	5	+	+	SYM
cet-2646	44	6	b	b	NOUN
cet-2646	44	7	+	+	CCONJ
cet-2646	44	8	+	+	CCONJ
cet-2646	44	9	→+	→+	NOUN
cet-2646	44	10	→	→	SYM
cet-2646	44	11	+	+	CCONJ
cet-2646	44	12	based	base	VERB
cet-2646	44	13	on	on	ADP
cet-2646	44	14	the	the	DET
cet-2646	44	15	monometallic	monometallic	PROPN
cet-2646	44	16	catalysis	catalysis	NOUN
cet-2646	44	17	,	,	PUNCT
cet-2646	44	18	this	this	DET
cet-2646	44	19	study	study	NOUN
cet-2646	44	20	uses	use	VERB
cet-2646	44	21	gaussian	gaussian	ADJ
cet-2646	44	22	computational	computational	ADJ
cet-2646	44	23	simulation	simulation	NOUN
cet-2646	44	24	to	to	PART
cet-2646	44	25	simulate	simulate	VERB
cet-2646	44	26	the	the	DET
cet-2646	44	27	transport	transport	NOUN
cet-2646	44	28	path	path	NOUN
cet-2646	44	29	of	of	ADP
cet-2646	44	30	the	the	DET
cet-2646	44	31	charge	charge	NOUN
cet-2646	44	32	,	,	PUNCT
cet-2646	44	33	as	as	SCONJ
cet-2646	44	34	shown	show	VERB
cet-2646	44	35	below	below	ADV
cet-2646	44	36	:	:	PUNCT
cet-2646	44	37	figure	figure	VERB
cet-2646	44	38	3	3	NUM
cet-2646	44	39	:	:	PUNCT
cet-2646	44	40	schematic	schematic	ADJ
cet-2646	44	41	diagram	diagram	NOUN
cet-2646	44	42	of	of	ADP
cet-2646	44	43	computational	computational	ADJ
cet-2646	44	44	simulation	simulation	NOUN
cet-2646	44	45	621	621	NUM
cet-2646	44	46	3	3	NUM
cet-2646	44	47	.	.	X
cet-2646	44	48	discussion	discussion	NOUN
cet-2646	44	49	the	the	DET
cet-2646	44	50	catalytic	catalytic	ADJ
cet-2646	44	51	cycle	cycle	NOUN
cet-2646	44	52	diagram	diagram	NOUN
cet-2646	44	53	is	be	AUX
cet-2646	44	54	the	the	DET
cet-2646	44	55	result	result	NOUN
cet-2646	44	56	of	of	ADP
cet-2646	44	57	a	a	DET
cet-2646	44	58	simulation	simulation	NOUN
cet-2646	44	59	.	.	PUNCT
cet-2646	45	1	as	as	SCONJ
cet-2646	45	2	can	can	AUX
cet-2646	45	3	be	be	AUX
cet-2646	45	4	seen	see	VERB
cet-2646	45	5	from	from	ADP
cet-2646	45	6	the	the	DET
cet-2646	45	7	figure	figure	NOUN
cet-2646	45	8	,	,	PUNCT
cet-2646	45	9	the	the	DET
cet-2646	45	10	trivalent	trivalent	NOUN
cet-2646	45	11	coiii	coiii	VERB
cet-2646	45	12	complex	complex	NOUN
cet-2646	45	13	absorbs	absorb	VERB
cet-2646	45	14	photo	photo	NOUN
cet-2646	45	15	-	-	PUNCT
cet-2646	45	16	induced	induce	VERB
cet-2646	45	17	electrons	electron	NOUN
cet-2646	45	18	and	and	CCONJ
cet-2646	45	19	becomes	become	VERB
cet-2646	45	20	a	a	DET
cet-2646	45	21	bivalent	bivalent	NOUN
cet-2646	45	22	coii	coii	NOUN
cet-2646	45	23	.	.	PUNCT
cet-2646	46	1	at	at	ADP
cet-2646	46	2	this	this	DET
cet-2646	46	3	time	time	NOUN
cet-2646	46	4	,	,	PUNCT
cet-2646	46	5	the	the	DET
cet-2646	46	6	axial	axial	ADJ
cet-2646	46	7	ligand	ligand	NOUN
cet-2646	46	8	cl	cl	NOUN
cet-2646	46	9	group	group	NOUN
cet-2646	46	10	breaks	break	VERB
cet-2646	46	11	away	away	ADV
cet-2646	46	12	from	from	ADP
cet-2646	46	13	the	the	DET
cet-2646	46	14	catalyst	catalyst	NOUN
cet-2646	46	15	center	center	NOUN
cet-2646	46	16	and	and	CCONJ
cet-2646	46	17	the	the	DET
cet-2646	46	18	divalent	divalent	NOUN
cet-2646	46	19	coii	coii	NOUN
cet-2646	46	20	complex	complex	ADJ
cet-2646	46	21	enters	enter	VERB
cet-2646	46	22	the	the	DET
cet-2646	46	23	true	true	ADJ
cet-2646	46	24	process	process	NOUN
cet-2646	46	25	of	of	ADP
cet-2646	46	26	catalytic	catalytic	ADJ
cet-2646	46	27	cycle	cycle	NOUN
cet-2646	46	28	.	.	PUNCT
cet-2646	47	1	as	as	SCONJ
cet-2646	47	2	shown	show	VERB
cet-2646	47	3	in	in	ADP
cet-2646	47	4	the	the	DET
cet-2646	47	5	figure	figure	NOUN
cet-2646	47	6	,	,	PUNCT
cet-2646	47	7	when	when	SCONJ
cet-2646	47	8	the	the	DET
cet-2646	47	9	catalytic	catalytic	ADJ
cet-2646	47	10	cycle	cycle	NOUN
cet-2646	47	11	is	be	AUX
cet-2646	47	12	ended	end	VERB
cet-2646	47	13	,	,	PUNCT
cet-2646	47	14	coii	coii	ADJ
cet-2646	47	15	complex	complex	NOUN
cet-2646	47	16	is	be	AUX
cet-2646	47	17	returned	return	VERB
cet-2646	47	18	;	;	PUNCT
cet-2646	47	19	the	the	DET
cet-2646	47	20	divalent	divalent	NOUN
cet-2646	47	21	coii	coii	NOUN
cet-2646	47	22	complex	complex	NOUN
cet-2646	47	23	continues	continue	VERB
cet-2646	47	24	to	to	PART
cet-2646	47	25	absorb	absorb	VERB
cet-2646	47	26	electrons	electron	NOUN
cet-2646	47	27	and	and	CCONJ
cet-2646	47	28	convert	convert	VERB
cet-2646	47	29	into	into	ADP
cet-2646	47	30	the	the	DET
cet-2646	47	31	monovalent	monovalent	NOUN
cet-2646	47	32	coi	coi	NOUN
cet-2646	47	33	complex	complex	NOUN
cet-2646	47	34	which	which	PRON
cet-2646	47	35	is	be	AUX
cet-2646	47	36	also	also	ADV
cet-2646	47	37	obviously	obviously	ADV
cet-2646	47	38	nucleophilic	nucleophilic	ADJ
cet-2646	47	39	to	to	PART
cet-2646	47	40	absorb	absorb	VERB
cet-2646	47	41	protons	proton	NOUN
cet-2646	47	42	,	,	PUNCT
cet-2646	47	43	generating	generate	VERB
cet-2646	47	44	trivalent	trivalent	NOUN
cet-2646	47	45	hydride	hydride	NOUN
cet-2646	47	46	coiiih	coiiih	NOUN
cet-2646	47	47	as	as	ADP
cet-2646	47	48	a	a	DET
cet-2646	47	49	key	key	ADJ
cet-2646	47	50	intermediate	intermediate	ADJ
cet-2646	47	51	product	product	NOUN
cet-2646	47	52	in	in	ADP
cet-2646	47	53	catalytic	catalytic	ADJ
cet-2646	47	54	hydrogen	hydrogen	NOUN
cet-2646	47	55	production	production	NOUN
cet-2646	47	56	,	,	PUNCT
cet-2646	47	57	and	and	CCONJ
cet-2646	47	58	difficult	difficult	ADJ
cet-2646	47	59	to	to	PART
cet-2646	47	60	be	be	AUX
cet-2646	47	61	observed	observe	VERB
cet-2646	47	62	in	in	ADP
cet-2646	47	63	the	the	DET
cet-2646	47	64	lab	lab	NOUN
cet-2646	47	65	but	but	CCONJ
cet-2646	47	66	clearly	clearly	ADV
cet-2646	47	67	visible	visible	ADJ
cet-2646	47	68	about	about	ADP
cet-2646	47	69	its	its	PRON
cet-2646	47	70	physical	physical	ADJ
cet-2646	47	71	properties	property	NOUN
cet-2646	47	72	in	in	ADP
cet-2646	47	73	the	the	DET
cet-2646	47	74	simulation	simulation	NOUN
cet-2646	47	75	;	;	PUNCT
cet-2646	47	76	then	then	ADV
cet-2646	47	77	the	the	DET
cet-2646	47	78	coiiih	coiiih	NOUN
cet-2646	47	79	hydride	hydride	NOUN
cet-2646	47	80	continues	continue	VERB
cet-2646	47	81	to	to	PART
cet-2646	47	82	react	react	VERB
cet-2646	47	83	with	with	ADP
cet-2646	47	84	protons	proton	NOUN
cet-2646	47	85	or	or	CCONJ
cet-2646	47	86	electrons	electron	NOUN
cet-2646	47	87	.	.	PUNCT
cet-2646	48	1	this	this	DET
cet-2646	48	2	reaction	reaction	NOUN
cet-2646	48	3	depends	depend	VERB
cet-2646	48	4	on	on	ADP
cet-2646	48	5	the	the	DET
cet-2646	48	6	acidic	acidic	ADJ
cet-2646	48	7	conditions	condition	NOUN
cet-2646	48	8	of	of	ADP
cet-2646	48	9	the	the	DET
cet-2646	48	10	photocatalysis	photocatalysis	NOUN
cet-2646	48	11	system	system	NOUN
cet-2646	48	12	.	.	PUNCT
cet-2646	49	1	when	when	SCONJ
cet-2646	49	2	the	the	DET
cet-2646	49	3	acidity	acidity	NOUN
cet-2646	49	4	is	be	AUX
cet-2646	49	5	strong	strong	ADJ
cet-2646	49	6	,	,	PUNCT
cet-2646	49	7	coiiih	coiiih	NOUN
cet-2646	49	8	hydride	hydride	NOUN
cet-2646	49	9	reacts	react	VERB
cet-2646	49	10	with	with	ADP
cet-2646	49	11	the	the	DET
cet-2646	49	12	protons	proton	NOUN
cet-2646	49	13	to	to	PART
cet-2646	49	14	generate	generate	VERB
cet-2646	49	15	coiii	coiii	NOUN
cet-2646	49	16	(	(	PUNCT
cet-2646	49	17	h2	h2	NOUN
cet-2646	49	18	)	)	PUNCT
cet-2646	49	19	.	.	PUNCT
cet-2646	50	1	in	in	ADP
cet-2646	50	2	fact	fact	NOUN
cet-2646	50	3	,	,	PUNCT
cet-2646	50	4	hydrogen	hydrogen	NOUN
cet-2646	50	5	has	have	AUX
cet-2646	50	6	been	be	AUX
cet-2646	50	7	generated	generate	VERB
cet-2646	50	8	now	now	ADV
cet-2646	50	9	.	.	PUNCT
cet-2646	51	1	when	when	SCONJ
cet-2646	51	2	h2	h2	PROPN
cet-2646	51	3	is	be	AUX
cet-2646	51	4	far	far	ADV
cet-2646	51	5	away	away	ADV
cet-2646	51	6	from	from	ADP
cet-2646	51	7	the	the	DET
cet-2646	51	8	catalytic	catalytic	ADJ
cet-2646	51	9	center	center	NOUN
cet-2646	51	10	co	co	VERB
cet-2646	51	11	by	by	ADP
cet-2646	51	12	a	a	DET
cet-2646	51	13	distance	distance	NOUN
cet-2646	51	14	of	of	ADP
cet-2646	51	15	5	5	NUM
cet-2646	51	16	å	å	NOUN
cet-2646	51	17	,	,	PUNCT
cet-2646	51	18	the	the	DET
cet-2646	51	19	energy	energy	NOUN
cet-2646	51	20	change	change	NOUN
cet-2646	51	21	is	be	AUX
cet-2646	51	22	negligible	negligible	ADJ
cet-2646	51	23	and	and	CCONJ
cet-2646	51	24	the	the	DET
cet-2646	51	25	trivalent	trivalent	NOUN
cet-2646	51	26	coiii	coiii	NOUN
cet-2646	51	27	complex	complex	NOUN
cet-2646	51	28	continues	continue	VERB
cet-2646	51	29	to	to	PART
cet-2646	51	30	absorb	absorb	VERB
cet-2646	51	31	electrons	electron	NOUN
cet-2646	51	32	to	to	PART
cet-2646	51	33	generate	generate	VERB
cet-2646	51	34	divalent	divalent	NOUN
cet-2646	51	35	coii	coii	ADJ
cet-2646	51	36	ones	one	NOUN
cet-2646	51	37	.	.	PUNCT
cet-2646	52	1	now	now	ADV
cet-2646	52	2	a	a	DET
cet-2646	52	3	cycle	cycle	NOUN
cet-2646	52	4	is	be	AUX
cet-2646	52	5	ended	end	VERB
cet-2646	52	6	.	.	PUNCT
cet-2646	53	1	when	when	SCONJ
cet-2646	53	2	the	the	DET
cet-2646	53	3	alkaline	alkaline	NOUN
cet-2646	53	4	in	in	ADP
cet-2646	53	5	the	the	DET
cet-2646	53	6	environmental	environmental	ADJ
cet-2646	53	7	system	system	NOUN
cet-2646	53	8	is	be	AUX
cet-2646	53	9	strong	strong	ADJ
cet-2646	53	10	,	,	PUNCT
cet-2646	53	11	coiiih	coiiih	ADJ
cet-2646	53	12	hydride	hydride	NOUN
cet-2646	53	13	interacts	interact	VERB
cet-2646	53	14	with	with	ADP
cet-2646	53	15	the	the	DET
cet-2646	53	16	electrons	electron	NOUN
cet-2646	53	17	to	to	PART
cet-2646	53	18	generate	generate	VERB
cet-2646	53	19	a	a	DET
cet-2646	53	20	divalent	divalent	ADJ
cet-2646	53	21	coiih	coiih	ADJ
cet-2646	53	22	hydride	hydride	NOUN
cet-2646	53	23	which	which	PRON
cet-2646	53	24	then	then	ADV
cet-2646	53	25	reacts	react	VERB
cet-2646	53	26	with	with	ADP
cet-2646	53	27	the	the	DET
cet-2646	53	28	electrons	electron	NOUN
cet-2646	53	29	to	to	PART
cet-2646	53	30	get	get	VERB
cet-2646	53	31	hydrogen	hydrogen	NOUN
cet-2646	53	32	and	and	CCONJ
cet-2646	53	33	divalent	divalent	NOUN
cet-2646	53	34	coii	coii	ADJ
cet-2646	53	35	complexes	complex	NOUN
cet-2646	53	36	.	.	PUNCT
cet-2646	54	1	till	till	SCONJ
cet-2646	54	2	now	now	ADV
cet-2646	54	3	,	,	PUNCT
cet-2646	54	4	a	a	DET
cet-2646	54	5	hydrogen	hydrogen	NOUN
cet-2646	54	6	production	production	NOUN
cet-2646	54	7	cycle	cycle	NOUN
cet-2646	54	8	is	be	AUX
cet-2646	54	9	over	over	ADV
cet-2646	54	10	.	.	PUNCT
cet-2646	55	1	in	in	ADP
cet-2646	55	2	the	the	DET
cet-2646	55	3	process	process	NOUN
cet-2646	55	4	of	of	ADP
cet-2646	55	5	the	the	DET
cet-2646	55	6	hydrogen	hydrogen	NOUN
cet-2646	55	7	production	production	NOUN
cet-2646	55	8	simulation	simulation	NOUN
cet-2646	55	9	cycle	cycle	NOUN
cet-2646	55	10	,	,	PUNCT
cet-2646	55	11	it	it	PRON
cet-2646	55	12	is	be	AUX
cet-2646	55	13	found	find	VERB
cet-2646	55	14	that	that	SCONJ
cet-2646	55	15	the	the	DET
cet-2646	55	16	reason	reason	NOUN
cet-2646	55	17	why	why	SCONJ
cet-2646	55	18	the	the	DET
cet-2646	55	19	charge	charge	NOUN
cet-2646	55	20	transfer	transfer	NOUN
cet-2646	55	21	is	be	AUX
cet-2646	55	22	impacted	impact	VERB
cet-2646	55	23	lies	lie	NOUN
cet-2646	55	24	in	in	ADP
cet-2646	55	25	the	the	DET
cet-2646	55	26	capacities	capacity	NOUN
cet-2646	55	27	of	of	ADP
cet-2646	55	28	each	each	DET
cet-2646	55	29	intermediate	intermediate	ADJ
cet-2646	55	30	product	product	NOUN
cet-2646	55	31	to	to	PART
cet-2646	55	32	absorb	absorb	VERB
cet-2646	55	33	and	and	CCONJ
cet-2646	55	34	donate	donate	VERB
cet-2646	55	35	electrons	electron	NOUN
cet-2646	55	36	.	.	PUNCT
cet-2646	56	1	in	in	ADP
cet-2646	56	2	order	order	NOUN
cet-2646	56	3	to	to	PART
cet-2646	56	4	validate	validate	VERB
cet-2646	56	5	the	the	DET
cet-2646	56	6	above	above	ADJ
cet-2646	56	7	charge	charge	NOUN
cet-2646	56	8	transport	transport	NOUN
cet-2646	56	9	process	process	NOUN
cet-2646	56	10	,	,	PUNCT
cet-2646	56	11	the	the	DET
cet-2646	56	12	physical	physical	ADJ
cet-2646	56	13	properties	property	NOUN
cet-2646	56	14	of	of	ADP
cet-2646	56	15	each	each	DET
cet-2646	56	16	intermediate	intermediate	ADJ
cet-2646	56	17	product	product	NOUN
cet-2646	56	18	,	,	PUNCT
cet-2646	56	19	mainly	mainly	ADV
cet-2646	56	20	the	the	DET
cet-2646	56	21	lumo	lumo	ADJ
cet-2646	56	22	and	and	CCONJ
cet-2646	56	23	homo	homo	NOUN
cet-2646	56	24	orbit	orbit	NOUN
cet-2646	56	25	distributions	distribution	NOUN
cet-2646	56	26	,	,	PUNCT
cet-2646	56	27	are	be	AUX
cet-2646	56	28	analyzed	analyze	VERB
cet-2646	56	29	for	for	ADP
cet-2646	56	30	the	the	DET
cet-2646	56	31	reasons	reason	NOUN
cet-2646	56	32	that	that	PRON
cet-2646	56	33	the	the	DET
cet-2646	56	34	energy	energy	NOUN
cet-2646	56	35	level	level	NOUN
cet-2646	56	36	of	of	ADP
cet-2646	56	37	the	the	DET
cet-2646	56	38	lumo	lumo	NOUN
cet-2646	56	39	orbits	orbit	NOUN
cet-2646	56	40	partly	partly	ADV
cet-2646	56	41	explain	explain	VERB
cet-2646	56	42	the	the	DET
cet-2646	56	43	capacity	capacity	NOUN
cet-2646	56	44	to	to	PART
cet-2646	56	45	absorb	absorb	VERB
cet-2646	56	46	the	the	DET
cet-2646	56	47	electrons	electron	NOUN
cet-2646	56	48	,	,	PUNCT
cet-2646	56	49	whereas	whereas	SCONJ
cet-2646	56	50	that	that	PRON
cet-2646	56	51	of	of	ADP
cet-2646	56	52	the	the	DET
cet-2646	56	53	homo	homo	NOUN
cet-2646	56	54	orbit	orbit	NOUN
cet-2646	56	55	shows	show	VERB
cet-2646	56	56	its	its	PRON
cet-2646	56	57	capacity	capacity	NOUN
cet-2646	56	58	to	to	PART
cet-2646	56	59	donate	donate	VERB
cet-2646	56	60	electrons	electron	NOUN
cet-2646	56	61	.	.	PUNCT
cet-2646	57	1	therefore	therefore	ADV
cet-2646	57	2	,	,	PUNCT
cet-2646	57	3	we	we	PRON
cet-2646	57	4	analyze	analyze	VERB
cet-2646	57	5	the	the	DET
cet-2646	57	6	charge	charge	NOUN
cet-2646	57	7	transfer	transfer	NOUN
cet-2646	57	8	process	process	NOUN
cet-2646	57	9	step	step	NOUN
cet-2646	57	10	by	by	ADP
cet-2646	57	11	step	step	NOUN
cet-2646	57	12	as	as	SCONJ
cet-2646	57	13	follows	follow	VERB
cet-2646	57	14	:	:	PUNCT
cet-2646	57	15	cobalt	cobalt	NOUN
cet-2646	57	16	oxime	oxime	NOUN
cet-2646	57	17	molecules	molecule	NOUN
cet-2646	57	18	first	first	ADV
cet-2646	57	19	absorb	absorb	VERB
cet-2646	57	20	light	light	ADV
cet-2646	57	21	-	-	PUNCT
cet-2646	57	22	induced	induce	VERB
cet-2646	57	23	electrons	electron	NOUN
cet-2646	57	24	and	and	CCONJ
cet-2646	57	25	turn	turn	VERB
cet-2646	57	26	from	from	ADP
cet-2646	57	27	trivalent	trivalent	NOUN
cet-2646	57	28	co	co	NOUN
cet-2646	57	29	into	into	ADP
cet-2646	57	30	divalent	divalent	PROPN
cet-2646	57	31	co.	co.	PROPN
cet-2646	57	32	in	in	ADP
cet-2646	57	33	the	the	DET
cet-2646	57	34	distributions	distribution	NOUN
cet-2646	57	35	of	of	ADP
cet-2646	57	36	the	the	DET
cet-2646	57	37	calculated	calculated	ADJ
cet-2646	57	38	homo	homo	NOUN
cet-2646	57	39	and	and	CCONJ
cet-2646	57	40	lumo	lumo	NOUN
cet-2646	57	41	orbital	orbital	ADJ
cet-2646	57	42	energy	energy	NOUN
cet-2646	57	43	levels	level	NOUN
cet-2646	57	44	,	,	PUNCT
cet-2646	57	45	the	the	DET
cet-2646	57	46	lumo	lumo	NOUN
cet-2646	57	47	orbit	orbit	NOUN
cet-2646	57	48	concentrates	concentrate	VERB
cet-2646	57	49	all	all	PRON
cet-2646	57	50	of	of	ADP
cet-2646	57	51	them	they	PRON
cet-2646	57	52	onto	onto	ADP
cet-2646	57	53	the	the	DET
cet-2646	57	54	pyridine	pyridine	ADJ
cet-2646	57	55	ligands	ligand	NOUN
cet-2646	57	56	,	,	PUNCT
cet-2646	57	57	and	and	CCONJ
cet-2646	57	58	the	the	DET
cet-2646	57	59	homo	homo	NOUN
cet-2646	57	60	orbit	orbit	NOUN
cet-2646	57	61	distribution	distribution	NOUN
cet-2646	57	62	changes	change	NOUN
cet-2646	57	63	obviously	obviously	ADV
cet-2646	57	64	from	from	ADP
cet-2646	57	65	the	the	DET
cet-2646	57	66	lateral	lateral	ADJ
cet-2646	57	67	ligands	ligand	NOUN
cet-2646	57	68	on	on	ADP
cet-2646	57	69	the	the	DET
cet-2646	57	70	trivalent	trivalent	NOUN
cet-2646	57	71	co	co	NOUN
cet-2646	57	72	to	to	ADP
cet-2646	57	73	the	the	DET
cet-2646	57	74	axial	axial	ADJ
cet-2646	57	75	ones	one	NOUN
cet-2646	57	76	on	on	ADP
cet-2646	57	77	the	the	DET
cet-2646	57	78	divalent	divalent	NOUN
cet-2646	57	79	co	co	NOUN
cet-2646	57	80	predominantly	predominantly	ADV
cet-2646	57	81	on	on	ADP
cet-2646	57	82	the	the	DET
cet-2646	57	83	cl	cl	NOUN
cet-2646	57	84	groups	group	NOUN
cet-2646	57	85	.	.	PUNCT
cet-2646	58	1	further	further	ADJ
cet-2646	58	2	analysis	analysis	NOUN
cet-2646	58	3	of	of	ADP
cet-2646	58	4	the	the	DET
cet-2646	58	5	homo	homo	NOUN
cet-2646	58	6	orbit	orbit	NOUN
cet-2646	58	7	distribution	distribution	NOUN
cet-2646	58	8	on	on	ADP
cet-2646	58	9	the	the	DET
cet-2646	58	10	cl	cl	NOUN
cet-2646	58	11	group	group	NOUN
cet-2646	58	12	shows	show	VERB
cet-2646	58	13	that	that	SCONJ
cet-2646	58	14	there	there	PRON
cet-2646	58	15	is	be	VERB
cet-2646	58	16	almost	almost	ADV
cet-2646	58	17	no	no	DET
cet-2646	58	18	common	common	ADJ
cet-2646	58	19	electron	electron	NOUN
cet-2646	58	20	owned	own	VERB
cet-2646	58	21	by	by	ADP
cet-2646	58	22	the	the	DET
cet-2646	58	23	cl	cl	NOUN
cet-2646	58	24	group	group	NOUN
cet-2646	58	25	and	and	CCONJ
cet-2646	58	26	the	the	DET
cet-2646	58	27	co	co	NOUN
cet-2646	58	28	center	center	NOUN
cet-2646	58	29	,	,	PUNCT
cet-2646	58	30	that	that	PRON
cet-2646	58	31	is	be	AUX
cet-2646	58	32	to	to	PART
cet-2646	58	33	say	say	VERB
cet-2646	58	34	,	,	PUNCT
cet-2646	58	35	the	the	DET
cet-2646	58	36	interaction	interaction	NOUN
cet-2646	58	37	between	between	ADP
cet-2646	58	38	both	both	PRON
cet-2646	58	39	is	be	AUX
cet-2646	58	40	relatively	relatively	ADV
cet-2646	58	41	low	low	ADJ
cet-2646	58	42	,	,	PUNCT
cet-2646	58	43	which	which	PRON
cet-2646	58	44	implies	imply	VERB
cet-2646	58	45	that	that	SCONJ
cet-2646	58	46	in	in	ADP
cet-2646	58	47	the	the	DET
cet-2646	58	48	process	process	NOUN
cet-2646	58	49	that	that	PRON
cet-2646	58	50	co	co	VERB
cet-2646	58	51	group	group	NOUN
cet-2646	58	52	converts	convert	VERB
cet-2646	58	53	from	from	ADP
cet-2646	58	54	trivalent	trivalent	NOUN
cet-2646	58	55	co	co	NOUN
cet-2646	58	56	to	to	PART
cet-2646	58	57	divalent	divalent	VERB
cet-2646	58	58	one	one	NUM
cet-2646	58	59	,	,	PUNCT
cet-2646	58	60	the	the	DET
cet-2646	58	61	cl	cl	NOUN
cet-2646	58	62	group	group	NOUN
cet-2646	58	63	detaches	detach	VERB
cet-2646	58	64	from	from	ADP
cet-2646	58	65	the	the	DET
cet-2646	58	66	cobalt	cobalt	NOUN
cet-2646	58	67	oxime	oxime	NOUN
cet-2646	58	68	molecule	molecule	NOUN
cet-2646	58	69	.	.	PUNCT
cet-2646	59	1	while	while	SCONJ
cet-2646	59	2	the	the	DET
cet-2646	59	3	distance	distance	NOUN
cet-2646	59	4	between	between	ADP
cet-2646	59	5	cl	cl	NOUN
cet-2646	59	6	and	and	CCONJ
cet-2646	59	7	co	co	NOUN
cet-2646	59	8	atoms	atom	NOUN
cet-2646	59	9	increases	increase	VERB
cet-2646	59	10	from	from	ADP
cet-2646	59	11	2.2545å	2.2545å	PROPN
cet-2646	59	12	in	in	ADP
cet-2646	59	13	trivalent	trivalent	NOUN
cet-2646	59	14	coiii	coiii	NOUN
cet-2646	59	15	complex	complex	NOUN
cet-2646	59	16	to	to	ADP
cet-2646	59	17	2.5588å	2.5588å	NUM
cet-2646	59	18	in	in	ADP
cet-2646	59	19	divalent	divalent	NOUN
cet-2646	59	20	coii	coii	NOUN
cet-2646	59	21	complex	complex	NOUN
cet-2646	59	22	,	,	PUNCT
cet-2646	59	23	which	which	PRON
cet-2646	59	24	further	far	ADV
cet-2646	59	25	interprets	interpret	VERB
cet-2646	59	26	that	that	SCONJ
cet-2646	59	27	there	there	PRON
cet-2646	59	28	is	be	VERB
cet-2646	59	29	a	a	DET
cet-2646	59	30	weak	weak	ADJ
cet-2646	59	31	interaction	interaction	NOUN
cet-2646	59	32	between	between	ADP
cet-2646	59	33	the	the	DET
cet-2646	59	34	cl	cl	NOUN
cet-2646	59	35	group	group	NOUN
cet-2646	59	36	and	and	CCONJ
cet-2646	59	37	the	the	DET
cet-2646	59	38	co	co	PROPN
cet-2646	59	39	catalytic	catalytic	ADJ
cet-2646	59	40	center	center	NOUN
cet-2646	59	41	.	.	PUNCT
cet-2646	60	1	the	the	DET
cet-2646	60	2	fact	fact	NOUN
cet-2646	60	3	that	that	SCONJ
cet-2646	60	4	cl	cl	NOUN
cet-2646	60	5	group	group	NOUN
cet-2646	60	6	detaches	detach	VERB
cet-2646	60	7	from	from	ADP
cet-2646	60	8	the	the	DET
cet-2646	60	9	divalent	divalent	NOUN
cet-2646	60	10	coii	coii	NOUN
cet-2646	60	11	complex	complex	NOUN
cet-2646	60	12	is	be	AUX
cet-2646	60	13	further	far	ADV
cet-2646	60	14	proved	prove	VERB
cet-2646	60	15	.	.	PUNCT
cet-2646	61	1	figure	figure	VERB
cet-2646	61	2	4	4	NUM
cet-2646	61	3	:	:	PUNCT
cet-2646	61	4	coiii	coiii	X
cet-2646	61	5	(	(	PUNCT
cet-2646	61	6	+	+	NOUN
cet-2646	61	7	e	e	NOUN
cet-2646	61	8	)	)	PUNCT
cet-2646	61	9	→	→	SYM
cet-2646	61	10	coii	coii	ADJ
cet-2646	61	11	figure	figure	NOUN
cet-2646	61	12	5	5	NUM
cet-2646	61	13	:	:	PUNCT
cet-2646	61	14	coii	coii	ADJ
cet-2646	61	15	(	(	PUNCT
cet-2646	61	16	+	+	NOUN
cet-2646	61	17	e	e	NOUN
cet-2646	61	18	)	)	PUNCT
cet-2646	61	19	→	→	SYM
cet-2646	61	20	coi	coi	NOUN
cet-2646	61	21	(	(	PUNCT
cet-2646	61	22	+	+	NOUN
cet-2646	61	23	h+	h+	X
cet-2646	61	24	)	)	PUNCT
cet-2646	61	25	→	→	SYM
cet-2646	61	26	coiiih	coiiih	NOUN
cet-2646	61	27	in	in	ADP
cet-2646	61	28	this	this	DET
cet-2646	61	29	process	process	NOUN
cet-2646	61	30	,	,	PUNCT
cet-2646	61	31	we	we	PRON
cet-2646	61	32	can	can	AUX
cet-2646	61	33	clearly	clearly	ADV
cet-2646	61	34	know	know	VERB
cet-2646	61	35	about	about	ADP
cet-2646	61	36	how	how	SCONJ
cet-2646	61	37	the	the	DET
cet-2646	61	38	homo	homo	NOUN
cet-2646	61	39	orbit	orbit	NOUN
cet-2646	61	40	energy	energy	NOUN
cet-2646	61	41	distribution	distribution	NOUN
cet-2646	61	42	changes	change	NOUN
cet-2646	61	43	.	.	PUNCT
cet-2646	62	1	the	the	DET
cet-2646	62	2	homo	homo	NOUN
cet-2646	62	3	orbit	orbit	NOUN
cet-2646	62	4	where	where	SCONJ
cet-2646	62	5	the	the	DET
cet-2646	62	6	monovalent	monovalent	NOUN
cet-2646	62	7	coi	coi	NOUN
cet-2646	62	8	complex	complex	NOUN
cet-2646	62	9	is	be	AUX
cet-2646	62	10	generated	generate	VERB
cet-2646	62	11	from	from	ADP
cet-2646	62	12	the	the	DET
cet-2646	62	13	divalent	divalent	NOUN
cet-2646	62	14	co	co	NOUN
cet-2646	62	15	by	by	ADP
cet-2646	62	16	absorbing	absorb	VERB
cet-2646	62	17	electrons	electron	NOUN
cet-2646	62	18	mainly	mainly	ADV
cet-2646	62	19	distributes	distribute	VERB
cet-2646	62	20	the	the	DET
cet-2646	62	21	energy	energy	NOUN
cet-2646	62	22	on	on	ADP
cet-2646	62	23	the	the	DET
cet-2646	62	24	catalytic	catalytic	ADJ
cet-2646	62	25	center	center	NOUN
cet-2646	62	26	co	co	NOUN
cet-2646	62	27	,	,	PUNCT
cet-2646	62	28	which	which	PRON
cet-2646	62	29	provides	provide	VERB
cet-2646	62	30	conditions	condition	NOUN
cet-2646	62	31	for	for	ADP
cet-2646	62	32	the	the	DET
cet-2646	62	33	next	next	ADJ
cet-2646	62	34	proton	proton	NOUN
cet-2646	62	35	absoption	absoption	NOUN
cet-2646	62	36	.	.	PUNCT
cet-2646	63	1	it	it	PRON
cet-2646	63	2	follows	follow	VERB
cet-2646	63	3	that	that	SCONJ
cet-2646	63	4	the	the	DET
cet-2646	63	5	bound	bound	NOUN
cet-2646	63	6	of	of	ADP
cet-2646	63	7	proton	proton	NOUN
cet-2646	63	8	with	with	ADP
cet-2646	63	9	cobalt	cobalt	NOUN
cet-2646	63	10	oxime	oxime	NOUN
cet-2646	63	11	molecule	molecule	NOUN
cet-2646	63	12	must	must	AUX
cet-2646	63	13	be	be	AUX
cet-2646	63	14	the	the	DET
cet-2646	63	15	linkage	linkage	NOUN
cet-2646	63	16	between	between	ADP
cet-2646	63	17	h	h	NOUN
cet-2646	63	18	+	+	X
cet-2646	63	19	and	and	CCONJ
cet-2646	63	20	co	co	VERB
cet-2646	63	21	,	,	PUNCT
cet-2646	63	22	and	and	CCONJ
cet-2646	63	23	the	the	DET
cet-2646	63	24	interatomic	interatomic	ADJ
cet-2646	63	25	distance	distance	NOUN
cet-2646	63	26	between	between	ADP
cet-2646	63	27	co	co	NOUN
cet-2646	63	28	and	and	CCONJ
cet-2646	63	29	h	h	PROPN
cet-2646	63	30	in	in	ADP
cet-2646	63	31	the	the	DET
cet-2646	63	32	coiiih	coiiih	NOUN
cet-2646	63	33	complex	complex	NOUN
cet-2646	63	34	is	be	AUX
cet-2646	63	35	only	only	ADV
cet-2646	63	36	1.497	1.497	NUM
cet-2646	63	37	å	å	NOUN
cet-2646	63	38	.	.	PUNCT
cet-2646	64	1	the	the	DET
cet-2646	64	2	fact	fact	NOUN
cet-2646	64	3	that	that	SCONJ
cet-2646	64	4	hydride	hydride	NOUN
cet-2646	64	5	coiiih	coiiih	NOUN
cet-2646	64	6	is	be	AUX
cet-2646	64	7	generated	generate	VERB
cet-2646	64	8	is	be	AUX
cet-2646	64	9	therefore	therefore	ADV
cet-2646	64	10	further	far	ADV
cet-2646	64	11	confirmed	confirm	VERB
cet-2646	64	12	.	.	PUNCT
cet-2646	65	1	this	this	PRON
cet-2646	65	2	is	be	AUX
cet-2646	65	3	to	to	PART
cet-2646	65	4	demonstrate	demonstrate	VERB
cet-2646	65	5	the	the	DET
cet-2646	65	6	h2	h2	NOUN
cet-2646	65	7	production	production	NOUN
cet-2646	65	8	process	process	NOUN
cet-2646	65	9	simply	simply	ADV
cet-2646	65	10	achieved	achieve	VERB
cet-2646	65	11	from	from	ADP
cet-2646	65	12	the	the	DET
cet-2646	65	13	interatomic	interatomic	ADJ
cet-2646	65	14	distance	distance	NOUN
cet-2646	65	15	.	.	PUNCT
cet-2646	66	1	when	when	SCONJ
cet-2646	66	2	the	the	DET
cet-2646	66	3	hydride	hydride	NOUN
cet-2646	66	4	coiiih	coiiih	NOUN
cet-2646	66	5	interacts	interact	VERB
cet-2646	66	6	with	with	ADP
cet-2646	66	7	the	the	DET
cet-2646	66	8	proton	proton	NOUN
cet-2646	66	9	,	,	PUNCT
cet-2646	66	10	it	it	PRON
cet-2646	66	11	is	be	AUX
cet-2646	66	12	found	find	VERB
cet-2646	66	13	that	that	SCONJ
cet-2646	66	14	the	the	DET
cet-2646	66	15	distances	distance	NOUN
cet-2646	66	16	of	of	ADP
cet-2646	66	17	catalytic	catalytic	ADJ
cet-2646	66	18	center	center	NOUN
cet-2646	66	19	co	co	VERB
cet-2646	66	20	from	from	ADP
cet-2646	66	21	two	two	NUM
cet-2646	66	22	h	h	NOUN
cet-2646	66	23	atoms	atom	NOUN
cet-2646	66	24	all	all	ADV
cet-2646	66	25	equal	equal	ADJ
cet-2646	66	26	to	to	ADP
cet-2646	66	27	1.8314	1.8314	NUM
cet-2646	66	28	å	å	NOUN
cet-2646	66	29	,	,	PUNCT
cet-2646	66	30	significantly	significantly	ADV
cet-2646	66	31	higher	high	ADJ
cet-2646	66	32	than	than	ADP
cet-2646	66	33	1.497å	1.497å	NUM
cet-2646	66	34	between	between	ADP
cet-2646	66	35	both	both	PRON
cet-2646	66	36	in	in	ADP
cet-2646	66	37	622	622	NUM
cet-2646	66	38	the	the	DET
cet-2646	66	39	trivalent	trivalent	ADJ
cet-2646	66	40	hydride	hydride	NOUN
cet-2646	66	41	coiiih	coiiih	NOUN
cet-2646	66	42	,	,	PUNCT
cet-2646	66	43	which	which	PRON
cet-2646	66	44	indicates	indicate	VERB
cet-2646	66	45	that	that	SCONJ
cet-2646	66	46	the	the	DET
cet-2646	66	47	interaction	interaction	NOUN
cet-2646	66	48	between	between	ADP
cet-2646	66	49	co	co	NOUN
cet-2646	66	50	and	and	CCONJ
cet-2646	66	51	h	h	NOUN
cet-2646	66	52	is	be	AUX
cet-2646	66	53	weaker	weak	ADJ
cet-2646	66	54	,	,	PUNCT
cet-2646	66	55	and	and	CCONJ
cet-2646	66	56	the	the	DET
cet-2646	66	57	distance	distance	NOUN
cet-2646	66	58	between	between	ADP
cet-2646	66	59	two	two	NUM
cet-2646	66	60	h	h	NOUN
cet-2646	66	61	atoms	atom	NOUN
cet-2646	66	62	in	in	ADP
cet-2646	66	63	the	the	DET
cet-2646	66	64	product	product	NOUN
cet-2646	66	65	as	as	SCONJ
cet-2646	66	66	generated	generate	VERB
cet-2646	66	67	is	be	AUX
cet-2646	66	68	0.7719	0.7719	NUM
cet-2646	66	69	å	å	NOUN
cet-2646	66	70	,	,	PUNCT
cet-2646	66	71	very	very	ADV
cet-2646	66	72	close	close	ADJ
cet-2646	66	73	to	to	ADP
cet-2646	66	74	the	the	DET
cet-2646	66	75	interatomic	interatomic	ADJ
cet-2646	66	76	distance	distance	NOUN
cet-2646	66	77	in	in	ADP
cet-2646	66	78	hydrogen	hydrogen	NOUN
cet-2646	66	79	.	.	PUNCT
cet-2646	67	1	we	we	PRON
cet-2646	67	2	can	can	AUX
cet-2646	67	3	therefore	therefore	ADV
cet-2646	67	4	believe	believe	VERB
cet-2646	67	5	that	that	SCONJ
cet-2646	67	6	hydrogen	hydrogen	NOUN
cet-2646	67	7	has	have	AUX
cet-2646	67	8	been	be	AUX
cet-2646	67	9	produced	produce	VERB
cet-2646	67	10	in	in	ADP
cet-2646	67	11	this	this	DET
cet-2646	67	12	process	process	NOUN
cet-2646	67	13	with	with	ADP
cet-2646	67	14	available	available	ADJ
cet-2646	67	15	trivalent	trivalent	NOUN
cet-2646	67	16	coiii	coiii	NOUN
cet-2646	67	17	complexes	complex	NOUN
cet-2646	67	18	.	.	PUNCT
cet-2646	68	1	figure	figure	VERB
cet-2646	68	2	6	6	NUM
cet-2646	68	3	:	:	PUNCT
cet-2646	68	4	coiiih	coiiih	NOUN
cet-2646	68	5	(	(	PUNCT
cet-2646	68	6	+	+	NOUN
cet-2646	68	7	h+	h+	X
cet-2646	68	8	)	)	PUNCT
cet-2646	68	9	→	→	SYM
cet-2646	68	10	coiii	coiii	X
cet-2646	68	11	+	+	CCONJ
cet-2646	68	12	h2	h2	NOUN
cet-2646	68	13	figure	figure	NOUN
cet-2646	68	14	7	7	NUM
cet-2646	68	15	:	:	PUNCT
cet-2646	68	16	coiii	coiii	X
cet-2646	68	17	(	(	PUNCT
cet-2646	68	18	+	+	NOUN
cet-2646	68	19	e	e	NOUN
cet-2646	68	20	)	)	PUNCT
cet-2646	68	21	→	→	AUX
cet-2646	68	22	coii	coii	NOUN
cet-2646	68	23	this	this	PRON
cet-2646	68	24	is	be	AUX
cet-2646	68	25	the	the	DET
cet-2646	68	26	last	last	ADJ
cet-2646	68	27	step	step	NOUN
cet-2646	68	28	to	to	PART
cet-2646	68	29	close	close	VERB
cet-2646	68	30	the	the	DET
cet-2646	68	31	cycle	cycle	NOUN
cet-2646	68	32	.	.	PUNCT
cet-2646	69	1	now	now	ADV
cet-2646	69	2	the	the	DET
cet-2646	69	3	resultant	resultant	NOUN
cet-2646	69	4	divalent	divalent	NOUN
cet-2646	69	5	coii	coii	NOUN
cet-2646	69	6	complex	complex	NOUN
cet-2646	69	7	should	should	AUX
cet-2646	69	8	be	be	AUX
cet-2646	69	9	equivalent	equivalent	ADJ
cet-2646	69	10	to	to	ADP
cet-2646	69	11	the	the	DET
cet-2646	69	12	initial	initial	ADJ
cet-2646	69	13	divalent	divalent	NOUN
cet-2646	69	14	coii	coii	NOUN
cet-2646	69	15	complex	complex	NOUN
cet-2646	69	16	.	.	PUNCT
cet-2646	70	1	the	the	DET
cet-2646	70	2	geometric	geometric	ADJ
cet-2646	70	3	structures	structure	NOUN
cet-2646	70	4	of	of	ADP
cet-2646	70	5	the	the	DET
cet-2646	70	6	divalent	divalent	NOUN
cet-2646	70	7	co	co	NOUN
cet-2646	70	8	complexes	complex	NOUN
cet-2646	70	9	at	at	ADP
cet-2646	70	10	the	the	DET
cet-2646	70	11	start	start	NOUN
cet-2646	70	12	and	and	CCONJ
cet-2646	70	13	at	at	ADP
cet-2646	70	14	the	the	DET
cet-2646	70	15	end	end	NOUN
cet-2646	70	16	of	of	ADP
cet-2646	70	17	the	the	DET
cet-2646	70	18	catalytic	catalytic	ADJ
cet-2646	70	19	cycles	cycle	NOUN
cet-2646	70	20	are	be	AUX
cet-2646	70	21	therefore	therefore	ADV
cet-2646	70	22	compared	compare	VERB
cet-2646	70	23	in	in	ADP
cet-2646	70	24	order	order	NOUN
cet-2646	70	25	to	to	PART
cet-2646	70	26	verify	verify	VERB
cet-2646	70	27	the	the	DET
cet-2646	70	28	closure	closure	NOUN
cet-2646	70	29	of	of	ADP
cet-2646	70	30	a	a	DET
cet-2646	70	31	catalytic	catalytic	ADJ
cet-2646	70	32	hydrogen	hydrogen	NOUN
cet-2646	70	33	production	production	NOUN
cet-2646	70	34	cycle	cycle	NOUN
cet-2646	70	35	.	.	PUNCT
cet-2646	71	1	for	for	ADP
cet-2646	71	2	the	the	DET
cet-2646	71	3	corresponding	correspond	VERB
cet-2646	71	4	coii	coii	ADJ
cet-2646	71	5	complexes	complex	NOUN
cet-2646	71	6	at	at	ADP
cet-2646	71	7	the	the	DET
cet-2646	71	8	start	start	NOUN
cet-2646	71	9	and	and	CCONJ
cet-2646	71	10	at	at	ADP
cet-2646	71	11	the	the	DET
cet-2646	71	12	end	end	NOUN
cet-2646	71	13	of	of	ADP
cet-2646	71	14	catalytic	catalytic	ADJ
cet-2646	71	15	cycles	cycle	NOUN
cet-2646	71	16	,	,	PUNCT
cet-2646	71	17	the	the	DET
cet-2646	71	18	geometric	geometric	ADJ
cet-2646	71	19	structures	structure	NOUN
cet-2646	71	20	of	of	ADP
cet-2646	71	21	the	the	DET
cet-2646	71	22	two	two	NUM
cet-2646	71	23	are	be	AUX
cet-2646	71	24	shown	show	VERB
cet-2646	71	25	in	in	ADP
cet-2646	71	26	table	table	NOUN
cet-2646	71	27	2	2	NUM
cet-2646	71	28	.	.	PUNCT
cet-2646	72	1	it	it	PRON
cet-2646	72	2	can	can	AUX
cet-2646	72	3	be	be	AUX
cet-2646	72	4	seen	see	VERB
cet-2646	72	5	from	from	ADP
cet-2646	72	6	the	the	DET
cet-2646	72	7	table	table	NOUN
cet-2646	72	8	that	that	SCONJ
cet-2646	72	9	there	there	PRON
cet-2646	72	10	is	be	VERB
cet-2646	72	11	a	a	DET
cet-2646	72	12	little	little	ADJ
cet-2646	72	13	difference	difference	NOUN
cet-2646	72	14	between	between	ADP
cet-2646	72	15	the	the	DET
cet-2646	72	16	combined	combine	VERB
cet-2646	72	17	constructions	construction	NOUN
cet-2646	72	18	of	of	ADP
cet-2646	72	19	initial	initial	ADJ
cet-2646	72	20	and	and	CCONJ
cet-2646	72	21	last	last	ADJ
cet-2646	72	22	coii	coii	ADJ
cet-2646	72	23	complexes	complex	NOUN
cet-2646	72	24	.	.	PUNCT
cet-2646	73	1	table	table	NOUN
cet-2646	73	2	2	2	NUM
cet-2646	73	3	:	:	PUNCT
cet-2646	73	4	the	the	DET
cet-2646	73	5	geometric	geometric	ADJ
cet-2646	73	6	structures	structure	NOUN
cet-2646	73	7	of	of	ADP
cet-2646	73	8	the	the	DET
cet-2646	73	9	corresponding	corresponding	ADJ
cet-2646	73	10	coii	coii	ADJ
cet-2646	73	11	complexes	complex	NOUN
cet-2646	73	12	at	at	ADP
cet-2646	73	13	the	the	DET
cet-2646	73	14	start	start	NOUN
cet-2646	73	15	and	and	CCONJ
cet-2646	73	16	at	at	ADP
cet-2646	73	17	the	the	DET
cet-2646	73	18	end	end	NOUN
cet-2646	73	19	of	of	ADP
cet-2646	73	20	catalytic	catalytic	ADJ
cet-2646	73	21	cycles	cycle	NOUN
cet-2646	73	22	bond	bond	NOUN
cet-2646	73	23	length(å)/angle	length(å)/angle	NOUN
cet-2646	73	24	(	(	PUNCT
cet-2646	73	25	º	º	NOUN
cet-2646	73	26	)	)	PUNCT
cet-2646	73	27	coii(last	coii(last	NOUN
cet-2646	73	28	)	)	PUNCT
cet-2646	73	29	coii(initial	coii(initial	PROPN
cet-2646	73	30	)	)	PUNCT
cet-2646	73	31	co	co	NOUN
cet-2646	73	32	-	-	NOUN
cet-2646	73	33	n11	n11	ADJ
cet-2646	73	34	1.92521	1.92521	NUM
cet-2646	73	35	1.92538	1.92538	NUM
cet-2646	73	36	co	co	NOUN
cet-2646	73	37	-	-	NOUN
cet-2646	73	38	n14	n14	ADJ
cet-2646	73	39	1.92590	1.92590	NUM
cet-2646	73	40	1.92576	1.92576	NUM
cet-2646	73	41	co	co	NOUN
cet-2646	73	42	-	-	NOUN
cet-2646	73	43	n21	n21	PROPN
cet-2646	73	44	1.92590	1.92590	NUM
cet-2646	73	45	1.92577	1.92577	NUM
cet-2646	73	46	co	co	NOUN
cet-2646	73	47	-	-	NOUN
cet-2646	73	48	n24	n24	PROPN
cet-2646	73	49	1.92522	1.92522	NUM
cet-2646	73	50	1.92537	1.92537	NUM
cet-2646	73	51	co1	co1	ADJ
cet-2646	73	52	-	-	ADJ
cet-2646	73	53	n31	n31	ADJ
cet-2646	73	54	2.14727	2.14727	NUM
cet-2646	73	55	2.1478	2.1478	NUM
cet-2646	73	56	n11	n11	NOUN
cet-2646	73	57	-	-	PUNCT
cet-2646	73	58	o15	o15	NOUN
cet-2646	73	59	1.36892	1.36892	NUM
cet-2646	73	60	1.36888	1.36888	NUM
cet-2646	73	61	n24	n24	NOUN
cet-2646	73	62	-	-	PUNCT
cet-2646	73	63	o26	o26	PROPN
cet-2646	73	64	1.36892	1.36892	NUM
cet-2646	73	65	1.36888	1.36888	NUM
cet-2646	73	66	n14	n14	NOUN
cet-2646	73	67	-	-	PUNCT
cet-2646	73	68	o16	o16	PROPN
cet-2646	73	69	1.30798	1.30798	NUM
cet-2646	73	70	1.30802	1.30802	NUM
cet-2646	73	71	n21	n21	NOUN
cet-2646	73	72	-	-	PUNCT
cet-2646	73	73	o25	o25	NOUN
cet-2646	73	74	1.30798	1.30798	NUM
cet-2646	73	75	1.30802	1.30802	NUM
cet-2646	73	76	n11	n11	PROPN
cet-2646	73	77	-	-	PUNCT
cet-2646	73	78	co	co	NOUN
cet-2646	73	79	-	-	NOUN
cet-2646	73	80	n24	n24	PROPN
cet-2646	73	81	167.14820	167.14820	NUM
cet-2646	73	82	167.1614	167.1614	NUM
cet-2646	73	83	n14	n14	NOUN
cet-2646	73	84	-	-	PUNCT
cet-2646	73	85	co	co	NOUN
cet-2646	73	86	-	-	NOUN
cet-2646	73	87	n21	n21	PROPN
cet-2646	73	88	173.88093	173.88093	NUM
cet-2646	73	89	173.8770	173.8770	NUM
cet-2646	73	90	n11	n11	PROPN
cet-2646	73	91	-	-	PUNCT
cet-2646	73	92	co	co	NOUN
cet-2646	73	93	-	-	NOUN
cet-2646	73	94	n21	n21	PROPN
cet-2646	73	95	97.63440	97.63440	NUM
cet-2646	73	96	97.63807	97.63807	NUM
cet-2646	73	97	n14	n14	NOUN
cet-2646	73	98	-	-	PUNCT
cet-2646	73	99	co1	co1	PROPN
cet-2646	73	100	-	-	PROPN
cet-2646	73	101	n24	n24	PROPN
cet-2646	73	102	97.63418	97.63418	NUM
cet-2646	73	103	97.63661	97.63661	NUM
cet-2646	73	104	n11	n11	PROPN
cet-2646	73	105	-	-	PUNCT
cet-2646	73	106	co1	co1	VERB
cet-2646	73	107	-	-	PUNCT
cet-2646	73	108	n14	n14	X
cet-2646	73	109	81.67445	81.67445	NUM
cet-2646	73	110	81.67181	81.67181	NUM
cet-2646	73	111	n21	n21	NOUN
cet-2646	73	112	-	-	PUNCT
cet-2646	73	113	co1	co1	PROPN
cet-2646	73	114	-	-	PROPN
cet-2646	73	115	n24	n24	PROPN
cet-2646	73	116	81.67455	81.67455	NUM
cet-2646	73	117	81.67161	81.67161	NUM
cet-2646	73	118	n11	n11	PROPN
cet-2646	73	119	-	-	PUNCT
cet-2646	73	120	co	co	NOUN
cet-2646	73	121	-	-	ADJ
cet-2646	73	122	n31	n31	ADJ
cet-2646	73	123	96.42585	96.42585	NUM
cet-2646	73	124	96.4198	96.4198	NUM
cet-2646	73	125	n14	n14	NOUN
cet-2646	73	126	-	-	PUNCT
cet-2646	73	127	co	co	NOUN
cet-2646	73	128	-	-	NOUN
cet-2646	73	129	n31	n31	ADJ
cet-2646	73	130	93.05958	93.05958	NUM
cet-2646	73	131	93.06174	93.06174	NUM
cet-2646	73	132	n21	n21	NOUN
cet-2646	73	133	-	-	PUNCT
cet-2646	73	134	co	co	NOUN
cet-2646	73	135	-	-	NOUN
cet-2646	73	136	n31	n31	ADJ
cet-2646	73	137	93.05958	93.05958	NUM
cet-2646	73	138	93.06123	93.06123	NUM
cet-2646	73	139	n24	n24	PROPN
cet-2646	73	140	-	-	PUNCT
cet-2646	73	141	co	co	NOUN
cet-2646	73	142	-	-	NOUN
cet-2646	73	143	n31	n31	ADJ
cet-2646	73	144	96.42595	96.42595	NUM
cet-2646	73	145	96.41878	96.41878	NUM
cet-2646	73	146	4	4	NUM
cet-2646	73	147	.	.	PUNCT
cet-2646	74	1	conclusion	conclusion	NOUN
cet-2646	74	2	in	in	ADP
cet-2646	74	3	this	this	DET
cet-2646	74	4	paper	paper	NOUN
cet-2646	74	5	,	,	PUNCT
cet-2646	74	6	the	the	DET
cet-2646	74	7	relevant	relevant	ADJ
cet-2646	74	8	intermediate	intermediate	ADJ
cet-2646	74	9	products	product	NOUN
cet-2646	74	10	can	can	AUX
cet-2646	74	11	be	be	AUX
cet-2646	74	12	clearly	clearly	ADV
cet-2646	74	13	captured	capture	VERB
cet-2646	74	14	by	by	ADP
cet-2646	74	15	the	the	DET
cet-2646	74	16	computational	computational	ADJ
cet-2646	74	17	simulation	simulation	NOUN
cet-2646	74	18	in	in	ADP
cet-2646	74	19	cyclic	cyclic	ADJ
cet-2646	74	20	process	process	NOUN
cet-2646	74	21	of	of	ADP
cet-2646	74	22	cobalt	cobalt	NOUN
cet-2646	74	23	oxime	oxime	NOUN
cet-2646	74	24	catalysis	catalysis	NOUN
cet-2646	74	25	,	,	PUNCT
cet-2646	74	26	and	and	CCONJ
cet-2646	74	27	the	the	DET
cet-2646	74	28	inherent	inherent	ADJ
cet-2646	74	29	relationship	relationship	NOUN
cet-2646	74	30	between	between	ADP
cet-2646	74	31	the	the	DET
cet-2646	74	32	electron	electron	NOUN
cet-2646	74	33	-	-	PUNCT
cet-2646	74	34	absorbing	absorb	VERB
cet-2646	74	35	and	and	CCONJ
cet-2646	74	36	electron	electron	NOUN
cet-2646	74	37	-	-	PUNCT
cet-2646	74	38	donating	donate	VERB
cet-2646	74	39	capacities	capacity	NOUN
cet-2646	74	40	and	and	CCONJ
cet-2646	74	41	its	its	PRON
cet-2646	74	42	catalytic	catalytic	ADJ
cet-2646	74	43	mechanism	mechanism	NOUN
cet-2646	74	44	are	be	AUX
cet-2646	74	45	grasped	grasp	VERB
cet-2646	74	46	as	as	ADP
cet-2646	74	47	the	the	DET
cet-2646	74	48	basis	basis	NOUN
cet-2646	74	49	for	for	ADP
cet-2646	74	50	further	far	ADV
cet-2646	74	51	recognizing	recognize	VERB
cet-2646	74	52	the	the	DET
cet-2646	74	53	difference	difference	NOUN
cet-2646	74	54	of	of	ADP
cet-2646	74	55	catalytic	catalytic	ADJ
cet-2646	74	56	hydrogen	hydrogen	NOUN
cet-2646	74	57	production	production	NOUN
cet-2646	74	58	cycles	cycle	NOUN
cet-2646	74	59	by	by	ADP
cet-2646	74	60	different	different	ADJ
cet-2646	74	61	structures	structure	NOUN
cet-2646	74	62	of	of	ADP
cet-2646	74	63	cobalt	cobalt	NOUN
cet-2646	74	64	oxime	oxime	NOUN
cet-2646	74	65	molecules	molecule	NOUN
cet-2646	74	66	and	and	CCONJ
cet-2646	74	67	the	the	DET
cet-2646	74	68	623	623	NUM
cet-2646	74	69	theoretical	theoretical	ADJ
cet-2646	74	70	basis	basis	NOUN
cet-2646	74	71	for	for	ADP
cet-2646	74	72	the	the	DET
cet-2646	74	73	dependence	dependence	NOUN
cet-2646	74	74	of	of	ADP
cet-2646	74	75	the	the	DET
cet-2646	74	76	hydrogen	hydrogen	NOUN
cet-2646	74	77	production	production	NOUN
cet-2646	74	78	efficiency	efficiency	NOUN
cet-2646	74	79	on	on	ADP
cet-2646	74	80	the	the	DET
cet-2646	74	81	catalyst	catalyst	NOUN
cet-2646	74	82	molecular	molecular	ADJ
cet-2646	74	83	structure	structure	NOUN
cet-2646	74	84	.	.	PUNCT
cet-2646	75	1	using	use	VERB
cet-2646	75	2	increasingly	increasingly	ADV
cet-2646	75	3	improved	improve	VERB
cet-2646	75	4	computational	computational	ADJ
cet-2646	75	5	simulation	simulation	NOUN
cet-2646	75	6	technique	technique	NOUN
cet-2646	75	7	,	,	PUNCT
cet-2646	75	8	and	and	CCONJ
cet-2646	75	9	on	on	ADP
cet-2646	75	10	several	several	ADJ
cet-2646	75	11	fronts	front	NOUN
cet-2646	75	12	such	such	ADJ
cet-2646	75	13	as	as	ADP
cet-2646	75	14	the	the	DET
cet-2646	75	15	impacts	impact	NOUN
cet-2646	75	16	of	of	ADP
cet-2646	75	17	the	the	DET
cet-2646	75	18	electronic	electronic	ADJ
cet-2646	75	19	properties	property	NOUN
cet-2646	75	20	of	of	ADP
cet-2646	75	21	the	the	DET
cet-2646	75	22	coordination	coordination	NOUN
cet-2646	75	23	group	group	NOUN
cet-2646	75	24	on	on	ADP
cet-2646	75	25	the	the	DET
cet-2646	75	26	electron	electron	NOUN
cet-2646	75	27	-	-	PUNCT
cet-2646	75	28	absorbing	absorb	VERB
cet-2646	75	29	capacity	capacity	NOUN
cet-2646	75	30	of	of	ADP
cet-2646	75	31	the	the	DET
cet-2646	75	32	catalyst	catalyst	NOUN
cet-2646	75	33	molecules	molecule	NOUN
cet-2646	75	34	,	,	PUNCT
cet-2646	75	35	and	and	CCONJ
cet-2646	75	36	the	the	DET
cet-2646	75	37	stability	stability	NOUN
cet-2646	75	38	of	of	ADP
cet-2646	75	39	coordination	coordination	NOUN
cet-2646	75	40	group	group	NOUN
cet-2646	75	41	in	in	ADP
cet-2646	75	42	the	the	DET
cet-2646	75	43	hydrogen	hydrogen	NOUN
cet-2646	75	44	production	production	NOUN
cet-2646	75	45	process	process	NOUN
cet-2646	75	46	and	and	CCONJ
cet-2646	75	47	its	its	PRON
cet-2646	75	48	impact	impact	NOUN
cet-2646	75	49	on	on	ADP
cet-2646	75	50	the	the	DET
cet-2646	75	51	electronic	electronic	ADJ
cet-2646	75	52	properties	property	NOUN
cet-2646	75	53	of	of	ADP
cet-2646	75	54	intermediate	intermediate	ADJ
cet-2646	75	55	products	product	NOUN
cet-2646	75	56	,	,	PUNCT
cet-2646	75	57	we	we	PRON
cet-2646	75	58	can	can	AUX
cet-2646	75	59	fully	fully	ADV
cet-2646	75	60	understand	understand	VERB
cet-2646	75	61	how	how	SCONJ
cet-2646	75	62	important	important	ADJ
cet-2646	75	63	the	the	DET
cet-2646	75	64	mechanism	mechanism	NOUN
cet-2646	75	65	the	the	DET
cet-2646	75	66	ligand	ligand	ADJ
cet-2646	75	67	structure	structure	NOUN
cet-2646	75	68	acts	act	VERB
cet-2646	75	69	on	on	ADP
cet-2646	75	70	the	the	DET
cet-2646	75	71	charge	charge	NOUN
cet-2646	75	72	transfer	transfer	NOUN
cet-2646	75	73	rate	rate	NOUN
cet-2646	75	74	in	in	ADP
cet-2646	75	75	the	the	DET
cet-2646	75	76	hydrogen	hydrogen	NOUN
cet-2646	75	77	production	production	NOUN
cet-2646	75	78	process	process	NOUN
cet-2646	75	79	is	be	AUX
cet-2646	75	80	as	as	ADP
cet-2646	75	81	a	a	DET
cet-2646	75	82	theoretical	theoretical	ADJ
cet-2646	75	83	basis	basis	NOUN
cet-2646	75	84	,	,	PUNCT
cet-2646	75	85	which	which	PRON
cet-2646	75	86	not	not	PART
cet-2646	75	87	only	only	ADV
cet-2646	75	88	provides	provide	VERB
cet-2646	75	89	a	a	DET
cet-2646	75	90	theoretical	theoretical	ADJ
cet-2646	75	91	guidance	guidance	NOUN
cet-2646	75	92	for	for	ADP
cet-2646	75	93	the	the	DET
cet-2646	75	94	design	design	NOUN
cet-2646	75	95	of	of	ADP
cet-2646	75	96	highly	highly	ADV
cet-2646	75	97	efficient	efficient	ADJ
cet-2646	75	98	photocatalyst	photocatalyst	NOUN
cet-2646	75	99	materials	material	NOUN
cet-2646	75	100	,	,	PUNCT
cet-2646	75	101	but	but	CCONJ
cet-2646	75	102	also	also	ADV
cet-2646	75	103	helps	helps	AUX
cet-2646	75	104	understand	understand	VERB
cet-2646	75	105	theoretically	theoretically	ADV
cet-2646	75	106	the	the	DET
cet-2646	75	107	dependence	dependence	NOUN
cet-2646	75	108	of	of	ADP
cet-2646	75	109	quantum	quantum	ADJ
cet-2646	75	110	yield	yield	NOUN
cet-2646	75	111	on	on	ADP
cet-2646	75	112	the	the	DET
cet-2646	75	113	experimental	experimental	ADJ
cet-2646	75	114	conditions	condition	NOUN
cet-2646	75	115	.	.	PUNCT
cet-2646	76	1	references	reference	NOUN
cet-2646	76	2	bernhard	bernhard	PROPN
cet-2646	76	3	k.	k.	PROPN
cet-2646	76	4	,	,	PUNCT
cet-2646	76	5	allen	allen	PROPN
cet-2646	76	6	j.b	j.b	PROPN
cet-2646	76	7	.	.	PROPN
cet-2646	76	8	,	,	PUNCT
cet-2646	76	9	1978	1978	NUM
cet-2646	76	10	,	,	PUNCT
cet-2646	76	11	heterogeneous	heterogeneous	ADJ
cet-2646	76	12	photocatalytic	photocatalytic	ADJ
cet-2646	76	13	decomposition	decomposition	NOUN
cet-2646	76	14	of	of	ADP
cet-2646	76	15	saturated	saturate	VERB
cet-2646	76	16	carboxylic	carboxylic	ADJ
cet-2646	76	17	acids	acid	NOUN
cet-2646	76	18	on	on	ADP
cet-2646	76	19	titanium	titanium	NOUN
cet-2646	76	20	dioxide	dioxide	NOUN
cet-2646	76	21	powder	powder	NOUN
cet-2646	76	22	.	.	PUNCT
cet-2646	77	1	decarboxylative	decarboxylative	ADJ
cet-2646	77	2	route	route	NOUN
cet-2646	77	3	to	to	ADP
cet-2646	77	4	alkanes	alkane	NOUN
cet-2646	77	5	,	,	PUNCT
cet-2646	77	6	journal	journal	NOUN
cet-2646	77	7	of	of	ADP
cet-2646	77	8	the	the	DET
cet-2646	77	9	american	american	PROPN
cet-2646	77	10	chemical	chemical	PROPN
cet-2646	77	11	society	society	PROPN
cet-2646	77	12	,	,	PUNCT
cet-2646	77	13	100(19	100(19	NUM
cet-2646	77	14	)	)	PUNCT
cet-2646	77	15	,	,	PUNCT
cet-2646	77	16	5985	5985	NUM
cet-2646	77	17	-	-	SYM
cet-2646	77	18	5992	5992	NUM
cet-2646	77	19	,	,	PUNCT
cet-2646	77	20	doi	doi	NOUN
cet-2646	77	21	:	:	PUNCT
cet-2646	77	22	10.1021	10.1021	NUM
cet-2646	77	23	/	/	SYM
cet-2646	77	24	ja00487a001	ja00487a001	NOUN
cet-2646	77	25	.	.	PUNCT
cet-2646	78	1	bigi	bigi	PROPN
cet-2646	78	2	j.p	j.p	PROPN
cet-2646	78	3	.	.	PROPN
cet-2646	78	4	,	,	PUNCT
cet-2646	78	5	hanna	hanna	PROPN
cet-2646	78	6	t.e	t.e	PROPN
cet-2646	78	7	.	.	PROPN
cet-2646	78	8	,	,	PUNCT
cet-2646	78	9	harman	harman	PROPN
cet-2646	78	10	w.h	w.h	PROPN
cet-2646	78	11	,	,	PUNCT
cet-2646	78	12	2010	2010	NUM
cet-2646	78	13	,	,	PUNCT
cet-2646	78	14	electrocatalytic	electrocatalytic	ADJ
cet-2646	78	15	reduction	reduction	NOUN
cet-2646	78	16	of	of	ADP
cet-2646	78	17	protons	proton	NOUN
cet-2646	78	18	to	to	ADP
cet-2646	78	19	hydrogen	hydrogen	NOUN
cet-2646	78	20	by	by	ADP
cet-2646	78	21	a	a	DET
cet-2646	78	22	watercompatible	watercompatible	ADJ
cet-2646	78	23	cobalt	cobalt	NOUN
cet-2646	78	24	polypyridyl	polypyridyl	NOUN
cet-2646	78	25	platform	platform	NOUN
cet-2646	78	26	,	,	PUNCT
cet-2646	78	27	chemical	chemical	NOUN
cet-2646	78	28	communications	communication	NOUN
cet-2646	78	29	,	,	PUNCT
cet-2646	78	30	46(6	46(6	NOUN
cet-2646	78	31	)	)	PUNCT
cet-2646	78	32	,	,	PUNCT
cet-2646	78	33	958	958	NUM
cet-2646	78	34	-	-	SYM
cet-2646	78	35	960	960	NUM
cet-2646	78	36	,	,	PUNCT
cet-2646	78	37	doi	doi	NOUN
cet-2646	78	38	:	:	PUNCT
cet-2646	78	39	10.1039	10.1039	NUM
cet-2646	78	40	/	/	SYM
cet-2646	78	41	b915846d	b915846d	NOUN
cet-2646	78	42	.	.	PROPN
cet-2646	78	43	esswein	esswein	PROPN
cet-2646	78	44	a.j	a.j	PROPN
cet-2646	78	45	.	.	PROPN
cet-2646	78	46	,	,	PUNCT
cet-2646	78	47	nocera	nocera	PROPN
cet-2646	78	48	d.g	d.g	PROPN
cet-2646	78	49	.	.	PROPN
cet-2646	78	50	,	,	PUNCT
cet-2646	78	51	2007	2007	NUM
cet-2646	78	52	,	,	PUNCT
cet-2646	78	53	hydrogen	hydrogen	NOUN
cet-2646	78	54	production	production	NOUN
cet-2646	78	55	by	by	ADP
cet-2646	78	56	molecular	molecular	ADJ
cet-2646	78	57	phothcatalysis	phothcatalysis	NOUN
cet-2646	78	58	,	,	PUNCT
cet-2646	78	59	chemical	chemical	NOUN
cet-2646	78	60	reviews	review	NOUN
cet-2646	78	61	,	,	PUNCT
cet-2646	78	62	107	107	NUM
cet-2646	78	63	,	,	PUNCT
cet-2646	78	64	4022	4022	NUM
cet-2646	78	65	-	-	SYM
cet-2646	78	66	4047	4047	NUM
cet-2646	78	67	,	,	PUNCT
cet-2646	78	68	doi	doi	NOUN
cet-2646	78	69	:	:	PUNCT
cet-2646	78	70	10.1016	10.1016	NUM
cet-2646	78	71	/	/	SYM
cet-2646	78	72	b978	b978	NUM
cet-2646	78	73	-	-	PUNCT
cet-2646	78	74	0	0	NUM
cet-2646	78	75	-	-	PUNCT
cet-2646	78	76	12	12	NUM
cet-2646	78	77	-	-	PUNCT
cet-2646	78	78	409547	409547	NUM
cet-2646	78	79	-	-	PUNCT
cet-2646	78	80	2.13795	2.13795	NUM
cet-2646	78	81	-	-	PUNCT
cet-2646	78	82	3	3	NUM
cet-2646	78	83	.	.	PUNCT
cet-2646	78	84	fujishima	fujishima	PROPN
cet-2646	78	85	a.	a.	PROPN
cet-2646	78	86	,	,	PUNCT
cet-2646	78	87	honda	honda	PROPN
cet-2646	78	88	k.	k.	PROPN
cet-2646	78	89	,	,	PUNCT
cet-2646	78	90	1972	1972	NUM
cet-2646	78	91	,	,	PUNCT
cet-2646	78	92	electrochemical	electrochemical	ADJ
cet-2646	78	93	photolysis	photolysis	NOUN
cet-2646	78	94	of	of	ADP
cet-2646	78	95	water	water	NOUN
cet-2646	78	96	at	at	ADP
cet-2646	78	97	a	a	DET
cet-2646	78	98	semiconductor	semiconductor	NOUN
cet-2646	78	99	electrode	electrode	NOUN
cet-2646	78	100	,	,	PUNCT
cet-2646	78	101	nature	nature	NOUN
cet-2646	78	102	,	,	PUNCT
cet-2646	78	103	238(5358	238(5358	NUM
cet-2646	78	104	)	)	PUNCT
cet-2646	78	105	,	,	PUNCT
cet-2646	78	106	37	37	NUM
cet-2646	78	107	-	-	SYM
cet-2646	78	108	40	40	NUM
cet-2646	78	109	,	,	PUNCT
cet-2646	78	110	doi	doi	NOUN
cet-2646	78	111	:	:	PUNCT
cet-2646	78	112	10.1038/238037a0	10.1038/238037a0	PROPN
cet-2646	78	113	.	.	PUNCT
cet-2646	78	114	kudo	kudo	PROPN
cet-2646	78	115	a.	a.	PROPN
cet-2646	78	116	,	,	PUNCT
cet-2646	78	117	miseki	miseki	PROPN
cet-2646	78	118	y.	y.	PROPN
cet-2646	78	119	,	,	PUNCT
cet-2646	78	120	2009	2009	NUM
cet-2646	78	121	,	,	PUNCT
cet-2646	78	122	heterogeneous	heterogeneous	ADJ
cet-2646	78	123	photocatalyst	photocatalyst	NOUN
cet-2646	78	124	materials	material	NOUN
cet-2646	78	125	for	for	ADP
cet-2646	78	126	water	water	NOUN
cet-2646	78	127	splitting	splitting	NOUN
cet-2646	78	128	,	,	PUNCT
cet-2646	78	129	chemical	chemical	ADJ
cet-2646	78	130	society	society	NOUN
cet-2646	78	131	reviews	review	NOUN
cet-2646	78	132	,	,	PUNCT
cet-2646	78	133	38	38	NUM
cet-2646	78	134	,	,	PUNCT
cet-2646	78	135	253	253	NUM
cet-2646	78	136	-	-	SYM
cet-2646	78	137	255	255	NUM
cet-2646	78	138	,	,	PUNCT
cet-2646	78	139	doi	doi	NOUN
cet-2646	78	140	:	:	PUNCT
cet-2646	78	141	10.1039	10.1039	NUM
cet-2646	78	142	/	/	SYM
cet-2646	78	143	b800489	b800489	PROPN
cet-2646	78	144	g.	g.	PROPN
cet-2646	78	145	mark	mark	PROPN
cet-2646	78	146	k.	k.	PROPN
cet-2646	78	147	,	,	PUNCT
cet-2646	78	148	mate	mate	NOUN
cet-2646	78	149	h.	h.	PROPN
cet-2646	78	150	,	,	PUNCT
cet-2646	78	151	2010	2010	NUM
cet-2646	78	152	,	,	PUNCT
cet-2646	78	153	heterogeneous	heterogeneous	ADJ
cet-2646	78	154	photocatalytic	photocatalytic	ADJ
cet-2646	78	155	cleavage	cleavage	NOUN
cet-2646	78	156	of	of	ADP
cet-2646	78	157	water	water	NOUN
cet-2646	78	158	,	,	PUNCT
cet-2646	78	159	journal	journal	NOUN
cet-2646	78	160	of	of	ADP
cet-2646	78	161	materials	material	NOUN
cet-2646	78	162	chemistry	chemistry	NOUN
cet-2646	78	163	,	,	PUNCT
cet-2646	78	164	20(4	20(4	NOUN
cet-2646	78	165	)	)	PUNCT
cet-2646	78	166	,	,	PUNCT
cet-2646	78	167	627	627	NUM
cet-2646	78	168	-	-	SYM
cet-2646	78	169	629	629	NUM
cet-2646	78	170	,	,	PUNCT
cet-2646	78	171	doi	doi	NOUN
cet-2646	78	172	:	:	PUNCT
cet-2646	78	173	10.1039	10.1039	NUM
cet-2646	78	174	/	/	SYM
cet-2646	78	175	b910180b	b910180b	PROPN
cet-2646	78	176	.	.	PROPN
cet-2646	78	177	osterloh	osterloh	PROPN
cet-2646	78	178	f.e	f.e	PROPN
cet-2646	78	179	.	.	PROPN
cet-2646	78	180	,	,	PUNCT
cet-2646	78	181	2008	2008	NUM
cet-2646	78	182	,	,	PUNCT
cet-2646	78	183	inorganic	inorganic	ADJ
cet-2646	78	184	materials	material	NOUN
cet-2646	78	185	as	as	ADP
cet-2646	78	186	catalysts	catalyst	NOUN
cet-2646	78	187	for	for	ADP
cet-2646	78	188	photochemical	photochemical	ADJ
cet-2646	78	189	splitting	splitting	NOUN
cet-2646	78	190	of	of	ADP
cet-2646	78	191	water	water	NOUN
cet-2646	78	192	,	,	PUNCT
cet-2646	78	193	chemistry	chemistry	NOUN
cet-2646	78	194	of	of	ADP
cet-2646	78	195	materials	material	NOUN
cet-2646	78	196	,	,	PUNCT
cet-2646	78	197	20(1	20(1	NUM
cet-2646	78	198	)	)	PUNCT
cet-2646	78	199	,	,	PUNCT
cet-2646	78	200	35	35	NUM
cet-2646	78	201	-	-	SYM
cet-2646	78	202	54	54	NUM
cet-2646	78	203	,	,	PUNCT
cet-2646	78	204	doi	doi	NOUN
cet-2646	78	205	:	:	PUNCT
cet-2646	78	206	10.1021	10.1021	NUM
cet-2646	78	207	/	/	SYM
cet-2646	78	208	cm7024203	cm7024203	NOUN
cet-2646	78	209	.	.	PUNCT
cet-2646	79	1	sun	sun	PROPN
cet-2646	79	2	l.c	l.c	PROPN
cet-2646	79	3	.	.	PROPN
cet-2646	79	4	,	,	PUNCT
cet-2646	79	5	hammarstroem	hammarstroem	PROPN
cet-2646	79	6	l.	l.	PROPN
cet-2646	79	7	,	,	PUNCT
cet-2646	79	8	aakermark	aakermark	PROPN
cet-2646	79	9	b.	b.	PROPN
cet-2646	79	10	,	,	PUNCT
cet-2646	79	11	styring	styre	VERB
cet-2646	79	12	s.	s.	PROPN
cet-2646	79	13	,	,	PUNCT
cet-2646	79	14	2001	2001	NUM
cet-2646	79	15	,	,	PUNCT
cet-2646	79	16	towards	towards	ADP
cet-2646	79	17	artificial	artificial	ADJ
cet-2646	79	18	photosynthesis	photosynthesis	NOUN
cet-2646	79	19	:	:	PUNCT
cet-2646	79	20	rutheniummanganese	rutheniummanganese	ADJ
cet-2646	79	21	chemistry	chemistry	NOUN
cet-2646	79	22	for	for	ADP
cet-2646	79	23	energy	energy	NOUN
cet-2646	79	24	production	production	NOUN
cet-2646	79	25	,	,	PUNCT
cet-2646	79	26	chemical	chemical	ADJ
cet-2646	79	27	society	society	NOUN
cet-2646	79	28	reviews	review	NOUN
cet-2646	79	29	,	,	PUNCT
cet-2646	79	30	30(47	30(47	NUM
cet-2646	79	31	)	)	PUNCT
cet-2646	79	32	,	,	PUNCT
cet-2646	79	33	36	36	NUM
cet-2646	79	34	-	-	SYM
cet-2646	79	35	49	49	NUM
cet-2646	79	36	,	,	PUNCT
cet-2646	79	37	doi	doi	NOUN
cet-2646	79	38	:	:	PUNCT
cet-2646	79	39	10.1039	10.1039	NUM
cet-2646	79	40	/	/	SYM
cet-2646	79	41	a801490f	a801490f	PROPN
cet-2646	79	42	.	.	PROPN
cet-2646	79	43	young	young	PROPN
cet-2646	79	44	r.c	r.c	PROPN
cet-2646	79	45	.	.	PROPN
cet-2646	79	46	,	,	PUNCT
cet-2646	79	47	meyer	meyer	PROPN
cet-2646	79	48	t.j	t.j	PROPN
cet-2646	79	49	.	.	PROPN
cet-2646	79	50	,	,	PUNCT
cet-2646	79	51	whitten	whitten	PROPN
cet-2646	79	52	d.g	d.g	PROPN
cet-2646	79	53	.	.	PROPN
cet-2646	79	54	,	,	PUNCT
cet-2646	79	55	1975	1975	NUM
cet-2646	79	56	,	,	PUNCT
cet-2646	79	57	kinetic	kinetic	ADJ
cet-2646	79	58	relaxation	relaxation	NOUN
cet-2646	79	59	measurement	measurement	NOUN
cet-2646	79	60	of	of	ADP
cet-2646	79	61	rapid	rapid	ADJ
cet-2646	79	62	electron	electron	NOUN
cet-2646	79	63	transfer	transfer	NOUN
cet-2646	79	64	reactions	reaction	NOUN
cet-2646	79	65	by	by	ADP
cet-2646	79	66	flash	flash	NOUN
cet-2646	79	67	photolysis	photolysis	NOUN
cet-2646	79	68	.	.	PUNCT
cet-2646	80	1	the	the	DET
cet-2646	80	2	conversion	conversion	NOUN
cet-2646	80	3	of	of	ADP
cet-2646	80	4	light	light	ADJ
cet-2646	80	5	energy	energy	NOUN
cet-2646	80	6	into	into	ADP
cet-2646	80	7	chemical	chemical	ADJ
cet-2646	80	8	energy	energy	NOUN
cet-2646	80	9	using	use	VERB
cet-2646	80	10	the	the	DET
cet-2646	80	11	ru(bpy)33+ru(bpy)32	ru(bpy)33+ru(bpy)32	NOUN
cet-2646	80	12	+	+	PROPN
cet-2646	80	13	*	*	NOUN
cet-2646	80	14	couple	couple	NOUN
cet-2646	80	15	,	,	PUNCT
cet-2646	80	16	journal	journal	NOUN
cet-2646	80	17	of	of	ADP
cet-2646	80	18	the	the	DET
cet-2646	80	19	american	american	PROPN
cet-2646	80	20	chemical	chemical	PROPN
cet-2646	80	21	society	society	PROPN
cet-2646	80	22	,	,	PUNCT
cet-2646	80	23	97(16	97(16	NOUN
cet-2646	80	24	)	)	PUNCT
cet-2646	80	25	,	,	PUNCT
cet-2646	80	26	4781	4781	NUM
cet-2646	80	27	-	-	SYM
cet-2646	80	28	4782	4782	NUM
cet-2646	80	29	,	,	PUNCT
cet-2646	80	30	doi	doi	NOUN
cet-2646	80	31	:	:	PUNCT
cet-2646	80	32	10.1002	10.1002	NUM
cet-2646	80	33	/	/	SYM
cet-2646	80	34	chin.197542426	chin.197542426	PROPN
cet-2646	80	35	624	624	NUM