id	sid	tid	token	lemma	pos
eurjchem-440	1	1	untitled	untitled	ADJ
eurjchem-440	1	2	studies	study	NOUN
eurjchem-440	1	3	o	o	PROPN
eurjchem-440	2	1	cobalt(ii	cobalt(ii	INTJ
eurjchem-440	2	2	farah	farah	PROPN
eurjchem-440	2	3	sami	sami	PROPN
eurjchem-440	2	4	ghassan	ghassan	PROPN
eurjchem-440	2	5	om	om	PROPN
eurjchem-440	2	6	a	a	DET
eurjchem-440	2	7	chemistry	chemistry	NOUN
eurjchem-440	2	8	depar	depar	NOUN
eurjchem-440	2	9	b	b	NOUN
eurjchem-440	2	10	chemistry	chemistry	NOUN
eurjchem-440	2	11	depar	depar	NOUN
eurjchem-440	2	12	*	*	PUNCT
eurjchem-440	2	13	corresponding	correspond	VERB
eurjchem-440	2	14	a	a	DET
eurjchem-440	2	15	fax	fax	NOUN
eurjchem-440	2	16	:	:	PUNCT
eurjchem-440	2	17	+2.034276590	+2.034276590	NUM
eurjchem-440	2	18	article	article	NOUN
eurjchem-440	2	19	info	info	NOUN
eurjchem-440	2	20	received	receive	VERB
eurjchem-440	2	21	:	:	PUNCT
eurjchem-440	2	22	13	13	NUM
eurjchem-440	2	23	apr	apr	NOUN
eurjchem-440	2	24	received	receive	VERB
eurjchem-440	2	25	in	in	ADP
eurjchem-440	2	26	revis	revis	PROPN
eurjchem-440	2	27	accepted	accept	VERB
eurjchem-440	2	28	:	:	PUNCT
eurjchem-440	2	29	05	05	NUM
eurjchem-440	2	30	july	july	PROPN
eurjchem-440	2	31	online	online	NOUN
eurjchem-440	2	32	:	:	PUNCT
eurjchem-440	2	33	31	31	NUM
eurjchem-440	2	34	decem	decem	NOUN
eurjchem-440	2	35	keywords	keyword	VERB
eurjchem-440	2	36	ion‐pair	ion‐pair	PRON
eurjchem-440	2	37	aquation	aquation	NOUN
eurjchem-440	2	38	solvent	solvent	NOUN
eurjchem-440	2	39	effect	effect	NOUN
eurjchem-440	2	40	cobalt(iii	cobalt(iii	NOUN
eurjchem-440	2	41	)	)	PUNCT
eurjchem-440	2	42	compl	compl	PROPN
eurjchem-440	2	43	dicarboxylic	dicarboxylic	ADJ
eurjchem-440	2	44	acid	acid	NOUN
eurjchem-440	2	45	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	2	46	1	1	X
eurjchem-440	2	47	.	.	PUNCT
eurjchem-440	3	1	introductio	introductio	VERB
eurjchem-440	3	2	transition	transition	NOUN
eurjchem-440	3	3	roles	role	NOUN
eurjchem-440	3	4	in	in	ADP
eurjchem-440	3	5	biolo	biolo	ADJ
eurjchem-440	3	6	complexes	complex	NOUN
eurjchem-440	3	7	hav	hav	AUX
eurjchem-440	3	8	rabbit	rabbit	NOUN
eurjchem-440	3	9	brain	brain	NOUN
eurjchem-440	4	1	an	an	DET
eurjchem-440	4	2	[	[	X
eurjchem-440	4	3	1‐2	1‐2	NOUN
eurjchem-440	4	4	]	]	X
eurjchem-440	4	5	.	.	PUNCT
eurjchem-440	5	1	also	also	ADV
eurjchem-440	5	2	cob	cob	NOUN
eurjchem-440	5	3	vitamin	vitamin	NOUN
eurjchem-440	5	4	b12	b12	NOUN
eurjchem-440	6	1	[	[	X
eurjchem-440	6	2	3	3	NUM
eurjchem-440	6	3	]	]	X
eurjchem-440	6	4	different	different	ADJ
eurjchem-440	6	5	s	s	PART
eurjchem-440	6	6	halogenopenta	halogenopenta	NOUN
eurjchem-440	6	7	investigations	investigation	NOUN
eurjchem-440	6	8	tial	tial	NOUN
eurjchem-440	6	9	,	,	PUNCT
eurjchem-440	6	10	selective	selective	ADJ
eurjchem-440	6	11	useful	useful	ADJ
eurjchem-440	6	12	in	in	ADP
eurjchem-440	6	13	accou	accou	NOUN
eurjchem-440	6	14	in	in	ADP
eurjchem-440	6	15	solution	solution	NOUN
eurjchem-440	6	16	.	.	PUNCT
eurjchem-440	7	1	it	it	PRON
eurjchem-440	7	2	w	w	VERB
eurjchem-440	7	3	some	some	DET
eurjchem-440	7	4	bivalen	bivalen	ADJ
eurjchem-440	7	5	chromium(iii	chromium(iii	NOUN
eurjchem-440	7	6	)	)	PUNCT
eurjchem-440	7	7	compared	compare	VERB
eurjchem-440	7	8	to	to	ADP
eurjchem-440	7	9	t	t	PROPN
eurjchem-440	7	10	pairing	pairing	NOUN
eurjchem-440	7	11	effects	effect	NOUN
eurjchem-440	7	12	cobalt(iii	cobalt(iii	NOUN
eurjchem-440	7	13	)	)	PUNCT
eurjchem-440	7	14	per	per	ADP
eurjchem-440	7	15	some	some	DET
eurjchem-440	7	16	dicarbo	dicarbo	NOUN
eurjchem-440	7	17	treatment	treatment	NOUN
eurjchem-440	7	18	for	for	ADP
eurjchem-440	7	19	fairly	fairly	ADV
eurjchem-440	7	20	establish	establish	VERB
eurjchem-440	7	21	aquated	aquate	VERB
eurjchem-440	7	22	by	by	ADP
eurjchem-440	7	23	an	an	DET
eurjchem-440	7	24	the	the	DET
eurjchem-440	7	25	aim	aim	NOUN
eurjchem-440	7	26	o	o	NOUN
eurjchem-440	7	27	bromopentaam	bromopentaam	NOUN
eurjchem-440	7	28	solutions	solution	NOUN
eurjchem-440	7	29	[	[	X
eurjchem-440	7	30	0.00	0.00	NUM
eurjchem-440	7	31	na2co3	na2co3	PROPN
eurjchem-440	7	32	contai	contai	NOUN
eurjchem-440	7	33	to	to	PART
eurjchem-440	7	34	determine	determine	VERB
eurjchem-440	7	35	extrathermody	extrathermody	NOUN
eurjchem-440	7	36	on	on	ADP
eurjchem-440	7	37	ion‐pai	ion‐pai	NOUN
eurjchem-440	7	38	i	i	NOUN
eurjchem-440	7	39	)	)	PUNCT
eurjchem-440	7	40	comple	comple	PROPN
eurjchem-440	7	41	ih	ih	X
eurjchem-440	7	42	zeitounia	zeitounia	PROPN
eurjchem-440	7	43	,	,	PUNCT
eurjchem-440	7	44	mar	mar	PROPN
eurjchem-440	7	45	younes	younes	PROPN
eurjchem-440	7	46	rtment	rtment	PROPN
eurjchem-440	7	47	,	,	PUNCT
eurjchem-440	7	48	faculty	faculty	NOUN
eurjchem-440	7	49	of	of	ADP
eurjchem-440	7	50	s	s	PROPN
eurjchem-440	7	51	rtment	rtment	NOUN
eurjchem-440	7	52	,	,	PUNCT
eurjchem-440	7	53	faculty	faculty	NOUN
eurjchem-440	7	54	of	of	ADP
eurjchem-440	7	55	s	s	PROPN
eurjchem-440	7	56	uthor	uthor	PROPN
eurjchem-440	7	57	at	at	ADP
eurjchem-440	7	58	:	:	PUNCT
eurjchem-440	7	59	chemistry	chemistry	NOUN
eurjchem-440	7	60	0	0	NUM
eurjchem-440	7	61	.	.	PUNCT
eurjchem-440	7	62	e‐mail	e‐mail	PUNCT
eurjchem-440	8	1	address	address	NOUN
eurjchem-440	8	2	:	:	PUNCT
eurjchem-440	8	3	f	f	PROPN
eurjchem-440	8	4	ormation	ormation	NOUN
eurjchem-440	8	5	il	il	PROPN
eurjchem-440	8	6	2011	2011	NUM
eurjchem-440	8	7	ed	ed	NOUN
eurjchem-440	8	8	form	form	NOUN
eurjchem-440	8	9	:	:	PUNCT
eurjchem-440	8	10	27	27	NUM
eurjchem-440	8	11	june	june	PROPN
eurjchem-440	8	12	2	2	NUM
eurjchem-440	8	13	y	y	PROPN
eurjchem-440	8	14	2011	2011	NUM
eurjchem-440	8	15	mber	mber	NOUN
eurjchem-440	8	16	2011	2011	NUM
eurjchem-440	8	17	lex	lex	PROPN
eurjchem-440	8	18	d	d	X
eurjchem-440	8	19	on	on	ADP
eurjchem-440	8	20	n	n	PRON
eurjchem-440	8	21	metal	metal	NOUN
eurjchem-440	8	22	comple	comple	ADJ
eurjchem-440	8	23	gical	gical	ADJ
eurjchem-440	8	24	systems	system	NOUN
eurjchem-440	8	25	.	.	PUNCT
eurjchem-440	9	1	ve	ve	AUX
eurjchem-440	9	2	been	be	AUX
eurjchem-440	9	3	the	the	DET
eurjchem-440	9	4	sub	sub	NOUN
eurjchem-440	9	5	nd	nd	ADP
eurjchem-440	9	6	the	the	DET
eurjchem-440	9	7	inhibitio	inhibitio	NOUN
eurjchem-440	9	8	balt(iii	balt(iii	PROPN
eurjchem-440	9	9	)	)	PUNCT
eurjchem-440	9	10	is	be	AUX
eurjchem-440	9	11	bene	bene	NOUN
eurjchem-440	9	12	]	]	PUNCT
eurjchem-440	9	13	.	.	PUNCT
eurjchem-440	10	1	studies	study	NOUN
eurjchem-440	10	2	had	have	VERB
eurjchem-440	10	3	des	des	X
eurjchem-440	10	4	aamminecobalt	aamminecobalt	PROPN
eurjchem-440	10	5	include	include	VERB
eurjchem-440	10	6	nume	nume	NOUN
eurjchem-440	10	7	and	and	CCONJ
eurjchem-440	10	8	specific	specific	ADJ
eurjchem-440	10	9	so	so	ADV
eurjchem-440	10	10	unting	unte	VERB
eurjchem-440	10	11	for	for	ADP
eurjchem-440	10	12	the	the	DET
eurjchem-440	10	13	e	e	NOUN
eurjchem-440	10	14	was	be	AUX
eurjchem-440	10	15	shown	show	VERB
eurjchem-440	10	16	[	[	PUNCT
eurjchem-440	10	17	9	9	NUM
eurjchem-440	10	18	]	]	SYM
eurjchem-440	10	19	t	t	NOUN
eurjchem-440	10	20	anions	anion	NOUN
eurjchem-440	10	21	and	and	CCONJ
eurjchem-440	10	22	)	)	PUNCT
eurjchem-440	10	23	cations	cation	NOUN
eurjchem-440	10	24	und	und	VERB
eurjchem-440	10	25	the	the	DET
eurjchem-440	10	26	free	free	ADJ
eurjchem-440	10	27	cation	cation	NOUN
eurjchem-440	10	28	s	s	NOUN
eurjchem-440	10	29	on	on	ADP
eurjchem-440	10	30	the	the	DET
eurjchem-440	10	31	rate	rate	NOUN
eurjchem-440	10	32	o	o	NOUN
eurjchem-440	10	33	rchlorate	rchlorate	NOUN
eurjchem-440	10	34	in	in	ADP
eurjchem-440	10	35	20	20	NUM
eurjchem-440	10	36	%	%	NOUN
eurjchem-440	10	37	oxylates	oxylate	NOUN
eurjchem-440	10	38	must	must	AUX
eurjchem-440	10	39	r	r	VERB
eurjchem-440	10	40	calculating	calculate	VERB
eurjchem-440	10	41	th	th	ADV
eurjchem-440	10	42	he	he	PRON
eurjchem-440	10	43	d	d	PROPN
eurjchem-440	10	44	that	that	DET
eurjchem-440	10	45	halop	halop	PROPN
eurjchem-440	10	46	essentially	essentially	ADV
eurjchem-440	10	47	diss	diss	ADJ
eurjchem-440	10	48	of	of	ADP
eurjchem-440	10	49	the	the	DET
eurjchem-440	10	50	present	present	NOUN
eurjchem-440	10	51	w	w	PROPN
eurjchem-440	10	52	mminecobalt(ii	mminecobalt(ii	PROPN
eurjchem-440	10	53	08‐0.040	08‐0.040	X
eurjchem-440	10	54	mol	mol	ADP
eurjchem-440	10	55	/	/	SYM
eurjchem-440	10	56	l	l	NOUN
eurjchem-440	10	57	ning	ning	NOUN
eurjchem-440	10	58	tert‐butan	tert‐butan	PROPN
eurjchem-440	10	59	e	e	PROPN
eurjchem-440	10	60	the	the	DET
eurjchem-440	10	61	solvent	solvent	ADJ
eurjchem-440	10	62	ynamic	ynamic	PROPN
eurjchem-440	10	63	parame	parame	NOUN
eurjchem-440	10	64	eu	eu	PROPN
eurjchem-440	10	65	issn	issn	PROPN
eurjchem-440	10	66	2153‐	2153‐	NUM
eurjchem-440	10	67	europ	europ	NOUN
eurjchem-440	10	68	j	j	PROPN
eurjchem-440	10	69	iring	iring	PROPN
eurjchem-440	10	70	effec	effec	PROPN
eurjchem-440	10	71	ex	ex	X
eurjchem-440	10	72	in	in	ADP
eurjchem-440	10	73	malo	malo	PROPN
eurjchem-440	10	74	,	,	PUNCT
eurjchem-440	10	75	gehan	gehan	PROPN
eurjchem-440	10	76	mou	mou	PROPN
eurjchem-440	10	77	a	a	PRON
eurjchem-440	10	78	and	and	CCONJ
eurjchem-440	10	79	moham	moham	PROPN
eurjchem-440	10	80	science	science	NOUN
eurjchem-440	10	81	,	,	PUNCT
eurjchem-440	10	82	beirut	beirut	PROPN
eurjchem-440	10	83	arab	arab	PROPN
eurjchem-440	10	84	science	science	PROPN
eurjchem-440	10	85	,	,	PUNCT
eurjchem-440	10	86	alexandria	alexandria	PROPN
eurjchem-440	10	87	y	y	PROPN
eurjchem-440	10	88	department	department	PROPN
eurjchem-440	10	89	,	,	PUNCT
eurjchem-440	10	90	facu	facu	PROPN
eurjchem-440	10	91	fawzyamira54@ya	fawzyamira54@ya	NOUN
eurjchem-440	10	92	2011	2011	NUM
eurjchem-440	10	93	exes	ex	NOUN
eurjchem-440	10	94	play	play	VERB
eurjchem-440	10	95	a	a	DET
eurjchem-440	10	96	va	va	NOUN
eurjchem-440	10	97	the	the	DET
eurjchem-440	10	98	biological	biological	ADJ
eurjchem-440	10	99	bject	bject	NOUN
eurjchem-440	10	100	of	of	ADP
eurjchem-440	10	101	studies	study	NOUN
eurjchem-440	10	102	on	on	ADP
eurjchem-440	10	103	of	of	ADP
eurjchem-440	10	104	soybean	soybean	NOUN
eurjchem-440	10	105	li	li	PROPN
eurjchem-440	10	106	ficial	ficial	NOUN
eurjchem-440	10	107	for	for	ADP
eurjchem-440	10	108	human	human	ADJ
eurjchem-440	10	109	scribed	scribed	NOUN
eurjchem-440	10	110	the	the	DET
eurjchem-440	10	111	kin	kin	NOUN
eurjchem-440	10	112	t(iii	t(iii	PROPN
eurjchem-440	10	113	)	)	PUNCT
eurjchem-440	10	114	in	in	ADP
eurjchem-440	10	115	differen	differen	NOUN
eurjchem-440	10	116	erous	erous	ADJ
eurjchem-440	10	117	factors	factor	NOUN
eurjchem-440	10	118	,	,	PUNCT
eurjchem-440	10	119	d	d	PRON
eurjchem-440	10	120	olute‐solvent	olute‐solvent	NOUN
eurjchem-440	10	121	in	in	ADP
eurjchem-440	10	122	quilibrium	quilibrium	ADJ
eurjchem-440	10	123	beh	beh	NOUN
eurjchem-440	10	124	that	that	SCONJ
eurjchem-440	10	125	the	the	DET
eurjchem-440	10	126	ion‐pa	ion‐pa	PROPN
eurjchem-440	10	127	halopentaamm	halopentaamm	PROPN
eurjchem-440	10	128	dergo	dergo	PROPN
eurjchem-440	10	129	aquation	aquation	NOUN
eurjchem-440	10	130	ns	ns	NOUN
eurjchem-440	10	131	.	.	PUNCT
eurjchem-440	11	1	it	it	PRON
eurjchem-440	11	2	was	be	AUX
eurjchem-440	11	3	found	find	VERB
eurjchem-440	11	4	of	of	ADP
eurjchem-440	11	5	aquation	aquation	NOUN
eurjchem-440	11	6	of	of	ADP
eurjchem-440	11	7	b	b	NUM
eurjchem-440	11	8	%	%	NOUN
eurjchem-440	11	9	(	(	PUNCT
eurjchem-440	11	10	v	v	NOUN
eurjchem-440	11	11	/	/	SYM
eurjchem-440	11	12	v	v	NOUN
eurjchem-440	11	13	)	)	PUNCT
eurjchem-440	11	14	ethylen	ethylen	NOUN
eurjchem-440	11	15	follow	follow	NOUN
eurjchem-440	11	16	waytt	waytt	NOUN
eurjchem-440	11	17	he	he	PRON
eurjchem-440	11	18	ion‐pair	ion‐pair	PROPN
eurjchem-440	12	1	rat	rat	NOUN
eurjchem-440	12	2	entaammine	entaammine	PROPN
eurjchem-440	12	3	co	co	PROPN
eurjchem-440	12	4	sociative	sociative	ADJ
eurjchem-440	12	5	proce	proce	PROPN
eurjchem-440	12	6	work	work	NOUN
eurjchem-440	12	7	is	be	AUX
eurjchem-440	12	8	to	to	PART
eurjchem-440	12	9	study	study	VERB
eurjchem-440	12	10	ii	ii	NUM
eurjchem-440	12	11	)	)	PUNCT
eurjchem-440	12	12	perchlorate	perchlorate	NOUN
eurjchem-440	12	13	l	l	NOUN
eurjchem-440	12	14	malonic	malonic	ADJ
eurjchem-440	12	15	acid	acid	NOUN
eurjchem-440	12	16	nol	nol	NOUN
eurjchem-440	12	17	(	(	PUNCT
eurjchem-440	12	18	10%:50	10%:50	NUM
eurjchem-440	12	19	%	%	NOUN
eurjchem-440	12	20	,	,	PUNCT
eurjchem-440	12	21	effects	effect	NOUN
eurjchem-440	12	22	on	on	ADP
eurjchem-440	12	23	th	th	NOUN
eurjchem-440	12	24	eters	eter	NOUN
eurjchem-440	12	25	of	of	ADP
eurjchem-440	12	26	activat	activat	PROPN
eurjchem-440	12	27	uropean	uropean	ADJ
eurjchem-440	12	28	journal	journal	PROPN
eurjchem-440	12	29	europe	europe	PROPN
eurjchem-440	12	30	2249	2249	NUM
eurjchem-440	12	31	(	(	PUNCT
eurjchem-440	12	32	print	print	NOUN
eurjchem-440	12	33	)	)	PUNCT
eurjchem-440	12	34	/	/	PUNCT
eurjchem-440	12	35	is	be	AUX
eurjchem-440	12	36	doi:10.5155	doi:10.5155	ADJ
eurjchem-440	12	37	pean	pean	PROPN
eurjchem-440	12	38	jo	jo	PROPN
eurjchem-440	12	39	journal	journal	PROPN
eurjchem-440	12	40	home	home	PROPN
eurjchem-440	12	41	cts	cts	PROPN
eurjchem-440	12	42	of	of	ADP
eurjchem-440	12	43	the	the	DET
eurjchem-440	12	44	onate	onate	PROPN
eurjchem-440	12	45	med	med	PROPN
eurjchem-440	12	46	ustafa	ustafa	PROPN
eurjchem-440	12	47	el‐sub	el‐sub	PROPN
eurjchem-440	12	48	mmad	mmad	PROPN
eurjchem-440	12	49	fawz	fawz	PROPN
eurjchem-440	12	50	b	b	PROPN
eurjchem-440	12	51	university	university	PROPN
eurjchem-440	12	52	,	,	PUNCT
eurjchem-440	12	53	riad	riad	PROPN
eurjchem-440	12	54	e	e	PROPN
eurjchem-440	12	55	a	a	DET
eurjchem-440	12	56	university	university	NOUN
eurjchem-440	12	57	,	,	PUNCT
eurjchem-440	12	58	ibrahim	ibrahim	PROPN
eurjchem-440	12	59	ulty	ulty	PROPN
eurjchem-440	12	60	of	of	ADP
eurjchem-440	12	61	science	science	PROPN
eurjchem-440	12	62	,	,	PUNCT
eurjchem-440	12	63	alex	alex	PROPN
eurjchem-440	12	64	ahoo.com	ahoo.com	X
eurjchem-440	12	65	(	(	PUNCT
eurjchem-440	12	66	m.f	m.f	PROPN
eurjchem-440	12	67	.	.	PROPN
eurjchem-440	12	68	ami	ami	PROPN
eurjchem-440	12	69	abstract	abstract	ADJ
eurjchem-440	12	70	the	the	DET
eurjchem-440	12	71	aquation	aquation	NOUN
eurjchem-440	12	72	o	o	NOUN
eurjchem-440	12	73	anion	anion	NOUN
eurjchem-440	12	74	in	in	ADP
eurjchem-440	12	75	mixe	mixe	PROPN
eurjchem-440	12	76	investigated	investigate	VERB
eurjchem-440	12	77	sp	sp	ADP
eurjchem-440	12	78	log	log	NOUN
eurjchem-440	12	79	(	(	PUNCT
eurjchem-440	12	80	kip	kip	PROPN
eurjchem-440	12	81	)	)	PUNCT
eurjchem-440	12	82	ion‐pa	ion‐pa	NOUN
eurjchem-440	12	83	water	water	NOUN
eurjchem-440	12	84	concentr	concentr	NOUN
eurjchem-440	12	85	extrathermody	extrathermody	NOUN
eurjchem-440	12	86	effect	effect	NOUN
eurjchem-440	12	87	on	on	ADP
eurjchem-440	12	88	the	the	DET
eurjchem-440	12	89	i	i	PROPN
eurjchem-440	12	90	systems	system	NOUN
eurjchem-440	12	91	indicat	indicat	VERB
eurjchem-440	12	92	the	the	DET
eurjchem-440	12	93	extrema	extrema	NOUN
eurjchem-440	12	94	fo	fo	INTJ
eurjchem-440	12	95	be	be	AUX
eurjchem-440	12	96	attributed	attribute	VERB
eurjchem-440	12	97	to	to	ADP
eurjchem-440	12	98	solvent	solvent	PROPN
eurjchem-440	12	99	structu	structu	ADJ
eurjchem-440	12	100	stability	stability	NOUN
eurjchem-440	12	101	of	of	ADP
eurjchem-440	12	102	the	the	DET
eurjchem-440	12	103	∆gip*with	∆gip*with	NOUN
eurjchem-440	12	104	the	the	DET
eurjchem-440	12	105	m	m	NOUN
eurjchem-440	12	106	between	between	ADP
eurjchem-440	12	107	∆hip	∆hip	NOUN
eurjchem-440	12	108	*	*	NUM
eurjchem-440	12	109	a	a	DET
eurjchem-440	12	110	ariety	ariety	NOUN
eurjchem-440	12	111	of	of	ADP
eurjchem-440	12	112	impo	impo	ADJ
eurjchem-440	12	113	activities	activity	NOUN
eurjchem-440	12	114	of	of	ADP
eurjchem-440	12	115	c	c	PROPN
eurjchem-440	12	116	on	on	ADP
eurjchem-440	12	117	the	the	DET
eurjchem-440	12	118	inhibiti	inhibiti	NOUN
eurjchem-440	12	119	poxygenase	poxygenase	PROPN
eurjchem-440	12	120	enz	enz	NOUN
eurjchem-440	12	121	n	n	CCONJ
eurjchem-440	12	122	since	since	SCONJ
eurjchem-440	12	123	it	it	PRON
eurjchem-440	12	124	is	be	AUX
eurjchem-440	12	125	a	a	DET
eurjchem-440	12	126	pa	pa	PROPN
eurjchem-440	12	127	netics	netic	NOUN
eurjchem-440	12	128	of	of	ADP
eurjchem-440	12	129	aquati	aquati	PROPN
eurjchem-440	12	130	nt	nt	PROPN
eurjchem-440	12	131	media	medium	NOUN
eurjchem-440	12	132	[	[	X
eurjchem-440	12	133	4‐8	4‐8	NOUN
eurjchem-440	12	134	]	]	PUNCT
eurjchem-440	12	135	.	.	PUNCT
eurjchem-440	13	1	describing	describe	VERB
eurjchem-440	13	2	prefe	prefe	ADJ
eurjchem-440	13	3	nteractions	nteraction	NOUN
eurjchem-440	13	4	and	and	CCONJ
eurjchem-440	13	5	havior	havior	ADJ
eurjchem-440	13	6	of	of	ADP
eurjchem-440	13	7	electro	electro	PROPN
eurjchem-440	13	8	airs	air	NOUN
eurjchem-440	13	9	formed	form	VERB
eurjchem-440	13	10	betw	betw	PROPN
eurjchem-440	13	11	mine	mine	NOUN
eurjchem-440	13	12	cobalt(iii	cobalt(iii	NOUN
eurjchem-440	13	13	)	)	PUNCT
eurjchem-440	14	1	n	n	CCONJ
eurjchem-440	14	2	at	at	ADP
eurjchem-440	14	3	a	a	DET
eurjchem-440	14	4	faster	fast	ADJ
eurjchem-440	14	5	d	d	NOUN
eurjchem-440	14	6	that	that	PRON
eurjchem-440	14	7	[	[	X
eurjchem-440	14	8	10	10	NUM
eurjchem-440	14	9	]	]	PUNCT
eurjchem-440	14	10	the	the	DET
eurjchem-440	14	11	bromopentaam	bromopentaam	PROPN
eurjchem-440	14	12	ne	ne	NOUN
eurjchem-440	14	13	glycol	glycol	NOUN
eurjchem-440	14	14	solutio	solutio	NOUN
eurjchem-440	14	15	t	t	PROPN
eurjchem-440	14	16	and	and	CCONJ
eurjchem-440	14	17	davies	davy	NOUN
eurjchem-440	14	18	te	te	ADP
eurjchem-440	14	19	coefficients	coefficient	NOUN
eurjchem-440	14	20	.	.	PUNCT
eurjchem-440	15	1	obalt(iii	obalt(iii	PROPN
eurjchem-440	15	2	)	)	PUNCT
eurjchem-440	15	3	comp	comp	NOUN
eurjchem-440	15	4	ess	ess	PUNCT
eurjchem-440	16	1	[	[	X
eurjchem-440	16	2	12	12	NUM
eurjchem-440	16	3	]	]	PUNCT
eurjchem-440	16	4	.	.	PUNCT
eurjchem-440	17	1	y	y	PROPN
eurjchem-440	17	2	of	of	ADP
eurjchem-440	17	3	the	the	DET
eurjchem-440	17	4	aquati	aquati	NOUN
eurjchem-440	17	5	in	in	ADP
eurjchem-440	17	6	malonate	malonate	PROPN
eurjchem-440	17	7	b	b	NOUN
eurjchem-440	17	8	neutralized	neutralize	VERB
eurjchem-440	17	9	by	by	ADP
eurjchem-440	17	10	v	v	NOUN
eurjchem-440	17	11	:	:	PUNCT
eurjchem-440	17	12	v	v	NOUN
eurjchem-440	17	13	)	)	PUNCT
eurjchem-440	17	14	]	]	PUNCT
eurjchem-440	17	15	in	in	ADP
eurjchem-440	17	16	an	an	DET
eurjchem-440	17	17	att	att	PROPN
eurjchem-440	17	18	hermodynamic	hermodynamic	NOUN
eurjchem-440	17	19	tion	tion	NOUN
eurjchem-440	17	20	where	where	SCONJ
eurjchem-440	17	21	the	the	PRON
eurjchem-440	17	22	of	of	ADP
eurjchem-440	17	23	chemistry	chemistry	NOUN
eurjchem-440	17	24	2	2	NUM
eurjchem-440	17	25	(	(	PUNCT
eurjchem-440	17	26	ean	ean	NOUN
eurjchem-440	17	27	journal	journal	NOUN
eurjchem-440	17	28	of	of	ADP
eurjchem-440	17	29	ch	ch	PROPN
eurjchem-440	17	30	ssn	ssn	PROPN
eurjchem-440	17	31	2153‐2257	2153‐2257	NUM
eurjchem-440	17	32	5	5	NUM
eurjchem-440	17	33	/	/	SYM
eurjchem-440	17	34	eurjchem.2.4.4	eurjchem.2.4.4	PROPN
eurjchem-440	17	35	ournal	ournal	ADJ
eurjchem-440	17	36	o	o	NOUN
eurjchem-440	17	37	epage	epage	NOUN
eurjchem-440	17	38	:	:	PUNCT
eurjchem-440	17	39	www.e	www.e	PROPN
eurjchem-440	17	40	kinetics	kinetics	PROPN
eurjchem-440	17	41	o	o	PROPN
eurjchem-440	17	42	dia	dia	PROPN
eurjchem-440	17	43	bruitib	bruitib	PROPN
eurjchem-440	17	44	,	,	PUNCT
eurjchem-440	17	45	zi	zi	NOUN
eurjchem-440	17	46	amirab	amirab	NOUN
eurjchem-440	17	47	,	,	PUNCT
eurjchem-440	17	48	*	*	PUNCT
eurjchem-440	17	49	el‐solh	el‐solh	PROPN
eurjchem-440	17	50	,	,	PUNCT
eurjchem-440	17	51	beirut‐11‐5	beirut‐11‐5	PROPN
eurjchem-440	17	52	mia	mia	PROPN
eurjchem-440	17	53	,	,	PUNCT
eurjchem-440	17	54	alexandria‐21	alexandria‐21	PROPN
eurjchem-440	17	55	xandria	xandria	PROPN
eurjchem-440	17	56	university	university	PROPN
eurjchem-440	17	57	,	,	PUNCT
eurjchem-440	17	58	ira	ira	PROPN
eurjchem-440	17	59	)	)	PUNCT
eurjchem-440	17	60	.	.	PUNCT
eurjchem-440	18	1	of	of	ADP
eurjchem-440	18	2	bromopentaa	bromopentaa	PROPN
eurjchem-440	18	3	ed	ed	PROPN
eurjchem-440	18	4	solvent	solvent	ADJ
eurjchem-440	18	5	med	med	ADJ
eurjchem-440	18	6	pectrophotometr	pectrophotometr	NOUN
eurjchem-440	18	7	air	air	NOUN
eurjchem-440	18	8	rate	rate	PROPN
eurjchem-440	18	9	constan	constan	ADJ
eurjchem-440	18	10	ration	ration	NOUN
eurjchem-440	18	11	and	and	CCONJ
eurjchem-440	18	12	grun	grun	VERB
eurjchem-440	18	13	namic	namic	ADJ
eurjchem-440	18	14	analyses	analysis	NOUN
eurjchem-440	18	15	ion‐pair	ion‐pair	PROPN
eurjchem-440	18	16	aquatio	aquatio	NOUN
eurjchem-440	18	17	te	te	ADP
eurjchem-440	18	18	the	the	DET
eurjchem-440	18	19	existence	existence	NOUN
eurjchem-440	18	20	und	und	VERB
eurjchem-440	18	21	in	in	ADP
eurjchem-440	18	22	the	the	DET
eurjchem-440	18	23	chan	chan	PROPN
eurjchem-440	18	24	o	o	NOUN
eurjchem-440	18	25	the	the	DET
eurjchem-440	18	26	change	change	NOUN
eurjchem-440	18	27	of	of	ADP
eurjchem-440	18	28	ure	ure	PROPN
eurjchem-440	18	29	.	.	PUNCT
eurjchem-440	19	1	application	application	NOUN
eurjchem-440	19	2	e	e	NOUN
eurjchem-440	19	3	initial	initial	NOUN
eurjchem-440	19	4	and	and	CCONJ
eurjchem-440	19	5	the	the	DET
eurjchem-440	19	6	mole	mole	NOUN
eurjchem-440	19	7	fraction	fraction	NOUN
eurjchem-440	19	8	of	of	ADP
eurjchem-440	19	9	and	and	CCONJ
eurjchem-440	19	10	∆sip	∆sip	NOUN
eurjchem-440	19	11	*	*	NOUN
eurjchem-440	19	12	.	.	PUNCT
eurjchem-440	20	1	ortant	ortant	ADJ
eurjchem-440	20	2	cobalt	cobalt	NOUN
eurjchem-440	20	3	on	on	ADP
eurjchem-440	20	4	of	of	ADP
eurjchem-440	20	5	zyme	zyme	PROPN
eurjchem-440	20	6	art	art	NOUN
eurjchem-440	20	7	of	of	ADP
eurjchem-440	20	8	on	on	ADP
eurjchem-440	20	9	of	of	ADP
eurjchem-440	20	10	such	such	ADJ
eurjchem-440	20	11	eren‐	eren‐	NOUN
eurjchem-440	20	12	d	d	NOUN
eurjchem-440	20	13	are	be	AUX
eurjchem-440	20	14	olytes	olyte	NOUN
eurjchem-440	20	15	ween	ween	NOUN
eurjchem-440	20	16	and	and	CCONJ
eurjchem-440	20	17	rate	rate	NOUN
eurjchem-440	20	18	e	e	PROPN
eurjchem-440	20	19	ion‐	ion‐	PROPN
eurjchem-440	20	20	mmine	mmine	VERB
eurjchem-440	20	21	ons	ons	PROPN
eurjchem-440	20	22	of	of	ADP
eurjchem-440	20	23	[	[	X
eurjchem-440	20	24	11	11	NUM
eurjchem-440	20	25	]	]	PUNCT
eurjchem-440	20	26	it	it	PRON
eurjchem-440	20	27	is	be	AUX
eurjchem-440	20	28	plexes	plexe	NOUN
eurjchem-440	20	29	on	on	ADP
eurjchem-440	20	30	of	of	ADP
eurjchem-440	20	31	buffer	buffer	NOUN
eurjchem-440	20	32	80	80	NUM
eurjchem-440	20	33	%	%	NOUN
eurjchem-440	20	34	tempt	tempt	NOUN
eurjchem-440	20	35	and	and	CCONJ
eurjchem-440	20	36	data	datum	NOUN
eurjchem-440	20	37	can	can	AUX
eurjchem-440	20	38	inter	inter	VERB
eurjchem-440	20	39	2	2	NUM
eurjchem-440	20	40	.	.	PUNCT
eurjchem-440	20	41	ex	ex	X
eurjchem-440	20	42	2.1	2.1	NUM
eurjchem-440	20	43	.	.	PUNCT
eurjchem-440	21	1	c	c	PROPN
eurjchem-440	21	2	malo	malo	PROPN
eurjchem-440	21	3	purc	purc	PROPN
eurjchem-440	21	4	purc	purc	NOUN
eurjchem-440	21	5	purc	purc	NOUN
eurjchem-440	21	6	acid	acid	NOUN
eurjchem-440	21	7	coba	coba	NOUN
eurjchem-440	21	8	meth	meth	NOUN
eurjchem-440	21	9	2.2	2.2	NUM
eurjchem-440	21	10	.	.	PUNCT
eurjchem-440	22	1	t	t	AUX
eurjchem-440	22	2	10	10	NUM
eurjchem-440	22	3	%	%	NOUN
eurjchem-440	22	4	30‐6	30‐6	NUM
eurjchem-440	22	5	heli	heli	PROPN
eurjchem-440	22	6	spec	spec	NOUN
eurjchem-440	22	7	heat	heat	VERB
eurjchem-440	22	8	the	the	DET
eurjchem-440	22	9	the	the	DET
eurjchem-440	22	10	m	m	PROPN
eurjchem-440	22	11	(	(	PUNCT
eurjchem-440	22	12	4	4	NUM
eurjchem-440	22	13	)	)	PUNCT
eurjchem-440	22	14	(	(	PUNCT
eurjchem-440	22	15	2011	2011	NUM
eurjchem-440	22	16	)	)	PUNCT
eurjchem-440	22	17	489‐4	489‐4	PROPN
eurjchem-440	22	18	hemistry	hemistry	NOUN
eurjchem-440	22	19	(	(	PUNCT
eurjchem-440	22	20	online	online	ADJ
eurjchem-440	22	21	)	)	PUNCT
eurjchem-440	22	22			NOUN
eurjchem-440	22	23	2011	2011	NUM
eurjchem-440	23	1	489‐494.440	489‐494.440	PROPN
eurjchem-440	23	2	of	of	ADP
eurjchem-440	23	3	chem	chem	NOUN
eurjchem-440	23	4	eurjchem.com	eurjchem.com	X
eurjchem-440	23	5	of	of	ADP
eurjchem-440	23	6	aquatio	aquatio	NOUN
eurjchem-440	23	7	5020	5020	NUM
eurjchem-440	23	8	,	,	PUNCT
eurjchem-440	23	9	lebanon	lebanon	PROPN
eurjchem-440	23	10	321	321	NUM
eurjchem-440	23	11	,	,	PUNCT
eurjchem-440	23	12	egypt	egypt	PROPN
eurjchem-440	23	13	p.o	p.o	PROPN
eurjchem-440	23	14	.	.	PROPN
eurjchem-440	23	15	box	box	PROPN
eurjchem-440	23	16	426	426	NUM
eurjchem-440	23	17	,	,	PUNCT
eurjchem-440	23	18	ibrah	ibrah	PROPN
eurjchem-440	23	19	mminecobalt(iii	mminecobalt(iii	PROPN
eurjchem-440	23	20	dia	dia	PROPN
eurjchem-440	23	21	of	of	ADP
eurjchem-440	23	22	water	water	PROPN
eurjchem-440	24	1	w	w	PROPN
eurjchem-440	24	2	rically	rically	ADV
eurjchem-440	24	3	at	at	ADP
eurjchem-440	24	4	differe	differe	X
eurjchem-440	24	5	nts	nt	NOUN
eurjchem-440	24	6	against	against	ADP
eurjchem-440	24	7	the	the	DET
eurjchem-440	24	8	nwald‐winstein	nwald‐winstein	NOUN
eurjchem-440	24	9	y	y	PROPN
eurjchem-440	24	10	of	of	ADP
eurjchem-440	24	11	the	the	DET
eurjchem-440	24	12	kinetic	kinetic	NOUN
eurjchem-440	24	13	on	on	ADP
eurjchem-440	24	14	reactions	reaction	NOUN
eurjchem-440	24	15	.	.	PUNCT
eurjchem-440	25	1	th	th	X
eurjchem-440	25	2	of	of	ADP
eurjchem-440	25	3	compensatio	compensatio	PROPN
eurjchem-440	25	4	ge	ge	PROPN
eurjchem-440	25	5	of	of	ADP
eurjchem-440	25	6	∆hip	∆hip	PROPN
eurjchem-440	25	7	*	*	PUNCT
eurjchem-440	25	8	and	and	CCONJ
eurjchem-440	25	9	∆	∆	PROPN
eurjchem-440	25	10	the	the	DET
eurjchem-440	25	11	physical	physical	ADJ
eurjchem-440	25	12	pr	pr	NOUN
eurjchem-440	25	13	of	of	ADP
eurjchem-440	25	14	a	a	DET
eurjchem-440	25	15	free	free	ADJ
eurjchem-440	25	16	energ	energ	NOUN
eurjchem-440	25	17	e	e	NOUN
eurjchem-440	25	18	transition	transition	NOUN
eurjchem-440	25	19	stat	stat	PROPN
eurjchem-440	25	20	f	f	PROPN
eurjchem-440	26	1	the	the	DET
eurjchem-440	26	2	co‐solvent	co‐solvent	ADJ
eurjchem-440	26	3	be	be	AUX
eurjchem-440	26	4	linked	link	VERB
eurjchem-440	26	5	to	to	ADP
eurjchem-440	26	6	o	o	PROPN
eurjchem-440	26	7	raction	raction	NOUN
eurjchem-440	26	8	.	.	PUNCT
eurjchem-440	27	1	xperimental	xperimental	ADJ
eurjchem-440	27	2	reagents	reagent	NOUN
eurjchem-440	27	3	cobalt(ii	cobalt(ii	ADJ
eurjchem-440	27	4	)	)	PUNCT
eurjchem-440	27	5	carb	carb	PROPN
eurjchem-440	27	6	onic	onic	ADJ
eurjchem-440	27	7	acid	acid	NOUN
eurjchem-440	27	8	,	,	PUNCT
eurjchem-440	27	9	so	so	ADV
eurjchem-440	27	10	chased	chase	VERB
eurjchem-440	27	11	from	from	ADP
eurjchem-440	27	12	f	f	PROPN
eurjchem-440	27	13	chased	chase	VERB
eurjchem-440	27	14	from	from	ADP
eurjchem-440	27	15	chased	chase	VERB
eurjchem-440	27	16	from	from	ADP
eurjchem-440	27	17	ch	ch	NOUN
eurjchem-440	27	18	60	60	NUM
eurjchem-440	27	19	%	%	NOUN
eurjchem-440	27	20	was	be	AUX
eurjchem-440	27	21	purc	purc	NOUN
eurjchem-440	27	22	alt(iii	alt(iii	NOUN
eurjchem-440	27	23	)	)	PUNCT
eurjchem-440	27	24	perchlo	perchlo	PROPN
eurjchem-440	27	25	hod	hod	NOUN
eurjchem-440	27	26	of	of	ADP
eurjchem-440	27	27	hynes	hynes	PROPN
eurjchem-440	27	28	[	[	X
eurjchem-440	27	29	1	1	NUM
eurjchem-440	27	30	procedure	procedure	NOUN
eurjchem-440	27	31	the	the	DET
eurjchem-440	27	32	rate	rate	NOUN
eurjchem-440	27	33	of	of	ADP
eurjchem-440	27	34	aq	aq	NOUN
eurjchem-440	27	35	%	%	NOUN
eurjchem-440	27	36	:	:	PUNCT
eurjchem-440	27	37	50	50	NUM
eurjchem-440	27	38	%	%	NOUN
eurjchem-440	27	39	(	(	PUNCT
eurjchem-440	27	40	v	v	NOUN
eurjchem-440	27	41	:	:	PUNCT
eurjchem-440	27	42	v	v	NOUN
eurjchem-440	27	43	)	)	PUNCT
eurjchem-440	27	44	of	of	ADP
eurjchem-440	27	45	t	t	PROPN
eurjchem-440	27	46	60	60	NUM
eurjchem-440	27	47	oc	oc	NOUN
eurjchem-440	27	48	was	be	AUX
eurjchem-440	27	49	follo	follo	PROPN
eurjchem-440	27	50	os	os	PROPN
eurjchem-440	28	1	alpha	alpha	NOUN
eurjchem-440	28	2	and	and	CCONJ
eurjchem-440	28	3	b	b	PROPN
eurjchem-440	28	4	ctrophotometer	ctrophotometer	NOUN
eurjchem-440	28	5	ted	te	VERB
eurjchem-440	28	6	by	by	ADP
eurjchem-440	28	7	water	water	NOUN
eurjchem-440	28	8	ci	ci	PROPN
eurjchem-440	28	9	inflow	inflow	NOUN
eurjchem-440	28	10	and	and	CCONJ
eurjchem-440	28	11	the	the	DET
eurjchem-440	28	12	mean	mean	ADJ
eurjchem-440	28	13	temperat	temperat	NOUN
eurjchem-440	28	14	494	494	NUM
eurjchem-440	28	15	1	1	NUM
eurjchem-440	28	16	eurjchem	eurjchem	PROPN
eurjchem-440	28	17	mistry	mistry	PROPN
eurjchem-440	28	18	m	m	VERB
eurjchem-440	28	19	on	on	ADP
eurjchem-440	28	20	of	of	ADP
eurjchem-440	28	21	brom	brom	PROPN
eurjchem-440	28	22	himia	himia	NOUN
eurjchem-440	28	23	,	,	PUNCT
eurjchem-440	28	24	alexandria‐2	alexandria‐2	PROPN
eurjchem-440	28	25	i	i	NOUN
eurjchem-440	28	26	)	)	PUNCT
eurjchem-440	28	27	ion	ion	NOUN
eurjchem-440	28	28	in	in	ADP
eurjchem-440	28	29	the	the	DET
eurjchem-440	28	30	pr	pr	NOUN
eurjchem-440	28	31	with	with	ADP
eurjchem-440	28	32	tert‐butano	tert‐butano	PROPN
eurjchem-440	28	33	nt	nt	ADP
eurjchem-440	28	34	temperatures	temperature	NOUN
eurjchem-440	28	35	reciprocal	reciprocal	ADJ
eurjchem-440	28	36	of	of	ADP
eurjchem-440	28	37	th	th	NUM
eurjchem-440	28	38	y	y	PROPN
eurjchem-440	28	39	values	value	NOUN
eurjchem-440	28	40	were	be	AUX
eurjchem-440	28	41	f	f	PROPN
eurjchem-440	28	42	data	datum	NOUN
eurjchem-440	28	43	have	have	AUX
eurjchem-440	28	44	been	be	AUX
eurjchem-440	28	45	he	he	PRON
eurjchem-440	28	46	obtained	obtain	VERB
eurjchem-440	28	47	iso	iso	NOUN
eurjchem-440	28	48	n	n	DET
eurjchem-440	28	49	effect	effect	NOUN
eurjchem-440	28	50	arising	arise	VERB
eurjchem-440	28	51	∆sip*with	∆sip*with	ADP
eurjchem-440	28	52	the	the	DET
eurjchem-440	28	53	mo	mo	PROPN
eurjchem-440	28	54	operties	opertie	NOUN
eurjchem-440	28	55	of	of	ADP
eurjchem-440	28	56	the	the	DET
eurjchem-440	28	57	gy	gy	PROPN
eurjchem-440	28	58	cycle	cycle	NOUN
eurjchem-440	28	59	is	be	AUX
eurjchem-440	28	60	perfo	perfo	ADJ
eurjchem-440	28	61	te	te	ADP
eurjchem-440	28	62	of	of	ADP
eurjchem-440	28	63	the	the	DET
eurjchem-440	28	64	compl	compl	NOUN
eurjchem-440	28	65	was	be	AUX
eurjchem-440	28	66	found	find	VERB
eurjchem-440	28	67	,	,	PUNCT
eurjchem-440	28	68	ind	ind	NOUN
eurjchem-440	28	69	obtain	obtain	VERB
eurjchem-440	28	70	informat	informat	ADJ
eurjchem-440	28	71	bonate	bonate	NOUN
eurjchem-440	28	72	,	,	PUNCT
eurjchem-440	28	73	hydrob	hydrob	PROPN
eurjchem-440	28	74	dium	dium	PROPN
eurjchem-440	28	75	carbona	carbona	PROPN
eurjchem-440	28	76	fluka	fluka	PROPN
eurjchem-440	28	77	chemika	chemika	PROPN
eurjchem-440	28	78	riedel‐de	riedel‐de	PROPN
eurjchem-440	28	79	haë	haë	PROPN
eurjchem-440	28	80	hemical	hemical	ADJ
eurjchem-440	28	81	manag	manag	PROPN
eurjchem-440	28	82	chased	chase	VERB
eurjchem-440	28	83	from	from	ADP
eurjchem-440	28	84	me	i	PRON
eurjchem-440	28	85	orate	orate	ADJ
eurjchem-440	28	86	complex	complex	ADJ
eurjchem-440	28	87	13	13	NUM
eurjchem-440	28	88	]	]	PUNCT
eurjchem-440	28	89	.	.	PUNCT
eurjchem-440	29	1	quation	quation	NOUN
eurjchem-440	29	2	of	of	ADP
eurjchem-440	29	3	[	[	X
eurjchem-440	29	4	co	co	NOUN
eurjchem-440	29	5	tert‐butanol	tert‐butanol	PROPN
eurjchem-440	29	6	wit	wit	NOUN
eurjchem-440	29	7	owed	owe	VERB
eurjchem-440	29	8	spectrop	spectrop	NOUN
eurjchem-440	29	9	beta	beta	NOUN
eurjchem-440	29	10	spectroph	spectroph	NOUN
eurjchem-440	29	11	r	r	NOUN
eurjchem-440	29	12	was	be	AUX
eurjchem-440	29	13	fitted	fit	VERB
eurjchem-440	29	14	wi	wi	PROPN
eurjchem-440	29	15	irculating	irculate	VERB
eurjchem-440	29	16	from	from	ADP
eurjchem-440	29	17	e	e	PROPN
eurjchem-440	29	18	outflow	outflow	NOUN
eurjchem-440	29	19	temp	temp	PROPN
eurjchem-440	29	20	ture	ture	PROPN
eurjchem-440	29	21	was	be	AUX
eurjchem-440	29	22	taken	take	VERB
eurjchem-440	29	23	a	a	DET
eurjchem-440	29	24	mopentaa	mopentaa	ADV
eurjchem-440	29	25	21321	21321	NUM
eurjchem-440	29	26	,	,	PUNCT
eurjchem-440	29	27	egypt	egypt	PROPN
eurjchem-440	29	28	.	.	PUNCT
eurjchem-440	30	1	tel	tel	PROPN
eurjchem-440	30	2	.	.	PUNCT
eurjchem-440	30	3	:	:	PUNCT
eurjchem-440	31	1	esence	esence	NOUN
eurjchem-440	31	2	of	of	ADP
eurjchem-440	31	3	ion‐p	ion‐p	PROPN
eurjchem-440	31	4	ol	ol	PROPN
eurjchem-440	31	5	(	(	PUNCT
eurjchem-440	31	6	10%:50	10%:50	NUM
eurjchem-440	31	7	%	%	NOUN
eurjchem-440	31	8	,	,	PUNCT
eurjchem-440	31	9	v	v	NOUN
eurjchem-440	31	10	s	s	X
eurjchem-440	31	11	(	(	PUNCT
eurjchem-440	31	12	30‐60	30‐60	NUM
eurjchem-440	31	13	oc	oc	NOUN
eurjchem-440	31	14	)	)	PUNCT
eurjchem-440	31	15	.	.	PUNCT
eurjchem-440	32	1	no	no	INTJ
eurjchem-440	32	2	he	he	PRON
eurjchem-440	32	3	dielectric	dielectric	ADJ
eurjchem-440	32	4	con	con	PROPN
eurjchem-440	32	5	found	find	VERB
eurjchem-440	32	6	.	.	PUNCT
eurjchem-440	33	1	the	the	DET
eurjchem-440	33	2	therm	therm	NOUN
eurjchem-440	33	3	n	n	CCONJ
eurjchem-440	33	4	discussed	discuss	VERB
eurjchem-440	33	5	in	in	ADP
eurjchem-440	33	6	te	te	PROPN
eurjchem-440	33	7	okinetic	okinetic	ADJ
eurjchem-440	33	8	temper	temper	NOUN
eurjchem-440	33	9	from	from	ADP
eurjchem-440	33	10	solute‐solv	solute‐solv	ADJ
eurjchem-440	33	11	ole	ole	ADJ
eurjchem-440	33	12	fraction	fraction	NOUN
eurjchem-440	33	13	of	of	ADP
eurjchem-440	33	14	th	th	NUM
eurjchem-440	33	15	solvent‐water	solvent‐water	NOUN
eurjchem-440	34	1	m	m	VERB
eurjchem-440	34	2	ormed	ormed	ADJ
eurjchem-440	34	3	to	to	PART
eurjchem-440	34	4	compa	compa	PROPN
eurjchem-440	34	5	ex	ex	PROPN
eurjchem-440	34	6	.	.	PUNCT
eurjchem-440	35	1	however	however	ADV
eurjchem-440	35	2	,	,	PUNCT
eurjchem-440	35	3	sm	sm	PROPN
eurjchem-440	35	4	dicating	dicate	VERB
eurjchem-440	35	5	a	a	DET
eurjchem-440	35	6	comp	comp	NOUN
eurjchem-440	35	7	tion	tion	NOUN
eurjchem-440	35	8	about	about	ADP
eurjchem-440	35	9	the	the	DET
eurjchem-440	35	10	bromic	bromic	ADJ
eurjchem-440	35	11	acid	acid	PROPN
eurjchem-440	35	12	4	4	NUM
eurjchem-440	35	13	ate	eat	VERB
eurjchem-440	35	14	and	and	CCONJ
eurjchem-440	35	15	tert‐	tert‐	VERB
eurjchem-440	35	16	a.	a.	NOUN
eurjchem-440	35	17	hydrogen	hydrogen	PROPN
eurjchem-440	35	18	p	p	PROPN
eurjchem-440	35	19	ën	ën	PROPN
eurjchem-440	35	20	.	.	PUNCT
eurjchem-440	36	1	hydrochlo	hydrochlo	PROPN
eurjchem-440	36	2	gement	gement	NOUN
eurjchem-440	36	3	consult	consult	NOUN
eurjchem-440	36	4	erck	erck	NOUN
eurjchem-440	36	5	.	.	PUNCT
eurjchem-440	37	1	the	the	DET
eurjchem-440	37	2	brom	brom	NOUN
eurjchem-440	37	3	was	be	AUX
eurjchem-440	37	4	prepared	prepare	VERB
eurjchem-440	37	5	o(nh3)5br](clo4	o(nh3)5br](clo4	PROPN
eurjchem-440	37	6	th	th	X
eurjchem-440	37	7	malonate	malonate	VERB
eurjchem-440	37	8	bu	bu	ADV
eurjchem-440	37	9	hotometrically	hotometrically	ADV
eurjchem-440	37	10	otometer	otometer	ADV
eurjchem-440	37	11	at	at	ADP
eurjchem-440	37	12	λ	λ	X
eurjchem-440	37	13	th	th	X
eurjchem-440	37	14	thermostate	thermostate	NOUN
eurjchem-440	37	15	a	a	DET
eurjchem-440	37	16	heto	heto	NOUN
eurjchem-440	37	17	hmt	hmt	NOUN
eurjchem-440	37	18	2	2	NUM
eurjchem-440	37	19	peratures	perature	NOUN
eurjchem-440	37	20	were	be	AUX
eurjchem-440	37	21	as	as	ADP
eurjchem-440	37	22	that	that	PRON
eurjchem-440	37	23	of	of	ADP
eurjchem-440	37	24	the	the	DET
eurjchem-440	37	25	ce	ce	PROPN
eurjchem-440	37	26	ammine	ammine	PROPN
eurjchem-440	37	27	+2.034276580	+2.034276580	PROPN
eurjchem-440	37	28	;	;	PUNCT
eurjchem-440	37	29	airing	air	VERB
eurjchem-440	37	30	malonate	malonate	VERB
eurjchem-440	37	31	v	v	ADP
eurjchem-440	37	32	:	:	PUNCT
eurjchem-440	37	33	v	v	NOUN
eurjchem-440	37	34	)	)	PUNCT
eurjchem-440	37	35	have	have	AUX
eurjchem-440	37	36	been	be	AUX
eurjchem-440	37	37	onlinear	onlinear	ADJ
eurjchem-440	37	38	plots	plot	NOUN
eurjchem-440	37	39	of	of	ADP
eurjchem-440	37	40	nstant	nstant	ADJ
eurjchem-440	37	41	d	d	PROPN
eurjchem-440	37	42	,	,	PUNCT
eurjchem-440	37	43	log	log	NOUN
eurjchem-440	37	44	of	of	ADP
eurjchem-440	37	45	modynamic	modynamic	NOUN
eurjchem-440	37	46	and	and	CCONJ
eurjchem-440	37	47	erms	erm	NOUN
eurjchem-440	37	48	of	of	ADP
eurjchem-440	37	49	solvent	solvent	ADJ
eurjchem-440	37	50	ratures	rature	NOUN
eurjchem-440	37	51	of	of	ADP
eurjchem-440	37	52	these	these	DET
eurjchem-440	37	53	vent	vent	NOUN
eurjchem-440	37	54	interaction	interaction	NOUN
eurjchem-440	37	55	e	e	NOUN
eurjchem-440	37	56	co‐solvent	co‐solvent	NOUN
eurjchem-440	37	57	can	can	AUX
eurjchem-440	37	58	mixture	mixture	VERB
eurjchem-440	37	59	with	with	ADP
eurjchem-440	37	60	the	the	PRON
eurjchem-440	37	61	are	be	AUX
eurjchem-440	37	62	between	between	ADP
eurjchem-440	37	63	the	the	DET
eurjchem-440	37	64	mall	mall	NOUN
eurjchem-440	37	65	changes	change	NOUN
eurjchem-440	37	66	in	in	ADP
eurjchem-440	37	67	ensating	ensate	VERB
eurjchem-440	37	68	effects	effect	NOUN
eurjchem-440	37	69	solute‐solvent	solute‐solvent	VERB
eurjchem-440	37	70	8	8	NUM
eurjchem-440	37	71	%	%	NOUN
eurjchem-440	37	72	,	,	PUNCT
eurjchem-440	37	73	ammonia	ammonia	NOUN
eurjchem-440	37	74	,	,	PUNCT
eurjchem-440	37	75	‐butanol	‐butanol	PROPN
eurjchem-440	37	76	were	be	AUX
eurjchem-440	37	77	peroxide	peroxide	ADJ
eurjchem-440	37	78	,	,	PUNCT
eurjchem-440	37	79	were	be	AUX
eurjchem-440	37	80	oric	oric	ADJ
eurjchem-440	37	81	acid	acid	PROPN
eurjchem-440	37	82	was	be	AUX
eurjchem-440	37	83	ting	te	VERB
eurjchem-440	37	84	.	.	PUNCT
eurjchem-440	38	1	perchloric	perchloric	ADJ
eurjchem-440	38	2	opentaammine	opentaammine	PROPN
eurjchem-440	39	1	d	d	VERB
eurjchem-440	39	2	by	by	ADP
eurjchem-440	39	3	using	use	VERB
eurjchem-440	39	4	the	the	DET
eurjchem-440	39	5	4)2	4)2	PROPN
eurjchem-440	39	6	complex	complex	NOUN
eurjchem-440	39	7	in	in	ADP
eurjchem-440	39	8	uffer	uffer	PROPN
eurjchem-440	39	9	solution	solution	NOUN
eurjchem-440	39	10	at	at	ADP
eurjchem-440	39	11	using	use	VERB
eurjchem-440	39	12	unicam	unicam	NOUN
eurjchem-440	39	13	=	=	VERB
eurjchem-440	40	1	250	250	NUM
eurjchem-440	40	2	nm	nm	NOUN
eurjchem-440	40	3	.	.	PUNCT
eurjchem-440	41	1	the	the	DET
eurjchem-440	41	2	ed	ed	PROPN
eurjchem-440	41	3	cell	cell	NOUN
eurjchem-440	41	4	holders	holder	NOUN
eurjchem-440	41	5	,	,	PUNCT
eurjchem-440	41	6	00	00	PUNCT
eurjchem-440	41	7	thermostat	thermostat	PROPN
eurjchem-440	41	8	.	.	PROPN
eurjchem-440	41	9	measured	measure	VERB
eurjchem-440	41	10	and	and	CCONJ
eurjchem-440	41	11	ell	ell	NOUN
eurjchem-440	41	12	.	.	PUNCT
eurjchem-440	42	1	e	e	PROPN
eurjchem-440	42	2	n	n	NUM
eurjchem-440	42	3	f	f	PROPN
eurjchem-440	42	4	f	f	PROPN
eurjchem-440	42	5	d	d	PROPN
eurjchem-440	42	6	t	t	PROPN
eurjchem-440	42	7	e	e	X
eurjchem-440	42	8	.	.	PUNCT
eurjchem-440	43	1	n	n	PROPN
eurjchem-440	43	2	e	e	NOUN
eurjchem-440	43	3	e	e	ADP
eurjchem-440	43	4	n	n	PROPN
eurjchem-440	43	5	s	s	PROPN
eurjchem-440	43	6	t	t	NOUN
eurjchem-440	43	7	,	,	PUNCT
eurjchem-440	43	8	e	e	X
eurjchem-440	43	9	e	e	NOUN
eurjchem-440	43	10	s	s	PROPN
eurjchem-440	43	11	c	c	NOUN
eurjchem-440	43	12	e	e	X
eurjchem-440	43	13	e	e	X
eurjchem-440	43	14	n	n	PROPN
eurjchem-440	43	15	t	t	PROPN
eurjchem-440	43	16	m	m	PROPN
eurjchem-440	43	17	e	e	NOUN
eurjchem-440	43	18	,	,	PUNCT
eurjchem-440	43	19	.	.	PUNCT
eurjchem-440	44	1	d	d	NOUN
eurjchem-440	44	2	490	490	NUM
eurjchem-440	44	3	zeitouni	zeitouni	NOUN
eurjchem-440	44	4	et	et	PROPN
eurjchem-440	44	5	al	al	PROPN
eurjchem-440	44	6	.	.	PUNCT
eurjchem-440	44	7	/	/	SYM
eurjchem-440	44	8	european	european	PROPN
eurjchem-440	44	9	journal	journal	PROPN
eurjchem-440	44	10	of	of	ADP
eurjchem-440	44	11	chemistry	chemistry	NOUN
eurjchem-440	44	12	2	2	NUM
eurjchem-440	44	13	(	(	PUNCT
eurjchem-440	44	14	4	4	NUM
eurjchem-440	44	15	)	)	PUNCT
eurjchem-440	44	16	(	(	PUNCT
eurjchem-440	44	17	2011	2011	NUM
eurjchem-440	44	18	)	)	PUNCT
eurjchem-440	44	19	489‐494	489‐494	NUM
eurjchem-440	44	20	table	table	NOUN
eurjchem-440	44	21	1	1	NUM
eurjchem-440	44	22	.	.	PUNCT
eurjchem-440	45	1	values	value	NOUN
eurjchem-440	45	2	of	of	ADP
eurjchem-440	45	3	rate	rate	NOUN
eurjchem-440	45	4	constants	constant	NOUN
eurjchem-440	45	5	(	(	PUNCT
eurjchem-440	45	6	kox106	kox106	NOUN
eurjchem-440	45	7	)	)	PUNCT
eurjchem-440	45	8	in	in	ADP
eurjchem-440	45	9	sec‐1	sec‐1	NUM
eurjchem-440	45	10	for	for	ADP
eurjchem-440	45	11	the	the	DET
eurjchem-440	45	12	aquation	aquation	NOUN
eurjchem-440	45	13	of	of	ADP
eurjchem-440	45	14	[	[	X
eurjchem-440	45	15	co(nh3)5br]2	co(nh3)5br]2	NOUN
eurjchem-440	45	16	+	+	X
eurjchem-440	45	17	in	in	ADP
eurjchem-440	45	18	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	45	19	(	(	PUNCT
eurjchem-440	45	20	10‐50	10‐50	NUM
eurjchem-440	45	21	%	%	NOUN
eurjchem-440	45	22	)	)	PUNCT
eurjchem-440	45	23	at	at	ADP
eurjchem-440	45	24	different	different	ADJ
eurjchem-440	45	25	temperatures	temperature	NOUN
eurjchem-440	45	26	.	.	PUNCT
eurjchem-440	46	1	t	t	PROPN
eurjchem-440	46	2	,	,	PUNCT
eurjchem-440	46	3	oc	oc	ADP
eurjchem-440	46	4	10	10	NUM
eurjchem-440	46	5	%	%	NOUN
eurjchem-440	46	6	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	46	7	20	20	NUM
eurjchem-440	46	8	%	%	NOUN
eurjchem-440	46	9	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	46	10	30	30	NUM
eurjchem-440	46	11	%	%	NOUN
eurjchem-440	46	12	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	46	13	40	40	NUM
eurjchem-440	46	14	%	%	NOUN
eurjchem-440	46	15	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	46	16	50	50	NUM
eurjchem-440	46	17	%	%	NOUN
eurjchem-440	46	18	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	46	19	30	30	NUM
eurjchem-440	46	20	2.96	2.96	NUM
eurjchem-440	46	21	2.68	2.68	NUM
eurjchem-440	46	22	0.11	0.11	NUM
eurjchem-440	46	23	0.61	0.61	NUM
eurjchem-440	46	24	4.45	4.45	NUM
eurjchem-440	46	25	35	35	NUM
eurjchem-440	46	26	3.32	3.32	NUM
eurjchem-440	46	27	7.12	7.12	NUM
eurjchem-440	46	28	0.72	0.72	NUM
eurjchem-440	46	29	1.09	1.09	NUM
eurjchem-440	46	30	4.61	4.61	NUM
eurjchem-440	46	31	40	40	NUM
eurjchem-440	46	32	12.10	12.10	NUM
eurjchem-440	46	33	17.00	17.00	NUM
eurjchem-440	46	34	4.83	4.83	NUM
eurjchem-440	46	35	18.30	18.30	NUM
eurjchem-440	46	36	9.60	9.60	NUM
eurjchem-440	46	37	50	50	NUM
eurjchem-440	46	38	92.30	92.30	NUM
eurjchem-440	46	39	93.90	93.90	NUM
eurjchem-440	46	40	95.70	95.70	NUM
eurjchem-440	46	41	44.80	44.80	NUM
eurjchem-440	46	42	94.20	94.20	NUM
eurjchem-440	46	43	60	60	NUM
eurjchem-440	46	44	364.00	364.00	NUM
eurjchem-440	46	45	224.00	224.00	NUM
eurjchem-440	46	46	227.00	227.00	NUM
eurjchem-440	46	47	208.00	208.00	NUM
eurjchem-440	46	48	180.00	180.00	NUM
eurjchem-440	46	49	table	table	NOUN
eurjchem-440	46	50	2	2	NUM
eurjchem-440	46	51	.	.	PUNCT
eurjchem-440	47	1	values	value	NOUN
eurjchem-440	47	2	of	of	ADP
eurjchem-440	47	3	rate	rate	NOUN
eurjchem-440	47	4	constants	constant	NOUN
eurjchem-440	47	5	(	(	PUNCT
eurjchem-440	47	6	kobsx106	kobsx106	PROPN
eurjchem-440	47	7	)	)	PUNCT
eurjchem-440	47	8	for	for	ADP
eurjchem-440	47	9	the	the	DET
eurjchem-440	47	10	aquation	aquation	NOUN
eurjchem-440	47	11	of	of	ADP
eurjchem-440	47	12	[	[	X
eurjchem-440	47	13	co(nh3)5br]2	co(nh3)5br]2	NOUN
eurjchem-440	47	14	+	+	X
eurjchem-440	47	15	in	in	ADP
eurjchem-440	47	16	malonate	malonate	ADJ
eurjchem-440	47	17	media	medium	NOUN
eurjchem-440	47	18	(	(	PUNCT
eurjchem-440	47	19	m1	m1	NOUN
eurjchem-440	47	20	)	)	PUNCT
eurjchem-440	47	21	containing	contain	VERB
eurjchem-440	47	22	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	47	23	(	(	PUNCT
eurjchem-440	47	24	10‐50	10‐50	NUM
eurjchem-440	47	25	%	%	NOUN
eurjchem-440	47	26	)	)	PUNCT
eurjchem-440	47	27	at	at	ADP
eurjchem-440	47	28	different	different	ADJ
eurjchem-440	47	29	temperatures	temperature	NOUN
eurjchem-440	47	30	.	.	PUNCT
eurjchem-440	48	1	m1	m1	PROPN
eurjchem-440	48	2	,	,	PUNCT
eurjchem-440	48	3	mol	mol	ADP
eurjchem-440	48	4	/	/	SYM
eurjchem-440	48	5	l	l	NOUN
eurjchem-440	48	6	temperature	temperature	NOUN
eurjchem-440	48	7	,	,	PUNCT
eurjchem-440	48	8	oc	oc	VERB
eurjchem-440	48	9	30	30	NUM
eurjchem-440	48	10	35	35	NUM
eurjchem-440	48	11	40	40	NUM
eurjchem-440	48	12	50	50	NUM
eurjchem-440	48	13	60	60	NUM
eurjchem-440	48	14	(	(	PUNCT
eurjchem-440	48	15	kobsx106	kobsx106	PROPN
eurjchem-440	48	16	)	)	PUNCT
eurjchem-440	48	17	in	in	ADP
eurjchem-440	48	18	10	10	NUM
eurjchem-440	48	19	%	%	NOUN
eurjchem-440	48	20	0.008	0.008	NUM
eurjchem-440	48	21	4.71	4.71	NUM
eurjchem-440	48	22	14.64	14.64	NUM
eurjchem-440	48	23	29.17	29.17	NUM
eurjchem-440	48	24	58.77	58.77	NUM
eurjchem-440	48	25	473.1	473.1	NUM
eurjchem-440	48	26	0.016	0.016	NUM
eurjchem-440	48	27	5.08	5.08	NUM
eurjchem-440	48	28	11.95	11.95	NUM
eurjchem-440	48	29	34.06	34.06	NUM
eurjchem-440	48	30	141.2	141.2	NUM
eurjchem-440	48	31	394.1	394.1	NUM
eurjchem-440	48	32	0.024	0.024	NUM
eurjchem-440	48	33	5.71	5.71	NUM
eurjchem-440	48	34	17.28	17.28	NUM
eurjchem-440	48	35	47.44	47.44	NUM
eurjchem-440	48	36	163.95	163.95	NUM
eurjchem-440	48	37	469.4	469.4	NUM
eurjchem-440	48	38	0.032	0.032	NUM
eurjchem-440	48	39	2.07	2.07	NUM
eurjchem-440	48	40	26.53	26.53	NUM
eurjchem-440	48	41	38.78	38.78	NUM
eurjchem-440	48	42	164.81	164.81	NUM
eurjchem-440	48	43	546.1	546.1	NUM
eurjchem-440	48	44	0.04	0.04	NUM
eurjchem-440	48	45	3.99	3.99	NUM
eurjchem-440	48	46	20.1	20.1	NUM
eurjchem-440	48	47	47.34	47.34	NUM
eurjchem-440	48	48	187.23	187.23	NUM
eurjchem-440	48	49	546.1	546.1	NUM
eurjchem-440	48	50	(	(	PUNCT
eurjchem-440	48	51	kobsx106	kobsx106	PROPN
eurjchem-440	48	52	)	)	PUNCT
eurjchem-440	48	53	in	in	ADP
eurjchem-440	48	54	20	20	NUM
eurjchem-440	48	55	%	%	NOUN
eurjchem-440	49	1	0.008	0.008	NUM
eurjchem-440	49	2	7.07	7.07	NUM
eurjchem-440	49	3	10.92	10.92	NUM
eurjchem-440	49	4	26.31	26.31	NUM
eurjchem-440	49	5	136.56	136.56	NUM
eurjchem-440	49	6	439.7	439.7	NUM
eurjchem-440	49	7	0.016	0.016	NUM
eurjchem-440	49	8	6.74	6.74	NUM
eurjchem-440	49	9	11.49	11.49	NUM
eurjchem-440	49	10	16.17	16.17	NUM
eurjchem-440	49	11	156.53	156.53	NUM
eurjchem-440	49	12	416.2	416.2	NUM
eurjchem-440	49	13	0.024	0.024	NUM
eurjchem-440	49	14	10.36	10.36	NUM
eurjchem-440	49	15	15.35	15.35	NUM
eurjchem-440	49	16	26.67	26.67	NUM
eurjchem-440	49	17	152.21	152.21	NUM
eurjchem-440	49	18	391.3	391.3	NUM
eurjchem-440	49	19	0.032	0.032	NUM
eurjchem-440	49	20	6.62	6.62	NUM
eurjchem-440	49	21	14.23	14.23	NUM
eurjchem-440	49	22	27.28	27.28	NUM
eurjchem-440	49	23	167.6	167.6	NUM
eurjchem-440	49	24	530.1	530.1	NUM
eurjchem-440	49	25	0.04	0.04	NUM
eurjchem-440	49	26	6.15	6.15	NUM
eurjchem-440	49	27	12.69	12.69	NUM
eurjchem-440	49	28	34.400	34.400	NUM
eurjchem-440	49	29	174.7	174.7	NUM
eurjchem-440	49	30	437.7	437.7	NUM
eurjchem-440	49	31	(	(	PUNCT
eurjchem-440	49	32	kobsx106	kobsx106	PROPN
eurjchem-440	49	33	)	)	PUNCT
eurjchem-440	49	34	in	in	ADP
eurjchem-440	49	35	30	30	NUM
eurjchem-440	49	36	%	%	NOUN
eurjchem-440	50	1	0.008	0.008	NUM
eurjchem-440	50	2	4.18	4.18	NUM
eurjchem-440	50	3	7.35	7.35	NUM
eurjchem-440	50	4	16.75	16.75	NUM
eurjchem-440	50	5	140.29	140.29	NUM
eurjchem-440	50	6	422.4	422.4	NUM
eurjchem-440	50	7	0.016	0.016	NUM
eurjchem-440	50	8	5.66	5.66	NUM
eurjchem-440	50	9	8.14	8.14	NUM
eurjchem-440	50	10	21.39	21.39	NUM
eurjchem-440	50	11	177.67	177.67	NUM
eurjchem-440	50	12	382.7	382.7	NUM
eurjchem-440	50	13	0.024	0.024	NUM
eurjchem-440	50	14	9.52	9.52	NUM
eurjchem-440	50	15	5.56	5.56	NUM
eurjchem-440	50	16	16.66	16.66	NUM
eurjchem-440	50	17	169.60	169.60	NUM
eurjchem-440	50	18	522.2	522.2	NUM
eurjchem-440	50	19	0.032	0.032	NUM
eurjchem-440	50	20	3.12	3.12	NUM
eurjchem-440	50	21	19.96	19.96	NUM
eurjchem-440	50	22	29.11	29.11	NUM
eurjchem-440	50	23	147.88	147.88	NUM
eurjchem-440	50	24	420.9	420.9	NUM
eurjchem-440	50	25	0.04	0.04	NUM
eurjchem-440	50	26	4.50	4.50	NUM
eurjchem-440	50	27	26.87	26.87	NUM
eurjchem-440	50	28	32.01	32.01	NUM
eurjchem-440	50	29	146.66	146.66	NUM
eurjchem-440	50	30	471.2	471.2	NUM
eurjchem-440	50	31	(	(	PUNCT
eurjchem-440	50	32	kobsx106	kobsx106	PROPN
eurjchem-440	50	33	)	)	PUNCT
eurjchem-440	50	34	in	in	ADP
eurjchem-440	50	35	40	40	NUM
eurjchem-440	50	36	%	%	NOUN
eurjchem-440	50	37	0.008	0.008	NUM
eurjchem-440	50	38	4.94	4.94	NUM
eurjchem-440	50	39	15.32	15.32	NUM
eurjchem-440	50	40	77.16	77.16	NUM
eurjchem-440	50	41	167.18	167.18	NUM
eurjchem-440	50	42	617.96	617.96	NUM
eurjchem-440	50	43	0.016	0.016	NUM
eurjchem-440	50	44	6.98	6.98	NUM
eurjchem-440	50	45	10.41	10.41	NUM
eurjchem-440	50	46	28.44	28.44	NUM
eurjchem-440	50	47	166.91	166.91	NUM
eurjchem-440	50	48	506.12	506.12	NUM
eurjchem-440	50	49	0.024	0.024	NUM
eurjchem-440	50	50	7.08	7.08	NUM
eurjchem-440	50	51	24.91	24.91	NUM
eurjchem-440	50	52	85.99	85.99	NUM
eurjchem-440	50	53	175.47	175.47	NUM
eurjchem-440	50	54	548.32	548.32	NUM
eurjchem-440	50	55	0.032	0.032	NUM
eurjchem-440	50	56	5.63	5.63	NUM
eurjchem-440	50	57	23.39	23.39	NUM
eurjchem-440	50	58	45.65	45.65	NUM
eurjchem-440	50	59	158.45	158.45	NUM
eurjchem-440	50	60	450.8	450.8	NUM
eurjchem-440	50	61	0.04	0.04	NUM
eurjchem-440	50	62	4.71	4.71	NUM
eurjchem-440	50	63	13.39	13.39	NUM
eurjchem-440	50	64	40.42	40.42	NUM
eurjchem-440	50	65	162.24	162.24	NUM
eurjchem-440	50	66	436.1	436.1	NUM
eurjchem-440	50	67	(	(	PUNCT
eurjchem-440	50	68	kobsx106	kobsx106	PROPN
eurjchem-440	50	69	)	)	PUNCT
eurjchem-440	50	70	in	in	ADP
eurjchem-440	50	71	50	50	NUM
eurjchem-440	50	72	%	%	NOUN
eurjchem-440	50	73	0.008	0.008	NUM
eurjchem-440	50	74	5.66	5.66	NUM
eurjchem-440	50	75	11.69	11.69	NUM
eurjchem-440	50	76	33.095	33.095	NUM
eurjchem-440	50	77	149.09	149.09	NUM
eurjchem-440	50	78	414.9	414.9	NUM
eurjchem-440	50	79	0.016	0.016	NUM
eurjchem-440	50	80	9.13	9.13	NUM
eurjchem-440	50	81	18.18	18.18	NUM
eurjchem-440	50	82	34.61	34.61	NUM
eurjchem-440	50	83	152.11	152.11	NUM
eurjchem-440	50	84	383.1	383.1	NUM
eurjchem-440	50	85	0.024	0.024	NUM
eurjchem-440	50	86	9.21	9.21	NUM
eurjchem-440	50	87	19.16	19.16	NUM
eurjchem-440	50	88	43.76	43.76	NUM
eurjchem-440	50	89	167.38	167.38	NUM
eurjchem-440	50	90	405.1	405.1	NUM
eurjchem-440	50	91	0.032	0.032	NUM
eurjchem-440	50	92	5.58	5.58	NUM
eurjchem-440	50	93	24.35	24.35	NUM
eurjchem-440	50	94	45.77	45.77	NUM
eurjchem-440	50	95	194.56	194.56	NUM
eurjchem-440	50	96	442.4	442.4	NUM
eurjchem-440	50	97	0.04	0.04	NUM
eurjchem-440	50	98	14.19	14.19	NUM
eurjchem-440	50	99	24.11	24.11	NUM
eurjchem-440	50	100	46.3	46.3	NUM
eurjchem-440	50	101	222.22	222.22	NUM
eurjchem-440	50	102	428.0	428.0	NUM
eurjchem-440	50	103	3	3	NUM
eurjchem-440	50	104	.	.	NOUN
eurjchem-440	50	105	results	result	NOUN
eurjchem-440	50	106	and	and	CCONJ
eurjchem-440	50	107	discussion	discussion	NOUN
eurjchem-440	50	108	plots	plot	NOUN
eurjchem-440	50	109	of	of	ADP
eurjchem-440	50	110	log	log	NOUN
eurjchem-440	50	111	(	(	PUNCT
eurjchem-440	50	112	at‐a∞	at‐a∞	PROPN
eurjchem-440	50	113	)	)	PUNCT
eurjchem-440	50	114	versus	versus	ADP
eurjchem-440	50	115	time	time	NOUN
eurjchem-440	50	116	were	be	AUX
eurjchem-440	50	117	found	find	VERB
eurjchem-440	50	118	to	to	PART
eurjchem-440	50	119	be	be	AUX
eurjchem-440	50	120	linear	linear	ADJ
eurjchem-440	50	121	for	for	ADP
eurjchem-440	50	122	the	the	DET
eurjchem-440	50	123	aquation	aquation	NOUN
eurjchem-440	50	124	of	of	ADP
eurjchem-440	50	125	[	[	X
eurjchem-440	50	126	co(nh3)5br](clo4)2	co(nh3)5br](clo4)2	ADJ
eurjchem-440	50	127	complex	complex	NOUN
eurjchem-440	50	128	.	.	PUNCT
eurjchem-440	51	1	the	the	DET
eurjchem-440	51	2	observed	observe	VERB
eurjchem-440	51	3	rate	rate	NOUN
eurjchem-440	51	4	constants	constant	NOUN
eurjchem-440	51	5	are	be	AUX
eurjchem-440	51	6	collected	collect	VERB
eurjchem-440	51	7	in	in	ADP
eurjchem-440	51	8	table	table	NOUN
eurjchem-440	51	9	1	1	NUM
eurjchem-440	51	10	and	and	CCONJ
eurjchem-440	51	11	2	2	NUM
eurjchem-440	51	12	.	.	X
eurjchem-440	52	1	the	the	DET
eurjchem-440	52	2	ion‐pair	ion‐pair	PROPN
eurjchem-440	52	3	rate	rate	NOUN
eurjchem-440	52	4	coefficient	coefficient	NOUN
eurjchem-440	52	5	(	(	PUNCT
eurjchem-440	52	6	kip	kip	PROPN
eurjchem-440	52	7	)	)	PUNCT
eurjchem-440	52	8	was	be	AUX
eurjchem-440	52	9	calculated	calculate	VERB
eurjchem-440	52	10	according	accord	VERB
eurjchem-440	52	11	to	to	ADP
eurjchem-440	52	12	the	the	DET
eurjchem-440	52	13	following	follow	VERB
eurjchem-440	52	14	wyatt	wyatt	PROPN
eurjchem-440	52	15	and	and	CCONJ
eurjchem-440	52	16	davis	davis	PROPN
eurjchem-440	52	17	equation	equation	NOUN
eurjchem-440	52	18	[	[	X
eurjchem-440	52	19	11	11	NUM
eurjchem-440	52	20	]	]	PUNCT
eurjchem-440	52	21	.	.	PUNCT
eurjchem-440	53	1	kobs.m3	kobs.m3	PROPN
eurjchem-440	53	2	=	=	PROPN
eurjchem-440	53	3	k0	k0	PROPN
eurjchem-440	54	1	[	[	X
eurjchem-440	54	2	cpx2	cpx2	PROPN
eurjchem-440	54	3	+	+	PROPN
eurjchem-440	54	4	]	]	X
eurjchem-440	54	5	+	+	CCONJ
eurjchem-440	54	6	kip	kip	PROPN
eurjchem-440	54	7	[	[	X
eurjchem-440	54	8	cpxl	cpxl	NOUN
eurjchem-440	54	9	]	]	X
eurjchem-440	54	10	(	(	PUNCT
eurjchem-440	54	11	1	1	X
eurjchem-440	54	12	)	)	PUNCT
eurjchem-440	54	13	where	where	SCONJ
eurjchem-440	54	14	,	,	PUNCT
eurjchem-440	54	15	k0	k0	PROPN
eurjchem-440	54	16	‐	‐	VERB
eurjchem-440	54	17	the	the	DET
eurjchem-440	54	18	observed	observe	VERB
eurjchem-440	54	19	rate	rate	NOUN
eurjchem-440	54	20	constant	constant	ADJ
eurjchem-440	54	21	in	in	ADP
eurjchem-440	54	22	the	the	DET
eurjchem-440	54	23	absence	absence	NOUN
eurjchem-440	54	24	of	of	ADP
eurjchem-440	54	25	dicarboxylate	dicarboxylate	ADJ
eurjchem-440	54	26	ion	ion	NOUN
eurjchem-440	54	27	,	,	PUNCT
eurjchem-440	54	28	kobs	kobs	PROPN
eurjchem-440	54	29	‐	‐	ADP
eurjchem-440	54	30	the	the	DET
eurjchem-440	54	31	observed	observe	VERB
eurjchem-440	54	32	rate	rate	NOUN
eurjchem-440	54	33	constant	constant	ADJ
eurjchem-440	54	34	in	in	ADP
eurjchem-440	54	35	the	the	DET
eurjchem-440	54	36	presence	presence	NOUN
eurjchem-440	54	37	of	of	ADP
eurjchem-440	54	38	dicarboxylate	dicarboxylate	ADJ
eurjchem-440	54	39	ion	ion	NOUN
eurjchem-440	54	40	,	,	PUNCT
eurjchem-440	54	41	m3	m3	PROPN
eurjchem-440	54	42	‐	‐	VERB
eurjchem-440	54	43	the	the	DET
eurjchem-440	54	44	stoichiometric	stoichiometric	ADJ
eurjchem-440	54	45	concentration	concentration	NOUN
eurjchem-440	54	46	of	of	ADP
eurjchem-440	54	47	the	the	DET
eurjchem-440	54	48	complex	complex	ADJ
eurjchem-440	54	49	salt	salt	NOUN
eurjchem-440	54	50	,	,	PUNCT
eurjchem-440	54	51	[	[	X
eurjchem-440	54	52	cpx2	cpx2	NOUN
eurjchem-440	54	53	+	+	X
eurjchem-440	54	54	]	]	X
eurjchem-440	54	55	‐	‐	VERB
eurjchem-440	54	56	the	the	DET
eurjchem-440	54	57	free	free	ADJ
eurjchem-440	54	58	complex	complex	ADJ
eurjchem-440	54	59	ion	ion	NOUN
eurjchem-440	54	60	concentration	concentration	NOUN
eurjchem-440	54	61	and	and	CCONJ
eurjchem-440	54	62	[	[	X
eurjchem-440	54	63	cpxl	cpxl	NOUN
eurjchem-440	54	64	]	]	PUNCT
eurjchem-440	54	65	‐	‐	ADP
eurjchem-440	54	66	the	the	DET
eurjchem-440	54	67	ion‐pair	ion‐pair	PROPN
eurjchem-440	54	68	concentration	concentration	NOUN
eurjchem-440	54	69	.	.	PUNCT
eurjchem-440	55	1	[	[	X
eurjchem-440	55	2	cpxl	cpxl	NOUN
eurjchem-440	55	3	]	]	PUNCT
eurjchem-440	55	4	was	be	AUX
eurjchem-440	55	5	calculated	calculate	VERB
eurjchem-440	55	6	with	with	ADP
eurjchem-440	55	7	the	the	DET
eurjchem-440	55	8	aid	aid	NOUN
eurjchem-440	55	9	of	of	ADP
eurjchem-440	55	10	the	the	DET
eurjchem-440	55	11	following	follow	VERB
eurjchem-440	55	12	equations	equation	NOUN
eurjchem-440	55	13	:	:	PUNCT
eurjchem-440	55	14	cpxl	cpxl	VERB
eurjchem-440	55	15	⇆	⇆	ADJ
eurjchem-440	55	16	cpx2	cpx2	PROPN
eurjchem-440	55	17	+	+	X
eurjchem-440	55	18	+	+	NUM
eurjchem-440	55	19	l2‐	l2‐	ADJ
eurjchem-440	55	20	kd	kd	NOUN
eurjchem-440	55	21	(	(	PUNCT
eurjchem-440	55	22	2	2	NUM
eurjchem-440	55	23	)	)	PUNCT
eurjchem-440	55	24	nal‐	nal‐	NOUN
eurjchem-440	55	25	⇆	⇆	PROPN
eurjchem-440	55	26	na+	na+	NOUN
eurjchem-440	55	27	+	+	CCONJ
eurjchem-440	55	28	l2‐	l2‐	NOUN
eurjchem-440	55	29	knal‐	knal‐	NOUN
eurjchem-440	55	30	(	(	PUNCT
eurjchem-440	55	31	3	3	X
eurjchem-440	55	32	)	)	PUNCT
eurjchem-440	55	33	h2l	h2l	NOUN
eurjchem-440	55	34	⇆	⇆	PROPN
eurjchem-440	55	35	hl‐	hl‐	PROPN
eurjchem-440	55	36	+	+	CCONJ
eurjchem-440	55	37	h+	h+	X
eurjchem-440	55	38	k1	k1	NOUN
eurjchem-440	55	39	(	(	PUNCT
eurjchem-440	55	40	4	4	NUM
eurjchem-440	55	41	)	)	PUNCT
eurjchem-440	55	42	hl‐	hl‐	NOUN
eurjchem-440	55	43	⇆	⇆	ADP
eurjchem-440	55	44	l2‐	l2‐	NOUN
eurjchem-440	55	45	+	+	CCONJ
eurjchem-440	55	46	h+	h+	X
eurjchem-440	55	47	k2	k2	X
eurjchem-440	55	48	(	(	PUNCT
eurjchem-440	55	49	5	5	NUM
eurjchem-440	55	50	)	)	PUNCT
eurjchem-440	55	51	where	where	SCONJ
eurjchem-440	55	52	;	;	PUNCT
eurjchem-440	55	53	kd	kd	PROPN
eurjchem-440	55	54	=	=	PUNCT
eurjchem-440	56	1	[	[	X
eurjchem-440	56	2	cpx2+][l2‐	cpx2+][l2‐	X
eurjchem-440	56	3	]	]	X
eurjchem-440	56	4	/	/	PUNCT
eurjchem-440	57	1	[	[	X
eurjchem-440	57	2	cpxl	cpxl	NOUN
eurjchem-440	57	3	]	]	X
eurjchem-440	57	4	(	(	PUNCT
eurjchem-440	57	5	l2‐	l2‐	NOUN
eurjchem-440	57	6	represents	represent	VERB
eurjchem-440	57	7	the	the	DET
eurjchem-440	57	8	dicarboxylate	dicarboxylate	ADJ
eurjchem-440	57	9	anion	anion	NOUN
eurjchem-440	57	10	)	)	PUNCT
eurjchem-440	57	11	(	(	PUNCT
eurjchem-440	57	12	6	6	X
eurjchem-440	57	13	)	)	PUNCT
eurjchem-440	57	14	k1	k1	NOUN
eurjchem-440	57	15	=	=	PUNCT
eurjchem-440	58	1	[	[	X
eurjchem-440	58	2	h+][hl‐	h+][hl‐	X
eurjchem-440	58	3	]	]	X
eurjchem-440	58	4	/[h2l	/[h2l	X
eurjchem-440	58	5	]	]	X
eurjchem-440	58	6	(	(	PUNCT
eurjchem-440	58	7	7	7	X
eurjchem-440	58	8	)	)	PUNCT
eurjchem-440	58	9	k2	k2	NOUN
eurjchem-440	58	10	=	=	PUNCT
eurjchem-440	59	1	[	[	X
eurjchem-440	59	2	h+	h+	X
eurjchem-440	59	3	]	]	X
eurjchem-440	59	4	[	[	X
eurjchem-440	59	5	l2‐	l2‐	X
eurjchem-440	59	6	]	]	PUNCT
eurjchem-440	59	7	γ2/	γ2/	NOUN
eurjchem-440	60	1	[	[	X
eurjchem-440	60	2	hl‐	hl‐	X
eurjchem-440	60	3	]	]	X
eurjchem-440	60	4	(	(	PUNCT
eurjchem-440	60	5	8)	8)	NUM
eurjchem-440	60	6	knal‐	knal‐	NOUN
eurjchem-440	60	7	=	=	PUNCT
eurjchem-440	61	1	[	[	X
eurjchem-440	61	2	na+	na+	X
eurjchem-440	61	3	]	]	X
eurjchem-440	61	4	[	[	X
eurjchem-440	61	5	l2‐	l2‐	X
eurjchem-440	61	6	]	]	PUNCT
eurjchem-440	61	7	γ2/	γ2/	NOUN
eurjchem-440	62	1	[	[	X
eurjchem-440	62	2	nal‐	nal‐	X
eurjchem-440	62	3	]	]	X
eurjchem-440	62	4	(	(	PUNCT
eurjchem-440	62	5	9	9	X
eurjchem-440	62	6	)	)	PUNCT
eurjchem-440	62	7	log	log	NOUN
eurjchem-440	62	8	γi	γi	NOUN
eurjchem-440	62	9	=	=	PUNCT
eurjchem-440	62	10	‐a	‐a	PROPN
eurjchem-440	62	11	(	(	PUNCT
eurjchem-440	62	12	i1/2/	i1/2/	PROPN
eurjchem-440	62	13	(	(	PUNCT
eurjchem-440	62	14	1	1	NUM
eurjchem-440	62	15	+	+	NOUN
eurjchem-440	62	16	1.3	1.3	NUM
eurjchem-440	62	17	i1/2)‐0.3i	i1/2)‐0.3i	NOUN
eurjchem-440	62	18	)	)	PUNCT
eurjchem-440	62	19	(	(	PUNCT
eurjchem-440	62	20	debye‐huckle	debye‐huckle	NOUN
eurjchem-440	62	21	equation	equation	NOUN
eurjchem-440	62	22	)	)	PUNCT
eurjchem-440	62	23	(	(	PUNCT
eurjchem-440	62	24	10	10	NUM
eurjchem-440	62	25	)	)	PUNCT
eurjchem-440	62	26	(	(	PUNCT
eurjchem-440	62	27	log	log	VERB
eurjchem-440	62	28	γ2	γ2	PROPN
eurjchem-440	62	29	=	=	SYM
eurjchem-440	62	30	4.log	4.log	PROPN
eurjchem-440	62	31	γ1	γ1	PROPN
eurjchem-440	62	32	)	)	PUNCT
eurjchem-440	62	33	,	,	PUNCT
eurjchem-440	62	34	(	(	PUNCT
eurjchem-440	62	35	i	i	PRON
eurjchem-440	62	36	is	be	AUX
eurjchem-440	62	37	the	the	DET
eurjchem-440	62	38	ionic	ionic	ADJ
eurjchem-440	62	39	strength	strength	NOUN
eurjchem-440	62	40	γ1	γ1	NOUN
eurjchem-440	62	41	and	and	CCONJ
eurjchem-440	62	42	γ2	γ2	PROPN
eurjchem-440	62	43	are	be	AUX
eurjchem-440	62	44	the	the	DET
eurjchem-440	62	45	activity	activity	NOUN
eurjchem-440	62	46	coefficients	coefficient	NOUN
eurjchem-440	62	47	of	of	ADP
eurjchem-440	62	48	the	the	DET
eurjchem-440	62	49	univalent	univalent	ADJ
eurjchem-440	62	50	and	and	CCONJ
eurjchem-440	62	51	divalent	divalent	ADJ
eurjchem-440	62	52	ions	ion	NOUN
eurjchem-440	62	53	,	,	PUNCT
eurjchem-440	62	54	respectively	respectively	ADV
eurjchem-440	62	55	)	)	PUNCT
eurjchem-440	62	56	.	.	PUNCT
eurjchem-440	63	1	i	i	PRON
eurjchem-440	63	2	=	=	NOUN
eurjchem-440	63	3	0.5	0.5	NUM
eurjchem-440	63	4	(	(	PUNCT
eurjchem-440	63	5	[	[	X
eurjchem-440	63	6	h+	h+	X
eurjchem-440	63	7	]	]	X
eurjchem-440	63	8	+	+	CCONJ
eurjchem-440	64	1	[	[	X
eurjchem-440	64	2	hl‐	hl‐	X
eurjchem-440	64	3	]	]	X
eurjchem-440	64	4	+4[l2‐	+4[l2‐	PROPN
eurjchem-440	64	5	]	]	X
eurjchem-440	64	6	+4[cpx2	+4[cpx2	ADP
eurjchem-440	64	7	+	+	PROPN
eurjchem-440	64	8	]	]	X
eurjchem-440	65	1	+2m3	+2m3	PROPN
eurjchem-440	65	2	+	+	SYM
eurjchem-440	65	3	[	[	X
eurjchem-440	65	4	na+	na+	X
eurjchem-440	65	5	]	]	X
eurjchem-440	65	6	+	+	CCONJ
eurjchem-440	65	7	[	[	X
eurjchem-440	65	8	nal1‐	nal1‐	X
eurjchem-440	65	9	]	]	PUNCT
eurjchem-440	65	10	)	)	PUNCT
eurjchem-440	65	11	(	(	PUNCT
eurjchem-440	65	12	11	11	NUM
eurjchem-440	65	13	)	)	PUNCT
eurjchem-440	65	14	m1=	m1=	NOUN
eurjchem-440	65	15	[	[	X
eurjchem-440	65	16	h2l	h2l	X
eurjchem-440	65	17	]	]	X
eurjchem-440	65	18	+	+	CCONJ
eurjchem-440	66	1	[	[	X
eurjchem-440	66	2	hl‐	hl‐	X
eurjchem-440	66	3	]	]	X
eurjchem-440	66	4	+	+	CCONJ
eurjchem-440	66	5	[	[	X
eurjchem-440	66	6	cpxl	cpxl	NOUN
eurjchem-440	66	7	]	]	X
eurjchem-440	66	8	+	+	CCONJ
eurjchem-440	67	1	[	[	X
eurjchem-440	67	2	nal‐	nal‐	X
eurjchem-440	67	3	]	]	X
eurjchem-440	67	4	(	(	PUNCT
eurjchem-440	67	5	12	12	NUM
eurjchem-440	67	6	)	)	PUNCT
eurjchem-440	67	7	m3=	m3=	NOUN
eurjchem-440	67	8	[	[	X
eurjchem-440	67	9	cpx2	cpx2	PROPN
eurjchem-440	67	10	+	+	PROPN
eurjchem-440	67	11	]	]	X
eurjchem-440	68	1	+	+	CCONJ
eurjchem-440	68	2	[	[	X
eurjchem-440	68	3	cpxl	cpxl	NOUN
eurjchem-440	68	4	]	]	X
eurjchem-440	68	5	(	(	PUNCT
eurjchem-440	68	6	13	13	NUM
eurjchem-440	68	7	)	)	PUNCT
eurjchem-440	68	8	the	the	DET
eurjchem-440	68	9	principle	principle	NOUN
eurjchem-440	68	10	of	of	ADP
eurjchem-440	68	11	calculations	calculation	NOUN
eurjchem-440	68	12	performed	perform	VERB
eurjchem-440	68	13	by	by	ADP
eurjchem-440	68	14	computer	computer	NOUN
eurjchem-440	68	15	programs	program	NOUN
eurjchem-440	68	16	can	can	AUX
eurjchem-440	68	17	be	be	AUX
eurjchem-440	68	18	summarized	summarize	VERB
eurjchem-440	68	19	as	as	ADP
eurjchem-440	68	20	:	:	PUNCT
eurjchem-440	68	21	for	for	ADP
eurjchem-440	68	22	the	the	DET
eurjchem-440	68	23	first	first	ADJ
eurjchem-440	68	24	cycle	cycle	NOUN
eurjchem-440	68	25	[	[	X
eurjchem-440	68	26	h+	h+	X
eurjchem-440	68	27	]	]	X
eurjchem-440	68	28	=	=	SYM
eurjchem-440	68	29	0	0	NUM
eurjchem-440	68	30	,	,	PUNCT
eurjchem-440	68	31	[	[	X
eurjchem-440	68	32	cpxl	cpxl	NOUN
eurjchem-440	68	33	]	]	X
eurjchem-440	68	34	=	=	SYM
eurjchem-440	68	35	0	0	NUM
eurjchem-440	68	36	,	,	PUNCT
eurjchem-440	68	37	[	[	X
eurjchem-440	68	38	nal‐	nal‐	X
eurjchem-440	68	39	]	]	X
eurjchem-440	68	40	=	=	SYM
eurjchem-440	68	41	0	0	NUM
eurjchem-440	68	42	,	,	PUNCT
eurjchem-440	68	43	(	(	PUNCT
eurjchem-440	68	44	14	14	NUM
eurjchem-440	68	45	)	)	PUNCT
eurjchem-440	69	1	[	[	X
eurjchem-440	69	2	cpx2	cpx2	NOUN
eurjchem-440	69	3	+	+	PROPN
eurjchem-440	69	4	]	]	X
eurjchem-440	69	5	=	=	PUNCT
eurjchem-440	69	6	m3	m3	PROPN
eurjchem-440	69	7	–	–	PUNCT
eurjchem-440	69	8	[	[	X
eurjchem-440	69	9	cpxl	cpxl	NOUN
eurjchem-440	69	10	]	]	X
eurjchem-440	69	11	,	,	PUNCT
eurjchem-440	69	12	[	[	X
eurjchem-440	69	13	hl‐	hl‐	X
eurjchem-440	69	14	]	]	X
eurjchem-440	69	15	=	=	SYM
eurjchem-440	69	16	0.5	0.5	NUM
eurjchem-440	69	17	m2	m2	PROPN
eurjchem-440	69	18	,	,	PUNCT
eurjchem-440	69	19	[	[	X
eurjchem-440	69	20	h2l	h2l	X
eurjchem-440	69	21	]	]	X
eurjchem-440	69	22	=	=	SYM
eurjchem-440	69	23	0.3m1	0.3m1	NUM
eurjchem-440	69	24	,	,	PUNCT
eurjchem-440	69	25	(	(	PUNCT
eurjchem-440	69	26	15	15	NUM
eurjchem-440	69	27	)	)	PUNCT
eurjchem-440	70	1	[	[	X
eurjchem-440	70	2	l2‐	l2‐	X
eurjchem-440	70	3	]	]	X
eurjchem-440	70	4	=	=	SYM
eurjchem-440	70	5	m1	m1	PROPN
eurjchem-440	70	6	–	–	PUNCT
eurjchem-440	71	1	[	[	X
eurjchem-440	71	2	hl‐	hl‐	X
eurjchem-440	71	3	]	]	X
eurjchem-440	71	4	–	–	PUNCT
eurjchem-440	71	5	[	[	X
eurjchem-440	71	6	cpxl	cpxl	NOUN
eurjchem-440	71	7	]	]	PUNCT
eurjchem-440	71	8	–	–	PUNCT
eurjchem-440	72	1	[	[	X
eurjchem-440	72	2	nal‐	nal‐	X
eurjchem-440	72	3	]	]	X
eurjchem-440	72	4	–	–	PUNCT
eurjchem-440	73	1	[	[	X
eurjchem-440	73	2	h2l	h2l	X
eurjchem-440	73	3	]	]	X
eurjchem-440	73	4	,	,	PUNCT
eurjchem-440	73	5	(	(	PUNCT
eurjchem-440	73	6	16	16	NUM
eurjchem-440	73	7	)	)	PUNCT
eurjchem-440	74	1	[	[	X
eurjchem-440	74	2	na+	na+	X
eurjchem-440	74	3	]	]	X
eurjchem-440	74	4	=	=	SYM
eurjchem-440	74	5	2m2	2m2	NUM
eurjchem-440	74	6	–	–	PUNCT
eurjchem-440	74	7	[	[	PUNCT
eurjchem-440	74	8	nal‐	nal‐	NOUN
eurjchem-440	74	9	]	]	X
eurjchem-440	74	10	.	.	PUNCT
eurjchem-440	75	1	(	(	PUNCT
eurjchem-440	75	2	17	17	NUM
eurjchem-440	75	3	)	)	PUNCT
eurjchem-440	75	4	where	where	SCONJ
eurjchem-440	75	5	,	,	PUNCT
eurjchem-440	75	6	m2	m2	PROPN
eurjchem-440	75	7	is	be	AUX
eurjchem-440	75	8	the	the	DET
eurjchem-440	75	9	concentration	concentration	NOUN
eurjchem-440	75	10	of	of	ADP
eurjchem-440	75	11	sodium	sodium	NOUN
eurjchem-440	75	12	carbonate	carbonate	NOUN
eurjchem-440	75	13	.	.	PUNCT
eurjchem-440	76	1	afterwards	afterwards	ADV
eurjchem-440	76	2	,	,	PUNCT
eurjchem-440	76	3	the	the	DET
eurjchem-440	76	4	ionic	ionic	ADJ
eurjchem-440	76	5	strength	strength	NOUN
eurjchem-440	76	6	takes	take	VERB
eurjchem-440	76	7	its	its	PRON
eurjchem-440	76	8	first	first	ADJ
eurjchem-440	76	9	approximated	approximate	VERB
eurjchem-440	76	10	value	value	NOUN
eurjchem-440	76	11	and	and	CCONJ
eurjchem-440	76	12	then	then	ADV
eurjchem-440	76	13	γ1and	γ1and	PROPN
eurjchem-440	76	14	γ2	γ2	PROPN
eurjchem-440	76	15	after	after	ADP
eurjchem-440	76	16	which	which	PRON
eurjchem-440	76	17	the	the	DET
eurjchem-440	76	18	following	follow	VERB
eurjchem-440	76	19	terms	term	NOUN
eurjchem-440	76	20	take	take	VERB
eurjchem-440	76	21	their	their	PRON
eurjchem-440	76	22	new	new	ADJ
eurjchem-440	76	23	value	value	NOUN
eurjchem-440	76	24	;	;	PUNCT
eurjchem-440	76	25	zeitouni	zeitouni	X
eurjchem-440	76	26	et	et	NOUN
eurjchem-440	76	27	al	al	PROPN
eurjchem-440	76	28	.	.	PUNCT
eurjchem-440	76	29	/	/	SYM
eurjchem-440	76	30	european	european	PROPN
eurjchem-440	76	31	journal	journal	PROPN
eurjchem-440	76	32	of	of	ADP
eurjchem-440	76	33	chemistry	chemistry	NOUN
eurjchem-440	76	34	2	2	NUM
eurjchem-440	76	35	(	(	PUNCT
eurjchem-440	76	36	4	4	NUM
eurjchem-440	76	37	)	)	PUNCT
eurjchem-440	76	38	(	(	PUNCT
eurjchem-440	76	39	2011	2011	NUM
eurjchem-440	76	40	)	)	PUNCT
eurjchem-440	76	41	489‐494	489‐494	NUM
eurjchem-440	76	42	491	491	NUM
eurjchem-440	77	1	[	[	X
eurjchem-440	77	2	h+	h+	X
eurjchem-440	77	3	]	]	X
eurjchem-440	77	4	=	=	SYM
eurjchem-440	77	5	k2	k2	PROPN
eurjchem-440	78	1	[	[	X
eurjchem-440	78	2	hl‐	hl‐	X
eurjchem-440	78	3	]	]	X
eurjchem-440	78	4	/	/	PUNCT
eurjchem-440	79	1	[	[	X
eurjchem-440	79	2	l2‐	l2‐	NOUN
eurjchem-440	79	3	]	]	X
eurjchem-440	79	4	γ2	γ2	NOUN
eurjchem-440	79	5	(	(	PUNCT
eurjchem-440	79	6	18	18	NUM
eurjchem-440	79	7	)	)	PUNCT
eurjchem-440	80	1	[	[	X
eurjchem-440	80	2	h2l	h2l	X
eurjchem-440	80	3	]	]	X
eurjchem-440	80	4	=	=	PUNCT
eurjchem-440	81	1	[	[	X
eurjchem-440	81	2	hl‐][h+	hl‐][h+	X
eurjchem-440	81	3	]	]	X
eurjchem-440	81	4	/	/	SYM
eurjchem-440	81	5	k1	k1	NOUN
eurjchem-440	81	6	(	(	PUNCT
eurjchem-440	81	7	19	19	NUM
eurjchem-440	81	8	)	)	PUNCT
eurjchem-440	82	1	[	[	X
eurjchem-440	82	2	hl‐	hl‐	X
eurjchem-440	82	3	]	]	X
eurjchem-440	82	4	=	=	SYM
eurjchem-440	82	5	2m1	2m1	NUM
eurjchem-440	82	6	‐2m2	‐2m2	PROPN
eurjchem-440	82	7	–	–	PUNCT
eurjchem-440	82	8	2[h2l	2[h2l	NUM
eurjchem-440	82	9	]	]	PUNCT
eurjchem-440	82	10	–	–	PUNCT
eurjchem-440	83	1	[	[	X
eurjchem-440	83	2	h+	h+	X
eurjchem-440	83	3	]	]	X
eurjchem-440	83	4	(	(	PUNCT
eurjchem-440	83	5	20	20	NUM
eurjchem-440	83	6	)	)	PUNCT
eurjchem-440	84	1	[	[	X
eurjchem-440	84	2	l2‐	l2‐	X
eurjchem-440	84	3	]	]	X
eurjchem-440	84	4	=	=	SYM
eurjchem-440	84	5	m1	m1	PROPN
eurjchem-440	84	6	–	–	PUNCT
eurjchem-440	84	7	[	[	X
eurjchem-440	84	8	hl‐	hl‐	X
eurjchem-440	84	9	]	]	X
eurjchem-440	84	10	–	–	PUNCT
eurjchem-440	84	11	[	[	X
eurjchem-440	84	12	h2l	h2l	X
eurjchem-440	84	13	]	]	X
eurjchem-440	84	14	–	–	PUNCT
eurjchem-440	84	15	[	[	X
eurjchem-440	84	16	cpxl	cpxl	NOUN
eurjchem-440	84	17	]	]	PUNCT
eurjchem-440	84	18	–	–	PUNCT
eurjchem-440	84	19	[	[	X
eurjchem-440	84	20	nal‐	nal‐	X
eurjchem-440	84	21	]	]	X
eurjchem-440	84	22	(	(	PUNCT
eurjchem-440	84	23	21	21	NUM
eurjchem-440	84	24	)	)	PUNCT
eurjchem-440	85	1	[	[	X
eurjchem-440	85	2	nal‐	nal‐	X
eurjchem-440	85	3	]	]	X
eurjchem-440	85	4	=	=	PUNCT
eurjchem-440	86	1	[	[	X
eurjchem-440	86	2	na+	na+	X
eurjchem-440	86	3	]	]	X
eurjchem-440	86	4	[	[	X
eurjchem-440	86	5	l2‐	l2‐	X
eurjchem-440	86	6	]	]	PUNCT
eurjchem-440	86	7	γ2/	γ2/	NOUN
eurjchem-440	86	8	knal‐	knal‐	PROPN
eurjchem-440	86	9	(	(	PUNCT
eurjchem-440	86	10	22	22	NUM
eurjchem-440	86	11	)	)	PUNCT
eurjchem-440	87	1	[	[	X
eurjchem-440	87	2	cpxl	cpxl	NOUN
eurjchem-440	87	3	]	]	X
eurjchem-440	87	4	=	=	PUNCT
eurjchem-440	87	5	m3/[(kd/	m3/[(kd/	NUM
eurjchem-440	88	1	[	[	X
eurjchem-440	88	2	l2‐	l2‐	NOUN
eurjchem-440	88	3	]	]	PUNCT
eurjchem-440	88	4	)	)	PUNCT
eurjchem-440	89	1	+1	+1	X
eurjchem-440	89	2	]	]	X
eurjchem-440	89	3	(	(	PUNCT
eurjchem-440	89	4	23	23	NUM
eurjchem-440	89	5	)	)	PUNCT
eurjchem-440	90	1	[	[	X
eurjchem-440	90	2	cpx2	cpx2	NOUN
eurjchem-440	90	3	+	+	PROPN
eurjchem-440	90	4	]	]	X
eurjchem-440	90	5	=	=	PUNCT
eurjchem-440	90	6	m3	m3	PROPN
eurjchem-440	90	7	–	–	PUNCT
eurjchem-440	90	8	[	[	X
eurjchem-440	90	9	cpxl	cpxl	NOUN
eurjchem-440	90	10	]	]	X
eurjchem-440	90	11	(	(	PUNCT
eurjchem-440	90	12	24	24	NUM
eurjchem-440	90	13	)	)	PUNCT
eurjchem-440	90	14	then	then	ADV
eurjchem-440	90	15	i	i	PRON
eurjchem-440	90	16	,	,	PUNCT
eurjchem-440	90	17	γ1	γ1	PROPN
eurjchem-440	90	18	and	and	CCONJ
eurjchem-440	90	19	γ2	γ2	PROPN
eurjchem-440	90	20	were	be	AUX
eurjchem-440	90	21	recalculated	recalculate	VERB
eurjchem-440	90	22	again	again	ADV
eurjchem-440	90	23	.	.	PUNCT
eurjchem-440	91	1	these	these	DET
eurjchem-440	91	2	steps	step	NOUN
eurjchem-440	91	3	of	of	ADP
eurjchem-440	91	4	calculations	calculation	NOUN
eurjchem-440	91	5	were	be	AUX
eurjchem-440	91	6	repeated	repeat	VERB
eurjchem-440	91	7	many	many	ADJ
eurjchem-440	91	8	times	time	NOUN
eurjchem-440	91	9	until	until	SCONJ
eurjchem-440	91	10	the	the	DET
eurjchem-440	91	11	difference	difference	NOUN
eurjchem-440	91	12	between	between	ADP
eurjchem-440	91	13	two	two	NUM
eurjchem-440	91	14	successive	successive	ADJ
eurjchem-440	91	15	values	value	NOUN
eurjchem-440	91	16	of	of	ADP
eurjchem-440	91	17	[	[	X
eurjchem-440	91	18	cpxl	cpxl	NOUN
eurjchem-440	91	19	]	]	PUNCT
eurjchem-440	91	20	becomes	become	VERB
eurjchem-440	91	21	equal	equal	ADJ
eurjchem-440	91	22	to	to	ADP
eurjchem-440	91	23	or	or	CCONJ
eurjchem-440	91	24	less	less	ADJ
eurjchem-440	91	25	than	than	ADP
eurjchem-440	91	26	10‐7	10‐7	NUM
eurjchem-440	91	27	.	.	PUNCT
eurjchem-440	92	1	the	the	DET
eurjchem-440	92	2	obtained	obtain	VERB
eurjchem-440	92	3	average	average	ADJ
eurjchem-440	92	4	values	value	NOUN
eurjchem-440	92	5	of	of	ADP
eurjchem-440	92	6	kip	kip	PROPN
eurjchem-440	92	7	in	in	ADP
eurjchem-440	92	8	malonate	malonate	ADJ
eurjchem-440	92	9	media	medium	NOUN
eurjchem-440	92	10	with	with	ADP
eurjchem-440	92	11	different	different	ADJ
eurjchem-440	92	12	percentage	percentage	NOUN
eurjchem-440	92	13	of	of	ADP
eurjchem-440	92	14	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	92	15	are	be	AUX
eurjchem-440	92	16	collected	collect	VERB
eurjchem-440	92	17	in	in	ADP
eurjchem-440	92	18	table	table	NOUN
eurjchem-440	92	19	3	3	NUM
eurjchem-440	92	20	.	.	PUNCT
eurjchem-440	92	21	table	table	NOUN
eurjchem-440	92	22	3	3	NUM
eurjchem-440	92	23	.	.	PUNCT
eurjchem-440	92	24	calculated	calculate	VERB
eurjchem-440	92	25	values	value	NOUN
eurjchem-440	92	26	of	of	ADP
eurjchem-440	92	27	rate	rate	NOUN
eurjchem-440	92	28	constants	constant	NOUN
eurjchem-440	92	29	(	(	PUNCT
eurjchem-440	92	30	kipx105	kipx105	PROPN
eurjchem-440	92	31	)	)	PUNCT
eurjchem-440	92	32	in	in	ADP
eurjchem-440	92	33	sec‐1	sec‐1	NUM
eurjchem-440	92	34	for	for	ADP
eurjchem-440	92	35	the	the	DET
eurjchem-440	92	36	aquation	aquation	NOUN
eurjchem-440	92	37	of	of	ADP
eurjchem-440	92	38	[	[	X
eurjchem-440	92	39	co(nh3)5br]2	co(nh3)5br]2	NOUN
eurjchem-440	92	40	+	+	SYM
eurjchem-440	92	41	in	in	ADP
eurjchem-440	92	42	malonate	malonate	ADJ
eurjchem-440	92	43	buffer	buffer	NOUN
eurjchem-440	92	44	containing	contain	VERB
eurjchem-440	92	45	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	92	46	(	(	PUNCT
eurjchem-440	92	47	10‐50	10‐50	NUM
eurjchem-440	92	48	%	%	NOUN
eurjchem-440	92	49	)	)	PUNCT
eurjchem-440	92	50	at	at	ADP
eurjchem-440	92	51	different	different	ADJ
eurjchem-440	92	52	temperatures	temperature	NOUN
eurjchem-440	92	53	.	.	PUNCT
eurjchem-440	93	1	temp	temp	NOUN
eurjchem-440	93	2	.	.	PUNCT
eurjchem-440	94	1	,	,	PUNCT
eurjchem-440	94	2	oc	oc	ADP
eurjchem-440	94	3	kip	kip	PROPN
eurjchem-440	94	4	x105	x105	PROPN
eurjchem-440	95	1	in	in	ADP
eurjchem-440	95	2	malonate	malonate	ADJ
eurjchem-440	95	3	buffer	buffer	NOUN
eurjchem-440	95	4	at	at	ADP
eurjchem-440	95	5	different	different	ADJ
eurjchem-440	95	6	%	%	NOUN
eurjchem-440	95	7	of	of	ADP
eurjchem-440	95	8	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	95	9	10	10	NUM
eurjchem-440	95	10	20	20	NUM
eurjchem-440	95	11	30	30	NUM
eurjchem-440	95	12	40	40	NUM
eurjchem-440	95	13	50	50	NUM
eurjchem-440	95	14	25	25	NUM
eurjchem-440	95	15	9.43	9.43	NUM
eurjchem-440	95	16	0.39	0.39	NUM
eurjchem-440	95	17	2.39	2.39	NUM
eurjchem-440	95	18	0.39	0.39	NUM
eurjchem-440	95	19	0.71	0.71	NUM
eurjchem-440	95	20	30	30	NUM
eurjchem-440	95	21	16.46	16.46	NUM
eurjchem-440	95	22	1.04	1.04	NUM
eurjchem-440	95	23	4.16	4.16	NUM
eurjchem-440	95	24	0.86	0.86	NUM
eurjchem-440	95	25	1.36	1.36	NUM
eurjchem-440	95	26	35	35	NUM
eurjchem-440	95	27	28.22	28.22	NUM
eurjchem-440	95	28	2.59	2.59	NUM
eurjchem-440	95	29	7.10	7.10	NUM
eurjchem-440	95	30	1.83	1.83	NUM
eurjchem-440	95	31	2.56	2.56	NUM
eurjchem-440	95	32	40	40	NUM
eurjchem-440	95	33	47.54	47.54	NUM
eurjchem-440	95	34	6.32	6.32	NUM
eurjchem-440	95	35	11.92	11.92	NUM
eurjchem-440	95	36	3.79	3.79	NUM
eurjchem-440	95	37	4.73	4.73	NUM
eurjchem-440	95	38	50	50	NUM
eurjchem-440	95	39	128.60	128.60	NUM
eurjchem-440	95	40	34.56	34.56	NUM
eurjchem-440	95	41	32.00	32.00	NUM
eurjchem-440	95	42	15.26	15.26	NUM
eurjchem-440	95	43	15.19	15.19	NUM
eurjchem-440	95	44	60	60	NUM
eurjchem-440	95	45	327.60	327.60	NUM
eurjchem-440	95	46	170.60	170.60	NUM
eurjchem-440	95	47	80.98	80.98	NUM
eurjchem-440	95	48	56.42	56.42	NUM
eurjchem-440	95	49	45.54	45.54	NUM
eurjchem-440	95	50	3.1	3.1	NUM
eurjchem-440	95	51	.	.	PUNCT
eurjchem-440	96	1	variation	variation	NOUN
eurjchem-440	96	2	of	of	ADP
eurjchem-440	96	3	ion‐pair	ion‐pair	PROPN
eurjchem-440	96	4	coefficients	coefficient	NOUN
eurjchem-440	96	5	(	(	PUNCT
eurjchem-440	96	6	kip	kip	PROPN
eurjchem-440	96	7	)	)	PUNCT
eurjchem-440	96	8	with	with	ADP
eurjchem-440	96	9	solvent	solvent	ADJ
eurjchem-440	96	10	parameters	parameter	NOUN
eurjchem-440	96	11	the	the	DET
eurjchem-440	96	12	effect	effect	NOUN
eurjchem-440	96	13	of	of	ADP
eurjchem-440	96	14	water	water	NOUN
eurjchem-440	96	15	concentration	concentration	NOUN
eurjchem-440	96	16	in	in	ADP
eurjchem-440	96	17	aqueous	aqueous	ADJ
eurjchem-440	96	18	organic	organic	ADJ
eurjchem-440	96	19	solvent	solvent	NOUN
eurjchem-440	96	20	mixture	mixture	NOUN
eurjchem-440	96	21	was	be	AUX
eurjchem-440	96	22	investigated	investigate	VERB
eurjchem-440	96	23	by	by	ADP
eurjchem-440	96	24	the	the	DET
eurjchem-440	96	25	plot	plot	NOUN
eurjchem-440	96	26	of	of	ADP
eurjchem-440	96	27	the	the	DET
eurjchem-440	96	28	log	log	NOUN
eurjchem-440	96	29	kip	kip	PROPN
eurjchem-440	96	30	versus	versus	ADP
eurjchem-440	96	31	log	log	PROPN
eurjchem-440	96	32	[	[	X
eurjchem-440	96	33	h2o	h2o	X
eurjchem-440	96	34	]	]	PUNCT
eurjchem-440	96	35	at	at	ADP
eurjchem-440	96	36	30	30	NUM
eurjchem-440	96	37	°	°	NOUN
eurjchem-440	96	38	c	c	NOUN
eurjchem-440	96	39	.	.	PUNCT
eurjchem-440	97	1	this	this	DET
eurjchem-440	97	2	plot	plot	NOUN
eurjchem-440	97	3	was	be	AUX
eurjchem-440	97	4	found	find	VERB
eurjchem-440	97	5	to	to	PART
eurjchem-440	97	6	be	be	AUX
eurjchem-440	97	7	nonlinear	nonlinear	ADJ
eurjchem-440	97	8	as	as	SCONJ
eurjchem-440	97	9	shown	show	VERB
eurjchem-440	97	10	in	in	ADP
eurjchem-440	97	11	figure	figure	NOUN
eurjchem-440	97	12	1	1	NUM
eurjchem-440	97	13	.	.	PUNCT
eurjchem-440	98	1	this	this	DET
eurjchem-440	98	2	nonlinearity	nonlinearity	NOUN
eurjchem-440	98	3	confirms	confirm	VERB
eurjchem-440	98	4	that	that	SCONJ
eurjchem-440	98	5	the	the	DET
eurjchem-440	98	6	internal	internal	ADJ
eurjchem-440	98	7	structure	structure	NOUN
eurjchem-440	98	8	of	of	ADP
eurjchem-440	98	9	the	the	DET
eurjchem-440	98	10	media	medium	NOUN
eurjchem-440	98	11	studied	study	VERB
eurjchem-440	98	12	suffered	suffer	VERB
eurjchem-440	98	13	from	from	ADP
eurjchem-440	98	14	serious	serious	ADJ
eurjchem-440	98	15	changes	change	NOUN
eurjchem-440	98	16	on	on	ADP
eurjchem-440	98	17	addition	addition	NOUN
eurjchem-440	98	18	of	of	ADP
eurjchem-440	98	19	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	98	20	in	in	ADP
eurjchem-440	98	21	the	the	DET
eurjchem-440	98	22	presence	presence	NOUN
eurjchem-440	98	23	of	of	ADP
eurjchem-440	98	24	malonate	malonate	ADJ
eurjchem-440	98	25	buffer	buffer	NOUN
eurjchem-440	98	26	,	,	PUNCT
eurjchem-440	98	27	indicating	indicate	VERB
eurjchem-440	98	28	that	that	SCONJ
eurjchem-440	98	29	the	the	DET
eurjchem-440	98	30	hydrogen	hydrogen	NOUN
eurjchem-440	98	31	bond	bond	NOUN
eurjchem-440	98	32	between	between	ADP
eurjchem-440	98	33	the	the	DET
eurjchem-440	98	34	organic	organic	ADJ
eurjchem-440	98	35	solvent	solvent	NOUN
eurjchem-440	98	36	and	and	CCONJ
eurjchem-440	98	37	the	the	DET
eurjchem-440	98	38	buffer	buffer	NOUN
eurjchem-440	98	39	added	add	VERB
eurjchem-440	98	40	to	to	ADP
eurjchem-440	98	41	water	water	NOUN
eurjchem-440	98	42	is	be	AUX
eurjchem-440	98	43	stronger	strong	ADJ
eurjchem-440	98	44	than	than	ADP
eurjchem-440	98	45	between	between	ADP
eurjchem-440	98	46	two	two	NUM
eurjchem-440	98	47	water	water	NOUN
eurjchem-440	98	48	molecules	molecule	NOUN
eurjchem-440	98	49	.	.	PUNCT
eurjchem-440	99	1	thus	thus	ADV
eurjchem-440	99	2	,	,	PUNCT
eurjchem-440	99	3	hydrogen	hydrogen	NOUN
eurjchem-440	99	4	bonding	bonding	NOUN
eurjchem-440	99	5	between	between	ADP
eurjchem-440	99	6	neighboring	neighbor	VERB
eurjchem-440	99	7	water	water	NOUN
eurjchem-440	99	8	molecules	molecule	NOUN
eurjchem-440	99	9	will	will	AUX
eurjchem-440	99	10	be	be	AUX
eurjchem-440	99	11	replaced	replace	VERB
eurjchem-440	99	12	gradually	gradually	ADV
eurjchem-440	99	13	by	by	ADP
eurjchem-440	99	14	hydrogen	hydrogen	NOUN
eurjchem-440	99	15	bonding	bonding	NOUN
eurjchem-440	99	16	with	with	ADP
eurjchem-440	99	17	solvent	solvent	NOUN
eurjchem-440	99	18	and	and	CCONJ
eurjchem-440	99	19	buffer	buffer	VERB
eurjchem-440	99	20	molecules	molecule	NOUN
eurjchem-440	99	21	where	where	SCONJ
eurjchem-440	99	22	the	the	DET
eurjchem-440	99	23	tetrahedral	tetrahedral	ADJ
eurjchem-440	99	24	structure	structure	NOUN
eurjchem-440	99	25	of	of	ADP
eurjchem-440	99	26	water	water	NOUN
eurjchem-440	99	27	is	be	AUX
eurjchem-440	99	28	largely	largely	ADV
eurjchem-440	99	29	broken	break	VERB
eurjchem-440	100	1	[	[	X
eurjchem-440	100	2	14	14	NUM
eurjchem-440	100	3	]	]	PUNCT
eurjchem-440	100	4	.	.	PUNCT
eurjchem-440	101	1	figure	figure	NOUN
eurjchem-440	101	2	1	1	NUM
eurjchem-440	101	3	.	.	PUNCT
eurjchem-440	102	1	log	log	VERB
eurjchem-440	102	2	kip	kip	PROPN
eurjchem-440	102	3	versus	versus	ADP
eurjchem-440	102	4	log	log	PROPN
eurjchem-440	102	5	[	[	X
eurjchem-440	102	6	h2o	h2o	X
eurjchem-440	102	7	]	]	PUNCT
eurjchem-440	102	8	at	at	ADP
eurjchem-440	102	9	30	30	NUM
eurjchem-440	102	10	oc	oc	NOUN
eurjchem-440	102	11	at	at	ADP
eurjchem-440	102	12	different	different	ADJ
eurjchem-440	102	13	concentrations	concentration	NOUN
eurjchem-440	102	14	of	of	ADP
eurjchem-440	102	15	malanote	malanote	ADJ
eurjchem-440	102	16	buffer	buffer	NOUN
eurjchem-440	102	17	.	.	PUNCT
eurjchem-440	103	1	the	the	DET
eurjchem-440	103	2	plot	plot	NOUN
eurjchem-440	103	3	of	of	ADP
eurjchem-440	103	4	log	log	NOUN
eurjchem-440	103	5	kip	kip	PROPN
eurjchem-440	103	6	against	against	ADP
eurjchem-440	103	7	the	the	DET
eurjchem-440	103	8	grunwald‐winstein	grunwald‐winstein	NOUN
eurjchem-440	103	9	y‐values	y‐values	PUNCT
eurjchem-440	103	10	was	be	AUX
eurjchem-440	103	11	found	find	VERB
eurjchem-440	103	12	to	to	PART
eurjchem-440	103	13	be	be	AUX
eurjchem-440	103	14	nonlinear	nonlinear	ADJ
eurjchem-440	103	15	as	as	SCONJ
eurjchem-440	103	16	shown	show	VERB
eurjchem-440	103	17	in	in	ADP
eurjchem-440	103	18	figure	figure	NOUN
eurjchem-440	103	19	2	2	NUM
eurjchem-440	103	20	.	.	PUNCT
eurjchem-440	104	1	this	this	PRON
eurjchem-440	104	2	confirms	confirm	VERB
eurjchem-440	104	3	the	the	DET
eurjchem-440	104	4	differential	differential	ADJ
eurjchem-440	104	5	effect	effect	NOUN
eurjchem-440	104	6	of	of	ADP
eurjchem-440	104	7	solvent	solvent	NOUN
eurjchem-440	104	8	structures	structure	NOUN
eurjchem-440	104	9	between	between	ADP
eurjchem-440	104	10	the	the	DET
eurjchem-440	104	11	initial	initial	NOUN
eurjchem-440	104	12	and	and	CCONJ
eurjchem-440	104	13	the	the	DET
eurjchem-440	104	14	transition	transition	NOUN
eurjchem-440	104	15	states	state	NOUN
eurjchem-440	104	16	.	.	PUNCT
eurjchem-440	105	1	figure	figure	NOUN
eurjchem-440	105	2	2	2	NUM
eurjchem-440	105	3	.	.	PUNCT
eurjchem-440	106	1	log	log	VERB
eurjchem-440	106	2	kip	kip	PROPN
eurjchem-440	106	3	versus	versus	ADP
eurjchem-440	106	4	y	y	PROPN
eurjchem-440	106	5	at	at	ADP
eurjchem-440	106	6	25	25	NUM
eurjchem-440	106	7	oc	oc	NOUN
eurjchem-440	106	8	at	at	ADP
eurjchem-440	106	9	different	different	ADJ
eurjchem-440	106	10	concentrations	concentration	NOUN
eurjchem-440	106	11	of	of	ADP
eurjchem-440	106	12	malonate	malonate	ADJ
eurjchem-440	106	13	buffer	buffer	NOUN
eurjchem-440	106	14	.	.	PUNCT
eurjchem-440	107	1	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	107	2	has	have	VERB
eurjchem-440	107	3	special	special	ADJ
eurjchem-440	107	4	effect	effect	NOUN
eurjchem-440	107	5	on	on	ADP
eurjchem-440	107	6	the	the	DET
eurjchem-440	107	7	formation	formation	NOUN
eurjchem-440	107	8	of	of	ADP
eurjchem-440	107	9	ion‐pair	ion‐pair	PROPN
eurjchem-440	107	10	.	.	PUNCT
eurjchem-440	108	1	this	this	DET
eurjchem-440	108	2	fact	fact	NOUN
eurjchem-440	108	3	was	be	AUX
eurjchem-440	108	4	also	also	ADV
eurjchem-440	108	5	proven	prove	VERB
eurjchem-440	108	6	in	in	ADP
eurjchem-440	108	7	previous	previous	ADJ
eurjchem-440	108	8	studies	study	NOUN
eurjchem-440	108	9	[	[	X
eurjchem-440	108	10	15‐16	15‐16	NUM
eurjchem-440	108	11	]	]	PUNCT
eurjchem-440	108	12	,	,	PUNCT
eurjchem-440	108	13	where	where	SCONJ
eurjchem-440	108	14	it	it	PRON
eurjchem-440	108	15	was	be	AUX
eurjchem-440	108	16	found	find	VERB
eurjchem-440	108	17	that	that	SCONJ
eurjchem-440	108	18	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	108	19	has	have	VERB
eurjchem-440	108	20	a	a	DET
eurjchem-440	108	21	greater	great	ADJ
eurjchem-440	108	22	effect	effect	NOUN
eurjchem-440	108	23	on	on	ADP
eurjchem-440	108	24	the	the	DET
eurjchem-440	108	25	water	water	NOUN
eurjchem-440	108	26	structure	structure	NOUN
eurjchem-440	108	27	than	than	ADP
eurjchem-440	108	28	the	the	DET
eurjchem-440	108	29	other	other	ADJ
eurjchem-440	108	30	solvents	solvent	NOUN
eurjchem-440	108	31	used	use	VERB
eurjchem-440	108	32	earlier	early	ADV
eurjchem-440	108	33	due	due	ADP
eurjchem-440	108	34	to	to	ADP
eurjchem-440	108	35	its	its	PRON
eurjchem-440	108	36	branched	branched	ADJ
eurjchem-440	108	37	chain	chain	NOUN
eurjchem-440	108	38	.	.	PUNCT
eurjchem-440	109	1	this	this	PRON
eurjchem-440	109	2	may	may	AUX
eurjchem-440	109	3	be	be	AUX
eurjchem-440	109	4	attributed	attribute	VERB
eurjchem-440	109	5	to	to	ADP
eurjchem-440	109	6	the	the	DET
eurjchem-440	109	7	variation	variation	NOUN
eurjchem-440	109	8	of	of	ADP
eurjchem-440	109	9	important	important	ADJ
eurjchem-440	109	10	properties	property	NOUN
eurjchem-440	109	11	of	of	ADP
eurjchem-440	109	12	the	the	DET
eurjchem-440	109	13	medium	medium	NOUN
eurjchem-440	109	14	,	,	PUNCT
eurjchem-440	109	15	such	such	ADJ
eurjchem-440	109	16	as	as	ADP
eurjchem-440	109	17	the	the	DET
eurjchem-440	109	18	structure	structure	NOUN
eurjchem-440	109	19	of	of	ADP
eurjchem-440	109	20	the	the	DET
eurjchem-440	109	21	solvent	solvent	NOUN
eurjchem-440	109	22	,	,	PUNCT
eurjchem-440	109	23	ionizing	ionize	VERB
eurjchem-440	109	24	power	power	NOUN
eurjchem-440	109	25	,	,	PUNCT
eurjchem-440	109	26	basicity	basicity	NOUN
eurjchem-440	109	27	and	and	CCONJ
eurjchem-440	109	28	dielectric	dielectric	ADJ
eurjchem-440	109	29	constant	constant	ADJ
eurjchem-440	109	30	,	,	PUNCT
eurjchem-440	109	31	which	which	PRON
eurjchem-440	109	32	greatly	greatly	ADV
eurjchem-440	109	33	influence	influence	VERB
eurjchem-440	109	34	the	the	DET
eurjchem-440	109	35	rate	rate	NOUN
eurjchem-440	109	36	of	of	ADP
eurjchem-440	109	37	the	the	DET
eurjchem-440	109	38	reaction	reaction	NOUN
eurjchem-440	109	39	.	.	PUNCT
eurjchem-440	110	1	in	in	ADP
eurjchem-440	110	2	addition	addition	NOUN
eurjchem-440	110	3	,	,	PUNCT
eurjchem-440	110	4	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	110	5	is	be	AUX
eurjchem-440	110	6	a	a	DET
eurjchem-440	110	7	dipolar	dipolar	ADJ
eurjchem-440	110	8	protic	protic	ADJ
eurjchem-440	110	9	solvent	solvent	NOUN
eurjchem-440	111	1	[	[	X
eurjchem-440	111	2	17	17	NUM
eurjchem-440	111	3	]	]	PUNCT
eurjchem-440	111	4	,	,	PUNCT
eurjchem-440	111	5	since	since	SCONJ
eurjchem-440	111	6	the	the	DET
eurjchem-440	111	7	oxygen	oxygen	NOUN
eurjchem-440	111	8	atom	atom	NOUN
eurjchem-440	111	9	of	of	ADP
eurjchem-440	111	10	an	an	DET
eurjchem-440	111	11	alcohol	alcohol	NOUN
eurjchem-440	111	12	molecule	molecule	NOUN
eurjchem-440	111	13	carries	carry	VERB
eurjchem-440	111	14	one	one	NUM
eurjchem-440	111	15	proton	proton	NOUN
eurjchem-440	111	16	and	and	CCONJ
eurjchem-440	111	17	two	two	NUM
eurjchem-440	111	18	lone	lone	ADJ
eurjchem-440	111	19	pairs	pair	NOUN
eurjchem-440	111	20	of	of	ADP
eurjchem-440	111	21	electrons	electron	NOUN
eurjchem-440	111	22	,	,	PUNCT
eurjchem-440	111	23	it	it	PRON
eurjchem-440	111	24	might	might	AUX
eurjchem-440	111	25	the	the	DET
eurjchem-440	111	26	expected	expect	VERB
eurjchem-440	111	27	to	to	PART
eurjchem-440	111	28	form	form	VERB
eurjchem-440	111	29	three	three	NUM
eurjchem-440	111	30	hydrogen	hydrogen	NOUN
eurjchem-440	111	31	bonds	bond	NOUN
eurjchem-440	111	32	with	with	ADP
eurjchem-440	111	33	its	its	PRON
eurjchem-440	111	34	neighbors	neighbor	NOUN
eurjchem-440	111	35	,	,	PUNCT
eurjchem-440	111	36	but	but	CCONJ
eurjchem-440	111	37	all	all	DET
eurjchem-440	111	38	the	the	DET
eurjchem-440	111	39	evidences	evidence	NOUN
eurjchem-440	111	40	show	show	VERB
eurjchem-440	111	41	that	that	SCONJ
eurjchem-440	111	42	no	no	DET
eurjchem-440	111	43	more	more	ADJ
eurjchem-440	111	44	than	than	ADP
eurjchem-440	111	45	two	two	NUM
eurjchem-440	111	46	bonds	bond	NOUN
eurjchem-440	111	47	are	be	AUX
eurjchem-440	111	48	formed	form	VERB
eurjchem-440	111	49	,	,	PUNCT
eurjchem-440	111	50	each	each	DET
eurjchem-440	111	51	oxygen	oxygen	NOUN
eurjchem-440	111	52	acting	act	VERB
eurjchem-440	111	53	once	once	ADV
eurjchem-440	111	54	as	as	ADP
eurjchem-440	111	55	proton	proton	NOUN
eurjchem-440	111	56	donor	donor	NOUN
eurjchem-440	111	57	and	and	CCONJ
eurjchem-440	111	58	once	once	ADV
eurjchem-440	111	59	as	as	ADP
eurjchem-440	111	60	proton	proton	NOUN
eurjchem-440	111	61	acceptors	acceptor	NOUN
eurjchem-440	111	62	due	due	ADJ
eurjchem-440	111	63	to	to	ADP
eurjchem-440	111	64	steric	steric	ADJ
eurjchem-440	111	65	effects	effect	NOUN
eurjchem-440	111	66	of	of	ADP
eurjchem-440	111	67	the	the	DET
eurjchem-440	111	68	alkyl	alkyl	ADJ
eurjchem-440	111	69	groups	group	NOUN
eurjchem-440	111	70	.	.	PUNCT
eurjchem-440	112	1	also	also	ADV
eurjchem-440	112	2	log	log	VERB
eurjchem-440	112	3	kip	kip	PROPN
eurjchem-440	112	4	was	be	AUX
eurjchem-440	112	5	plotted	plot	VERB
eurjchem-440	112	6	against	against	ADP
eurjchem-440	112	7	reciprocal	reciprocal	NOUN
eurjchem-440	112	8	of	of	ADP
eurjchem-440	112	9	the	the	DET
eurjchem-440	112	10	dielectric	dielectric	ADJ
eurjchem-440	112	11	constant	constant	ADJ
eurjchem-440	112	12	d	d	NOUN
eurjchem-440	112	13	at	at	ADP
eurjchem-440	112	14	25	25	NUM
eurjchem-440	112	15	oc	oc	NOUN
eurjchem-440	112	16	,	,	PUNCT
eurjchem-440	112	17	where	where	SCONJ
eurjchem-440	112	18	the	the	DET
eurjchem-440	112	19	dielectric	dielectric	ADJ
eurjchem-440	112	20	constant	constant	ADJ
eurjchem-440	112	21	values	value	NOUN
eurjchem-440	112	22	of	of	ADP
eurjchem-440	112	23	different	different	ADJ
eurjchem-440	112	24	compositions	composition	NOUN
eurjchem-440	112	25	are	be	AUX
eurjchem-440	112	26	obtained	obtain	VERB
eurjchem-440	112	27	from	from	ADP
eurjchem-440	112	28	akerlof	akerlof	NOUN
eurjchem-440	112	29	data	datum	NOUN
eurjchem-440	112	30	[	[	X
eurjchem-440	112	31	18	18	NUM
eurjchem-440	112	32	]	]	PUNCT
eurjchem-440	112	33	.	.	PUNCT
eurjchem-440	113	1	as	as	SCONJ
eurjchem-440	113	2	shown	show	VERB
eurjchem-440	113	3	in	in	ADP
eurjchem-440	113	4	figure(3	figure(3	NOUN
eurjchem-440	113	5	)	)	PUNCT
eurjchem-440	113	6	,	,	PUNCT
eurjchem-440	113	7	the	the	DET
eurjchem-440	113	8	plot	plot	NOUN
eurjchem-440	113	9	was	be	AUX
eurjchem-440	113	10	found	find	VERB
eurjchem-440	113	11	to	to	PART
eurjchem-440	113	12	be	be	AUX
eurjchem-440	113	13	non	non	ADJ
eurjchem-440	113	14	linear	linear	ADJ
eurjchem-440	113	15	in	in	ADP
eurjchem-440	113	16	accordance	accordance	NOUN
eurjchem-440	113	17	with	with	ADP
eurjchem-440	113	18	the	the	DET
eurjchem-440	113	19	general	general	ADJ
eurjchem-440	113	20	observations	observation	NOUN
eurjchem-440	113	21	found	find	VERB
eurjchem-440	113	22	in	in	ADP
eurjchem-440	113	23	the	the	DET
eurjchem-440	113	24	aquation	aquation	NOUN
eurjchem-440	113	25	of	of	ADP
eurjchem-440	113	26	a	a	DET
eurjchem-440	113	27	large	large	ADJ
eurjchem-440	113	28	number	number	NOUN
eurjchem-440	113	29	of	of	ADP
eurjchem-440	113	30	other	other	ADJ
eurjchem-440	113	31	cobalt(iii	cobalt(iii	NOUN
eurjchem-440	113	32	)	)	PUNCT
eurjchem-440	113	33	complexes	complex	NOUN
eurjchem-440	113	34	[	[	X
eurjchem-440	113	35	19‐20	19‐20	NUM
eurjchem-440	113	36	]	]	PUNCT
eurjchem-440	113	37	in	in	ADP
eurjchem-440	113	38	water‐cosolvent	water‐cosolvent	PROPN
eurjchem-440	113	39	mixtures	mixture	NOUN
eurjchem-440	113	40	,	,	PUNCT
eurjchem-440	113	41	which	which	PRON
eurjchem-440	113	42	led	lead	VERB
eurjchem-440	113	43	to	to	ADP
eurjchem-440	113	44	a	a	DET
eurjchem-440	113	45	conclusion	conclusion	NOUN
eurjchem-440	113	46	,	,	PUNCT
eurjchem-440	113	47	that	that	SCONJ
eurjchem-440	113	48	the	the	DET
eurjchem-440	113	49	contribution	contribution	NOUN
eurjchem-440	113	50	of	of	ADP
eurjchem-440	113	51	the	the	DET
eurjchem-440	113	52	non	non	ADJ
eurjchem-440	113	53	electrostatic	electrostatic	ADJ
eurjchem-440	113	54	part	part	NOUN
eurjchem-440	113	55	of	of	ADP
eurjchem-440	113	56	solvent	solvent	ADJ
eurjchem-440	113	57	effect	effect	NOUN
eurjchem-440	113	58	,	,	PUNCT
eurjchem-440	113	59	overcomes	overcome	VERB
eurjchem-440	113	60	the	the	DET
eurjchem-440	113	61	electrostatic	electrostatic	ADJ
eurjchem-440	113	62	component	component	NOUN
eurjchem-440	113	63	part	part	NOUN
eurjchem-440	113	64	.	.	PUNCT
eurjchem-440	114	1	also	also	ADV
eurjchem-440	114	2	,	,	PUNCT
eurjchem-440	114	3	these	these	DET
eurjchem-440	114	4	parameter	parameter	NOUN
eurjchem-440	114	5	measures	measure	VERB
eurjchem-440	114	6	macroscopic	macroscopic	ADJ
eurjchem-440	114	7	properties	property	NOUN
eurjchem-440	114	8	,	,	PUNCT
eurjchem-440	114	9	while	while	SCONJ
eurjchem-440	114	10	specific	specific	ADJ
eurjchem-440	114	11	solute‐solvent	solute‐solvent	NOUN
eurjchem-440	114	12	interactions	interaction	NOUN
eurjchem-440	114	13	occur	occur	VERB
eurjchem-440	114	14	on	on	ADP
eurjchem-440	114	15	a	a	DET
eurjchem-440	114	16	microscopic	microscopic	ADJ
eurjchem-440	114	17	scale	scale	NOUN
eurjchem-440	114	18	are	be	AUX
eurjchem-440	114	19	completely	completely	ADV
eurjchem-440	114	20	neglected	neglect	VERB
eurjchem-440	114	21	.	.	PUNCT
eurjchem-440	115	1	in	in	ADP
eurjchem-440	115	2	such	such	ADJ
eurjchem-440	115	3	cases	case	NOUN
eurjchem-440	115	4	,	,	PUNCT
eurjchem-440	115	5	the	the	DET
eurjchem-440	115	6	differential	differential	ADJ
eurjchem-440	115	7	solvation	solvation	NOUN
eurjchem-440	115	8	of	of	ADP
eurjchem-440	115	9	the	the	DET
eurjchem-440	115	10	initial	initial	ADJ
eurjchem-440	115	11	and	and	CCONJ
eurjchem-440	115	12	transition	transition	NOUN
eurjchem-440	115	13	states	state	NOUN
eurjchem-440	115	14	is	be	AUX
eurjchem-440	115	15	the	the	DET
eurjchem-440	115	16	controlling	control	VERB
eurjchem-440	115	17	factor	factor	NOUN
eurjchem-440	115	18	for	for	ADP
eurjchem-440	115	19	the	the	DET
eurjchem-440	115	20	changes	change	NOUN
eurjchem-440	115	21	in	in	ADP
eurjchem-440	115	22	the	the	DET
eurjchem-440	115	23	rate	rate	NOUN
eurjchem-440	115	24	constant	constant	ADJ
eurjchem-440	115	25	[	[	X
eurjchem-440	115	26	21	21	NUM
eurjchem-440	115	27	]	]	PUNCT
eurjchem-440	115	28	.	.	PUNCT
eurjchem-440	116	1	figure	figure	NOUN
eurjchem-440	116	2	3	3	NUM
eurjchem-440	116	3	.	.	PUNCT
eurjchem-440	117	1	log	log	VERB
eurjchem-440	117	2	kip	kip	PROPN
eurjchem-440	117	3	versus	versus	ADP
eurjchem-440	117	4	1	1	NUM
eurjchem-440	117	5	/	/	SYM
eurjchem-440	117	6	d	d	NOUN
eurjchem-440	117	7	at	at	ADP
eurjchem-440	117	8	30	30	NUM
eurjchem-440	117	9	oc	oc	NOUN
eurjchem-440	117	10	at	at	ADP
eurjchem-440	117	11	different	different	ADJ
eurjchem-440	117	12	percentages	percentage	NOUN
eurjchem-440	117	13	of	of	ADP
eurjchem-440	117	14	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	117	15	in	in	ADP
eurjchem-440	117	16	malonate	malonate	ADJ
eurjchem-440	117	17	buffer	buffer	NOUN
eurjchem-440	117	18	media	medium	NOUN
eurjchem-440	117	19	.	.	PUNCT
eurjchem-440	118	1	however	however	ADV
eurjchem-440	118	2	,	,	PUNCT
eurjchem-440	118	3	elsemongy	elsemongy	VERB
eurjchem-440	118	4	and	and	CCONJ
eurjchem-440	118	5	amira	amira	PROPN
eurjchem-440	119	1	[	[	X
eurjchem-440	119	2	22	22	NUM
eurjchem-440	119	3	]	]	PUNCT
eurjchem-440	119	4	proposed	propose	VERB
eurjchem-440	119	5	a	a	DET
eurjchem-440	119	6	general	general	ADJ
eurjchem-440	119	7	equation	equation	NOUN
eurjchem-440	119	8	for	for	ADP
eurjchem-440	119	9	the	the	DET
eurjchem-440	119	10	variation	variation	NOUN
eurjchem-440	119	11	of	of	ADP
eurjchem-440	119	12	specific	specific	ADJ
eurjchem-440	119	13	rate	rate	NOUN
eurjchem-440	119	14	constant	constant	ADJ
eurjchem-440	119	15	(	(	PUNCT
eurjchem-440	119	16	k	k	NOUN
eurjchem-440	119	17	)	)	PUNCT
eurjchem-440	119	18	with	with	ADP
eurjchem-440	119	19	the	the	DET
eurjchem-440	119	20	dielectric	dielectric	ADJ
eurjchem-440	119	21	constant	constant	ADJ
eurjchem-440	119	22	(	(	PUNCT
eurjchem-440	119	23	d	d	NOUN
eurjchem-440	119	24	)	)	PUNCT
eurjchem-440	119	25	for	for	ADP
eurjchem-440	119	26	any	any	DET
eurjchem-440	119	27	reaction	reaction	NOUN
eurjchem-440	119	28	,	,	PUNCT
eurjchem-440	119	29	in	in	ADP
eurjchem-440	119	30	which	which	PRON
eurjchem-440	119	31	the	the	DET
eurjchem-440	119	32	transition	transition	NOUN
eurjchem-440	119	33	state	state	NOUN
eurjchem-440	119	34	may	may	AUX
eurjchem-440	119	35	or	or	CCONJ
eurjchem-440	119	36	may	may	AUX
eurjchem-440	119	37	not	not	PART
eurjchem-440	119	38	polarized	polarize	VERB
eurjchem-440	119	39	.	.	PUNCT
eurjchem-440	120	1	this	this	DET
eurjchem-440	120	2	equation	equation	NOUN
eurjchem-440	120	3	was	be	AUX
eurjchem-440	120	4	proved	prove	VERB
eurjchem-440	120	5	to	to	PART
eurjchem-440	120	6	be	be	AUX
eurjchem-440	120	7	applicable	applicable	ADJ
eurjchem-440	120	8	to	to	ADP
eurjchem-440	120	9	usual	usual	ADJ
eurjchem-440	120	10	reactions	reaction	NOUN
eurjchem-440	120	11	,	,	PUNCT
eurjchem-440	120	12	as	as	ADV
eurjchem-440	120	13	well	well	ADV
eurjchem-440	120	14	as	as	ADP
eurjchem-440	120	15	those	those	PRON
eurjchem-440	120	16	exhibiting	exhibit	VERB
eurjchem-440	120	17	minima	minima	NOUN
eurjchem-440	120	18	or	or	CCONJ
eurjchem-440	120	19	maxima	maxima	NOUN
eurjchem-440	120	20	with	with	ADP
eurjchem-440	120	21	solvent	solvent	NOUN
eurjchem-440	120	22	composition	composition	NOUN
eurjchem-440	120	23	variation	variation	NOUN
eurjchem-440	120	24	.	.	PUNCT
eurjchem-440	121	1	their	their	PRON
eurjchem-440	121	2	equation	equation	NOUN
eurjchem-440	121	3	takes	take	VERB
eurjchem-440	121	4	the	the	DET
eurjchem-440	121	5	following	following	NOUN
eurjchem-440	121	6	for	for	ADP
eurjchem-440	121	7	log	log	NOUN
eurjchem-440	122	1	a	a	PRON
eurjchem-440	122	2	/	/	SYM
eurjchem-440	122	3	k	k	NOUN
eurjchem-440	122	4	=	=	PUNCT
eurjchem-440	122	5	e.b/2.302.r.log	e.b/2.302.r.log	PROPN
eurjchem-440	122	6	c	c	X
eurjchem-440	122	7	/	/	SYM
eurjchem-440	122	8	d	d	NOUN
eurjchem-440	122	9	(	(	PUNCT
eurjchem-440	122	10	25	25	NUM
eurjchem-440	122	11	)	)	PUNCT
eurjchem-440	122	12	log	log	NOUN
eurjchem-440	122	13	c	c	NOUN
eurjchem-440	123	1	=	=	PRON
eurjchem-440	123	2	log	log	VERB
eurjchem-440	123	3	a	a	DET
eurjchem-440	123	4	+	+	NOUN
eurjchem-440	123	5	293.15b	293.15b	NUM
eurjchem-440	123	6	(	(	PUNCT
eurjchem-440	123	7	26	26	NUM
eurjchem-440	123	8	)	)	PUNCT
eurjchem-440	123	9	492	492	NUM
eurjchem-440	123	10	zeitouni	zeitouni	NOUN
eurjchem-440	123	11	et	et	PROPN
eurjchem-440	123	12	al	al	PROPN
eurjchem-440	123	13	.	.	PUNCT
eurjchem-440	123	14	/	/	SYM
eurjchem-440	123	15	european	european	PROPN
eurjchem-440	123	16	journal	journal	PROPN
eurjchem-440	123	17	of	of	ADP
eurjchem-440	123	18	chemistry	chemistry	NOUN
eurjchem-440	123	19	2	2	NUM
eurjchem-440	123	20	(	(	PUNCT
eurjchem-440	123	21	4	4	NUM
eurjchem-440	123	22	)	)	PUNCT
eurjchem-440	123	23	(	(	PUNCT
eurjchem-440	123	24	2011	2011	NUM
eurjchem-440	123	25	)	)	PUNCT
eurjchem-440	123	26	489‐494	489‐494	NOUN
eurjchem-440	123	27	where	where	SCONJ
eurjchem-440	123	28	a	a	PRON
eurjchem-440	123	29	is	be	AUX
eurjchem-440	123	30	the	the	DET
eurjchem-440	123	31	frequency	frequency	NOUN
eurjchem-440	123	32	factor	factor	NOUN
eurjchem-440	123	33	,	,	PUNCT
eurjchem-440	123	34	a	a	PRON
eurjchem-440	123	35	and	and	CCONJ
eurjchem-440	123	36	b	b	NOUN
eurjchem-440	123	37	are	be	AUX
eurjchem-440	123	38	akerlof	akerlof	ADJ
eurjchem-440	123	39	’s	’s	PART
eurjchem-440	123	40	empirical	empirical	ADJ
eurjchem-440	123	41	constants	constant	NOUN
eurjchem-440	123	42	[	[	X
eurjchem-440	123	43	17	17	NUM
eurjchem-440	123	44	]	]	PUNCT
eurjchem-440	123	45	.	.	PUNCT
eurjchem-440	124	1	the	the	DET
eurjchem-440	124	2	plot	plot	NOUN
eurjchem-440	124	3	log	log	NOUN
eurjchem-440	124	4	a	a	PRON
eurjchem-440	124	5	/	/	SYM
eurjchem-440	124	6	k	k	PROPN
eurjchem-440	124	7	versus	versus	ADP
eurjchem-440	124	8	e.b	e.b	PROPN
eurjchem-440	124	9	/	/	SYM
eurjchem-440	124	10	log	log	NOUN
eurjchem-440	124	11	c	c	NOUN
eurjchem-440	124	12	/	/	SYM
eurjchem-440	124	13	d	d	NOUN
eurjchem-440	124	14	as	as	SCONJ
eurjchem-440	124	15	shown	show	VERB
eurjchem-440	124	16	in	in	ADP
eurjchem-440	124	17	figure	figure	NOUN
eurjchem-440	124	18	4	4	NUM
eurjchem-440	124	19	,	,	PUNCT
eurjchem-440	124	20	gives	give	VERB
eurjchem-440	124	21	a	a	DET
eurjchem-440	124	22	good	good	ADJ
eurjchem-440	124	23	straight	straight	ADJ
eurjchem-440	124	24	line	line	NOUN
eurjchem-440	124	25	with	with	ADP
eurjchem-440	124	26	a	a	DET
eurjchem-440	124	27	slope	slope	NOUN
eurjchem-440	124	28	approximately	approximately	ADV
eurjchem-440	124	29	equals	equal	VERB
eurjchem-440	124	30	to	to	ADP
eurjchem-440	124	31	0.052	0.052	NUM
eurjchem-440	124	32	,	,	PUNCT
eurjchem-440	124	33	which	which	PRON
eurjchem-440	124	34	is	be	AUX
eurjchem-440	124	35	equal	equal	ADJ
eurjchem-440	124	36	to	to	ADP
eurjchem-440	124	37	1/2.302.r	1/2.302.r	NUM
eurjchem-440	124	38	=	=	SYM
eurjchem-440	124	39	0.052	0.052	NUM
eurjchem-440	124	40	.	.	PUNCT
eurjchem-440	125	1	this	this	DET
eurjchem-440	125	2	result	result	NOUN
eurjchem-440	125	3	adds	add	VERB
eurjchem-440	125	4	a	a	DET
eurjchem-440	125	5	further	further	ADJ
eurjchem-440	125	6	support	support	NOUN
eurjchem-440	125	7	of	of	ADP
eurjchem-440	125	8	the	the	DET
eurjchem-440	125	9	validity	validity	NOUN
eurjchem-440	125	10	of	of	ADP
eurjchem-440	125	11	the	the	DET
eurjchem-440	125	12	above	above	ADJ
eurjchem-440	125	13	equation	equation	NOUN
eurjchem-440	125	14	in	in	ADP
eurjchem-440	125	15	the	the	DET
eurjchem-440	125	16	case	case	NOUN
eurjchem-440	125	17	of	of	ADP
eurjchem-440	125	18	aquation	aquation	NOUN
eurjchem-440	125	19	of	of	ADP
eurjchem-440	125	20	bromo‐	bromo‐	PROPN
eurjchem-440	125	21	pentaamminecobalt(iii	pentaamminecobalt(iii	NOUN
eurjchem-440	125	22	)	)	PUNCT
eurjchem-440	125	23	complex	complex	ADJ
eurjchem-440	125	24	ion	ion	NOUN
eurjchem-440	125	25	in	in	ADP
eurjchem-440	125	26	water‐tert‐butanol	water‐tert‐butanol	PROPN
eurjchem-440	125	27	medium	medium	NOUN
eurjchem-440	125	28	.	.	PUNCT
eurjchem-440	126	1	figure	figure	NOUN
eurjchem-440	126	2	4	4	NUM
eurjchem-440	126	3	.	.	PUNCT
eurjchem-440	126	4	correlation	correlation	NOUN
eurjchem-440	126	5	between	between	ADP
eurjchem-440	126	6	the	the	DET
eurjchem-440	126	7	rate	rate	NOUN
eurjchem-440	126	8	constant	constant	ADJ
eurjchem-440	126	9	and	and	CCONJ
eurjchem-440	126	10	the	the	DET
eurjchem-440	126	11	dielectric	dielectric	ADJ
eurjchem-440	126	12	constant	constant	ADJ
eurjchem-440	126	13	for	for	ADP
eurjchem-440	126	14	malonate	malonate	ADJ
eurjchem-440	126	15	buffer	buffer	NOUN
eurjchem-440	126	16	.	.	PUNCT
eurjchem-440	127	1	3.2	3.2	NUM
eurjchem-440	127	2	.	.	PUNCT
eurjchem-440	128	1	thermodynamic	thermodynamic	ADJ
eurjchem-440	128	2	parameters	parameter	NOUN
eurjchem-440	128	3	of	of	ADP
eurjchem-440	128	4	the	the	DET
eurjchem-440	128	5	ion‐pair	ion‐pair	PROPN
eurjchem-440	128	6	aquation	aquation	NOUN
eurjchem-440	128	7	reactions	reaction	NOUN
eurjchem-440	128	8	the	the	DET
eurjchem-440	128	9	thermodynamic	thermodynamic	ADJ
eurjchem-440	128	10	parameters	parameter	NOUN
eurjchem-440	128	11	of	of	ADP
eurjchem-440	128	12	the	the	DET
eurjchem-440	128	13	activated	activate	VERB
eurjchem-440	128	14	complex	complex	NOUN
eurjchem-440	128	15	at	at	ADP
eurjchem-440	128	16	40	40	NUM
eurjchem-440	128	17	oc	oc	NOUN
eurjchem-440	128	18	were	be	AUX
eurjchem-440	128	19	collected	collect	VERB
eurjchem-440	128	20	in	in	ADP
eurjchem-440	128	21	table	table	NOUN
eurjchem-440	128	22	4	4	NUM
eurjchem-440	128	23	.	.	PUNCT
eurjchem-440	128	24	table	table	NOUN
eurjchem-440	128	25	4	4	NUM
eurjchem-440	128	26	.	.	PUNCT
eurjchem-440	129	1	values	value	NOUN
eurjchem-440	129	2	of	of	ADP
eurjchem-440	129	3	the	the	DET
eurjchem-440	129	4	thermodynamic	thermodynamic	ADJ
eurjchem-440	129	5	parameters	parameter	NOUN
eurjchem-440	129	6	of	of	ADP
eurjchem-440	129	7	the	the	DET
eurjchem-440	129	8	ion‐	ion‐	PUNCT
eurjchem-440	129	9	pairing	pair	VERB
eurjchem-440	129	10	aquation	aquation	NOUN
eurjchem-440	129	11	of	of	ADP
eurjchem-440	129	12	[	[	X
eurjchem-440	129	13	co(nh3)5br]2	co(nh3)5br]2	NOUN
eurjchem-440	129	14	+	+	SYM
eurjchem-440	129	15	in	in	ADP
eurjchem-440	129	16	malonate	malonate	ADJ
eurjchem-440	129	17	buffer	buffer	NOUN
eurjchem-440	129	18	at	at	ADP
eurjchem-440	129	19	different	different	ADJ
eurjchem-440	129	20	mole	mole	NOUN
eurjchem-440	129	21	fraction	fraction	NOUN
eurjchem-440	129	22	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	129	23	at	at	ADP
eurjchem-440	129	24	40	40	NUM
eurjchem-440	129	25	oc	oc	NOUN
eurjchem-440	129	26	.	.	PUNCT
eurjchem-440	129	27	temp	temp	NOUN
eurjchem-440	129	28	.	.	PUNCT
eurjchem-440	130	1	,	,	PUNCT
eurjchem-440	130	2	oc	oc	ADP
eurjchem-440	130	3	x2	x2	INTJ
eurjchem-440	130	4	(	(	PUNCT
eurjchem-440	130	5	mole	mole	NOUN
eurjchem-440	130	6	fraction	fraction	NOUN
eurjchem-440	130	7	)	)	PUNCT
eurjchem-440	130	8	∆hip	∆hip	NOUN
eurjchem-440	130	9	*	*	SYM
eurjchem-440	130	10	(	(	PUNCT
eurjchem-440	130	11	kj	kj	NOUN
eurjchem-440	130	12	/	/	SYM
eurjchem-440	130	13	mole	mole	NOUN
eurjchem-440	130	14	)	)	PUNCT
eurjchem-440	130	15	∆sip	∆sip	NOUN
eurjchem-440	130	16	*	*	SYM
eurjchem-440	130	17	(	(	PUNCT
eurjchem-440	130	18	j	j	PROPN
eurjchem-440	130	19	/	/	SYM
eurjchem-440	130	20	k.mole	k.mole	NOUN
eurjchem-440	130	21	)	)	PUNCT
eurjchem-440	130	22	∆gip	∆gip	NOUN
eurjchem-440	130	23	*	*	PRON
eurjchem-440	130	24	(	(	PUNCT
eurjchem-440	130	25	kj	kj	NOUN
eurjchem-440	130	26	/	/	SYM
eurjchem-440	130	27	mole	mole	NOUN
eurjchem-440	130	28	)	)	PUNCT
eurjchem-440	130	29	40	40	NUM
eurjchem-440	130	30	0.02	0.02	NUM
eurjchem-440	130	31	81.11	81.11	NUM
eurjchem-440	130	32	‐49.81	‐49.81	PROPN
eurjchem-440	130	33	96.69	96.69	NUM
eurjchem-440	130	34	0.045	0.045	NUM
eurjchem-440	130	35	140.23	140.23	NUM
eurjchem-440	130	36	122.51	122.51	NUM
eurjchem-440	130	37	101.94	101.94	NUM
eurjchem-440	130	38	0.075	0.075	NUM
eurjchem-440	130	39	80.50	80.50	NUM
eurjchem-440	130	40	‐63.23	‐63.23	PROPN
eurjchem-440	130	41	100.29	100.29	NUM
eurjchem-440	130	42	0.112	0.112	NUM
eurjchem-440	130	43	114.42	114.42	NUM
eurjchem-440	130	44	35.62	35.62	NUM
eurjchem-440	130	45	103.27	103.27	NUM
eurjchem-440	130	46	0.116	0.116	NUM
eurjchem-440	130	47	95.66	95.66	NUM
eurjchem-440	130	48	‐22.49	‐22.49	ADP
eurjchem-440	130	49	102.42	102.42	NUM
eurjchem-440	130	50	a	a	DET
eurjchem-440	130	51	linear	linear	ADJ
eurjchem-440	130	52	plot	plot	NOUN
eurjchem-440	130	53	of	of	ADP
eurjchem-440	130	54	∆gip	∆gip	NOUN
eurjchem-440	130	55	*	*	PUNCT
eurjchem-440	130	56	against	against	ADP
eurjchem-440	130	57	∆gass	∆gass	PROPN
eurjchem-440	130	58	*	*	SYM
eurjchem-440	130	59	(	(	PUNCT
eurjchem-440	130	60	free	free	ADJ
eurjchem-440	130	61	energy	energy	NOUN
eurjchem-440	130	62	of	of	ADP
eurjchem-440	130	63	ion‐pair	ion‐pair	PROPN
eurjchem-440	130	64	formed	form	VERB
eurjchem-440	130	65	)	)	PUNCT
eurjchem-440	130	66	is	be	AUX
eurjchem-440	130	67	obtained	obtain	VERB
eurjchem-440	130	68	as	as	SCONJ
eurjchem-440	130	69	shown	show	VERB
eurjchem-440	130	70	in	in	ADP
eurjchem-440	130	71	figure	figure	NOUN
eurjchem-440	130	72	5	5	NUM
eurjchem-440	130	73	,	,	PUNCT
eurjchem-440	130	74	which	which	PRON
eurjchem-440	130	75	takes	take	VERB
eurjchem-440	130	76	the	the	DET
eurjchem-440	130	77	form	form	NOUN
eurjchem-440	130	78	,	,	PUNCT
eurjchem-440	130	79	δg∗	δg∗	ADV
eurjchem-440	130	80	=	=	NOUN
eurjchem-440	130	81	′δg	′δg	VERB
eurjchem-440	130	82	+	+	NOUN
eurjchem-440	130	83	b	b	NOUN
eurjchem-440	130	84	’	'	PUNCT
eurjchem-440	130	85	(	(	PUNCT
eurjchem-440	130	86	27	27	NUM
eurjchem-440	130	87	)	)	PUNCT
eurjchem-440	130	88	  	  	SPACE
eurjchem-440	130	89	figure	figure	NOUN
eurjchem-440	130	90	5	5	NUM
eurjchem-440	130	91	.	.	PUNCT
eurjchem-440	131	1	∆gip*versus	∆gip*versus	PROPN
eurjchem-440	131	2	∆gass*for	∆gass*for	PROPN
eurjchem-440	131	3	malonate	malonate	ADJ
eurjchem-440	131	4	buffer	buffer	NOUN
eurjchem-440	131	5	at	at	ADP
eurjchem-440	131	6	different	different	ADJ
eurjchem-440	131	7	solvent	solvent	ADJ
eurjchem-440	131	8	compositions	composition	NOUN
eurjchem-440	131	9	at	at	ADP
eurjchem-440	131	10	40	40	NUM
eurjchem-440	131	11	oc	oc	NOUN
eurjchem-440	131	12	.	.	PUNCT
eurjchem-440	132	1	the	the	DET
eurjchem-440	132	2	relationship	relationship	NOUN
eurjchem-440	132	3	between	between	ADP
eurjchem-440	132	4	the	the	DET
eurjchem-440	132	5	enthalpy	enthalpy	NOUN
eurjchem-440	132	6	of	of	ADP
eurjchem-440	132	7	activation	activation	NOUN
eurjchem-440	132	8	∆hip*and	∆hip*and	CCONJ
eurjchem-440	132	9	the	the	DET
eurjchem-440	132	10	enthalpy	enthalpy	NOUN
eurjchem-440	132	11	of	of	ADP
eurjchem-440	132	12	association	association	NOUN
eurjchem-440	132	13	(	(	PUNCT
eurjchem-440	132	14	ion‐pair	ion‐pair	NOUN
eurjchem-440	132	15	formation	formation	NOUN
eurjchem-440	132	16	)	)	PUNCT
eurjchem-440	132	17	δh	δh	ADP
eurjchem-440	132	18	at	at	ADP
eurjchem-440	132	19	different	different	ADJ
eurjchem-440	132	20	solvent	solvent	ADJ
eurjchem-440	132	21	compositions	composition	NOUN
eurjchem-440	132	22	is	be	AUX
eurjchem-440	132	23	shown	show	VERB
eurjchem-440	132	24	in	in	ADP
eurjchem-440	132	25	figure	figure	NOUN
eurjchem-440	132	26	6	6	NUM
eurjchem-440	132	27	.	.	PUNCT
eurjchem-440	133	1	the	the	DET
eurjchem-440	133	2	plot	plot	NOUN
eurjchem-440	133	3	shows	show	VERB
eurjchem-440	133	4	a	a	DET
eurjchem-440	133	5	linear	linear	ADJ
eurjchem-440	133	6	correlation	correlation	NOUN
eurjchem-440	133	7	which	which	PRON
eurjchem-440	133	8	takes	take	VERB
eurjchem-440	133	9	the	the	DET
eurjchem-440	133	10	form	form	NOUN
eurjchem-440	133	11	of	of	ADP
eurjchem-440	133	12	equation	equation	NOUN
eurjchem-440	133	13	(	(	PUNCT
eurjchem-440	133	14	28	28	NUM
eurjchem-440	133	15	):	):	PUNCT
eurjchem-440	133	16	∆hip	∆hip	NOUN
eurjchem-440	133	17	*	*	SYM
eurjchem-440	134	1	=	=	NOUN
eurjchem-440	134	2	c∆hass	c∆hass	NOUN
eurjchem-440	134	3	*	*	PUNCT
eurjchem-440	135	1	+	+	NUM
eurjchem-440	135	2	d	d	X
eurjchem-440	135	3	’	'	PUNCT
eurjchem-440	135	4	(	(	PUNCT
eurjchem-440	135	5	28	28	NUM
eurjchem-440	135	6	)	)	PUNCT
eurjchem-440	135	7	this	this	DET
eurjchem-440	135	8	behavior	behavior	NOUN
eurjchem-440	135	9	is	be	AUX
eurjchem-440	135	10	due	due	ADJ
eurjchem-440	135	11	to	to	ADP
eurjchem-440	135	12	the	the	DET
eurjchem-440	135	13	interaction	interaction	NOUN
eurjchem-440	135	14	between	between	ADP
eurjchem-440	135	15	the	the	DET
eurjchem-440	135	16	mixed	mixed	ADJ
eurjchem-440	135	17	solvent	solvent	NOUN
eurjchem-440	135	18	medium	medium	NOUN
eurjchem-440	135	19	containing	contain	VERB
eurjchem-440	135	20	the	the	DET
eurjchem-440	135	21	dicarboxylate	dicarboxylate	ADJ
eurjchem-440	135	22	anions	anion	NOUN
eurjchem-440	135	23	and	and	CCONJ
eurjchem-440	135	24	water	water	NOUN
eurjchem-440	135	25	.	.	PUNCT
eurjchem-440	136	1	these	these	DET
eurjchem-440	136	2	interactions	interaction	NOUN
eurjchem-440	136	3	are	be	AUX
eurjchem-440	136	4	attributed	attribute	VERB
eurjchem-440	136	5	to	to	ADP
eurjchem-440	136	6	the	the	DET
eurjchem-440	136	7	essentially	essentially	ADV
eurjchem-440	136	8	co‐operative	co‐operative	ADJ
eurjchem-440	136	9	nature	nature	NOUN
eurjchem-440	136	10	of	of	ADP
eurjchem-440	136	11	hydrogen	hydrogen	NOUN
eurjchem-440	136	12	bonding	bonding	NOUN
eurjchem-440	136	13	;	;	PUNCT
eurjchem-440	136	14	together	together	ADV
eurjchem-440	136	15	with	with	ADP
eurjchem-440	136	16	the	the	DET
eurjchem-440	136	17	unfavorable	unfavorable	ADJ
eurjchem-440	136	18	steric	steric	ADJ
eurjchem-440	136	19	effected	effect	VERB
eurjchem-440	136	20	of	of	ADP
eurjchem-440	136	21	the	the	DET
eurjchem-440	136	22	organic	organic	ADJ
eurjchem-440	136	23	group	group	NOUN
eurjchem-440	136	24	for	for	ADP
eurjchem-440	136	25	both	both	CCONJ
eurjchem-440	136	26	the	the	DET
eurjchem-440	136	27	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	136	28	and	and	CCONJ
eurjchem-440	136	29	the	the	DET
eurjchem-440	136	30	malonate	malonate	ADJ
eurjchem-440	136	31	buffer	buffer	NOUN
eurjchem-440	136	32	.	.	PUNCT
eurjchem-440	137	1	thus	thus	ADV
eurjchem-440	137	2	,	,	PUNCT
eurjchem-440	137	3	it	it	PRON
eurjchem-440	137	4	restricts	restrict	VERB
eurjchem-440	137	5	the	the	DET
eurjchem-440	137	6	degree	degree	NOUN
eurjchem-440	137	7	of	of	ADP
eurjchem-440	137	8	order	order	NOUN
eurjchem-440	137	9	,	,	PUNCT
eurjchem-440	137	10	which	which	PRON
eurjchem-440	137	11	can	can	AUX
eurjchem-440	137	12	be	be	AUX
eurjchem-440	137	13	established	establish	VERB
eurjchem-440	137	14	in	in	ADP
eurjchem-440	137	15	the	the	DET
eurjchem-440	137	16	liquid	liquid	ADJ
eurjchem-440	137	17	state	state	NOUN
eurjchem-440	137	18	,	,	PUNCT
eurjchem-440	137	19	and	and	CCONJ
eurjchem-440	137	20	precludes	preclude	VERB
eurjchem-440	137	21	the	the	DET
eurjchem-440	137	22	kind	kind	NOUN
eurjchem-440	137	23	of	of	ADP
eurjchem-440	137	24	three	three	NUM
eurjchem-440	137	25	dimensional	dimensional	ADJ
eurjchem-440	137	26	associations	association	NOUN
eurjchem-440	137	27	which	which	PRON
eurjchem-440	137	28	is	be	AUX
eurjchem-440	137	29	dominant	dominant	ADJ
eurjchem-440	137	30	in	in	ADP
eurjchem-440	137	31	water	water	NOUN
eurjchem-440	137	32	.	.	PUNCT
eurjchem-440	138	1	figure	figure	VERB
eurjchem-440	138	2	6	6	NUM
eurjchem-440	138	3	.	.	PUNCT
eurjchem-440	138	4	δh∗	δh∗	NOUN
eurjchem-440	138	5	versus	versus	ADP
eurjchem-440	138	6	∆h	∆h	NOUN
eurjchem-440	138	7	for	for	ADP
eurjchem-440	138	8	malonate	malonate	ADJ
eurjchem-440	138	9	buffer	buffer	NOUN
eurjchem-440	138	10	at	at	ADP
eurjchem-440	138	11	different	different	ADJ
eurjchem-440	138	12	solvent	solvent	ADJ
eurjchem-440	138	13	compositions	composition	NOUN
eurjchem-440	138	14	at	at	ADP
eurjchem-440	138	15	40	40	NUM
eurjchem-440	138	16	oc	oc	NOUN
eurjchem-440	138	17	.	.	PUNCT
eurjchem-440	139	1	finally	finally	ADV
eurjchem-440	139	2	,	,	PUNCT
eurjchem-440	139	3	the	the	DET
eurjchem-440	139	4	plots	plot	NOUN
eurjchem-440	139	5	of	of	ADP
eurjchem-440	139	6	δs∗	δs∗	NOUN
eurjchem-440	139	7	versus	versus	ADP
eurjchem-440	139	8	δs	δs	VERB
eurjchem-440	139	9	for	for	ADP
eurjchem-440	139	10	different	different	ADJ
eurjchem-440	139	11	solvent	solvent	NOUN
eurjchem-440	139	12	compositions	composition	NOUN
eurjchem-440	139	13	are	be	AUX
eurjchem-440	139	14	also	also	ADV
eurjchem-440	139	15	found	find	VERB
eurjchem-440	139	16	to	to	PART
eurjchem-440	139	17	be	be	AUX
eurjchem-440	139	18	linear	linear	ADJ
eurjchem-440	139	19	as	as	SCONJ
eurjchem-440	139	20	represented	represent	VERB
eurjchem-440	139	21	in	in	ADP
eurjchem-440	139	22	figure	figure	NOUN
eurjchem-440	139	23	7	7	NUM
eurjchem-440	139	24	according	accord	VERB
eurjchem-440	139	25	to	to	ADP
eurjchem-440	139	26	equation	equation	NOUN
eurjchem-440	139	27	(	(	PUNCT
eurjchem-440	139	28	29	29	NUM
eurjchem-440	139	29	):	):	PUNCT
eurjchem-440	139	30	δs∗	δs∗	NOUN
eurjchem-440	139	31	=	=	SYM
eurjchem-440	139	32	e	e	NOUN
eurjchem-440	139	33	δs	δs	NOUN
eurjchem-440	139	34	+	+	CCONJ
eurjchem-440	139	35	f	f	X
eurjchem-440	139	36	(	(	PUNCT
eurjchem-440	139	37	29	29	NUM
eurjchem-440	139	38	)	)	PUNCT
eurjchem-440	139	39	the	the	DET
eurjchem-440	139	40	obtained	obtain	VERB
eurjchem-440	139	41	correspondence	correspondence	NOUN
eurjchem-440	139	42	suggests	suggest	VERB
eurjchem-440	139	43	that	that	SCONJ
eurjchem-440	139	44	both	both	DET
eurjchem-440	139	45	entropies	entropy	NOUN
eurjchem-440	139	46	of	of	ADP
eurjchem-440	139	47	activation	activation	NOUN
eurjchem-440	139	48	δs∗	δs∗	NOUN
eurjchem-440	139	49	and	and	CCONJ
eurjchem-440	139	50	association	association	NOUN
eurjchem-440	139	51	δs	δs	NOUN
eurjchem-440	139	52	are	be	AUX
eurjchem-440	139	53	largely	largely	ADV
eurjchem-440	139	54	charge‐	charge‐	NOUN
eurjchem-440	139	55	controlled	control	VERB
eurjchem-440	139	56	.	.	PUNCT
eurjchem-440	140	1	figure	figure	NOUN
eurjchem-440	140	2	7	7	NUM
eurjchem-440	140	3	.	.	PUNCT
eurjchem-440	140	4	δs∗	δs∗	NOUN
eurjchem-440	140	5	versus	versus	ADP
eurjchem-440	140	6	∆s	∆s	NOUN
eurjchem-440	140	7	for	for	ADP
eurjchem-440	140	8	malonate	malonate	ADJ
eurjchem-440	140	9	buffer	buffer	NOUN
eurjchem-440	140	10	at	at	ADP
eurjchem-440	140	11	different	different	ADJ
eurjchem-440	140	12	solvent	solvent	ADJ
eurjchem-440	140	13	compositions	composition	NOUN
eurjchem-440	140	14	at	at	ADP
eurjchem-440	140	15	40	40	NUM
eurjchem-440	140	16	oc	oc	NOUN
eurjchem-440	140	17	.	.	PROPN
eurjchem-440	141	1	3.3	3.3	NUM
eurjchem-440	141	2	.	.	PUNCT
eurjchem-440	142	1	variation	variation	NOUN
eurjchem-440	142	2	of	of	ADP
eurjchem-440	142	3	activation	activation	NOUN
eurjchem-440	142	4	parameters	parameter	NOUN
eurjchem-440	142	5	with	with	ADP
eurjchem-440	142	6	solvent	solvent	ADJ
eurjchem-440	142	7	composition	composition	NOUN
eurjchem-440	142	8	the	the	DET
eurjchem-440	142	9	variation	variation	NOUN
eurjchem-440	142	10	of	of	ADP
eurjchem-440	142	11	the	the	DET
eurjchem-440	142	12	thermodynamic	thermodynamic	ADJ
eurjchem-440	142	13	parameters	parameter	NOUN
eurjchem-440	142	14	of	of	ADP
eurjchem-440	142	15	activation	activation	NOUN
eurjchem-440	142	16	δg∗	δg∗	ADV
eurjchem-440	142	17	,	,	PUNCT
eurjchem-440	142	18	δh	δh	ADP
eurjchem-440	142	19	∗	∗	NOUN
eurjchem-440	142	20	and	and	CCONJ
eurjchem-440	142	21	δs	δs	ADP
eurjchem-440	142	22	∗	∗	NOUN
eurjchem-440	142	23	with	with	ADP
eurjchem-440	142	24	the	the	DET
eurjchem-440	142	25	mole	mole	NOUN
eurjchem-440	142	26	fraction	fraction	NOUN
eurjchem-440	142	27	of	of	ADP
eurjchem-440	142	28	the	the	DET
eurjchem-440	142	29	tert‐	tert‐	PROPN
eurjchem-440	142	30	butanol	butanol	NOUN
eurjchem-440	142	31	x2	x2	PROPN
eurjchem-440	142	32	is	be	AUX
eurjchem-440	142	33	introduced	introduce	VERB
eurjchem-440	142	34	in	in	ADP
eurjchem-440	142	35	figure	figure	NOUN
eurjchem-440	142	36	8	8	NUM
eurjchem-440	142	37	at	at	ADP
eurjchem-440	142	38	different	different	ADJ
eurjchem-440	142	39	composition	composition	NOUN
eurjchem-440	142	40	of	of	ADP
eurjchem-440	142	41	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	142	42	.	.	PUNCT
eurjchem-440	143	1	δh	δh	ADP
eurjchem-440	143	2	∗	∗	NOUN
eurjchem-440	143	3	and	and	CCONJ
eurjchem-440	143	4	δs∗	δs∗	VERB
eurjchem-440	143	5	plots	plot	NOUN
eurjchem-440	143	6	versus	versus	ADP
eurjchem-440	143	7	mole	mole	NOUN
eurjchem-440	143	8	fraction	fraction	NOUN
eurjchem-440	143	9	of	of	ADP
eurjchem-440	143	10	the	the	DET
eurjchem-440	143	11	co‐	co‐	NOUN
eurjchem-440	143	12	solvent	solvent	NOUN
eurjchem-440	143	13	x2	x2	NOUN
eurjchem-440	143	14	displayed	display	VERB
eurjchem-440	143	15	extrema	extrema	NOUN
eurjchem-440	143	16	at	at	ADP
eurjchem-440	143	17	different	different	ADJ
eurjchem-440	143	18	values	value	NOUN
eurjchem-440	143	19	of	of	ADP
eurjchem-440	143	20	x2	x2	PROPN
eurjchem-440	143	21	,	,	PUNCT
eurjchem-440	143	22	indicating	indicate	VERB
eurjchem-440	143	23	that	that	SCONJ
eurjchem-440	143	24	the	the	DET
eurjchem-440	143	25	addition	addition	NOUN
eurjchem-440	143	26	of	of	ADP
eurjchem-440	143	27	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	143	28	in	in	ADP
eurjchem-440	143	29	small	small	ADJ
eurjchem-440	143	30	amounts	amount	NOUN
eurjchem-440	143	31	plays	play	VERB
eurjchem-440	143	32	an	an	DET
eurjchem-440	143	33	important	important	ADJ
eurjchem-440	143	34	role	role	NOUN
eurjchem-440	143	35	.	.	PUNCT
eurjchem-440	144	1	this	this	PRON
eurjchem-440	144	2	was	be	AUX
eurjchem-440	144	3	also	also	ADV
eurjchem-440	144	4	observed	observe	VERB
eurjchem-440	144	5	for	for	ADP
eurjchem-440	144	6	trans‐[copy4cl2]1	trans‐[copy4cl2]1	NOUN
eurjchem-440	144	7	+	+	PROPN
eurjchem-440	145	1	[	[	X
eurjchem-440	145	2	23	23	NUM
eurjchem-440	145	3	]	]	PUNCT
eurjchem-440	145	4	and	and	CCONJ
eurjchem-440	145	5	[	[	X
eurjchem-440	145	6	co	co	X
eurjchem-440	145	7	(	(	PUNCT
eurjchem-440	145	8	nh3)5br]2	nh3)5br]2	NUM
eurjchem-440	145	9	+	+	NOUN
eurjchem-440	145	10	[	[	X
eurjchem-440	145	11	24	24	NUM
eurjchem-440	145	12	]	]	PUNCT
eurjchem-440	145	13	where	where	SCONJ
eurjchem-440	145	14	the	the	DET
eurjchem-440	145	15	structure	structure	NOUN
eurjchem-440	145	16	formation	formation	NOUN
eurjchem-440	145	17	becomes	become	VERB
eurjchem-440	145	18	greater	great	ADJ
eurjchem-440	145	19	at	at	ADP
eurjchem-440	145	20	lower	low	ADJ
eurjchem-440	145	21	values	value	NOUN
eurjchem-440	145	22	of	of	ADP
eurjchem-440	145	23	x2	x2	PROPN
eurjchem-440	145	24	.	.	PUNCT
eurjchem-440	146	1	at	at	ADP
eurjchem-440	146	2	the	the	DET
eurjchem-440	146	3	lower	low	ADJ
eurjchem-440	146	4	x2	x2	NOUN
eurjchem-440	146	5	(	(	PUNCT
eurjchem-440	146	6	between	between	ADP
eurjchem-440	146	7	20	20	NUM
eurjchem-440	146	8	%	%	NOUN
eurjchem-440	146	9	to	to	PART
eurjchem-440	146	10	30	30	NUM
eurjchem-440	146	11	%	%	NOUN
eurjchem-440	146	12	;	;	PUNCT
eurjchem-440	146	13	v	v	NOUN
eurjchem-440	146	14	:	:	PUNCT
eurjchem-440	146	15	v	v	NOUN
eurjchem-440	146	16	of	of	ADP
eurjchem-440	146	17	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	146	18	)	)	PUNCT
eurjchem-440	146	19	,	,	PUNCT
eurjchem-440	146	20	the	the	DET
eurjchem-440	146	21	water	water	NOUN
eurjchem-440	146	22	is	be	AUX
eurjchem-440	146	23	rich	rich	ADJ
eurjchem-440	146	24	in	in	ADP
eurjchem-440	146	25	the	the	DET
eurjchem-440	146	26	media	medium	NOUN
eurjchem-440	146	27	where	where	SCONJ
eurjchem-440	146	28	the	the	DET
eurjchem-440	146	29	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	146	30	molecules	molecule	NOUN
eurjchem-440	146	31	progressively	progressively	ADV
eurjchem-440	146	32	occupy	occupy	VERB
eurjchem-440	146	33	the	the	DET
eurjchem-440	146	34	cavities	cavity	NOUN
eurjchem-440	146	35	in	in	ADP
eurjchem-440	146	36	the	the	DET
eurjchem-440	146	37	water	water	NOUN
eurjchem-440	146	38	network	network	NOUN
eurjchem-440	146	39	without	without	ADP
eurjchem-440	146	40	enhancing	enhance	VERB
eurjchem-440	146	41	the	the	DET
eurjchem-440	146	42	water	water	NOUN
eurjchem-440	146	43	structure	structure	NOUN
eurjchem-440	146	44	.	.	PUNCT
eurjchem-440	147	1	however	however	ADV
eurjchem-440	147	2	,	,	PUNCT
eurjchem-440	147	3	with	with	ADP
eurjchem-440	147	4	an	an	DET
eurjchem-440	147	5	increase	increase	NOUN
eurjchem-440	147	6	in	in	ADP
eurjchem-440	147	7	the	the	DET
eurjchem-440	147	8	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	147	9	concentration	concentration	NOUN
eurjchem-440	147	10	,	,	PUNCT
eurjchem-440	147	11	the	the	DET
eurjchem-440	147	12	water	water	NOUN
eurjchem-440	147	13	structure	structure	NOUN
eurjchem-440	147	14	undergoes	undergo	VERB
eurjchem-440	147	15	a	a	DET
eurjchem-440	147	16	gradual	gradual	ADJ
eurjchem-440	147	17	disruption	disruption	NOUN
eurjchem-440	147	18	and	and	CCONJ
eurjchem-440	147	19	clusters	cluster	NOUN
eurjchem-440	147	20	are	be	AUX
eurjchem-440	147	21	formed	form	VERB
eurjchem-440	147	22	through	through	ADP
eurjchem-440	147	23	the	the	DET
eurjchem-440	147	24	formation	formation	NOUN
eurjchem-440	147	25	of	of	ADP
eurjchem-440	147	26	hydrogen	hydrogen	NOUN
eurjchem-440	147	27	bonding	bonding	NOUN
eurjchem-440	147	28	.	.	PUNCT
eurjchem-440	148	1	by	by	ADP
eurjchem-440	148	2	adding	add	VERB
eurjchem-440	148	3	more	more	ADJ
eurjchem-440	148	4	and	and	CCONJ
eurjchem-440	148	5	more	more	ADJ
eurjchem-440	148	6	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	148	7	,	,	PUNCT
eurjchem-440	148	8	it	it	PRON
eurjchem-440	148	9	zeitouni	zeitouni	NOUN
eurjchem-440	148	10	et	et	NOUN
eurjchem-440	148	11	al	al	PROPN
eurjchem-440	148	12	.	.	PUNCT
eurjchem-440	148	13	/	/	SYM
eurjchem-440	148	14	european	european	PROPN
eurjchem-440	148	15	journal	journal	PROPN
eurjchem-440	148	16	of	of	ADP
eurjchem-440	148	17	chemistry	chemistry	NOUN
eurjchem-440	148	18	2	2	NUM
eurjchem-440	148	19	(	(	PUNCT
eurjchem-440	148	20	4	4	NUM
eurjchem-440	148	21	)	)	PUNCT
eurjchem-440	148	22	(	(	PUNCT
eurjchem-440	148	23	2011	2011	NUM
eurjchem-440	148	24	)	)	PUNCT
eurjchem-440	148	25	489‐494	489‐494	NUM
eurjchem-440	148	26	493	493	NUM
eurjchem-440	148	27	has	have	VERB
eurjchem-440	148	28	characteristics	characteristic	NOUN
eurjchem-440	148	29	that	that	SCONJ
eurjchem-440	148	30	the	the	DET
eurjchem-440	148	31	alkyl	alkyl	ADJ
eurjchem-440	148	32	groups	group	NOUN
eurjchem-440	148	33	cooperative	cooperative	ADJ
eurjchem-440	148	34	ordering	ordering	NOUN
eurjchem-440	148	35	of	of	ADP
eurjchem-440	148	36	water	water	NOUN
eurjchem-440	148	37	molecules	molecule	NOUN
eurjchem-440	148	38	by	by	ADP
eurjchem-440	148	39	a	a	DET
eurjchem-440	148	40	hydrophobic	hydrophobic	NOUN
eurjchem-440	148	41	hydration	hydration	NOUN
eurjchem-440	148	42	effect	effect	NOUN
eurjchem-440	148	43	.	.	PUNCT
eurjchem-440	149	1	the	the	DET
eurjchem-440	149	2	changing	changing	NOUN
eurjchem-440	149	3	of	of	ADP
eurjchem-440	149	4	solvent	solvent	ADJ
eurjchem-440	149	5	composition	composition	NOUN
eurjchem-440	149	6	has	have	VERB
eurjchem-440	149	7	little	little	ADJ
eurjchem-440	149	8	effect	effect	NOUN
eurjchem-440	149	9	on	on	ADP
eurjchem-440	149	10	δg∗	δg∗	NOUN
eurjchem-440	149	11	as	as	SCONJ
eurjchem-440	149	12	shown	show	VERB
eurjchem-440	149	13	in	in	ADP
eurjchem-440	149	14	table	table	NOUN
eurjchem-440	149	15	4	4	NUM
eurjchem-440	149	16	by	by	ADP
eurjchem-440	149	17	which	which	PRON
eurjchem-440	149	18	linear	linear	ADJ
eurjchem-440	149	19	plots	plot	NOUN
eurjchem-440	149	20	are	be	AUX
eurjchem-440	149	21	observed	observe	VERB
eurjchem-440	149	22	between	between	ADP
eurjchem-440	149	23	δg∗	δg∗	NOUN
eurjchem-440	149	24	against	against	ADP
eurjchem-440	149	25	x2	x2	PROPN
eurjchem-440	149	26	,	,	PUNCT
eurjchem-440	149	27	indicating	indicate	VERB
eurjchem-440	149	28	the	the	DET
eurjchem-440	149	29	presence	presence	NOUN
eurjchem-440	149	30	of	of	ADP
eurjchem-440	149	31	compensation	compensation	NOUN
eurjchem-440	149	32	effect	effect	NOUN
eurjchem-440	149	33	between	between	ADP
eurjchem-440	149	34	δh	δh	ADP
eurjchem-440	149	35	∗	∗	NOUN
eurjchem-440	149	36	and	and	CCONJ
eurjchem-440	149	37	δs∗	δs∗	NOUN
eurjchem-440	149	38	.	.	PUNCT
eurjchem-440	150	1	figure	figure	NOUN
eurjchem-440	150	2	8	8	NUM
eurjchem-440	150	3	.	.	PUNCT
eurjchem-440	151	1	δg∗	δg∗	NOUN
eurjchem-440	151	2	,	,	PUNCT
eurjchem-440	151	3	δh∗	δh∗	NOUN
eurjchem-440	151	4	and	and	CCONJ
eurjchem-440	151	5	δs∗	δs∗	VERB
eurjchem-440	151	6	versus	versus	ADP
eurjchem-440	151	7	x2	x2	PROPN
eurjchem-440	151	8	for	for	ADP
eurjchem-440	151	9	malonate	malonate	ADJ
eurjchem-440	151	10	buffer	buffer	NOUN
eurjchem-440	151	11	at	at	ADP
eurjchem-440	151	12	different	different	ADJ
eurjchem-440	151	13	solvent	solvent	ADJ
eurjchem-440	151	14	compositions	composition	NOUN
eurjchem-440	151	15	.	.	PUNCT
eurjchem-440	152	1	figure	figure	NOUN
eurjchem-440	152	2	9	9	NUM
eurjchem-440	152	3	shows	show	VERB
eurjchem-440	152	4	the	the	DET
eurjchem-440	152	5	plots	plot	NOUN
eurjchem-440	152	6	of	of	ADP
eurjchem-440	152	7	δh	δh	ADP
eurjchem-440	152	8	∗	∗	NOUN
eurjchem-440	152	9	versus	versus	ADP
eurjchem-440	152	10	δs∗	δs∗	VERB
eurjchem-440	152	11	for	for	ADP
eurjchem-440	152	12	the	the	DET
eurjchem-440	152	13	ion‐	ion‐	PUNCT
eurjchem-440	152	14	pair	pair	NOUN
eurjchem-440	152	15	aquation	aquation	NOUN
eurjchem-440	152	16	reactions	reaction	NOUN
eurjchem-440	152	17	at	at	ADP
eurjchem-440	152	18	different	different	ADJ
eurjchem-440	152	19	compositions	composition	NOUN
eurjchem-440	152	20	of	of	ADP
eurjchem-440	152	21	tert‐	tert‐	PROPN
eurjchem-440	152	22	butanol	butanol	NOUN
eurjchem-440	152	23	with	with	ADP
eurjchem-440	152	24	an	an	DET
eurjchem-440	152	25	isokinetic	isokinetic	ADJ
eurjchem-440	152	26	temperature	temperature	NOUN
eurjchem-440	152	27	,	,	PUNCT
eurjchem-440	152	28	β=58	β=58	SYM
eurjchem-440	152	29	oc	oc	NOUN
eurjchem-440	152	30	,	,	PUNCT
eurjchem-440	152	31	which	which	PRON
eurjchem-440	152	32	lies	lie	VERB
eurjchem-440	152	33	within	within	ADP
eurjchem-440	152	34	the	the	DET
eurjchem-440	152	35	temperature	temperature	NOUN
eurjchem-440	152	36	range	range	NOUN
eurjchem-440	152	37	studied	study	VERB
eurjchem-440	152	38	(	(	PUNCT
eurjchem-440	152	39	30‐60	30‐60	NUM
eurjchem-440	152	40	oc	oc	NOUN
eurjchem-440	152	41	)	)	PUNCT
eurjchem-440	152	42	,	,	PUNCT
eurjchem-440	152	43	this	this	PRON
eurjchem-440	152	44	emphasizes	emphasize	VERB
eurjchem-440	152	45	the	the	DET
eurjchem-440	152	46	compensation	compensation	NOUN
eurjchem-440	152	47	effect	effect	NOUN
eurjchem-440	152	48	.	.	PUNCT
eurjchem-440	153	1	the	the	DET
eurjchem-440	153	2	true	true	ADJ
eurjchem-440	153	3	explanation	explanation	NOUN
eurjchem-440	153	4	of	of	ADP
eurjchem-440	153	5	compensation	compensation	NOUN
eurjchem-440	153	6	effect	effect	NOUN
eurjchem-440	153	7	lies	lie	VERB
eurjchem-440	153	8	in	in	ADP
eurjchem-440	153	9	solute‐solvent	solute‐solvent	NOUN
eurjchem-440	153	10	interactions	interaction	NOUN
eurjchem-440	153	11	,	,	PUNCT
eurjchem-440	153	12	where	where	SCONJ
eurjchem-440	153	13	the	the	DET
eurjchem-440	153	14	interaction	interaction	NOUN
eurjchem-440	153	15	between	between	ADP
eurjchem-440	153	16	the	the	DET
eurjchem-440	153	17	solute	solute	NOUN
eurjchem-440	153	18	and	and	CCONJ
eurjchem-440	153	19	one	one	NUM
eurjchem-440	153	20	of	of	ADP
eurjchem-440	153	21	the	the	DET
eurjchem-440	153	22	solvent	solvent	ADJ
eurjchem-440	153	23	components	component	NOUN
eurjchem-440	153	24	,	,	PUNCT
eurjchem-440	153	25	which	which	PRON
eurjchem-440	153	26	is	be	AUX
eurjchem-440	153	27	tert‐butanol	tert‐butanol	ADJ
eurjchem-440	153	28	,	,	PUNCT
eurjchem-440	153	29	is	be	AUX
eurjchem-440	153	30	particularly	particularly	ADV
eurjchem-440	153	31	strong	strong	ADJ
eurjchem-440	153	32	.	.	PUNCT
eurjchem-440	154	1	this	this	PRON
eurjchem-440	154	2	will	will	AUX
eurjchem-440	154	3	lower	lower	VERB
eurjchem-440	154	4	the	the	DET
eurjchem-440	154	5	enthalpy	enthalpy	NOUN
eurjchem-440	154	6	;	;	PUNCT
eurjchem-440	154	7	it	it	PRON
eurjchem-440	154	8	will	will	AUX
eurjchem-440	154	9	also	also	ADV
eurjchem-440	154	10	,	,	PUNCT
eurjchem-440	154	11	by	by	ADP
eurjchem-440	154	12	restricting	restrict	VERB
eurjchem-440	154	13	the	the	DET
eurjchem-440	154	14	freedom	freedom	NOUN
eurjchem-440	154	15	of	of	ADP
eurjchem-440	154	16	vibration	vibration	NOUN
eurjchem-440	154	17	and	and	CCONJ
eurjchem-440	154	18	of	of	ADP
eurjchem-440	154	19	rotation	rotation	NOUN
eurjchem-440	154	20	of	of	ADP
eurjchem-440	154	21	the	the	DET
eurjchem-440	154	22	solvent	solvent	ADJ
eurjchem-440	154	23	molecules	molecule	NOUN
eurjchem-440	154	24	,	,	PUNCT
eurjchem-440	154	25	will	will	AUX
eurjchem-440	154	26	lower	lower	VERB
eurjchem-440	154	27	the	the	DET
eurjchem-440	154	28	entropy	entropy	NOUN
eurjchem-440	154	29	.	.	PUNCT
eurjchem-440	154	30	  	  	SPACE
eurjchem-440	154	31	figure	figure	NOUN
eurjchem-440	154	32	9	9	NUM
eurjchem-440	154	33	.	.	PUNCT
eurjchem-440	154	34	h∗	h∗	PROPN
eurjchem-440	154	35	versus	versus	ADP
eurjchem-440	154	36	s∗	s∗	PROPN
eurjchem-440	154	37	for	for	ADP
eurjchem-440	154	38	malonate	malonate	ADJ
eurjchem-440	154	39	buffer	buffer	NOUN
eurjchem-440	154	40	at	at	ADP
eurjchem-440	154	41	different	different	ADJ
eurjchem-440	154	42	solvent	solvent	ADJ
eurjchem-440	154	43	compositions	composition	NOUN
eurjchem-440	154	44	at	at	ADP
eurjchem-440	154	45	60	60	NUM
eurjchem-440	154	46	oc	oc	NOUN
eurjchem-440	154	47	.	.	PROPN
eurjchem-440	154	48	3.4	3.4	NUM
eurjchem-440	154	49	.	.	PUNCT
eurjchem-440	155	1	variation	variation	NOUN
eurjchem-440	155	2	of	of	ADP
eurjchem-440	155	3	free	free	ADJ
eurjchem-440	155	4	energy	energy	NOUN
eurjchem-440	155	5	of	of	ADP
eurjchem-440	155	6	transfer	transfer	NOUN
eurjchem-440	155	7	with	with	ADP
eurjchem-440	155	8	solvent	solvent	ADJ
eurjchem-440	155	9	composition	composition	NOUN
eurjchem-440	155	10	it	it	PRON
eurjchem-440	155	11	has	have	AUX
eurjchem-440	155	12	long	long	ADV
eurjchem-440	155	13	been	be	AUX
eurjchem-440	155	14	recognized	recognize	VERB
eurjchem-440	155	15	that	that	SCONJ
eurjchem-440	155	16	the	the	DET
eurjchem-440	155	17	solvolysis	solvolysis	NOUN
eurjchem-440	155	18	reactions	reaction	NOUN
eurjchem-440	155	19	of	of	ADP
eurjchem-440	155	20	co(iii	co(iii	NOUN
eurjchem-440	155	21	)	)	PUNCT
eurjchem-440	155	22	complexes	complex	NOUN
eurjchem-440	155	23	[	[	X
eurjchem-440	155	24	25,26	25,26	NUM
eurjchem-440	155	25	]	]	PUNCT
eurjchem-440	155	26	,	,	PUNCT
eurjchem-440	155	27	proceed	proceed	VERB
eurjchem-440	155	28	via	via	ADP
eurjchem-440	155	29	the	the	DET
eurjchem-440	155	30	i	i	PROPN
eurjchem-440	155	31	d	d	PROPN
eurjchem-440	155	32	mechanism	mechanism	NOUN
eurjchem-440	155	33	[	[	X
eurjchem-440	155	34	27,28	27,28	NOUN
eurjchem-440	155	35	]	]	PUNCT
eurjchem-440	155	36	involving	involve	VERB
eurjchem-440	155	37	the	the	DET
eurjchem-440	155	38	rate‐determining	rate‐determining	NOUN
eurjchem-440	155	39	loss	loss	NOUN
eurjchem-440	155	40	of	of	ADP
eurjchem-440	155	41	the	the	DET
eurjchem-440	155	42	halide	halide	NOUN
eurjchem-440	155	43	ion	ion	NOUN
eurjchem-440	155	44	according	accord	VERB
eurjchem-440	155	45	to	to	ADP
eurjchem-440	155	46	the	the	DET
eurjchem-440	155	47	following	following	ADJ
eurjchem-440	155	48	equations	equation	NOUN
eurjchem-440	155	49	:	:	PUNCT
eurjchem-440	155	50	(	(	PUNCT
eurjchem-440	155	51	30	30	NUM
eurjchem-440	155	52	)	)	PUNCT
eurjchem-440	155	53	(	(	PUNCT
eurjchem-440	155	54	31	31	NUM
eurjchem-440	155	55	)	)	PUNCT
eurjchem-440	155	56	the	the	DET
eurjchem-440	155	57	extreme	extreme	ADJ
eurjchem-440	155	58	extension	extension	NOUN
eurjchem-440	155	59	of	of	ADP
eurjchem-440	155	60	co‐x	co‐x	NOUN
eurjchem-440	155	61	bond	bond	NOUN
eurjchem-440	155	62	in	in	ADP
eurjchem-440	155	63	the	the	DET
eurjchem-440	155	64	transition	transition	NOUN
eurjchem-440	155	65	state	state	NOUN
eurjchem-440	155	66	is	be	AUX
eurjchem-440	155	67	revealed	reveal	VERB
eurjchem-440	155	68	by	by	ADP
eurjchem-440	155	69	a	a	DET
eurjchem-440	155	70	comparison	comparison	NOUN
eurjchem-440	155	71	of	of	ADP
eurjchem-440	155	72	the	the	DET
eurjchem-440	155	73	volumes	volume	NOUN
eurjchem-440	155	74	of	of	ADP
eurjchem-440	155	75	activation	activation	NOUN
eurjchem-440	155	76	with	with	ADP
eurjchem-440	155	77	the	the	DET
eurjchem-440	155	78	overall	overall	ADJ
eurjchem-440	155	79	volume	volume	NOUN
eurjchem-440	155	80	changes	change	NOUN
eurjchem-440	155	81	for	for	ADP
eurjchem-440	155	82	related	related	ADJ
eurjchem-440	155	83	co(iii	co(iii	NOUN
eurjchem-440	155	84	)	)	PUNCT
eurjchem-440	155	85	complexes	complex	NOUN
eurjchem-440	155	86	.	.	PUNCT
eurjchem-440	156	1	the	the	DET
eurjchem-440	156	2	situation	situation	NOUN
eurjchem-440	156	3	affects	affect	VERB
eurjchem-440	156	4	the	the	DET
eurjchem-440	156	5	ions	ion	NOUN
eurjchem-440	156	6	in	in	ADP
eurjchem-440	156	7	the	the	DET
eurjchem-440	156	8	transition	transition	NOUN
eurjchem-440	156	9	state	state	NOUN
eurjchem-440	156	10	to	to	PART
eurjchem-440	156	11	be	be	AUX
eurjchem-440	156	12	independently	independently	ADV
eurjchem-440	156	13	solvated	solvate	VERB
eurjchem-440	156	14	,	,	PUNCT
eurjchem-440	156	15	which	which	PRON
eurjchem-440	156	16	allows	allow	VERB
eurjchem-440	156	17	the	the	DET
eurjchem-440	156	18	application	application	NOUN
eurjchem-440	156	19	of	of	ADP
eurjchem-440	156	20	a	a	DET
eurjchem-440	156	21	free	free	ADJ
eurjchem-440	156	22	energy	energy	NOUN
eurjchem-440	156	23	cycle	cycle	NOUN
eurjchem-440	156	24	constructed	construct	VERB
eurjchem-440	156	25	by	by	ADP
eurjchem-440	156	26	wells	well	NOUN
eurjchem-440	156	27	[	[	X
eurjchem-440	156	28	29	29	NUM
eurjchem-440	156	29	]	]	PUNCT
eurjchem-440	156	30	,	,	PUNCT
eurjchem-440	156	31	relating	relate	VERB
eurjchem-440	156	32	the	the	DET
eurjchem-440	156	33	process	process	NOUN
eurjchem-440	156	34	initial	initial	ADJ
eurjchem-440	156	35	state	state	NOUN
eurjchem-440	156	36	into	into	ADP
eurjchem-440	156	37	transition	transition	NOUN
eurjchem-440	156	38	state	state	NOUN
eurjchem-440	156	39	for	for	ADP
eurjchem-440	156	40	the	the	DET
eurjchem-440	156	41	aquation	aquation	NOUN
eurjchem-440	156	42	of	of	ADP
eurjchem-440	156	43	the	the	DET
eurjchem-440	156	44	six	six	NUM
eurjchem-440	156	45	co‐	co‐	NOUN
eurjchem-440	156	46	ordinated	ordinated	ADJ
eurjchem-440	156	47	complex	complex	NOUN
eurjchem-440	156	48	[	[	X
eurjchem-440	156	49	co(nh3)5x]+2	co(nh3)5x]+2	VERB
eurjchem-440	156	50	to	to	PART
eurjchem-440	156	51	give	give	VERB
eurjchem-440	156	52	five	five	NUM
eurjchem-440	156	53	co‐ordinated	co‐ordinate	VERB
eurjchem-440	156	54	[	[	PUNCT
eurjchem-440	156	55	co(nh3)5x]+3	co(nh3)5x]+3	NOUN
eurjchem-440	156	56	intermediate	intermediate	ADJ
eurjchem-440	156	57	together	together	ADV
eurjchem-440	156	58	with	with	ADP
eurjchem-440	156	59	the	the	DET
eurjchem-440	156	60	halide	halide	NOUN
eurjchem-440	156	61	ion	ion	NOUN
eurjchem-440	156	62	in	in	ADP
eurjchem-440	156	63	the	the	DET
eurjchem-440	156	64	transition	transition	NOUN
eurjchem-440	156	65	state	state	NOUN
eurjchem-440	156	66	in	in	ADP
eurjchem-440	156	67	water	water	NOUN
eurjchem-440	156	68	(	(	PUNCT
eurjchem-440	156	69	w	w	NOUN
eurjchem-440	156	70	)	)	PUNCT
eurjchem-440	156	71	and	and	CCONJ
eurjchem-440	156	72	in	in	ADP
eurjchem-440	156	73	the	the	DET
eurjchem-440	156	74	mixed	mixed	ADJ
eurjchem-440	156	75	solvent	solvent	NOUN
eurjchem-440	156	76	(	(	PUNCT
eurjchem-440	156	77	s	s	NOUN
eurjchem-440	156	78	)	)	PUNCT
eurjchem-440	157	1	[	[	X
eurjchem-440	157	2	29‐	29‐	NUM
eurjchem-440	157	3	30	30	NUM
eurjchem-440	157	4	]	]	PUNCT
eurjchem-440	157	5	according	accord	VERB
eurjchem-440	157	6	to	to	ADP
eurjchem-440	157	7	the	the	DET
eurjchem-440	157	8	following	follow	VERB
eurjchem-440	157	9	scheme	scheme	NOUN
eurjchem-440	157	10	:	:	PUNCT
eurjchem-440	157	11	initial	initial	ADJ
eurjchem-440	157	12	state	state	NOUN
eurjchem-440	157	13	transition	transition	NOUN
eurjchem-440	157	14	state	state	NOUN
eurjchem-440	157	15	where	where	SCONJ
eurjchem-440	157	16	δg	δg	ADP
eurjchem-440	157	17	∗is	∗is	VERB
eurjchem-440	157	18	the	the	DET
eurjchem-440	157	19	activation	activation	NOUN
eurjchem-440	157	20	free	free	ADJ
eurjchem-440	157	21	energy	energy	NOUN
eurjchem-440	157	22	in	in	ADP
eurjchem-440	157	23	the	the	DET
eurjchem-440	157	24	medium	medium	NOUN
eurjchem-440	157	25	i	i	NOUN
eurjchem-440	157	26	(	(	PUNCT
eurjchem-440	157	27	i	i	NOUN
eurjchem-440	157	28	=	=	SYM
eurjchem-440	157	29	w	w	PROPN
eurjchem-440	157	30	for	for	ADP
eurjchem-440	157	31	water	water	NOUN
eurjchem-440	157	32	and	and	CCONJ
eurjchem-440	157	33	s	s	X
eurjchem-440	157	34	for	for	ADP
eurjchem-440	157	35	the	the	DET
eurjchem-440	157	36	mixed	mixed	ADJ
eurjchem-440	157	37	solvent	solvent	NOUN
eurjchem-440	157	38	)	)	PUNCT
eurjchem-440	157	39	.	.	PUNCT
eurjchem-440	158	1	equation	equation	NOUN
eurjchem-440	158	2	(	(	PUNCT
eurjchem-440	158	3	32	32	NUM
eurjchem-440	158	4	)	)	PUNCT
eurjchem-440	158	5	results	result	NOUN
eurjchem-440	158	6	from	from	ADP
eurjchem-440	158	7	this	this	DET
eurjchem-440	158	8	cycle	cycle	NOUN
eurjchem-440	158	9	,	,	PUNCT
eurjchem-440	158	10	where	where	SCONJ
eurjchem-440	158	11	δg	δg	VERB
eurjchem-440	158	12	(	(	PUNCT
eurjchem-440	158	13	i	i	NOUN
eurjchem-440	158	14	)	)	PUNCT
eurjchem-440	158	15	is	be	AUX
eurjchem-440	158	16	the	the	DET
eurjchem-440	158	17	free	free	ADJ
eurjchem-440	158	18	energy	energy	NOUN
eurjchem-440	158	19	of	of	ADP
eurjchem-440	158	20	transfer	transfer	NOUN
eurjchem-440	158	21	of	of	ADP
eurjchem-440	158	22	species	specie	NOUN
eurjchem-440	158	23	(	(	PUNCT
eurjchem-440	158	24	i	i	NOUN
eurjchem-440	158	25	)	)	PUNCT
eurjchem-440	158	26	between	between	ADP
eurjchem-440	158	27	water	water	NOUN
eurjchem-440	158	28	and	and	CCONJ
eurjchem-440	158	29	the	the	DET
eurjchem-440	158	30	mixed	mixed	ADJ
eurjchem-440	158	31	solvent	solvent	NOUN
eurjchem-440	158	32	.	.	PUNCT
eurjchem-440	159	1	δg∗	δg∗	PROPN
eurjchem-440	159	2	–	–	PUNCT
eurjchem-440	159	3	δg∗	δg∗	ADV
eurjchem-440	159	4	=	=	PUNCT
eurjchem-440	159	5	δg	δg	ADP
eurjchem-440	159	6	[	[	NOUN
eurjchem-440	159	7	co(nh3)5)]+3	co(nh3)5)]+3	NOUN
eurjchem-440	159	8	+	+	CCONJ
eurjchem-440	159	9	δg	δg	ADJ
eurjchem-440	159	10	(	(	PUNCT
eurjchem-440	159	11	x	x	NOUN
eurjchem-440	159	12	)	)	PUNCT
eurjchem-440	159	13	–	–	PUNCT
eurjchem-440	159	14	δg	δg	ADP
eurjchem-440	159	15	[	[	X
eurjchem-440	159	16	co(nh3)5x]+2	co(nh3)5x]+2	NOUN
eurjchem-440	159	17	(	(	PUNCT
eurjchem-440	159	18	32	32	NUM
eurjchem-440	159	19	)	)	PUNCT
eurjchem-440	159	20	converting	convert	VERB
eurjchem-440	159	21	free	free	ADJ
eurjchem-440	159	22	energies	energy	NOUN
eurjchem-440	159	23	of	of	ADP
eurjchem-440	159	24	activation	activation	NOUN
eurjchem-440	159	25	,	,	PUNCT
eurjchem-440	159	26	δg	δg	PROPN
eurjchem-440	159	27	*	*	NOUN
eurjchem-440	159	28	,	,	PUNCT
eurjchem-440	159	29	into	into	ADP
eurjchem-440	159	30	rate	rate	NOUN
eurjchem-440	159	31	constant	constant	ADJ
eurjchem-440	159	32	(	(	PUNCT
eurjchem-440	159	33	32	32	NUM
eurjchem-440	159	34	)	)	PUNCT
eurjchem-440	159	35	can	can	AUX
eurjchem-440	159	36	be	be	AUX
eurjchem-440	159	37	rearranged	rearrange	VERB
eurjchem-440	159	38	to	to	ADP
eurjchem-440	159	39	equation	equation	NOUN
eurjchem-440	159	40	(	(	PUNCT
eurjchem-440	159	41	33	33	NUM
eurjchem-440	159	42	):	):	PUNCT
eurjchem-440	159	43	2.303.r.t.log	2.303.r.t.log	NUM
eurjchem-440	159	44	‐δg	‐δg	X
eurjchem-440	159	45	(	(	PUNCT
eurjchem-440	159	46	x	x	X
eurjchem-440	159	47	)	)	PUNCT
eurjchem-440	159	48	=	=	PUNCT
eurjchem-440	159	49	δg	δg	ADP
eurjchem-440	159	50	[	[	NOUN
eurjchem-440	159	51	co(nh3)5)]+3	co(nh3)5)]+3	X
eurjchem-440	159	52	–	–	PUNCT
eurjchem-440	159	53	δg	δg	ADP
eurjchem-440	159	54	[	[	PUNCT
eurjchem-440	159	55	co(nh3)5x]+2	co(nh3)5x]+2	NOUN
eurjchem-440	159	56	(	(	PUNCT
eurjchem-440	159	57	33	33	NUM
eurjchem-440	159	58	)	)	PUNCT
eurjchem-440	159	59	which	which	PRON
eurjchem-440	159	60	relates	relate	VERB
eurjchem-440	159	61	the	the	DET
eurjchem-440	159	62	rate	rate	NOUN
eurjchem-440	159	63	constant	constant	ADJ
eurjchem-440	159	64	with	with	ADP
eurjchem-440	159	65	non‐electrostatic	non‐electrostatic	ADJ
eurjchem-440	159	66	component	component	NOUN
eurjchem-440	159	67	of	of	ADP
eurjchem-440	159	68	the	the	DET
eurjchem-440	159	69	solvent	solvent	NOUN
eurjchem-440	159	70	mixture	mixture	NOUN
eurjchem-440	159	71	.	.	PUNCT
eurjchem-440	160	1	while	while	SCONJ
eurjchem-440	160	2	applying	apply	VERB
eurjchem-440	160	3	the	the	DET
eurjchem-440	160	4	free	free	ADJ
eurjchem-440	160	5	energy	energy	NOUN
eurjchem-440	160	6	cycle	cycle	NOUN
eurjchem-440	160	7	for	for	ADP
eurjchem-440	160	8	the	the	DET
eurjchem-440	160	9	ion‐pair	ion‐pair	PROPN
eurjchem-440	160	10	effect	effect	NOUN
eurjchem-440	160	11	on	on	ADP
eurjchem-440	160	12	the	the	DET
eurjchem-440	160	13	aquation	aquation	NOUN
eurjchem-440	160	14	of	of	ADP
eurjchem-440	160	15	the	the	DET
eurjchem-440	160	16	bromopentaamminecobalt(iii	bromopentaamminecobalt(iii	NOUN
eurjchem-440	160	17	)	)	PUNCT
eurjchem-440	160	18	complex	complex	ADJ
eurjchem-440	160	19	ion	ion	NOUN
eurjchem-440	160	20	in	in	ADP
eurjchem-440	160	21	the	the	DET
eurjchem-440	160	22	dicarboxylates	dicarboxylate	NOUN
eurjchem-440	160	23	media	medium	NOUN
eurjchem-440	160	24	follow	follow	VERB
eurjchem-440	160	25	the	the	DET
eurjchem-440	160	26	following	follow	VERB
eurjchem-440	160	27	equations	equation	NOUN
eurjchem-440	160	28	:	:	PUNCT
eurjchem-440	160	29	(	(	PUNCT
eurjchem-440	160	30	34	34	NUM
eurjchem-440	160	31	)	)	PUNCT
eurjchem-440	160	32	(	(	PUNCT
eurjchem-440	160	33	35	35	NUM
eurjchem-440	160	34	)	)	PUNCT
eurjchem-440	160	35	however	however	ADV
eurjchem-440	160	36	,	,	PUNCT
eurjchem-440	160	37	equation	equation	NOUN
eurjchem-440	160	38	(	(	PUNCT
eurjchem-440	160	39	33	33	NUM
eurjchem-440	160	40	)	)	PUNCT
eurjchem-440	160	41	can	can	AUX
eurjchem-440	160	42	be	be	AUX
eurjchem-440	160	43	converted	convert	VERB
eurjchem-440	160	44	to	to	ADP
eurjchem-440	160	45	equation	equation	NOUN
eurjchem-440	160	46	(	(	PUNCT
eurjchem-440	160	47	36	36	NUM
eurjchem-440	160	48	)	)	PUNCT
eurjchem-440	160	49	2.303.r.t.log	2.303.r.t.log	NUM
eurjchem-440	160	50	‐δg	‐δg	X
eurjchem-440	160	51	(	(	PUNCT
eurjchem-440	160	52	x	x	X
eurjchem-440	160	53	)	)	PUNCT
eurjchem-440	160	54	=	=	SYM
eurjchem-440	160	55	δg	δg	ADJ
eurjchem-440	160	56	(	(	PUNCT
eurjchem-440	160	57	l‐2	l‐2	NOUN
eurjchem-440	160	58	…	…	X
eurjchem-440	160	59	[co(nh3)5)]+3	[co(nh3)5)]+3	NOUN
eurjchem-440	160	60	–	–	PUNCT
eurjchem-440	160	61	δg	δg	PRON
eurjchem-440	160	62	(	(	PUNCT
eurjchem-440	160	63	l‐2	l‐2	NOUN
eurjchem-440	160	64	…	…	PUNCT
eurjchem-440	160	65	[co(nh3)5x]+2	[co(nh3)5x]+2	X
eurjchem-440	160	66	(	(	PUNCT
eurjchem-440	160	67	36	36	NUM
eurjchem-440	160	68	)	)	PUNCT
eurjchem-440	160	69	values	value	NOUN
eurjchem-440	160	70	of	of	ADP
eurjchem-440	160	71	k0	k0	PROPN
eurjchem-440	160	72	and	and	CCONJ
eurjchem-440	160	73	kip	kip	PROPN
eurjchem-440	160	74	at	at	ADP
eurjchem-440	160	75	25	25	NUM
eurjchem-440	160	76	°	°	NOUN
eurjchem-440	160	77	c	c	NOUN
eurjchem-440	160	78	were	be	AUX
eurjchem-440	160	79	obtained	obtain	VERB
eurjchem-440	160	80	from	from	ADP
eurjchem-440	160	81	the	the	DET
eurjchem-440	160	82	interpolation	interpolation	NOUN
eurjchem-440	160	83	of	of	ADP
eurjchem-440	160	84	arrhenius	arrhenius	PROPN
eurjchem-440	160	85	plot	plot	NOUN
eurjchem-440	160	86	and	and	CCONJ
eurjchem-440	160	87	values	value	NOUN
eurjchem-440	160	88	of	of	ADP
eurjchem-440	160	89	δg	δg	PROPN
eurjchem-440	160	90	(	(	PUNCT
eurjchem-440	160	91	br‐	br‐	X
eurjchem-440	160	92	)	)	PUNCT
eurjchem-440	160	93	were	be	AUX
eurjchem-440	160	94	obtained	obtain	VERB
eurjchem-440	160	95	from	from	ADP
eurjchem-440	160	96	the	the	DET
eurjchem-440	160	97	literature	literature	NOUN
eurjchem-440	160	98	[	[	X
eurjchem-440	160	99	29	29	NUM
eurjchem-440	160	100	]	]	PUNCT
eurjchem-440	160	101	,	,	PUNCT
eurjchem-440	160	102	for	for	ADP
eurjchem-440	160	103	tert‐butanol‐water	tert‐butanol‐water	NOUN
eurjchem-440	160	104	mixtures	mixture	NOUN
eurjchem-440	160	105	with	with	ADP
eurjchem-440	160	106	a	a	DET
eurjchem-440	160	107	range	range	NOUN
eurjchem-440	160	108	of	of	ADP
eurjchem-440	160	109	co‐solvent	co‐solvent	ADJ
eurjchem-440	160	110	.	.	PUNCT
eurjchem-440	161	1	figure	figure	NOUN
eurjchem-440	161	2	10	10	NUM
eurjchem-440	161	3	depicts	depict	VERB
eurjchem-440	161	4	the	the	DET
eurjchem-440	161	5	variation	variation	NOUN
eurjchem-440	161	6	of	of	ADP
eurjchem-440	161	7	the	the	DET
eurjchem-440	161	8	values	value	NOUN
eurjchem-440	161	9	of	of	ADP
eurjchem-440	161	10	the	the	DET
eurjchem-440	161	11	left	left	ADJ
eurjchem-440	161	12	hand	hand	NOUN
eurjchem-440	161	13	side	side	NOUN
eurjchem-440	161	14	of	of	ADP
eurjchem-440	161	15	the	the	DET
eurjchem-440	161	16	equation	equation	NOUN
eurjchem-440	161	17	(	(	PUNCT
eurjchem-440	161	18	36	36	NUM
eurjchem-440	161	19	)	)	PUNCT
eurjchem-440	161	20	at	at	ADP
eurjchem-440	161	21	25	25	NUM
eurjchem-440	161	22	°	°	NOUN
eurjchem-440	161	23	c	c	NOUN
eurjchem-440	161	24	as	as	ADP
eurjchem-440	161	25	a	a	DET
eurjchem-440	161	26	function	function	NOUN
eurjchem-440	161	27	of	of	ADP
eurjchem-440	161	28	mole	mole	ADJ
eurjchem-440	161	29	fraction	fraction	NOUN
eurjchem-440	161	30	of	of	ADP
eurjchem-440	161	31	the	the	DET
eurjchem-440	161	32	co‐solvent	co‐solvent	NOUN
eurjchem-440	161	33	from	from	ADP
eurjchem-440	161	34	which	which	PRON
eurjchem-440	161	35	the	the	DET
eurjchem-440	161	36	differential	differential	ADJ
eurjchem-440	161	37	solvating	solvate	VERB
eurjchem-440	161	38	behavior	behavior	NOUN
eurjchem-440	161	39	of	of	ADP
eurjchem-440	161	40	different	different	ADJ
eurjchem-440	161	41	malonate	malonate	NOUN
eurjchem-440	161	42	buffer	buffer	NOUN
eurjchem-440	161	43	for	for	ADP
eurjchem-440	161	44	the	the	DET
eurjchem-440	161	45	initial	initial	ADJ
eurjchem-440	161	46	and	and	CCONJ
eurjchem-440	161	47	transition	transition	NOUN
eurjchem-440	161	48	state	state	NOUN
eurjchem-440	161	49	is	be	AUX
eurjchem-440	161	50	clearly	clearly	ADV
eurjchem-440	161	51	evident	evident	ADJ
eurjchem-440	161	52	.	.	PUNCT
eurjchem-440	162	1	all	all	DET
eurjchem-440	162	2	the	the	DET
eurjchem-440	162	3	values	value	NOUN
eurjchem-440	162	4	on	on	ADP
eurjchem-440	162	5	the	the	DET
eurjchem-440	162	6	left	left	ADJ
eurjchem-440	162	7	hand	hand	NOUN
eurjchem-440	162	8	side	side	NOUN
eurjchem-440	162	9	of	of	ADP
eurjchem-440	162	10	equation	equation	NOUN
eurjchem-440	162	11	(	(	PUNCT
eurjchem-440	162	12	36	36	NUM
eurjchem-440	162	13	)	)	PUNCT
eurjchem-440	162	14	are	be	AUX
eurjchem-440	162	15	negative	negative	ADJ
eurjchem-440	162	16	as	as	SCONJ
eurjchem-440	162	17	found	find	VERB
eurjchem-440	162	18	for	for	ADP
eurjchem-440	162	19	the	the	DET
eurjchem-440	162	20	aquation	aquation	NOUN
eurjchem-440	162	21	of	of	ADP
eurjchem-440	162	22	a	a	DET
eurjchem-440	162	23	wide	wide	ADJ
eurjchem-440	162	24	range	range	NOUN
eurjchem-440	162	25	of	of	ADP
eurjchem-440	162	26	cobalt(iii	cobalt(iii	NOUN
eurjchem-440	162	27	)	)	PUNCT
eurjchem-440	162	28	complexes	complex	NOUN
eurjchem-440	162	29	in	in	ADP
eurjchem-440	162	30	a	a	DET
eurjchem-440	162	31	mixture	mixture	NOUN
eurjchem-440	162	32	of	of	ADP
eurjchem-440	162	33	water	water	NOUN
eurjchem-440	162	34	with	with	ADP
eurjchem-440	162	35	different	different	ADJ
eurjchem-440	162	36	co‐solvents	co‐solvent	NOUN
eurjchem-440	162	37	[	[	X
eurjchem-440	162	38	31‐33	31‐33	NUM
eurjchem-440	162	39	]	]	PUNCT
eurjchem-440	162	40	.	.	PUNCT
eurjchem-440	163	1	in	in	ADP
eurjchem-440	163	2	all	all	DET
eurjchem-440	163	3	these	these	DET
eurjchem-440	163	4	cases	case	NOUN
eurjchem-440	163	5	,	,	PUNCT
eurjchem-440	163	6	the	the	DET
eurjchem-440	163	7	effect	effect	NOUN
eurjchem-440	163	8	of	of	ADP
eurjchem-440	163	9	changing	change	VERB
eurjchem-440	163	10	solvent	solvent	ADJ
eurjchem-440	163	11	structure	structure	NOUN
eurjchem-440	163	12	on	on	ADP
eurjchem-440	163	13	the	the	DET
eurjchem-440	163	14	pentacoordinatedcobalt	pentacoordinatedcobalt	NOUN
eurjchem-440	163	15	cation	cation	NOUN
eurjchem-440	163	16	in	in	ADP
eurjchem-440	163	17	the	the	DET
eurjchem-440	163	18	transition	transition	NOUN
eurjchem-440	163	19	state	state	NOUN
eurjchem-440	163	20	dominate	dominate	VERB
eurjchem-440	163	21	the	the	DET
eurjchem-440	163	22	effect	effect	NOUN
eurjchem-440	163	23	on	on	ADP
eurjchem-440	163	24	the	the	DET
eurjchem-440	163	25	hexacoordinatedcobalt(iii	hexacoordinatedcobalt(iii	NOUN
eurjchem-440	163	26	)	)	PUNCT
eurjchem-440	163	27	cation	cation	NOUN
eurjchem-440	163	28	in	in	ADP
eurjchem-440	163	29	the	the	DET
eurjchem-440	163	30	initial	initial	ADJ
eurjchem-440	163	31	state	state	NOUN
eurjchem-440	163	32	.	.	PUNCT
eurjchem-440	164	1	thus	thus	ADV
eurjchem-440	164	2	,	,	PUNCT
eurjchem-440	164	3	these	these	DET
eurjchem-440	164	4	negative	negative	ADJ
eurjchem-440	164	5	values	value	NOUN
eurjchem-440	164	6	in	in	ADP
eurjchem-440	164	7	the	the	DET
eurjchem-440	164	8	left	left	ADJ
eurjchem-440	164	9	hand	hand	NOUN
eurjchem-440	164	10	side	side	NOUN
eurjchem-440	164	11	of	of	ADP
eurjchem-440	164	12	equation	equation	NOUN
eurjchem-440	164	13	(	(	PUNCT
eurjchem-440	164	14	36	36	NUM
eurjchem-440	164	15	)	)	PUNCT
eurjchem-440	164	16	indicate	indicate	VERB
eurjchem-440	164	17	that	that	SCONJ
eurjchem-440	164	18	[	[	X
eurjchem-440	164	19	co(nh3)5]+3	co(nh3)5]+3	NOUN
eurjchem-440	164	20	is	be	AUX
eurjchem-440	164	21	more	more	ADV
eurjchem-440	164	22	stable	stable	ADJ
eurjchem-440	164	23	in	in	ADP
eurjchem-440	164	24	tert‐	tert‐	PROPN
eurjchem-440	164	25	butanol‐water	butanol‐water	NOUN
eurjchem-440	164	26	in	in	ADP
eurjchem-440	164	27	the	the	DET
eurjchem-440	164	28	presence	presence	NOUN
eurjchem-440	164	29	of	of	ADP
eurjchem-440	164	30	malonate	malonate	ADJ
eurjchem-440	164	31	buffer	buffer	NOUN
eurjchem-440	164	32	than	than	ADP
eurjchem-440	164	33	[	[	X
eurjchem-440	164	34	co(nh3)5br]+2	co(nh3)5br]+2	NOUN
eurjchem-440	164	35	.	.	NOUN
eurjchem-440	164	36	moreover	moreover	ADV
eurjchem-440	164	37	,	,	PUNCT
eurjchem-440	164	38	the	the	DET
eurjchem-440	164	39	presence	presence	NOUN
eurjchem-440	164	40	of	of	ADP
eurjchem-440	164	41	the	the	DET
eurjchem-440	164	42	malonate	malonate	ADJ
eurjchem-440	164	43	buffer	buffer	NOUN
eurjchem-440	164	44	in	in	ADP
eurjchem-440	164	45	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	164	46	stabilizes	stabilize	VERB
eurjchem-440	164	47	the	the	DET
eurjchem-440	164	48	complex	complex	NOUN
eurjchem-440	164	49	more	more	ADJ
eurjchem-440	164	50	than	than	ADP
eurjchem-440	164	51	the	the	DET
eurjchem-440	164	52	free	free	ADJ
eurjchem-440	164	53	solvent	solvent	NOUN
eurjchem-440	164	54	.	.	PUNCT
eurjchem-440	165	1	this	this	PRON
eurjchem-440	165	2	is	be	AUX
eurjchem-440	165	3	obvious	obvious	ADJ
eurjchem-440	165	4	from	from	ADP
eurjchem-440	165	5	the	the	DET
eurjchem-440	165	6	more	more	ADJ
eurjchem-440	165	7	negativity	negativity	NOUN
eurjchem-440	165	8	of	of	ADP
eurjchem-440	165	9	left	left	ADJ
eurjchem-440	165	10	hand	hand	NOUN
eurjchem-440	165	11	side	side	NOUN
eurjchem-440	165	12	of	of	ADP
eurjchem-440	165	13	the	the	DET
eurjchem-440	165	14	equation	equation	NOUN
eurjchem-440	165	15	(	(	PUNCT
eurjchem-440	165	16	36	36	NUM
eurjchem-440	165	17	)	)	PUNCT
eurjchem-440	165	18	of	of	ADP
eurjchem-440	165	19	malonate	malonate	ADJ
eurjchem-440	165	20	media	medium	NOUN
eurjchem-440	165	21	and	and	CCONJ
eurjchem-440	165	22	the	the	DET
eurjchem-440	165	23	free	free	ADJ
eurjchem-440	165	24	complex	complex	NOUN
eurjchem-440	165	25	.	.	PUNCT
eurjchem-440	166	1	494	494	NUM
eurjchem-440	166	2	zeitouni	zeitouni	NOUN
eurjchem-440	166	3	et	et	PROPN
eurjchem-440	166	4	al	al	PROPN
eurjchem-440	166	5	.	.	PUNCT
eurjchem-440	166	6	/	/	SYM
eurjchem-440	166	7	european	european	PROPN
eurjchem-440	166	8	journal	journal	PROPN
eurjchem-440	166	9	of	of	ADP
eurjchem-440	166	10	chemistry	chemistry	NOUN
eurjchem-440	166	11	2	2	NUM
eurjchem-440	166	12	(	(	PUNCT
eurjchem-440	166	13	4	4	NUM
eurjchem-440	166	14	)	)	PUNCT
eurjchem-440	166	15	(	(	PUNCT
eurjchem-440	166	16	2011	2011	NUM
eurjchem-440	166	17	)	)	PUNCT
eurjchem-440	166	18	489‐494	489‐494	NUM
eurjchem-440	166	19	figure	figure	NOUN
eurjchem-440	166	20	10	10	NUM
eurjchem-440	166	21	.	.	PUNCT
eurjchem-440	167	1	variation	variation	NOUN
eurjchem-440	167	2	of	of	ADP
eurjchem-440	167	3	the	the	DET
eurjchem-440	167	4	value	value	NOUN
eurjchem-440	167	5	of	of	ADP
eurjchem-440	167	6	l.h.s	l.h.s	NOUN
eurjchem-440	167	7	.	.	PUNCT
eurjchem-440	168	1	of	of	ADP
eurjchem-440	168	2	equation	equation	NOUN
eurjchem-440	168	3	(	(	PUNCT
eurjchem-440	168	4	36	36	NUM
eurjchem-440	168	5	)	)	PUNCT
eurjchem-440	168	6	versus	versus	ADP
eurjchem-440	168	7	the	the	DET
eurjchem-440	168	8	mole	mole	NOUN
eurjchem-440	168	9	fraction	fraction	NOUN
eurjchem-440	168	10	x2	x2	PROPN
eurjchem-440	169	1	at	at	ADP
eurjchem-440	169	2	25	25	NUM
eurjchem-440	169	3	oc	oc	NOUN
eurjchem-440	169	4	.	.	PROPN
eurjchem-440	169	5	4	4	NUM
eurjchem-440	169	6	.	.	X
eurjchem-440	169	7	conclusion	conclusion	NOUN
eurjchem-440	169	8	in	in	ADP
eurjchem-440	169	9	conclusion	conclusion	NOUN
eurjchem-440	169	10	from	from	ADP
eurjchem-440	169	11	all	all	DET
eurjchem-440	169	12	the	the	DET
eurjchem-440	169	13	above	above	ADJ
eurjchem-440	169	14	discussion	discussion	NOUN
eurjchem-440	169	15	,	,	PUNCT
eurjchem-440	169	16	the	the	DET
eurjchem-440	169	17	aquation	aquation	NOUN
eurjchem-440	169	18	reaction	reaction	NOUN
eurjchem-440	169	19	was	be	AUX
eurjchem-440	169	20	accelerated	accelerate	VERB
eurjchem-440	169	21	in	in	ADP
eurjchem-440	169	22	the	the	DET
eurjchem-440	169	23	presence	presence	NOUN
eurjchem-440	169	24	of	of	ADP
eurjchem-440	169	25	malonate	malonate	ADJ
eurjchem-440	169	26	buffer	buffer	NOUN
eurjchem-440	169	27	due	due	ADP
eurjchem-440	169	28	to	to	ADP
eurjchem-440	169	29	the	the	DET
eurjchem-440	169	30	formation	formation	NOUN
eurjchem-440	169	31	of	of	ADP
eurjchem-440	169	32	ion‐pair	ion‐pair	NOUN
eurjchem-440	169	33	between	between	ADP
eurjchem-440	169	34	the	the	DET
eurjchem-440	169	35	complex	complex	ADJ
eurjchem-440	169	36	cation	cation	NOUN
eurjchem-440	169	37	and	and	CCONJ
eurjchem-440	169	38	the	the	DET
eurjchem-440	169	39	added	add	VERB
eurjchem-440	169	40	anion	anion	NOUN
eurjchem-440	169	41	.	.	PUNCT
eurjchem-440	170	1	the	the	DET
eurjchem-440	170	2	plot	plot	NOUN
eurjchem-440	170	3	of	of	ADP
eurjchem-440	170	4	log	log	NOUN
eurjchem-440	170	5	kip	kip	PROPN
eurjchem-440	170	6	versus	versus	ADP
eurjchem-440	170	7	the	the	DET
eurjchem-440	170	8	dielectric	dielectric	ADJ
eurjchem-440	170	9	constant	constant	NOUN
eurjchem-440	170	10	is	be	AUX
eurjchem-440	170	11	non	non	ADJ
eurjchem-440	170	12	linear	linear	ADJ
eurjchem-440	170	13	which	which	PRON
eurjchem-440	170	14	means	mean	VERB
eurjchem-440	170	15	that	that	SCONJ
eurjchem-440	170	16	the	the	DET
eurjchem-440	170	17	internal	internal	ADJ
eurjchem-440	170	18	structure	structure	NOUN
eurjchem-440	170	19	of	of	ADP
eurjchem-440	170	20	the	the	DET
eurjchem-440	170	21	medium	medium	NOUN
eurjchem-440	170	22	is	be	AUX
eurjchem-440	170	23	suffered	suffer	VERB
eurjchem-440	170	24	from	from	ADP
eurjchem-440	170	25	serious	serious	ADJ
eurjchem-440	170	26	changes	change	NOUN
eurjchem-440	170	27	on	on	ADP
eurjchem-440	170	28	the	the	DET
eurjchem-440	170	29	progress	progress	NOUN
eurjchem-440	170	30	addition	addition	NOUN
eurjchem-440	170	31	of	of	ADP
eurjchem-440	170	32	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	170	33	to	to	ADP
eurjchem-440	170	34	water	water	VERB
eurjchem-440	170	35	.	.	PUNCT
eurjchem-440	171	1	as	as	ADV
eurjchem-440	171	2	well	well	ADV
eurjchem-440	171	3	as	as	ADP
eurjchem-440	171	4	,	,	PUNCT
eurjchem-440	171	5	the	the	DET
eurjchem-440	171	6	non	non	X
eurjchem-440	171	7	linearity	linearity	NOUN
eurjchem-440	171	8	of	of	ADP
eurjchem-440	171	9	log	log	NOUN
eurjchem-440	171	10	kip	kip	PROPN
eurjchem-440	171	11	versus	versus	ADP
eurjchem-440	171	12	log	log	PROPN
eurjchem-440	171	13	[	[	X
eurjchem-440	171	14	h2o	h2o	X
eurjchem-440	171	15	]	]	PUNCT
eurjchem-440	171	16	and	and	CCONJ
eurjchem-440	171	17	the	the	DET
eurjchem-440	171	18	grunwald‐winstein	grunwald‐winstein	ADJ
eurjchem-440	171	19	y‐values	y‐values	PUNCT
eurjchem-440	172	1	confirms	confirm	VERB
eurjchem-440	172	2	the	the	DET
eurjchem-440	172	3	differential	differential	ADJ
eurjchem-440	172	4	effect	effect	NOUN
eurjchem-440	172	5	of	of	ADP
eurjchem-440	172	6	solvent	solvent	NOUN
eurjchem-440	172	7	structures	structure	NOUN
eurjchem-440	172	8	between	between	ADP
eurjchem-440	172	9	the	the	DET
eurjchem-440	172	10	initial	initial	NOUN
eurjchem-440	172	11	and	and	CCONJ
eurjchem-440	172	12	the	the	DET
eurjchem-440	172	13	transition	transition	NOUN
eurjchem-440	172	14	states	state	NOUN
eurjchem-440	172	15	.	.	PUNCT
eurjchem-440	173	1	from	from	ADP
eurjchem-440	173	2	the	the	DET
eurjchem-440	173	3	extrathermodynamic	extrathermodynamic	ADJ
eurjchem-440	173	4	correlations	correlation	NOUN
eurjchem-440	173	5	,	,	PUNCT
eurjchem-440	173	6	there	there	PRON
eurjchem-440	173	7	is	be	VERB
eurjchem-440	173	8	marked	mark	VERB
eurjchem-440	173	9	effect	effect	NOUN
eurjchem-440	173	10	of	of	ADP
eurjchem-440	173	11	both	both	DET
eurjchem-440	173	12	solute‐solvent	solute‐solvent	NOUN
eurjchem-440	173	13	and	and	CCONJ
eurjchem-440	173	14	solvent‐solvent	solvent‐solvent	NOUN
eurjchem-440	173	15	interactions	interaction	NOUN
eurjchem-440	173	16	on	on	ADP
eurjchem-440	173	17	the	the	DET
eurjchem-440	173	18	ion‐	ion‐	PUNCT
eurjchem-440	173	19	pair	pair	NOUN
eurjchem-440	173	20	formation	formation	NOUN
eurjchem-440	173	21	and	and	CCONJ
eurjchem-440	173	22	aquation	aquation	NOUN
eurjchem-440	173	23	reaction	reaction	NOUN
eurjchem-440	173	24	.	.	PUNCT
eurjchem-440	174	1	the	the	DET
eurjchem-440	174	2	free	free	ADJ
eurjchem-440	174	3	energy	energy	NOUN
eurjchem-440	174	4	of	of	ADP
eurjchem-440	174	5	activation	activation	NOUN
eurjchem-440	174	6	∆g∗	∆g∗	NOUN
eurjchem-440	174	7	is	be	AUX
eurjchem-440	174	8	more	more	ADV
eurjchem-440	174	9	or	or	CCONJ
eurjchem-440	174	10	less	less	ADV
eurjchem-440	174	11	linearly	linearly	ADV
eurjchem-440	174	12	varied	varied	ADJ
eurjchem-440	174	13	with	with	ADP
eurjchem-440	174	14	the	the	DET
eurjchem-440	174	15	mole	mole	NOUN
eurjchem-440	174	16	fraction	fraction	NOUN
eurjchem-440	174	17	of	of	ADP
eurjchem-440	174	18	tert‐butanol	tert‐butanol	NOUN
eurjchem-440	174	19	indicating	indicate	VERB
eurjchem-440	174	20	of	of	ADP
eurjchem-440	174	21	the	the	DET
eurjchem-440	174	22	presence	presence	NOUN
eurjchem-440	174	23	of	of	ADP
eurjchem-440	174	24	compensation	compensation	NOUN
eurjchem-440	174	25	effect	effect	NOUN
eurjchem-440	174	26	between	between	ADP
eurjchem-440	174	27	∆h∗	∆h∗	NOUN
eurjchem-440	174	28	and	and	CCONJ
eurjchem-440	174	29	∆s∗	∆s∗	NOUN
eurjchem-440	174	30	.	.	PUNCT
eurjchem-440	175	1	from	from	ADP
eurjchem-440	175	2	the	the	DET
eurjchem-440	175	3	negative	negative	ADJ
eurjchem-440	175	4	values	value	NOUN
eurjchem-440	175	5	of	of	ADP
eurjchem-440	175	6	left	left	ADJ
eurjchem-440	175	7	hand	hand	NOUN
eurjchem-440	175	8	side	side	NOUN
eurjchem-440	175	9	of	of	ADP
eurjchem-440	175	10	equation	equation	NOUN
eurjchem-440	175	11	(	(	PUNCT
eurjchem-440	175	12	32	32	NUM
eurjchem-440	175	13	)	)	PUNCT
eurjchem-440	175	14	,	,	PUNCT
eurjchem-440	175	15	we	we	PRON
eurjchem-440	175	16	can	can	AUX
eurjchem-440	175	17	conclude	conclude	VERB
eurjchem-440	175	18	that	that	SCONJ
eurjchem-440	175	19	the	the	DET
eurjchem-440	175	20	ions	ion	NOUN
eurjchem-440	175	21	in	in	ADP
eurjchem-440	175	22	the	the	DET
eurjchem-440	175	23	transition	transition	NOUN
eurjchem-440	175	24	are	be	AUX
eurjchem-440	175	25	more	more	ADV
eurjchem-440	175	26	stable	stable	ADJ
eurjchem-440	175	27	than	than	ADP
eurjchem-440	175	28	the	the	DET
eurjchem-440	175	29	initial	initial	ADJ
eurjchem-440	175	30	state	state	NOUN
eurjchem-440	175	31	.	.	PUNCT
eurjchem-440	176	1	acknowledgements	acknowledgement	NOUN
eurjchem-440	176	2	the	the	DET
eurjchem-440	176	3	authors	author	NOUN
eurjchem-440	176	4	are	be	AUX
eurjchem-440	176	5	thankful	thankful	ADJ
eurjchem-440	176	6	to	to	ADP
eurjchem-440	176	7	beirut	beirut	PROPN
eurjchem-440	176	8	arab	arab	PROPN
eurjchem-440	176	9	university	university	PROPN
eurjchem-440	176	10	,	,	PUNCT
eurjchem-440	176	11	faculty	faculty	NOUN
eurjchem-440	176	12	of	of	ADP
eurjchem-440	176	13	science	science	NOUN
eurjchem-440	176	14	,	,	PUNCT
eurjchem-440	176	15	chemistry	chemistry	NOUN
eurjchem-440	176	16	department	department	NOUN
eurjchem-440	176	17	,	,	PUNCT
eurjchem-440	176	18	for	for	ADP
eurjchem-440	176	19	providing	provide	VERB
eurjchem-440	176	20	the	the	DET
eurjchem-440	176	21	facilities	facility	NOUN
eurjchem-440	176	22	used	use	VERB
eurjchem-440	176	23	in	in	ADP
eurjchem-440	176	24	this	this	DET
eurjchem-440	176	25	work	work	NOUN
eurjchem-440	176	26	.	.	PUNCT
eurjchem-440	177	1	references	reference	NOUN
eurjchem-440	177	2	[	[	X
eurjchem-440	177	3	1	1	NUM
eurjchem-440	177	4	]	]	PUNCT
eurjchem-440	177	5	.	.	PUNCT
eurjchem-440	178	1	shaban	shaban	PROPN
eurjchem-440	178	2	,	,	PUNCT
eurjchem-440	178	3	n.	n.	PROPN
eurjchem-440	178	4	z.	z.	PROPN
eurjchem-440	178	5	;	;	PUNCT
eurjchem-440	178	6	el‐subruiti	el‐subruiti	PROPN
eurjchem-440	178	7	,	,	PUNCT
eurjchem-440	178	8	g.	g.	PROPN
eurjchem-440	178	9	m.	m.	PROPN
eurjchem-440	178	10	alex	alex	PROPN
eurjchem-440	178	11	.	.	PUNCT
eurjchem-440	179	1	j.	j.	PROPN
eurjchem-440	179	2	pharm	pharm	PROPN
eurjchem-440	179	3	.	.	PUNCT
eurjchem-440	180	1	sci	sci	PROPN
eurjchem-440	180	2	.	.	PROPN
eurjchem-440	180	3	1992	1992	NUM
eurjchem-440	180	4	,	,	PUNCT
eurjchem-440	180	5	6(1	6(1	NUM
eurjchem-440	180	6	)	)	PUNCT
eurjchem-440	180	7	,	,	PUNCT
eurjchem-440	180	8	79‐82	79‐82	NOUN
eurjchem-440	180	9	.	.	PUNCT
eurjchem-440	181	1	[	[	X
eurjchem-440	181	2	2	2	NUM
eurjchem-440	181	3	]	]	PUNCT
eurjchem-440	181	4	.	.	PUNCT
eurjchem-440	182	1	shaban	shaban	PROPN
eurjchem-440	182	2	,	,	PUNCT
eurjchem-440	182	3	n.	n.	PROPN
eurjchem-440	182	4	z.	z.	PROPN
eurjchem-440	182	5	;	;	PUNCT
eurjchem-440	182	6	el‐subruiti	el‐subruiti	PROPN
eurjchem-440	182	7	,	,	PUNCT
eurjchem-440	182	8	g.	g.	PROPN
eurjchem-440	182	9	m.	m.	PROPN
eurjchem-440	182	10	j.	j.	PROPN
eurjchem-440	182	11	pest	pest	PROPN
eurjchem-440	182	12	.	.	PUNCT
eurjchem-440	183	1	control	control	NOUN
eurjchem-440	183	2	and	and	CCONJ
eurjchem-440	183	3	environ	environ	PROPN
eurjchem-440	183	4	.	.	PUNCT
eurjchem-440	184	1	sci	sci	PROPN
eurjchem-440	184	2	.	.	PROPN
eurjchem-440	184	3	1990	1990	NUM
eurjchem-440	184	4	,	,	PUNCT
eurjchem-440	184	5	2	2	NUM
eurjchem-440	184	6	,	,	PUNCT
eurjchem-440	184	7	91‐102	91‐102	NUM
eurjchem-440	184	8	.	.	PUNCT
eurjchem-440	185	1	[	[	X
eurjchem-440	185	2	3	3	NUM
eurjchem-440	185	3	]	]	PUNCT
eurjchem-440	185	4	.	.	PUNCT
eurjchem-440	186	1	belkov	belkov	PROPN
eurjchem-440	186	2	,	,	PUNCT
eurjchem-440	186	3	v.	v.	ADP
eurjchem-440	186	4	m.	m.	NOUN
eurjchem-440	186	5	;	;	PUNCT
eurjchem-440	186	6	krynetskaya	krynetskaya	PROPN
eurjchem-440	186	7	,	,	PUNCT
eurjchem-440	186	8	n.	n.	PROPN
eurjchem-440	186	9	f.	f.	PROPN
eurjchem-440	186	10	;	;	PUNCT
eurjchem-440	186	11	shabarova	shabarova	PROPN
eurjchem-440	186	12	,	,	PUNCT
eurjchem-440	186	13	z.	z.	PROPN
eurjchem-440	186	14	a.	a.	PROPN
eurjchem-440	186	15	;	;	PUNCT
eurjchem-440	186	16	novodarova	novodarova	PROPN
eurjchem-440	186	17	,	,	PUNCT
eurjchem-440	186	18	g.	g.	PROPN
eurjchem-440	186	19	n.	n.	PROPN
eurjchem-440	186	20	;	;	PUNCT
eurjchem-440	186	21	volpin	volpin	NOUN
eurjchem-440	186	22	,	,	PUNCT
eurjchem-440	186	23	m.	m.	PROPN
eurjchem-440	186	24	e.	e.	PROPN
eurjchem-440	186	25	russ	russ	PROPN
eurjchem-440	186	26	.	.	PROPN
eurjchem-440	187	1	chem	chem	PROPN
eurjchem-440	187	2	.	.	PUNCT
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eurjchem-440	188	2	,	,	PUNCT
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eurjchem-440	188	4	,	,	PUNCT
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eurjchem-440	188	6	)	)	PUNCT
eurjchem-440	188	7	,	,	PUNCT
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eurjchem-440	188	9	.	.	PUNCT
eurjchem-440	189	1	[	[	X
eurjchem-440	189	2	4	4	NUM
eurjchem-440	189	3	]	]	PUNCT
eurjchem-440	189	4	.	.	PUNCT
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eurjchem-440	190	2	,	,	PUNCT
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eurjchem-440	190	5	;	;	PUNCT
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eurjchem-440	190	9	k.	k.	PROPN
eurjchem-440	190	10	j.	j.	PROPN
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eurjchem-440	190	12	.	.	PUNCT
eurjchem-440	191	1	nucl	nucl	PROPN
eurjchem-440	191	2	.	.	PUNCT
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eurjchem-440	192	2	.	.	PUNCT
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eurjchem-440	193	2	,	,	PUNCT
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eurjchem-440	193	4	,	,	PUNCT
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eurjchem-440	193	6	.	.	PUNCT
eurjchem-440	194	1	[	[	X
eurjchem-440	194	2	5	5	NUM
eurjchem-440	194	3	]	]	PUNCT
eurjchem-440	194	4	.	.	PUNCT
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eurjchem-440	195	2	,	,	PUNCT
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eurjchem-440	195	5	;	;	PUNCT
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eurjchem-440	195	7	,	,	PUNCT
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eurjchem-440	195	9	k.	k.	PROPN
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eurjchem-440	195	13	.	.	PUNCT
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eurjchem-440	196	2	.	.	PUNCT
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eurjchem-440	197	2	,	,	PUNCT
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eurjchem-440	197	4	)	)	PUNCT
eurjchem-440	197	5	,	,	PUNCT
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eurjchem-440	197	7	.	.	PUNCT
eurjchem-440	198	1	[	[	X
eurjchem-440	198	2	6	6	NUM
eurjchem-440	198	3	]	]	PUNCT
eurjchem-440	198	4	.	.	PUNCT
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eurjchem-440	199	2	,	,	PUNCT
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eurjchem-440	199	5	;	;	PUNCT
eurjchem-440	199	6	phillips	phillips	PROPN
eurjchem-440	199	7	,	,	PUNCT
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eurjchem-440	199	9	k.	k.	PROPN
eurjchem-440	199	10	j.	j.	PROPN
eurjchem-440	199	11	chem	chem	PROPN
eurjchem-440	199	12	.	.	PUNCT
eurjchem-440	200	1	soc	soc	PROPN
eurjchem-440	200	2	.	.	PUNCT
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eurjchem-440	201	2	,	,	PUNCT
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eurjchem-440	201	4	.	.	PUNCT
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eurjchem-440	202	3	]	]	PUNCT
eurjchem-440	202	4	.	.	PUNCT
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eurjchem-440	203	2	,	,	PUNCT
eurjchem-440	203	3	m.	m.	PROPN
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eurjchem-440	203	5	;	;	PUNCT
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eurjchem-440	203	7	,	,	PUNCT
eurjchem-440	203	8	f.	f.	PROPN
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eurjchem-440	203	16	.	.	PUNCT
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eurjchem-440	204	2	.	.	PUNCT
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eurjchem-440	205	2	.	.	PUNCT
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eurjchem-440	206	3	,	,	PUNCT
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eurjchem-440	206	5	,	,	PUNCT
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eurjchem-440	206	7	.	.	PUNCT
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eurjchem-440	207	3	]	]	PUNCT
eurjchem-440	207	4	.	.	PUNCT
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eurjchem-440	208	2	,	,	PUNCT
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eurjchem-440	208	5	;	;	PUNCT
eurjchem-440	208	6	seleim	seleim	PROPN
eurjchem-440	208	7	,	,	PUNCT
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eurjchem-440	208	10	;	;	PUNCT
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eurjchem-440	208	12	,	,	PUNCT
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eurjchem-440	209	4	f.	f.	PROPN
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eurjchem-440	209	7	.	.	PUNCT
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eurjchem-440	210	2	.	.	PUNCT
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eurjchem-440	211	2	,	,	PUNCT
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eurjchem-440	211	4	,	,	PUNCT
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eurjchem-440	211	6	.	.	PUNCT
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eurjchem-440	212	3	]	]	PUNCT
eurjchem-440	212	4	.	.	PUNCT
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eurjchem-440	213	2	,	,	PUNCT
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eurjchem-440	213	4	;	;	PUNCT
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eurjchem-440	213	6	,	,	PUNCT
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eurjchem-440	213	9	;	;	PUNCT
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eurjchem-440	214	2	.	.	PUNCT
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eurjchem-440	215	3	.	.	PROPN
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eurjchem-440	215	5	,	,	PUNCT
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eurjchem-440	215	7	,	,	PUNCT
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eurjchem-440	215	9	.	.	PUNCT
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eurjchem-440	216	3	]	]	PUNCT
eurjchem-440	216	4	.	.	PUNCT
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eurjchem-440	217	2	,	,	PUNCT
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eurjchem-440	217	5	;	;	PUNCT
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eurjchem-440	217	7	,	,	PUNCT
eurjchem-440	217	8	f.	f.	PROPN
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eurjchem-440	217	10	;	;	PUNCT
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eurjchem-440	218	2	.	.	PUNCT
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eurjchem-440	219	2	,	,	PUNCT
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eurjchem-440	219	4	,	,	PUNCT
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eurjchem-440	219	6	.	.	PUNCT
eurjchem-440	220	1	[	[	X
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eurjchem-440	220	3	]	]	PUNCT
eurjchem-440	220	4	.	.	PUNCT
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eurjchem-440	221	2	,	,	PUNCT
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eurjchem-440	221	6	;	;	PUNCT
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eurjchem-440	221	12	.	.	PUNCT
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eurjchem-440	222	3	.	.	PUNCT
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eurjchem-440	223	2	,	,	PUNCT
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eurjchem-440	223	4	,	,	PUNCT
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eurjchem-440	223	6	.	.	PUNCT
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eurjchem-440	224	4	.	.	PUNCT
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eurjchem-440	225	2	,	,	PUNCT
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eurjchem-440	225	5	;	;	PUNCT
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eurjchem-440	225	7	,	,	PUNCT
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eurjchem-440	225	11	.	.	PUNCT
eurjchem-440	226	1	chem	chem	PROPN
eurjchem-440	226	2	.	.	PUNCT
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eurjchem-440	227	2	.	.	PUNCT
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eurjchem-440	228	2	,	,	PUNCT
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eurjchem-440	228	4	,	,	PUNCT
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eurjchem-440	228	6	.	.	PUNCT
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eurjchem-440	229	3	]	]	PUNCT
eurjchem-440	229	4	.	.	PUNCT
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eurjchem-440	229	6	,	,	PUNCT
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eurjchem-440	229	8	;	;	PUNCT
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eurjchem-440	229	10	,	,	PUNCT
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eurjchem-440	229	13	;	;	PUNCT
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eurjchem-440	229	15	,	,	PUNCT
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eurjchem-440	229	19	.	.	PUNCT
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eurjchem-440	230	2	.	.	PUNCT
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eurjchem-440	231	2	.	.	PUNCT
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eurjchem-440	232	2	,	,	PUNCT
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eurjchem-440	232	4	,	,	PUNCT
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eurjchem-440	232	7	.	.	PUNCT
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eurjchem-440	233	4	.	.	PUNCT
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eurjchem-440	234	2	,	,	PUNCT
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eurjchem-440	234	4	;	;	PUNCT
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eurjchem-440	234	6	,	,	PUNCT
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eurjchem-440	234	8	;	;	PUNCT
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eurjchem-440	234	10	,	,	PUNCT
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eurjchem-440	234	12	;	;	PUNCT
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eurjchem-440	234	21	.	.	PUNCT
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eurjchem-440	235	2	.	.	PUNCT
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eurjchem-440	236	2	.	.	PROPN
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eurjchem-440	236	4	,	,	PUNCT
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eurjchem-440	236	8	.	.	PUNCT
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eurjchem-440	237	4	.	.	PUNCT
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eurjchem-440	237	9	;	;	PUNCT
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eurjchem-440	238	2	.	.	PUNCT
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eurjchem-440	239	3	.	.	PROPN
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eurjchem-440	239	5	,	,	PUNCT
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eurjchem-440	239	7	,	,	PUNCT
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eurjchem-440	239	9	.	.	PUNCT
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eurjchem-440	240	3	]	]	PUNCT
eurjchem-440	240	4	.	.	PUNCT
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eurjchem-440	241	8	.	.	PUNCT
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eurjchem-440	242	2	,	,	PUNCT
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eurjchem-440	242	6	.	.	PUNCT
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eurjchem-440	243	4	.	.	PUNCT
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eurjchem-440	245	3	]	]	PUNCT
eurjchem-440	245	4	.	.	PUNCT
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eurjchem-440	246	8	.	.	PUNCT
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eurjchem-440	247	2	.	.	PUNCT
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eurjchem-440	248	2	,	,	PUNCT
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eurjchem-440	248	4	,	,	PUNCT
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eurjchem-440	248	6	.	.	PUNCT
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eurjchem-440	252	2	.	.	PUNCT
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eurjchem-440	253	2	,	,	PUNCT
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eurjchem-440	254	3	]	]	PUNCT
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eurjchem-440	255	7	,	,	PUNCT
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eurjchem-440	255	17	,	,	PUNCT
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eurjchem-440	255	21	.	.	PUNCT
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eurjchem-440	257	2	.	.	PUNCT
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eurjchem-440	258	2	,	,	PUNCT
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eurjchem-440	258	6	.	.	PUNCT
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eurjchem-440	259	3	]	]	PUNCT
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eurjchem-440	260	2	,	,	PUNCT
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eurjchem-440	260	7	,	,	PUNCT
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eurjchem-440	261	3	.	.	PUNCT
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eurjchem-440	262	2	,	,	PUNCT
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eurjchem-440	262	4	,	,	PUNCT
eurjchem-440	262	5	200‐	200‐	NUM
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eurjchem-440	262	7	.	.	PUNCT
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eurjchem-440	263	2	22	22	NUM
eurjchem-440	263	3	]	]	PUNCT
eurjchem-440	263	4	.	.	PUNCT
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eurjchem-440	263	6	,	,	PUNCT
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eurjchem-440	263	14	indian	indian	PROPN
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eurjchem-440	263	16	.	.	PUNCT
eurjchem-440	264	1	soc	soc	PROPN
eurjchem-440	264	2	.	.	PUNCT
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eurjchem-440	265	2	,	,	PUNCT
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eurjchem-440	265	4	,	,	PUNCT
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eurjchem-440	265	6	.	.	PUNCT
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eurjchem-440	266	3	]	]	PUNCT
eurjchem-440	266	4	.	.	PUNCT
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eurjchem-440	267	7	,	,	PUNCT
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eurjchem-440	268	2	.	.	PUNCT
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eurjchem-440	269	3	.	.	PROPN
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eurjchem-440	269	5	,	,	PUNCT
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eurjchem-440	269	7	,	,	PUNCT
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eurjchem-440	270	3	]	]	PUNCT
eurjchem-440	270	4	.	.	PUNCT
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eurjchem-440	271	2	,	,	PUNCT
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eurjchem-440	271	5	;	;	PUNCT
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eurjchem-440	271	7	,	,	PUNCT
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eurjchem-440	272	2	.	.	PUNCT
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eurjchem-440	273	3	.	.	PROPN
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eurjchem-440	273	5	,	,	PUNCT
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eurjchem-440	273	7	,	,	PUNCT
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eurjchem-440	275	2	,	,	PUNCT
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eurjchem-440	275	5	;	;	PUNCT
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eurjchem-440	275	7	,	,	PUNCT
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eurjchem-440	276	2	.	.	PUNCT
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eurjchem-440	277	3	.	.	PROPN
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eurjchem-440	277	5	,	,	PUNCT
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eurjchem-440	277	7	,	,	PUNCT
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eurjchem-440	277	12	.	.	PUNCT
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eurjchem-440	278	3	]	]	PUNCT
eurjchem-440	278	4	.	.	PUNCT
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eurjchem-440	278	9	;	;	PUNCT
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eurjchem-440	279	2	.	.	PUNCT
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eurjchem-440	280	3	.	.	PUNCT
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eurjchem-440	281	3	,	,	PUNCT
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eurjchem-440	282	4	.	.	PUNCT
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eurjchem-440	283	2	,	,	PUNCT
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eurjchem-440	283	5	;	;	PUNCT
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eurjchem-440	283	7	,	,	PUNCT
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eurjchem-440	284	3	.	.	PUNCT
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eurjchem-440	285	2	,	,	PUNCT
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eurjchem-440	285	4	,	,	PUNCT
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eurjchem-440	285	7	.	.	PUNCT
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eurjchem-440	286	4	.	.	PUNCT
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eurjchem-440	287	7	,	,	PUNCT
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eurjchem-440	289	2	.	.	PROPN
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eurjchem-440	289	4	,	,	PUNCT
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eurjchem-440	292	2	.	.	PUNCT
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eurjchem-440	293	2	,	,	PUNCT
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eurjchem-440	295	2	.	.	PUNCT
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eurjchem-440	296	3	.	.	PROPN
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eurjchem-440	296	5	,	,	PUNCT
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eurjchem-440	299	2	,	,	PUNCT
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eurjchem-440	299	5	,	,	PUNCT
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eurjchem-440	299	7	.	.	PUNCT
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eurjchem-440	300	4	.	.	PUNCT
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eurjchem-440	301	5	;	;	PUNCT
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eurjchem-440	305	6	,	,	PUNCT
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eurjchem-440	307	2	.	.	PUNCT
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eurjchem-440	308	2	.	.	PROPN
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eurjchem-440	308	4	,	,	PUNCT
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eurjchem-440	309	3	]	]	SYM
eurjchem-440	309	4	.	.	PUNCT
eurjchem-440	309	5	fathalla	fathalla	PROPN
eurjchem-440	309	6	,	,	PUNCT
eurjchem-440	309	7	m.	m.	NOUN
eurjchem-440	309	8	f.	f.	PROPN
eurjchem-440	309	9	;	;	PUNCT
eurjchem-440	309	10	el‐subruiti	el‐subruiti	PROPN
eurjchem-440	309	11	,	,	PUNCT
eurjchem-440	309	12	g.	g.	PROPN
eurjchem-440	309	13	m.	m.	NOUN
eurjchem-440	309	14	;	;	PUNCT
eurjchem-440	309	15	el‐marasi	el‐marasi	PROPN
eurjchem-440	309	16	y.	y.	PROPN
eurjchem-440	309	17	r.	r.	PROPN
eurjchem-440	309	18	prog	prog	PROPN
eurjchem-440	309	19	.	.	PUNCT
eurjchem-440	310	1	react	react	VERB
eurjchem-440	310	2	.	.	PUNCT
eurjchem-440	311	1	kinet	kinet	PROPN
eurjchem-440	311	2	.	.	PUNCT
eurjchem-440	312	1	mec	mec	PROPN
eurjchem-440	312	2	.	.	PROPN
eurjchem-440	312	3	2009	2009	NUM
eurjchem-440	312	4	,	,	PUNCT
eurjchem-440	312	5	14	14	NUM
eurjchem-440	312	6	,	,	PUNCT
eurjchem-440	312	7	169‐183	169‐183	NUM
eurjchem-440	312	8	.	.	PUNCT