id	sid	tid	token	lemma	pos
eurjchem-448	1	1	untitled	untitle	VERB
eurjchem-448	1	2	european	european	PROPN
eurjchem-448	1	3	journal	journal	PROPN
eurjchem-448	1	4	of	of	ADP
eurjchem-448	1	5	chemistry	chemistry	NOUN
eurjchem-448	1	6	3	3	NUM
eurjchem-448	1	7	(	(	PUNCT
eurjchem-448	1	8	1	1	NUM
eurjchem-448	1	9	)	)	PUNCT
eurjchem-448	1	10	(	(	PUNCT
eurjchem-448	1	11	2012	2012	NUM
eurjchem-448	1	12	)	)	PUNCT
eurjchem-448	1	13	57‐64	57‐64	NUM
eurjchem-448	1	14	european	european	PROPN
eurjchem-448	1	15	journal	journal	PROPN
eurjchem-448	1	16	of	of	ADP
eurjchem-448	1	17	chemistry	chemistry	NOUN
eurjchem-448	1	18	issn	issn	PROPN
eurjchem-448	1	19	2153‐2249	2153‐2249	PROPN
eurjchem-448	1	20	(	(	PUNCT
eurjchem-448	1	21	print	print	NOUN
eurjchem-448	1	22	)	)	PUNCT
eurjchem-448	1	23	/	/	SYM
eurjchem-448	1	24	issn	issn	PROPN
eurjchem-448	1	25	2153‐2257	2153‐2257	NUM
eurjchem-448	1	26	(	(	PUNCT
eurjchem-448	1	27	online	online	ADJ
eurjchem-448	1	28	)	)	PUNCT
eurjchem-448	1	29			NOUN
eurjchem-448	1	30	2012	2012	NUM
eurjchem-448	1	31	eurjchem	eurjchem	PROPN
eurjchem-448	1	32	doi:10.5155	doi:10.5155	PROPN
eurjchem-448	1	33	/	/	SYM
eurjchem-448	1	34	eurjchem.3.1.57‐64.448	eurjchem.3.1.57‐64.448	PROPN
eurjchem-448	1	35	european	european	ADJ
eurjchem-448	1	36	journal	journal	PROPN
eurjchem-448	1	37	of	of	ADP
eurjchem-448	1	38	chemistry	chemistry	PROPN
eurjchem-448	1	39	journal	journal	PROPN
eurjchem-448	1	40	homepage	homepage	NOUN
eurjchem-448	1	41	:	:	PUNCT
eurjchem-448	2	1	www.eurjchem.com	www.eurjchem.com	X
eurjchem-448	2	2	synthesis	synthesis	NOUN
eurjchem-448	2	3	,	,	PUNCT
eurjchem-448	2	4	structural	structural	ADJ
eurjchem-448	2	5	elucidation	elucidation	NOUN
eurjchem-448	2	6	and	and	CCONJ
eurjchem-448	2	7	antimicrobial	antimicrobial	ADJ
eurjchem-448	2	8	effectiveness	effectiveness	NOUN
eurjchem-448	2	9	of	of	ADP
eurjchem-448	2	10	coordination	coordination	NOUN
eurjchem-448	2	11	entities	entity	NOUN
eurjchem-448	2	12	of	of	ADP
eurjchem-448	2	13	cobalt	cobalt	NOUN
eurjchem-448	2	14	(	(	PUNCT
eurjchem-448	2	15	ii	ii	NOUN
eurjchem-448	2	16	)	)	PUNCT
eurjchem-448	2	17	and	and	CCONJ
eurjchem-448	2	18	nickel	nickel	NOUN
eurjchem-448	2	19	(	(	PUNCT
eurjchem-448	2	20	ii	ii	NOUN
eurjchem-448	2	21	)	)	PUNCT
eurjchem-448	2	22	derived	derive	VERB
eurjchem-448	2	23	from	from	ADP
eurjchem-448	2	24	9,17‐diaza‐2,6,11,15‐	9,17‐diaza‐2,6,11,15‐	NUM
eurjchem-448	2	25	tetrathia‐1,7,10,16‐(1,2)‐tetrabenzenacyclooctadecaphan‐8,17‐diene	tetrathia‐1,7,10,16‐(1,2)‐tetrabenzenacyclooctadecaphan‐8,17‐diene	NOUN
eurjchem-448	2	26	rajiv	rajiv	PROPN
eurjchem-448	2	27	kumara	kumara	NOUN
eurjchem-448	2	28	,	,	PUNCT
eurjchem-448	2	29	*	*	PUNCT
eurjchem-448	2	30	,	,	PUNCT
eurjchem-448	2	31	rajni	rajni	NOUN
eurjchem-448	2	32	joharb	joharb	NOUN
eurjchem-448	2	33	and	and	CCONJ
eurjchem-448	2	34	anil	anil	PROPN
eurjchem-448	2	35	krishan	krishan	PROPN
eurjchem-448	2	36	aggarwala	aggarwala	ADP
eurjchem-448	2	37	a	a	DET
eurjchem-448	2	38	department	department	NOUN
eurjchem-448	2	39	of	of	ADP
eurjchem-448	2	40	chemistry	chemistry	NOUN
eurjchem-448	2	41	,	,	PUNCT
eurjchem-448	2	42	shivaji	shivaji	PROPN
eurjchem-448	2	43	college	college	PROPN
eurjchem-448	2	44	university	university	PROPN
eurjchem-448	2	45	of	of	ADP
eurjchem-448	2	46	delhi	delhi	PROPN
eurjchem-448	2	47	,	,	PUNCT
eurjchem-448	2	48	new	new	ADJ
eurjchem-448	2	49	delhi	delhi	PROPN
eurjchem-448	2	50	,	,	PUNCT
eurjchem-448	2	51	110027	110027	NUM
eurjchem-448	2	52	,	,	PUNCT
eurjchem-448	2	53	india	india	PROPN
eurjchem-448	2	54	b	b	PROPN
eurjchem-448	2	55	department	department	PROPN
eurjchem-448	2	56	of	of	ADP
eurjchem-448	2	57	chemistry	chemistry	NOUN
eurjchem-448	2	58	,	,	PUNCT
eurjchem-448	2	59	guru	guru	NOUN
eurjchem-448	2	60	govind	govind	PROPN
eurjchem-448	2	61	singh	singh	PROPN
eurjchem-448	2	62	indraprashtha	indraprashtha	PROPN
eurjchem-448	2	63	university	university	PROPN
eurjchem-448	2	64	,	,	PUNCT
eurjchem-448	2	65	new	new	ADJ
eurjchem-448	2	66	delhi	delhi	PROPN
eurjchem-448	2	67	,	,	PUNCT
eurjchem-448	2	68	110002	110002	NUM
eurjchem-448	2	69	,	,	PUNCT
eurjchem-448	2	70	india	india	PROPN
eurjchem-448	2	71	*	*	PUNCT
eurjchem-448	2	72	corresponding	correspond	VERB
eurjchem-448	2	73	author	author	NOUN
eurjchem-448	2	74	at	at	ADP
eurjchem-448	2	75	:	:	PUNCT
eurjchem-448	2	76	department	department	NOUN
eurjchem-448	2	77	of	of	ADP
eurjchem-448	2	78	chemistry	chemistry	PROPN
eurjchem-448	2	79	,	,	PUNCT
eurjchem-448	2	80	shivaji	shivaji	PROPN
eurjchem-448	2	81	college	college	PROPN
eurjchem-448	2	82	university	university	PROPN
eurjchem-448	2	83	of	of	ADP
eurjchem-448	2	84	delhi	delhi	PROPN
eurjchem-448	2	85	,	,	PUNCT
eurjchem-448	2	86	new	new	ADJ
eurjchem-448	2	87	delhi	delhi	PROPN
eurjchem-448	2	88	,	,	PUNCT
eurjchem-448	2	89	110027	110027	NUM
eurjchem-448	2	90	,	,	PUNCT
eurjchem-448	2	91	india	india	PROPN
eurjchem-448	2	92	.	.	PUNCT
eurjchem-448	3	1	tel	tel	PROPN
eurjchem-448	3	2	.	.	PUNCT
eurjchem-448	3	3	:	:	PUNCT
eurjchem-448	4	1	+91.98.10742944	+91.98.10742944	NUM
eurjchem-448	4	2	;	;	PUNCT
eurjchem-448	4	3	fax	fax	NOUN
eurjchem-448	4	4	:	:	PUNCT
eurjchem-448	4	5	+91.11.25155551	+91.11.25155551	NUM
eurjchem-448	4	6	.	.	PUNCT
eurjchem-448	4	7	e‐mail	e‐mail	PUNCT
eurjchem-448	5	1	address	address	NOUN
eurjchem-448	5	2	:	:	PUNCT
eurjchem-448	5	3	chemistry_rajiv@hotmail.com	chemistry_rajiv@hotmail.com	X
eurjchem-448	5	4	(	(	PUNCT
eurjchem-448	5	5	r.	r.	PROPN
eurjchem-448	5	6	kumar	kumar	PROPN
eurjchem-448	5	7	)	)	PUNCT
eurjchem-448	5	8	.	.	PUNCT
eurjchem-448	6	1	article	article	NOUN
eurjchem-448	6	2	information	information	PROPN
eurjchem-448	6	3	abstract	abstract	ADV
eurjchem-448	6	4	received	receive	VERB
eurjchem-448	6	5	:	:	PUNCT
eurjchem-448	6	6	24	24	NUM
eurjchem-448	6	7	april	april	PROPN
eurjchem-448	6	8	2011	2011	NUM
eurjchem-448	6	9	received	receive	VERB
eurjchem-448	6	10	in	in	ADP
eurjchem-448	6	11	revised	revise	VERB
eurjchem-448	6	12	form	form	NOUN
eurjchem-448	6	13	:	:	PUNCT
eurjchem-448	6	14	01	01	NUM
eurjchem-448	6	15	june	june	PROPN
eurjchem-448	6	16	2011	2011	NUM
eurjchem-448	6	17	accepted	accept	VERB
eurjchem-448	6	18	:	:	PUNCT
eurjchem-448	6	19	17	17	NUM
eurjchem-448	6	20	june	june	PROPN
eurjchem-448	6	21	2011	2011	NUM
eurjchem-448	6	22	online	online	ADV
eurjchem-448	6	23	:	:	PUNCT
eurjchem-448	6	24	31	31	NUM
eurjchem-448	6	25	march	march	NOUN
eurjchem-448	6	26	2012	2012	NUM
eurjchem-448	6	27	keywords	keyword	NOUN
eurjchem-448	6	28	9,17‐diaza‐2,6,11,15‐tetrathia‐1,7,10,16‐(1,2)‐tetrabenzenacyclooctadecaphan‐8,17‐diene	9,17‐diaza‐2,6,11,15‐tetrathia‐1,7,10,16‐(1,2)‐tetrabenzenacyclooctadecaphan‐8,17‐diene	NUM
eurjchem-448	6	29	,	,	PUNCT
eurjchem-448	6	30	macrocycle	macrocycle	NOUN
eurjchem-448	6	31	was	be	AUX
eurjchem-448	6	32	synthesized	synthesize	VERB
eurjchem-448	6	33	,	,	PUNCT
eurjchem-448	6	34	thereafter	thereafter	ADV
eurjchem-448	6	35	formulation	formulation	NOUN
eurjchem-448	6	36	and	and	CCONJ
eurjchem-448	6	37	designing	designing	NOUN
eurjchem-448	6	38	strategies	strategy	NOUN
eurjchem-448	6	39	applied	apply	VERB
eurjchem-448	6	40	for	for	ADP
eurjchem-448	6	41	the	the	DET
eurjchem-448	6	42	preparation	preparation	NOUN
eurjchem-448	6	43	of	of	ADP
eurjchem-448	6	44	coordination	coordination	NOUN
eurjchem-448	6	45	entities	entity	NOUN
eurjchem-448	6	46	of	of	ADP
eurjchem-448	6	47	co(ii	co(ii	ADJ
eurjchem-448	6	48	)	)	PUNCT
eurjchem-448	6	49	and	and	CCONJ
eurjchem-448	6	50	ni(ii	ni(ii	NOUN
eurjchem-448	6	51	)	)	PUNCT
eurjchem-448	6	52	.	.	PUNCT
eurjchem-448	7	1	coordination	coordination	NOUN
eurjchem-448	7	2	behaviour	behaviour	NOUN
eurjchem-448	7	3	of	of	ADP
eurjchem-448	7	4	n2s4	n2s4	PRON
eurjchem-448	7	5	donor	donor	NOUN
eurjchem-448	7	6	macrocycle	macrocycle	NOUN
eurjchem-448	7	7	towards	towards	ADP
eurjchem-448	7	8	metal	metal	PROPN
eurjchem-448	7	9	ion(s	ion(s	PROPN
eurjchem-448	7	10	)	)	PUNCT
eurjchem-448	7	11	was	be	AUX
eurjchem-448	7	12	assessed	assess	VERB
eurjchem-448	7	13	by	by	ADP
eurjchem-448	7	14	physiochemical	physiochemical	ADJ
eurjchem-448	7	15	measurements	measurement	NOUN
eurjchem-448	7	16	and	and	CCONJ
eurjchem-448	7	17	spectral	spectral	ADJ
eurjchem-448	7	18	investigations	investigation	NOUN
eurjchem-448	7	19	viz	viz	NOUN
eurjchem-448	7	20	.	.	PUNCT
eurjchem-448	8	1	elemental	elemental	ADJ
eurjchem-448	8	2	analysis	analysis	NOUN
eurjchem-448	8	3	,	,	PUNCT
eurjchem-448	8	4	molar	molar	ADJ
eurjchem-448	8	5	conductance	conductance	NOUN
eurjchem-448	8	6	,	,	PUNCT
eurjchem-448	8	7	magnetic	magnetic	ADJ
eurjchem-448	8	8	susceptibility	susceptibility	NOUN
eurjchem-448	8	9	measurements	measurement	NOUN
eurjchem-448	8	10	,	,	PUNCT
eurjchem-448	8	11	infrared	infrare	VERB
eurjchem-448	8	12	,	,	PUNCT
eurjchem-448	8	13	uv‐vis	uv‐vis	PROPN
eurjchem-448	8	14	,	,	PUNCT
eurjchem-448	8	15	1h	1h	NUM
eurjchem-448	8	16	and	and	CCONJ
eurjchem-448	8	17	13	13	NUM
eurjchem-448	8	18	c	c	PROPN
eurjchem-448	8	19	nmr	nmr	NOUN
eurjchem-448	8	20	,	,	PUNCT
eurjchem-448	8	21	mass	mass	NOUN
eurjchem-448	8	22	spectroscopy	spectroscopy	NOUN
eurjchem-448	8	23	,	,	PUNCT
eurjchem-448	8	24	electron	electron	NOUN
eurjchem-448	8	25	paramagnetic	paramagnetic	ADJ
eurjchem-448	8	26	resonance	resonance	NOUN
eurjchem-448	8	27	(	(	PUNCT
eurjchem-448	8	28	epr	epr	PROPN
eurjchem-448	8	29	)	)	PUNCT
eurjchem-448	8	30	,	,	PUNCT
eurjchem-448	8	31	cyclic	cyclic	ADJ
eurjchem-448	8	32	voltammetry	voltammetry	NOUN
eurjchem-448	8	33	and	and	CCONJ
eurjchem-448	8	34	molecular	molecular	ADJ
eurjchem-448	8	35	modeling	modeling	NOUN
eurjchem-448	8	36	.	.	PUNCT
eurjchem-448	9	1	side‐by‐side	side‐by‐side	ADV
eurjchem-448	9	2	comparison	comparison	NOUN
eurjchem-448	9	3	of	of	ADP
eurjchem-448	9	4	the	the	DET
eurjchem-448	9	5	spectral	spectral	ADJ
eurjchem-448	9	6	findings	finding	NOUN
eurjchem-448	9	7	exposed	expose	VERB
eurjchem-448	9	8	different	different	ADJ
eurjchem-448	9	9	geometrical	geometrical	ADJ
eurjchem-448	9	10	aspects	aspect	NOUN
eurjchem-448	9	11	of	of	ADP
eurjchem-448	9	12	macrocycle	macrocycle	NOUN
eurjchem-448	9	13	and	and	CCONJ
eurjchem-448	9	14	coordination	coordination	NOUN
eurjchem-448	9	15	entities	entity	NOUN
eurjchem-448	9	16	.	.	PUNCT
eurjchem-448	10	1	cyclic	cyclic	ADJ
eurjchem-448	10	2	voltammogram	voltammogram	NOUN
eurjchem-448	10	3	showed	show	VERB
eurjchem-448	10	4	fully	fully	ADV
eurjchem-448	10	5	oxidized	oxidize	VERB
eurjchem-448	10	6	and	and	CCONJ
eurjchem-448	10	7	reduced	reduce	VERB
eurjchem-448	10	8	species	specie	NOUN
eurjchem-448	10	9	in	in	ADP
eurjchem-448	10	10	one	one	NUM
eurjchem-448	10	11	unified	unified	ADJ
eurjchem-448	10	12	experiment	experiment	NOUN
eurjchem-448	10	13	.	.	PUNCT
eurjchem-448	11	1	macrocycle	macrocycle	NOUN
eurjchem-448	11	2	and	and	CCONJ
eurjchem-448	11	3	coordination	coordination	NOUN
eurjchem-448	11	4	entities	entity	NOUN
eurjchem-448	11	5	were	be	AUX
eurjchem-448	11	6	screened	screen	VERB
eurjchem-448	11	7	for	for	ADP
eurjchem-448	11	8	antimicrobial	antimicrobial	ADJ
eurjchem-448	11	9	effectiveness	effectiveness	NOUN
eurjchem-448	11	10	(	(	PUNCT
eurjchem-448	11	11	antifungal	antifungal	ADJ
eurjchem-448	11	12	properties	property	NOUN
eurjchem-448	11	13	against	against	ADP
eurjchem-448	11	14	aspergillus‐niger	aspergillus‐niger	PROPN
eurjchem-448	11	15	)	)	PUNCT
eurjchem-448	11	16	.	.	PUNCT
eurjchem-448	12	1	epr	epr	PROPN
eurjchem-448	12	2	antimicrobial	antimicrobial	ADJ
eurjchem-448	12	3	molecular	molecular	ADJ
eurjchem-448	12	4	modeling	model	VERB
eurjchem-448	12	5	potential	potential	ADJ
eurjchem-448	12	6	separation	separation	NOUN
eurjchem-448	12	7	splitting	split	VERB
eurjchem-448	12	8	parameters	parameter	NOUN
eurjchem-448	12	9	coordination	coordination	NOUN
eurjchem-448	12	10	entities	entity	NOUN
eurjchem-448	12	11	1	1	NUM
eurjchem-448	12	12	.	.	PUNCT
eurjchem-448	13	1	introduction	introduction	NOUN
eurjchem-448	13	2	the	the	DET
eurjchem-448	13	3	ligand	ligand	NOUN
eurjchem-448	13	4	binds	bind	VERB
eurjchem-448	13	5	metal	metal	PROPN
eurjchem-448	13	6	ion(s	ion(s	PROPN
eurjchem-448	13	7	)	)	PUNCT
eurjchem-448	13	8	to	to	PART
eurjchem-448	13	9	form	form	VERB
eurjchem-448	13	10	mixed	mixed	ADJ
eurjchem-448	13	11	multi‐	multi‐	PROPN
eurjchem-448	13	12	functional	functional	ADJ
eurjchem-448	13	13	materials	material	NOUN
eurjchem-448	13	14	capable	capable	ADJ
eurjchem-448	13	15	of	of	ADP
eurjchem-448	13	16	furnishing	furnish	VERB
eurjchem-448	13	17	ligand	ligand	ADJ
eurjchem-448	13	18	field	field	NOUN
eurjchem-448	13	19	strength	strength	NOUN
eurjchem-448	13	20	around	around	ADP
eurjchem-448	13	21	metal	metal	NOUN
eurjchem-448	13	22	ion(s	ion(s	PROPN
eurjchem-448	13	23	)	)	PUNCT
eurjchem-448	13	24	to	to	PART
eurjchem-448	13	25	develop	develop	VERB
eurjchem-448	13	26	molecular	molecular	ADJ
eurjchem-448	13	27	recognitions	recognition	NOUN
eurjchem-448	13	28	.	.	PUNCT
eurjchem-448	14	1	ligand	ligand	PROPN
eurjchem-448	14	2	works	work	VERB
eurjchem-448	14	3	as	as	ADP
eurjchem-448	14	4	a	a	DET
eurjchem-448	14	5	system	system	NOUN
eurjchem-448	14	6	limit	limit	VERB
eurjchem-448	14	7	adverse	adverse	ADJ
eurjchem-448	14	8	effects	effect	NOUN
eurjchem-448	14	9	of	of	ADP
eurjchem-448	14	10	metal	metal	NOUN
eurjchem-448	14	11	ion(s	ion(s	PROPN
eurjchem-448	14	12	)	)	PUNCT
eurjchem-448	14	13	overload	overload	NOUN
eurjchem-448	14	14	,	,	PUNCT
eurjchem-448	14	15	inhibit	inhibit	VERB
eurjchem-448	14	16	selected	select	VERB
eurjchem-448	14	17	metalloenzymes	metalloenzyme	NOUN
eurjchem-448	14	18	activity	activity	NOUN
eurjchem-448	14	19	,	,	PUNCT
eurjchem-448	14	20	facilitate	facilitate	NOUN
eurjchem-448	14	21	metal	metal	NOUN
eurjchem-448	14	22	ion(s	ion(s	PROPN
eurjchem-448	14	23	)	)	PUNCT
eurjchem-448	14	24	re‐distribution	re‐distribution	NOUN
eurjchem-448	14	25	,	,	PUNCT
eurjchem-448	14	26	detect	detect	VERB
eurjchem-448	14	27	and	and	CCONJ
eurjchem-448	14	28	detoxify	detoxify	VERB
eurjchem-448	14	29	toxic	toxic	ADJ
eurjchem-448	14	30	metals	metal	NOUN
eurjchem-448	14	31	.	.	PUNCT
eurjchem-448	15	1	their	their	PRON
eurjchem-448	15	2	synthetic	synthetic	ADJ
eurjchem-448	15	3	protocols	protocol	NOUN
eurjchem-448	15	4	depend	depend	VERB
eurjchem-448	15	5	significantly	significantly	ADV
eurjchem-448	15	6	on	on	ADP
eurjchem-448	15	7	the	the	DET
eurjchem-448	15	8	dimensions	dimension	NOUN
eurjchem-448	15	9	of	of	ADP
eurjchem-448	15	10	their	their	PRON
eurjchem-448	15	11	internal	internal	ADJ
eurjchem-448	15	12	cavity	cavity	NOUN
eurjchem-448	15	13	,	,	PUNCT
eurjchem-448	15	14	rigidity	rigidity	NOUN
eurjchem-448	15	15	of	of	ADP
eurjchem-448	15	16	ligand	ligand	NOUN
eurjchem-448	15	17	,	,	PUNCT
eurjchem-448	15	18	nature	nature	NOUN
eurjchem-448	15	19	of	of	ADP
eurjchem-448	15	20	donor	donor	NOUN
eurjchem-448	15	21	atoms	atom	NOUN
eurjchem-448	15	22	and	and	CCONJ
eurjchem-448	15	23	as	as	ADP
eurjchem-448	15	24	a	a	DET
eurjchem-448	15	25	whole	whole	NOUN
eurjchem-448	15	26	the	the	DET
eurjchem-448	15	27	great	great	ADJ
eurjchem-448	15	28	availability	availability	NOUN
eurjchem-448	15	29	as	as	ADP
eurjchem-448	15	30	ligand	ligand	NOUN
eurjchem-448	15	31	with	with	ADP
eurjchem-448	15	32	coordinating	coordinate	VERB
eurjchem-448	15	33	abilities	ability	NOUN
eurjchem-448	15	34	of	of	ADP
eurjchem-448	15	35	anion(s	anion(s	NOUN
eurjchem-448	15	36	)	)	PUNCT
eurjchem-448	15	37	involved	involve	VERB
eurjchem-448	15	38	[	[	PUNCT
eurjchem-448	15	39	1,2	1,2	NUM
eurjchem-448	15	40	]	]	PUNCT
eurjchem-448	15	41	.	.	PUNCT
eurjchem-448	16	1	macrocycle	macrocycle	PROPN
eurjchem-448	16	2	(	(	PUNCT
eurjchem-448	16	3	mc	mc	PROPN
eurjchem-448	16	4	)	)	PUNCT
eurjchem-448	16	5	and	and	CCONJ
eurjchem-448	16	6	its	its	PRON
eurjchem-448	16	7	derivatives	derivative	NOUN
eurjchem-448	16	8	act	act	VERB
eurjchem-448	16	9	as	as	ADP
eurjchem-448	16	10	donor	donor	NOUN
eurjchem-448	16	11	centre	centre	NOUN
eurjchem-448	16	12	capable	capable	ADJ
eurjchem-448	16	13	of	of	ADP
eurjchem-448	16	14	performing	perform	VERB
eurjchem-448	16	15	various	various	ADJ
eurjchem-448	16	16	specific	specific	ADJ
eurjchem-448	16	17	molecular	molecular	ADJ
eurjchem-448	16	18	activities	activity	NOUN
eurjchem-448	16	19	with	with	ADP
eurjchem-448	16	20	perfect	perfect	ADJ
eurjchem-448	16	21	use	use	NOUN
eurjchem-448	16	22	to	to	PART
eurjchem-448	16	23	design	design	VERB
eurjchem-448	16	24	and	and	CCONJ
eurjchem-448	16	25	develop	develop	VERB
eurjchem-448	16	26	magnetic	magnetic	ADJ
eurjchem-448	16	27	resonance	resonance	NOUN
eurjchem-448	16	28	imaging	imaging	NOUN
eurjchem-448	16	29	(	(	PUNCT
eurjchem-448	16	30	mri	mri	NOUN
eurjchem-448	16	31	)	)	PUNCT
eurjchem-448	16	32	contrasting	contrast	VERB
eurjchem-448	16	33	agents	agent	NOUN
eurjchem-448	16	34	,	,	PUNCT
eurjchem-448	16	35	radiopharmaceuticals	radiopharmaceutical	NOUN
eurjchem-448	16	36	and	and	CCONJ
eurjchem-448	16	37	chemotherapeutics	chemotherapeutic	NOUN
eurjchem-448	16	38	[	[	X
eurjchem-448	16	39	3,4	3,4	NUM
eurjchem-448	16	40	]	]	PUNCT
eurjchem-448	16	41	.	.	PUNCT
eurjchem-448	17	1	further	far	ADV
eurjchem-448	17	2	,	,	PUNCT
eurjchem-448	17	3	computational	computational	ADJ
eurjchem-448	17	4	calculations	calculation	NOUN
eurjchem-448	17	5	offer	offer	VERB
eurjchem-448	17	6	a	a	DET
eurjchem-448	17	7	deep	deep	ADJ
eurjchem-448	17	8	appreciation	appreciation	NOUN
eurjchem-448	17	9	in	in	ADP
eurjchem-448	17	10	theoretical	theoretical	ADJ
eurjchem-448	17	11	interest	interest	NOUN
eurjchem-448	17	12	and	and	CCONJ
eurjchem-448	17	13	evaluation	evaluation	NOUN
eurjchem-448	17	14	of	of	ADP
eurjchem-448	17	15	practical	practical	ADJ
eurjchem-448	17	16	findings	finding	NOUN
eurjchem-448	17	17	to	to	PART
eurjchem-448	17	18	determine	determine	VERB
eurjchem-448	17	19	their	their	PRON
eurjchem-448	17	20	great	great	ADJ
eurjchem-448	17	21	availability	availability	NOUN
eurjchem-448	17	22	and	and	CCONJ
eurjchem-448	17	23	flexibility	flexibility	NOUN
eurjchem-448	17	24	as	as	ADP
eurjchem-448	17	25	ligand	ligand	ADJ
eurjchem-448	17	26	.	.	PUNCT
eurjchem-448	18	1	biotransformational	biotransformational	ADJ
eurjchem-448	18	2	enzymes	enzyme	NOUN
eurjchem-448	18	3	and	and	CCONJ
eurjchem-448	18	4	their	their	PRON
eurjchem-448	18	5	cofactors	cofactor	NOUN
eurjchem-448	18	6	can	can	AUX
eurjchem-448	18	7	be	be	AUX
eurjchem-448	18	8	explored	explore	VERB
eurjchem-448	18	9	with	with	ADP
eurjchem-448	18	10	the	the	DET
eurjchem-448	18	11	help	help	NOUN
eurjchem-448	18	12	of	of	ADP
eurjchem-448	18	13	such	such	ADJ
eurjchem-448	18	14	hypothetical	hypothetical	ADJ
eurjchem-448	18	15	calculations	calculation	NOUN
eurjchem-448	18	16	to	to	PART
eurjchem-448	18	17	design	design	VERB
eurjchem-448	18	18	good	good	ADJ
eurjchem-448	18	19	models	model	NOUN
eurjchem-448	18	20	[	[	X
eurjchem-448	18	21	5	5	NUM
eurjchem-448	18	22	]	]	PUNCT
eurjchem-448	18	23	.	.	PUNCT
eurjchem-448	19	1	herein	herein	PROPN
eurjchem-448	19	2	,	,	PUNCT
eurjchem-448	19	3	n2s4	n2s4	ADJ
eurjchem-448	19	4	donor	donor	NOUN
eurjchem-448	19	5	coordination	coordination	NOUN
eurjchem-448	19	6	entities	entity	NOUN
eurjchem-448	19	7	of	of	ADP
eurjchem-448	19	8	co(ii	co(ii	ADJ
eurjchem-448	19	9	)	)	PUNCT
eurjchem-448	19	10	and	and	CCONJ
eurjchem-448	19	11	ni(ii	ni(ii	PROPN
eurjchem-448	19	12	)	)	PUNCT
eurjchem-448	19	13	were	be	AUX
eurjchem-448	19	14	derived	derive	VERB
eurjchem-448	19	15	from	from	ADP
eurjchem-448	19	16	macrocycle	macrocycle	NOUN
eurjchem-448	19	17	i.e.	i.e.	X
eurjchem-448	19	18	9,17‐diaza‐2,6,11,15‐tetrathia‐1,7,10,16‐(1,2)‐tetrabenzen	9,17‐diaza‐2,6,11,15‐tetrathia‐1,7,10,16‐(1,2)‐tetrabenzen	NUM
eurjchem-448	19	19	acyclooctadecaphan‐8,17‐diene	acyclooctadecaphan‐8,17‐diene	NOUN
eurjchem-448	19	20	.	.	PUNCT
eurjchem-448	20	1	an	an	DET
eurjchem-448	20	2	explanatory	explanatory	ADJ
eurjchem-448	20	3	note	note	NOUN
eurjchem-448	20	4	is	be	AUX
eurjchem-448	20	5	presented	present	VERB
eurjchem-448	20	6	having	have	VERB
eurjchem-448	20	7	spectral	spectral	ADJ
eurjchem-448	20	8	findings	finding	NOUN
eurjchem-448	20	9	on	on	ADP
eurjchem-448	20	10	selection	selection	NOUN
eurjchem-448	20	11	and	and	CCONJ
eurjchem-448	20	12	coordination	coordination	NOUN
eurjchem-448	20	13	potential	potential	NOUN
eurjchem-448	20	14	of	of	ADP
eurjchem-448	20	15	donor	donor	NOUN
eurjchem-448	20	16	atoms	atom	NOUN
eurjchem-448	20	17	of	of	ADP
eurjchem-448	20	18	macrocycle	macrocycle	NOUN
eurjchem-448	20	19	with	with	ADP
eurjchem-448	20	20	metal(s	metal(s	PROPN
eurjchem-448	20	21	)	)	PUNCT
eurjchem-448	20	22	.	.	PUNCT
eurjchem-448	21	1	molecular	molecular	ADJ
eurjchem-448	21	2	models	model	NOUN
eurjchem-448	21	3	for	for	ADP
eurjchem-448	21	4	coordination	coordination	NOUN
eurjchem-448	21	5	entities	entity	NOUN
eurjchem-448	21	6	(	(	PUNCT
eurjchem-448	21	7	ces	ce	NOUN
eurjchem-448	21	8	)	)	PUNCT
eurjchem-448	21	9	were	be	AUX
eurjchem-448	21	10	obtained	obtain	VERB
eurjchem-448	21	11	to	to	PART
eurjchem-448	21	12	get	get	VERB
eurjchem-448	21	13	minimum	minimum	ADJ
eurjchem-448	21	14	energy	energy	NOUN
eurjchem-448	21	15	through	through	ADP
eurjchem-448	21	16	computational	computational	ADJ
eurjchem-448	21	17	calculation	calculation	NOUN
eurjchem-448	21	18	.	.	PUNCT
eurjchem-448	22	1	inhibiting	inhibit	VERB
eurjchem-448	22	2	potential	potential	NOUN
eurjchem-448	22	3	(	(	PUNCT
eurjchem-448	22	4	antifungal	antifungal	ADJ
eurjchem-448	22	5	against	against	ADP
eurjchem-448	22	6	aspergillus‐	aspergillus‐	NOUN
eurjchem-448	22	7	niger	niger	PROPN
eurjchem-448	22	8	)	)	PUNCT
eurjchem-448	22	9	was	be	AUX
eurjchem-448	22	10	screened	screen	VERB
eurjchem-448	22	11	and	and	CCONJ
eurjchem-448	22	12	results	result	NOUN
eurjchem-448	22	13	obtained	obtain	VERB
eurjchem-448	22	14	were	be	AUX
eurjchem-448	22	15	arranged	arrange	VERB
eurjchem-448	22	16	graphically	graphically	ADV
eurjchem-448	22	17	.	.	PUNCT
eurjchem-448	23	1	2	2	X
eurjchem-448	23	2	.	.	X
eurjchem-448	23	3	experimental	experimental	ADJ
eurjchem-448	23	4	2.1	2.1	NUM
eurjchem-448	23	5	.	.	PUNCT
eurjchem-448	23	6	materials	material	NOUN
eurjchem-448	23	7	and	and	CCONJ
eurjchem-448	23	8	chemicals	chemical	NOUN
eurjchem-448	23	9	all	all	DET
eurjchem-448	23	10	the	the	DET
eurjchem-448	23	11	chemicals	chemical	NOUN
eurjchem-448	23	12	used	use	VERB
eurjchem-448	23	13	were	be	AUX
eurjchem-448	23	14	of	of	ADP
eurjchem-448	23	15	analytical	analytical	ADJ
eurjchem-448	23	16	reagent	reagent	ADJ
eurjchem-448	23	17	grade	grade	NOUN
eurjchem-448	23	18	procured	procure	VERB
eurjchem-448	23	19	from	from	ADP
eurjchem-448	23	20	sigma‐aldrich	sigma‐aldrich	PROPN
eurjchem-448	23	21	.	.	PUNCT
eurjchem-448	24	1	metal	metal	NOUN
eurjchem-448	24	2	salts	salt	NOUN
eurjchem-448	24	3	were	be	AUX
eurjchem-448	24	4	purchased	purchase	VERB
eurjchem-448	24	5	from	from	ADP
eurjchem-448	24	6	e.	e.	PROPN
eurjchem-448	24	7	merck	merck	PROPN
eurjchem-448	24	8	.	.	PUNCT
eurjchem-448	25	1	all	all	DET
eurjchem-448	25	2	reagents	reagent	NOUN
eurjchem-448	25	3	were	be	AUX
eurjchem-448	25	4	used	use	VERB
eurjchem-448	25	5	without	without	ADP
eurjchem-448	25	6	further	further	ADJ
eurjchem-448	25	7	purification	purification	NOUN
eurjchem-448	25	8	.	.	PUNCT
eurjchem-448	26	1	2.2	2.2	NUM
eurjchem-448	26	2	.	.	PUNCT
eurjchem-448	27	1	instrumentation	instrumentation	NOUN
eurjchem-448	27	2	analytical	analytical	ADJ
eurjchem-448	27	3	data	datum	NOUN
eurjchem-448	27	4	(	(	PUNCT
eurjchem-448	27	5	c	c	NOUN
eurjchem-448	27	6	,	,	PUNCT
eurjchem-448	27	7	h	h	NOUN
eurjchem-448	27	8	and	and	CCONJ
eurjchem-448	27	9	n	n	CCONJ
eurjchem-448	27	10	)	)	PUNCT
eurjchem-448	27	11	of	of	ADP
eurjchem-448	27	12	mc	mc	PROPN
eurjchem-448	27	13	and	and	CCONJ
eurjchem-448	27	14	ces	ces	PROPN
eurjchem-448	27	15	were	be	AUX
eurjchem-448	27	16	obtained	obtain	VERB
eurjchem-448	27	17	with	with	ADP
eurjchem-448	27	18	a	a	DET
eurjchem-448	27	19	carlo‐ebra	carlo‐ebra	NOUN
eurjchem-448	27	20	1106	1106	NUM
eurjchem-448	27	21	elemental	elemental	ADJ
eurjchem-448	27	22	analyzer	analyzer	NOUN
eurjchem-448	27	23	.	.	PUNCT
eurjchem-448	28	1	molar	molar	ADJ
eurjchem-448	28	2	conductance	conductance	NOUN
eurjchem-448	28	3	was	be	AUX
eurjchem-448	28	4	measured	measure	VERB
eurjchem-448	28	5	on	on	ADP
eurjchem-448	28	6	leeds	leed	NOUN
eurjchem-448	28	7	northrup	northrup	PROPN
eurjchem-448	28	8	4995	4995	NUM
eurjchem-448	28	9	conductivity	conductivity	NOUN
eurjchem-448	28	10	bridge	bridge	NOUN
eurjchem-448	28	11	.	.	PUNCT
eurjchem-448	29	1	molar	molar	ADJ
eurjchem-448	29	2	magnetic	magnetic	ADJ
eurjchem-448	29	3	susceptibility	susceptibility	NOUN
eurjchem-448	29	4	was	be	AUX
eurjchem-448	29	5	measured	measure	VERB
eurjchem-448	29	6	with	with	ADP
eurjchem-448	29	7	powdered	powdered	ADJ
eurjchem-448	29	8	samples	sample	NOUN
eurjchem-448	29	9	using	use	VERB
eurjchem-448	29	10	faraday	faraday	PROPN
eurjchem-448	29	11	method	method	NOUN
eurjchem-448	29	12	.	.	PUNCT
eurjchem-448	30	1	diamagnetic	diamagnetic	ADJ
eurjchem-448	30	2	corrections	correction	NOUN
eurjchem-448	30	3	were	be	AUX
eurjchem-448	30	4	made	make	VERB
eurjchem-448	30	5	using	use	VERB
eurjchem-448	30	6	pascal	pascal	NOUN
eurjchem-448	30	7	’s	’s	PART
eurjchem-448	30	8	constant	constant	ADJ
eurjchem-448	30	9	and	and	CCONJ
eurjchem-448	30	10	hg[co(scn)4	hg[co(scn)4	ADJ
eurjchem-448	30	11	]	]	PUNCT
eurjchem-448	30	12	as	as	ADP
eurjchem-448	30	13	calibrant	calibrant	ADJ
eurjchem-448	30	14	at	at	ADP
eurjchem-448	30	15	room	room	NOUN
eurjchem-448	30	16	temperature	temperature	NOUN
eurjchem-448	30	17	(	(	PUNCT
eurjchem-448	30	18	χg	χg	NOUN
eurjchem-448	30	19	=	=	SYM
eurjchem-448	30	20	16.44	16.44	NUM
eurjchem-448	30	21	×10‐6	×10‐6	PROPN
eurjchem-448	30	22	in	in	ADP
eurjchem-448	30	23	c.g.s	c.g.	NOUN
eurjchem-448	30	24	.	.	PUNCT
eurjchem-448	31	1	units	unit	NOUN
eurjchem-448	31	2	)	)	PUNCT
eurjchem-448	31	3	.	.	PUNCT
eurjchem-448	32	1	ir	ir	PROPN
eurjchem-448	32	2	spectra	spectra	PROPN
eurjchem-448	32	3	were	be	AUX
eurjchem-448	32	4	recorded	record	VERB
eurjchem-448	32	5	on	on	ADP
eurjchem-448	32	6	perkin	perkin	PROPN
eurjchem-448	32	7	elmer	elmer	PROPN
eurjchem-448	32	8	137	137	NUM
eurjchem-448	32	9	instrument	instrument	NOUN
eurjchem-448	32	10	as	as	ADP
eurjchem-448	32	11	kbr	kbr	PROPN
eurjchem-448	32	12	pellets	pellet	NOUN
eurjchem-448	32	13	in	in	ADP
eurjchem-448	32	14	wave	wave	NOUN
eurjchem-448	32	15	number	number	NOUN
eurjchem-448	32	16	region	region	NOUN
eurjchem-448	32	17	4000‐400	4000‐400	NUM
eurjchem-448	32	18	cm‐1	cm‐1	NOUN
eurjchem-448	32	19	.	.	PUNCT
eurjchem-448	33	1	1h	1h	NUM
eurjchem-448	33	2	and	and	CCONJ
eurjchem-448	33	3	13c	13c	NOUN
eurjchem-448	33	4	nmr	nmr	NOUN
eurjchem-448	33	5	spectra	spectra	NOUN
eurjchem-448	33	6	were	be	AUX
eurjchem-448	33	7	recorded	record	VERB
eurjchem-448	33	8	at	at	ADP
eurjchem-448	33	9	ambient	ambient	ADJ
eurjchem-448	33	10	temperatures	temperature	NOUN
eurjchem-448	33	11	on	on	ADP
eurjchem-448	33	12	bruker	bruker	PROPN
eurjchem-448	33	13	amx400	amx400	PROPN
eurjchem-448	33	14	and	and	CCONJ
eurjchem-448	33	15	drx500	drx500	PROPN
eurjchem-448	33	16	spectrometers	spectrometer	NOUN
eurjchem-448	33	17	with	with	ADP
eurjchem-448	33	18	tetramethylsilane	tetramethylsilane	PROPN
eurjchem-448	33	19	(	(	PUNCT
eurjchem-448	33	20	tms	tms	PROPN
eurjchem-448	33	21	)	)	PUNCT
eurjchem-448	33	22	as	as	ADP
eurjchem-448	33	23	internal	internal	ADJ
eurjchem-448	33	24	reference	reference	NOUN
eurjchem-448	33	25	and	and	CCONJ
eurjchem-448	33	26	cdcl3	cdcl3	NOUN
eurjchem-448	33	27	as	as	ADP
eurjchem-448	33	28	solvent	solvent	NOUN
eurjchem-448	33	29	.	.	PUNCT
eurjchem-448	34	1	chemical	chemical	ADJ
eurjchem-448	34	2	shifts	shift	NOUN
eurjchem-448	34	3	(	(	PUNCT
eurjchem-448	34	4	δ	δ	NOUN
eurjchem-448	34	5	)	)	PUNCT
eurjchem-448	34	6	were	be	AUX
eurjchem-448	34	7	expressed	express	VERB
eurjchem-448	34	8	in	in	ADP
eurjchem-448	34	9	parts	part	NOUN
eurjchem-448	34	10	per	per	ADP
eurjchem-448	34	11	million	million	NUM
eurjchem-448	34	12	(	(	PUNCT
eurjchem-448	34	13	ppm	ppm	NOUN
eurjchem-448	34	14	)	)	PUNCT
eurjchem-448	34	15	relative	relative	NOUN
eurjchem-448	34	16	to	to	ADP
eurjchem-448	34	17	tms	tms	PROPN
eurjchem-448	34	18	.	.	PUNCT
eurjchem-448	35	1	uv‐	uv‐	PROPN
eurjchem-448	35	2	vis	vis	X
eurjchem-448	35	3	spectra	spectra	PROPN
eurjchem-448	35	4	were	be	AUX
eurjchem-448	35	5	recorded	record	VERB
eurjchem-448	35	6	on	on	ADP
eurjchem-448	35	7	a	a	DET
eurjchem-448	35	8	shimadzu	shimadzu	ADJ
eurjchem-448	35	9	uv	uv	NOUN
eurjchem-448	35	10	mini	mini	ADJ
eurjchem-448	35	11	1240	1240	NUM
eurjchem-448	35	12	spectrometer	spectrometer	NOUN
eurjchem-448	35	13	.	.	PUNCT
eurjchem-448	36	1	electron	electron	PROPN
eurjchem-448	36	2	impact	impact	PROPN
eurjchem-448	36	3	mass	mass	PROPN
eurjchem-448	36	4	spectra	spectra	PROPN
eurjchem-448	36	5	were	be	AUX
eurjchem-448	36	6	recorded	record	VERB
eurjchem-448	36	7	on	on	ADP
eurjchem-448	36	8	jeol	jeol	PROPN
eurjchem-448	36	9	,	,	PUNCT
eurjchem-448	36	10	jms	jms	PROPN
eurjchem-448	36	11	,	,	PUNCT
eurjchem-448	36	12	dx‐303	dx‐303	PROPN
eurjchem-448	36	13	mass	mass	NOUN
eurjchem-448	36	14	spectrometer	spectrometer	NOUN
eurjchem-448	36	15	.	.	PUNCT
eurjchem-448	37	1	electron	electron	PROPN
eurjchem-448	37	2	paramagnetic	paramagnetic	ADJ
eurjchem-448	37	3	resonance	resonance	NOUN
eurjchem-448	37	4	(	(	PUNCT
eurjchem-448	37	5	epr	epr	PROPN
eurjchem-448	37	6	)	)	PUNCT
eurjchem-448	37	7	spectra	spectra	NOUN
eurjchem-448	37	8	of	of	ADP
eurjchem-448	37	9	ces	ce	NOUN
eurjchem-448	37	10	were	be	AUX
eurjchem-448	37	11	recorded	record	VERB
eurjchem-448	37	12	as	as	ADP
eurjchem-448	37	13	polycrystalline	polycrystalline	ADJ
eurjchem-448	37	14	sample	sample	NOUN
eurjchem-448	37	15	as	as	ADV
eurjchem-448	37	16	well	well	ADV
eurjchem-448	37	17	as	as	ADP
eurjchem-448	37	18	in	in	ADP
eurjchem-448	37	19	solution	solution	NOUN
eurjchem-448	37	20	(	(	PUNCT
eurjchem-448	37	21	at	at	ADP
eurjchem-448	37	22	room	room	NOUN
eurjchem-448	37	23	tempera‐	tempera‐	PROPN
eurjchem-448	37	24	58	58	NUM
eurjchem-448	37	25	kumar	kumar	PROPN
eurjchem-448	37	26	et	et	PROPN
eurjchem-448	37	27	al	al	PROPN
eurjchem-448	37	28	.	.	PUNCT
eurjchem-448	37	29	/	/	SYM
eurjchem-448	37	30	european	european	PROPN
eurjchem-448	37	31	journal	journal	PROPN
eurjchem-448	37	32	of	of	ADP
eurjchem-448	37	33	chemistry	chemistry	NOUN
eurjchem-448	37	34	3	3	NUM
eurjchem-448	37	35	(	(	PUNCT
eurjchem-448	37	36	1	1	NUM
eurjchem-448	37	37	)	)	PUNCT
eurjchem-448	37	38	(	(	PUNCT
eurjchem-448	37	39	2012	2012	NUM
eurjchem-448	37	40	)	)	PUNCT
eurjchem-448	38	1	57‐64	57‐64	NUM
eurjchem-448	38	2	scheme	scheme	VERB
eurjchem-448	38	3	1	1	NUM
eurjchem-448	38	4	‐ture	‐ture	NUM
eurjchem-448	38	5	and	and	CCONJ
eurjchem-448	38	6	liquid‐nitrogen	liquid‐nitrogen	NOUN
eurjchem-448	38	7	temperature	temperature	NOUN
eurjchem-448	38	8	(	(	PUNCT
eurjchem-448	38	9	lnt	lnt	NOUN
eurjchem-448	38	10	)	)	PUNCT
eurjchem-448	38	11	)	)	PUNCT
eurjchem-448	38	12	on	on	ADP
eurjchem-448	38	13	varion	varion	NOUN
eurjchem-448	38	14	e‐4	e‐4	PROPN
eurjchem-448	38	15	epr	epr	PROPN
eurjchem-448	38	16	spectrometer	spectrometer	NOUN
eurjchem-448	38	17	using	use	VERB
eurjchem-448	38	18	diphenylpicrylhydrazyl	diphenylpicrylhydrazyl	NOUN
eurjchem-448	38	19	(	(	PUNCT
eurjchem-448	38	20	dpph	dpph	PROPN
eurjchem-448	38	21	)	)	PUNCT
eurjchem-448	38	22	as	as	ADP
eurjchem-448	38	23	the	the	DET
eurjchem-448	38	24	g‐marker	g‐marker	NOUN
eurjchem-448	38	25	.	.	PUNCT
eurjchem-448	38	26	cyclic	cyclic	ADJ
eurjchem-448	38	27	voltammetry	voltammetry	NOUN
eurjchem-448	38	28	measurements	measurement	NOUN
eurjchem-448	38	29	were	be	AUX
eurjchem-448	38	30	made	make	VERB
eurjchem-448	38	31	in	in	ADP
eurjchem-448	38	32	a	a	DET
eurjchem-448	38	33	single	single	ADJ
eurjchem-448	38	34	compartment	compartment	NOUN
eurjchem-448	38	35	cell	cell	NOUN
eurjchem-448	38	36	with	with	ADP
eurjchem-448	38	37	a	a	DET
eurjchem-448	38	38	platinum	platinum	NOUN
eurjchem-448	38	39	counter	counter	NOUN
eurjchem-448	38	40	electrode	electrode	NOUN
eurjchem-448	38	41	and	and	CCONJ
eurjchem-448	38	42	ag	ag	PROPN
eurjchem-448	38	43	/	/	SYM
eurjchem-448	38	44	ag+	ag+	PROPN
eurjchem-448	38	45	reference	reference	NOUN
eurjchem-448	38	46	electrode	electrode	NOUN
eurjchem-448	38	47	at	at	ADP
eurjchem-448	38	48	room	room	NOUN
eurjchem-448	38	49	temperature	temperature	NOUN
eurjchem-448	38	50	.	.	PUNCT
eurjchem-448	39	1	tetraethylammonium	tetraethylammonium	NOUN
eurjchem-448	39	2	perchlorate	perchlorate	NOUN
eurjchem-448	39	3	(	(	PUNCT
eurjchem-448	39	4	teap	teap	NOUN
eurjchem-448	39	5	)	)	PUNCT
eurjchem-448	39	6	was	be	AUX
eurjchem-448	39	7	used	use	VERB
eurjchem-448	39	8	as	as	ADP
eurjchem-448	39	9	a	a	DET
eurjchem-448	39	10	supporting	support	VERB
eurjchem-448	39	11	electrolyte	electrolyte	NOUN
eurjchem-448	39	12	.	.	PUNCT
eurjchem-448	40	1	2.3	2.3	NUM
eurjchem-448	40	2	.	.	PUNCT
eurjchem-448	41	1	synthesis	synthesis	NOUN
eurjchem-448	41	2	2.3.1	2.3.1	NUM
eurjchem-448	41	3	synthesis	synthesis	NOUN
eurjchem-448	41	4	of	of	ADP
eurjchem-448	41	5	9,17‐diaza‐2,6,11,15‐tetrathia‐1,7,10,16‐	9,17‐diaza‐2,6,11,15‐tetrathia‐1,7,10,16‐	NUM
eurjchem-448	41	6	(	(	PUNCT
eurjchem-448	41	7	1,2)tetrabenzenacyclooctadecaphan‐8,17‐diene	1,2)tetrabenzenacyclooctadecaphan‐8,17‐diene	PROPN
eurjchem-448	41	8	(	(	PUNCT
eurjchem-448	41	9	mc	mc	PROPN
eurjchem-448	41	10	)	)	PUNCT
eurjchem-448	41	11	mc	mc	PROPN
eurjchem-448	42	1	having	have	VERB
eurjchem-448	42	2	azomethine	azomethine	NOUN
eurjchem-448	42	3	(	(	PUNCT
eurjchem-448	42	4	‐ch	‐ch	X
eurjchem-448	42	5	=	=	SYM
eurjchem-448	42	6	n‐	n‐	NOUN
eurjchem-448	42	7	)	)	PUNCT
eurjchem-448	42	8	and	and	CCONJ
eurjchem-448	42	9	thioether	thioether	ADJ
eurjchem-448	42	10	(	(	PUNCT
eurjchem-448	42	11	‐c6h4‐s‐	‐c6h4‐s‐	ADV
eurjchem-448	42	12	ch2‐	ch2‐	NOUN
eurjchem-448	42	13	)	)	PUNCT
eurjchem-448	42	14	linkages	linkage	NOUN
eurjchem-448	42	15	were	be	AUX
eurjchem-448	42	16	synthesized	synthesize	VERB
eurjchem-448	42	17	as	as	SCONJ
eurjchem-448	42	18	follows	follow	VERB
eurjchem-448	42	19	:	:	PUNCT
eurjchem-448	42	20	condensation	condensation	NOUN
eurjchem-448	42	21	reaction	reaction	NOUN
eurjchem-448	42	22	of	of	ADP
eurjchem-448	42	23	an	an	DET
eurjchem-448	42	24	amine	amine	ADJ
eurjchem-448	42	25	and	and	CCONJ
eurjchem-448	42	26	aldehyde	aldehyde	NOUN
eurjchem-448	42	27	generated	generate	VERB
eurjchem-448	42	28	proposed	propose	VERB
eurjchem-448	42	29	macrocycle	macrocycle	NOUN
eurjchem-448	42	30	(	(	PUNCT
eurjchem-448	42	31	scheme	scheme	NOUN
eurjchem-448	42	32	1	1	NUM
eurjchem-448	42	33	)	)	PUNCT
eurjchem-448	42	34	.	.	PUNCT
eurjchem-448	43	1	an	an	DET
eurjchem-448	43	2	earlier	early	ADV
eurjchem-448	43	3	reported	report	VERB
eurjchem-448	43	4	synthetic	synthetic	ADJ
eurjchem-448	43	5	route	route	NOUN
eurjchem-448	43	6	[	[	X
eurjchem-448	43	7	6	6	NUM
eurjchem-448	43	8	]	]	PUNCT
eurjchem-448	43	9	was	be	AUX
eurjchem-448	43	10	followed	follow	VERB
eurjchem-448	43	11	,	,	PUNCT
eurjchem-448	43	12	with	with	ADP
eurjchem-448	43	13	slight	slight	ADJ
eurjchem-448	43	14	modification	modification	NOUN
eurjchem-448	43	15	,	,	PUNCT
eurjchem-448	43	16	as	as	SCONJ
eurjchem-448	43	17	required	require	VERB
eurjchem-448	43	18	for	for	ADP
eurjchem-448	43	19	the	the	DET
eurjchem-448	43	20	preparation	preparation	NOUN
eurjchem-448	43	21	of	of	ADP
eurjchem-448	43	22	1,5‐bis(o‐aminothiol)propane	1,5‐bis(o‐aminothiol)propane	PROPN
eurjchem-448	43	23	.	.	PUNCT
eurjchem-448	44	1	a	a	DET
eurjchem-448	44	2	detailed	detailed	ADJ
eurjchem-448	44	3	methodology	methodology	NOUN
eurjchem-448	44	4	for	for	ADP
eurjchem-448	44	5	the	the	DET
eurjchem-448	44	6	synthesis	synthesis	NOUN
eurjchem-448	44	7	of	of	ADP
eurjchem-448	44	8	mc	mc	PROPN
eurjchem-448	44	9	with	with	ADP
eurjchem-448	44	10	azomethine	azomethine	PROPN
eurjchem-448	44	11	(	(	PUNCT
eurjchem-448	44	12	‐ch	‐ch	X
eurjchem-448	44	13	=	=	SYM
eurjchem-448	44	14	n‐	n‐	NOUN
eurjchem-448	44	15	)	)	PUNCT
eurjchem-448	44	16	and	and	CCONJ
eurjchem-448	44	17	thioether	thioether	ADJ
eurjchem-448	44	18	(	(	PUNCT
eurjchem-448	44	19	‐c6h4‐s‐ch2‐	‐c6h4‐s‐ch2‐	NOUN
eurjchem-448	44	20	)	)	PUNCT
eurjchem-448	44	21	linkages	linkage	NOUN
eurjchem-448	44	22	,	,	PUNCT
eurjchem-448	44	23	was	be	AUX
eurjchem-448	44	24	as	as	SCONJ
eurjchem-448	44	25	follows	follow	VERB
eurjchem-448	44	26	:	:	PUNCT
eurjchem-448	44	27	hot	hot	ADJ
eurjchem-448	44	28	etoh	etoh	NOUN
eurjchem-448	44	29	solution	solution	NOUN
eurjchem-448	44	30	(	(	PUNCT
eurjchem-448	44	31	30	30	NUM
eurjchem-448	44	32	ml	ml	NOUN
eurjchem-448	44	33	,	,	PUNCT
eurjchem-448	44	34	absolute	absolute	ADJ
eurjchem-448	44	35	)	)	PUNCT
eurjchem-448	44	36	of	of	ADP
eurjchem-448	44	37	1,5‐bis(o‐aminothiol)propane	1,5‐bis(o‐aminothiol)propane	PROPN
eurjchem-448	44	38	(	(	PUNCT
eurjchem-448	44	39	1	1	NUM
eurjchem-448	44	40	mmole	mmole	NOUN
eurjchem-448	44	41	)	)	PUNCT
eurjchem-448	44	42	was	be	AUX
eurjchem-448	44	43	mixed	mix	VERB
eurjchem-448	44	44	with	with	ADP
eurjchem-448	44	45	hot	hot	ADJ
eurjchem-448	44	46	etoh	etoh	NOUN
eurjchem-448	44	47	solution	solution	NOUN
eurjchem-448	44	48	(	(	PUNCT
eurjchem-448	44	49	30	30	NUM
eurjchem-448	44	50	ml	ml	NOUN
eurjchem-448	44	51	,	,	PUNCT
eurjchem-448	44	52	absolute	absolute	ADJ
eurjchem-448	44	53	)	)	PUNCT
eurjchem-448	44	54	of	of	ADP
eurjchem-448	44	55	1,5‐bis(2‐formylphenyl)‐1,5‐dithiapropane	1,5‐bis(2‐formylphenyl)‐1,5‐dithiapropane	NUM
eurjchem-448	44	56	(	(	PUNCT
eurjchem-448	44	57	0.1	0.1	NUM
eurjchem-448	44	58	mol	mol	NOUN
eurjchem-448	44	59	)	)	PUNCT
eurjchem-448	44	60	in	in	ADP
eurjchem-448	44	61	round	round	ADJ
eurjchem-448	44	62	bottom	bottom	ADJ
eurjchem-448	44	63	flask	flask	NOUN
eurjchem-448	44	64	(	(	PUNCT
eurjchem-448	44	65	100	100	NUM
eurjchem-448	44	66	ml	ml	NOUN
eurjchem-448	44	67	)	)	PUNCT
eurjchem-448	44	68	in	in	ADP
eurjchem-448	44	69	presence	presence	NOUN
eurjchem-448	44	70	of	of	ADP
eurjchem-448	44	71	few	few	ADJ
eurjchem-448	44	72	drops	drop	NOUN
eurjchem-448	44	73	of	of	ADP
eurjchem-448	44	74	concentrated	concentrate	VERB
eurjchem-448	44	75	hcl	hcl	PROPN
eurjchem-448	44	76	.	.	PUNCT
eurjchem-448	45	1	after	after	ADP
eurjchem-448	45	2	complete	complete	ADJ
eurjchem-448	45	3	addition	addition	NOUN
eurjchem-448	45	4	,	,	PUNCT
eurjchem-448	45	5	the	the	DET
eurjchem-448	45	6	solution	solution	NOUN
eurjchem-448	45	7	mixture	mixture	NOUN
eurjchem-448	45	8	was	be	AUX
eurjchem-448	45	9	refluxed	refluxe	VERB
eurjchem-448	45	10	for	for	ADP
eurjchem-448	45	11	2	2	NUM
eurjchem-448	45	12	h	h	NOUN
eurjchem-448	45	13	at	at	ADP
eurjchem-448	45	14	80‐82	80‐82	NUM
eurjchem-448	45	15	°	°	ADP
eurjchem-448	45	16	c	c	X
eurjchem-448	45	17	.	.	PUNCT
eurjchem-448	46	1	yellow	yellow	ADJ
eurjchem-448	46	2	white	white	ADJ
eurjchem-448	46	3	powdered	powdered	ADJ
eurjchem-448	46	4	compound	compound	NOUN
eurjchem-448	46	5	was	be	AUX
eurjchem-448	46	6	obtained	obtain	VERB
eurjchem-448	46	7	,	,	PUNCT
eurjchem-448	46	8	dried	dry	VERB
eurjchem-448	46	9	and	and	CCONJ
eurjchem-448	46	10	dissolved	dissolve	VERB
eurjchem-448	46	11	in	in	ADP
eurjchem-448	46	12	minimum	minimum	NOUN
eurjchem-448	46	13	amount	amount	NOUN
eurjchem-448	46	14	of	of	ADP
eurjchem-448	46	15	ch2cl2	ch2cl2	NOUN
eurjchem-448	46	16	.	.	PUNCT
eurjchem-448	46	17	small	small	ADJ
eurjchem-448	46	18	amount	amount	NOUN
eurjchem-448	46	19	of	of	ADP
eurjchem-448	46	20	n‐hexane	n‐hexane	NUM
eurjchem-448	46	21	was	be	AUX
eurjchem-448	46	22	added	add	VERB
eurjchem-448	46	23	to	to	PART
eurjchem-448	46	24	precipitate	precipitate	VERB
eurjchem-448	46	25	out	out	ADP
eurjchem-448	46	26	required	require	VERB
eurjchem-448	46	27	compound	compound	NOUN
eurjchem-448	46	28	and	and	CCONJ
eurjchem-448	46	29	finally	finally	ADV
eurjchem-448	46	30	filtered	filter	VERB
eurjchem-448	46	31	as	as	ADP
eurjchem-448	46	32	a	a	DET
eurjchem-448	46	33	dull	dull	ADJ
eurjchem-448	46	34	yellow	yellow	ADJ
eurjchem-448	46	35	crystalline	crystalline	NOUN
eurjchem-448	46	36	solid	solid	ADJ
eurjchem-448	46	37	.	.	PUNCT
eurjchem-448	47	1	the	the	DET
eurjchem-448	47	2	mixture	mixture	NOUN
eurjchem-448	47	3	was	be	AUX
eurjchem-448	47	4	cooled	cool	VERB
eurjchem-448	47	5	at	at	ADP
eurjchem-448	47	6	room	room	NOUN
eurjchem-448	47	7	temperature	temperature	NOUN
eurjchem-448	47	8	and	and	CCONJ
eurjchem-448	47	9	excess	excess	ADJ
eurjchem-448	47	10	solvent	solvent	NOUN
eurjchem-448	47	11	removed	remove	VERB
eurjchem-448	47	12	under	under	ADP
eurjchem-448	47	13	reduced	reduced	ADJ
eurjchem-448	47	14	pressure	pressure	NOUN
eurjchem-448	47	15	until	until	SCONJ
eurjchem-448	47	16	a	a	DET
eurjchem-448	47	17	solid	solid	ADJ
eurjchem-448	47	18	product	product	NOUN
eurjchem-448	47	19	was	be	AUX
eurjchem-448	47	20	formed	form	VERB
eurjchem-448	47	21	.	.	PUNCT
eurjchem-448	48	1	yield	yield	NOUN
eurjchem-448	48	2	:	:	PUNCT
eurjchem-448	48	3	63	63	NUM
eurjchem-448	48	4	%	%	NOUN
eurjchem-448	48	5	.	.	PUNCT
eurjchem-448	49	1	m.p	m.p	PROPN
eurjchem-448	49	2	.	.	PROPN
eurjchem-448	49	3	:	:	PUNCT
eurjchem-448	50	1	191	191	NUM
eurjchem-448	50	2	°	°	SYM
eurjchem-448	50	3	c	c	NOUN
eurjchem-448	50	4	.	.	PUNCT
eurjchem-448	50	5	2.3.2	2.3.2	NUM
eurjchem-448	50	6	synthesis	synthesis	NOUN
eurjchem-448	50	7	of	of	ADP
eurjchem-448	50	8	ces	ces	X
eurjchem-448	50	9	ces	ce	NOUN
eurjchem-448	50	10	of	of	ADP
eurjchem-448	50	11	co(ii	co(ii	ADJ
eurjchem-448	50	12	)	)	PUNCT
eurjchem-448	50	13	or	or	CCONJ
eurjchem-448	50	14	ni(ii	ni(ii	PROPN
eurjchem-448	50	15	)	)	PUNCT
eurjchem-448	50	16	were	be	AUX
eurjchem-448	50	17	prepared	prepare	VERB
eurjchem-448	50	18	by	by	ADP
eurjchem-448	50	19	mixing	mix	VERB
eurjchem-448	50	20	equimolar	equimolar	NOUN
eurjchem-448	50	21	amounts	amount	NOUN
eurjchem-448	50	22	of	of	ADP
eurjchem-448	50	23	mc	mc	PROPN
eurjchem-448	50	24	(	(	PUNCT
eurjchem-448	50	25	0.05	0.05	NUM
eurjchem-448	50	26	mol	mol	NOUN
eurjchem-448	50	27	)	)	PUNCT
eurjchem-448	50	28	and	and	CCONJ
eurjchem-448	50	29	corresponding	corresponding	ADJ
eurjchem-448	50	30	metal	metal	NOUN
eurjchem-448	50	31	salts	salt	NOUN
eurjchem-448	50	32	,	,	PUNCT
eurjchem-448	50	33	it	it	PRON
eurjchem-448	50	34	can	can	AUX
eurjchem-448	50	35	be	be	AUX
eurjchem-448	50	36	cocl2	cocl2	NOUN
eurjchem-448	50	37	or	or	CCONJ
eurjchem-448	50	38	nicl2	nicl2	NOUN
eurjchem-448	50	39	(	(	PUNCT
eurjchem-448	50	40	0.5	0.5	NUM
eurjchem-448	50	41	mmol	mmol	NOUN
eurjchem-448	50	42	)	)	PUNCT
eurjchem-448	50	43	in	in	ADP
eurjchem-448	50	44	minimum	minimum	ADJ
eurjchem-448	50	45	quantity	quantity	NOUN
eurjchem-448	50	46	of	of	ADP
eurjchem-448	50	47	etoh	etoh	NOUN
eurjchem-448	50	48	(	(	PUNCT
eurjchem-448	50	49	25	25	NUM
eurjchem-448	50	50	ml	ml	ADJ
eurjchem-448	50	51	,	,	PUNCT
eurjchem-448	50	52	absolute	absolute	ADJ
eurjchem-448	50	53	)	)	PUNCT
eurjchem-448	50	54	for	for	ADP
eurjchem-448	50	55	nearly	nearly	ADV
eurjchem-448	50	56	3‐4	3‐4	ADJ
eurjchem-448	50	57	h	h	NOUN
eurjchem-448	50	58	at	at	ADP
eurjchem-448	50	59	~81‐82	~81‐82	PROPN
eurjchem-448	50	60	°	°	ADP
eurjchem-448	50	61	c	c	NOUN
eurjchem-448	50	62	on	on	ADP
eurjchem-448	50	63	a	a	DET
eurjchem-448	50	64	water	water	NOUN
eurjchem-448	50	65	bath	bath	NOUN
eurjchem-448	50	66	until	until	SCONJ
eurjchem-448	50	67	volume	volume	NOUN
eurjchem-448	50	68	was	be	AUX
eurjchem-448	50	69	reduced	reduce	VERB
eurjchem-448	50	70	to	to	PART
eurjchem-448	50	71	~12	~12	PRON
eurjchem-448	50	72	ml	ml	NOUN
eurjchem-448	50	73	.	.	PUNCT
eurjchem-448	51	1	a	a	DET
eurjchem-448	51	2	solid	solid	ADJ
eurjchem-448	51	3	mass	mass	NOUN
eurjchem-448	51	4	separated	separate	VERB
eurjchem-448	51	5	out	out	ADP
eurjchem-448	51	6	on	on	ADP
eurjchem-448	51	7	cooling	cool	VERB
eurjchem-448	51	8	at	at	ADP
eurjchem-448	51	9	~5	~5	ADJ
eurjchem-448	51	10	°	°	ADP
eurjchem-448	51	11	c	c	NOUN
eurjchem-448	51	12	was	be	AUX
eurjchem-448	51	13	refrigerated	refrigerate	VERB
eurjchem-448	51	14	for	for	ADP
eurjchem-448	51	15	better	well	ADJ
eurjchem-448	51	16	crystallization	crystallization	NOUN
eurjchem-448	51	17	.	.	PUNCT
eurjchem-448	52	1	it	it	PRON
eurjchem-448	52	2	was	be	AUX
eurjchem-448	52	3	then	then	ADV
eurjchem-448	52	4	filtered	filter	VERB
eurjchem-448	52	5	,	,	PUNCT
eurjchem-448	52	6	washed	wash	VERB
eurjchem-448	52	7	with	with	ADP
eurjchem-448	52	8	etoh	etoh	NOUN
eurjchem-448	52	9	and	and	CCONJ
eurjchem-448	52	10	dried	dry	VERB
eurjchem-448	52	11	over	over	ADP
eurjchem-448	52	12	p2o5	p2o5	PROPN
eurjchem-448	52	13	under	under	ADP
eurjchem-448	52	14	vacuum	vacuum	NOUN
eurjchem-448	52	15	.	.	PUNCT
eurjchem-448	53	1	the	the	DET
eurjchem-448	53	2	crystals	crystal	NOUN
eurjchem-448	53	3	were	be	AUX
eurjchem-448	53	4	redissolved	redissolve	VERB
eurjchem-448	53	5	for	for	ADP
eurjchem-448	53	6	recrystallization	recrystallization	NOUN
eurjchem-448	53	7	with	with	ADP
eurjchem-448	53	8	warm	warm	ADJ
eurjchem-448	53	9	ethanol	ethanol	NOUN
eurjchem-448	53	10	,	,	PUNCT
eurjchem-448	53	11	resulting	result	VERB
eurjchem-448	53	12	in	in	ADP
eurjchem-448	53	13	a	a	DET
eurjchem-448	53	14	clear	clear	ADJ
eurjchem-448	53	15	solution	solution	NOUN
eurjchem-448	53	16	,	,	PUNCT
eurjchem-448	53	17	formed	form	VERB
eurjchem-448	53	18	small	small	ADJ
eurjchem-448	53	19	crystals	crystal	NOUN
eurjchem-448	53	20	when	when	SCONJ
eurjchem-448	53	21	left	leave	VERB
eurjchem-448	53	22	undisturbed	undisturbed	ADJ
eurjchem-448	53	23	for	for	ADP
eurjchem-448	53	24	weeks	week	NOUN
eurjchem-448	53	25	.	.	PUNCT
eurjchem-448	54	1	ces	ce	NOUN
eurjchem-448	54	2	were	be	AUX
eurjchem-448	54	3	soluble	soluble	ADJ
eurjchem-448	54	4	in	in	ADP
eurjchem-448	54	5	dmso	dmso	NOUN
eurjchem-448	54	6	,	,	PUNCT
eurjchem-448	54	7	but	but	CCONJ
eurjchem-448	54	8	insoluble	insoluble	ADJ
eurjchem-448	54	9	in	in	ADP
eurjchem-448	54	10	common	common	ADJ
eurjchem-448	54	11	organic	organic	ADJ
eurjchem-448	54	12	solvents	solvent	NOUN
eurjchem-448	54	13	and	and	CCONJ
eurjchem-448	54	14	h2o	h2o	NOUN
eurjchem-448	54	15	and	and	CCONJ
eurjchem-448	54	16	were	be	AUX
eurjchem-448	54	17	thermally	thermally	ADV
eurjchem-448	54	18	stable	stable	ADJ
eurjchem-448	54	19	up	up	ADP
eurjchem-448	54	20	to	to	ADP
eurjchem-448	54	21	~210‐243	~210‐243	PROPN
eurjchem-448	54	22	°	°	ADP
eurjchem-448	54	23	c	c	NOUN
eurjchem-448	54	24	and	and	CCONJ
eurjchem-448	54	25	then	then	ADV
eurjchem-448	54	26	decomposed	decompose	VERB
eurjchem-448	54	27	.	.	PUNCT
eurjchem-448	55	1	2.4	2.4	NUM
eurjchem-448	55	2	.	.	PUNCT
eurjchem-448	56	1	molecular	molecular	ADJ
eurjchem-448	56	2	modeling	model	VERB
eurjchem-448	56	3	the	the	DET
eurjchem-448	56	4	mm2	mm2	NOUN
eurjchem-448	56	5	option	option	NOUN
eurjchem-448	56	6	of	of	ADP
eurjchem-448	56	7	the	the	DET
eurjchem-448	56	8	macromodel	macromodel	ADJ
eurjchem-448	56	9	2.7	2.7	NUM
eurjchem-448	56	10	program	program	NOUN
eurjchem-448	56	11	was	be	AUX
eurjchem-448	56	12	used	use	VERB
eurjchem-448	56	13	with	with	ADP
eurjchem-448	56	14	the	the	DET
eurjchem-448	56	15	default	default	NOUN
eurjchem-448	56	16	equations	equation	NOUN
eurjchem-448	56	17	in	in	ADP
eurjchem-448	56	18	all	all	DET
eurjchem-448	56	19	molecular	molecular	ADJ
eurjchem-448	56	20	mechanical	mechanical	ADJ
eurjchem-448	56	21	calculations	calculation	NOUN
eurjchem-448	56	22	.	.	PUNCT
eurjchem-448	57	1	the	the	DET
eurjchem-448	57	2	macromodel	macromodel	PROPN
eurjchem-448	57	3	force	force	NOUN
eurjchem-448	57	4	field	field	NOUN
eurjchem-448	57	5	was	be	AUX
eurjchem-448	57	6	used	use	VERB
eurjchem-448	57	7	to	to	PART
eurjchem-448	57	8	describe	describe	VERB
eurjchem-448	57	9	the	the	DET
eurjchem-448	57	10	organic	organic	ADJ
eurjchem-448	57	11	moiety	moiety	NOUN
eurjchem-448	57	12	of	of	ADP
eurjchem-448	57	13	the	the	DET
eurjchem-448	57	14	complex	complex	NOUN
eurjchem-448	57	15	,	,	PUNCT
eurjchem-448	57	16	with	with	ADP
eurjchem-448	57	17	preference	preference	NOUN
eurjchem-448	57	18	given	give	VERB
eurjchem-448	57	19	to	to	ADP
eurjchem-448	57	20	the	the	DET
eurjchem-448	57	21	mm2	mm2	NOUN
eurjchem-448	57	22	parameters	parameter	NOUN
eurjchem-448	57	23	.	.	PUNCT
eurjchem-448	58	1	correct	correct	ADJ
eurjchem-448	58	2	sequence	sequence	NOUN
eurjchem-448	58	3	of	of	ADP
eurjchem-448	58	4	atoms	atom	NOUN
eurjchem-448	58	5	was	be	AUX
eurjchem-448	58	6	obtained	obtain	VERB
eurjchem-448	58	7	to	to	PART
eurjchem-448	58	8	get	get	VERB
eurjchem-448	58	9	reasonable	reasonable	ADJ
eurjchem-448	58	10	low	low	ADJ
eurjchem-448	58	11	energy	energy	NOUN
eurjchem-448	58	12	molecular	molecular	ADJ
eurjchem-448	58	13	models	model	NOUN
eurjchem-448	58	14	to	to	PART
eurjchem-448	58	15	determine	determine	VERB
eurjchem-448	58	16	their	their	PRON
eurjchem-448	58	17	molecular	molecular	ADJ
eurjchem-448	58	18	representation	representation	NOUN
eurjchem-448	58	19	in	in	ADP
eurjchem-448	58	20	three	three	NUM
eurjchem-448	58	21	dimensions	dimension	NOUN
eurjchem-448	58	22	.	.	PUNCT
eurjchem-448	59	1	complications	complication	NOUN
eurjchem-448	59	2	of	of	ADP
eurjchem-448	59	3	biochemical	biochemical	ADJ
eurjchem-448	59	4	transformations	transformation	NOUN
eurjchem-448	59	5	may	may	AUX
eurjchem-448	59	6	be	be	AUX
eurjchem-448	59	7	explored	explore	VERB
eurjchem-448	59	8	using	use	VERB
eurjchem-448	59	9	output	output	NOUN
eurjchem-448	59	10	obtained	obtain	VERB
eurjchem-448	59	11	.	.	PUNCT
eurjchem-448	60	1	an	an	DET
eurjchem-448	60	2	attempt	attempt	NOUN
eurjchem-448	60	3	to	to	PART
eurjchem-448	60	4	gain	gain	VERB
eurjchem-448	60	5	a	a	DET
eurjchem-448	60	6	better	well	ADJ
eurjchem-448	60	7	insight	insight	NOUN
eurjchem-448	60	8	on	on	ADP
eurjchem-448	60	9	the	the	DET
eurjchem-448	60	10	molecular	molecular	ADJ
eurjchem-448	60	11	structure	structure	NOUN
eurjchem-448	60	12	of	of	ADP
eurjchem-448	60	13	the	the	DET
eurjchem-448	60	14	ligand	ligand	NOUN
eurjchem-448	60	15	and	and	CCONJ
eurjchem-448	60	16	its	its	PRON
eurjchem-448	60	17	complexes	complex	NOUN
eurjchem-448	60	18	,	,	PUNCT
eurjchem-448	60	19	geometric	geometric	ADJ
eurjchem-448	60	20	optimization	optimization	NOUN
eurjchem-448	60	21	and	and	CCONJ
eurjchem-448	60	22	conformational	conformational	ADJ
eurjchem-448	60	23	analysis	analysis	NOUN
eurjchem-448	60	24	has	have	AUX
eurjchem-448	60	25	been	be	AUX
eurjchem-448	60	26	performed	perform	VERB
eurjchem-448	60	27	using	use	VERB
eurjchem-448	60	28	mm+	mm+	NOUN
eurjchem-448	61	1	[	[	X
eurjchem-448	61	2	7	7	NUM
eurjchem-448	61	3	]	]	SYM
eurjchem-448	61	4	force	force	NOUN
eurjchem-448	61	5	field	field	NOUN
eurjchem-448	61	6	.	.	PUNCT
eurjchem-448	62	1	2.5	2.5	NUM
eurjchem-448	62	2	.	.	PUNCT
eurjchem-448	63	1	pharmacology	pharmacology	NOUN
eurjchem-448	63	2	(	(	PUNCT
eurjchem-448	63	3	in‐vitro	in‐vitro	X
eurjchem-448	63	4	antifungal	antifungal	ADJ
eurjchem-448	63	5	assay	assay	VERB
eurjchem-448	63	6	)	)	PUNCT
eurjchem-448	63	7	antimicrobial	antimicrobial	ADJ
eurjchem-448	63	8	activities	activity	NOUN
eurjchem-448	63	9	(	(	PUNCT
eurjchem-448	63	10	antifungal	antifungal	PROPN
eurjchem-448	63	11	)	)	PUNCT
eurjchem-448	63	12	of	of	ADP
eurjchem-448	63	13	mc	mc	PROPN
eurjchem-448	63	14	and	and	CCONJ
eurjchem-448	63	15	ces	ces	PROPN
eurjchem-448	63	16	were	be	AUX
eurjchem-448	63	17	screened	screen	VERB
eurjchem-448	63	18	against	against	ADP
eurjchem-448	63	19	aspergillus‐niger	aspergillus‐niger	PROPN
eurjchem-448	63	20	.	.	PUNCT
eurjchem-448	64	1	fresh	fresh	ADJ
eurjchem-448	64	2	stock	stock	NOUN
eurjchem-448	64	3	solutions	solution	NOUN
eurjchem-448	64	4	of	of	ADP
eurjchem-448	64	5	ligand	ligand	NOUN
eurjchem-448	64	6	and	and	CCONJ
eurjchem-448	64	7	ces	ce	NOUN
eurjchem-448	64	8	were	be	AUX
eurjchem-448	64	9	prepared	prepare	VERB
eurjchem-448	64	10	in	in	ADP
eurjchem-448	64	11	dmso	dmso	NOUN
eurjchem-448	64	12	according	accord	VERB
eurjchem-448	64	13	to	to	ADP
eurjchem-448	64	14	required	require	VERB
eurjchem-448	64	15	concentrations	concentration	NOUN
eurjchem-448	64	16	for	for	ADP
eurjchem-448	64	17	experiments	experiment	NOUN
eurjchem-448	64	18	.	.	PUNCT
eurjchem-448	65	1	to	to	PART
eurjchem-448	65	2	ensure	ensure	VERB
eurjchem-448	65	3	the	the	DET
eurjchem-448	65	4	effect	effect	NOUN
eurjchem-448	65	5	of	of	ADP
eurjchem-448	65	6	solvent	solvent	NOUN
eurjchem-448	65	7	on	on	ADP
eurjchem-448	65	8	bacterial	bacterial	ADJ
eurjchem-448	65	9	growth	growth	NOUN
eurjchem-448	65	10	,	,	PUNCT
eurjchem-448	65	11	a	a	DET
eurjchem-448	65	12	control	control	NOUN
eurjchem-448	65	13	test	test	NOUN
eurjchem-448	65	14	was	be	AUX
eurjchem-448	65	15	performed	perform	VERB
eurjchem-448	65	16	with	with	ADP
eurjchem-448	65	17	test	test	NOUN
eurjchem-448	65	18	medium	medium	NOUN
eurjchem-448	65	19	supplemented	supplement	VERB
eurjchem-448	65	20	with	with	ADP
eurjchem-448	65	21	dmso	dmso	NOUN
eurjchem-448	65	22	.	.	PUNCT
eurjchem-448	66	1	growth	growth	NOUN
eurjchem-448	66	2	of	of	ADP
eurjchem-448	66	3	fungus	fungus	NOUN
eurjchem-448	66	4	was	be	AUX
eurjchem-448	66	5	measured	measure	VERB
eurjchem-448	66	6	by	by	ADP
eurjchem-448	66	7	reading	read	VERB
eurjchem-448	66	8	diameter	diameter	NOUN
eurjchem-448	66	9	of	of	ADP
eurjchem-448	66	10	fungal	fungal	ADJ
eurjchem-448	66	11	colony	colony	NOUN
eurjchem-448	66	12	.	.	PUNCT
eurjchem-448	67	1	screening	screen	VERB
eurjchem-448	67	2	for	for	ADP
eurjchem-448	67	3	antifungal	antifungal	ADJ
eurjchem-448	67	4	activities	activity	NOUN
eurjchem-448	67	5	was	be	AUX
eurjchem-448	67	6	carried	carry	VERB
eurjchem-448	67	7	out	out	ADP
eurjchem-448	67	8	in	in	ADP
eurjchem-448	67	9	vitro	vitro	X
eurjchem-448	67	10	against	against	ADP
eurjchem-448	67	11	aspergillus‐niger	aspergillus‐niger	PROPN
eurjchem-448	67	12	,	,	PUNCT
eurjchem-448	67	13	following	follow	VERB
eurjchem-448	67	14	the	the	DET
eurjchem-448	67	15	procedure	procedure	NOUN
eurjchem-448	67	16	outlined	outline	VERB
eurjchem-448	67	17	[	[	X
eurjchem-448	67	18	8	8	NUM
eurjchem-448	67	19	]	]	PUNCT
eurjchem-448	67	20	and	and	CCONJ
eurjchem-448	67	21	their	their	PRON
eurjchem-448	67	22	relative	relative	ADJ
eurjchem-448	67	23	inhibitory	inhibitory	ADJ
eurjchem-448	67	24	ratios	ratio	NOUN
eurjchem-448	67	25	(	(	PUNCT
eurjchem-448	67	26	%	%	INTJ
eurjchem-448	67	27	)	)	PUNCT
eurjchem-448	67	28	were	be	AUX
eurjchem-448	67	29	determined	determine	VERB
eurjchem-448	67	30	using	use	VERB
eurjchem-448	67	31	mycelium	mycelium	NOUN
eurjchem-448	67	32	growth	growth	NOUN
eurjchem-448	67	33	rate	rate	NOUN
eurjchem-448	67	34	method	method	NOUN
eurjchem-448	67	35	.	.	PUNCT
eurjchem-448	68	1	on	on	ADP
eurjchem-448	68	2	complete	complete	ADJ
eurjchem-448	68	3	mycelia	mycelium	NOUN
eurjchem-448	68	4	growth	growth	NOUN
eurjchem-448	68	5	,	,	PUNCT
eurjchem-448	68	6	its	its	PRON
eurjchem-448	68	7	diameters	diameter	NOUN
eurjchem-448	68	8	were	be	AUX
eurjchem-448	68	9	measured	measure	VERB
eurjchem-448	68	10	and	and	CCONJ
eurjchem-448	68	11	inhibition	inhibition	NOUN
eurjchem-448	68	12	rate	rate	NOUN
eurjchem-448	68	13	was	be	AUX
eurjchem-448	68	14	calculated	calculate	VERB
eurjchem-448	68	15	according	accord	VERB
eurjchem-448	68	16	to	to	ADP
eurjchem-448	68	17	equation	equation	NOUN
eurjchem-448	68	18	1	1	NUM
eurjchem-448	68	19	.	.	PUNCT
eurjchem-448	69	1	kumar	kumar	PROPN
eurjchem-448	69	2	et	et	PROPN
eurjchem-448	69	3	al	al	PROPN
eurjchem-448	69	4	.	.	PUNCT
eurjchem-448	69	5	/	/	SYM
eurjchem-448	69	6	european	european	PROPN
eurjchem-448	69	7	journal	journal	PROPN
eurjchem-448	69	8	of	of	ADP
eurjchem-448	69	9	chemistry	chemistry	NOUN
eurjchem-448	69	10	3	3	NUM
eurjchem-448	69	11	(	(	PUNCT
eurjchem-448	69	12	1	1	NUM
eurjchem-448	69	13	)	)	PUNCT
eurjchem-448	69	14	(	(	PUNCT
eurjchem-448	69	15	2012	2012	NUM
eurjchem-448	69	16	)	)	PUNCT
eurjchem-448	69	17	57‐64	57‐64	NUM
eurjchem-448	69	18	59	59	NUM
eurjchem-448	70	1	i	i	NOUN
eurjchem-448	70	2	=	=	NOUN
eurjchem-448	70	3	100	100	NUM
eurjchem-448	70	4	)	)	PUNCT
eurjchem-448	70	5	(	(	PUNCT
eurjchem-448	70	6			AUX
eurjchem-448	70	7			VERB
eurjchem-448	70	8	i	i	PRON
eurjchem-448	70	9	oi	oi	VERB
eurjchem-448	71	1	d	d	X
eurjchem-448	71	2	dd	dd	PROPN
eurjchem-448	71	3	(	(	PUNCT
eurjchem-448	71	4	1	1	NUM
eurjchem-448	71	5	)	)	PUNCT
eurjchem-448	71	6	where	where	SCONJ
eurjchem-448	71	7	i	i	PRON
eurjchem-448	71	8	is	be	AUX
eurjchem-448	71	9	inhibition	inhibition	NOUN
eurjchem-448	71	10	rate	rate	NOUN
eurjchem-448	71	11	,	,	PUNCT
eurjchem-448	71	12	di	di	X
eurjchem-448	71	13	is	be	AUX
eurjchem-448	71	14	average	average	ADJ
eurjchem-448	71	15	diameter	diameter	NOUN
eurjchem-448	71	16	of	of	ADP
eurjchem-448	71	17	mycelia	mycelia	NOUN
eurjchem-448	71	18	in	in	ADP
eurjchem-448	71	19	the	the	DET
eurjchem-448	71	20	blank	blank	ADJ
eurjchem-448	71	21	test	test	NOUN
eurjchem-448	71	22	and	and	CCONJ
eurjchem-448	71	23	do	do	VERB
eurjchem-448	71	24	being	be	AUX
eurjchem-448	71	25	average	average	ADJ
eurjchem-448	71	26	diameter	diameter	NOUN
eurjchem-448	71	27	of	of	ADP
eurjchem-448	71	28	mycelia	mycelia	NOUN
eurjchem-448	71	29	in	in	ADP
eurjchem-448	71	30	presence	presence	NOUN
eurjchem-448	71	31	of	of	ADP
eurjchem-448	71	32	ces	ces	X
eurjchem-448	71	33	.	.	NOUN
eurjchem-448	71	34	3	3	NUM
eurjchem-448	71	35	.	.	NOUN
eurjchem-448	71	36	results	result	NOUN
eurjchem-448	71	37	and	and	CCONJ
eurjchem-448	71	38	discussion	discussion	NOUN
eurjchem-448	71	39	3.1	3.1	NUM
eurjchem-448	71	40	.	.	PUNCT
eurjchem-448	72	1	characterization	characterization	NOUN
eurjchem-448	72	2	of	of	ADP
eurjchem-448	72	3	mc	mc	PROPN
eurjchem-448	72	4	3.1.1	3.1.1	NUM
eurjchem-448	72	5	.	.	PUNCT
eurjchem-448	73	1	ir	ir	PROPN
eurjchem-448	73	2	spectrum	spectrum	NOUN
eurjchem-448	73	3	of	of	ADP
eurjchem-448	73	4	mc	mc	PROPN
eurjchem-448	73	5	no	no	DET
eurjchem-448	73	6	pair	pair	NOUN
eurjchem-448	73	7	of	of	ADP
eurjchem-448	73	8	bands	band	NOUN
eurjchem-448	73	9	appeared	appear	VERB
eurjchem-448	73	10	in	in	ADP
eurjchem-448	73	11	infrared	infrared	ADJ
eurjchem-448	73	12	spectrum	spectrum	NOUN
eurjchem-448	73	13	of	of	ADP
eurjchem-448	73	14	mc	mc	PROPN
eurjchem-448	73	15	at	at	ADP
eurjchem-448	73	16	3352‐3349	3352‐3349	NUM
eurjchem-448	73	17	and	and	CCONJ
eurjchem-448	73	18	1685	1685	NUM
eurjchem-448	73	19	cm‐1	cm‐1	NOUN
eurjchem-448	73	20	corresponding	correspond	VERB
eurjchem-448	73	21	to	to	ADP
eurjchem-448	73	22	ν(‐nh2	ν(‐nh2	PROPN
eurjchem-448	73	23	)	)	PUNCT
eurjchem-448	73	24	group	group	NOUN
eurjchem-448	73	25	of	of	ADP
eurjchem-448	73	26	1,5‐bis(o‐aminothiol)propane	1,5‐bis(o‐aminothiol)propane	PROPN
eurjchem-448	73	27	and	and	CCONJ
eurjchem-448	73	28	ν(>c	ν(>c	NOUN
eurjchem-448	73	29	=	=	SYM
eurjchem-448	73	30	o	o	NOUN
eurjchem-448	73	31	)	)	PUNCT
eurjchem-448	73	32	group	group	NOUN
eurjchem-448	73	33	of	of	ADP
eurjchem-448	73	34	1,5‐bis(2‐	1,5‐bis(2‐	NUM
eurjchem-448	73	35	formylphenyl)‐1,5‐dithiapropane	formylphenyl)‐1,5‐dithiapropane	NOUN
eurjchem-448	73	36	confirmed	confirm	VERB
eurjchem-448	73	37	condensation	condensation	NOUN
eurjchem-448	73	38	.	.	PUNCT
eurjchem-448	74	1	new	new	ADJ
eurjchem-448	74	2	medium	medium	NOUN
eurjchem-448	74	3	to	to	ADP
eurjchem-448	74	4	strong	strong	ADJ
eurjchem-448	74	5	stretching	stretching	NOUN
eurjchem-448	74	6	vibration	vibration	NOUN
eurjchem-448	74	7	at	at	ADP
eurjchem-448	74	8	1611	1611	NUM
eurjchem-448	74	9	cm‐1	cm‐1	NOUN
eurjchem-448	74	10	assigned	assign	VERB
eurjchem-448	74	11	to	to	ADP
eurjchem-448	74	12	ν(‐ch	ν(‐ch	NOUN
eurjchem-448	74	13	=	=	NOUN
eurjchem-448	74	14	n‐)(m	n‐)(m	NOUN
eurjchem-448	74	15	)	)	PUNCT
eurjchem-448	74	16	appeared	appear	VERB
eurjchem-448	74	17	[	[	X
eurjchem-448	74	18	9	9	NUM
eurjchem-448	74	19	]	]	PUNCT
eurjchem-448	74	20	.	.	PUNCT
eurjchem-448	75	1	the	the	DET
eurjchem-448	75	2	characteristic	characteristic	ADJ
eurjchem-448	75	3	ν(‐	ν(‐	NUM
eurjchem-448	75	4	ch2‐	ch2‐	NOUN
eurjchem-448	75	5	)	)	PUNCT
eurjchem-448	75	6	modes	mode	NOUN
eurjchem-448	75	7	of	of	ADP
eurjchem-448	75	8	aliphatic	aliphatic	ADJ
eurjchem-448	75	9	groups	group	NOUN
eurjchem-448	75	10	were	be	AUX
eurjchem-448	75	11	observed	observe	VERB
eurjchem-448	75	12	in	in	ADP
eurjchem-448	75	13	the	the	DET
eurjchem-448	75	14	wave	wave	NOUN
eurjchem-448	75	15	region	region	NOUN
eurjchem-448	75	16	2951‐2920	2951‐2920	NUM
eurjchem-448	75	17	and	and	CCONJ
eurjchem-448	75	18	2891	2891	NUM
eurjchem-448	75	19	cm‐1	cm‐1	NOUN
eurjchem-448	75	20	.	.	PUNCT
eurjchem-448	76	1	a	a	DET
eurjchem-448	76	2	group	group	NOUN
eurjchem-448	76	3	of	of	ADP
eurjchem-448	76	4	strong	strong	ADJ
eurjchem-448	76	5	to	to	PART
eurjchem-448	76	6	medium	medium	ADJ
eurjchem-448	76	7	intense	intense	ADJ
eurjchem-448	76	8	bands	band	NOUN
eurjchem-448	76	9	were	be	AUX
eurjchem-448	76	10	found	find	VERB
eurjchem-448	76	11	in	in	ADP
eurjchem-448	76	12	different	different	ADJ
eurjchem-448	76	13	wave	wave	NOUN
eurjchem-448	76	14	regions	region	NOUN
eurjchem-448	76	15	3051‐3050	3051‐3050	NUM
eurjchem-448	76	16	,	,	PUNCT
eurjchem-448	76	17	1572‐1550	1572‐1550	NUM
eurjchem-448	76	18	,	,	PUNCT
eurjchem-448	76	19	1165‐1140	1165‐1140	NUM
eurjchem-448	76	20	and	and	CCONJ
eurjchem-448	76	21	771‐760	771‐760	NUM
eurjchem-448	76	22	cm‐1	cm‐1	NOUN
eurjchem-448	76	23	,	,	PUNCT
eurjchem-448	76	24	due	due	ADP
eurjchem-448	76	25	to	to	ADP
eurjchem-448	76	26	ν(ar‐ch‐	ν(ar‐ch‐	NOUN
eurjchem-448	76	27	)	)	PUNCT
eurjchem-448	76	28	aromatic	aromatic	ADJ
eurjchem-448	76	29	stretching	stretching	NOUN
eurjchem-448	76	30	vibrations	vibration	NOUN
eurjchem-448	76	31	.	.	PUNCT
eurjchem-448	77	1	another	another	PRON
eurjchem-448	77	2	strong	strong	ADJ
eurjchem-448	77	3	to	to	ADP
eurjchem-448	77	4	medium	medium	ADJ
eurjchem-448	77	5	stretching	stretch	VERB
eurjchem-448	77	6	frequency	frequency	NOUN
eurjchem-448	77	7	bands	band	NOUN
eurjchem-448	77	8	were	be	AUX
eurjchem-448	77	9	observed	observe	VERB
eurjchem-448	77	10	at	at	ADP
eurjchem-448	77	11	810‐801	810‐801	PROPN
eurjchem-448	77	12	cm‐1	cm‐1	PROPN
eurjchem-448	77	13	corresponding	correspond	VERB
eurjchem-448	77	14	to	to	ADP
eurjchem-448	77	15	ν(c‐s	ν(c‐s	NUM
eurjchem-448	77	16	)	)	PUNCT
eurjchem-448	77	17	characteristic	characteristic	ADJ
eurjchem-448	77	18	stretching	stretching	NOUN
eurjchem-448	77	19	modes	mode	NOUN
eurjchem-448	77	20	[	[	X
eurjchem-448	77	21	10	10	NUM
eurjchem-448	77	22	]	]	PUNCT
eurjchem-448	77	23	.	.	PUNCT
eurjchem-448	78	1	ft‐ir	ft‐ir	NOUN
eurjchem-448	78	2	spectrum	spectrum	NOUN
eurjchem-448	78	3	of	of	ADP
eurjchem-448	78	4	mc	mc	PROPN
eurjchem-448	78	5	have	have	VERB
eurjchem-448	78	6	all	all	DET
eurjchem-448	78	7	typical	typical	ADJ
eurjchem-448	78	8	features	feature	NOUN
eurjchem-448	78	9	as	as	SCONJ
eurjchem-448	78	10	given	give	VERB
eurjchem-448	78	11	above	above	ADV
eurjchem-448	78	12	were	be	AUX
eurjchem-448	78	13	clearly	clearly	ADV
eurjchem-448	78	14	compatible	compatible	ADJ
eurjchem-448	78	15	with	with	ADP
eurjchem-448	78	16	the	the	DET
eurjchem-448	78	17	structural	structural	ADJ
eurjchem-448	78	18	model	model	NOUN
eurjchem-448	78	19	of	of	ADP
eurjchem-448	78	20	mc	mc	PROPN
eurjchem-448	78	21	.	.	PROPN
eurjchem-448	78	22	3.1.2	3.1.2	NUM
eurjchem-448	78	23	.	.	NOUN
eurjchem-448	79	1	1h	1h	NUM
eurjchem-448	79	2	nmr	nmr	NOUN
eurjchem-448	79	3	spectrum	spectrum	NOUN
eurjchem-448	79	4	of	of	ADP
eurjchem-448	79	5	mc	mc	PROPN
eurjchem-448	79	6	1h	1h	NUM
eurjchem-448	79	7	nmr	nmr	PROPN
eurjchem-448	79	8	spectrum	spectrum	NOUN
eurjchem-448	79	9	of	of	ADP
eurjchem-448	79	10	mc	mc	PROPN
eurjchem-448	79	11	do	do	AUX
eurjchem-448	79	12	not	not	PART
eurjchem-448	79	13	give	give	VERB
eurjchem-448	79	14	any	any	DET
eurjchem-448	79	15	signal	signal	NOUN
eurjchem-448	79	16	corresponding	correspond	VERB
eurjchem-448	79	17	to	to	ADP
eurjchem-448	79	18	primary	primary	ADJ
eurjchem-448	79	19	amine	amine	NOUN
eurjchem-448	79	20	(	(	PUNCT
eurjchem-448	79	21	‐nh2	‐nh2	NUM
eurjchem-448	79	22	)	)	PUNCT
eurjchem-448	79	23	at	at	ADP
eurjchem-448	79	24	6.7	6.7	NUM
eurjchem-448	79	25	ppm	ppm	NOUN
eurjchem-448	79	26	and	and	CCONJ
eurjchem-448	79	27	carbonyl	carbonyl	NOUN
eurjchem-448	79	28	(	(	PUNCT
eurjchem-448	79	29	‐hc	‐hc	NOUN
eurjchem-448	79	30	=	=	SYM
eurjchem-448	79	31	o	o	NOUN
eurjchem-448	79	32	)	)	PUNCT
eurjchem-448	79	33	protons	proton	NOUN
eurjchem-448	79	34	at	at	ADP
eurjchem-448	79	35	9.1	9.1	NUM
eurjchem-448	79	36	ppm	ppm	NOUN
eurjchem-448	79	37	confirmed	confirm	VERB
eurjchem-448	79	38	complete	complete	ADJ
eurjchem-448	79	39	condensation	condensation	NOUN
eurjchem-448	79	40	.	.	PUNCT
eurjchem-448	80	1	earlier	early	ADJ
eurjchem-448	80	2	evidences	evidence	NOUN
eurjchem-448	80	3	obtained	obtain	VERB
eurjchem-448	80	4	from	from	ADP
eurjchem-448	80	5	infrared	infrared	ADJ
eurjchem-448	80	6	spectrum	spectrum	NOUN
eurjchem-448	80	7	have	have	AUX
eurjchem-448	80	8	also	also	ADV
eurjchem-448	80	9	suggested	suggest	VERB
eurjchem-448	80	10	cyclic	cyclic	ADJ
eurjchem-448	80	11	nature	nature	NOUN
eurjchem-448	80	12	of	of	ADP
eurjchem-448	80	13	ligand	ligand	NOUN
eurjchem-448	80	14	.	.	PUNCT
eurjchem-448	81	1	in	in	ADP
eurjchem-448	81	2	addition	addition	NOUN
eurjchem-448	81	3	,	,	PUNCT
eurjchem-448	81	4	methylene	methylene	NOUN
eurjchem-448	81	5	chains	chain	NOUN
eurjchem-448	81	6	(	(	PUNCT
eurjchem-448	81	7	‐ch2‐	‐ch2‐	NOUN
eurjchem-448	81	8	)	)	PUNCT
eurjchem-448	81	9	were	be	AUX
eurjchem-448	81	10	detected	detect	VERB
eurjchem-448	81	11	as	as	ADP
eurjchem-448	81	12	a	a	DET
eurjchem-448	81	13	bridge	bridge	NOUN
eurjchem-448	81	14	between	between	ADP
eurjchem-448	81	15	two	two	NUM
eurjchem-448	81	16	sulphur	sulphur	NOUN
eurjchem-448	81	17	atoms	atom	NOUN
eurjchem-448	81	18	at	at	ADP
eurjchem-448	81	19	2.70‐2.60	2.70‐2.60	NUM
eurjchem-448	81	20	ppm	ppm	NOUN
eurjchem-448	81	21	.	.	PUNCT
eurjchem-448	82	1	other	other	ADJ
eurjchem-448	82	2	multiplets	multiplet	NOUN
eurjchem-448	82	3	were	be	AUX
eurjchem-448	82	4	observed	observe	VERB
eurjchem-448	82	5	at	at	ADP
eurjchem-448	82	6	8.40‐7.33	8.40‐7.33	NUM
eurjchem-448	82	7	ppm	ppm	NOUN
eurjchem-448	82	8	(	(	PUNCT
eurjchem-448	82	9	m	m	PROPN
eurjchem-448	82	10	,	,	PUNCT
eurjchem-448	82	11	j	j	PROPN
eurjchem-448	82	12	=	=	SYM
eurjchem-448	82	13	8	8	NUM
eurjchem-448	82	14	hz	hz	NOUN
eurjchem-448	82	15	)	)	PUNCT
eurjchem-448	82	16	confirming	confirm	VERB
eurjchem-448	82	17	the	the	DET
eurjchem-448	82	18	presence	presence	NOUN
eurjchem-448	82	19	of	of	ADP
eurjchem-448	82	20	‐c6h4‐.	‐c6h4‐.	PROPN
eurjchem-448	82	21	another	another	DET
eurjchem-448	82	22	important	important	ADJ
eurjchem-448	82	23	signals	signal	NOUN
eurjchem-448	82	24	were	be	AUX
eurjchem-448	82	25	observed	observe	VERB
eurjchem-448	82	26	at	at	ADP
eurjchem-448	82	27	9.60‐9.50	9.60‐9.50	NUM
eurjchem-448	82	28	and	and	CCONJ
eurjchem-448	82	29	2.96‐2.90	2.96‐2.90	NUM
eurjchem-448	82	30	ppm	ppm	NOUN
eurjchem-448	82	31	due	due	ADP
eurjchem-448	82	32	to	to	ADP
eurjchem-448	82	33	the	the	DET
eurjchem-448	82	34	presence	presence	NOUN
eurjchem-448	82	35	of	of	ADP
eurjchem-448	82	36	azomethine	azomethine	PROPN
eurjchem-448	82	37	(	(	PUNCT
eurjchem-448	82	38	‐hc	‐hc	NOUN
eurjchem-448	82	39	=	=	NOUN
eurjchem-448	82	40	n‐	n‐	NOUN
eurjchem-448	82	41	)	)	PUNCT
eurjchem-448	82	42	and	and	CCONJ
eurjchem-448	82	43	sulphur	sulphur	NOUN
eurjchem-448	82	44	(	(	PUNCT
eurjchem-448	82	45	‐ch2‐s‐	‐ch2‐s‐	NOUN
eurjchem-448	82	46	)	)	PUNCT
eurjchem-448	82	47	protons	proton	NOUN
eurjchem-448	82	48	,	,	PUNCT
eurjchem-448	82	49	respectively	respectively	ADV
eurjchem-448	82	50	.	.	PUNCT
eurjchem-448	83	1	the	the	DET
eurjchem-448	83	2	occurrence	occurrence	NOUN
eurjchem-448	83	3	of	of	ADP
eurjchem-448	83	4	this	this	DET
eurjchem-448	83	5	resonance	resonance	NOUN
eurjchem-448	83	6	in	in	ADP
eurjchem-448	83	7	each	each	PRON
eurjchem-448	83	8	of	of	ADP
eurjchem-448	83	9	the	the	DET
eurjchem-448	83	10	above	above	ADJ
eurjchem-448	83	11	species	specie	NOUN
eurjchem-448	83	12	as	as	ADP
eurjchem-448	83	13	a	a	DET
eurjchem-448	83	14	‘	'	PUNCT
eurjchem-448	83	15	clean	clean	ADJ
eurjchem-448	83	16	’	'	PUNCT
eurjchem-448	83	17	singlet	singlet	NOUN
eurjchem-448	83	18	confirms	confirm	VERB
eurjchem-448	83	19	the	the	DET
eurjchem-448	83	20	presence	presence	NOUN
eurjchem-448	83	21	of	of	ADP
eurjchem-448	83	22	intact	intact	ADJ
eurjchem-448	83	23	(	(	PUNCT
eurjchem-448	83	24	non	non	X
eurjchem-448	83	25	hydrolyzed	hydrolyzed	ADJ
eurjchem-448	83	26	)	)	PUNCT
eurjchem-448	83	27	imine	imine	NOUN
eurjchem-448	83	28	groups	group	NOUN
eurjchem-448	83	29	in	in	ADP
eurjchem-448	83	30	each	each	DET
eurjchem-448	83	31	case	case	NOUN
eurjchem-448	83	32	[	[	X
eurjchem-448	83	33	11	11	NUM
eurjchem-448	83	34	]	]	PUNCT
eurjchem-448	83	35	.	.	PUNCT
eurjchem-448	84	1	mc	mc	PROPN
eurjchem-448	84	2	is	be	AUX
eurjchem-448	84	3	soluble	soluble	ADJ
eurjchem-448	84	4	in	in	ADP
eurjchem-448	84	5	common	common	ADJ
eurjchem-448	84	6	organic	organic	ADJ
eurjchem-448	84	7	solvent	solvent	NOUN
eurjchem-448	84	8	such	such	ADJ
eurjchem-448	84	9	as	as	ADP
eurjchem-448	84	10	etoh	etoh	NOUN
eurjchem-448	84	11	(	(	PUNCT
eurjchem-448	84	12	40	40	NUM
eurjchem-448	84	13	oc	oc	NOUN
eurjchem-448	84	14	)	)	PUNCT
eurjchem-448	84	15	.	.	PUNCT
eurjchem-448	85	1	1h	1h	NUM
eurjchem-448	85	2	nmr	nmr	NOUN
eurjchem-448	85	3	(	(	PUNCT
eurjchem-448	85	4	200	200	NUM
eurjchem-448	85	5	mhz	mhz	NOUN
eurjchem-448	85	6	,	,	PUNCT
eurjchem-448	85	7	cdcl3	cdcl3	PROPN
eurjchem-448	85	8	,	,	PUNCT
eurjchem-448	85	9	δ	δ	PROPN
eurjchem-448	85	10	,	,	PUNCT
eurjchem-448	85	11	ppm	ppm	NOUN
eurjchem-448	85	12	):	):	PUNCT
eurjchem-448	85	13	9.60‐9.50	9.60‐9.50	NUM
eurjchem-448	85	14	(	(	PUNCT
eurjchem-448	85	15	s	s	PROPN
eurjchem-448	85	16	,	,	PUNCT
eurjchem-448	85	17	2h	2h	NUM
eurjchem-448	85	18	,	,	PUNCT
eurjchem-448	85	19	‐ch	‐ch	NOUN
eurjchem-448	85	20	=	=	SYM
eurjchem-448	85	21	n‐	n‐	NOUN
eurjchem-448	85	22	)	)	PUNCT
eurjchem-448	85	23	,	,	PUNCT
eurjchem-448	85	24	8.40‐7.33	8.40‐7.33	NUM
eurjchem-448	85	25	(	(	PUNCT
eurjchem-448	85	26	m	m	PROPN
eurjchem-448	85	27	,	,	PUNCT
eurjchem-448	85	28	16h	16h	NUM
eurjchem-448	85	29	,	,	PUNCT
eurjchem-448	85	30	j	j	PROPN
eurjchem-448	85	31	=	=	SYM
eurjchem-448	85	32	9.2	9.2	NUM
eurjchem-448	85	33	hz	hz	NOUN
eurjchem-448	85	34	,	,	PUNCT
eurjchem-448	85	35	‐c6h4‐	‐c6h4‐	PROPN
eurjchem-448	85	36	)	)	PUNCT
eurjchem-448	85	37	,	,	PUNCT
eurjchem-448	85	38	2.70‐2.60	2.70‐2.60	NUM
eurjchem-448	85	39	(	(	PUNCT
eurjchem-448	85	40	m	m	PROPN
eurjchem-448	85	41	,	,	PUNCT
eurjchem-448	85	42	4h	4h	NUM
eurjchem-448	85	43	,	,	PUNCT
eurjchem-448	85	44	j	j	PROPN
eurjchem-448	86	1	=	=	SYM
eurjchem-448	86	2	4.2	4.2	NUM
eurjchem-448	86	3	hz	hz	NOUN
eurjchem-448	86	4	,	,	PUNCT
eurjchem-448	86	5	‐ch2‐	‐ch2‐	PROPN
eurjchem-448	86	6	)	)	PUNCT
eurjchem-448	86	7	,	,	PUNCT
eurjchem-448	86	8	2.96‐2.90	2.96‐2.90	NUM
eurjchem-448	86	9	(	(	PUNCT
eurjchem-448	86	10	t	t	PROPN
eurjchem-448	86	11	,	,	PUNCT
eurjchem-448	86	12	8h	8h	NUM
eurjchem-448	86	13	,	,	PUNCT
eurjchem-448	86	14	j1	j1	PROPN
eurjchem-448	86	15	=	=	NUM
eurjchem-448	86	16	7.8	7.8	NUM
eurjchem-448	86	17	hz	hz	NOUN
eurjchem-448	86	18	,	,	PUNCT
eurjchem-448	86	19	j2	j2	PROPN
eurjchem-448	86	20	=	=	SYM
eurjchem-448	86	21	8.5	8.5	NUM
eurjchem-448	86	22	hz	hz	NOUN
eurjchem-448	86	23	,	,	PUNCT
eurjchem-448	86	24	‐s‐ch2‐	‐s‐ch2‐	NOUN
eurjchem-448	86	25	)	)	PUNCT
eurjchem-448	86	26	.	.	PUNCT
eurjchem-448	87	1	3.1.3	3.1.3	NUM
eurjchem-448	87	2	.	.	NOUN
eurjchem-448	87	3	13c	13c	NOUN
eurjchem-448	87	4	nmr	nmr	NOUN
eurjchem-448	87	5	spectrum	spectrum	NOUN
eurjchem-448	87	6	of	of	ADP
eurjchem-448	87	7	mc	mc	PROPN
eurjchem-448	87	8	13c	13c	PROPN
eurjchem-448	87	9	nmr	nmr	NOUN
eurjchem-448	87	10	spectrum	spectrum	NOUN
eurjchem-448	87	11	of	of	ADP
eurjchem-448	87	12	mc	mc	PROPN
eurjchem-448	87	13	displayed	display	VERB
eurjchem-448	87	14	strong	strong	ADJ
eurjchem-448	87	15	signals	signal	NOUN
eurjchem-448	87	16	at	at	ADP
eurjchem-448	87	17	δ	δ	PROPN
eurjchem-448	87	18	163.10‐161.02	163.10‐161.02	NUM
eurjchem-448	87	19	ppm	ppm	NOUN
eurjchem-448	87	20	and	and	CCONJ
eurjchem-448	87	21	δ	δ	PROPN
eurjchem-448	87	22	124.60‐121.10	124.60‐121.10	NUM
eurjchem-448	87	23	ppm	ppm	NOUN
eurjchem-448	87	24	due	due	ADP
eurjchem-448	87	25	to	to	ADP
eurjchem-448	87	26	the	the	DET
eurjchem-448	87	27	presence	presence	NOUN
eurjchem-448	87	28	of	of	ADP
eurjchem-448	87	29	‐ch	‐ch	NOUN
eurjchem-448	87	30	=	=	NOUN
eurjchem-448	87	31	n‐	n‐	NOUN
eurjchem-448	87	32	and	and	CCONJ
eurjchem-448	87	33	aromatic	aromatic	ADJ
eurjchem-448	87	34	carbon	carbon	NOUN
eurjchem-448	87	35	.	.	PUNCT
eurjchem-448	88	1	further	far	ADV
eurjchem-448	88	2	,	,	PUNCT
eurjchem-448	88	3	important	important	ADJ
eurjchem-448	88	4	signals	signal	NOUN
eurjchem-448	88	5	were	be	AUX
eurjchem-448	88	6	found	find	VERB
eurjchem-448	88	7	at	at	ADP
eurjchem-448	88	8	δ	δ	PROPN
eurjchem-448	88	9	34.20‐34.00	34.20‐34.00	NUM
eurjchem-448	88	10	ppm	ppm	NOUN
eurjchem-448	88	11	attributed	attribute	VERB
eurjchem-448	88	12	to	to	ADP
eurjchem-448	88	13	‐ch2‐	‐ch2‐	PROPN
eurjchem-448	88	14	[	[	X
eurjchem-448	88	15	12	12	NUM
eurjchem-448	88	16	]	]	PUNCT
eurjchem-448	88	17	.	.	PUNCT
eurjchem-448	89	1	13c	13c	NOUN
eurjchem-448	89	2	nmr	nmr	NOUN
eurjchem-448	89	3	(	(	PUNCT
eurjchem-448	89	4	125	125	NUM
eurjchem-448	89	5	mhz	mhz	NOUN
eurjchem-448	89	6	,	,	PUNCT
eurjchem-448	89	7	cdcl3	cdcl3	PROPN
eurjchem-448	89	8	,	,	PUNCT
eurjchem-448	89	9	δ	δ	PROPN
eurjchem-448	89	10	,	,	PUNCT
eurjchem-448	89	11	ppm	ppm	NUM
eurjchem-448	89	12	):	):	PUNCT
eurjchem-448	89	13	124.60‐121.10	124.60‐121.10	NUM
eurjchem-448	89	14	(	(	PUNCT
eurjchem-448	89	15	c	c	NOUN
eurjchem-448	89	16	:	:	PUNCT
eurjchem-448	89	17	2	2	NUM
eurjchem-448	89	18	,	,	PUNCT
eurjchem-448	89	19	3	3	NUM
eurjchem-448	89	20	,	,	PUNCT
eurjchem-448	89	21	4	4	NUM
eurjchem-448	89	22	,	,	PUNCT
eurjchem-448	89	23	5	5	NUM
eurjchem-448	89	24	,	,	PUNCT
eurjchem-448	89	25	8	8	NUM
eurjchem-448	89	26	,	,	PUNCT
eurjchem-448	89	27	9	9	NUM
eurjchem-448	89	28	,	,	PUNCT
eurjchem-448	89	29	10	10	NUM
eurjchem-448	89	30	,	,	PUNCT
eurjchem-448	89	31	11	11	NUM
eurjchem-448	89	32	,	,	PUNCT
eurjchem-448	89	33	12	12	NUM
eurjchem-448	89	34	,	,	PUNCT
eurjchem-448	89	35	18	18	NUM
eurjchem-448	89	36	,	,	PUNCT
eurjchem-448	89	37	19	19	NUM
eurjchem-448	89	38	,	,	PUNCT
eurjchem-448	89	39	20	20	NUM
eurjchem-448	89	40	,	,	PUNCT
eurjchem-448	89	41	21	21	NUM
eurjchem-448	89	42	,	,	PUNCT
eurjchem-448	89	43	22	22	NUM
eurjchem-448	89	44	,	,	PUNCT
eurjchem-448	89	45	25	25	NUM
eurjchem-448	89	46	,	,	PUNCT
eurjchem-448	89	47	26	26	NUM
eurjchem-448	89	48	,	,	PUNCT
eurjchem-448	89	49	27	27	NUM
eurjchem-448	89	50	,	,	PUNCT
eurjchem-448	89	51	28	28	NUM
eurjchem-448	89	52	)	)	PUNCT
eurjchem-448	89	53	,	,	PUNCT
eurjchem-448	89	54	131.01‐	131.01‐	ADV
eurjchem-448	89	55	129.64	129.64	NUM
eurjchem-448	89	56	(	(	PUNCT
eurjchem-448	89	57	c	c	NOUN
eurjchem-448	89	58	:	:	PUNCT
eurjchem-448	89	59	1	1	NUM
eurjchem-448	89	60	,	,	PUNCT
eurjchem-448	89	61	13	13	NUM
eurjchem-448	89	62	,	,	PUNCT
eurjchem-448	89	63	17	17	NUM
eurjchem-448	89	64	,	,	PUNCT
eurjchem-448	89	65	29	29	NUM
eurjchem-448	89	66	)	)	PUNCT
eurjchem-448	89	67	,	,	PUNCT
eurjchem-448	89	68	129.23‐128.02	129.23‐128.02	NUM
eurjchem-448	89	69	(	(	PUNCT
eurjchem-448	89	70	c	c	NOUN
eurjchem-448	89	71	:	:	PUNCT
eurjchem-448	89	72	14	14	NUM
eurjchem-448	89	73	,	,	PUNCT
eurjchem-448	89	74	16	16	NUM
eurjchem-448	89	75	,	,	PUNCT
eurjchem-448	89	76	30	30	NUM
eurjchem-448	89	77	,	,	PUNCT
eurjchem-448	89	78	32	32	NUM
eurjchem-448	89	79	)	)	PUNCT
eurjchem-448	89	80	,	,	PUNCT
eurjchem-448	89	81	163.10‐161.02	163.10‐161.02	NUM
eurjchem-448	89	82	(	(	PUNCT
eurjchem-448	89	83	c	c	NOUN
eurjchem-448	89	84	:	:	PUNCT
eurjchem-448	89	85	7	7	NUM
eurjchem-448	89	86	,	,	PUNCT
eurjchem-448	89	87	23	23	NUM
eurjchem-448	89	88	)	)	PUNCT
eurjchem-448	89	89	,	,	PUNCT
eurjchem-448	89	90	151.01‐150.92	151.01‐150.92	NUM
eurjchem-448	89	91	(	(	PUNCT
eurjchem-448	89	92	c	c	NOUN
eurjchem-448	89	93	:	:	PUNCT
eurjchem-448	89	94	6	6	NUM
eurjchem-448	89	95	,	,	PUNCT
eurjchem-448	89	96	24	24	NUM
eurjchem-448	89	97	)	)	PUNCT
eurjchem-448	89	98	,	,	PUNCT
eurjchem-448	89	99	34.20‐34.00	34.20‐34.00	NUM
eurjchem-448	89	100	(	(	PUNCT
eurjchem-448	89	101	c	c	NOUN
eurjchem-448	89	102	:	:	PUNCT
eurjchem-448	89	103	15	15	NUM
eurjchem-448	89	104	,	,	PUNCT
eurjchem-448	89	105	31	31	NUM
eurjchem-448	89	106	)	)	PUNCT
eurjchem-448	89	107	.	.	PUNCT
eurjchem-448	90	1	3.1.4	3.1.4	NUM
eurjchem-448	90	2	.	.	PUNCT
eurjchem-448	90	3	electron	electron	NOUN
eurjchem-448	90	4	impact	impact	NOUN
eurjchem-448	90	5	(	(	PUNCT
eurjchem-448	90	6	ei	ei	NOUN
eurjchem-448	90	7	)	)	PUNCT
eurjchem-448	90	8	mass	mass	NOUN
eurjchem-448	90	9	spectrum	spectrum	NOUN
eurjchem-448	90	10	of	of	ADP
eurjchem-448	90	11	mc	mc	PROPN
eurjchem-448	90	12	in	in	ADP
eurjchem-448	90	13	the	the	DET
eurjchem-448	90	14	mass	mass	NOUN
eurjchem-448	90	15	spectrum	spectrum	NOUN
eurjchem-448	90	16	,	,	PUNCT
eurjchem-448	90	17	different	different	ADJ
eurjchem-448	90	18	intensities	intensity	NOUN
eurjchem-448	90	19	were	be	AUX
eurjchem-448	90	20	observed	observe	VERB
eurjchem-448	90	21	corresponding	correspond	VERB
eurjchem-448	90	22	to	to	ADP
eurjchem-448	90	23	various	various	ADJ
eurjchem-448	90	24	fragments	fragment	NOUN
eurjchem-448	90	25	of	of	ADP
eurjchem-448	90	26	mc	mc	PROPN
eurjchem-448	90	27	directly	directly	ADV
eurjchem-448	90	28	reflecting	reflect	VERB
eurjchem-448	90	29	with	with	ADP
eurjchem-448	90	30	their	their	PRON
eurjchem-448	90	31	stabilities	stability	NOUN
eurjchem-448	90	32	.	.	PUNCT
eurjchem-448	91	1	the	the	DET
eurjchem-448	91	2	base	base	NOUN
eurjchem-448	91	3	peak	peak	NOUN
eurjchem-448	91	4	(	(	PUNCT
eurjchem-448	91	5	100	100	NUM
eurjchem-448	91	6	%	%	NOUN
eurjchem-448	91	7	)	)	PUNCT
eurjchem-448	91	8	m+	m+	NUM
eurjchem-448	91	9	indicated	indicate	VERB
eurjchem-448	91	10	facile	facile	ADJ
eurjchem-448	91	11	loss	loss	NOUN
eurjchem-448	91	12	of	of	ADP
eurjchem-448	91	13	hydrogen	hydrogen	NOUN
eurjchem-448	91	14	radical	radical	NOUN
eurjchem-448	91	15	,	,	PUNCT
eurjchem-448	91	16	a	a	DET
eurjchem-448	91	17	molecular	molecular	ADJ
eurjchem-448	91	18	ion	ion	NOUN
eurjchem-448	91	19	peak	peak	NOUN
eurjchem-448	91	20	ms	ms	PROPN
eurjchem-448	91	21	(	(	PUNCT
eurjchem-448	91	22	ei	ei	PROPN
eurjchem-448	91	23	,	,	PUNCT
eurjchem-448	91	24	m	m	PROPN
eurjchem-448	91	25	/	/	SYM
eurjchem-448	91	26	z	z	PROPN
eurjchem-448	91	27	(	(	PUNCT
eurjchem-448	91	28	%	%	NOUN
eurjchem-448	91	29	)	)	PUNCT
eurjchem-448	91	30	):	):	PUNCT
eurjchem-448	91	31	569	569	NUM
eurjchem-448	91	32	(	(	PUNCT
eurjchem-448	91	33	m+	m+	NOUN
eurjchem-448	91	34	)	)	PUNCT
eurjchem-448	91	35	corresponds	correspond	VERB
eurjchem-448	91	36	to	to	ADP
eurjchem-448	91	37	molecular	molecular	ADJ
eurjchem-448	91	38	weight	weight	NOUN
eurjchem-448	91	39	of	of	ADP
eurjchem-448	91	40	mc	mc	PROPN
eurjchem-448	91	41	.	.	PUNCT
eurjchem-448	92	1	a	a	DET
eurjchem-448	92	2	general	general	ADJ
eurjchem-448	92	3	fragmentation	fragmentation	NOUN
eurjchem-448	92	4	pattern	pattern	NOUN
eurjchem-448	92	5	evidenced	evidence	VERB
eurjchem-448	92	6	primary	primary	ADJ
eurjchem-448	92	7	cleavages	cleavage	NOUN
eurjchem-448	92	8	at	at	ADP
eurjchem-448	92	9	hetero‐	hetero‐	PROPN
eurjchem-448	92	10	carbon	carbon	NOUN
eurjchem-448	92	11	bonds	bond	NOUN
eurjchem-448	92	12	.	.	PUNCT
eurjchem-448	93	1	beside	beside	ADP
eurjchem-448	93	2	this	this	DET
eurjchem-448	93	3	several	several	ADJ
eurjchem-448	93	4	other	other	ADJ
eurjchem-448	93	5	peaks	peak	NOUN
eurjchem-448	93	6	of	of	ADP
eurjchem-448	93	7	different	different	ADJ
eurjchem-448	93	8	intensities	intensity	NOUN
eurjchem-448	93	9	were	be	AUX
eurjchem-448	93	10	observed	observe	VERB
eurjchem-448	93	11	having	have	VERB
eurjchem-448	93	12	corresponding	correspond	VERB
eurjchem-448	93	13	m	m	PROPN
eurjchem-448	93	14	/	/	SYM
eurjchem-448	93	15	z	z	NOUN
eurjchem-448	93	16	values	value	NOUN
eurjchem-448	93	17	according	accord	VERB
eurjchem-448	93	18	to	to	ADP
eurjchem-448	93	19	the	the	DET
eurjchem-448	93	20	molecular	molecular	ADJ
eurjchem-448	93	21	masses	masse	NOUN
eurjchem-448	93	22	of	of	ADP
eurjchem-448	93	23	different	different	ADJ
eurjchem-448	93	24	constituents	constituent	NOUN
eurjchem-448	93	25	[	[	X
eurjchem-448	93	26	13	13	NUM
eurjchem-448	93	27	]	]	PUNCT
eurjchem-448	93	28	.	.	PUNCT
eurjchem-448	94	1	initiation	initiation	NOUN
eurjchem-448	94	2	in	in	ADP
eurjchem-448	94	3	the	the	DET
eurjchem-448	94	4	cleavage	cleavage	NOUN
eurjchem-448	94	5	in	in	ADP
eurjchem-448	94	6	form	form	NOUN
eurjchem-448	94	7	of	of	ADP
eurjchem-448	94	8	different	different	ADJ
eurjchem-448	94	9	pathways	pathway	NOUN
eurjchem-448	94	10	took	take	VERB
eurjchem-448	94	11	place	place	NOUN
eurjchem-448	94	12	through	through	ADP
eurjchem-448	94	13	the	the	DET
eurjchem-448	94	14	loss	loss	NOUN
eurjchem-448	94	15	of	of	ADP
eurjchem-448	94	16	fragment	fragment	NOUN
eurjchem-448	94	17	(	(	PUNCT
eurjchem-448	94	18	‐s‐ch2‐ch2‐	‐s‐ch2‐ch2‐	NUM
eurjchem-448	94	19	)	)	PUNCT
eurjchem-448	94	20	from	from	ADP
eurjchem-448	94	21	the	the	DET
eurjchem-448	94	22	parent	parent	NOUN
eurjchem-448	94	23	molecule	molecule	NOUN
eurjchem-448	94	24	,	,	PUNCT
eurjchem-448	94	25	followed	follow	VERB
eurjchem-448	94	26	by	by	ADP
eurjchem-448	94	27	‐s‐ch2‐	‐s‐ch2‐	ADJ
eurjchem-448	94	28	elimination	elimination	NOUN
eurjchem-448	94	29	as	as	ADP
eurjchem-448	94	30	evident	evident	ADJ
eurjchem-448	94	31	in	in	ADP
eurjchem-448	94	32	mass	mass	ADJ
eurjchem-448	94	33	spectrum	spectrum	NOUN
eurjchem-448	94	34	obtained	obtain	VERB
eurjchem-448	94	35	.	.	PUNCT
eurjchem-448	95	1	in	in	ADP
eurjchem-448	95	2	conclusion	conclusion	NOUN
eurjchem-448	95	3	,	,	PUNCT
eurjchem-448	95	4	presented	present	VERB
eurjchem-448	95	5	molecular	molecular	ADJ
eurjchem-448	95	6	model	model	NOUN
eurjchem-448	95	7	for	for	ADP
eurjchem-448	95	8	mc	mc	PROPN
eurjchem-448	95	9	in	in	ADP
eurjchem-448	95	10	figure	figure	NOUN
eurjchem-448	95	11	1	1	NUM
eurjchem-448	95	12	,	,	PUNCT
eurjchem-448	95	13	is	be	AUX
eurjchem-448	95	14	in	in	ADP
eurjchem-448	95	15	best	good	ADJ
eurjchem-448	95	16	accordance	accordance	NOUN
eurjchem-448	95	17	with	with	ADP
eurjchem-448	95	18	the	the	DET
eurjchem-448	95	19	elemental	elemental	ADJ
eurjchem-448	95	20	analysis	analysis	NOUN
eurjchem-448	95	21	,	,	PUNCT
eurjchem-448	95	22	ir	ir	INTJ
eurjchem-448	95	23	,	,	PUNCT
eurjchem-448	95	24	1h	1h	NUM
eurjchem-448	95	25	nmr	nmr	NOUN
eurjchem-448	95	26	,	,	PUNCT
eurjchem-448	95	27	13c	13c	NOUN
eurjchem-448	95	28	nmr	nmr	NOUN
eurjchem-448	95	29	and	and	CCONJ
eurjchem-448	95	30	mass	mass	PROPN
eurjchem-448	95	31	spectra	spectra	PROPN
eurjchem-448	95	32	.	.	PUNCT
eurjchem-448	95	33	figure	figure	NOUN
eurjchem-448	95	34	1	1	NUM
eurjchem-448	95	35	.	.	PUNCT
eurjchem-448	96	1	molecular	molecular	ADJ
eurjchem-448	96	2	structure	structure	NOUN
eurjchem-448	96	3	of	of	ADP
eurjchem-448	96	4	macrocycle	macrocycle	NOUN
eurjchem-448	96	5	;	;	PUNCT
eurjchem-448	96	6	color	color	NOUN
eurjchem-448	96	7	code	code	NOUN
eurjchem-448	96	8	:	:	PUNCT
eurjchem-448	97	1	c	c	X
eurjchem-448	97	2	,	,	PUNCT
eurjchem-448	97	3	light	light	ADJ
eurjchem-448	97	4	grey	grey	NOUN
eurjchem-448	97	5	;	;	PUNCT
eurjchem-448	97	6	n	n	CCONJ
eurjchem-448	97	7	,	,	PUNCT
eurjchem-448	97	8	blue	blue	ADJ
eurjchem-448	97	9	;	;	PUNCT
eurjchem-448	97	10	s	s	X
eurjchem-448	97	11	,	,	PUNCT
eurjchem-448	97	12	yellow	yellow	ADJ
eurjchem-448	97	13	.	.	PUNCT
eurjchem-448	98	1	3.2	3.2	NUM
eurjchem-448	98	2	.	.	PUNCT
eurjchem-448	98	3	characterization	characterization	NOUN
eurjchem-448	98	4	of	of	ADP
eurjchem-448	98	5	ces	ces	X
eurjchem-448	98	6	ces	ce	NOUN
eurjchem-448	98	7	are	be	AUX
eurjchem-448	98	8	colored	color	VERB
eurjchem-448	98	9	,	,	PUNCT
eurjchem-448	98	10	non‐hygroscopic	non‐hygroscopic	ADJ
eurjchem-448	98	11	solids	solid	NOUN
eurjchem-448	98	12	,	,	PUNCT
eurjchem-448	98	13	stable	stable	ADJ
eurjchem-448	98	14	in	in	ADP
eurjchem-448	98	15	air	air	NOUN
eurjchem-448	98	16	.	.	PUNCT
eurjchem-448	99	1	their	their	PRON
eurjchem-448	99	2	chemical	chemical	NOUN
eurjchem-448	99	3	compositions	composition	NOUN
eurjchem-448	99	4	confirmed	confirm	VERB
eurjchem-448	99	5	purity	purity	NOUN
eurjchem-448	99	6	and	and	CCONJ
eurjchem-448	99	7	stoichiometry	stoichiometry	NOUN
eurjchem-448	99	8	of	of	ADP
eurjchem-448	99	9	neat	neat	ADJ
eurjchem-448	99	10	and	and	CCONJ
eurjchem-448	99	11	encapsulated	encapsulate	VERB
eurjchem-448	99	12	ces	ce	NOUN
eurjchem-448	99	13	.	.	NOUN
eurjchem-448	99	14	oligo	oligo	NOUN
eurjchem-448	99	15	and	and	CCONJ
eurjchem-448	99	16	polymerization	polymerization	NOUN
eurjchem-448	99	17	occurred	occur	VERB
eurjchem-448	99	18	after	after	ADP
eurjchem-448	99	19	elimination	elimination	NOUN
eurjchem-448	99	20	of	of	ADP
eurjchem-448	99	21	water	water	NOUN
eurjchem-448	99	22	or	or	CCONJ
eurjchem-448	99	23	other	other	ADJ
eurjchem-448	99	24	molecules	molecule	NOUN
eurjchem-448	99	25	,	,	PUNCT
eurjchem-448	99	26	finally	finally	ADV
eurjchem-448	99	27	effect	effect	VERB
eurjchem-448	99	28	the	the	DET
eurjchem-448	99	29	accuracy	accuracy	NOUN
eurjchem-448	99	30	of	of	ADP
eurjchem-448	99	31	c	c	PROPN
eurjchem-448	99	32	,	,	PUNCT
eurjchem-448	99	33	h	h	NOUN
eurjchem-448	99	34	and	and	CCONJ
eurjchem-448	99	35	n	n	PROPN
eurjchem-448	99	36	(	(	PUNCT
eurjchem-448	99	37	analytical	analytical	ADJ
eurjchem-448	99	38	data	datum	NOUN
eurjchem-448	99	39	)	)	PUNCT
eurjchem-448	99	40	.	.	PUNCT
eurjchem-448	100	1	further	further	ADJ
eurjchem-448	100	2	results	result	NOUN
eurjchem-448	100	3	obtained	obtain	VERB
eurjchem-448	100	4	had	have	VERB
eurjchem-448	100	5	a	a	DET
eurjchem-448	100	6	good	good	ADJ
eurjchem-448	100	7	agreement	agreement	NOUN
eurjchem-448	100	8	with	with	ADP
eurjchem-448	100	9	ms	ms	PROPN
eurjchem-448	100	10	spectral	spectral	PROPN
eurjchem-448	100	11	findings	finding	NOUN
eurjchem-448	100	12	and	and	CCONJ
eurjchem-448	100	13	suggests	suggest	VERB
eurjchem-448	100	14	monomeric	monomeric	ADJ
eurjchem-448	100	15	nature	nature	NOUN
eurjchem-448	100	16	of	of	ADP
eurjchem-448	100	17	ces	ce	NOUN
eurjchem-448	100	18	.	.	PUNCT
eurjchem-448	101	1	on	on	ADP
eurjchem-448	101	2	the	the	DET
eurjchem-448	101	3	basis	basis	NOUN
eurjchem-448	101	4	of	of	ADP
eurjchem-448	101	5	elemental	elemental	ADJ
eurjchem-448	101	6	analysis	analysis	NOUN
eurjchem-448	101	7	arranged	arrange	VERB
eurjchem-448	101	8	in	in	ADP
eurjchem-448	101	9	table	table	NOUN
eurjchem-448	101	10	1	1	NUM
eurjchem-448	101	11	,	,	PUNCT
eurjchem-448	101	12	a	a	DET
eurjchem-448	101	13	general	general	ADJ
eurjchem-448	101	14	composition	composition	NOUN
eurjchem-448	101	15	m(l)x2	m(l)x2	NOUN
eurjchem-448	101	16	,	,	PUNCT
eurjchem-448	101	17	[	[	X
eurjchem-448	101	18	where	where	SCONJ
eurjchem-448	101	19	m	m	NOUN
eurjchem-448	101	20	=	=	SYM
eurjchem-448	101	21	co(ii	co(ii	PROPN
eurjchem-448	101	22	)	)	PUNCT
eurjchem-448	101	23	and	and	CCONJ
eurjchem-448	101	24	ni(ii	ni(ii	NOUN
eurjchem-448	101	25	)	)	PUNCT
eurjchem-448	101	26	,	,	PUNCT
eurjchem-448	101	27	l	l	NOUN
eurjchem-448	102	1	=	=	PUNCT
eurjchem-448	102	2	ligand	ligand	NOUN
eurjchem-448	102	3	and	and	CCONJ
eurjchem-448	102	4	x	x	X
eurjchem-448	102	5	=	=	SYM
eurjchem-448	102	6	cl‐	cl‐	NOUN
eurjchem-448	102	7	,	,	PUNCT
eurjchem-448	102	8	no3‐	no3‐	NOUN
eurjchem-448	102	9	,	,	PUNCT
eurjchem-448	102	10	ncs‐	ncs‐	X
eurjchem-448	102	11	and	and	CCONJ
eurjchem-448	102	12	½	½	NOUN
eurjchem-448	102	13	so42‐	so42‐	PROPN
eurjchem-448	102	14	]	]	PUNCT
eurjchem-448	102	15	was	be	AUX
eurjchem-448	102	16	proposed	propose	VERB
eurjchem-448	102	17	.	.	PUNCT
eurjchem-448	103	1	molar	molar	ADJ
eurjchem-448	103	2	conductance	conductance	NOUN
eurjchem-448	103	3	measurements	measurement	NOUN
eurjchem-448	103	4	found	find	VERB
eurjchem-448	103	5	170‐182	170‐182	PROPN
eurjchem-448	103	6	ω‐1cm2mol‐1	ω‐1cm2mol‐1	NOUN
eurjchem-448	103	7	corresponds	correspond	VERB
eurjchem-448	103	8	to	to	ADP
eurjchem-448	103	9	1:2	1:2	NUM
eurjchem-448	103	10	electrolytes	electrolyte	NOUN
eurjchem-448	103	11	.	.	PUNCT
eurjchem-448	104	1	on	on	ADP
eurjchem-448	104	2	the	the	DET
eurjchem-448	104	3	basis	basis	NOUN
eurjchem-448	104	4	of	of	ADP
eurjchem-448	104	5	results	result	NOUN
eurjchem-448	104	6	obtained	obtain	VERB
eurjchem-448	104	7	,	,	PUNCT
eurjchem-448	104	8	ces	ce	NOUN
eurjchem-448	104	9	were	be	AUX
eurjchem-448	104	10	formulated	formulate	VERB
eurjchem-448	104	11	as	as	ADP
eurjchem-448	104	12	[	[	X
eurjchem-448	104	13	m(l)]x2	m(l)]x2	NOUN
eurjchem-448	104	14	.	.	PUNCT
eurjchem-448	104	15	cavity	cavity	NOUN
eurjchem-448	104	16	of	of	ADP
eurjchem-448	104	17	mc	mc	PROPN
eurjchem-448	104	18	had	have	VERB
eurjchem-448	104	19	two	two	NUM
eurjchem-448	104	20	different	different	ADJ
eurjchem-448	104	21	donor	donor	NOUN
eurjchem-448	104	22	subunits	subunit	NOUN
eurjchem-448	104	23	(	(	PUNCT
eurjchem-448	104	24	‐ch2‐s‐ch2‐	‐ch2‐s‐ch2‐	ADJ
eurjchem-448	104	25	and	and	CCONJ
eurjchem-448	104	26	‐ch	‐ch	NOUN
eurjchem-448	104	27	=	=	NOUN
eurjchem-448	104	28	n‐	n‐	NOUN
eurjchem-448	104	29	)	)	PUNCT
eurjchem-448	104	30	approached	approach	VERB
eurjchem-448	104	31	central	central	ADJ
eurjchem-448	104	32	metal	metal	NOUN
eurjchem-448	104	33	ion(s	ion(s	PROPN
eurjchem-448	104	34	)	)	PUNCT
eurjchem-448	104	35	with	with	ADP
eurjchem-448	104	36	different	different	ADJ
eurjchem-448	104	37	electron	electron	NOUN
eurjchem-448	104	38	density	density	NOUN
eurjchem-448	104	39	.	.	PUNCT
eurjchem-448	105	1	qualitative	qualitative	ADJ
eurjchem-448	105	2	reactions	reaction	NOUN
eurjchem-448	105	3	revealed	reveal	VERB
eurjchem-448	105	4	the	the	DET
eurjchem-448	105	5	absence	absence	NOUN
eurjchem-448	105	6	of	of	ADP
eurjchem-448	105	7	anion(s	anion(s	NOUN
eurjchem-448	105	8	)	)	PUNCT
eurjchem-448	105	9	in	in	ADP
eurjchem-448	105	10	[	[	X
eurjchem-448	105	11	m(l)](x)2	m(l)](x)2	NOUN
eurjchem-448	105	12	as	as	ADP
eurjchem-448	105	13	counter	counter	NOUN
eurjchem-448	105	14	ion(s	ion(s	PROPN
eurjchem-448	105	15	)	)	PUNCT
eurjchem-448	105	16	.	.	PUNCT
eurjchem-448	106	1	beside	beside	ADP
eurjchem-448	106	2	analytical	analytical	ADJ
eurjchem-448	106	3	analysis	analysis	NOUN
eurjchem-448	106	4	and	and	CCONJ
eurjchem-448	106	5	spectral	spectral	ADJ
eurjchem-448	106	6	presentation	presentation	NOUN
eurjchem-448	106	7	(	(	PUNCT
eurjchem-448	106	8	mass	mass	ADJ
eurjchem-448	106	9	,	,	PUNCT
eurjchem-448	106	10	electronic	electronic	ADJ
eurjchem-448	106	11	,	,	PUNCT
eurjchem-448	106	12	infrared	infrare	VERB
eurjchem-448	106	13	,	,	PUNCT
eurjchem-448	106	14	1h	1h	NUM
eurjchem-448	106	15	and	and	CCONJ
eurjchem-448	106	16	13c	13c	NOUN
eurjchem-448	106	17	nmr	nmr	NOUN
eurjchem-448	106	18	)	)	PUNCT
eurjchem-448	106	19	,	,	PUNCT
eurjchem-448	106	20	magnetic	magnetic	ADJ
eurjchem-448	106	21	properties	property	NOUN
eurjchem-448	106	22	were	be	AUX
eurjchem-448	106	23	also	also	ADV
eurjchem-448	106	24	summarized	summarize	VERB
eurjchem-448	106	25	and	and	CCONJ
eurjchem-448	106	26	presented	present	VERB
eurjchem-448	106	27	in	in	ADP
eurjchem-448	106	28	results	result	NOUN
eurjchem-448	106	29	and	and	CCONJ
eurjchem-448	106	30	discussion	discussion	NOUN
eurjchem-448	106	31	.	.	PUNCT
eurjchem-448	107	1	3.2.1	3.2.1	X
eurjchem-448	107	2	.	.	X
eurjchem-448	107	3	ir	ir	PROPN
eurjchem-448	107	4	spectra	spectra	PROPN
eurjchem-448	107	5	of	of	ADP
eurjchem-448	107	6	ces	ce	NOUN
eurjchem-448	107	7	appearance	appearance	NOUN
eurjchem-448	107	8	of	of	ADP
eurjchem-448	107	9	medium	medium	NOUN
eurjchem-448	107	10	to	to	ADP
eurjchem-448	107	11	strong	strong	ADJ
eurjchem-448	107	12	stretching	stretch	VERB
eurjchem-448	107	13	vibrations	vibration	NOUN
eurjchem-448	107	14	of	of	ADP
eurjchem-448	107	15	azomethine	azomethine	NOUN
eurjchem-448	107	16	comparatively	comparatively	ADV
eurjchem-448	107	17	in	in	ADP
eurjchem-448	107	18	lower	low	ADJ
eurjchem-448	107	19	regions	region	NOUN
eurjchem-448	107	20	at	at	ADP
eurjchem-448	107	21	1509‐1501	1509‐1501	NUM
eurjchem-448	107	22	cm‐1	cm‐1	NOUN
eurjchem-448	107	23	than	than	ADP
eurjchem-448	107	24	the	the	DET
eurjchem-448	107	25	expected	expect	VERB
eurjchem-448	107	26	value	value	NOUN
eurjchem-448	107	27	1611	1611	NUM
eurjchem-448	107	28	cm‐1	cm‐1	NOUN
eurjchem-448	107	29	of	of	ADP
eurjchem-448	107	30	mc	mc	PROPN
eurjchem-448	107	31	worked	work	VERB
eurjchem-448	107	32	as	as	ADP
eurjchem-448	107	33	a	a	DET
eurjchem-448	107	34	new	new	ADJ
eurjchem-448	107	35	coordination	coordination	NOUN
eurjchem-448	107	36	centre	centre	NOUN
eurjchem-448	107	37	.	.	PUNCT
eurjchem-448	108	1	lowering	lower	VERB
eurjchem-448	108	2	in	in	ADP
eurjchem-448	108	3	shift	shift	NOUN
eurjchem-448	108	4	in	in	ADP
eurjchem-448	108	5	ir	ir	PROPN
eurjchem-448	108	6	spectra	spectra	NOUN
eurjchem-448	108	7	of	of	ADP
eurjchem-448	108	8	ces	ces	X
eurjchem-448	108	9	may	may	AUX
eurjchem-448	108	10	be	be	AUX
eurjchem-448	108	11	explained	explain	VERB
eurjchem-448	108	12	on	on	ADP
eurjchem-448	108	13	basis	basis	NOUN
eurjchem-448	108	14	of	of	ADP
eurjchem-448	108	15	drift	drift	NOUN
eurjchem-448	108	16	of	of	ADP
eurjchem-448	108	17	lone	lone	ADJ
eurjchem-448	108	18	pair	pair	NOUN
eurjchem-448	108	19	density	density	NOUN
eurjchem-448	108	20	of	of	ADP
eurjchem-448	108	21	azomethine	azomethine	PROPN
eurjchem-448	108	22	nitrogen	nitrogen	PROPN
eurjchem-448	108	23	towards	towards	ADP
eurjchem-448	108	24	the	the	DET
eurjchem-448	108	25	central	central	ADJ
eurjchem-448	108	26	metal	metal	NOUN
eurjchem-448	108	27	hence	hence	ADV
eurjchem-448	108	28	confirmed	confirm	VERB
eurjchem-448	108	29	encapsulation	encapsulation	NOUN
eurjchem-448	109	1	[	[	X
eurjchem-448	109	2	14	14	NUM
eurjchem-448	109	3	]	]	PUNCT
eurjchem-448	109	4	.	.	PUNCT
eurjchem-448	110	1	presence	presence	NOUN
eurjchem-448	110	2	of	of	ADP
eurjchem-448	110	3	new	new	ADJ
eurjchem-448	110	4	medium	medium	ADJ
eurjchem-448	110	5	strong	strong	ADJ
eurjchem-448	110	6	stretching	stretch	VERB
eurjchem-448	110	7	vibrations	vibration	NOUN
eurjchem-448	110	8	at	at	ADP
eurjchem-448	110	9	552‐543	552‐543	PROPN
eurjchem-448	110	10	cm‐1	cm‐1	NOUN
eurjchem-448	110	11	confirmed	confirm	VERB
eurjchem-448	110	12	the	the	DET
eurjchem-448	110	13	formation	formation	NOUN
eurjchem-448	110	14	of	of	ADP
eurjchem-448	110	15	new	new	ADJ
eurjchem-448	110	16	bonds	bond	NOUN
eurjchem-448	110	17	i.e.	i.e.	X
eurjchem-448	110	18	ν(m‐n	ν(m‐n	NUM
eurjchem-448	110	19	)	)	PUNCT
eurjchem-448	110	20	between	between	ADP
eurjchem-448	110	21	central	central	ADJ
eurjchem-448	110	22	metal	metal	NOUN
eurjchem-448	110	23	ion	ion	NOUN
eurjchem-448	110	24	and	and	CCONJ
eurjchem-448	110	25	nitrogen	nitrogen	NOUN
eurjchem-448	110	26	of	of	ADP
eurjchem-448	110	27	azomethine	azomethine	NOUN
eurjchem-448	110	28	.	.	PUNCT
eurjchem-448	111	1	in	in	ADP
eurjchem-448	111	2	addition	addition	NOUN
eurjchem-448	111	3	,	,	PUNCT
eurjchem-448	111	4	medium	medium	NOUN
eurjchem-448	111	5	to	to	ADP
eurjchem-448	111	6	high	high	ADJ
eurjchem-448	111	7	intense	intense	ADJ
eurjchem-448	111	8	bands	band	NOUN
eurjchem-448	111	9	were	be	AUX
eurjchem-448	111	10	observed	observe	VERB
eurjchem-448	111	11	in	in	ADP
eurjchem-448	111	12	far	far	ADV
eurjchem-448	111	13	infrared	infrared	ADJ
eurjchem-448	111	14	regions	region	NOUN
eurjchem-448	111	15	at	at	ADP
eurjchem-448	111	16	396‐371	396‐371	PROPN
eurjchem-448	111	17	cm‐1	cm‐1	PROPN
eurjchem-448	111	18	because	because	SCONJ
eurjchem-448	111	19	of	of	ADP
eurjchem-448	111	20	bathochromic	bathochromic	ADJ
eurjchem-448	111	21	shift	shift	NOUN
eurjchem-448	111	22	coupled	couple	VERB
eurjchem-448	111	23	with	with	ADP
eurjchem-448	111	24	lower	low	ADJ
eurjchem-448	111	25	vibrational	vibrational	ADJ
eurjchem-448	111	26	modes	mode	NOUN
eurjchem-448	111	27	of	of	ADP
eurjchem-448	111	28	s	s	PRON
eurjchem-448	111	29	and	and	CCONJ
eurjchem-448	111	30	favored	favor	VERB
eurjchem-448	111	31	it	it	PRON
eurjchem-448	111	32	coordination	coordination	NOUN
eurjchem-448	111	33	with	with	ADP
eurjchem-448	111	34	central	central	ADJ
eurjchem-448	111	35	metal	metal	NOUN
eurjchem-448	112	1	[	[	NOUN
eurjchem-448	112	2	15,16	15,16	NUM
eurjchem-448	112	3	]	]	PUNCT
eurjchem-448	112	4	.	.	PUNCT
eurjchem-448	113	1	this	this	DET
eurjchem-448	113	2	phenomenon	phenomenon	NOUN
eurjchem-448	113	3	attributes	attribute	VERB
eurjchem-448	113	4	host	host	NOUN
eurjchem-448	113	5	/	/	SYM
eurjchem-448	113	6	guest	guest	NOUN
eurjchem-448	113	7	stability	stability	NOUN
eurjchem-448	113	8	in	in	ADP
eurjchem-448	113	9	a	a	DET
eurjchem-448	113	10	defined	define	VERB
eurjchem-448	113	11	way	way	NOUN
eurjchem-448	113	12	.	.	PUNCT
eurjchem-448	114	1	related	relate	VERB
eurjchem-448	114	2	infrared	infrared	ADJ
eurjchem-448	114	3	spectral	spectral	ADJ
eurjchem-448	114	4	data	datum	NOUN
eurjchem-448	114	5	were	be	AUX
eurjchem-448	114	6	presented	present	VERB
eurjchem-448	114	7	in	in	ADP
eurjchem-448	114	8	table	table	NOUN
eurjchem-448	114	9	2	2	NUM
eurjchem-448	114	10	.	.	X
eurjchem-448	114	11	60	60	NUM
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eurjchem-448	114	13	et	et	PROPN
eurjchem-448	114	14	al	al	PROPN
eurjchem-448	114	15	.	.	PUNCT
eurjchem-448	114	16	/	/	SYM
eurjchem-448	114	17	european	european	PROPN
eurjchem-448	114	18	journal	journal	PROPN
eurjchem-448	114	19	of	of	ADP
eurjchem-448	114	20	chemistry	chemistry	NOUN
eurjchem-448	114	21	3	3	NUM
eurjchem-448	114	22	(	(	PUNCT
eurjchem-448	114	23	1	1	NUM
eurjchem-448	114	24	)	)	PUNCT
eurjchem-448	114	25	(	(	PUNCT
eurjchem-448	114	26	2012	2012	NUM
eurjchem-448	114	27	)	)	PUNCT
eurjchem-448	114	28	57‐64	57‐64	NUM
eurjchem-448	114	29	table	table	NOUN
eurjchem-448	114	30	1	1	NUM
eurjchem-448	114	31	.	.	PUNCT
eurjchem-448	114	32	molar	molar	ADJ
eurjchem-448	114	33	conductance	conductance	NOUN
eurjchem-448	114	34	and	and	CCONJ
eurjchem-448	114	35	elemental	elemental	ADJ
eurjchem-448	114	36	analysis	analysis	NOUN
eurjchem-448	114	37	of	of	ADP
eurjchem-448	114	38	mc	mc	PROPN
eurjchem-448	114	39	and	and	CCONJ
eurjchem-448	114	40	ces	ces	X
eurjchem-448	114	41	with	with	ADP
eurjchem-448	114	42	co(ii	co(ii	PROPN
eurjchem-448	114	43	)	)	PUNCT
eurjchem-448	114	44	and	and	CCONJ
eurjchem-448	114	45	ni(ii	ni(ii	NOUN
eurjchem-448	114	46	)	)	PUNCT
eurjchem-448	114	47	.	.	PUNCT
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eurjchem-448	115	2	and	and	CCONJ
eurjchem-448	115	3	ces	ces	X
eurjchem-448	115	4	molecular	molecular	ADJ
eurjchem-448	115	5	formula	formula	NOUN
eurjchem-448	115	6	ʌm(ω‐1cm2	ʌm(ω‐1cm2	ADJ
eurjchem-448	115	7	mol‐1	mol‐1	NOUN
eurjchem-448	115	8	)	)	PUNCT
eurjchem-448	115	9	calcd	calcd	NOUN
eurjchem-448	115	10	.	.	PUNCT
eurjchem-448	116	1	(	(	PUNCT
eurjchem-448	116	2	found	find	VERB
eurjchem-448	116	3	)	)	PUNCT
eurjchem-448	116	4	%	%	NOUN
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eurjchem-448	117	2	c	c	NOUN
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eurjchem-448	117	6	mc‐l	mc‐l	PROPN
eurjchem-448	117	7	)	)	PUNCT
eurjchem-448	117	8	c32h30n2s4	c32h30n2s4	NOUN
eurjchem-448	117	9	‐	‐	VERB
eurjchem-448	117	10	‐	‐	ADP
eurjchem-448	117	11	67.33(67.01	67.33(67.01	NOUN
eurjchem-448	117	12	)	)	PUNCT
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eurjchem-448	117	16	)	)	PUNCT
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eurjchem-448	118	5	8.41(8.34	8.41(8.34	NUM
eurjchem-448	118	6	)	)	PUNCT
eurjchem-448	118	7	54.85(54.65	54.85(54.65	NUM
eurjchem-448	118	8	)	)	PUNCT
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eurjchem-448	118	12	)	)	PUNCT
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eurjchem-448	119	6	)	)	PUNCT
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eurjchem-448	120	6	)	)	PUNCT
eurjchem-448	120	7	50.99(50.75	50.99(50.75	NUM
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eurjchem-448	126	15	)	)	PUNCT
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eurjchem-448	126	17	)	)	PUNCT
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eurjchem-448	126	19	)	)	PUNCT
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eurjchem-448	126	21	so4=	so4=	NOUN
eurjchem-448	126	22	)	)	PUNCT
eurjchem-448	126	23	c30h26n2s4(l	c30h26n2s4(l	NOUN
eurjchem-448	126	24	)	)	PUNCT
eurjchem-448	126	25	1611s	1611s	NUM
eurjchem-448	126	26	2991w	2991w	NOUN
eurjchem-448	126	27	‐	‐	VERB
eurjchem-448	126	28	‐	‐	ADV
eurjchem-448	126	29	‐	‐	ADV
eurjchem-448	126	30	‐	‐	ADV
eurjchem-448	126	31	‐	‐	ADV
eurjchem-448	126	32	[	[	X
eurjchem-448	126	33	co(l)]cl2	co(l)]cl2	X
eurjchem-448	126	34	1602s	1602	NOUN
eurjchem-448	126	35	2970w	2970w	NUM
eurjchem-448	126	36	542	542	NUM
eurjchem-448	126	37	m	m	NUM
eurjchem-448	126	38	380	380	NUM
eurjchem-448	126	39	m	m	NUM
eurjchem-448	126	40	‐	‐	NOUN
eurjchem-448	126	41	‐	‐	ADV
eurjchem-448	126	42	‐	‐	ADV
eurjchem-448	126	43	[	[	X
eurjchem-448	126	44	co(l)](ncs)2	co(l)](ncs)2	NOUN
eurjchem-448	126	45	1609s	1609s	NUM
eurjchem-448	126	46	2972w	2972w	NUM
eurjchem-448	126	47	546	546	NUM
eurjchem-448	126	48	m	m	NOUN
eurjchem-448	126	49	385	385	NUM
eurjchem-448	126	50	m	m	NUM
eurjchem-448	126	51	‐	‐	NOUN
eurjchem-448	126	52	2048s	2048s	NUM
eurjchem-448	126	53	‐	‐	ADP
eurjchem-448	126	54	[	[	X
eurjchem-448	126	55	co(l)](no3)2	co(l)](no3)2	PROPN
eurjchem-448	126	56	1606s	1606s	NUM
eurjchem-448	126	57	2977w	2977w	NUM
eurjchem-448	126	58	542	542	NUM
eurjchem-448	126	59	m	m	NUM
eurjchem-448	126	60	341	341	NUM
eurjchem-448	126	61	m	m	NOUN
eurjchem-448	126	62	1385s	1385	NOUN
eurjchem-448	126	63	,	,	PUNCT
eurjchem-448	126	64	824(w	824(w	NUM
eurjchem-448	126	65	)	)	PUNCT
eurjchem-448	126	66	,	,	PUNCT
eurjchem-448	126	67	275(w	275(w	NUM
eurjchem-448	126	68	)	)	PUNCT
eurjchem-448	126	69	‐	‐	ADV
eurjchem-448	126	70	‐	‐	NOUN
eurjchem-448	126	71	[	[	X
eurjchem-448	126	72	co(l)](oso3	co(l)](oso3	NOUN
eurjchem-448	126	73	)	)	PUNCT
eurjchem-448	126	74	1609s	1609	NOUN
eurjchem-448	126	75	2978w	2978w	NUM
eurjchem-448	126	76	552	552	NUM
eurjchem-448	126	77	m	m	NOUN
eurjchem-448	126	78	342	342	NUM
eurjchem-448	126	79	m	m	NUM
eurjchem-448	126	80	‐	‐	NOUN
eurjchem-448	126	81	‐	‐	ADV
eurjchem-448	126	82	1132s	1132s	NUM
eurjchem-448	126	83	,	,	PUNCT
eurjchem-448	126	84	1104s	1104s	NUM
eurjchem-448	126	85	,	,	PUNCT
eurjchem-448	126	86	615	615	NUM
eurjchem-448	126	87	m	m	NOUN
eurjchem-448	126	88	[	[	X
eurjchem-448	126	89	ni(l)]cl2	ni(l)]cl2	X
eurjchem-448	126	90	1603s	1603s	X
eurjchem-448	126	91	2977w	2977w	NUM
eurjchem-448	126	92	523	523	NUM
eurjchem-448	126	93	m	m	NOUN
eurjchem-448	126	94	390	390	NUM
eurjchem-448	126	95	m	m	NUM
eurjchem-448	126	96	‐	‐	NOUN
eurjchem-448	126	97	‐	‐	ADV
eurjchem-448	126	98	‐	‐	NOUN
eurjchem-448	126	99	[	[	X
eurjchem-448	126	100	ni(l)](ncs)2	ni(l)](ncs)2	PROPN
eurjchem-448	126	101	1602s	1602	NOUN
eurjchem-448	126	102	2975w	2975w	NOUN
eurjchem-448	126	103	543	543	NUM
eurjchem-448	126	104	m	m	NUM
eurjchem-448	126	105	396	396	NUM
eurjchem-448	126	106	m	m	NOUN
eurjchem-448	126	107	‐	‐	NOUN
eurjchem-448	126	108	2049s	2049s	PUNCT
eurjchem-448	126	109	‐	‐	ADP
eurjchem-448	126	110	[	[	X
eurjchem-448	126	111	ni(l)](no3)2	ni(l)](no3)2	PROPN
eurjchem-448	126	112	1608s	1608s	NUM
eurjchem-448	126	113	2974w	2974w	NUM
eurjchem-448	126	114	526	526	NUM
eurjchem-448	126	115	m	m	NUM
eurjchem-448	126	116	389	389	NUM
eurjchem-448	126	117	m	m	NOUN
eurjchem-448	126	118	1384s	1384s	NUM
eurjchem-448	126	119	‐	‐	NOUN
eurjchem-448	126	120	‐	‐	ADV
eurjchem-448	126	121	[	[	X
eurjchem-448	126	122	ni(l)](oso3	ni(l)](oso3	NOUN
eurjchem-448	126	123	)	)	PUNCT
eurjchem-448	126	124	1601s	1601s	NUM
eurjchem-448	126	125	2972w	2972w	NUM
eurjchem-448	126	126	551	551	NUM
eurjchem-448	126	127	m	m	NOUN
eurjchem-448	126	128	387	387	NUM
eurjchem-448	126	129	m	m	NUM
eurjchem-448	126	130	‐	‐	NOUN
eurjchem-448	126	131	‐	‐	ADV
eurjchem-448	126	132	1131s	1131s	NUM
eurjchem-448	126	133	,	,	PUNCT
eurjchem-448	126	134	1102	1102	NUM
eurjchem-448	126	135	m	m	NOUN
eurjchem-448	126	136	,	,	PUNCT
eurjchem-448	126	137	613	613	NUM
eurjchem-448	126	138	m	m	NUM
eurjchem-448	126	139	3.2.2	3.2.2	NUM
eurjchem-448	126	140	.	.	PUNCT
eurjchem-448	127	1	magnetic	magnetic	ADJ
eurjchem-448	127	2	moments	moment	NOUN
eurjchem-448	127	3	of	of	ADP
eurjchem-448	127	4	ces	ces	X
eurjchem-448	127	5	magnetic	magnetic	ADJ
eurjchem-448	127	6	moments	moment	NOUN
eurjchem-448	127	7	of	of	ADP
eurjchem-448	127	8	ces	ce	NOUN
eurjchem-448	127	9	of	of	ADP
eurjchem-448	127	10	co(ii	co(ii	ADJ
eurjchem-448	127	11	)	)	PUNCT
eurjchem-448	127	12	and	and	CCONJ
eurjchem-448	127	13	ni(ii	ni(ii	PROPN
eurjchem-448	127	14	)	)	PUNCT
eurjchem-448	127	15	obtained	obtain	VERB
eurjchem-448	127	16	at	at	ADP
eurjchem-448	127	17	room	room	NOUN
eurjchem-448	127	18	temperature	temperature	NOUN
eurjchem-448	127	19	and	and	CCONJ
eurjchem-448	127	20	were	be	AUX
eurjchem-448	127	21	usually	usually	ADV
eurjchem-448	127	22	similar	similar	ADJ
eurjchem-448	127	23	to	to	ADP
eurjchem-448	127	24	spin‐only	spin‐only	ADV
eurjchem-448	127	25	value	value	NOUN
eurjchem-448	127	26	,	,	PUNCT
eurjchem-448	127	27	i.e.	i.e.	X
eurjchem-448	127	28	µiso	µiso	NOUN
eurjchem-448	127	29	=	=	SYM
eurjchem-448	127	30	2[s(s+1)]½.	2[s(s+1)]½.	NUM
eurjchem-448	127	31	in	in	ADP
eurjchem-448	127	32	general	general	ADJ
eurjchem-448	127	33	,	,	PUNCT
eurjchem-448	127	34	this	this	PRON
eurjchem-448	127	35	is	be	AUX
eurjchem-448	127	36	directly	directly	ADV
eurjchem-448	127	37	proportional	proportional	ADJ
eurjchem-448	127	38	to	to	ADP
eurjchem-448	127	39	the	the	DET
eurjchem-448	127	40	number	number	NOUN
eurjchem-448	127	41	of	of	ADP
eurjchem-448	127	42	unpaired	unpaired	ADJ
eurjchem-448	127	43	electrons	electron	NOUN
eurjchem-448	127	44	in	in	ADP
eurjchem-448	127	45	metal	metal	NOUN
eurjchem-448	127	46	ion(s	ion(s	PROPN
eurjchem-448	127	47	)	)	PUNCT
eurjchem-448	127	48	.	.	PUNCT
eurjchem-448	128	1	ces	ce	NOUN
eurjchem-448	128	2	of	of	ADP
eurjchem-448	128	3	ni(ii	ni(ii	NOUN
eurjchem-448	128	4	)	)	PUNCT
eurjchem-448	128	5	and	and	CCONJ
eurjchem-448	128	6	co(ii	co(ii	VERB
eurjchem-448	128	7	)	)	PUNCT
eurjchem-448	128	8	showed	show	VERB
eurjchem-448	128	9	magnetic	magnetic	ADJ
eurjchem-448	128	10	moment	moment	NOUN
eurjchem-448	128	11	2.94‐2.97	2.94‐2.97	NUM
eurjchem-448	128	12	and	and	CCONJ
eurjchem-448	128	13	4.76‐	4.76‐	NUM
eurjchem-448	128	14	4.91	4.91	NUM
eurjchem-448	129	1	b.m	b.m	NOUN
eurjchem-448	129	2	corresponding	correspond	VERB
eurjchem-448	129	3	to	to	ADP
eurjchem-448	129	4	two	two	NUM
eurjchem-448	129	5	and	and	CCONJ
eurjchem-448	129	6	three	three	NUM
eurjchem-448	129	7	unpaired	unpaired	ADJ
eurjchem-448	129	8	electrons	electron	NOUN
eurjchem-448	129	9	,	,	PUNCT
eurjchem-448	129	10	respectively	respectively	ADV
eurjchem-448	129	11	.	.	PUNCT
eurjchem-448	130	1	it	it	PRON
eurjchem-448	130	2	is	be	AUX
eurjchem-448	130	3	thus	thus	ADV
eurjchem-448	130	4	in	in	ADP
eurjchem-448	130	5	good	good	ADJ
eurjchem-448	130	6	agreement	agreement	NOUN
eurjchem-448	130	7	with	with	ADP
eurjchem-448	130	8	high	high	ADJ
eurjchem-448	130	9	spin	spin	NOUN
eurjchem-448	130	10	configuration	configuration	NOUN
eurjchem-448	130	11	[	[	X
eurjchem-448	130	12	17	17	NUM
eurjchem-448	130	13	]	]	PUNCT
eurjchem-448	130	14	.	.	PUNCT
eurjchem-448	131	1	for	for	ADP
eurjchem-448	131	2	the	the	DET
eurjchem-448	131	3	octahedral	octahedral	ADJ
eurjchem-448	131	4	co(ii	co(ii	PROPN
eurjchem-448	131	5	)	)	PUNCT
eurjchem-448	131	6	(	(	PUNCT
eurjchem-448	131	7	s	s	NOUN
eurjchem-448	131	8	=	=	SYM
eurjchem-448	131	9	3/2	3/2	NUM
eurjchem-448	131	10	)	)	PUNCT
eurjchem-448	131	11	complexes	complex	NOUN
eurjchem-448	131	12	,	,	PUNCT
eurjchem-448	131	13	the	the	DET
eurjchem-448	131	14	orbital	orbital	ADJ
eurjchem-448	131	15	angular	angular	ADJ
eurjchem-448	131	16	momentum	momentum	NOUN
eurjchem-448	131	17	present	present	ADJ
eurjchem-448	131	18	in	in	ADP
eurjchem-448	131	19	the	the	DET
eurjchem-448	131	20	ground	ground	NOUN
eurjchem-448	131	21	t‐term	t‐term	NUM
eurjchem-448	131	22	reflects	reflect	VERB
eurjchem-448	131	23	heavily	heavily	ADV
eurjchem-448	131	24	on	on	ADP
eurjchem-448	131	25	the	the	DET
eurjchem-448	131	26	magnetic	magnetic	ADJ
eurjchem-448	131	27	properties	property	NOUN
eurjchem-448	131	28	.	.	PUNCT
eurjchem-448	132	1	on	on	ADP
eurjchem-448	132	2	exposing	expose	VERB
eurjchem-448	132	3	complexes	complex	NOUN
eurjchem-448	132	4	to	to	ADP
eurjchem-448	132	5	d4h	d4h	PROPN
eurjchem-448	132	6	symmetry	symmetry	NOUN
eurjchem-448	132	7	,	,	PUNCT
eurjchem-448	132	8	further	further	ADJ
eurjchem-448	132	9	splitting	splitting	NOUN
eurjchem-448	132	10	occurs	occur	VERB
eurjchem-448	132	11	.	.	PUNCT
eurjchem-448	133	1	4t1	4t1	NUM
eurjchem-448	134	1	g	g	PROPN
eurjchem-448	134	2	term	term	NOUN
eurjchem-448	134	3	splits	split	VERB
eurjchem-448	134	4	into	into	ADP
eurjchem-448	134	5	4eg	4eg	NOUN
eurjchem-448	134	6	and	and	CCONJ
eurjchem-448	134	7	4a2	4a2	PRON
eurjchem-448	134	8	g	g	NOUN
eurjchem-448	134	9	,	,	PUNCT
eurjchem-448	134	10	where	where	SCONJ
eurjchem-448	134	11	4a2	4a2	NUM
eurjchem-448	134	12	g	g	PROPN
eurjchem-448	134	13	is	be	AUX
eurjchem-448	134	14	the	the	DET
eurjchem-448	134	15	ground	ground	NOUN
eurjchem-448	134	16	state	state	NOUN
eurjchem-448	134	17	.	.	PUNCT
eurjchem-448	135	1	the	the	DET
eurjchem-448	135	2	spin‐orbit	spin‐orbit	NOUN
eurjchem-448	135	3	coupling	coupling	NOUN
eurjchem-448	135	4	splits	split	VERB
eurjchem-448	135	5	this	this	DET
eurjchem-448	135	6	term	term	NOUN
eurjchem-448	135	7	into	into	ADP
eurjchem-448	135	8	kramers	kramer	NOUN
eurjchem-448	135	9	doublets	doublets	VERB
eurjchem-448	135	10	ґ6	ґ6	NUM
eurjchem-448	135	11	and	and	CCONJ
eurjchem-448	135	12	ґ7	ґ7	NOUN
eurjchem-448	135	13	.	.	PUNCT
eurjchem-448	136	1	the	the	DET
eurjchem-448	136	2	difference	difference	NOUN
eurjchem-448	136	3	of	of	ADP
eurjchem-448	136	4	these	these	DET
eurjchem-448	136	5	states	state	NOUN
eurjchem-448	136	6	can	can	AUX
eurjchem-448	136	7	be	be	AUX
eurjchem-448	136	8	assigned	assign	VERB
eurjchem-448	136	9	as	as	ADP
eurjchem-448	136	10	2d	2d	NUM
eurjchem-448	136	11	[	[	X
eurjchem-448	136	12	18	18	NUM
eurjchem-448	136	13	]	]	PUNCT
eurjchem-448	136	14	.	.	PUNCT
eurjchem-448	137	1	3.2.3	3.2.3	X
eurjchem-448	137	2	.	.	X
eurjchem-448	137	3	electronic	electronic	ADJ
eurjchem-448	137	4	spectra	spectra	NOUN
eurjchem-448	137	5	of	of	ADP
eurjchem-448	137	6	ces	ce	NOUN
eurjchem-448	137	7	in	in	ADP
eurjchem-448	137	8	the	the	DET
eurjchem-448	137	9	both	both	DET
eurjchem-448	137	10	series	series	NOUN
eurjchem-448	137	11	of	of	ADP
eurjchem-448	137	12	ces	ce	NOUN
eurjchem-448	137	13	,	,	PUNCT
eurjchem-448	137	14	d‐d	d‐d	PRON
eurjchem-448	137	15	transitions	transition	NOUN
eurjchem-448	137	16	were	be	AUX
eurjchem-448	137	17	happened	happen	VERB
eurjchem-448	137	18	due	due	ADP
eurjchem-448	137	19	to	to	ADP
eurjchem-448	137	20	the	the	DET
eurjchem-448	137	21	presence	presence	NOUN
eurjchem-448	137	22	of	of	ADP
eurjchem-448	137	23	‐ch	‐ch	NOUN
eurjchem-448	137	24	=	=	NOUN
eurjchem-448	137	25	n‐	n‐	NOUN
eurjchem-448	137	26	linkage	linkage	NOUN
eurjchem-448	137	27	and	and	CCONJ
eurjchem-448	137	28	charge	charge	NOUN
eurjchem-448	137	29	transfer	transfer	NOUN
eurjchem-448	137	30	transitions	transition	NOUN
eurjchem-448	137	31	.	.	PUNCT
eurjchem-448	138	1	such	such	ADJ
eurjchem-448	138	2	transitions	transition	NOUN
eurjchem-448	138	3	arose	arise	VERB
eurjchem-448	138	4	because	because	SCONJ
eurjchem-448	138	5	of	of	ADP
eurjchem-448	138	6	delocalization	delocalization	NOUN
eurjchem-448	138	7	of	of	ADP
eurjchem-448	138	8	‐electrons	‐electron	NOUN
eurjchem-448	138	9	between	between	ADP
eurjchem-448	138	10	central	central	ADJ
eurjchem-448	138	11	metal	metal	NOUN
eurjchem-448	138	12	and	and	CCONJ
eurjchem-448	138	13	donor	donor	NOUN
eurjchem-448	138	14	atoms	atom	NOUN
eurjchem-448	138	15	(	(	PUNCT
eurjchem-448	138	16	n	n	CCONJ
eurjchem-448	138	17	/	/	SYM
eurjchem-448	138	18	s	s	NOUN
eurjchem-448	138	19	)	)	PUNCT
eurjchem-448	138	20	.	.	PUNCT
eurjchem-448	139	1	finally	finally	ADV
eurjchem-448	139	2	,	,	PUNCT
eurjchem-448	139	3	it	it	PRON
eurjchem-448	139	4	is	be	AUX
eurjchem-448	139	5	a	a	DET
eurjchem-448	139	6	metal‐to‐ligand	metal‐to‐ligand	PROPN
eurjchem-448	139	7	(	(	PUNCT
eurjchem-448	139	8	mlct	mlct	PROPN
eurjchem-448	139	9	)	)	PUNCT
eurjchem-448	139	10	or	or	CCONJ
eurjchem-448	139	11	ligand‐to‐metal	ligand‐to‐metal	ADJ
eurjchem-448	139	12	(	(	PUNCT
eurjchem-448	139	13	lmct	lmct	NOUN
eurjchem-448	139	14	)	)	PUNCT
eurjchem-448	139	15	charge	charge	NOUN
eurjchem-448	139	16	(	(	PUNCT
eurjchem-448	139	17	electron	electron	NOUN
eurjchem-448	139	18	)	)	PUNCT
eurjchem-448	139	19	transfer	transfer	NOUN
eurjchem-448	139	20	[	[	NOUN
eurjchem-448	139	21	19	19	NUM
eurjchem-448	139	22	]	]	PUNCT
eurjchem-448	139	23	.	.	PUNCT
eurjchem-448	140	1	electronic	electronic	ADJ
eurjchem-448	140	2	spectra	spectra	NOUN
eurjchem-448	140	3	of	of	ADP
eurjchem-448	140	4	ces	ce	NOUN
eurjchem-448	140	5	of	of	ADP
eurjchem-448	140	6	co(ii	co(ii	PROPN
eurjchem-448	140	7	)	)	PUNCT
eurjchem-448	140	8	,	,	PUNCT
eurjchem-448	140	9	three	three	NUM
eurjchem-448	140	10	d‐d	d‐d	NUM
eurjchem-448	140	11	transitions	transition	NOUN
eurjchem-448	140	12	bands	band	NOUN
eurjchem-448	140	13	observed	observe	VERB
eurjchem-448	140	14	around	around	ADP
eurjchem-448	140	15	14,780‐11,754	14,780‐11,754	NUM
eurjchem-448	140	16	cm‐1	cm‐1	NOUN
eurjchem-448	140	17	and	and	CCONJ
eurjchem-448	140	18	21,624‐	21,624‐	NUM
eurjchem-448	140	19	16,710	16,710	NUM
eurjchem-448	140	20	cm‐1	cm‐1	NOUN
eurjchem-448	140	21	,	,	PUNCT
eurjchem-448	140	22	27,430‐24,462	27,430‐24,462	NUM
eurjchem-448	140	23	cm‐1	cm‐1	NOUN
eurjchem-448	140	24	may	may	AUX
eurjchem-448	140	25	be	be	AUX
eurjchem-448	140	26	assigned	assign	VERB
eurjchem-448	140	27	to	to	ADP
eurjchem-448	140	28	4t1g(4f	4t1g(4f	NOUN
eurjchem-448	140	29	)	)	PUNCT
eurjchem-448	140	30			PUNCT
eurjchem-448	141	1	4t2g(4f	4t2g(4f	ADJ
eurjchem-448	141	2	)	)	PUNCT
eurjchem-448	141	3	(	(	PUNCT
eurjchem-448	141	4	υ1	υ1	PROPN
eurjchem-448	141	5	)	)	PUNCT
eurjchem-448	141	6	,	,	PUNCT
eurjchem-448	141	7	4t1g(4f	4t1g(4f	NOUN
eurjchem-448	141	8	)	)	PUNCT
eurjchem-448	141	9			PUNCT
eurjchem-448	142	1	4a2g(4f	4a2g(4f	NUM
eurjchem-448	142	2	)	)	PUNCT
eurjchem-448	142	3	(	(	PUNCT
eurjchem-448	142	4	υ2	υ2	NOUN
eurjchem-448	142	5	)	)	PUNCT
eurjchem-448	142	6	and	and	CCONJ
eurjchem-448	142	7	4t1g(4f	4t1g(4f	NOUN
eurjchem-448	142	8	)	)	PUNCT
eurjchem-448	142	9			PROPN
eurjchem-448	142	10	4t1g(4p	4t1g(4p	NOUN
eurjchem-448	142	11	)	)	PUNCT
eurjchem-448	142	12	(	(	PUNCT
eurjchem-448	142	13	υ3	υ3	NOUN
eurjchem-448	142	14	)	)	PUNCT
eurjchem-448	142	15	transitions	transition	NOUN
eurjchem-448	142	16	,	,	PUNCT
eurjchem-448	142	17	respectively	respectively	ADV
eurjchem-448	142	18	[	[	X
eurjchem-448	142	19	20	20	NUM
eurjchem-448	142	20	]	]	PUNCT
eurjchem-448	142	21	,	,	PUNCT
eurjchem-448	142	22	characteristic	characteristic	ADJ
eurjchem-448	142	23	of	of	ADP
eurjchem-448	142	24	an	an	DET
eurjchem-448	142	25	octahedral	octahedral	ADJ
eurjchem-448	142	26	geometry	geometry	NOUN
eurjchem-448	142	27	.	.	PUNCT
eurjchem-448	143	1	in	in	ADP
eurjchem-448	143	2	electronic	electronic	ADJ
eurjchem-448	143	3	spectra	spectra	NOUN
eurjchem-448	143	4	of	of	ADP
eurjchem-448	143	5	ces	ce	NOUN
eurjchem-448	143	6	of	of	ADP
eurjchem-448	143	7	ni(ii	ni(ii	NOUN
eurjchem-448	143	8	)	)	PUNCT
eurjchem-448	143	9	,	,	PUNCT
eurjchem-448	143	10	three	three	NUM
eurjchem-448	143	11	d‐d	d‐d	NUM
eurjchem-448	143	12	transition	transition	NOUN
eurjchem-448	143	13	bands	band	NOUN
eurjchem-448	143	14	observed	observe	VERB
eurjchem-448	143	15	around	around	ADP
eurjchem-448	143	16	9,920‐8,410	9,920‐8,410	NUM
eurjchem-448	143	17	cm‐1	cm‐1	NOUN
eurjchem-448	143	18	,	,	PUNCT
eurjchem-448	143	19	15,840‐13,880	15,840‐13,880	NUM
eurjchem-448	143	20	cm‐1	cm‐1	NOUN
eurjchem-448	143	21	,	,	PUNCT
eurjchem-448	143	22	and	and	CCONJ
eurjchem-448	143	23	27,880‐27,481	27,880‐27,481	NUM
eurjchem-448	143	24	cm‐1	cm‐1	NOUN
eurjchem-448	143	25	may	may	AUX
eurjchem-448	143	26	be	be	AUX
eurjchem-448	143	27	assigned	assign	VERB
eurjchem-448	143	28	to	to	ADP
eurjchem-448	143	29	1a1	1a1	NUM
eurjchem-448	143	30	g	g	NOUN
eurjchem-448	143	31			NOUN
eurjchem-448	143	32	1a2	1a2	PRON
eurjchem-448	143	33	g	g	NOUN
eurjchem-448	143	34	,	,	PUNCT
eurjchem-448	143	35	1a1	1a1	NUM
eurjchem-448	143	36	g	g	NOUN
eurjchem-448	143	37			NOUN
eurjchem-448	144	1	1b1	1b1	NUM
eurjchem-448	144	2	g	g	PROPN
eurjchem-448	144	3	(	(	PUNCT
eurjchem-448	144	4	υ1	υ1	PROPN
eurjchem-448	144	5	)	)	PUNCT
eurjchem-448	144	6	,	,	PUNCT
eurjchem-448	144	7	1a1	1a1	NUM
eurjchem-448	144	8	g	g	NOUN
eurjchem-448	144	9			NOUN
eurjchem-448	144	10	1eg	1eg	ADJ
eurjchem-448	144	11	,	,	PUNCT
eurjchem-448	144	12	3a1	3a1	NUM
eurjchem-448	144	13	g	g	NOUN
eurjchem-448	144	14			NOUN
eurjchem-448	144	15	3t2g(f	3t2g(f	NUM
eurjchem-448	144	16	)	)	PUNCT
eurjchem-448	144	17	(	(	PUNCT
eurjchem-448	144	18	υ2	υ2	NOUN
eurjchem-448	144	19	)	)	PUNCT
eurjchem-448	144	20	and	and	CCONJ
eurjchem-448	144	21	3a2	3a2	NUM
eurjchem-448	144	22	g	g	NOUN
eurjchem-448	144	23			NOUN
eurjchem-448	144	24	3t1g(f	3t1g(f	NUM
eurjchem-448	144	25	)	)	PUNCT
eurjchem-448	144	26	3a2	3a2	NUM
eurjchem-448	144	27	g	g	NOUN
eurjchem-448	144	28			NOUN
eurjchem-448	145	1	3t1	3t1	PROPN
eurjchem-448	145	2	g	g	NOUN
eurjchem-448	145	3	(	(	PUNCT
eurjchem-448	145	4	p	p	NOUN
eurjchem-448	145	5	)	)	PUNCT
eurjchem-448	145	6	(	(	PUNCT
eurjchem-448	145	7	υ3	υ3	NOUN
eurjchem-448	145	8	)	)	PUNCT
eurjchem-448	145	9	transitions	transition	NOUN
eurjchem-448	145	10	,	,	PUNCT
eurjchem-448	145	11	respectively	respectively	ADV
eurjchem-448	145	12	,	,	PUNCT
eurjchem-448	145	13	characteristic	characteristic	ADJ
eurjchem-448	145	14	of	of	ADP
eurjchem-448	145	15	an	an	DET
eurjchem-448	145	16	octahedral	octahedral	ADJ
eurjchem-448	145	17	geometry	geometry	NOUN
eurjchem-448	145	18	.	.	PUNCT
eurjchem-448	146	1	3.2.4	3.2.4	NUM
eurjchem-448	146	2	.	.	PUNCT
eurjchem-448	146	3	ligand	ligand	ADJ
eurjchem-448	146	4	field	field	NOUN
eurjchem-448	146	5	parameters	parameter	NOUN
eurjchem-448	146	6	of	of	ADP
eurjchem-448	146	7	ces	ce	NOUN
eurjchem-448	146	8	on	on	ADP
eurjchem-448	146	9	basis	basis	NOUN
eurjchem-448	146	10	of	of	ADP
eurjchem-448	146	11	bands	band	NOUN
eurjchem-448	146	12	shapes	shape	NOUN
eurjchem-448	146	13	and	and	CCONJ
eurjchem-448	146	14	their	their	PRON
eurjchem-448	146	15	different	different	ADJ
eurjchem-448	146	16	positions	position	NOUN
eurjchem-448	146	17	(	(	PUNCT
eurjchem-448	146	18	assigned	assign	VERB
eurjchem-448	146	19	on	on	ADP
eurjchem-448	146	20	the	the	DET
eurjchem-448	146	21	basis	basis	NOUN
eurjchem-448	146	22	of	of	ADP
eurjchem-448	146	23	oh	oh	NUM
eurjchem-448	146	24	symmetry	symmetry	NOUN
eurjchem-448	146	25	)	)	PUNCT
eurjchem-448	146	26	,	,	PUNCT
eurjchem-448	146	27	ligand	ligand	ADJ
eurjchem-448	146	28	field	field	NOUN
eurjchem-448	146	29	splitting	split	VERB
eurjchem-448	146	30	energy	energy	NOUN
eurjchem-448	146	31	(	(	PUNCT
eurjchem-448	146	32	dq	dq	NOUN
eurjchem-448	146	33	)	)	PUNCT
eurjchem-448	146	34	and	and	CCONJ
eurjchem-448	146	35	ligand	ligand	ADJ
eurjchem-448	146	36	field	field	NOUN
eurjchem-448	146	37	stabilization	stabilization	NOUN
eurjchem-448	146	38	energy	energy	NOUN
eurjchem-448	146	39	(	(	PUNCT
eurjchem-448	146	40	lfse	lfse	ADJ
eurjchem-448	146	41	)	)	PUNCT
eurjchem-448	146	42	were	be	AUX
eurjchem-448	146	43	calculated	calculate	VERB
eurjchem-448	146	44	.	.	PUNCT
eurjchem-448	147	1	mcclure	mcclure	PROPN
eurjchem-448	147	2	’s	’s	PART
eurjchem-448	147	3	parameters	parameter	NOUN
eurjchem-448	147	4	t2	t2	PROPN
eurjchem-448	147	5	g	g	NOUN
eurjchem-448	147	6	and	and	CCONJ
eurjchem-448	147	7	eg	eg	NOUN
eurjchem-448	147	8	depend	depend	VERB
eurjchem-448	147	9	upon	upon	SCONJ
eurjchem-448	147	10	the	the	DET
eurjchem-448	147	11	splitting	splitting	NOUN
eurjchem-448	147	12	of	of	ADP
eurjchem-448	147	13	t2	t2	NOUN
eurjchem-448	147	14	g	g	PROPN
eurjchem-448	147	15	and	and	CCONJ
eurjchem-448	147	16	eg	eg	NOUN
eurjchem-448	147	17	orbitals	orbital	NOUN
eurjchem-448	147	18	observed	observe	VERB
eurjchem-448	147	19	from	from	ADP
eurjchem-448	147	20	crystal	crystal	NOUN
eurjchem-448	147	21	field	field	NOUN
eurjchem-448	147	22	parameters	parameter	NOUN
eurjchem-448	147	23	(	(	PUNCT
eurjchem-448	147	24	ds	ds	ADJ
eurjchem-448	147	25	,	,	PUNCT
eurjchem-448	147	26	dt	dt	NOUN
eurjchem-448	147	27	)	)	PUNCT
eurjchem-448	147	28	.	.	PUNCT
eurjchem-448	148	1	it	it	PRON
eurjchem-448	148	2	confirmed	confirm	VERB
eurjchem-448	148	3	‐bonding	‐bonde	VERB
eurjchem-448	148	4	effect	effect	NOUN
eurjchem-448	148	5	to	to	PART
eurjchem-448	148	6	be	be	AUX
eurjchem-448	148	7	relatively	relatively	ADV
eurjchem-448	148	8	more	more	ADV
eurjchem-448	148	9	important	important	ADJ
eurjchem-448	148	10	along	along	ADP
eurjchem-448	148	11	axial	axial	ADJ
eurjchem-448	148	12	direction	direction	NOUN
eurjchem-448	148	13	than	than	ADP
eurjchem-448	148	14	‐bonding	‐bonde	VERB
eurjchem-448	148	15	.	.	PUNCT
eurjchem-448	149	1	σ‐bonding	σ‐bonde	VERB
eurjchem-448	149	2	along	along	ADP
eurjchem-448	149	3	with	with	ADP
eurjchem-448	149	4	xy‐plane	xy‐plane	PROPN
eurjchem-448	149	5	was	be	AUX
eurjchem-448	149	6	strongly	strongly	ADV
eurjchem-448	149	7	related	relate	VERB
eurjchem-448	149	8	to	to	ADP
eurjchem-448	149	9	negative	negative	ADJ
eurjchem-448	149	10	sign	sign	NOUN
eurjchem-448	149	11	of	of	ADP
eurjchem-448	149	12	σ‐parameter	σ‐parameter	PUNCT
eurjchem-448	149	13	values	value	NOUN
eurjchem-448	149	14	.	.	PUNCT
eurjchem-448	150	1	δ	δ	NOUN
eurjchem-448	150	2	values	value	NOUN
eurjchem-448	150	3	indicate	indicate	VERB
eurjchem-448	150	4	π‐	π‐	ADJ
eurjchem-448	150	5	bonding	bonding	NOUN
eurjchem-448	150	6	effect	effect	NOUN
eurjchem-448	150	7	to	to	PART
eurjchem-448	150	8	be	be	AUX
eurjchem-448	150	9	relatively	relatively	ADV
eurjchem-448	150	10	more	more	ADV
eurjchem-448	150	11	important	important	ADJ
eurjchem-448	150	12	along	along	ADP
eurjchem-448	150	13	the	the	DET
eurjchem-448	150	14	axial	axial	ADJ
eurjchem-448	150	15	direction	direction	NOUN
eurjchem-448	150	16	than	than	ADP
eurjchem-448	150	17	σ‐bonding	σ‐bonde	VERB
eurjchem-448	150	18	.	.	PUNCT
eurjchem-448	151	1	racah	racah	PROPN
eurjchem-448	151	2	inter‐electronic	inter‐electronic	PUNCT
eurjchem-448	151	3	repulsion	repulsion	NOUN
eurjchem-448	151	4	parameter	parameter	NOUN
eurjchem-448	151	5	(	(	PUNCT
eurjchem-448	151	6	bl	bl	INTJ
eurjchem-448	151	7	)	)	PUNCT
eurjchem-448	151	8	was	be	AUX
eurjchem-448	151	9	calculated	calculate	VERB
eurjchem-448	151	10	for	for	ADP
eurjchem-448	151	11	ces	ce	NOUN
eurjchem-448	151	12	of	of	ADP
eurjchem-448	151	13	co(ii	co(ii	PROPN
eurjchem-448	151	14	)	)	PUNCT
eurjchem-448	151	15	using	use	VERB
eurjchem-448	151	16	equation	equation	NOUN
eurjchem-448	151	17	2	2	NUM
eurjchem-448	151	18	.	.	PUNCT
eurjchem-448	151	19	bl	bl	PROPN
eurjchem-448	152	1	=	=	SYM
eurjchem-448	152	2	1/510[7(ν3–2ν2	1/510[7(ν3–2ν2	NUM
eurjchem-448	152	3	)	)	PUNCT
eurjchem-448	153	1	+	+	CCONJ
eurjchem-448	153	2	3{81ν32–16	3{81ν32–16	NUM
eurjchem-448	153	3	ν2(ν2	ν2(ν2	NUM
eurjchem-448	153	4	–	–	PUNCT
eurjchem-448	153	5	ν3)}1/2	ν3)}1/2	NOUN
eurjchem-448	153	6	(	(	PUNCT
eurjchem-448	153	7	2	2	NUM
eurjchem-448	153	8	)	)	PUNCT
eurjchem-448	153	9	values	value	NOUN
eurjchem-448	153	10	of	of	ADP
eurjchem-448	153	11	ligand	ligand	ADJ
eurjchem-448	153	12	field	field	NOUN
eurjchem-448	153	13	parameters	parameter	NOUN
eurjchem-448	153	14	(	(	PUNCT
eurjchem-448	153	15	dq	dq	PROPN
eurjchem-448	153	16	,	,	PUNCT
eurjchem-448	153	17	b	b	NOUN
eurjchem-448	153	18	,	,	PUNCT
eurjchem-448	153	19	β	β	X
eurjchem-448	153	20	and	and	CCONJ
eurjchem-448	153	21	lfse	lfse	ADJ
eurjchem-448	153	22	)	)	PUNCT
eurjchem-448	153	23	and	and	CCONJ
eurjchem-448	153	24	lowering	lower	VERB
eurjchem-448	153	25	in	in	ADP
eurjchem-448	153	26	b	b	PROPN
eurjchem-448	153	27	value	value	NOUN
eurjchem-448	153	28	from	from	ADP
eurjchem-448	153	29	free	free	ADJ
eurjchem-448	153	30	ion	ion	NOUN
eurjchem-448	153	31	value	value	NOUN
eurjchem-448	153	32	for	for	ADP
eurjchem-448	153	33	co(ii	co(ii	ADJ
eurjchem-448	153	34	)	)	PUNCT
eurjchem-448	153	35	i.e.	i.e.	X
eurjchem-448	153	36	1120	1120	NUM
eurjchem-448	153	37	cm‐1	cm‐1	NOUN
eurjchem-448	153	38	,	,	PUNCT
eurjchem-448	153	39	were	be	AUX
eurjchem-448	153	40	determined	determine	VERB
eurjchem-448	153	41	.	.	PUNCT
eurjchem-448	154	1	these	these	DET
eurjchem-448	154	2	results	result	NOUN
eurjchem-448	154	3	suggested	suggest	VERB
eurjchem-448	154	4	37	37	NUM
eurjchem-448	154	5	to	to	PART
eurjchem-448	154	6	44	44	NUM
eurjchem-448	154	7	%	%	NOUN
eurjchem-448	154	8	covalent	covalent	NOUN
eurjchem-448	154	9	nature	nature	NOUN
eurjchem-448	154	10	in	in	ADP
eurjchem-448	154	11	bonding	bonding	NOUN
eurjchem-448	154	12	.	.	PUNCT
eurjchem-448	155	1	racah	racah	PROPN
eurjchem-448	155	2	inter‐electronic	inter‐electronic	PUNCT
eurjchem-448	155	3	repulsion	repulsion	NOUN
eurjchem-448	155	4	parameter	parameter	NOUN
eurjchem-448	155	5	(	(	PUNCT
eurjchem-448	155	6	bl	bl	INTJ
eurjchem-448	155	7	)	)	PUNCT
eurjchem-448	155	8	was	be	AUX
eurjchem-448	155	9	calculated	calculate	VERB
eurjchem-448	155	10	by	by	ADP
eurjchem-448	155	11	equation	equation	NOUN
eurjchem-448	155	12	3	3	NUM
eurjchem-448	155	13	.	.	PUNCT
eurjchem-448	155	14	bl	bl	PUNCT
eurjchem-448	156	1	=	=	NOUN
eurjchem-448	156	2	υ2	υ2	PROPN
eurjchem-448	156	3	+	+	CCONJ
eurjchem-448	156	4	υ3	υ3	PROPN
eurjchem-448	156	5	‐	‐	PUNCT
eurjchem-448	156	6	3υ1/15	3υ1/15	NUM
eurjchem-448	156	7	(	(	PUNCT
eurjchem-448	156	8	3	3	NUM
eurjchem-448	156	9	)	)	PUNCT
eurjchem-448	156	10	for	for	ADP
eurjchem-448	156	11	ni(ii	ni(ii	ADJ
eurjchem-448	156	12	)	)	PUNCT
eurjchem-448	156	13	complex	complex	ADJ
eurjchem-448	156	14	,	,	PUNCT
eurjchem-448	156	15	10dq	10dq	NOUN
eurjchem-448	156	16	=	=	SYM
eurjchem-448	156	17	υ1	υ1	ADJ
eurjchem-448	156	18	and	and	CCONJ
eurjchem-448	156	19	covalence	covalence	NOUN
eurjchem-448	156	20	factor	factor	NOUN
eurjchem-448	156	21	(	(	PUNCT
eurjchem-448	156	22	β	β	NOUN
eurjchem-448	156	23	)	)	PUNCT
eurjchem-448	156	24	was	be	AUX
eurjchem-448	156	25	obtained	obtain	VERB
eurjchem-448	156	26	in	in	ADP
eurjchem-448	156	27	the	the	DET
eurjchem-448	156	28	following	following	ADJ
eurjchem-448	156	29	manner	manner	NOUN
eurjchem-448	156	30	,	,	PUNCT
eurjchem-448	156	31	β	β	X
eurjchem-448	156	32	=	=	PUNCT
eurjchem-448	156	33	bl	bl	PROPN
eurjchem-448	156	34	/	/	SYM
eurjchem-448	156	35	b	b	PROPN
eurjchem-448	156	36	,	,	PUNCT
eurjchem-448	156	37	(	(	PUNCT
eurjchem-448	156	38	where	where	SCONJ
eurjchem-448	156	39	b	b	NOUN
eurjchem-448	156	40	is	be	AUX
eurjchem-448	156	41	free	free	ADJ
eurjchem-448	156	42	ion	ion	NOUN
eurjchem-448	156	43	value	value	NOUN
eurjchem-448	156	44	)	)	PUNCT
eurjchem-448	156	45	.	.	PUNCT
eurjchem-448	157	1	lfse	lfse	PROPN
eurjchem-448	157	2	was	be	AUX
eurjchem-448	157	3	calculated	calculate	VERB
eurjchem-448	157	4	and	and	CCONJ
eurjchem-448	157	5	found	find	VERB
eurjchem-448	157	6	equivalent	equivalent	ADJ
eurjchem-448	157	7	to	to	ADP
eurjchem-448	157	8	12dq	12dq	ADJ
eurjchem-448	157	9	.	.	PUNCT
eurjchem-448	158	1	due	due	ADP
eurjchem-448	158	2	to	to	ADP
eurjchem-448	158	3	splitting	splitting	NOUN
eurjchem-448	158	4	of	of	ADP
eurjchem-448	158	5	υ1	υ1	PROPN
eurjchem-448	158	6	,	,	PUNCT
eurjchem-448	158	7	in	in	ADP
eurjchem-448	158	8	electronic	electronic	ADJ
eurjchem-448	158	9	spectra	spectra	NOUN
eurjchem-448	158	10	of	of	ADP
eurjchem-448	158	11	ces	ce	NOUN
eurjchem-448	158	12	of	of	ADP
eurjchem-448	158	13	ni(ii	ni(ii	NOUN
eurjchem-448	158	14	)	)	PUNCT
eurjchem-448	158	15	,	,	PUNCT
eurjchem-448	158	16	different	different	ADJ
eurjchem-448	158	17	ligand	ligand	ADJ
eurjchem-448	158	18	field	field	NOUN
eurjchem-448	158	19	parameters	parameter	NOUN
eurjchem-448	158	20	i.e.	i.e.	X
eurjchem-448	158	21	hamiltonian	hamiltonian	ADJ
eurjchem-448	158	22	parameters	parameter	NOUN
eurjchem-448	158	23	ds	ds	VERB
eurjchem-448	158	24	,	,	PUNCT
eurjchem-448	158	25	dt	dt	PROPN
eurjchem-448	158	26	,	,	PUNCT
eurjchem-448	158	27	dqxy	dqxy	PROPN
eurjchem-448	158	28	and	and	CCONJ
eurjchem-448	158	29	dqz	dqz	ADJ
eurjchem-448	158	30	were	be	AUX
eurjchem-448	158	31	derived	derive	VERB
eurjchem-448	158	32	from	from	ADP
eurjchem-448	158	33	the	the	DET
eurjchem-448	158	34	transition	transition	NOUN
eurjchem-448	158	35	energy	energy	NOUN
eurjchem-448	158	36	.	.	PUNCT
eurjchem-448	159	1	these	these	DET
eurjchem-448	159	2	values	value	NOUN
eurjchem-448	159	3	helped	help	VERB
eurjchem-448	159	4	to	to	PART
eurjchem-448	159	5	figure	figure	VERB
eurjchem-448	159	6	out	out	ADP
eurjchem-448	159	7	different	different	ADJ
eurjchem-448	159	8	geometrical	geometrical	ADJ
eurjchem-448	159	9	features	feature	NOUN
eurjchem-448	159	10	.	.	PUNCT
eurjchem-448	160	1	dqxy	dqxy	PROPN
eurjchem-448	160	2	and	and	CCONJ
eurjchem-448	160	3	dqz	dqz	ADJ
eurjchem-448	160	4	were	be	AUX
eurjchem-448	160	5	the	the	DET
eurjchem-448	160	6	splitting	splitting	NOUN
eurjchem-448	160	7	parameters	parameter	NOUN
eurjchem-448	160	8	directly	directly	ADV
eurjchem-448	160	9	related	relate	VERB
eurjchem-448	160	10	to	to	ADP
eurjchem-448	160	11	the	the	DET
eurjchem-448	160	12	splitting	splitting	NOUN
eurjchem-448	160	13	in‐plane	in‐plane	ADJ
eurjchem-448	160	14	and	and	CCONJ
eurjchem-448	160	15	axial	axial	ADJ
eurjchem-448	160	16	positions	position	NOUN
eurjchem-448	160	17	[	[	X
eurjchem-448	160	18	21	21	NUM
eurjchem-448	160	19	]	]	PUNCT
eurjchem-448	160	20	.	.	PUNCT
eurjchem-448	161	1	b	b	NOUN
eurjchem-448	161	2	values	value	NOUN
eurjchem-448	161	3	showed	show	VERB
eurjchem-448	161	4	74‐75	74‐75	ADJ
eurjchem-448	161	5	%	%	NOUN
eurjchem-448	161	6	ionic	ionic	ADJ
eurjchem-448	161	7	character	character	NOUN
eurjchem-448	161	8	for	for	ADP
eurjchem-448	161	9	free	free	ADJ
eurjchem-448	161	10	ion	ion	NOUN
eurjchem-448	161	11	(	(	PUNCT
eurjchem-448	161	12	b	b	NOUN
eurjchem-448	161	13	°	°	NUM
eurjchem-448	161	14	=	=	SYM
eurjchem-448	161	15	1041	1041	NUM
eurjchem-448	161	16	cm‐1	cm‐1	NOUN
eurjchem-448	161	17	)	)	PUNCT
eurjchem-448	161	18	.	.	PUNCT
eurjchem-448	162	1	the	the	DET
eurjchem-448	162	2	nephelauxetic	nephelauxetic	ADJ
eurjchem-448	162	3	parameters	parameter	NOUN
eurjchem-448	162	4	calculated	calculate	VERB
eurjchem-448	162	5	had	have	VERB
eurjchem-448	162	6	values	value	NOUN
eurjchem-448	162	7	in	in	ADP
eurjchem-448	162	8	the	the	DET
eurjchem-448	162	9	range	range	NOUN
eurjchem-448	162	10	0.81‐0.78	0.81‐0.78	PROPN
eurjchem-448	162	11	.	.	PUNCT
eurjchem-448	163	1	on	on	ADP
eurjchem-448	163	2	the	the	DET
eurjchem-448	163	3	basis	basis	NOUN
eurjchem-448	163	4	of	of	ADP
eurjchem-448	163	5	these	these	DET
eurjchem-448	163	6	values	value	NOUN
eurjchem-448	163	7	,	,	PUNCT
eurjchem-448	163	8	studied	study	VERB
eurjchem-448	163	9	mc	mc	PROPN
eurjchem-448	163	10	can	can	AUX
eurjchem-448	163	11	be	be	AUX
eurjchem-448	163	12	fitted	fit	VERB
eurjchem-448	163	13	in	in	ADP
eurjchem-448	163	14	the	the	DET
eurjchem-448	163	15	middle	middle	NOUN
eurjchem-448	163	16	of	of	ADP
eurjchem-448	163	17	the	the	DET
eurjchem-448	163	18	nephelauxetic	nephelauxetic	ADJ
eurjchem-448	163	19	series	series	NOUN
eurjchem-448	163	20	.	.	PUNCT
eurjchem-448	164	1	results	result	NOUN
eurjchem-448	164	2	obtained	obtain	VERB
eurjchem-448	164	3	were	be	AUX
eurjchem-448	164	4	helped	help	VERB
eurjchem-448	164	5	to	to	PART
eurjchem-448	164	6	propose	propose	VERB
eurjchem-448	164	7	octahedral	octahedral	ADJ
eurjchem-448	164	8	geometrical	geometrical	ADJ
eurjchem-448	164	9	arrangement	arrangement	NOUN
eurjchem-448	164	10	of	of	ADP
eurjchem-448	164	11	atoms	atom	NOUN
eurjchem-448	164	12	around	around	ADP
eurjchem-448	164	13	ni(ii	ni(ii	NOUN
eurjchem-448	164	14	)	)	PUNCT
eurjchem-448	164	15	and	and	CCONJ
eurjchem-448	164	16	co(ii	co(ii	VERB
eurjchem-448	164	17	)	)	PUNCT
eurjchem-448	164	18	in	in	ADP
eurjchem-448	164	19	ces	ce	NOUN
eurjchem-448	164	20	having	have	VERB
eurjchem-448	164	21	n2s4	n2s4	NOUN
eurjchem-448	164	22	chromophore	chromophore	NOUN
eurjchem-448	164	23	.	.	PUNCT
eurjchem-448	165	1	3.2.5	3.2.5	NUM
eurjchem-448	165	2	.	.	X
eurjchem-448	165	3	electron	electron	NOUN
eurjchem-448	165	4	paramagnetic	paramagnetic	ADJ
eurjchem-448	165	5	resonance	resonance	NOUN
eurjchem-448	165	6	of	of	ADP
eurjchem-448	165	7	ces	ces	X
eurjchem-448	165	8	epr	epr	PROPN
eurjchem-448	165	9	spectra	spectra	NOUN
eurjchem-448	165	10	of	of	ADP
eurjchem-448	165	11	ces	ce	NOUN
eurjchem-448	165	12	of	of	ADP
eurjchem-448	165	13	co(ii	co(ii	PROPN
eurjchem-448	165	14	)	)	PUNCT
eurjchem-448	165	15	were	be	AUX
eurjchem-448	165	16	recorded	record	VERB
eurjchem-448	165	17	using	use	VERB
eurjchem-448	165	18	dpph	dpph	PROPN
eurjchem-448	165	19	as	as	ADP
eurjchem-448	165	20	a	a	DET
eurjchem-448	165	21	reference	reference	NOUN
eurjchem-448	165	22	standard	standard	NOUN
eurjchem-448	165	23	at	at	ADP
eurjchem-448	165	24	liquid	liquid	ADJ
eurjchem-448	165	25	nitrogen	nitrogen	NOUN
eurjchem-448	165	26	temperature	temperature	NOUN
eurjchem-448	165	27	(	(	PUNCT
eurjchem-448	165	28	lnt	lnt	PROPN
eurjchem-448	165	29	)	)	PUNCT
eurjchem-448	165	30	since	since	SCONJ
eurjchem-448	165	31	the	the	DET
eurjchem-448	165	32	rapid	rapid	ADJ
eurjchem-448	165	33	relaxation	relaxation	NOUN
eurjchem-448	165	34	of	of	ADP
eurjchem-448	165	35	co(ii	co(ii	PROPN
eurjchem-448	165	36	)	)	PUNCT
eurjchem-448	165	37	broadened	broaden	VERB
eurjchem-448	165	38	the	the	DET
eurjchem-448	165	39	lines	line	NOUN
eurjchem-448	165	40	at	at	ADP
eurjchem-448	165	41	higher	high	ADJ
eurjchem-448	165	42	temperature	temperature	NOUN
eurjchem-448	165	43	.	.	PUNCT
eurjchem-448	166	1	ces	ce	NOUN
eurjchem-448	166	2	of	of	ADP
eurjchem-448	166	3	co(ii	co(ii	PROPN
eurjchem-448	166	4	)	)	PUNCT
eurjchem-448	166	5	exhibited	exhibit	VERB
eurjchem-448	166	6	a	a	DET
eurjchem-448	166	7	set	set	NOUN
eurjchem-448	166	8	of	of	ADP
eurjchem-448	166	9	six	six	NUM
eurjchem-448	166	10	line	line	NOUN
eurjchem-448	166	11	pattern	pattern	NOUN
eurjchem-448	166	12	and	and	CCONJ
eurjchem-448	166	13	showed	show	VERB
eurjchem-448	166	14	a	a	DET
eurjchem-448	166	15	clear	clear	ADJ
eurjchem-448	166	16	picture	picture	NOUN
eurjchem-448	166	17	about	about	ADP
eurjchem-448	166	18	change	change	NOUN
eurjchem-448	166	19	in	in	ADP
eurjchem-448	166	20	configuration	configuration	NOUN
eurjchem-448	166	21	of	of	ADP
eurjchem-448	166	22	electrons	electron	NOUN
eurjchem-448	166	23	along	along	ADP
eurjchem-448	166	24	their	their	PRON
eurjchem-448	166	25	distribution	distribution	NOUN
eurjchem-448	166	26	around	around	ADP
eurjchem-448	166	27	central	central	ADJ
eurjchem-448	166	28	metal	metal	NOUN
eurjchem-448	166	29	atom	atom	NOUN
eurjchem-448	166	30	after	after	ADP
eurjchem-448	166	31	π‐electrons	π‐electrons	PUNCT
eurjchem-448	166	32	interaction	interaction	NOUN
eurjchem-448	166	33	with	with	ADP
eurjchem-448	166	34	mc	mc	PROPN
eurjchem-448	166	35	represented	represent	VERB
eurjchem-448	166	36	in	in	ADP
eurjchem-448	166	37	figure	figure	NOUN
eurjchem-448	166	38	2	2	NUM
eurjchem-448	166	39	.	.	PUNCT
eurjchem-448	166	40	values	value	NOUN
eurjchem-448	166	41	of	of	ADP
eurjchem-448	166	42	g||	g||	NOUN
eurjchem-448	166	43	,	,	PUNCT
eurjchem-448	166	44	giso	giso	NOUN
eurjchem-448	166	45	and	and	CCONJ
eurjchem-448	166	46	g	g	PROPN
eurjchem-448	166	47	were	be	AUX
eurjchem-448	166	48	found	find	VERB
eurjchem-448	166	49	in	in	ADP
eurjchem-448	166	50	range	range	NOUN
eurjchem-448	166	51	3.95‐3.70	3.95‐3.70	NUM
eurjchem-448	166	52	,	,	PUNCT
eurjchem-448	166	53	2.57‐2.40	2.57‐2.40	NUM
eurjchem-448	166	54	and	and	CCONJ
eurjchem-448	166	55	1.89‐1.64	1.89‐1.64	NUM
eurjchem-448	166	56	,	,	PUNCT
eurjchem-448	166	57	respectively	respectively	ADV
eurjchem-448	166	58	.	.	PUNCT
eurjchem-448	167	1	large	large	ADJ
eurjchem-448	167	2	deviation	deviation	NOUN
eurjchem-448	167	3	in	in	ADP
eurjchem-448	167	4	g	g	NOUN
eurjchem-448	167	5	values	value	NOUN
eurjchem-448	167	6	was	be	AUX
eurjchem-448	167	7	due	due	ADJ
eurjchem-448	167	8	to	to	ADP
eurjchem-448	167	9	large	large	ADJ
eurjchem-448	167	10	angular	angular	ADJ
eurjchem-448	167	11	momentum	momentum	NOUN
eurjchem-448	167	12	contribution	contribution	NOUN
eurjchem-448	167	13	from	from	ADP
eurjchem-448	167	14	the	the	DET
eurjchem-448	167	15	spin	spin	NOUN
eurjchem-448	167	16	only	only	ADV
eurjchem-448	167	17	value	value	NOUN
eurjchem-448	167	18	i.e.	i.e.	X
eurjchem-448	167	19	kumar	kumar	PROPN
eurjchem-448	167	20	et	et	PROPN
eurjchem-448	167	21	al	al	PROPN
eurjchem-448	167	22	.	.	PUNCT
eurjchem-448	167	23	/	/	SYM
eurjchem-448	167	24	european	european	PROPN
eurjchem-448	167	25	journal	journal	PROPN
eurjchem-448	167	26	of	of	ADP
eurjchem-448	167	27	chemistry	chemistry	NOUN
eurjchem-448	167	28	3	3	NUM
eurjchem-448	167	29	(	(	PUNCT
eurjchem-448	167	30	1	1	NUM
eurjchem-448	167	31	)	)	PUNCT
eurjchem-448	167	32	(	(	PUNCT
eurjchem-448	167	33	2012	2012	NUM
eurjchem-448	167	34	)	)	PUNCT
eurjchem-448	167	35	57‐64	57‐64	NUM
eurjchem-448	167	36	61	61	NUM
eurjchem-448	167	37	2.0023	2.0023	NUM
eurjchem-448	167	38	.	.	PUNCT
eurjchem-448	168	1	the	the	DET
eurjchem-448	168	2	main	main	ADJ
eurjchem-448	168	3	observed	observed	ADJ
eurjchem-448	168	4	signals	signal	NOUN
eurjchem-448	168	5	were	be	AUX
eurjchem-448	168	6	typical	typical	ADJ
eurjchem-448	168	7	of	of	ADP
eurjchem-448	168	8	high‐spin	high‐spin	ADJ
eurjchem-448	168	9	co(ii	co(ii	ADJ
eurjchem-448	168	10	)	)	PUNCT
eurjchem-448	168	11	complexes	complex	NOUN
eurjchem-448	168	12	(	(	PUNCT
eurjchem-448	168	13	s	s	NOUN
eurjchem-448	168	14	=	=	SYM
eurjchem-448	168	15	3/2	3/2	NUM
eurjchem-448	168	16	)	)	PUNCT
eurjchem-448	168	17	in	in	ADP
eurjchem-448	168	18	a	a	DET
eurjchem-448	168	19	rhombically	rhombically	ADV
eurjchem-448	168	20	distorted	distort	VERB
eurjchem-448	168	21	octahedral	octahedral	ADJ
eurjchem-448	168	22	complex	complex	NOUN
eurjchem-448	168	23	,	,	PUNCT
eurjchem-448	168	24	interpreted	interpret	VERB
eurjchem-448	168	25	using	use	VERB
eurjchem-448	168	26	an	an	DET
eurjchem-448	168	27	effective	effective	ADJ
eurjchem-448	168	28	s	s	NOUN
eurjchem-448	168	29	=	=	SYM
eurjchem-448	168	30	1/2	1/2	NUM
eurjchem-448	168	31	spin	spin	NOUN
eurjchem-448	168	32	hamiltonian	hamiltonian	NOUN
eurjchem-448	168	33	.	.	PUNCT
eurjchem-448	169	1	epr	epr	PROPN
eurjchem-448	169	2	spectra	spectra	PROPN
eurjchem-448	169	3	of	of	ADP
eurjchem-448	169	4	ces	ce	NOUN
eurjchem-448	169	5	of	of	ADP
eurjchem-448	169	6	co(ii	co(ii	PROPN
eurjchem-448	169	7	)	)	PUNCT
eurjchem-448	169	8	,	,	PUNCT
eurjchem-448	169	9	a	a	DET
eurjchem-448	169	10	frozen	frozen	ADJ
eurjchem-448	169	11	glass	glass	NOUN
eurjchem-448	169	12	at	at	ADP
eurjchem-448	169	13	77	77	NUM
eurjchem-448	169	14	k	k	NOUN
eurjchem-448	169	15	showed	show	VERB
eurjchem-448	169	16	expected	expect	VERB
eurjchem-448	169	17	59co	59co	NOUN
eurjchem-448	169	18	(	(	PUNCT
eurjchem-448	169	19	i	i	NOUN
eurjchem-448	169	20	=	=	SYM
eurjchem-448	169	21	7/2	7/2	NUM
eurjchem-448	169	22	)	)	PUNCT
eurjchem-448	169	23	octet	octet	NOUN
eurjchem-448	169	24	with	with	ADP
eurjchem-448	169	25	gav	gav	PROPN
eurjchem-448	169	26	=	=	PROPN
eurjchem-448	169	27	2.11	2.11	NUM
eurjchem-448	169	28	and	and	CCONJ
eurjchem-448	169	29	hyperfine	hyperfine	ADJ
eurjchem-448	169	30	coupling	couple	VERB
eurjchem-448	169	31	constant	constant	ADJ
eurjchem-448	169	32	aiso	aiso	NOUN
eurjchem-448	169	33	=	=	SYM
eurjchem-448	169	34	38.47	38.47	NUM
eurjchem-448	169	35	g.	g.	NOUN
eurjchem-448	169	36	the	the	DET
eurjchem-448	169	37	frozen‐solution	frozen‐solution	NOUN
eurjchem-448	169	38	spectra	spectra	PROPN
eurjchem-448	169	39	indicated	indicate	VERB
eurjchem-448	169	40	a	a	DET
eurjchem-448	169	41	rhombic	rhombic	ADJ
eurjchem-448	169	42	system	system	NOUN
eurjchem-448	169	43	where	where	SCONJ
eurjchem-448	169	44	all	all	DET
eurjchem-448	169	45	three	three	NUM
eurjchem-448	169	46	axes	axis	NOUN
eurjchem-448	169	47	were	be	AUX
eurjchem-448	169	48	equivalent	equivalent	ADJ
eurjchem-448	169	49	,	,	PUNCT
eurjchem-448	169	50	consistent	consistent	ADJ
eurjchem-448	169	51	with	with	ADP
eurjchem-448	169	52	the	the	DET
eurjchem-448	169	53	geometry	geometry	NOUN
eurjchem-448	169	54	of	of	ADP
eurjchem-448	169	55	the	the	DET
eurjchem-448	169	56	molecule	molecule	NOUN
eurjchem-448	170	1	[	[	X
eurjchem-448	170	2	22	22	NUM
eurjchem-448	170	3	]	]	PUNCT
eurjchem-448	170	4	.	.	PUNCT
eurjchem-448	171	1	figure	figure	NOUN
eurjchem-448	171	2	2	2	NUM
eurjchem-448	171	3	.	.	PUNCT
eurjchem-448	171	4	epr	epr	PROPN
eurjchem-448	171	5	spectrum	spectrum	PROPN
eurjchem-448	171	6	of	of	ADP
eurjchem-448	171	7	reduced	reduce	VERB
eurjchem-448	171	8	ce	ce	PROPN
eurjchem-448	171	9	of	of	ADP
eurjchem-448	171	10	co(ii)cl2	co(ii)cl2	PROPN
eurjchem-448	171	11	at	at	ADP
eurjchem-448	171	12	77	77	NUM
eurjchem-448	171	13	k	k	NOUN
eurjchem-448	171	14	;	;	PUNCT
eurjchem-448	171	15	frequency	frequency	NOUN
eurjchem-448	171	16	9.47	9.47	NUM
eurjchem-448	171	17	ghz	ghz	NOUN
eurjchem-448	171	18	.	.	PUNCT
eurjchem-448	172	1	3.2.6	3.2.6	NUM
eurjchem-448	172	2	.	.	PUNCT
eurjchem-448	172	3	electrochemistry	electrochemistry	NOUN
eurjchem-448	172	4	of	of	ADP
eurjchem-448	172	5	ces	ces	X
eurjchem-448	172	6	the	the	DET
eurjchem-448	172	7	cyclic	cyclic	ADJ
eurjchem-448	172	8	voltammograms	voltammogram	NOUN
eurjchem-448	172	9	(	(	PUNCT
eurjchem-448	172	10	cvs	cvs	PROPN
eurjchem-448	172	11	)	)	PUNCT
eurjchem-448	172	12	of	of	ADP
eurjchem-448	172	13	ces	ce	NOUN
eurjchem-448	172	14	were	be	AUX
eurjchem-448	172	15	observed	observe	VERB
eurjchem-448	172	16	at	at	ADP
eurjchem-448	172	17	oxidation	oxidation	NOUN
eurjchem-448	172	18	and	and	CCONJ
eurjchem-448	172	19	reduction	reduction	NOUN
eurjchem-448	172	20	potentials	potential	NOUN
eurjchem-448	172	21	versus	versus	ADP
eurjchem-448	172	22	different	different	ADJ
eurjchem-448	172	23	scan	scan	ADJ
eurjchem-448	172	24	rates	rate	NOUN
eurjchem-448	172	25	.	.	PUNCT
eurjchem-448	173	1	it	it	PRON
eurjchem-448	173	2	was	be	AUX
eurjchem-448	173	3	evident	evident	ADJ
eurjchem-448	173	4	that	that	SCONJ
eurjchem-448	173	5	used	use	VERB
eurjchem-448	173	6	macrocycle	macrocycle	NOUN
eurjchem-448	173	7	had	have	VERB
eurjchem-448	173	8	lewis	lewis	PROPN
eurjchem-448	173	9	basicities	basicitie	NOUN
eurjchem-448	173	10	due	due	ADJ
eurjchem-448	173	11	to	to	ADP
eurjchem-448	173	12	the	the	DET
eurjchem-448	173	13	presence	presence	NOUN
eurjchem-448	173	14	of	of	ADP
eurjchem-448	173	15	n2s4	n2s4	PRON
eurjchem-448	173	16	donor	donor	NOUN
eurjchem-448	173	17	set	set	VERB
eurjchem-448	173	18	in	in	ADP
eurjchem-448	173	19	macrocycle	macrocycle	NOUN
eurjchem-448	173	20	(	(	PUNCT
eurjchem-448	173	21	mc	mc	PROPN
eurjchem-448	173	22	)	)	PUNCT
eurjchem-448	173	23	.	.	PUNCT
eurjchem-448	174	1	the	the	DET
eurjchem-448	174	2	inherent	inherent	ADJ
eurjchem-448	174	3	kinetic	kinetic	ADJ
eurjchem-448	174	4	stability	stability	NOUN
eurjchem-448	174	5	imparted	impart	VERB
eurjchem-448	174	6	by	by	ADP
eurjchem-448	174	7	n2s4	n2s4	PROPN
eurjchem-448	174	8	macrocycle	macrocycle	NOUN
eurjchem-448	174	9	was	be	AUX
eurjchem-448	174	10	manifested	manifest	VERB
eurjchem-448	174	11	in	in	ADP
eurjchem-448	174	12	the	the	DET
eurjchem-448	174	13	electro‐chemical	electro‐chemical	ADJ
eurjchem-448	174	14	processes	process	NOUN
eurjchem-448	174	15	of	of	ADP
eurjchem-448	174	16	[	[	X
eurjchem-448	174	17	m(l)]x2	m(l)]x2	X
eurjchem-448	174	18	(	(	PUNCT
eurjchem-448	174	19	m	m	PROPN
eurjchem-448	174	20	=	=	SYM
eurjchem-448	174	21	co	co	X
eurjchem-448	174	22	,	,	PUNCT
eurjchem-448	174	23	ni	ni	NOUN
eurjchem-448	174	24	)	)	PUNCT
eurjchem-448	174	25	to	to	PART
eurjchem-448	174	26	generate	generate	VERB
eurjchem-448	174	27	reversible	reversible	ADJ
eurjchem-448	174	28	or	or	CCONJ
eurjchem-448	174	29	quasi	quasi	ADJ
eurjchem-448	174	30	reversible	reversible	ADJ
eurjchem-448	174	31	redox	redox	ADJ
eurjchem-448	174	32	couples	couple	NOUN
eurjchem-448	174	33	in	in	ADP
eurjchem-448	174	34	solutions	solution	NOUN
eurjchem-448	174	35	.	.	PUNCT
eurjchem-448	175	1	ces	ce	NOUN
eurjchem-448	175	2	of	of	ADP
eurjchem-448	175	3	ni(ii	ni(ii	NOUN
eurjchem-448	175	4	)	)	PUNCT
eurjchem-448	175	5	showed	show	VERB
eurjchem-448	175	6	two	two	NUM
eurjchem-448	175	7	successive	successive	ADJ
eurjchem-448	175	8	one	one	NUM
eurjchem-448	175	9	electron	electron	NOUN
eurjchem-448	175	10	processes	process	NOUN
eurjchem-448	175	11	.	.	PUNCT
eurjchem-448	176	1	first	first	ADV
eurjchem-448	176	2	one	one	NUM
eurjchem-448	176	3	being	be	AUX
eurjchem-448	176	4	a	a	DET
eurjchem-448	176	5	irreversible	irreversible	ADJ
eurjchem-448	176	6	couple	couple	NOUN
eurjchem-448	176	7	ni(ii)/ni(i	ni(ii)/ni(i	PROPN
eurjchem-448	176	8	)	)	PUNCT
eurjchem-448	176	9	observed	observe	VERB
eurjchem-448	176	10	at	at	ADP
eurjchem-448	176	11	‐	‐	NOUN
eurjchem-448	176	12	1.48	1.48	NUM
eurjchem-448	176	13	to	to	ADP
eurjchem-448	176	14	‐1.50	‐1.50	NUM
eurjchem-448	176	15	(	(	PUNCT
eurjchem-448	176	16	v	v	NOUN
eurjchem-448	176	17	)	)	PUNCT
eurjchem-448	176	18	and	and	CCONJ
eurjchem-448	176	19	assigned	assign	VERB
eurjchem-448	176	20	as	as	ADP
eurjchem-448	176	21	ni(ii)l	ni(ii)l	NOUN
eurjchem-448	176	22	+	+	CCONJ
eurjchem-448	176	23	e‐	e‐	PROPN
eurjchem-448	176	24	→	→	SYM
eurjchem-448	176	25	ni(i)l	ni(i)l	NUM
eurjchem-448	176	26	.	.	PUNCT
eurjchem-448	177	1	the	the	DET
eurjchem-448	177	2	cathodic	cathodic	NOUN
eurjchem-448	177	3	peak	peak	NOUN
eurjchem-448	177	4	potential	potential	ADJ
eurjchem-448	177	5	difference	difference	NOUN
eurjchem-448	177	6	increased	increase	VERB
eurjchem-448	177	7	with	with	ADP
eurjchem-448	177	8	scan	scan	ADJ
eurjchem-448	177	9	rate	rate	NOUN
eurjchem-448	177	10	.	.	PUNCT
eurjchem-448	178	1	the	the	DET
eurjchem-448	178	2	peak	peak	ADJ
eurjchem-448	178	3	current	current	ADJ
eurjchem-448	178	4	ratio	ratio	NOUN
eurjchem-448	178	5	ipa	ipa	PROPN
eurjchem-448	178	6	/	/	SYM
eurjchem-448	178	7	ipc	ipc	PROPN
eurjchem-448	178	8	was	be	AUX
eurjchem-448	178	9	found	find	VERB
eurjchem-448	178	10	less	less	ADJ
eurjchem-448	178	11	than	than	ADP
eurjchem-448	178	12	unity	unity	NOUN
eurjchem-448	178	13	showing	show	VERB
eurjchem-448	178	14	electron	electron	NOUN
eurjchem-448	178	15	transfer	transfer	NOUN
eurjchem-448	178	16	reaction	reaction	NOUN
eurjchem-448	178	17	to	to	PART
eurjchem-448	178	18	follow	follow	VERB
eurjchem-448	178	19	a	a	DET
eurjchem-448	178	20	chemical	chemical	NOUN
eurjchem-448	178	21	reaction	reaction	NOUN
eurjchem-448	178	22	(	(	PUNCT
eurjchem-448	178	23	ec	ec	PROPN
eurjchem-448	178	24	mechanism	mechanism	NOUN
eurjchem-448	178	25	)	)	PUNCT
eurjchem-448	178	26	.	.	PUNCT
eurjchem-448	179	1	it	it	PRON
eurjchem-448	179	2	seemed	seem	VERB
eurjchem-448	179	3	possible	possible	ADJ
eurjchem-448	179	4	that	that	SCONJ
eurjchem-448	179	5	+1	+1	ADJ
eurjchem-448	179	6	oxidation	oxidation	NOUN
eurjchem-448	179	7	state	state	NOUN
eurjchem-448	179	8	of	of	ADP
eurjchem-448	179	9	nickel	nickel	NOUN
eurjchem-448	179	10	acquired	acquire	VERB
eurjchem-448	179	11	d9	d9	PROPN
eurjchem-448	179	12	or	or	CCONJ
eurjchem-448	179	13	(	(	PUNCT
eurjchem-448	179	14	t62	t62	NOUN
eurjchem-448	179	15	g	g	NOUN
eurjchem-448	179	16	,	,	PUNCT
eurjchem-448	179	17	e3	e3	NOUN
eurjchem-448	179	18	g	g	NOUN
eurjchem-448	179	19	)	)	PUNCT
eurjchem-448	179	20	ground	ground	NOUN
eurjchem-448	179	21	state	state	NOUN
eurjchem-448	179	22	electronic	electronic	ADJ
eurjchem-448	179	23	configuration	configuration	NOUN
eurjchem-448	179	24	and	and	CCONJ
eurjchem-448	179	25	experiences	experience	VERB
eurjchem-448	179	26	dynamic	dynamic	ADJ
eurjchem-448	179	27	jahn‐teller	jahn‐teller	NOUN
eurjchem-448	179	28	distortion	distortion	NOUN
eurjchem-448	179	29	.	.	PUNCT
eurjchem-448	180	1	it	it	PRON
eurjchem-448	180	2	hence	hence	ADV
eurjchem-448	180	3	got	get	AUX
eurjchem-448	180	4	stabilized	stabilize	VERB
eurjchem-448	180	5	because	because	SCONJ
eurjchem-448	180	6	of	of	ADP
eurjchem-448	180	7	possible	possible	ADJ
eurjchem-448	180	8	gain	gain	NOUN
eurjchem-448	180	9	in	in	ADP
eurjchem-448	180	10	crystal	crystal	NOUN
eurjchem-448	180	11	field	field	NOUN
eurjchem-448	180	12	stabilization	stabilization	NOUN
eurjchem-448	180	13	energy	energy	NOUN
eurjchem-448	180	14	(	(	PUNCT
eurjchem-448	180	15	cfse	cfse	ADJ
eurjchem-448	180	16	)	)	PUNCT
eurjchem-448	180	17	.	.	PUNCT
eurjchem-448	181	1	second	second	ADJ
eurjchem-448	181	2	electrode	electrode	NOUN
eurjchem-448	181	3	being	be	AUX
eurjchem-448	181	4	an	an	DET
eurjchem-448	181	5	irreversible	irreversible	ADJ
eurjchem-448	181	6	process	process	NOUN
eurjchem-448	181	7	couple	couple	NOUN
eurjchem-448	181	8	each	each	DET
eurjchem-448	181	9	electrode	electrode	NOUN
eurjchem-448	181	10	couple	couple	NOUN
eurjchem-448	181	11	,	,	PUNCT
eurjchem-448	181	12	showed	show	VERB
eurjchem-448	181	13	ni(ii)/ni(iii	ni(ii)/ni(iii	ADP
eurjchem-448	181	14	)	)	PUNCT
eurjchem-448	181	15	at	at	ADP
eurjchem-448	181	16	1.05	1.05	NUM
eurjchem-448	181	17	to	to	ADP
eurjchem-448	181	18	0.97	0.97	NUM
eurjchem-448	181	19	(	(	PUNCT
eurjchem-448	181	20	v	v	NOUN
eurjchem-448	181	21	)	)	PUNCT
eurjchem-448	181	22	assigned	assign	VERB
eurjchem-448	181	23	as	as	ADP
eurjchem-448	181	24	ni(ii)l	ni(ii)l	NOUN
eurjchem-448	181	25	→	→	SYM
eurjchem-448	181	26	ni(iii)l	ni(iii)l	PROPN
eurjchem-448	182	1	+	+	CCONJ
eurjchem-448	182	2	e‐	e‐	PROPN
eurjchem-448	182	3	peak	peak	NOUN
eurjchem-448	182	4	to	to	PART
eurjchem-448	182	5	peak	peak	VERB
eurjchem-448	182	6	potential	potential	ADJ
eurjchem-448	182	7	separation	separation	NOUN
eurjchem-448	182	8	(	(	PUNCT
eurjchem-448	182	9	∆e	∆e	PROPN
eurjchem-448	182	10	)	)	PUNCT
eurjchem-448	182	11	.	.	PUNCT
eurjchem-448	183	1	the	the	DET
eurjchem-448	183	2	approximately	approximately	ADV
eurjchem-448	183	3	unit	unit	NOUN
eurjchem-448	183	4	value	value	NOUN
eurjchem-448	183	5	of	of	ADP
eurjchem-448	183	6	the	the	DET
eurjchem-448	183	7	cathodic	cathodic	NOUN
eurjchem-448	183	8	to	to	ADP
eurjchem-448	183	9	anodic	anodic	ADJ
eurjchem-448	183	10	peak	peak	NOUN
eurjchem-448	183	11	current	current	ADJ
eurjchem-448	183	12	ratio	ratio	NOUN
eurjchem-448	183	13	(	(	PUNCT
eurjchem-448	183	14	ipa	ipa	PROPN
eurjchem-448	183	15	/	/	SYM
eurjchem-448	183	16	ipc	ipc	PROPN
eurjchem-448	183	17	)	)	PUNCT
eurjchem-448	183	18	was	be	AUX
eurjchem-448	183	19	detected	detect	VERB
eurjchem-448	183	20	for	for	ADP
eurjchem-448	183	21	this	this	DET
eurjchem-448	183	22	couple	couple	NOUN
eurjchem-448	183	23	within	within	ADP
eurjchem-448	183	24	the	the	DET
eurjchem-448	183	25	range	range	NOUN
eurjchem-448	183	26	0.010‐1.000	0.010‐1.000	PUNCT
eurjchem-448	184	1	vs‐1	vs‐1	X
eurjchem-448	184	2	scan	scan	PROPN
eurjchem-448	184	3	rates	rate	NOUN
eurjchem-448	184	4	.	.	PUNCT
eurjchem-448	185	1	it	it	PRON
eurjchem-448	185	2	further	far	ADV
eurjchem-448	185	3	indicated	indicate	VERB
eurjchem-448	185	4	the	the	DET
eurjchem-448	185	5	absence	absence	NOUN
eurjchem-448	185	6	of	of	ADP
eurjchem-448	185	7	subsequent	subsequent	ADJ
eurjchem-448	185	8	chemical	chemical	NOUN
eurjchem-448	185	9	reactions	reaction	NOUN
eurjchem-448	185	10	and	and	CCONJ
eurjchem-448	185	11	stability	stability	NOUN
eurjchem-448	185	12	of	of	ADP
eurjchem-448	185	13	the	the	DET
eurjchem-448	185	14	electrochemically	electrochemically	ADV
eurjchem-448	185	15	generated	generate	VERB
eurjchem-448	185	16	ni(iii	ni(iii	NOUN
eurjchem-448	185	17	)	)	PUNCT
eurjchem-448	185	18	species	specie	NOUN
eurjchem-448	185	19	[	[	X
eurjchem-448	185	20	23	23	NUM
eurjchem-448	185	21	]	]	PUNCT
eurjchem-448	185	22	.	.	PUNCT
eurjchem-448	186	1	figures	figure	NOUN
eurjchem-448	186	2	3	3	NUM
eurjchem-448	186	3	and	and	CCONJ
eurjchem-448	186	4	4	4	NUM
eurjchem-448	186	5	explain	explain	VERB
eurjchem-448	186	6	above	above	ADP
eurjchem-448	186	7	discussed	discuss	VERB
eurjchem-448	186	8	explanatory	explanatory	ADJ
eurjchem-448	186	9	note	note	NOUN
eurjchem-448	186	10	.	.	PUNCT
eurjchem-448	187	1	figure	figure	VERB
eurjchem-448	187	2	3	3	NUM
eurjchem-448	187	3	.	.	PUNCT
eurjchem-448	187	4	cyclic	cyclic	PROPN
eurjchem-448	187	5	voltammogram	voltammogram	PROPN
eurjchem-448	187	6	ce	ce	PROPN
eurjchem-448	187	7	of	of	ADP
eurjchem-448	187	8	ni(ii)cl2	ni(ii)cl2	PROPN
eurjchem-448	187	9	in	in	ADP
eurjchem-448	187	10	the	the	DET
eurjchem-448	187	11	cathodic	cathodic	NOUN
eurjchem-448	187	12	region	region	NOUN
eurjchem-448	187	13	.	.	PUNCT
eurjchem-448	188	1	figure	figure	VERB
eurjchem-448	188	2	4	4	NUM
eurjchem-448	188	3	.	.	PUNCT
eurjchem-448	188	4	cyclic	cyclic	PROPN
eurjchem-448	188	5	voltammogram	voltammogram	PROPN
eurjchem-448	188	6	ce	ce	PROPN
eurjchem-448	188	7	of	of	ADP
eurjchem-448	188	8	ni(ii)cl2	ni(ii)cl2	PROPN
eurjchem-448	188	9	in	in	ADP
eurjchem-448	188	10	the	the	DET
eurjchem-448	188	11	anodic	anodic	ADJ
eurjchem-448	188	12	region	region	NOUN
eurjchem-448	188	13	.	.	PUNCT
eurjchem-448	189	1	cyclic	cyclic	ADJ
eurjchem-448	189	2	voltammograms	voltammogram	NOUN
eurjchem-448	189	3	(	(	PUNCT
eurjchem-448	189	4	cvs	cvs	PROPN
eurjchem-448	189	5	)	)	PUNCT
eurjchem-448	189	6	of	of	ADP
eurjchem-448	189	7	ces	ce	NOUN
eurjchem-448	189	8	of	of	ADP
eurjchem-448	189	9	co(ii	co(ii	PROPN
eurjchem-448	189	10	)	)	PUNCT
eurjchem-448	189	11	were	be	AUX
eurjchem-448	189	12	observed	observe	VERB
eurjchem-448	189	13	in	in	ADP
eurjchem-448	189	14	potential	potential	ADJ
eurjchem-448	189	15	range	range	NOUN
eurjchem-448	189	16	1.05	1.05	NUM
eurjchem-448	189	17	to	to	ADP
eurjchem-448	189	18	‐1.50	‐1.50	PROPN
eurjchem-448	189	19	(	(	PUNCT
eurjchem-448	189	20	v	v	NOUN
eurjchem-448	189	21	)	)	PUNCT
eurjchem-448	189	22	versus	versus	ADP
eurjchem-448	189	23	ag	ag	PROPN
eurjchem-448	189	24	/	/	SYM
eurjchem-448	189	25	agcl	agcl	NOUN
eurjchem-448	189	26	for	for	ADP
eurjchem-448	189	27	scan	scan	ADJ
eurjchem-448	189	28	rate	rate	NOUN
eurjchem-448	189	29	of	of	ADP
eurjchem-448	189	30	0.025	0.025	NUM
eurjchem-448	189	31	to	to	ADP
eurjchem-448	189	32	0.50	0.50	NUM
eurjchem-448	189	33	vs‐1	vs‐1	NOUN
eurjchem-448	189	34	.	.	PUNCT
eurjchem-448	190	1	the	the	DET
eurjchem-448	190	2	half‐wave	half‐wave	PROPN
eurjchem-448	190	3	potentials	potential	VERB
eurjchem-448	190	4	for	for	SCONJ
eurjchem-448	190	5	the	the	DET
eurjchem-448	190	6	reversible	reversible	ADJ
eurjchem-448	190	7	co(iii)/co(ii	co(iii)/co(ii	PROPN
eurjchem-448	190	8	)	)	PUNCT
eurjchem-448	190	9	and	and	CCONJ
eurjchem-448	190	10	co(ii)/co(i	co(ii)/co(i	PROPN
eurjchem-448	190	11	)	)	PUNCT
eurjchem-448	190	12	redox	redox	ADJ
eurjchem-448	190	13	couples	couple	NOUN
eurjchem-448	190	14	were	be	AUX
eurjchem-448	190	15	determined	determine	VERB
eurjchem-448	190	16	as	as	ADP
eurjchem-448	190	17	average	average	ADJ
eurjchem-448	190	18	of	of	ADP
eurjchem-448	190	19	cathodic	cathodic	NOUN
eurjchem-448	190	20	and	and	CCONJ
eurjchem-448	190	21	anodic	anodic	ADJ
eurjchem-448	190	22	peak	peak	NOUN
eurjchem-448	190	23	potentials	potential	NOUN
eurjchem-448	190	24	of	of	ADP
eurjchem-448	190	25	the	the	DET
eurjchem-448	190	26	processes	process	NOUN
eurjchem-448	190	27	.	.	PUNCT
eurjchem-448	191	1	in	in	ADP
eurjchem-448	191	2	anodic	anodic	ADJ
eurjchem-448	191	3	region	region	NOUN
eurjchem-448	191	4	,	,	PUNCT
eurjchem-448	191	5	one	one	NUM
eurjchem-448	191	6	quasi‐reversible	quasi‐reversible	ADJ
eurjchem-448	191	7	oxidation	oxidation	NOUN
eurjchem-448	191	8	process	process	NOUN
eurjchem-448	191	9	at	at	ADP
eurjchem-448	191	10	0.25	0.25	NUM
eurjchem-448	191	11	to	to	ADP
eurjchem-448	191	12	0.20	0.20	NUM
eurjchem-448	191	13	(	(	PUNCT
eurjchem-448	191	14	v	v	NOUN
eurjchem-448	191	15	)	)	PUNCT
eurjchem-448	191	16	was	be	AUX
eurjchem-448	191	17	observed	observe	VERB
eurjchem-448	191	18	.	.	PUNCT
eurjchem-448	192	1	in	in	ADP
eurjchem-448	192	2	addition	addition	NOUN
eurjchem-448	192	3	,	,	PUNCT
eurjchem-448	192	4	it	it	PRON
eurjchem-448	192	5	exhibited	exhibit	VERB
eurjchem-448	192	6	a	a	DET
eurjchem-448	192	7	cathodic	cathodic	ADJ
eurjchem-448	192	8	wave	wave	NOUN
eurjchem-448	192	9	at	at	ADP
eurjchem-448	192	10	‐1.25	‐1.25	NOUN
eurjchem-448	192	11	to	to	ADP
eurjchem-448	192	12	‐1.20	‐1.20	X
eurjchem-448	192	13	(	(	PUNCT
eurjchem-448	192	14	v	v	NOUN
eurjchem-448	192	15	)	)	PUNCT
eurjchem-448	192	16	corresponding	correspond	VERB
eurjchem-448	192	17	to	to	ADP
eurjchem-448	192	18	co(ii	co(ii	VERB
eurjchem-448	192	19	)	)	PUNCT
eurjchem-448	192	20	centered	center	VERB
eurjchem-448	192	21	reduction	reduction	NOUN
eurjchem-448	192	22	process	process	NOUN
eurjchem-448	192	23	.	.	PUNCT
eurjchem-448	193	1	first	first	ADJ
eurjchem-448	193	2	reduction	reduction	NOUN
eurjchem-448	193	3	process	process	NOUN
eurjchem-448	193	4	had	have	VERB
eurjchem-448	193	5	about	about	ADP
eurjchem-448	193	6	a	a	DET
eurjchem-448	193	7	unit	unit	NOUN
eurjchem-448	193	8	ratio	ratio	NOUN
eurjchem-448	193	9	of	of	ADP
eurjchem-448	193	10	anodic	anodic	NOUN
eurjchem-448	193	11	to	to	ADP
eurjchem-448	193	12	cathodic	cathodic	NOUN
eurjchem-448	193	13	peak	peak	NOUN
eurjchem-448	193	14	currents	current	NOUN
eurjchem-448	193	15	(	(	PUNCT
eurjchem-448	193	16	ipa	ipa	PROPN
eurjchem-448	193	17	/	/	SYM
eurjchem-448	193	18	ipc	ipc	PROPN
eurjchem-448	193	19	)	)	PUNCT
eurjchem-448	193	20	.	.	PUNCT
eurjchem-448	194	1	the	the	DET
eurjchem-448	194	2	ratio	ratio	NOUN
eurjchem-448	194	3	observed	observe	VERB
eurjchem-448	194	4	for	for	ADP
eurjchem-448	194	5	second	second	ADJ
eurjchem-448	194	6	reduction	reduction	NOUN
eurjchem-448	194	7	process	process	NOUN
eurjchem-448	194	8	was	be	AUX
eurjchem-448	194	9	different	different	ADJ
eurjchem-448	194	10	and	and	CCONJ
eurjchem-448	194	11	showed	show	VERB
eurjchem-448	194	12	deviations	deviation	NOUN
eurjchem-448	194	13	from	from	ADP
eurjchem-448	194	14	unity	unity	NOUN
eurjchem-448	194	15	due	due	ADJ
eurjchem-448	194	16	to	to	ADP
eurjchem-448	194	17	residual	residual	ADJ
eurjchem-448	194	18	current	current	NOUN
eurjchem-448	194	19	at	at	ADP
eurjchem-448	194	20	a	a	DET
eurjchem-448	194	21	low	low	ADJ
eurjchem-448	194	22	potential	potential	NOUN
eurjchem-448	194	23	.	.	PUNCT
eurjchem-448	195	1	the	the	DET
eurjchem-448	195	2	ipa	ipa	PROPN
eurjchem-448	195	3	/	/	SYM
eurjchem-448	195	4	ipc	ipc	PROPN
eurjchem-448	195	5	values	value	NOUN
eurjchem-448	195	6	at	at	ADP
eurjchem-448	195	7	slow	slow	ADJ
eurjchem-448	195	8	scan	scan	ADJ
eurjchem-448	195	9	rates	rate	NOUN
eurjchem-448	195	10	were	be	AUX
eurjchem-448	195	11	slightly	slightly	ADV
eurjchem-448	195	12	lower	low	ADJ
eurjchem-448	195	13	than	than	ADP
eurjchem-448	195	14	unity	unity	NOUN
eurjchem-448	195	15	but	but	CCONJ
eurjchem-448	195	16	increased	increase	VERB
eurjchem-448	195	17	with	with	ADP
eurjchem-448	195	18	increasing	increase	VERB
eurjchem-448	195	19	scan	scan	ADJ
eurjchem-448	195	20	rates	rate	NOUN
eurjchem-448	195	21	.	.	PUNCT
eurjchem-448	196	1	it	it	PRON
eurjchem-448	196	2	was	be	AUX
eurjchem-448	196	3	a	a	DET
eurjchem-448	196	4	characteristic	characteristic	ADJ
eurjchem-448	196	5	response	response	NOUN
eurjchem-448	196	6	of	of	ADP
eurjchem-448	196	7	a	a	DET
eurjchem-448	196	8	slow	slow	ADJ
eurjchem-448	196	9	chemical	chemical	NOUN
eurjchem-448	196	10	reaction	reaction	NOUN
eurjchem-448	196	11	succeeding	succeed	VERB
eurjchem-448	196	12	the	the	DET
eurjchem-448	196	13	electron	electron	NOUN
eurjchem-448	196	14	transfer	transfer	NOUN
eurjchem-448	196	15	reaction	reaction	NOUN
eurjchem-448	196	16	.	.	PUNCT
eurjchem-448	197	1	these	these	DET
eurjchem-448	197	2	results	result	NOUN
eurjchem-448	197	3	were	be	AUX
eurjchem-448	197	4	assigned	assign	VERB
eurjchem-448	197	5	to	to	ADP
eurjchem-448	197	6	simple	simple	ADJ
eurjchem-448	197	7	one‐electron	one‐electron	ADJ
eurjchem-448	197	8	processes	process	NOUN
eurjchem-448	197	9	:	:	PUNCT
eurjchem-448	198	1	[	[	X
eurjchem-448	198	2	co(iii)l	co(iii)l	X
eurjchem-448	198	3	]	]	X
eurjchem-448	198	4	+	+	CCONJ
eurjchem-448	198	5	‐e	‐e	NOUN
eurjchem-448	198	6	→	→	SYM
eurjchem-448	198	7	[	[	X
eurjchem-448	198	8	co(ii)l]‐	co(ii)l]‐	X
eurjchem-448	198	9	(	(	PUNCT
eurjchem-448	198	10	4	4	NUM
eurjchem-448	198	11	)	)	PUNCT
eurjchem-448	198	12	and	and	CCONJ
eurjchem-448	198	13	[	[	X
eurjchem-448	198	14	co(ii)l]‐	co(ii)l]‐	X
eurjchem-448	198	15	+	+	CCONJ
eurjchem-448	198	16	‐e	‐e	NOUN
eurjchem-448	198	17	→	→	SYM
eurjchem-448	198	18	[	[	X
eurjchem-448	198	19	co(i)l]2‐	co(i)l]2‐	X
eurjchem-448	198	20	(	(	PUNCT
eurjchem-448	198	21	5	5	NUM
eurjchem-448	198	22	)	)	PUNCT
eurjchem-448	198	23	with	with	ADP
eurjchem-448	198	24	different	different	ADJ
eurjchem-448	198	25	values	value	NOUN
eurjchem-448	198	26	of	of	ADP
eurjchem-448	198	27	anodic	anodic	ADJ
eurjchem-448	198	28	and	and	CCONJ
eurjchem-448	198	29	cathodic	cathodic	NOUN
eurjchem-448	198	30	peak	peak	NOUN
eurjchem-448	198	31	separation	separation	NOUN
eurjchem-448	198	32	.	.	PUNCT
eurjchem-448	199	1	in	in	ADP
eurjchem-448	199	2	controlled	control	VERB
eurjchem-448	199	3	potential	potential	ADJ
eurjchem-448	199	4	electrolysis	electrolysis	NOUN
eurjchem-448	199	5	,	,	PUNCT
eurjchem-448	199	6	it	it	PRON
eurjchem-448	199	7	was	be	AUX
eurjchem-448	199	8	revealed	reveal	VERB
eurjchem-448	199	9	that	that	SCONJ
eurjchem-448	199	10	a	a	DET
eurjchem-448	199	11	single	single	ADJ
eurjchem-448	199	12	electron	electron	NOUN
eurjchem-448	199	13	was	be	AUX
eurjchem-448	199	14	involved	involve	VERB
eurjchem-448	199	15	in	in	ADP
eurjchem-448	199	16	each	each	DET
eurjchem-448	199	17	reduction	reduction	NOUN
eurjchem-448	199	18	step	step	NOUN
eurjchem-448	199	19	.	.	PUNCT
eurjchem-448	200	1	the	the	DET
eurjchem-448	200	2	low	low	ADJ
eurjchem-448	200	3	peak	peak	NOUN
eurjchem-448	200	4	separation	separation	NOUN
eurjchem-448	200	5	was	be	AUX
eurjchem-448	200	6	observed	observe	VERB
eurjchem-448	200	7	for	for	ADP
eurjchem-448	200	8	the	the	DET
eurjchem-448	200	9	co(iii)/co(ii	co(iii)/co(ii	PROPN
eurjchem-448	200	10	)	)	PUNCT
eurjchem-448	200	11	and	and	CCONJ
eurjchem-448	200	12	co(ii)/co(i	co(ii)/co(i	PROPN
eurjchem-448	200	13	)	)	PUNCT
eurjchem-448	200	14	couples	couple	NOUN
eurjchem-448	200	15	which	which	PRON
eurjchem-448	200	16	explained	explain	VERB
eurjchem-448	200	17	stable	stable	ADJ
eurjchem-448	200	18	behaviour	behaviour	NOUN
eurjchem-448	200	19	of	of	ADP
eurjchem-448	200	20	ces	ce	NOUN
eurjchem-448	200	21	and	and	CCONJ
eurjchem-448	200	22	remained	remain	VERB
eurjchem-448	200	23	unchanged	unchanged	ADJ
eurjchem-448	200	24	during	during	ADP
eurjchem-448	200	25	the	the	DET
eurjchem-448	200	26	reduction	reduction	NOUN
eurjchem-448	200	27	processes	process	NOUN
eurjchem-448	200	28	.	.	PUNCT
eurjchem-448	201	1	electron	electron	NOUN
eurjchem-448	201	2	transfer	transfer	NOUN
eurjchem-448	201	3	processes	process	NOUN
eurjchem-448	201	4	were	be	AUX
eurjchem-448	201	5	not	not	PART
eurjchem-448	201	6	followed	follow	VERB
eurjchem-448	201	7	by	by	ADP
eurjchem-448	201	8	a	a	DET
eurjchem-448	201	9	chemical	chemical	NOUN
eurjchem-448	201	10	reaction	reaction	NOUN
eurjchem-448	201	11	upon	upon	SCONJ
eurjchem-448	201	12	a	a	DET
eurjchem-448	201	13	reversal	reversal	NOUN
eurjchem-448	201	14	scan	scan	NOUN
eurjchem-448	201	15	.	.	PUNCT
eurjchem-448	202	1	e0.5	e0.5	NOUN
eurjchem-448	202	2	values	value	NOUN
eurjchem-448	202	3	were	be	AUX
eurjchem-448	202	4	found	find	VERB
eurjchem-448	202	5	independent	independent	ADJ
eurjchem-448	202	6	of	of	ADP
eurjchem-448	202	7	scan	scan	ADJ
eurjchem-448	202	8	rate	rate	NOUN
eurjchem-448	202	9	but	but	CCONJ
eurjchem-448	202	10	showed	show	VERB
eurjchem-448	202	11	small	small	ADJ
eurjchem-448	202	12	dependence	dependence	NOUN
eurjchem-448	202	13	peak	peak	NOUN
eurjchem-448	202	14	potential	potential	NOUN
eurjchem-448	202	15	.	.	PUNCT
eurjchem-448	203	1	ep	ep	NOUN
eurjchem-448	203	2	depends	depend	VERB
eurjchem-448	203	3	totally	totally	ADV
eurjchem-448	203	4	on	on	ADP
eurjchem-448	203	5	scan	scan	ADJ
eurjchem-448	203	6	rate	rate	NOUN
eurjchem-448	203	7	observed	observe	VERB
eurjchem-448	203	8	in	in	ADP
eurjchem-448	203	9	range	range	NOUN
eurjchem-448	203	10	60‐800	60‐800	NUM
eurjchem-448	203	11	mvs‐1	mvs‐1	NOUN
eurjchem-448	203	12	.	.	PUNCT
eurjchem-448	204	1	after	after	ADP
eurjchem-448	204	2	scanning	scan	VERB
eurjchem-448	204	3	the	the	DET
eurjchem-448	204	4	second	second	ADJ
eurjchem-448	204	5	cycle	cycle	NOUN
eurjchem-448	204	6	,	,	PUNCT
eurjchem-448	204	7	no	no	DET
eurjchem-448	204	8	change	change	NOUN
eurjchem-448	204	9	in	in	ADP
eurjchem-448	204	10	potential	potential	NOUN
eurjchem-448	204	11	was	be	AUX
eurjchem-448	204	12	observed	observe	VERB
eurjchem-448	204	13	in	in	ADP
eurjchem-448	204	14	cathodic	cathodic	NOUN
eurjchem-448	204	15	and	and	CCONJ
eurjchem-448	204	16	anodic	anodic	ADJ
eurjchem-448	204	17	waves	wave	NOUN
eurjchem-448	204	18	for	for	ADP
eurjchem-448	204	19	these	these	DET
eurjchem-448	204	20	electrode	electrode	NOUN
eurjchem-448	204	21	processes	process	NOUN
eurjchem-448	204	22	comparatively	comparatively	ADV
eurjchem-448	204	23	to	to	ADP
eurjchem-448	204	24	the	the	DET
eurjchem-448	204	25	reductions	reduction	NOUN
eurjchem-448	204	26	occurred	occur	VERB
eurjchem-448	204	27	at	at	ADP
eurjchem-448	204	28	the	the	DET
eurjchem-448	204	29	same	same	ADJ
eurjchem-448	204	30	potentials	potential	NOUN
eurjchem-448	204	31	as	as	SCONJ
eurjchem-448	204	32	observed	observe	VERB
eurjchem-448	204	33	in	in	ADP
eurjchem-448	204	34	the	the	DET
eurjchem-448	204	35	first	first	ADJ
eurjchem-448	204	36	cycle	cycle	NOUN
eurjchem-448	204	37	.	.	PUNCT
eurjchem-448	205	1	the	the	DET
eurjchem-448	205	2	shifts	shift	NOUN
eurjchem-448	205	3	and	and	CCONJ
eurjchem-448	205	4	reversibility	reversibility	NOUN
eurjchem-448	205	5	were	be	AUX
eurjchem-448	205	6	apparently	apparently	ADV
eurjchem-448	205	7	close	close	ADJ
eurjchem-448	205	8	to	to	ADP
eurjchem-448	205	9	high	high	ADJ
eurjchem-448	205	10	degree	degree	NOUN
eurjchem-448	205	11	of	of	ADP
eurjchem-448	205	12	electron	electron	NOUN
eurjchem-448	205	13	delocalization	delocalization	NOUN
eurjchem-448	205	14	in	in	ADP
eurjchem-448	205	15	ces	ce	NOUN
eurjchem-448	205	16	with	with	ADP
eurjchem-448	205	17	n2s4	n2s4	PRON
eurjchem-448	205	18	donor	donor	NOUN
eurjchem-448	205	19	set	set	VERB
eurjchem-448	205	20	and	and	CCONJ
eurjchem-448	205	21	additional	additional	ADJ
eurjchem-448	205	22	benzene	benzene	NOUN
eurjchem-448	205	23	units	unit	NOUN
eurjchem-448	205	24	.	.	PUNCT
eurjchem-448	206	1	the	the	DET
eurjchem-448	206	2	lower	low	ADJ
eurjchem-448	206	3	oxidation	oxidation	NOUN
eurjchem-448	206	4	states	state	NOUN
eurjchem-448	206	5	,	,	PUNCT
eurjchem-448	206	6	co(i	co(i	NUM
eurjchem-448	206	7	)	)	PUNCT
eurjchem-448	206	8	was	be	AUX
eurjchem-448	206	9	probably	probably	ADV
eurjchem-448	206	10	stabilized	stabilize	VERB
eurjchem-448	206	11	by	by	ADP
eurjchem-448	206	12	thiol	thiol	PROPN
eurjchem-448	206	13	schiff‐base	schiff‐base	PROPN
eurjchem-448	206	14	ligand	ligand	PROPN
eurjchem-448	206	15	unit	unit	NOUN
eurjchem-448	206	16	due	due	ADP
eurjchem-448	206	17	to	to	ADP
eurjchem-448	206	18	sulphur	sulphur	NOUN
eurjchem-448	206	19	atom	atom	NOUN
eurjchem-448	206	20	having	have	VERB
eurjchem-448	206	21	dπ	dπ	ADP
eurjchem-448	206	22	orbitals	orbital	NOUN
eurjchem-448	206	23	.	.	PUNCT
eurjchem-448	207	1	imines	imine	NOUN
eurjchem-448	207	2	groups	group	NOUN
eurjchem-448	207	3	played	play	VERB
eurjchem-448	207	4	an	an	DET
eurjchem-448	207	5	effective	effective	ADJ
eurjchem-448	207	6	role	role	NOUN
eurjchem-448	207	7	with	with	ADP
eurjchem-448	207	8	back	back	ADJ
eurjchem-448	207	9	donation	donation	NOUN
eurjchem-448	207	10	and	and	CCONJ
eurjchem-448	207	11	formed	form	VERB
eurjchem-448	207	12	equality	equality	NOUN
eurjchem-448	207	13	bridges	bridge	NOUN
eurjchem-448	207	14	.	.	PUNCT
eurjchem-448	208	1	on	on	ADP
eurjchem-448	208	2	increasing	increase	VERB
eurjchem-448	208	3	the	the	DET
eurjchem-448	208	4	number	number	NOUN
eurjchem-448	208	5	of	of	ADP
eurjchem-448	208	6	aromatic	aromatic	ADJ
eurjchem-448	208	7	rings	ring	NOUN
eurjchem-448	208	8	or	or	CCONJ
eurjchem-448	208	9	double	double	ADJ
eurjchem-448	208	10	bonds	bond	NOUN
eurjchem-448	208	11	in	in	ADP
eurjchem-448	208	12	mcs	mcs	PROPN
eurjchem-448	208	13	,	,	PUNCT
eurjchem-448	208	14	reduction	reduction	NOUN
eurjchem-448	208	15	of	of	ADP
eurjchem-448	208	16	co(ii	co(ii	PROPN
eurjchem-448	208	17	)	)	PUNCT
eurjchem-448	208	18	to	to	ADP
eurjchem-448	208	19	co(i	co(i	ADV
eurjchem-448	208	20	)	)	PUNCT
eurjchem-448	208	21	facilitates	facilitate	VERB
eurjchem-448	208	22	.	.	PUNCT
eurjchem-448	209	1	the	the	DET
eurjchem-448	209	2	electro‐generated	electro‐generate	VERB
eurjchem-448	209	3	co(i	co(i	X
eurjchem-448	209	4	)	)	PUNCT
eurjchem-448	209	5	species	specie	NOUN
eurjchem-448	209	6	exhibited	exhibit	VERB
eurjchem-448	209	7	reversible	reversible	ADJ
eurjchem-448	209	8	and	and	CCONJ
eurjchem-448	209	9	stable	stable	ADJ
eurjchem-448	209	10	character	character	NOUN
eurjchem-448	209	11	.	.	PUNCT
eurjchem-448	210	1	it	it	PRON
eurjchem-448	210	2	will	will	AUX
eurjchem-448	210	3	likely	likely	ADV
eurjchem-448	210	4	facilitate	facilitate	VERB
eurjchem-448	210	5	a	a	DET
eurjchem-448	210	6	catalytic	catalytic	ADJ
eurjchem-448	210	7	reduction	reduction	NOUN
eurjchem-448	210	8	of	of	ADP
eurjchem-448	210	9	halogenated	halogenated	ADJ
eurjchem-448	210	10	organic	organic	ADJ
eurjchem-448	210	11	species	specie	NOUN
eurjchem-448	210	12	as	as	ADV
eurjchem-448	210	13	well	well	ADV
eurjchem-448	210	14	as	as	ADP
eurjchem-448	210	15	co(iii)/co(ii	co(iii)/co(ii	NOUN
eurjchem-448	210	16	)	)	PUNCT
eurjchem-448	210	17	species	specie	NOUN
eurjchem-448	210	18	.	.	PUNCT
eurjchem-448	211	1	so	so	ADV
eurjchem-448	211	2	the	the	DET
eurjchem-448	211	3	oxidation	oxidation	NOUN
eurjchem-448	211	4	processes	process	NOUN
eurjchem-448	211	5	and	and	CCONJ
eurjchem-448	211	6	the	the	DET
eurjchem-448	211	7	splitting	splitting	NOUN
eurjchem-448	211	8	of	of	ADP
eurjchem-448	211	9	the	the	DET
eurjchem-448	211	10	wave	wave	NOUN
eurjchem-448	211	11	were	be	AUX
eurjchem-448	211	12	based	base	VERB
eurjchem-448	211	13	on	on	ADP
eurjchem-448	211	14	mcs	mcs	PROPN
eurjchem-448	211	15	and	and	CCONJ
eurjchem-448	211	16	probably	probably	ADV
eurjchem-448	211	17	due	due	ADP
eurjchem-448	211	18	to	to	ADP
eurjchem-448	211	19	the	the	DET
eurjchem-448	211	20	presence	presence	NOUN
eurjchem-448	211	21	of	of	ADP
eurjchem-448	211	22	four	four	NUM
eurjchem-448	211	23	thiolate	thiolate	ADJ
eurjchem-448	211	24	groups	group	NOUN
eurjchem-448	211	25	of	of	ADP
eurjchem-448	211	26	ces	ce	NOUN
eurjchem-448	211	27	,	,	PUNCT
eurjchem-448	211	28	oxidized	oxidize	VERB
eurjchem-448	211	29	at	at	ADP
eurjchem-448	211	30	the	the	DET
eurjchem-448	211	31	different	different	ADJ
eurjchem-448	211	32	potentials	potential	NOUN
eurjchem-448	211	33	.	.	PUNCT
eurjchem-448	212	1	the	the	DET
eurjchem-448	212	2	magnitude	magnitude	NOUN
eurjchem-448	212	3	of	of	ADP
eurjchem-448	212	4	half	half	ADJ
eurjchem-448	212	5	wave	wave	NOUN
eurjchem-448	212	6	potential	potential	NOUN
eurjchem-448	212	7	(	(	PUNCT
eurjchem-448	212	8	e0.5	e0.5	NOUN
eurjchem-448	212	9	)	)	PUNCT
eurjchem-448	212	10	generally	generally	ADV
eurjchem-448	212	11	shifts	shift	NOUN
eurjchem-448	212	12	towards	towards	ADP
eurjchem-448	212	13	negative	negative	ADJ
eurjchem-448	212	14	potential	potential	NOUN
eurjchem-448	212	15	when	when	SCONJ
eurjchem-448	212	16	metal	metal	NOUN
eurjchem-448	212	17	ion	ion	NOUN
eurjchem-448	212	18	chelated	chelate	VERB
eurjchem-448	212	19	with	with	ADP
eurjchem-448	212	20	62	62	NUM
eurjchem-448	212	21	kumar	kumar	PROPN
eurjchem-448	212	22	et	et	PROPN
eurjchem-448	212	23	al	al	PROPN
eurjchem-448	212	24	.	.	PUNCT
eurjchem-448	212	25	/	/	SYM
eurjchem-448	212	26	european	european	PROPN
eurjchem-448	212	27	journal	journal	PROPN
eurjchem-448	212	28	of	of	ADP
eurjchem-448	212	29	chemistry	chemistry	NOUN
eurjchem-448	212	30	3	3	NUM
eurjchem-448	212	31	(	(	PUNCT
eurjchem-448	212	32	1	1	NUM
eurjchem-448	212	33	)	)	PUNCT
eurjchem-448	212	34	(	(	PUNCT
eurjchem-448	212	35	2012	2012	NUM
eurjchem-448	212	36	)	)	PUNCT
eurjchem-448	212	37	57‐64	57‐64	NUM
eurjchem-448	212	38	strong	strong	ADJ
eurjchem-448	212	39	σ‐donor	σ‐donor	X
eurjchem-448	212	40	ligands	ligand	NOUN
eurjchem-448	212	41	.	.	PUNCT
eurjchem-448	213	1	the	the	DET
eurjchem-448	213	2	present	present	ADJ
eurjchem-448	213	3	n2s4	n2s4	PROPN
eurjchem-448	213	4	donor	donor	NOUN
eurjchem-448	213	5	macrocycle	macrocycle	NOUN
eurjchem-448	213	6	,	,	PUNCT
eurjchem-448	213	7	a	a	DET
eurjchem-448	213	8	mimic	mimic	NOUN
eurjchem-448	213	9	to	to	ADP
eurjchem-448	213	10	cyclic	cyclic	ADJ
eurjchem-448	213	11	hexadentate	hexadentate	NOUN
eurjchem-448	213	12	,	,	PUNCT
eurjchem-448	213	13	behaves	behave	VERB
eurjchem-448	213	14	as	as	ADP
eurjchem-448	213	15	a	a	DET
eurjchem-448	213	16	good	good	ADJ
eurjchem-448	213	17	σ‐chelator	σ‐chelator	NOUN
eurjchem-448	213	18	through	through	ADP
eurjchem-448	213	19	amine	amine	NOUN
eurjchem-448	213	20	/	/	SYM
eurjchem-448	213	21	thioether	thioether	NOUN
eurjchem-448	213	22	group	group	NOUN
eurjchem-448	213	23	.	.	PUNCT
eurjchem-448	214	1	however	however	ADV
eurjchem-448	214	2	,	,	PUNCT
eurjchem-448	214	3	the	the	DET
eurjchem-448	214	4	position	position	NOUN
eurjchem-448	214	5	of	of	ADP
eurjchem-448	214	6	redox	redox	ADJ
eurjchem-448	214	7	wave	wave	NOUN
eurjchem-448	214	8	depends	depend	VERB
eurjchem-448	214	9	on	on	ADP
eurjchem-448	214	10	various	various	ADJ
eurjchem-448	214	11	factors	factor	NOUN
eurjchem-448	214	12	such	such	ADJ
eurjchem-448	214	13	as	as	ADP
eurjchem-448	214	14	nature	nature	NOUN
eurjchem-448	214	15	of	of	ADP
eurjchem-448	214	16	exo‐cyclic	exo‐cyclic	ADJ
eurjchem-448	214	17	substituents	substituent	NOUN
eurjchem-448	214	18	donor	donor	NOUN
eurjchem-448	214	19	sites	site	NOUN
eurjchem-448	214	20	their	their	PRON
eurjchem-448	214	21	π‐bonding	π‐bonde	VERB
eurjchem-448	214	22	character	character	NOUN
eurjchem-448	214	23	within	within	ADP
eurjchem-448	214	24	ligand	ligand	NOUN
eurjchem-448	214	25	[	[	X
eurjchem-448	214	26	24	24	NUM
eurjchem-448	214	27	]	]	PUNCT
eurjchem-448	214	28	.	.	PUNCT
eurjchem-448	215	1	3.2.7	3.2.7	NUM
eurjchem-448	215	2	.	.	PUNCT
eurjchem-448	215	3	electron	electron	NOUN
eurjchem-448	215	4	impact	impact	PROPN
eurjchem-448	215	5	mass	mass	PROPN
eurjchem-448	215	6	spectra	spectra	NOUN
eurjchem-448	215	7	of	of	ADP
eurjchem-448	215	8	ces	ces	X
eurjchem-448	215	9	mass	mass	NOUN
eurjchem-448	215	10	spectral	spectral	ADJ
eurjchem-448	215	11	study	study	NOUN
eurjchem-448	215	12	was	be	AUX
eurjchem-448	215	13	applied	apply	VERB
eurjchem-448	215	14	to	to	PART
eurjchem-448	215	15	investigate	investigate	VERB
eurjchem-448	215	16	complete	complete	ADJ
eurjchem-448	215	17	fragmentation	fragmentation	NOUN
eurjchem-448	215	18	patterns	pattern	NOUN
eurjchem-448	215	19	of	of	ADP
eurjchem-448	215	20	ni	ni	PROPN
eurjchem-448	215	21	and	and	CCONJ
eurjchem-448	215	22	co‐ces	co‐ce	NOUN
eurjchem-448	215	23	.	.	PUNCT
eurjchem-448	216	1	in	in	ADP
eurjchem-448	216	2	electron	electron	NOUN
eurjchem-448	216	3	impact	impact	NOUN
eurjchem-448	216	4	mass	mass	PROPN
eurjchem-448	216	5	spectra	spectra	NOUN
eurjchem-448	216	6	,	,	PUNCT
eurjchem-448	216	7	peaks	peak	NOUN
eurjchem-448	216	8	of	of	ADP
eurjchem-448	216	9	different	different	ADJ
eurjchem-448	216	10	intensities	intensity	NOUN
eurjchem-448	216	11	corresponding	correspond	VERB
eurjchem-448	216	12	to	to	ADP
eurjchem-448	216	13	various	various	ADJ
eurjchem-448	216	14	fragments	fragment	NOUN
eurjchem-448	216	15	of	of	ADP
eurjchem-448	216	16	ces	ce	NOUN
eurjchem-448	216	17	of	of	ADP
eurjchem-448	216	18	co(ii	co(ii	ADJ
eurjchem-448	216	19	)	)	PUNCT
eurjchem-448	216	20	and	and	CCONJ
eurjchem-448	216	21	ni(ii	ni(ii	PROPN
eurjchem-448	216	22	)	)	PUNCT
eurjchem-448	216	23	were	be	AUX
eurjchem-448	216	24	obtained	obtain	VERB
eurjchem-448	216	25	along	along	ADP
eurjchem-448	216	26	with	with	ADP
eurjchem-448	216	27	their	their	PRON
eurjchem-448	216	28	stabilities	stability	NOUN
eurjchem-448	216	29	.	.	PUNCT
eurjchem-448	217	1	a	a	DET
eurjchem-448	217	2	base	base	NOUN
eurjchem-448	217	3	peak	peak	NOUN
eurjchem-448	217	4	m+	m+	NUM
eurjchem-448	217	5	,	,	PUNCT
eurjchem-448	217	6	indicated	indicate	VERB
eurjchem-448	217	7	the	the	DET
eurjchem-448	217	8	facile	facile	ADJ
eurjchem-448	217	9	loss	loss	NOUN
eurjchem-448	217	10	of	of	ADP
eurjchem-448	217	11	hydrogen	hydrogen	NOUN
eurjchem-448	217	12	radical	radical	ADJ
eurjchem-448	217	13	at	at	ADP
eurjchem-448	217	14	ms	ms	PROPN
eurjchem-448	217	15	(	(	PUNCT
eurjchem-448	217	16	ei	ei	PROPN
eurjchem-448	217	17	,	,	PUNCT
eurjchem-448	217	18	m	m	PROPN
eurjchem-448	217	19	/	/	SYM
eurjchem-448	217	20	z	z	PROPN
eurjchem-448	217	21	(	(	PUNCT
eurjchem-448	217	22	%	%	NOUN
eurjchem-448	217	23	)	)	PUNCT
eurjchem-448	217	24	):	):	PUNCT
eurjchem-448	217	25	699	699	NUM
eurjchem-448	217	26	(	(	PUNCT
eurjchem-448	217	27	m+	m+	NUM
eurjchem-448	217	28	,	,	PUNCT
eurjchem-448	217	29	65	65	NUM
eurjchem-448	217	30	%	%	NOUN
eurjchem-448	217	31	)	)	PUNCT
eurjchem-448	217	32	and	and	CCONJ
eurjchem-448	217	33	698	698	NUM
eurjchem-448	217	34	(	(	PUNCT
eurjchem-448	217	35	61	61	NUM
eurjchem-448	217	36	%	%	NOUN
eurjchem-448	217	37	)	)	PUNCT
eurjchem-448	217	38	a.m.u	a.m.u	NOUN
eurjchem-448	217	39	.	.	PUNCT
eurjchem-448	218	1	for	for	ADP
eurjchem-448	218	2	ces	ce	NOUN
eurjchem-448	218	3	of	of	ADP
eurjchem-448	218	4	co(ii	co(ii	ADJ
eurjchem-448	218	5	)	)	PUNCT
eurjchem-448	218	6	and	and	CCONJ
eurjchem-448	218	7	ni(ii	ni(ii	NOUN
eurjchem-448	218	8	)	)	PUNCT
eurjchem-448	218	9	,	,	PUNCT
eurjchem-448	218	10	respectively	respectively	ADV
eurjchem-448	218	11	confirmed	confirm	VERB
eurjchem-448	218	12	monomeric	monomeric	ADJ
eurjchem-448	218	13	nature	nature	NOUN
eurjchem-448	218	14	of	of	ADP
eurjchem-448	218	15	ces	ce	NOUN
eurjchem-448	218	16	and	and	CCONJ
eurjchem-448	218	17	proposed	propose	VERB
eurjchem-448	218	18	formula	formula	NOUN
eurjchem-448	218	19	derived	derive	VERB
eurjchem-448	218	20	from	from	ADP
eurjchem-448	218	21	elemental	elemental	ADJ
eurjchem-448	218	22	analysis	analysis	NOUN
eurjchem-448	218	23	.	.	PUNCT
eurjchem-448	219	1	general	general	ADJ
eurjchem-448	219	2	fragmentation	fragmentation	NOUN
eurjchem-448	219	3	pattern	pattern	NOUN
eurjchem-448	219	4	revealed	reveal	VERB
eurjchem-448	219	5	primary	primary	ADJ
eurjchem-448	219	6	cleavages	cleavage	NOUN
eurjchem-448	219	7	to	to	PART
eurjchem-448	219	8	occur	occur	VERB
eurjchem-448	219	9	at	at	ADP
eurjchem-448	219	10	hetero‐carbon	hetero‐carbon	NOUN
eurjchem-448	219	11	bonds	bond	NOUN
eurjchem-448	219	12	.	.	PUNCT
eurjchem-448	220	1	several	several	ADJ
eurjchem-448	220	2	other	other	ADJ
eurjchem-448	220	3	peaks	peak	NOUN
eurjchem-448	220	4	were	be	AUX
eurjchem-448	220	5	observed	observe	VERB
eurjchem-448	220	6	having	have	VERB
eurjchem-448	220	7	various	various	ADJ
eurjchem-448	220	8	m	m	PROPN
eurjchem-448	220	9	/	/	SYM
eurjchem-448	220	10	z	z	NOUN
eurjchem-448	220	11	values	value	NOUN
eurjchem-448	220	12	at	at	ADP
eurjchem-448	220	13	different	different	ADJ
eurjchem-448	220	14	intensities	intensity	NOUN
eurjchem-448	220	15	corresponding	correspond	VERB
eurjchem-448	220	16	to	to	ADP
eurjchem-448	220	17	molecular	molecular	ADJ
eurjchem-448	220	18	masses	masse	NOUN
eurjchem-448	220	19	of	of	ADP
eurjchem-448	220	20	different	different	ADJ
eurjchem-448	220	21	constituents	constituent	NOUN
eurjchem-448	220	22	.	.	PUNCT
eurjchem-448	221	1	their	their	PRON
eurjchem-448	221	2	intensities	intensity	NOUN
eurjchem-448	221	3	gave	give	VERB
eurjchem-448	221	4	an	an	DET
eurjchem-448	221	5	idea	idea	NOUN
eurjchem-448	221	6	about	about	ADP
eurjchem-448	221	7	their	their	PRON
eurjchem-448	221	8	stabilities	stability	NOUN
eurjchem-448	221	9	along	along	ADP
eurjchem-448	221	10	with	with	ADP
eurjchem-448	221	11	geometrical	geometrical	ADJ
eurjchem-448	221	12	configurations	configuration	NOUN
eurjchem-448	221	13	[	[	X
eurjchem-448	221	14	25	25	NUM
eurjchem-448	221	15	]	]	PUNCT
eurjchem-448	221	16	.	.	PUNCT
eurjchem-448	222	1	the	the	DET
eurjchem-448	222	2	major	major	ADJ
eurjchem-448	222	3	cleavage	cleavage	NOUN
eurjchem-448	222	4	pathways	pathway	NOUN
eurjchem-448	222	5	took	take	VERB
eurjchem-448	222	6	place	place	NOUN
eurjchem-448	222	7	through	through	ADP
eurjchem-448	222	8	the	the	DET
eurjchem-448	222	9	loss	loss	NOUN
eurjchem-448	222	10	of	of	ADP
eurjchem-448	222	11	‐s‐ch2‐	‐s‐ch2‐	ADJ
eurjchem-448	222	12	ch2‐	ch2‐	NOUN
eurjchem-448	222	13	fragment	fragment	NOUN
eurjchem-448	222	14	,	,	PUNCT
eurjchem-448	222	15	followed	follow	VERB
eurjchem-448	222	16	by	by	ADP
eurjchem-448	222	17	the	the	DET
eurjchem-448	222	18	elimination	elimination	NOUN
eurjchem-448	222	19	of	of	ADP
eurjchem-448	222	20	‐ch2‐.	‐ch2‐.	NUM
eurjchem-448	222	21	in	in	ADP
eurjchem-448	222	22	conclusion	conclusion	NOUN
eurjchem-448	222	23	,	,	PUNCT
eurjchem-448	222	24	presented	present	VERB
eurjchem-448	222	25	generic	generic	ADJ
eurjchem-448	222	26	models	model	NOUN
eurjchem-448	222	27	had	have	VERB
eurjchem-448	222	28	1:1	1:1	NUM
eurjchem-448	222	29	stoichiometry	stoichiometry	NOUN
eurjchem-448	222	30	.	.	PUNCT
eurjchem-448	223	1	3.2.8	3.2.8	X
eurjchem-448	223	2	.	.	PUNCT
eurjchem-448	223	3	molecular	molecular	ADJ
eurjchem-448	223	4	modeling	modeling	NOUN
eurjchem-448	223	5	of	of	ADP
eurjchem-448	223	6	mc	mc	PROPN
eurjchem-448	223	7	and	and	CCONJ
eurjchem-448	223	8	ces	ces	X
eurjchem-448	223	9	molecular	molecular	ADJ
eurjchem-448	223	10	modeling	modeling	NOUN
eurjchem-448	223	11	is	be	AUX
eurjchem-448	223	12	a	a	DET
eurjchem-448	223	13	mathematical	mathematical	ADJ
eurjchem-448	223	14	concept	concept	NOUN
eurjchem-448	223	15	to	to	PART
eurjchem-448	223	16	impersonate	impersonate	VERB
eurjchem-448	223	17	correlated	correlate	VERB
eurjchem-448	223	18	significant	significant	ADJ
eurjchem-448	223	19	features	feature	NOUN
eurjchem-448	223	20	i.e.	i.e.	X
eurjchem-448	223	21	molecular	molecular	ADJ
eurjchem-448	223	22	geometries	geometry	NOUN
eurjchem-448	223	23	,	,	PUNCT
eurjchem-448	223	24	bond	bond	NOUN
eurjchem-448	223	25	energies	energy	NOUN
eurjchem-448	223	26	,	,	PUNCT
eurjchem-448	223	27	torsion	torsion	NOUN
eurjchem-448	223	28	angles	angle	NOUN
eurjchem-448	223	29	and	and	CCONJ
eurjchem-448	223	30	cartesian	cartesian	ADJ
eurjchem-448	223	31	coordinates	coordinate	NOUN
eurjchem-448	223	32	of	of	ADP
eurjchem-448	223	33	concerned	concerned	ADJ
eurjchem-448	223	34	molecular	molecular	ADJ
eurjchem-448	223	35	topologies	topology	NOUN
eurjchem-448	223	36	.	.	PUNCT
eurjchem-448	224	1	bond	bond	NOUN
eurjchem-448	224	2	lengths	length	NOUN
eurjchem-448	224	3	,	,	PUNCT
eurjchem-448	224	4	bond	bond	NOUN
eurjchem-448	224	5	angles	angle	NOUN
eurjchem-448	224	6	and	and	CCONJ
eurjchem-448	224	7	atomic	atomic	ADJ
eurjchem-448	224	8	coordinates	coordinate	NOUN
eurjchem-448	224	9	depend	depend	VERB
eurjchem-448	224	10	on	on	ADP
eurjchem-448	224	11	the	the	DET
eurjchem-448	224	12	hybridization	hybridization	NOUN
eurjchem-448	224	13	of	of	ADP
eurjchem-448	224	14	an	an	DET
eurjchem-448	224	15	atom	atom	NOUN
eurjchem-448	224	16	and	and	CCONJ
eurjchem-448	224	17	mode	mode	NOUN
eurjchem-448	224	18	of	of	ADP
eurjchem-448	224	19	bonding	bonding	NOUN
eurjchem-448	224	20	.	.	PUNCT
eurjchem-448	225	1	thus	thus	ADV
eurjchem-448	225	2	,	,	PUNCT
eurjchem-448	225	3	molecular	molecular	ADJ
eurjchem-448	225	4	modeling	modeling	NOUN
eurjchem-448	225	5	had	have	AUX
eurjchem-448	225	6	been	be	AUX
eurjchem-448	225	7	successfully	successfully	ADV
eurjchem-448	225	8	used	use	VERB
eurjchem-448	225	9	to	to	PART
eurjchem-448	225	10	demonstrate	demonstrate	VERB
eurjchem-448	225	11	three	three	NUM
eurjchem-448	225	12	dimensional	dimensional	ADJ
eurjchem-448	225	13	arrangements	arrangement	NOUN
eurjchem-448	225	14	of	of	ADP
eurjchem-448	225	15	the	the	DET
eurjchem-448	225	16	atoms	atom	NOUN
eurjchem-448	225	17	.	.	PUNCT
eurjchem-448	226	1	molecular	molecular	ADJ
eurjchem-448	226	2	models	model	NOUN
eurjchem-448	226	3	were	be	AUX
eurjchem-448	226	4	proposed	propose	VERB
eurjchem-448	226	5	as	as	ADP
eurjchem-448	226	6	a	a	DET
eurjchem-448	226	7	standard	standard	NOUN
eurjchem-448	226	8	to	to	PART
eurjchem-448	226	9	judge	judge	VERB
eurjchem-448	226	10	specific	specific	ADJ
eurjchem-448	226	11	interactions	interaction	NOUN
eurjchem-448	226	12	in	in	ADP
eurjchem-448	226	13	topologies	topology	NOUN
eurjchem-448	226	14	of	of	ADP
eurjchem-448	226	15	the	the	DET
eurjchem-448	226	16	molecules	molecule	NOUN
eurjchem-448	226	17	of	of	ADP
eurjchem-448	226	18	mc	mc	PROPN
eurjchem-448	226	19	and	and	CCONJ
eurjchem-448	226	20	derived	derive	VERB
eurjchem-448	226	21	ces	ce	NOUN
eurjchem-448	226	22	.	.	PUNCT
eurjchem-448	226	23	beside	beside	ADP
eurjchem-448	226	24	this	this	PRON
eurjchem-448	226	25	,	,	PUNCT
eurjchem-448	226	26	if	if	SCONJ
eurjchem-448	226	27	deviations	deviation	NOUN
eurjchem-448	226	28	in	in	ADP
eurjchem-448	226	29	distances	distance	NOUN
eurjchem-448	226	30	,	,	PUNCT
eurjchem-448	226	31	angles	angle	NOUN
eurjchem-448	226	32	or	or	CCONJ
eurjchem-448	226	33	torsion	torsion	NOUN
eurjchem-448	226	34	were	be	AUX
eurjchem-448	226	35	evidenced	evidence	VERB
eurjchem-448	226	36	,	,	PUNCT
eurjchem-448	226	37	specific	specific	ADJ
eurjchem-448	226	38	electronic	electronic	ADJ
eurjchem-448	226	39	interactions	interaction	NOUN
eurjchem-448	226	40	should	should	AUX
eurjchem-448	226	41	perhaps	perhaps	ADV
eurjchem-448	226	42	be	be	AUX
eurjchem-448	226	43	pursued	pursue	VERB
eurjchem-448	226	44	.	.	PUNCT
eurjchem-448	227	1	in	in	ADP
eurjchem-448	227	2	order	order	NOUN
eurjchem-448	227	3	to	to	PART
eurjchem-448	227	4	ascertain	ascertain	VERB
eurjchem-448	227	5	the	the	DET
eurjchem-448	227	6	structural	structural	ADJ
eurjchem-448	227	7	features	feature	NOUN
eurjchem-448	227	8	and	and	CCONJ
eurjchem-448	227	9	related	relate	VERB
eurjchem-448	227	10	preferences	preference	NOUN
eurjchem-448	227	11	to	to	PART
eurjchem-448	227	12	confirm	confirm	VERB
eurjchem-448	227	13	the	the	DET
eurjchem-448	227	14	obtained	obtain	VERB
eurjchem-448	227	15	spectral	spectral	ADJ
eurjchem-448	227	16	evidences	evidence	NOUN
eurjchem-448	227	17	.	.	PUNCT
eurjchem-448	228	1	the	the	DET
eurjchem-448	228	2	coordination	coordination	NOUN
eurjchem-448	228	3	capabilities	capability	NOUN
eurjchem-448	228	4	of	of	ADP
eurjchem-448	228	5	mc	mc	PROPN
eurjchem-448	228	6	towards	towards	ADP
eurjchem-448	228	7	metal	metal	PROPN
eurjchem-448	228	8	ion(s	ion(s	PROPN
eurjchem-448	228	9	)	)	PUNCT
eurjchem-448	228	10	along	along	ADP
eurjchem-448	228	11	with	with	ADP
eurjchem-448	228	12	its	its	PRON
eurjchem-448	228	13	impact	impact	NOUN
eurjchem-448	228	14	on	on	ADP
eurjchem-448	228	15	bond	bond	NOUN
eurjchem-448	228	16	lengths	length	NOUN
eurjchem-448	228	17	and	and	CCONJ
eurjchem-448	228	18	bond	bond	NOUN
eurjchem-448	228	19	angles	angle	NOUN
eurjchem-448	228	20	,	,	PUNCT
eurjchem-448	228	21	thereby	thereby	ADV
eurjchem-448	228	22	,	,	PUNCT
eurjchem-448	228	23	were	be	AUX
eurjchem-448	228	24	demonstrated	demonstrate	VERB
eurjchem-448	228	25	and	and	CCONJ
eurjchem-448	228	26	presented	present	VERB
eurjchem-448	228	27	through	through	ADP
eurjchem-448	228	28	the	the	DET
eurjchem-448	228	29	molecular	molecular	ADJ
eurjchem-448	228	30	models	model	NOUN
eurjchem-448	228	31	of	of	ADP
eurjchem-448	228	32	mc	mc	PROPN
eurjchem-448	228	33	and	and	CCONJ
eurjchem-448	228	34	ces	ces	PROPN
eurjchem-448	228	35	.	.	PROPN
eurjchem-448	228	36	physical	physical	ADJ
eurjchem-448	228	37	dimensions	dimension	NOUN
eurjchem-448	228	38	of	of	ADP
eurjchem-448	228	39	the	the	DET
eurjchem-448	228	40	molecules	molecule	NOUN
eurjchem-448	228	41	helped	help	VERB
eurjchem-448	228	42	out	out	ADP
eurjchem-448	228	43	to	to	PART
eurjchem-448	228	44	demonstrate	demonstrate	VERB
eurjchem-448	228	45	the	the	DET
eurjchem-448	228	46	changes	change	NOUN
eurjchem-448	228	47	occurred	occur	VERB
eurjchem-448	228	48	during	during	ADP
eurjchem-448	228	49	their	their	PRON
eurjchem-448	228	50	topological	topological	ADJ
eurjchem-448	228	51	assemblies	assembly	NOUN
eurjchem-448	228	52	.	.	PUNCT
eurjchem-448	229	1	the	the	DET
eurjchem-448	229	2	process	process	NOUN
eurjchem-448	229	3	of	of	ADP
eurjchem-448	229	4	determining	determine	VERB
eurjchem-448	229	5	energy	energy	NOUN
eurjchem-448	229	6	minimization	minimization	NOUN
eurjchem-448	229	7	was	be	AUX
eurjchem-448	229	8	repeated	repeat	VERB
eurjchem-448	229	9	several	several	ADJ
eurjchem-448	229	10	times	time	NOUN
eurjchem-448	229	11	to	to	PART
eurjchem-448	229	12	find	find	VERB
eurjchem-448	229	13	global	global	ADJ
eurjchem-448	229	14	minimum	minimum	ADJ
eurjchem-448	229	15	energy	energy	NOUN
eurjchem-448	230	1	[	[	X
eurjchem-448	230	2	26	26	NUM
eurjchem-448	230	3	]	]	PUNCT
eurjchem-448	230	4	.	.	PUNCT
eurjchem-448	231	1	data	datum	NOUN
eurjchem-448	231	2	analysis	analysis	NOUN
eurjchem-448	231	3	of	of	ADP
eurjchem-448	231	4	bond	bond	NOUN
eurjchem-448	231	5	lengths	length	NOUN
eurjchem-448	231	6	and	and	CCONJ
eurjchem-448	231	7	angles	angle	NOUN
eurjchem-448	231	8	were	be	AUX
eurjchem-448	231	9	presented	present	VERB
eurjchem-448	231	10	in	in	ADP
eurjchem-448	231	11	table	table	NOUN
eurjchem-448	231	12	3	3	NUM
eurjchem-448	231	13	to	to	ADP
eurjchem-448	231	14	6	6	NUM
eurjchem-448	231	15	.	.	PUNCT
eurjchem-448	232	1	on	on	ADP
eurjchem-448	232	2	the	the	DET
eurjchem-448	232	3	basis	basis	NOUN
eurjchem-448	232	4	reported	report	VERB
eurjchem-448	232	5	data	datum	NOUN
eurjchem-448	232	6	,	,	PUNCT
eurjchem-448	232	7	following	follow	VERB
eurjchem-448	232	8	remarks	remark	NOUN
eurjchem-448	232	9	were	be	AUX
eurjchem-448	232	10	concluded	conclude	VERB
eurjchem-448	232	11	as	as	SCONJ
eurjchem-448	232	12	follows	follow	VERB
eurjchem-448	232	13	:	:	PUNCT
eurjchem-448	232	14	bond	bond	NOUN
eurjchem-448	232	15	angles	angle	NOUN
eurjchem-448	232	16	between	between	ADP
eurjchem-448	232	17	metal	metal	NOUN
eurjchem-448	232	18	and	and	CCONJ
eurjchem-448	232	19	donor	donor	NOUN
eurjchem-448	232	20	atoms	atom	NOUN
eurjchem-448	232	21	in	in	ADP
eurjchem-448	232	22	mc	mc	PROPN
eurjchem-448	232	23	moiety	moiety	PROPN
eurjchem-448	232	24	were	be	AUX
eurjchem-448	232	25	altered	alter	VERB
eurjchem-448	232	26	somewhat	somewhat	ADV
eurjchem-448	232	27	upon	upon	SCONJ
eurjchem-448	232	28	coordination	coordination	NOUN
eurjchem-448	232	29	;	;	PUNCT
eurjchem-448	232	30	bonds	bond	NOUN
eurjchem-448	232	31	angles	angle	VERB
eurjchem-448	232	32	s(28)‐co(39)‐s(10	s(28)‐co(39)‐s(10	PROPN
eurjchem-448	232	33	)	)	PUNCT
eurjchem-448	232	34	and	and	CCONJ
eurjchem-448	232	35	s(27)‐co(39)‐s(09	s(27)‐co(39)‐s(09	NOUN
eurjchem-448	232	36	)	)	PUNCT
eurjchem-448	232	37	were	be	AUX
eurjchem-448	232	38	179.4	179.4	NUM
eurjchem-448	232	39	°	°	NOUN
eurjchem-448	232	40	and	and	CCONJ
eurjchem-448	232	41	180.0	180.0	NUM
eurjchem-448	232	42	°	°	NOUN
eurjchem-448	232	43	,	,	PUNCT
eurjchem-448	232	44	respectively	respectively	ADV
eurjchem-448	232	45	as	as	ADP
eurjchem-448	232	46	a	a	DET
eurjchem-448	232	47	consequence	consequence	NOUN
eurjchem-448	232	48	of	of	ADP
eurjchem-448	232	49	bonding	bonding	NOUN
eurjchem-448	232	50	.	.	PUNCT
eurjchem-448	233	1	bond	bond	NOUN
eurjchem-448	233	2	angles	angle	NOUN
eurjchem-448	233	3	in	in	ADP
eurjchem-448	233	4	ces	ce	NOUN
eurjchem-448	233	5	were	be	AUX
eurjchem-448	233	6	quite	quite	ADV
eurjchem-448	233	7	near	near	ADJ
eurjchem-448	233	8	to	to	ADP
eurjchem-448	233	9	an	an	DET
eurjchem-448	233	10	octahedral	octahedral	ADJ
eurjchem-448	233	11	geometry	geometry	NOUN
eurjchem-448	233	12	.	.	PUNCT
eurjchem-448	234	1	it	it	PRON
eurjchem-448	234	2	is	be	AUX
eurjchem-448	234	3	clear	clear	ADJ
eurjchem-448	234	4	that	that	SCONJ
eurjchem-448	234	5	all	all	DET
eurjchem-448	234	6	the	the	DET
eurjchem-448	234	7	active	active	ADJ
eurjchem-448	234	8	groups	group	NOUN
eurjchem-448	234	9	taking	take	VERB
eurjchem-448	234	10	part	part	NOUN
eurjchem-448	234	11	in	in	ADP
eurjchem-448	234	12	coordination	coordination	NOUN
eurjchem-448	234	13	and	and	CCONJ
eurjchem-448	234	14	had	have	VERB
eurjchem-448	234	15	longer	long	ADJ
eurjchem-448	234	16	bonds	bond	NOUN
eurjchem-448	234	17	than	than	ADP
eurjchem-448	234	18	already	already	ADV
eurjchem-448	234	19	existing	exist	VERB
eurjchem-448	234	20	in	in	ADP
eurjchem-448	234	21	ligand	ligand	NOUN
eurjchem-448	234	22	in	in	ADP
eurjchem-448	234	23	‐c‐s‐c‐	‐c‐s‐c‐	PROPN
eurjchem-448	234	24	and	and	CCONJ
eurjchem-448	234	25	>	>	X
eurjchem-448	234	26	c	c	X
eurjchem-448	234	27	=	=	NOUN
eurjchem-448	234	28	n‐	n‐	NOUN
eurjchem-448	234	29	linkages	linkage	NOUN
eurjchem-448	234	30	.	.	PUNCT
eurjchem-448	235	1	coordination	coordination	NOUN
eurjchem-448	235	2	significantly	significantly	ADV
eurjchem-448	235	3	shortens	shorten	VERB
eurjchem-448	235	4	as	as	ADP
eurjchem-448	235	5	1.8	1.8	NUM
eurjchem-448	235	6	å	å	PROPN
eurjchem-448	235	7	for	for	ADP
eurjchem-448	235	8	n(38)‐ni(39	n(38)‐ni(39	PROPN
eurjchem-448	235	9	)	)	PUNCT
eurjchem-448	235	10	as	as	SCONJ
eurjchem-448	235	11	compared	compare	VERB
eurjchem-448	235	12	to	to	ADP
eurjchem-448	235	13	2.1	2.1	NUM
eurjchem-448	235	14	å	å	NOUN
eurjchem-448	235	15	for	for	ADP
eurjchem-448	235	16	s(27)‐co(39	s(27)‐co(39	PROPN
eurjchem-448	235	17	)	)	PUNCT
eurjchem-448	235	18	.	.	PUNCT
eurjchem-448	236	1	this	this	PRON
eurjchem-448	236	2	is	be	AUX
eurjchem-448	236	3	because	because	SCONJ
eurjchem-448	236	4	of	of	ADP
eurjchem-448	236	5	bond	bond	NOUN
eurjchem-448	236	6	lengths	length	NOUN
eurjchem-448	236	7	in	in	ADP
eurjchem-448	236	8	mc	mc	PROPN
eurjchem-448	236	9	between	between	ADP
eurjchem-448	236	10	donor	donor	NOUN
eurjchem-448	236	11	atoms	atom	NOUN
eurjchem-448	236	12	probably	probably	ADV
eurjchem-448	236	13	gets	get	AUX
eurjchem-448	236	14	affected	affect	VERB
eurjchem-448	236	15	due	due	ADP
eurjchem-448	236	16	to	to	ADP
eurjchem-448	236	17	the	the	DET
eurjchem-448	236	18	presence	presence	NOUN
eurjchem-448	236	19	of	of	ADP
eurjchem-448	236	20	hydrogen	hydrogen	NOUN
eurjchem-448	236	21	in	in	ADP
eurjchem-448	236	22	azomethine	azomethine	NOUN
eurjchem-448	236	23	(	(	PUNCT
eurjchem-448	236	24	‐	‐	ADP
eurjchem-448	236	25	ch	ch	NOUN
eurjchem-448	236	26	=	=	NOUN
eurjchem-448	236	27	n‐	n‐	NOUN
eurjchem-448	236	28	)	)	PUNCT
eurjchem-448	236	29	.	.	PUNCT
eurjchem-448	237	1	there	there	PRON
eurjchem-448	237	2	is	be	VERB
eurjchem-448	237	3	a	a	DET
eurjchem-448	237	4	large	large	ADJ
eurjchem-448	237	5	variation	variation	NOUN
eurjchem-448	237	6	in	in	ADP
eurjchem-448	237	7	n(37)‐n(38	n(37)‐n(38	NOUN
eurjchem-448	237	8	)	)	PUNCT
eurjchem-448	237	9	bond	bond	NOUN
eurjchem-448	237	10	lengths	length	NOUN
eurjchem-448	237	11	on	on	ADP
eurjchem-448	237	12	complexation	complexation	NOUN
eurjchem-448	237	13	and	and	CCONJ
eurjchem-448	237	14	becomes	become	VERB
eurjchem-448	237	15	slightly	slightly	ADV
eurjchem-448	237	16	longer	long	ADJ
eurjchem-448	237	17	as	as	SCONJ
eurjchem-448	237	18	the	the	DET
eurjchem-448	237	19	coordination	coordination	NOUN
eurjchem-448	237	20	took	take	VERB
eurjchem-448	237	21	place	place	NOUN
eurjchem-448	237	22	via	via	ADP
eurjchem-448	237	23	n	n	PRON
eurjchem-448	237	24	atom	atom	NOUN
eurjchem-448	237	25	of	of	ADP
eurjchem-448	237	26	‐ch	‐ch	NOUN
eurjchem-448	237	27	=	=	NOUN
eurjchem-448	237	28	n‐.	n‐.	VERB
eurjchem-448	237	29	based	base	VERB
eurjchem-448	237	30	on	on	ADP
eurjchem-448	237	31	spectral	spectral	ADJ
eurjchem-448	237	32	and	and	CCONJ
eurjchem-448	237	33	analytical	analytical	ADJ
eurjchem-448	237	34	analysis	analysis	NOUN
eurjchem-448	237	35	(	(	PUNCT
eurjchem-448	237	36	elemental	elemental	ADJ
eurjchem-448	237	37	analysis	analysis	NOUN
eurjchem-448	237	38	,	,	PUNCT
eurjchem-448	237	39	conductance	conductance	NOUN
eurjchem-448	237	40	measurements	measurement	NOUN
eurjchem-448	237	41	,	,	PUNCT
eurjchem-448	237	42	magnetic	magnetic	ADJ
eurjchem-448	237	43	susceptibilities	susceptibility	NOUN
eurjchem-448	237	44	,	,	PUNCT
eurjchem-448	237	45	infrared	infrare	VERB
eurjchem-448	237	46	,	,	PUNCT
eurjchem-448	237	47	1h	1h	NUM
eurjchem-448	237	48	and	and	CCONJ
eurjchem-448	237	49	13c	13c	NOUN
eurjchem-448	237	50	nmr	nmr	NOUN
eurjchem-448	237	51	,	,	PUNCT
eurjchem-448	237	52	electronic	electronic	ADJ
eurjchem-448	237	53	,	,	PUNCT
eurjchem-448	237	54	mass	mass	PROPN
eurjchem-448	237	55	,	,	PUNCT
eurjchem-448	237	56	epr	epr	ADJ
eurjchem-448	237	57	,	,	PUNCT
eurjchem-448	237	58	cyclic	cyclic	ADJ
eurjchem-448	237	59	voltammetry	voltammetry	NOUN
eurjchem-448	237	60	and	and	CCONJ
eurjchem-448	237	61	molecular	molecular	ADJ
eurjchem-448	237	62	modeling	modeling	NOUN
eurjchem-448	237	63	)	)	PUNCT
eurjchem-448	237	64	solvent	solvent	ADJ
eurjchem-448	237	65	accessible	accessible	ADJ
eurjchem-448	237	66	surface	surface	NOUN
eurjchem-448	237	67	model	model	NOUN
eurjchem-448	237	68	of	of	ADP
eurjchem-448	237	69	mc	mc	PROPN
eurjchem-448	237	70	and	and	CCONJ
eurjchem-448	237	71	molecular	molecular	ADJ
eurjchem-448	237	72	models	model	NOUN
eurjchem-448	237	73	of	of	ADP
eurjchem-448	237	74	ces	ce	NOUN
eurjchem-448	237	75	of	of	ADP
eurjchem-448	237	76	ni(ii	ni(ii	NOUN
eurjchem-448	237	77	)	)	PUNCT
eurjchem-448	237	78	were	be	AUX
eurjchem-448	237	79	designed	design	VERB
eurjchem-448	237	80	and	and	CCONJ
eurjchem-448	237	81	presented	present	VERB
eurjchem-448	237	82	as	as	ADP
eurjchem-448	237	83	figure	figure	NOUN
eurjchem-448	237	84	5	5	NUM
eurjchem-448	237	85	and	and	CCONJ
eurjchem-448	237	86	6	6	NUM
eurjchem-448	237	87	.	.	NOUN
eurjchem-448	237	88	table	table	NOUN
eurjchem-448	237	89	3	3	NUM
eurjchem-448	237	90	.	.	NUM
eurjchem-448	237	91	selected	select	VERB
eurjchem-448	237	92	bond	bond	NOUN
eurjchem-448	237	93	lengths	length	NOUN
eurjchem-448	237	94	of	of	ADP
eurjchem-448	237	95	ces	ce	NOUN
eurjchem-448	237	96	of	of	ADP
eurjchem-448	237	97	co(ii	co(ii	PROPN
eurjchem-448	237	98	)	)	PUNCT
eurjchem-448	237	99	.	.	PUNCT
eurjchem-448	238	1	selected	select	VERB
eurjchem-448	238	2	bond	bond	NOUN
eurjchem-448	238	3	bond	bond	NOUN
eurjchem-448	238	4	length	length	NOUN
eurjchem-448	238	5	,	,	PUNCT
eurjchem-448	238	6	å	å	PROPN
eurjchem-448	238	7	s(27)‐co(39	s(27)‐co(39	PROPN
eurjchem-448	238	8	)	)	PUNCT
eurjchem-448	238	9	2.18	2.18	NUM
eurjchem-448	238	10	s(28)‐co(39	s(28)‐co(39	ADJ
eurjchem-448	238	11	)	)	PUNCT
eurjchem-448	238	12	2.18	2.18	NUM
eurjchem-448	238	13	n(37)‐co(39	n(37)‐co(39	PROPN
eurjchem-448	238	14	)	)	PUNCT
eurjchem-448	238	15	1.83	1.83	NUM
eurjchem-448	238	16	n(38)‐co(39	n(38)‐co(39	NOUN
eurjchem-448	238	17	)	)	PUNCT
eurjchem-448	238	18	1.83	1.83	NUM
eurjchem-448	238	19	s(09)‐co(39	s(09)‐co(39	NOUN
eurjchem-448	238	20	)	)	PUNCT
eurjchem-448	238	21	2.18	2.18	NUM
eurjchem-448	238	22	s(10)‐co(39	s(10)‐co(39	PROPN
eurjchem-448	238	23	)	)	PUNCT
eurjchem-448	238	24	2.18	2.18	NUM
eurjchem-448	238	25	table	table	NOUN
eurjchem-448	238	26	4	4	NUM
eurjchem-448	238	27	selected	select	VERB
eurjchem-448	238	28	bond	bond	NOUN
eurjchem-448	238	29	lengths	length	NOUN
eurjchem-448	238	30	[	[	X
eurjchem-448	238	31	å	å	X
eurjchem-448	238	32	]	]	X
eurjchem-448	238	33	of	of	ADP
eurjchem-448	238	34	ces	ce	NOUN
eurjchem-448	238	35	of	of	ADP
eurjchem-448	238	36	ni(ii	ni(ii	NOUN
eurjchem-448	238	37	)	)	PUNCT
eurjchem-448	238	38	.	.	PUNCT
eurjchem-448	239	1	selected	select	VERB
eurjchem-448	239	2	bond	bond	NOUN
eurjchem-448	239	3	bond	bond	NOUN
eurjchem-448	239	4	length	length	NOUN
eurjchem-448	239	5	,	,	PUNCT
eurjchem-448	239	6	å	å	PROPN
eurjchem-448	239	7	s(27)‐ni(39	s(27)‐ni(39	PROPN
eurjchem-448	239	8	)	)	PUNCT
eurjchem-448	239	9	2.17	2.17	NUM
eurjchem-448	239	10	s(28)‐ni(39	s(28)‐ni(39	X
eurjchem-448	239	11	)	)	PUNCT
eurjchem-448	239	12	2.17	2.17	NUM
eurjchem-448	239	13	n(37)‐ni(39	n(37)‐ni(39	PROPN
eurjchem-448	239	14	)	)	PUNCT
eurjchem-448	239	15	1.82	1.82	NUM
eurjchem-448	239	16	n(38)‐ni(39	n(38)‐ni(39	PROPN
eurjchem-448	239	17	)	)	PUNCT
eurjchem-448	239	18	1.82	1.82	NUM
eurjchem-448	239	19	s(09)‐ni(39	s(09)‐ni(39	PROPN
eurjchem-448	239	20	)	)	PUNCT
eurjchem-448	239	21	2.17	2.17	NUM
eurjchem-448	239	22	s(10)‐ni(39	s(10)‐ni(39	X
eurjchem-448	239	23	)	)	PUNCT
eurjchem-448	239	24	2.17	2.17	NUM
eurjchem-448	239	25	table	table	NOUN
eurjchem-448	239	26	5	5	NUM
eurjchem-448	239	27	.	.	PUNCT
eurjchem-448	239	28	selected	select	VERB
eurjchem-448	239	29	bond	bond	NOUN
eurjchem-448	239	30	angles	angle	NOUN
eurjchem-448	239	31	of	of	ADP
eurjchem-448	239	32	ces	ce	NOUN
eurjchem-448	239	33	of	of	ADP
eurjchem-448	239	34	co(ii	co(ii	ADJ
eurjchem-448	239	35	)	)	PUNCT
eurjchem-448	239	36	selected	select	VERB
eurjchem-448	239	37	bond	bond	NOUN
eurjchem-448	239	38	bond	bond	NOUN
eurjchem-448	239	39	angles	angle	NOUN
eurjchem-448	239	40	,	,	PUNCT
eurjchem-448	239	41	o	o	PROPN
eurjchem-448	239	42	s(28)‐co(39)‐s(10	s(28)‐co(39)‐s(10	PROPN
eurjchem-448	239	43	)	)	PUNCT
eurjchem-448	239	44	179.4	179.4	NUM
eurjchem-448	239	45	s(27)‐co(39)‐s(09	s(27)‐co(39)‐s(09	NOUN
eurjchem-448	239	46	)	)	PUNCT
eurjchem-448	239	47	180.0	180.0	NUM
eurjchem-448	239	48	co(39)‐n(38)‐c(29	co(39)‐n(38)‐c(29	NOUN
eurjchem-448	239	49	)	)	PUNCT
eurjchem-448	239	50	122.1	122.1	NUM
eurjchem-448	239	51	co(39)‐n(37)‐c(25	co(39)‐n(37)‐c(25	NOUN
eurjchem-448	239	52	)	)	PUNCT
eurjchem-448	239	53	111.0	111.0	NUM
eurjchem-448	239	54	co(39)‐n(37)‐c(20	co(39)‐n(37)‐c(20	NOUN
eurjchem-448	239	55	)	)	PUNCT
eurjchem-448	239	56	117.3	117.3	NUM
eurjchem-448	239	57	co(39)‐s(28)‐c(36	co(39)‐s(28)‐c(36	NOUN
eurjchem-448	239	58	)	)	PUNCT
eurjchem-448	239	59	109.5	109.5	NUM
eurjchem-448	239	60	co(39)‐s(28)‐c(30	co(39)‐s(28)‐c(30	NOUN
eurjchem-448	239	61	)	)	PUNCT
eurjchem-448	239	62	104.0	104.0	NUM
eurjchem-448	239	63	co(39)‐s(27)‐c(35	co(39)‐s(27)‐c(35	NOUN
eurjchem-448	239	64	)	)	PUNCT
eurjchem-448	239	65	109.5	109.5	NUM
eurjchem-448	239	66	co(39)‐s(27)‐c(24	co(39)‐s(27)‐c(24	PROPN
eurjchem-448	239	67	)	)	PUNCT
eurjchem-448	239	68	104.0	104.0	NUM
eurjchem-448	239	69	co(39)‐s(09)‐c(06	co(39)‐s(09)‐c(06	NOUN
eurjchem-448	239	70	)	)	PUNCT
eurjchem-448	239	71	109.5	109.5	NUM
eurjchem-448	239	72	table	table	NOUN
eurjchem-448	239	73	6	6	NUM
eurjchem-448	239	74	.	.	PUNCT
eurjchem-448	239	75	selected	select	VERB
eurjchem-448	239	76	bond	bond	NOUN
eurjchem-448	239	77	angles	angle	NOUN
eurjchem-448	239	78	of	of	ADP
eurjchem-448	239	79	ces	ce	NOUN
eurjchem-448	239	80	of	of	ADP
eurjchem-448	239	81	ni(ii	ni(ii	NOUN
eurjchem-448	239	82	)	)	PUNCT
eurjchem-448	239	83	.	.	PUNCT
eurjchem-448	240	1	selected	select	VERB
eurjchem-448	240	2	bond	bond	NOUN
eurjchem-448	240	3	bond	bond	NOUN
eurjchem-448	240	4	angles	angle	NOUN
eurjchem-448	240	5	,	,	PUNCT
eurjchem-448	240	6	o	o	NOUN
eurjchem-448	240	7	n(38)‐ni(39)‐s(27	n(38)‐ni(39)‐s(27	X
eurjchem-448	240	8	)	)	PUNCT
eurjchem-448	240	9	170.0	170.0	NUM
eurjchem-448	240	10	n(37)‐ni(39)‐s(27	n(37)‐ni(39)‐s(27	NOUN
eurjchem-448	240	11	)	)	PUNCT
eurjchem-448	240	12	170.0	170.0	NUM
eurjchem-448	240	13	s(28)‐ni(39)‐s(27	s(28)‐ni(39)‐s(27	ADJ
eurjchem-448	240	14	)	)	PUNCT
eurjchem-448	240	15	165.8	165.8	NUM
eurjchem-448	240	16	ni(39)‐n(38)‐c(29	ni(39)‐n(38)‐c(29	NOUN
eurjchem-448	240	17	)	)	PUNCT
eurjchem-448	240	18	111.0	111.0	NUM
eurjchem-448	240	19	ni(39)‐n(38)‐c(19	ni(39)‐n(38)‐c(19	NOUN
eurjchem-448	240	20	)	)	PUNCT
eurjchem-448	240	21	119.9	119.9	NUM
eurjchem-448	240	22	ni(39)‐n(37)‐c(25	ni(39)‐n(37)‐c(25	NOUN
eurjchem-448	240	23	)	)	PUNCT
eurjchem-448	240	24	111.0	111.0	NUM
eurjchem-448	240	25	ni(39)‐s(28)‐c(36	ni(39)‐s(28)‐c(36	ADV
eurjchem-448	240	26	)	)	PUNCT
eurjchem-448	240	27	109.5	109.5	NUM
eurjchem-448	240	28	ni(39)‐s(28)‐c(30	ni(39)‐s(28)‐c(30	NOUN
eurjchem-448	240	29	)	)	PUNCT
eurjchem-448	240	30	104.0	104.0	NUM
eurjchem-448	240	31	ni(39)‐s(27)‐c(35	ni(39)‐s(27)‐c(35	NOUN
eurjchem-448	240	32	)	)	PUNCT
eurjchem-448	240	33	109.5	109.5	NUM
eurjchem-448	240	34	ni(39)‐s(27)‐c(24	ni(39)‐s(27)‐c(24	ADV
eurjchem-448	240	35	)	)	PUNCT
eurjchem-448	240	36	104.0	104.0	NUM
eurjchem-448	240	37	figure	figure	NOUN
eurjchem-448	240	38	5	5	NUM
eurjchem-448	240	39	.	.	PUNCT
eurjchem-448	241	1	solvent	solvent	ADJ
eurjchem-448	241	2	accessible	accessible	ADJ
eurjchem-448	241	3	surface	surface	NOUN
eurjchem-448	241	4	model	model	NOUN
eurjchem-448	241	5	of	of	ADP
eurjchem-448	241	6	macrocycle	macrocycle	NOUN
eurjchem-448	241	7	.	.	PUNCT
eurjchem-448	242	1	3.2.9	3.2.9	X
eurjchem-448	242	2	.	.	PUNCT
eurjchem-448	243	1	pharmaceutical	pharmaceutical	ADJ
eurjchem-448	243	2	activities	activity	NOUN
eurjchem-448	243	3	of	of	ADP
eurjchem-448	243	4	ces	ces	X
eurjchem-448	243	5	designing	designing	NOUN
eurjchem-448	243	6	and	and	CCONJ
eurjchem-448	243	7	tailoring	tailoring	NOUN
eurjchem-448	243	8	of	of	ADP
eurjchem-448	243	9	new	new	ADJ
eurjchem-448	243	10	biologically	biologically	ADV
eurjchem-448	243	11	active	active	ADJ
eurjchem-448	243	12	ces	ce	NOUN
eurjchem-448	243	13	are	be	AUX
eurjchem-448	243	14	crucial	crucial	ADJ
eurjchem-448	243	15	and	and	CCONJ
eurjchem-448	243	16	depends	depend	VERB
eurjchem-448	243	17	on	on	ADP
eurjchem-448	243	18	the	the	DET
eurjchem-448	243	19	utilization	utilization	NOUN
eurjchem-448	243	20	of	of	ADP
eurjchem-448	243	21	new	new	ADJ
eurjchem-448	243	22	methodologies	methodology	NOUN
eurjchem-448	243	23	and	and	CCONJ
eurjchem-448	243	24	implemented	implement	VERB
eurjchem-448	243	25	techniques	technique	NOUN
eurjchem-448	243	26	significantly	significantly	ADV
eurjchem-448	243	27	.	.	PUNCT
eurjchem-448	244	1	antimicrobial	antimicrobial	ADJ
eurjchem-448	244	2	effectiveness	effectiveness	NOUN
eurjchem-448	244	3	of	of	ADP
eurjchem-448	244	4	ces	ce	NOUN
eurjchem-448	244	5	depends	depend	VERB
eurjchem-448	244	6	upon	upon	SCONJ
eurjchem-448	244	7	several	several	ADJ
eurjchem-448	244	8	factors	factor	NOUN
eurjchem-448	244	9	i.e.	i.e.	X
eurjchem-448	244	10	metal	metal	NOUN
eurjchem-448	244	11	ion(s	ion(s	PROPN
eurjchem-448	244	12	)	)	PUNCT
eurjchem-448	244	13	,	,	PUNCT
eurjchem-448	244	14	chromophore	chromophore	NOUN
eurjchem-448	244	15	set	set	NOUN
eurjchem-448	244	16	of	of	ADP
eurjchem-448	244	17	mc	mc	PROPN
eurjchem-448	244	18	moiety	moiety	PROPN
eurjchem-448	244	19	and	and	CCONJ
eurjchem-448	244	20	other	other	ADJ
eurjchem-448	244	21	geometrical	geometrical	ADJ
eurjchem-448	244	22	features	feature	NOUN
eurjchem-448	244	23	.	.	PUNCT
eurjchem-448	245	1	the	the	DET
eurjchem-448	245	2	combined	combine	VERB
eurjchem-448	245	3	impact	impact	NOUN
eurjchem-448	245	4	of	of	ADP
eurjchem-448	245	5	these	these	DET
eurjchem-448	245	6	factors	factor	NOUN
eurjchem-448	245	7	makes	make	VERB
eurjchem-448	245	8	mc	mc	PROPN
eurjchem-448	245	9	moiety	moiety	NOUN
eurjchem-448	245	10	competent	competent	ADJ
eurjchem-448	245	11	as	as	SCONJ
eurjchem-448	245	12	desired	desire	VERB
eurjchem-448	245	13	.	.	PUNCT
eurjchem-448	246	1	mcs	mcs	PROPN
eurjchem-448	246	2	having	having	AUX
eurjchem-448	246	3	tailored	tailor	VERB
eurjchem-448	246	4	architectures	architecture	NOUN
eurjchem-448	246	5	and	and	CCONJ
eurjchem-448	246	6	antimicrobial	antimicrobial	ADJ
eurjchem-448	246	7	effectiveness	effectiveness	NOUN
eurjchem-448	246	8	are	be	AUX
eurjchem-448	246	9	well	well	ADV
eurjchem-448	246	10	known	know	VERB
eurjchem-448	246	11	.	.	PUNCT
eurjchem-448	247	1	designed	design	VERB
eurjchem-448	247	2	ces	ce	NOUN
eurjchem-448	247	3	having	have	VERB
eurjchem-448	247	4	appropriate	appropriate	ADJ
eurjchem-448	247	5	metal	metal	NOUN
eurjchem-448	247	6	/	/	SYM
eurjchem-448	247	7	ligand	ligand	NOUN
eurjchem-448	247	8	stability	stability	NOUN
eurjchem-448	247	9	within	within	ADP
eurjchem-448	247	10	the	the	DET
eurjchem-448	247	11	cavity	cavity	NOUN
eurjchem-448	247	12	of	of	ADP
eurjchem-448	247	13	macrocycle	macrocycle	NOUN
eurjchem-448	247	14	moiety	moiety	PROPN
eurjchem-448	247	15	were	be	AUX
eurjchem-448	247	16	discussed	discuss	VERB
eurjchem-448	247	17	.	.	PUNCT
eurjchem-448	248	1	moreover	moreover	ADV
eurjchem-448	248	2	,	,	PUNCT
eurjchem-448	248	3	coordination	coordination	NOUN
eurjchem-448	248	4	reduces	reduce	VERB
eurjchem-448	248	5	the	the	DET
eurjchem-448	248	6	polarity	polarity	NOUN
eurjchem-448	248	7	of	of	ADP
eurjchem-448	248	8	metal	metal	NOUN
eurjchem-448	248	9	ion(s	ion(s	PROPN
eurjchem-448	248	10	)	)	PUNCT
eurjchem-448	248	11	because	because	SCONJ
eurjchem-448	248	12	of	of	ADP
eurjchem-448	248	13	partial	partial	ADJ
eurjchem-448	248	14	sharing	sharing	NOUN
eurjchem-448	248	15	of	of	ADP
eurjchem-448	248	16	its	its	PRON
eurjchem-448	248	17	positive	positive	ADJ
eurjchem-448	248	18	charge	charge	NOUN
eurjchem-448	248	19	with	with	ADP
eurjchem-448	248	20	donor	donor	NOUN
eurjchem-448	248	21	atoms	atom	NOUN
eurjchem-448	248	22	within	within	ADP
eurjchem-448	248	23	the	the	DET
eurjchem-448	248	24	cavity	cavity	NOUN
eurjchem-448	248	25	of	of	ADP
eurjchem-448	248	26	mc	mc	PROPN
eurjchem-448	248	27	.	.	PROPN
eurjchem-448	249	1	kumar	kumar	PROPN
eurjchem-448	249	2	et	et	PROPN
eurjchem-448	249	3	al	al	PROPN
eurjchem-448	249	4	.	.	PUNCT
eurjchem-448	249	5	/	/	SYM
eurjchem-448	249	6	european	european	PROPN
eurjchem-448	249	7	journal	journal	PROPN
eurjchem-448	249	8	of	of	ADP
eurjchem-448	249	9	chemistry	chemistry	NOUN
eurjchem-448	249	10	3	3	NUM
eurjchem-448	249	11	(	(	PUNCT
eurjchem-448	249	12	1	1	NUM
eurjchem-448	249	13	)	)	PUNCT
eurjchem-448	249	14	(	(	PUNCT
eurjchem-448	249	15	2012	2012	NUM
eurjchem-448	249	16	)	)	PUNCT
eurjchem-448	249	17	57‐64	57‐64	NUM
eurjchem-448	249	18	63	63	NUM
eurjchem-448	249	19	during	during	ADP
eurjchem-448	249	20	this	this	DET
eurjchem-448	249	21	process	process	NOUN
eurjchem-448	249	22	,	,	PUNCT
eurjchem-448	249	23	lipophilic	lipophilic	ADJ
eurjchem-448	249	24	nature	nature	NOUN
eurjchem-448	249	25	of	of	ADP
eurjchem-448	249	26	central	central	ADJ
eurjchem-448	249	27	metal	metal	NOUN
eurjchem-448	249	28	atom	atom	NOUN
eurjchem-448	249	29	increases	increase	NOUN
eurjchem-448	249	30	as	as	ADP
eurjchem-448	249	31	a	a	DET
eurjchem-448	249	32	result	result	NOUN
eurjchem-448	249	33	favors	favor	VERB
eurjchem-448	249	34	permeation	permeation	NOUN
eurjchem-448	249	35	more	more	ADV
eurjchem-448	249	36	efficiently	efficiently	ADV
eurjchem-448	249	37	through	through	ADP
eurjchem-448	249	38	the	the	DET
eurjchem-448	249	39	lipid	lipid	NOUN
eurjchem-448	249	40	layer	layer	NOUN
eurjchem-448	249	41	of	of	ADP
eurjchem-448	249	42	the	the	DET
eurjchem-448	249	43	microorganism	microorganism	NOUN
eurjchem-448	249	44	to	to	PART
eurjchem-448	249	45	destroy	destroy	VERB
eurjchem-448	249	46	them	they	PRON
eurjchem-448	249	47	more	more	ADV
eurjchem-448	249	48	aggressively	aggressively	ADV
eurjchem-448	249	49	.	.	PUNCT
eurjchem-448	250	1	besides	besides	SCONJ
eurjchem-448	250	2	this	this	PRON
eurjchem-448	250	3	,	,	PUNCT
eurjchem-448	250	4	probably	probably	ADV
eurjchem-448	250	5	there	there	PRON
eurjchem-448	250	6	may	may	AUX
eurjchem-448	250	7	be	be	AUX
eurjchem-448	250	8	other	other	ADJ
eurjchem-448	250	9	factors	factor	NOUN
eurjchem-448	250	10	such	such	ADJ
eurjchem-448	250	11	as	as	ADP
eurjchem-448	250	12	solubility	solubility	NOUN
eurjchem-448	250	13	,	,	PUNCT
eurjchem-448	250	14	dipole	dipole	NOUN
eurjchem-448	250	15	moment	moment	NOUN
eurjchem-448	250	16	and	and	CCONJ
eurjchem-448	250	17	conductivity	conductivity	NOUN
eurjchem-448	250	18	which	which	PRON
eurjchem-448	250	19	may	may	AUX
eurjchem-448	250	20	be	be	AUX
eurjchem-448	250	21	influenced	influence	VERB
eurjchem-448	250	22	by	by	ADP
eurjchem-448	250	23	metal	metal	NOUN
eurjchem-448	250	24	ion(s	ion(s	PROPN
eurjchem-448	250	25	)	)	PUNCT
eurjchem-448	250	26	.	.	PUNCT
eurjchem-448	251	1	these	these	PRON
eurjchem-448	251	2	could	could	AUX
eurjchem-448	251	3	be	be	AUX
eurjchem-448	251	4	major	major	ADJ
eurjchem-448	251	5	reasons	reason	NOUN
eurjchem-448	251	6	behind	behind	ADP
eurjchem-448	251	7	the	the	DET
eurjchem-448	251	8	higher	high	ADJ
eurjchem-448	251	9	antimicrobial	antimicrobial	ADJ
eurjchem-448	251	10	effectiveness	effectiveness	NOUN
eurjchem-448	251	11	of	of	ADP
eurjchem-448	251	12	the	the	DET
eurjchem-448	251	13	ces	ce	NOUN
eurjchem-448	251	14	than	than	ADP
eurjchem-448	251	15	mcs	mcs	PROPN
eurjchem-448	252	1	[	[	X
eurjchem-448	252	2	27	27	NUM
eurjchem-448	252	3	]	]	PUNCT
eurjchem-448	252	4	.	.	PUNCT
eurjchem-448	253	1	figure	figure	NOUN
eurjchem-448	253	2	6	6	NUM
eurjchem-448	253	3	.	.	PUNCT
eurjchem-448	254	1	molecular	molecular	ADJ
eurjchem-448	254	2	model	model	NOUN
eurjchem-448	254	3	of	of	ADP
eurjchem-448	254	4	ce	ce	PROPN
eurjchem-448	254	5	of	of	ADP
eurjchem-448	254	6	ni(ii)so4	ni(ii)so4	PROPN
eurjchem-448	254	7	.	.	PUNCT
eurjchem-448	255	1	color	color	PROPN
eurjchem-448	255	2	code	code	PROPN
eurjchem-448	255	3	:	:	PUNCT
eurjchem-448	255	4	ni	ni	ADJ
eurjchem-448	255	5	,	,	PUNCT
eurjchem-448	255	6	dark	dark	ADJ
eurjchem-448	255	7	black	black	NOUN
eurjchem-448	255	8	;	;	PUNCT
eurjchem-448	255	9	c	c	X
eurjchem-448	255	10	,	,	PUNCT
eurjchem-448	255	11	light	light	ADJ
eurjchem-448	255	12	grey	grey	NOUN
eurjchem-448	255	13	;	;	PUNCT
eurjchem-448	255	14	n	n	CCONJ
eurjchem-448	255	15	,	,	PUNCT
eurjchem-448	255	16	blue	blue	ADJ
eurjchem-448	255	17	;	;	PUNCT
eurjchem-448	255	18	s	s	X
eurjchem-448	255	19	,	,	PUNCT
eurjchem-448	255	20	yellow	yellow	ADJ
eurjchem-448	255	21	.	.	PUNCT
eurjchem-448	256	1	ces	ces	PROPN
eurjchem-448	256	2	were	be	AUX
eurjchem-448	256	3	directly	directly	ADV
eurjchem-448	256	4	mixed	mix	VERB
eurjchem-448	256	5	in	in	ADP
eurjchem-448	256	6	a	a	DET
eurjchem-448	256	7	medium	medium	NOUN
eurjchem-448	256	8	of	of	ADP
eurjchem-448	256	9	different	different	ADJ
eurjchem-448	256	10	concentrations	concentration	NOUN
eurjchem-448	256	11	.	.	PUNCT
eurjchem-448	257	1	the	the	DET
eurjchem-448	257	2	fungus	fungus	NOUN
eurjchem-448	257	3	was	be	AUX
eurjchem-448	257	4	positioned	position	VERB
eurjchem-448	257	5	in	in	ADP
eurjchem-448	257	6	the	the	DET
eurjchem-448	257	7	medium	medium	NOUN
eurjchem-448	257	8	with	with	ADP
eurjchem-448	257	9	help	help	NOUN
eurjchem-448	257	10	of	of	ADP
eurjchem-448	257	11	an	an	DET
eurjchem-448	257	12	inoculum	inoculum	NOUN
eurjchem-448	257	13	’s	’s	PART
eurjchem-448	257	14	needle	needle	NOUN
eurjchem-448	257	15	.	.	PUNCT
eurjchem-448	258	1	petri	petri	ADJ
eurjchem-448	258	2	dishes	dish	NOUN
eurjchem-448	258	3	wrapped	wrap	VERB
eurjchem-448	258	4	in	in	ADP
eurjchem-448	258	5	polythene	polythene	NOUN
eurjchem-448	258	6	sheets	sheet	NOUN
eurjchem-448	258	7	containing	contain	VERB
eurjchem-448	258	8	some	some	DET
eurjchem-448	258	9	drops	drop	NOUN
eurjchem-448	258	10	of	of	ADP
eurjchem-448	258	11	c2h5oh	c2h5oh	PROPN
eurjchem-448	258	12	were	be	AUX
eurjchem-448	258	13	put	put	VERB
eurjchem-448	258	14	in	in	ADP
eurjchem-448	258	15	an	an	DET
eurjchem-448	258	16	incubator	incubator	NOUN
eurjchem-448	258	17	at	at	ADP
eurjchem-448	258	18	30±3	30±3	PROPN
eurjchem-448	258	19	°	°	ADP
eurjchem-448	258	20	c	c	NOUN
eurjchem-448	258	21	for	for	ADP
eurjchem-448	258	22	70‐90	70‐90	NUM
eurjchem-448	258	23	hrs	hrs	NOUN
eurjchem-448	258	24	.	.	PUNCT
eurjchem-448	259	1	the	the	DET
eurjchem-448	259	2	enlargement	enlargement	NOUN
eurjchem-448	259	3	of	of	ADP
eurjchem-448	259	4	fungal	fungal	ADJ
eurjchem-448	259	5	colony	colony	NOUN
eurjchem-448	259	6	was	be	AUX
eurjchem-448	259	7	measured	measure	VERB
eurjchem-448	259	8	in	in	ADP
eurjchem-448	259	9	diameter	diameter	NOUN
eurjchem-448	259	10	.	.	PUNCT
eurjchem-448	260	1	antifungal	antifungal	ADJ
eurjchem-448	260	2	activity	activity	NOUN
eurjchem-448	260	3	of	of	ADP
eurjchem-448	260	4	mc	mc	PROPN
eurjchem-448	260	5	and	and	CCONJ
eurjchem-448	260	6	ces	ces	PROPN
eurjchem-448	260	7	were	be	AUX
eurjchem-448	260	8	performed	perform	VERB
eurjchem-448	260	9	by	by	ADP
eurjchem-448	260	10	agar	agar	NOUN
eurjchem-448	260	11	plate	plate	NOUN
eurjchem-448	260	12	technique	technique	NOUN
eurjchem-448	260	13	against	against	ADP
eurjchem-448	260	14	aspergillus‐niger	aspergillus‐niger	NOUN
eurjchem-448	260	15	and	and	CCONJ
eurjchem-448	260	16	screened	screen	VERB
eurjchem-448	260	17	values	value	NOUN
eurjchem-448	260	18	were	be	AUX
eurjchem-448	260	19	arranged	arrange	VERB
eurjchem-448	260	20	graphically	graphically	ADV
eurjchem-448	260	21	in	in	ADP
eurjchem-448	260	22	figure	figure	NOUN
eurjchem-448	260	23	7	7	NUM
eurjchem-448	260	24	.	.	PUNCT
eurjchem-448	260	25	figure	figure	VERB
eurjchem-448	260	26	7	7	NUM
eurjchem-448	260	27	.	.	PUNCT
eurjchem-448	260	28	comparative	comparative	ADJ
eurjchem-448	260	29	aspects	aspect	NOUN
eurjchem-448	260	30	of	of	ADP
eurjchem-448	260	31	antifungal	antifungal	ADJ
eurjchem-448	260	32	findings	finding	NOUN
eurjchem-448	260	33	.	.	PUNCT
eurjchem-448	261	1	results	result	NOUN
eurjchem-448	261	2	indicate	indicate	VERB
eurjchem-448	261	3	that	that	SCONJ
eurjchem-448	261	4	ces	ce	NOUN
eurjchem-448	261	5	have	have	VERB
eurjchem-448	261	6	potential	potential	NOUN
eurjchem-448	261	7	to	to	PART
eurjchem-448	261	8	generate	generate	VERB
eurjchem-448	261	9	novel	novel	ADJ
eurjchem-448	261	10	antimicrobial	antimicrobial	ADJ
eurjchem-448	261	11	agent	agent	NOUN
eurjchem-448	261	12	by	by	ADP
eurjchem-448	261	13	displaying	display	VERB
eurjchem-448	261	14	moderate	moderate	ADJ
eurjchem-448	261	15	to	to	ADP
eurjchem-448	261	16	high	high	ADJ
eurjchem-448	261	17	affinities	affinity	NOUN
eurjchem-448	261	18	for	for	ADP
eurjchem-448	261	19	most	most	ADJ
eurjchem-448	261	20	of	of	ADP
eurjchem-448	261	21	the	the	DET
eurjchem-448	261	22	receptors	receptor	NOUN
eurjchem-448	261	23	particularly	particularly	ADV
eurjchem-448	261	24	in	in	ADP
eurjchem-448	261	25	case	case	NOUN
eurjchem-448	261	26	of	of	ADP
eurjchem-448	261	27	ni(ii)mc(scn)2	ni(ii)mc(scn)2	PROPN
eurjchem-448	261	28	.	.	PUNCT
eurjchem-448	262	1	cell	cell	NOUN
eurjchem-448	262	2	permeability	permeability	NOUN
eurjchem-448	262	3	is	be	AUX
eurjchem-448	262	4	due	due	ADJ
eurjchem-448	262	5	to	to	ADP
eurjchem-448	262	6	its	its	PRON
eurjchem-448	262	7	surrounding	surround	VERB
eurjchem-448	262	8	by	by	ADP
eurjchem-448	262	9	lipid	lipid	ADJ
eurjchem-448	262	10	membrane	membrane	NOUN
eurjchem-448	262	11	and	and	CCONJ
eurjchem-448	262	12	acts	act	NOUN
eurjchem-448	262	13	as	as	ADP
eurjchem-448	262	14	a	a	DET
eurjchem-448	262	15	special	special	ADJ
eurjchem-448	262	16	passage	passage	NOUN
eurjchem-448	262	17	for	for	ADP
eurjchem-448	262	18	lipid	lipid	ADJ
eurjchem-448	262	19	soluble	soluble	ADJ
eurjchem-448	262	20	materials	material	NOUN
eurjchem-448	262	21	.	.	PUNCT
eurjchem-448	263	1	so	so	ADV
eurjchem-448	263	2	,	,	PUNCT
eurjchem-448	263	3	it	it	PRON
eurjchem-448	263	4	showed	show	VERB
eurjchem-448	263	5	liposolubility	liposolubility	NOUN
eurjchem-448	263	6	and	and	CCONJ
eurjchem-448	263	7	increased	increase	VERB
eurjchem-448	263	8	antimicrobial	antimicrobial	ADJ
eurjchem-448	263	9	resistance	resistance	NOUN
eurjchem-448	263	10	in	in	ADP
eurjchem-448	263	11	a	a	DET
eurjchem-448	263	12	cell	cell	NOUN
eurjchem-448	263	13	.	.	PUNCT
eurjchem-448	264	1	this	this	PRON
eurjchem-448	264	2	is	be	AUX
eurjchem-448	264	3	known	know	VERB
eurjchem-448	264	4	as	as	ADP
eurjchem-448	264	5	the	the	DET
eurjchem-448	264	6	most	most	ADV
eurjchem-448	264	7	important	important	ADJ
eurjchem-448	264	8	biological	biological	ADJ
eurjchem-448	264	9	phenomenon	phenomenon	NOUN
eurjchem-448	264	10	in	in	ADP
eurjchem-448	264	11	regard	regard	NOUN
eurjchem-448	264	12	to	to	ADP
eurjchem-448	264	13	antifungal	antifungal	ADJ
eurjchem-448	264	14	aspects	aspect	NOUN
eurjchem-448	264	15	.	.	PUNCT
eurjchem-448	265	1	keeping	keep	VERB
eurjchem-448	265	2	in	in	ADP
eurjchem-448	265	3	view	view	NOUN
eurjchem-448	265	4	the	the	DET
eurjchem-448	265	5	problem	problem	NOUN
eurjchem-448	265	6	of	of	ADP
eurjchem-448	265	7	antimicrobial	antimicrobial	ADJ
eurjchem-448	265	8	resistance	resistance	NOUN
eurjchem-448	265	9	,	,	PUNCT
eurjchem-448	265	10	reported	report	VERB
eurjchem-448	265	11	ces	ce	NOUN
eurjchem-448	265	12	show	show	NOUN
eurjchem-448	265	13	good	good	ADJ
eurjchem-448	265	14	antimicrobial	antimicrobial	ADJ
eurjchem-448	265	15	character	character	NOUN
eurjchem-448	265	16	.	.	PUNCT
eurjchem-448	266	1	polarity	polarity	NOUN
eurjchem-448	266	2	is	be	AUX
eurjchem-448	266	3	directly	directly	ADV
eurjchem-448	266	4	influenced	influence	VERB
eurjchem-448	266	5	by	by	ADP
eurjchem-448	266	6	coordination	coordination	NOUN
eurjchem-448	266	7	abilities	ability	NOUN
eurjchem-448	266	8	of	of	ADP
eurjchem-448	266	9	the	the	DET
eurjchem-448	266	10	metal	metal	NOUN
eurjchem-448	266	11	because	because	SCONJ
eurjchem-448	266	12	of	of	ADP
eurjchem-448	266	13	partial	partial	ADJ
eurjchem-448	266	14	sharing	sharing	NOUN
eurjchem-448	266	15	of	of	ADP
eurjchem-448	266	16	its	its	PRON
eurjchem-448	266	17	positive	positive	ADJ
eurjchem-448	266	18	charge	charge	NOUN
eurjchem-448	266	19	within	within	ADP
eurjchem-448	266	20	mc	mc	PROPN
eurjchem-448	266	21	system	system	PROPN
eurjchem-448	266	22	having	have	VERB
eurjchem-448	266	23	π‐electron	π‐electron	PUNCT
eurjchem-448	266	24	delocalization	delocalization	NOUN
eurjchem-448	266	25	.	.	PUNCT
eurjchem-448	267	1	ces	ce	NOUN
eurjchem-448	267	2	have	have	VERB
eurjchem-448	267	3	higher	high	ADJ
eurjchem-448	267	4	activity	activity	NOUN
eurjchem-448	267	5	than	than	ADP
eurjchem-448	267	6	free	free	ADJ
eurjchem-448	267	7	ligand	ligand	NOUN
eurjchem-448	267	8	because	because	SCONJ
eurjchem-448	267	9	of	of	ADP
eurjchem-448	267	10	increased	increase	VERB
eurjchem-448	267	11	activity	activity	NOUN
eurjchem-448	267	12	of	of	ADP
eurjchem-448	267	13	metal	metal	NOUN
eurjchem-448	267	14	chelates	chelate	NOUN
eurjchem-448	267	15	according	accord	VERB
eurjchem-448	267	16	to	to	ADP
eurjchem-448	267	17	overtone	overtone	NOUN
eurjchem-448	267	18	's	's	PART
eurjchem-448	267	19	concept	concept	NOUN
eurjchem-448	267	20	.	.	PUNCT
eurjchem-448	268	1	the	the	DET
eurjchem-448	268	2	inhibition	inhibition	NOUN
eurjchem-448	268	3	activity	activity	NOUN
eurjchem-448	268	4	of	of	ADP
eurjchem-448	268	5	compounds	compound	NOUN
eurjchem-448	268	6	seems	seem	VERB
eurjchem-448	268	7	to	to	PART
eurjchem-448	268	8	govern	govern	VERB
eurjchem-448	268	9	with	with	ADP
eurjchem-448	268	10	certain	certain	ADJ
eurjchem-448	268	11	degree	degree	NOUN
eurjchem-448	268	12	as	as	ADP
eurjchem-448	268	13	per	per	ADP
eurjchem-448	268	14	the	the	DET
eurjchem-448	268	15	availability	availability	NOUN
eurjchem-448	268	16	percentile	percentile	NOUN
eurjchem-448	268	17	of	of	ADP
eurjchem-448	268	18	sulphur	sulphur	NOUN
eurjchem-448	268	19	atoms	atom	NOUN
eurjchem-448	268	20	in	in	ADP
eurjchem-448	268	21	mc	mc	PROPN
eurjchem-448	268	22	and	and	CCONJ
eurjchem-448	268	23	ces	ces	PROPN
eurjchem-448	268	24	.	.	PUNCT
eurjchem-448	269	1	this	this	PRON
eurjchem-448	269	2	is	be	AUX
eurjchem-448	269	3	because	because	SCONJ
eurjchem-448	269	4	tetrathia	tetrathia	NOUN
eurjchem-448	269	5	macrocycle	macrocycle	NOUN
eurjchem-448	269	6	shows	show	VERB
eurjchem-448	269	7	more	more	ADJ
eurjchem-448	269	8	activity	activity	NOUN
eurjchem-448	269	9	against	against	ADP
eurjchem-448	269	10	aspergillus	aspergillus	NOUN
eurjchem-448	269	11	niger	niger	NOUN
eurjchem-448	269	12	compared	compare	VERB
eurjchem-448	269	13	to	to	ADP
eurjchem-448	269	14	those	those	PRON
eurjchem-448	269	15	having	have	VERB
eurjchem-448	269	16	lesser	less	ADJ
eurjchem-448	269	17	number	number	NOUN
eurjchem-448	269	18	of	of	ADP
eurjchem-448	269	19	sulphur	sulphur	NOUN
eurjchem-448	269	20	atoms	atom	NOUN
eurjchem-448	269	21	within	within	ADP
eurjchem-448	269	22	the	the	DET
eurjchem-448	269	23	system	system	NOUN
eurjchem-448	269	24	.	.	PUNCT
eurjchem-448	270	1	4	4	X
eurjchem-448	270	2	.	.	X
eurjchem-448	270	3	conclusions	conclusion	NOUN
eurjchem-448	270	4	various	various	ADJ
eurjchem-448	270	5	properties	property	NOUN
eurjchem-448	270	6	of	of	ADP
eurjchem-448	270	7	macrocycles	macrocycle	NOUN
eurjchem-448	270	8	i.e.	i.e.	X
eurjchem-448	270	9	dimension	dimension	NOUN
eurjchem-448	270	10	of	of	ADP
eurjchem-448	270	11	internal	internal	ADJ
eurjchem-448	270	12	cavity	cavity	NOUN
eurjchem-448	270	13	,	,	PUNCT
eurjchem-448	270	14	rigidity	rigidity	NOUN
eurjchem-448	270	15	,	,	PUNCT
eurjchem-448	270	16	nature	nature	NOUN
eurjchem-448	270	17	and	and	CCONJ
eurjchem-448	270	18	number	number	NOUN
eurjchem-448	270	19	of	of	ADP
eurjchem-448	270	20	donor	donor	NOUN
eurjchem-448	270	21	atoms	atom	NOUN
eurjchem-448	270	22	and	and	CCONJ
eurjchem-448	270	23	type	type	NOUN
eurjchem-448	270	24	of	of	ADP
eurjchem-448	270	25	anion(s	anion(s	NOUN
eurjchem-448	270	26	)	)	PUNCT
eurjchem-448	270	27	involved	involve	VERB
eurjchem-448	270	28	in	in	ADP
eurjchem-448	270	29	coordination	coordination	NOUN
eurjchem-448	270	30	depend	depend	VERB
eurjchem-448	270	31	on	on	ADP
eurjchem-448	270	32	synthetic	synthetic	ADJ
eurjchem-448	270	33	protocols	protocol	NOUN
eurjchem-448	270	34	and	and	CCONJ
eurjchem-448	270	35	nature	nature	NOUN
eurjchem-448	270	36	of	of	ADP
eurjchem-448	270	37	ces	ce	NOUN
eurjchem-448	270	38	significantly	significantly	ADV
eurjchem-448	270	39	.	.	PUNCT
eurjchem-448	271	1	keeping	keep	VERB
eurjchem-448	271	2	in	in	ADP
eurjchem-448	271	3	view	view	NOUN
eurjchem-448	271	4	the	the	DET
eurjchem-448	271	5	importance	importance	NOUN
eurjchem-448	271	6	of	of	ADP
eurjchem-448	271	7	pederson	pederson	PROPN
eurjchem-448	271	8	’s	’s	PART
eurjchem-448	271	9	findings	finding	NOUN
eurjchem-448	271	10	,	,	PUNCT
eurjchem-448	271	11	it	it	PRON
eurjchem-448	271	12	is	be	AUX
eurjchem-448	271	13	a	a	DET
eurjchem-448	271	14	challenge	challenge	NOUN
eurjchem-448	271	15	to	to	PART
eurjchem-448	271	16	design	design	VERB
eurjchem-448	271	17	macrocycle	macrocycle	NOUN
eurjchem-448	271	18	topologies	topology	NOUN
eurjchem-448	271	19	having	having	AUX
eurjchem-448	271	20	desired	desire	VERB
eurjchem-448	271	21	properties	property	NOUN
eurjchem-448	271	22	[	[	X
eurjchem-448	271	23	28,29	28,29	NUM
eurjchem-448	271	24	]	]	X
eurjchem-448	271	25	.	.	PUNCT
eurjchem-448	272	1	a	a	DET
eurjchem-448	272	2	22‐	22‐	NUM
eurjchem-448	272	3	membered	membere	VERB
eurjchem-448	272	4	n2s4	n2s4	NOUN
eurjchem-448	272	5	chromophore	chromophore	NOUN
eurjchem-448	272	6	containing	contain	VERB
eurjchem-448	272	7	mc	mc	PROPN
eurjchem-448	272	8	was	be	AUX
eurjchem-448	272	9	designed	design	VERB
eurjchem-448	272	10	and	and	CCONJ
eurjchem-448	272	11	synthesized	synthesize	VERB
eurjchem-448	272	12	successfully	successfully	ADV
eurjchem-448	272	13	for	for	ADP
eurjchem-448	272	14	architecture	architecture	NOUN
eurjchem-448	272	15	and	and	CCONJ
eurjchem-448	272	16	tailoring	tailoring	NOUN
eurjchem-448	272	17	of	of	ADP
eurjchem-448	272	18	ces	ce	NOUN
eurjchem-448	272	19	of	of	ADP
eurjchem-448	272	20	ni(ii	ni(ii	NOUN
eurjchem-448	272	21	)	)	PUNCT
eurjchem-448	272	22	and	and	CCONJ
eurjchem-448	272	23	co(ii	co(ii	PROPN
eurjchem-448	272	24	)	)	PUNCT
eurjchem-448	272	25	.	.	PUNCT
eurjchem-448	273	1	molecular	molecular	ADJ
eurjchem-448	273	2	models	model	NOUN
eurjchem-448	273	3	confirmed	confirm	VERB
eurjchem-448	273	4	the	the	DET
eurjchem-448	273	5	location	location	NOUN
eurjchem-448	273	6	of	of	ADP
eurjchem-448	273	7	metal	metal	NOUN
eurjchem-448	273	8	ion(s	ion(s	PROPN
eurjchem-448	273	9	)	)	PUNCT
eurjchem-448	273	10	surrounded	surround	VERB
eurjchem-448	273	11	by	by	ADP
eurjchem-448	273	12	four	four	NUM
eurjchem-448	273	13	sulphur	sulphur	NOUN
eurjchem-448	273	14	and	and	CCONJ
eurjchem-448	273	15	two	two	NUM
eurjchem-448	273	16	nitrogen	nitrogen	NOUN
eurjchem-448	273	17	donor	donor	NOUN
eurjchem-448	273	18	sites	site	NOUN
eurjchem-448	273	19	in	in	ADP
eurjchem-448	273	20	equatorial	equatorial	ADJ
eurjchem-448	273	21	plane	plane	NOUN
eurjchem-448	273	22	acting	act	VERB
eurjchem-448	273	23	as	as	ADP
eurjchem-448	273	24	lewis	lewis	PROPN
eurjchem-448	273	25	base	base	NOUN
eurjchem-448	273	26	within	within	ADP
eurjchem-448	273	27	the	the	DET
eurjchem-448	273	28	cavity	cavity	NOUN
eurjchem-448	273	29	.	.	PUNCT
eurjchem-448	274	1	the	the	DET
eurjchem-448	274	2	interest	interest	NOUN
eurjchem-448	274	3	in	in	ADP
eurjchem-448	274	4	such	such	ADJ
eurjchem-448	274	5	species	specie	NOUN
eurjchem-448	274	6	stems	stem	VERB
eurjchem-448	274	7	from	from	ADP
eurjchem-448	274	8	the	the	DET
eurjchem-448	274	9	application	application	NOUN
eurjchem-448	274	10	of	of	ADP
eurjchem-448	274	11	these	these	DET
eurjchem-448	274	12	complexes	complex	NOUN
eurjchem-448	274	13	ranging	range	VERB
eurjchem-448	274	14	from	from	ADP
eurjchem-448	274	15	modeling	model	VERB
eurjchem-448	274	16	the	the	DET
eurjchem-448	274	17	active	active	ADJ
eurjchem-448	274	18	sites	site	NOUN
eurjchem-448	274	19	of	of	ADP
eurjchem-448	274	20	many	many	ADJ
eurjchem-448	274	21	metalloenzymes	metalloenzyme	NOUN
eurjchem-448	274	22	to	to	PART
eurjchem-448	274	23	host	host	VERB
eurjchem-448	274	24	and	and	CCONJ
eurjchem-448	274	25	carry	carry	VERB
eurjchem-448	274	26	small	small	ADJ
eurjchem-448	274	27	molecules	molecule	NOUN
eurjchem-448	274	28	or	or	CCONJ
eurjchem-448	274	29	catalysis	catalysis	NOUN
eurjchem-448	274	30	.	.	PUNCT
eurjchem-448	275	1	ces	ce	NOUN
eurjchem-448	275	2	were	be	AUX
eurjchem-448	275	3	screened	screen	VERB
eurjchem-448	275	4	against	against	ADP
eurjchem-448	275	5	a	a	DET
eurjchem-448	275	6	fungus	fungus	NOUN
eurjchem-448	275	7	caused	cause	VERB
eurjchem-448	275	8	a	a	DET
eurjchem-448	275	9	disease	disease	NOUN
eurjchem-448	275	10	black	black	ADJ
eurjchem-448	275	11	mold	mold	NOUN
eurjchem-448	275	12	on	on	ADP
eurjchem-448	275	13	certain	certain	ADJ
eurjchem-448	275	14	fruits	fruit	NOUN
eurjchem-448	275	15	and	and	CCONJ
eurjchem-448	275	16	vegetables	vegetable	NOUN
eurjchem-448	275	17	such	such	ADJ
eurjchem-448	275	18	as	as	ADP
eurjchem-448	275	19	grapes	grape	NOUN
eurjchem-448	275	20	,	,	PUNCT
eurjchem-448	275	21	onions	onion	NOUN
eurjchem-448	275	22	,	,	PUNCT
eurjchem-448	275	23	peanuts	peanut	NOUN
eurjchem-448	275	24	,	,	PUNCT
eurjchem-448	275	25	as	as	SCONJ
eurjchem-448	275	26	it	it	PRON
eurjchem-448	275	27	is	be	AUX
eurjchem-448	275	28	a	a	DET
eurjchem-448	275	29	common	common	ADJ
eurjchem-448	275	30	contaminant	contaminant	NOUN
eurjchem-448	275	31	of	of	ADP
eurjchem-448	275	32	food	food	NOUN
eurjchem-448	275	33	.	.	PUNCT
eurjchem-448	276	1	ces	ces	PROPN
eurjchem-448	276	2	disturbed	disturbed	ADJ
eurjchem-448	276	3	respiration	respiration	NOUN
eurjchem-448	276	4	process	process	NOUN
eurjchem-448	276	5	of	of	ADP
eurjchem-448	276	6	cell	cell	NOUN
eurjchem-448	276	7	and	and	CCONJ
eurjchem-448	276	8	blocked	block	VERB
eurjchem-448	276	9	proteins	protein	NOUN
eurjchem-448	276	10	synthesis	synthesis	NOUN
eurjchem-448	276	11	.	.	PUNCT
eurjchem-448	277	1	it	it	PRON
eurjchem-448	277	2	evidenced	evidence	VERB
eurjchem-448	277	3	that	that	PRON
eurjchem-448	277	4	hydrophobicity	hydrophobicity	NOUN
eurjchem-448	277	5	and	and	CCONJ
eurjchem-448	277	6	steric	steric	ADJ
eurjchem-448	277	7	effects	effect	NOUN
eurjchem-448	277	8	comprise	comprise	VERB
eurjchem-448	277	9	two	two	NUM
eurjchem-448	277	10	major	major	ADJ
eurjchem-448	277	11	factors	factor	NOUN
eurjchem-448	277	12	that	that	PRON
eurjchem-448	277	13	govern	govern	VERB
eurjchem-448	277	14	antimicrobial	antimicrobial	ADJ
eurjchem-448	277	15	effectiveness	effectiveness	NOUN
eurjchem-448	277	16	.	.	PUNCT
eurjchem-448	278	1	electron	electron	NOUN
eurjchem-448	278	2	delocalization	delocalization	NOUN
eurjchem-448	278	3	along	along	ADP
eurjchem-448	278	4	with	with	ADP
eurjchem-448	278	5	main	main	ADJ
eurjchem-448	278	6	chain	chain	NOUN
eurjchem-448	278	7	of	of	ADP
eurjchem-448	278	8	‐s‐(ch2)3‐	‐s‐(ch2)3‐	PRON
eurjchem-448	278	9	s‐	s‐	PROPN
eurjchem-448	278	10	bounds	bound	VERB
eurjchem-448	278	11	metal	metal	PROPN
eurjchem-448	278	12	ion(s	ion(s	PROPN
eurjchem-448	278	13	)	)	PUNCT
eurjchem-448	278	14	and	and	CCONJ
eurjchem-448	278	15	can	can	AUX
eurjchem-448	278	16	be	be	AUX
eurjchem-448	278	17	considered	consider	VERB
eurjchem-448	278	18	as	as	ADP
eurjchem-448	278	19	a	a	DET
eurjchem-448	278	20	main	main	ADJ
eurjchem-448	278	21	substituent	substituent	NOUN
eurjchem-448	278	22	group	group	NOUN
eurjchem-448	278	23	along	along	ADP
eurjchem-448	278	24	macrocyclic	macrocyclic	NOUN
eurjchem-448	278	25	backbone	backbone	NOUN
eurjchem-448	278	26	or	or	CCONJ
eurjchem-448	278	27	vice	vice	NOUN
eurjchem-448	278	28	versa	versa	ADV
eurjchem-448	278	29	.	.	PUNCT
eurjchem-448	279	1	in	in	ADP
eurjchem-448	279	2	both	both	DET
eurjchem-448	279	3	situations	situation	NOUN
eurjchem-448	279	4	it	it	PRON
eurjchem-448	279	5	is	be	AUX
eurjchem-448	279	6	important	important	ADJ
eurjchem-448	279	7	to	to	PART
eurjchem-448	279	8	modulate	modulate	VERB
eurjchem-448	279	9	chemical	chemical	NOUN
eurjchem-448	279	10	and	and	CCONJ
eurjchem-448	279	11	physical	physical	ADJ
eurjchem-448	279	12	features	feature	NOUN
eurjchem-448	279	13	of	of	ADP
eurjchem-448	279	14	ligand	ligand	NOUN
eurjchem-448	279	15	and	and	CCONJ
eurjchem-448	279	16	also	also	ADV
eurjchem-448	279	17	on	on	ADP
eurjchem-448	279	18	the	the	DET
eurjchem-448	279	19	properties	property	NOUN
eurjchem-448	279	20	of	of	ADP
eurjchem-448	279	21	ces	ce	NOUN
eurjchem-448	279	22	.	.	PUNCT
eurjchem-448	280	1	in	in	ADP
eurjchem-448	280	2	electronic	electronic	ADJ
eurjchem-448	280	3	spectra	spectra	ADJ
eurjchem-448	280	4	main	main	ADJ
eurjchem-448	280	5	bands	band	NOUN
eurjchem-448	280	6	may	may	AUX
eurjchem-448	280	7	be	be	AUX
eurjchem-448	280	8	attributed	attribute	VERB
eurjchem-448	280	9	to	to	ADP
eurjchem-448	280	10	thio	thio	NOUN
eurjchem-448	280	11	s(σ	s(σ	PROPN
eurjchem-448	280	12	)	)	PUNCT
eurjchem-448	280	13	→	→	SYM
eurjchem-448	280	14	co(ii	co(ii	PROPN
eurjchem-448	280	15	)	)	PUNCT
eurjchem-448	280	16	(	(	PUNCT
eurjchem-448	280	17	dπ	dπ	NOUN
eurjchem-448	280	18	)	)	PUNCT
eurjchem-448	280	19	and	and	CCONJ
eurjchem-448	280	20	thio	thio	NOUN
eurjchem-448	280	21	s(π	s(π	PROPN
eurjchem-448	280	22	)	)	PUNCT
eurjchem-448	280	23	→	→	SYM
eurjchem-448	280	24	co(ii	co(ii	PROPN
eurjchem-448	280	25	)	)	PUNCT
eurjchem-448	280	26	(	(	PUNCT
eurjchem-448	280	27	dπ	dπ	INTJ
eurjchem-448	280	28	)	)	PUNCT
eurjchem-448	280	29	as	as	SCONJ
eurjchem-448	280	30	ligand	ligand	ADJ
eurjchem-448	280	31	to	to	PART
eurjchem-448	280	32	metal	metal	NOUN
eurjchem-448	280	33	charge	charge	NOUN
eurjchem-448	280	34	transfer	transfer	NOUN
eurjchem-448	280	35	transitions	transition	NOUN
eurjchem-448	280	36	(	(	PUNCT
eurjchem-448	280	37	lmct	lmct	NOUN
eurjchem-448	280	38	)	)	PUNCT
eurjchem-448	280	39	.	.	PUNCT
eurjchem-448	281	1	acknowledgements	acknowledgement	NOUN
eurjchem-448	281	2	one	one	NUM
eurjchem-448	281	3	of	of	ADP
eurjchem-448	281	4	the	the	DET
eurjchem-448	281	5	authors	author	NOUN
eurjchem-448	281	6	(	(	PUNCT
eurjchem-448	281	7	rajiv	rajiv	PROPN
eurjchem-448	281	8	kumar	kumar	PROPN
eurjchem-448	281	9	)	)	PUNCT
eurjchem-448	281	10	gratefully	gratefully	ADV
eurjchem-448	281	11	acknowledges	acknowledge	VERB
eurjchem-448	281	12	his	his	PRON
eurjchem-448	281	13	younger	young	ADJ
eurjchem-448	281	14	brother	brother	NOUN
eurjchem-448	281	15	bitto	bitto	VERB
eurjchem-448	281	16	and	and	CCONJ
eurjchem-448	281	17	sister	sister	NOUN
eurjchem-448	281	18	renu	renu	NOUN
eurjchem-448	281	19	for	for	ADP
eurjchem-448	281	20	motivation	motivation	NOUN
eurjchem-448	281	21	.	.	PUNCT
eurjchem-448	282	1	authors	author	NOUN
eurjchem-448	282	2	acknowledge	acknowledge	VERB
eurjchem-448	282	3	central	central	ADJ
eurjchem-448	282	4	science	science	NOUN
eurjchem-448	282	5	library	library	NOUN
eurjchem-448	282	6	,	,	PUNCT
eurjchem-448	282	7	university	university	PROPN
eurjchem-448	282	8	delhi	delhi	PROPN
eurjchem-448	282	9	,	,	PUNCT
eurjchem-448	282	10	delhi	delhi	PROPN
eurjchem-448	282	11	for	for	ADP
eurjchem-448	282	12	providing	provide	VERB
eurjchem-448	282	13	computer	computer	NOUN
eurjchem-448	282	14	facilities	facility	NOUN
eurjchem-448	282	15	,	,	PUNCT
eurjchem-448	282	16	indian	indian	PROPN
eurjchem-448	282	17	institute	institute	PROPN
eurjchem-448	282	18	of	of	ADP
eurjchem-448	282	19	technology	technology	PROPN
eurjchem-448	282	20	bombay	bombay	PROPN
eurjchem-448	282	21	and	and	CCONJ
eurjchem-448	282	22	indian	indian	PROPN
eurjchem-448	282	23	institute	institute	PROPN
eurjchem-448	282	24	of	of	ADP
eurjchem-448	282	25	technology	technology	PROPN
eurjchem-448	282	26	delhi	delhi	ADJ
eurjchem-448	282	27	for	for	ADP
eurjchem-448	282	28	recording	record	VERB
eurjchem-448	282	29	epr	epr	PROPN
eurjchem-448	282	30	,	,	PUNCT
eurjchem-448	282	31	1h	1h	NUM
eurjchem-448	282	32	nmr	nmr	NOUN
eurjchem-448	282	33	and	and	CCONJ
eurjchem-448	282	34	13c	13c	NOUN
eurjchem-448	282	35	nmr	nmr	NOUN
eurjchem-448	282	36	spectra	spectra	NOUN
eurjchem-448	282	37	respectively	respectively	ADV
eurjchem-448	282	38	and	and	CCONJ
eurjchem-448	282	39	to	to	ADP
eurjchem-448	282	40	indian	indian	PROPN
eurjchem-448	282	41	institute	institute	PROPN
eurjchem-448	282	42	of	of	ADP
eurjchem-448	282	43	technology	technology	PROPN
eurjchem-448	282	44	roorkee	roorkee	PROPN
eurjchem-448	282	45	,	,	PUNCT
eurjchem-448	282	46	india	india	PROPN
eurjchem-448	282	47	for	for	ADP
eurjchem-448	282	48	recording	record	VERB
eurjchem-448	282	49	magnetic	magnetic	ADJ
eurjchem-448	282	50	moments	moment	NOUN
eurjchem-448	282	51	.	.	PUNCT
eurjchem-448	283	1	references	reference	NOUN
eurjchem-448	283	2	[	[	X
eurjchem-448	283	3	1	1	NUM
eurjchem-448	283	4	]	]	PUNCT
eurjchem-448	283	5	.	.	PUNCT
eurjchem-448	284	1	saeeda	saeeda	PROPN
eurjchem-448	284	2	,	,	PUNCT
eurjchem-448	284	3	s.	s.	PROPN
eurjchem-448	284	4	;	;	PUNCT
eurjchem-448	284	5	rashid	rashid	PROPN
eurjchem-448	284	6	,	,	PUNCT
eurjchem-448	284	7	n.	n.	PROPN
eurjchem-448	284	8	;	;	PUNCT
eurjchem-448	284	9	ali	ali	PROPN
eurjchem-448	284	10	,	,	PUNCT
eurjchem-448	284	11	m.	m.	NOUN
eurjchem-448	284	12	;	;	PUNCT
eurjchem-448	284	13	hussain	hussain	PROPN
eurjchem-448	284	14	,	,	PUNCT
eurjchem-448	284	15	r.	r.	PROPN
eurjchem-448	284	16	;	;	PUNCT
eurjchem-448	284	17	jones	jones	PROPN
eurjchem-448	284	18	,	,	PUNCT
eurjchem-448	284	19	p.	p.	PROPN
eurjchem-448	284	20	eur	eur	PROPN
eurjchem-448	284	21	.	.	PUNCT
eurjchem-448	285	1	j.	j.	PROPN
eurjchem-448	285	2	chem	chem	PROPN
eurjchem-448	285	3	.	.	PUNCT
eurjchem-448	286	1	2010	2010	NUM
eurjchem-448	286	2	,	,	PUNCT
eurjchem-448	286	3	1(3	1(3	NUM
eurjchem-448	286	4	)	)	PUNCT
eurjchem-448	286	5	,	,	PUNCT
eurjchem-448	286	6	221‐227	221‐227	PROPN
eurjchem-448	286	7	.	.	PUNCT
eurjchem-448	287	1	[	[	X
eurjchem-448	287	2	2	2	NUM
eurjchem-448	287	3	]	]	PUNCT
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eurjchem-448	290	2	,	,	PUNCT
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eurjchem-448	290	4	,	,	PUNCT
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eurjchem-448	290	6	.	.	PUNCT
eurjchem-448	291	1	[	[	X
eurjchem-448	291	2	3	3	NUM
eurjchem-448	291	3	]	]	PUNCT
eurjchem-448	291	4	.	.	PUNCT
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eurjchem-448	292	25	f.	f.	PROPN
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eurjchem-448	292	28	,	,	PUNCT
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eurjchem-448	292	30	eur	eur	PROPN
eurjchem-448	292	31	.	.	PUNCT
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eurjchem-448	294	2	,	,	PUNCT
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eurjchem-448	294	4	,	,	PUNCT
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eurjchem-448	294	6	.	.	PUNCT
eurjchem-448	295	1	[	[	X
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eurjchem-448	296	9	s.	s.	PROPN
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eurjchem-448	296	13	,	,	PUNCT
eurjchem-448	296	14	i.	i.	PROPN
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eurjchem-448	296	22	,	,	PUNCT
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eurjchem-448	296	24	.	.	PROPN
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eurjchem-448	297	2	.	.	X
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eurjchem-448	297	8	.	.	PUNCT
eurjchem-448	298	1	[	[	X
eurjchem-448	298	2	5	5	NUM
eurjchem-448	298	3	]	]	PUNCT
eurjchem-448	298	4	.	.	PUNCT
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eurjchem-448	299	2	,	,	PUNCT
eurjchem-448	299	3	s.	s.	PROPN
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eurjchem-448	300	1	[	[	X
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eurjchem-448	300	4	.	.	PUNCT
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eurjchem-448	301	2	,	,	PUNCT
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eurjchem-448	302	2	,	,	PUNCT
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eurjchem-448	302	4	,	,	PUNCT
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eurjchem-448	302	6	.	.	PUNCT
eurjchem-448	303	1	[	[	X
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eurjchem-448	303	3	]	]	PUNCT
eurjchem-448	303	4	.	.	PUNCT
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eurjchem-448	303	11	.	.	PUNCT
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eurjchem-448	305	2	.	.	PUNCT
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eurjchem-448	306	2	,	,	PUNCT
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eurjchem-448	306	6	.	.	PUNCT
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eurjchem-448	307	4	.	.	PUNCT
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eurjchem-448	315	2	.	.	PUNCT
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eurjchem-448	317	4	.	.	PUNCT
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eurjchem-448	323	2	.	.	PUNCT
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eurjchem-448	324	2	,	,	PUNCT
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eurjchem-448	325	4	.	.	PUNCT
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eurjchem-448	328	2	,	,	PUNCT
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eurjchem-448	328	21	(	(	PUNCT
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eurjchem-448	332	4	,	,	PUNCT
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eurjchem-448	332	6	.	.	PUNCT
eurjchem-448	333	1	[	[	X
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eurjchem-448	333	3	]	]	PUNCT
eurjchem-448	333	4	.	.	PUNCT
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eurjchem-448	339	3	]	]	PUNCT
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eurjchem-448	344	2	,	,	PUNCT
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eurjchem-448	345	3	]	]	PUNCT
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eurjchem-448	367	2	.	.	PUNCT
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eurjchem-448	368	2	,	,	PUNCT
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