id	sid	tid	token	lemma	pos
eurjchem-460	1	1	untitled	untitle	VERB
eurjchem-460	1	2	european	european	PROPN
eurjchem-460	1	3	journal	journal	PROPN
eurjchem-460	1	4	of	of	ADP
eurjchem-460	1	5	chemistry	chemistry	NOUN
eurjchem-460	1	6	3	3	NUM
eurjchem-460	1	7	(	(	PUNCT
eurjchem-460	1	8	2	2	NUM
eurjchem-460	1	9	)	)	PUNCT
eurjchem-460	1	10	(	(	PUNCT
eurjchem-460	1	11	2012	2012	NUM
eurjchem-460	1	12	)	)	PUNCT
eurjchem-460	1	13	235‐240	235‐240	NUM
eurjchem-460	1	14	european	european	PROPN
eurjchem-460	1	15	journal	journal	PROPN
eurjchem-460	1	16	of	of	ADP
eurjchem-460	1	17	chemistry	chemistry	NOUN
eurjchem-460	1	18	issn	issn	PROPN
eurjchem-460	1	19	2153‐2249	2153‐2249	PROPN
eurjchem-460	1	20	(	(	PUNCT
eurjchem-460	1	21	print	print	NOUN
eurjchem-460	1	22	)	)	PUNCT
eurjchem-460	1	23	/	/	SYM
eurjchem-460	1	24	issn	issn	PROPN
eurjchem-460	1	25	2153‐2257	2153‐2257	NUM
eurjchem-460	1	26	(	(	PUNCT
eurjchem-460	1	27	online	online	ADJ
eurjchem-460	1	28	)	)	PUNCT
eurjchem-460	1	29			NOUN
eurjchem-460	1	30	2012	2012	NUM
eurjchem-460	1	31	eurjchem	eurjchem	PROPN
eurjchem-460	1	32	doi:10.5155	doi:10.5155	PROPN
eurjchem-460	1	33	/	/	SYM
eurjchem-460	1	34	eurjchem.3.2.235‐240.460	eurjchem.3.2.235‐240.460	ADV
eurjchem-460	1	35	european	european	ADJ
eurjchem-460	1	36	journal	journal	PROPN
eurjchem-460	1	37	of	of	ADP
eurjchem-460	1	38	chemistry	chemistry	PROPN
eurjchem-460	1	39	journal	journal	PROPN
eurjchem-460	1	40	homepage	homepage	NOUN
eurjchem-460	1	41	:	:	PUNCT
eurjchem-460	1	42	www.eurjchem.com	www.eurjchem.com	X
eurjchem-460	1	43	synthesis	synthesis	NOUN
eurjchem-460	1	44	of	of	ADP
eurjchem-460	1	45	ethylene	ethylene	NOUN
eurjchem-460	1	46	carbonate	carbonate	NOUN
eurjchem-460	1	47	from	from	ADP
eurjchem-460	1	48	cyclocondensation	cyclocondensation	NOUN
eurjchem-460	1	49	of	of	ADP
eurjchem-460	1	50	ethylene	ethylene	NOUN
eurjchem-460	1	51	glycol	glycol	NOUN
eurjchem-460	1	52	and	and	CCONJ
eurjchem-460	1	53	urea	urea	NOUN
eurjchem-460	1	54	over	over	ADP
eurjchem-460	1	55	zno•cr2o3	zno•cr2o3	PROPN
eurjchem-460	1	56	catalyst	catalyst	NOUN
eurjchem-460	1	57	system	system	NOUN
eurjchem-460	1	58	controlled	control	VERB
eurjchem-460	1	59	by	by	ADP
eurjchem-460	1	60	co‐precipitation	co‐precipitation	PROPN
eurjchem-460	1	61	method	method	PROPN
eurjchem-460	1	62	sheenu	sheenu	PROPN
eurjchem-460	1	63	bhadauriaa	bhadauriaa	ADJ
eurjchem-460	1	64	,	,	PUNCT
eurjchem-460	1	65	samidha	samidha	PROPN
eurjchem-460	1	66	saxenaa	saxenaa	PROPN
eurjchem-460	1	67	,	,	PUNCT
eurjchem-460	1	68	rajendra	rajendra	PROPN
eurjchem-460	1	69	prasada	prasada	PROPN
eurjchem-460	1	70	,	,	PUNCT
eurjchem-460	1	71	prabhakar	prabhakar	PROPN
eurjchem-460	1	72	sharmaa	sharmaa	VERB
eurjchem-460	1	73	,	,	PUNCT
eurjchem-460	1	74	rajendra	rajendra	PROPN
eurjchem-460	1	75	prasadb	prasadb	PROPN
eurjchem-460	1	76	and	and	CCONJ
eurjchem-460	1	77	reena	reena	PROPN
eurjchem-460	1	78	dwivedia	dwivedia	PROPN
eurjchem-460	1	79	,	,	PUNCT
eurjchem-460	1	80	*	*	PUNCT
eurjchem-460	1	81	a	a	DET
eurjchem-460	1	82	catalysis	catalysis	NOUN
eurjchem-460	1	83	and	and	CCONJ
eurjchem-460	1	84	nanomaterials	nanomaterial	NOUN
eurjchem-460	1	85	research	research	NOUN
eurjchem-460	1	86	laboratory	laboratory	NOUN
eurjchem-460	1	87	,	,	PUNCT
eurjchem-460	1	88	school	school	NOUN
eurjchem-460	1	89	of	of	ADP
eurjchem-460	1	90	chemical	chemical	NOUN
eurjchem-460	1	91	sciences	sciences	PROPN
eurjchem-460	1	92	,	,	PUNCT
eurjchem-460	1	93	devi	devi	PROPN
eurjchem-460	1	94	ahilya	ahilya	PROPN
eurjchem-460	1	95	university	university	PROPN
eurjchem-460	1	96	,	,	PUNCT
eurjchem-460	1	97	indore	indore	NOUN
eurjchem-460	1	98	,	,	PUNCT
eurjchem-460	1	99	452001	452001	NUM
eurjchem-460	1	100	,	,	PUNCT
eurjchem-460	1	101	india	india	PROPN
eurjchem-460	1	102	b	b	PROPN
eurjchem-460	1	103	department	department	PROPN
eurjchem-460	1	104	of	of	ADP
eurjchem-460	1	105	chemistry	chemistry	PROPN
eurjchem-460	1	106	,	,	PUNCT
eurjchem-460	1	107	amravati	amravati	PROPN
eurjchem-460	1	108	university	university	PROPN
eurjchem-460	1	109	,	,	PUNCT
eurjchem-460	1	110	amravati	amravati	PROPN
eurjchem-460	1	111	,	,	PUNCT
eurjchem-460	1	112	444602	444602	NUM
eurjchem-460	1	113	,	,	PUNCT
eurjchem-460	1	114	india	india	PROPN
eurjchem-460	1	115	*	*	PUNCT
eurjchem-460	1	116	corresponding	correspond	VERB
eurjchem-460	1	117	author	author	NOUN
eurjchem-460	1	118	at	at	ADP
eurjchem-460	1	119	:	:	PUNCT
eurjchem-460	1	120	catalysis	catalysis	NOUN
eurjchem-460	1	121	and	and	CCONJ
eurjchem-460	1	122	nanomaterials	nanomaterial	NOUN
eurjchem-460	1	123	research	research	NOUN
eurjchem-460	1	124	laboratory	laboratory	NOUN
eurjchem-460	1	125	,	,	PUNCT
eurjchem-460	1	126	school	school	NOUN
eurjchem-460	1	127	of	of	ADP
eurjchem-460	1	128	chemical	chemical	NOUN
eurjchem-460	1	129	sciences	sciences	PROPN
eurjchem-460	1	130	,	,	PUNCT
eurjchem-460	1	131	devi	devi	PROPN
eurjchem-460	1	132	ahilya	ahilya	PROPN
eurjchem-460	1	133	university	university	PROPN
eurjchem-460	1	134	,	,	PUNCT
eurjchem-460	1	135	indore	indore	NOUN
eurjchem-460	1	136	,	,	PUNCT
eurjchem-460	1	137	452001	452001	NUM
eurjchem-460	1	138	,	,	PUNCT
eurjchem-460	1	139	india	india	PROPN
eurjchem-460	1	140	.	.	PUNCT
eurjchem-460	2	1	tel	tel	PROPN
eurjchem-460	2	2	.	.	PUNCT
eurjchem-460	2	3	:	:	PUNCT
eurjchem-460	3	1	+91.731.2460208	+91.731.2460208	NUM
eurjchem-460	3	2	;	;	PUNCT
eurjchem-460	3	3	fax	fax	NOUN
eurjchem-460	3	4	:	:	PUNCT
eurjchem-460	3	5	+91.731.2763618	+91.731.2763618	NUM
eurjchem-460	3	6	.	.	PUNCT
eurjchem-460	3	7	e‐mail	e‐mail	PUNCT
eurjchem-460	4	1	address	address	NOUN
eurjchem-460	4	2	:	:	PUNCT
eurjchem-460	4	3	drreenadwivedi@rediffmail.com	drreenadwivedi@rediffmail.com	X
eurjchem-460	4	4	(	(	PUNCT
eurjchem-460	4	5	r.	r.	PROPN
eurjchem-460	4	6	dwivedi	dwivedi	PROPN
eurjchem-460	4	7	)	)	PUNCT
eurjchem-460	4	8	.	.	PUNCT
eurjchem-460	5	1	article	article	NOUN
eurjchem-460	5	2	information	information	PROPN
eurjchem-460	5	3	abstract	abstract	ADV
eurjchem-460	5	4	received	receive	VERB
eurjchem-460	5	5	:	:	PUNCT
eurjchem-460	5	6	12	12	NUM
eurjchem-460	5	7	may	may	PROPN
eurjchem-460	5	8	2011	2011	NUM
eurjchem-460	5	9	received	receive	VERB
eurjchem-460	5	10	in	in	ADP
eurjchem-460	5	11	revised	revise	VERB
eurjchem-460	5	12	form	form	NOUN
eurjchem-460	5	13	:	:	PUNCT
eurjchem-460	5	14	16	16	NUM
eurjchem-460	5	15	february	february	PROPN
eurjchem-460	5	16	2012	2012	NUM
eurjchem-460	5	17	accepted	accept	VERB
eurjchem-460	5	18	:	:	PUNCT
eurjchem-460	5	19	08	08	NUM
eurjchem-460	5	20	march	march	PROPN
eurjchem-460	5	21	2012	2012	NUM
eurjchem-460	5	22	online	online	NOUN
eurjchem-460	5	23	:	:	PUNCT
eurjchem-460	5	24	30	30	NUM
eurjchem-460	5	25	june	june	PROPN
eurjchem-460	5	26	2012	2012	NUM
eurjchem-460	5	27	keywords	keyword	NOUN
eurjchem-460	5	28	zno·cr2o3	zno·cr2o3	PROPN
eurjchem-460	5	29	catalyst	catalyst	NOUN
eurjchem-460	5	30	has	have	AUX
eurjchem-460	5	31	been	be	AUX
eurjchem-460	5	32	synthesized	synthesize	VERB
eurjchem-460	5	33	by	by	ADP
eurjchem-460	5	34	low	low	ADJ
eurjchem-460	5	35	temperature	temperature	NOUN
eurjchem-460	5	36	,	,	PUNCT
eurjchem-460	5	37	ph	ph	PROPN
eurjchem-460	5	38	controlled	control	VERB
eurjchem-460	5	39	co‐precipitation	co‐precipitation	NOUN
eurjchem-460	5	40	route	route	NOUN
eurjchem-460	5	41	and	and	CCONJ
eurjchem-460	5	42	characterized	characterize	VERB
eurjchem-460	5	43	employing	employ	VERB
eurjchem-460	5	44	techniques	technique	NOUN
eurjchem-460	5	45	of	of	ADP
eurjchem-460	5	46	brunauer	brunauer	NOUN
eurjchem-460	5	47	,	,	PUNCT
eurjchem-460	5	48	emmett	emmett	PROPN
eurjchem-460	5	49	,	,	PUNCT
eurjchem-460	5	50	and	and	CCONJ
eurjchem-460	5	51	teller	teller	NOUN
eurjchem-460	5	52	(	(	PUNCT
eurjchem-460	5	53	bet	bet	NOUN
eurjchem-460	5	54	)	)	PUNCT
eurjchem-460	5	55	surface	surface	NOUN
eurjchem-460	5	56	area	area	NOUN
eurjchem-460	5	57	measurement	measurement	NOUN
eurjchem-460	5	58	,	,	PUNCT
eurjchem-460	5	59	ammonia	ammonia	ADJ
eurjchem-460	5	60	desorption	desorption	NOUN
eurjchem-460	5	61	technique	technique	NOUN
eurjchem-460	5	62	,	,	PUNCT
eurjchem-460	5	63	x‐ray	x‐ray	PROPN
eurjchem-460	5	64	diffraction	diffraction	NOUN
eurjchem-460	5	65	(	(	PUNCT
eurjchem-460	5	66	xrd	xrd	PROPN
eurjchem-460	5	67	)	)	PUNCT
eurjchem-460	5	68	and	and	CCONJ
eurjchem-460	5	69	scanning	scan	VERB
eurjchem-460	5	70	electron	electron	NOUN
eurjchem-460	5	71	microscopy	microscopy	NOUN
eurjchem-460	5	72	(	(	PUNCT
eurjchem-460	5	73	sem	sem	NOUN
eurjchem-460	5	74	)	)	PUNCT
eurjchem-460	5	75	.	.	PUNCT
eurjchem-460	6	1	these	these	DET
eurjchem-460	6	2	characterizations	characterization	NOUN
eurjchem-460	6	3	reveal	reveal	VERB
eurjchem-460	6	4	the	the	DET
eurjchem-460	6	5	catalyst	catalyst	NOUN
eurjchem-460	6	6	to	to	PART
eurjchem-460	6	7	possess	possess	VERB
eurjchem-460	6	8	zno·zncr2o4	zno·zncr2o4	PROPN
eurjchem-460	6	9	composition	composition	NOUN
eurjchem-460	6	10	.	.	PUNCT
eurjchem-460	7	1	the	the	DET
eurjchem-460	7	2	catalysts	catalyst	NOUN
eurjchem-460	7	3	have	have	AUX
eurjchem-460	7	4	been	be	AUX
eurjchem-460	7	5	tested	test	VERB
eurjchem-460	7	6	for	for	ADP
eurjchem-460	7	7	their	their	PRON
eurjchem-460	7	8	performance	performance	NOUN
eurjchem-460	7	9	for	for	ADP
eurjchem-460	7	10	the	the	DET
eurjchem-460	7	11	first	first	ADJ
eurjchem-460	7	12	time	time	NOUN
eurjchem-460	7	13	,	,	PUNCT
eurjchem-460	7	14	in	in	ADP
eurjchem-460	7	15	the	the	DET
eurjchem-460	7	16	synthesis	synthesis	NOUN
eurjchem-460	7	17	of	of	ADP
eurjchem-460	7	18	ethylene	ethylene	NOUN
eurjchem-460	7	19	carbonate	carbonate	NOUN
eurjchem-460	7	20	from	from	ADP
eurjchem-460	7	21	cyclocondensation	cyclocondensation	NOUN
eurjchem-460	7	22	of	of	ADP
eurjchem-460	7	23	ethylene	ethylene	NOUN
eurjchem-460	7	24	glycol	glycol	NOUN
eurjchem-460	7	25	and	and	CCONJ
eurjchem-460	7	26	urea	urea	NOUN
eurjchem-460	7	27	.	.	PUNCT
eurjchem-460	8	1	effect	effect	NOUN
eurjchem-460	8	2	of	of	ADP
eurjchem-460	8	3	catalyst	catalyst	NOUN
eurjchem-460	8	4	concentration	concentration	NOUN
eurjchem-460	8	5	,	,	PUNCT
eurjchem-460	8	6	temperature	temperature	NOUN
eurjchem-460	8	7	and	and	CCONJ
eurjchem-460	8	8	molar	molar	ADJ
eurjchem-460	8	9	ratio	ratio	NOUN
eurjchem-460	8	10	of	of	ADP
eurjchem-460	8	11	reactants	reactant	NOUN
eurjchem-460	8	12	has	have	AUX
eurjchem-460	8	13	been	be	AUX
eurjchem-460	8	14	studied	study	VERB
eurjchem-460	8	15	to	to	PART
eurjchem-460	8	16	obtain	obtain	VERB
eurjchem-460	8	17	the	the	DET
eurjchem-460	8	18	optimum	optimum	ADJ
eurjchem-460	8	19	conversion	conversion	NOUN
eurjchem-460	8	20	and	and	CCONJ
eurjchem-460	8	21	selectivity	selectivity	NOUN
eurjchem-460	8	22	of	of	ADP
eurjchem-460	8	23	ethylene	ethylene	NOUN
eurjchem-460	8	24	glycol	glycol	NOUN
eurjchem-460	8	25	and	and	CCONJ
eurjchem-460	8	26	urea	urea	NOUN
eurjchem-460	8	27	to	to	ADP
eurjchem-460	8	28	ethylene	ethylene	NOUN
eurjchem-460	8	29	carbonate	carbonate	NOUN
eurjchem-460	8	30	.	.	PUNCT
eurjchem-460	9	1	a	a	DET
eurjchem-460	9	2	maximum	maximum	ADJ
eurjchem-460	9	3	yield	yield	NOUN
eurjchem-460	9	4	of	of	ADP
eurjchem-460	9	5	85.75	85.75	NUM
eurjchem-460	9	6	%	%	NOUN
eurjchem-460	9	7	of	of	ADP
eurjchem-460	9	8	ethylene	ethylene	NOUN
eurjchem-460	9	9	carbonate	carbonate	NOUN
eurjchem-460	9	10	was	be	AUX
eurjchem-460	9	11	obtained	obtain	VERB
eurjchem-460	9	12	at	at	ADP
eurjchem-460	9	13	a	a	DET
eurjchem-460	9	14	temperature	temperature	NOUN
eurjchem-460	9	15	of	of	ADP
eurjchem-460	9	16	423	423	NUM
eurjchem-460	9	17	k	k	NOUN
eurjchem-460	9	18	and	and	CCONJ
eurjchem-460	9	19	urea	urea	NOUN
eurjchem-460	9	20	:	:	PUNCT
eurjchem-460	9	21	ethylene	ethylene	NOUN
eurjchem-460	9	22	glycol	glycol	NOUN
eurjchem-460	9	23	molar	molar	ADJ
eurjchem-460	9	24	ratio	ratio	NOUN
eurjchem-460	9	25	of	of	ADP
eurjchem-460	9	26	1:1.5	1:1.5	NUM
eurjchem-460	9	27	.	.	PUNCT
eurjchem-460	10	1	a	a	DET
eurjchem-460	10	2	tentative	tentative	ADJ
eurjchem-460	10	3	mechanism	mechanism	NOUN
eurjchem-460	10	4	of	of	ADP
eurjchem-460	10	5	the	the	DET
eurjchem-460	10	6	reaction	reaction	NOUN
eurjchem-460	10	7	is	be	AUX
eurjchem-460	10	8	proposed	propose	VERB
eurjchem-460	10	9	on	on	ADP
eurjchem-460	10	10	the	the	DET
eurjchem-460	10	11	basis	basis	NOUN
eurjchem-460	10	12	of	of	ADP
eurjchem-460	10	13	analysis	analysis	NOUN
eurjchem-460	10	14	of	of	ADP
eurjchem-460	10	15	reactants	reactant	NOUN
eurjchem-460	10	16	,	,	PUNCT
eurjchem-460	10	17	products	product	NOUN
eurjchem-460	10	18	and	and	CCONJ
eurjchem-460	10	19	modeling	modeling	NOUN
eurjchem-460	10	20	of	of	ADP
eurjchem-460	10	21	the	the	DET
eurjchem-460	10	22	transition	transition	NOUN
eurjchem-460	10	23	state	state	NOUN
eurjchem-460	10	24	for	for	ADP
eurjchem-460	10	25	the	the	DET
eurjchem-460	10	26	reaction	reaction	NOUN
eurjchem-460	10	27	under	under	ADP
eurjchem-460	10	28	density	density	NOUN
eurjchem-460	10	29	function	function	NOUN
eurjchem-460	10	30	theory	theory	NOUN
eurjchem-460	10	31	using	use	VERB
eurjchem-460	10	32	gaussian09w	gaussian09w	ADJ
eurjchem-460	10	33	software	software	NOUN
eurjchem-460	10	34	.	.	PUNCT
eurjchem-460	11	1	our	our	PRON
eurjchem-460	11	2	studies	study	NOUN
eurjchem-460	11	3	suggest	suggest	VERB
eurjchem-460	11	4	a	a	DET
eurjchem-460	11	5	consecutive	consecutive	ADJ
eurjchem-460	11	6	mechanism	mechanism	NOUN
eurjchem-460	11	7	for	for	ADP
eurjchem-460	11	8	the	the	DET
eurjchem-460	11	9	reaction	reaction	NOUN
eurjchem-460	11	10	.	.	PUNCT
eurjchem-460	12	1	in	in	ADP
eurjchem-460	12	2	the	the	DET
eurjchem-460	12	3	first	first	ADJ
eurjchem-460	12	4	step	step	NOUN
eurjchem-460	12	5	,	,	PUNCT
eurjchem-460	12	6	urea	urea	NOUN
eurjchem-460	12	7	and	and	CCONJ
eurjchem-460	12	8	ethylene	ethylene	NOUN
eurjchem-460	12	9	glycol	glycol	NOUN
eurjchem-460	12	10	react	react	VERB
eurjchem-460	12	11	to	to	PART
eurjchem-460	12	12	produce	produce	VERB
eurjchem-460	12	13	2‐hydroxyethyl	2‐hydroxyethyl	PROPN
eurjchem-460	12	14	carbamate	carbamate	PROPN
eurjchem-460	12	15	,	,	PUNCT
eurjchem-460	12	16	which	which	PRON
eurjchem-460	12	17	undergoes	undergo	VERB
eurjchem-460	12	18	further	further	ADJ
eurjchem-460	12	19	reaction	reaction	NOUN
eurjchem-460	12	20	to	to	PART
eurjchem-460	12	21	produce	produce	VERB
eurjchem-460	12	22	ethylene	ethylene	NOUN
eurjchem-460	12	23	carbonate	carbonate	NOUN
eurjchem-460	12	24	(	(	PUNCT
eurjchem-460	12	25	ec	ec	PROPN
eurjchem-460	12	26	)	)	PUNCT
eurjchem-460	12	27	and	and	CCONJ
eurjchem-460	12	28	ammonia	ammonia	NOUN
eurjchem-460	12	29	.	.	PUNCT
eurjchem-460	13	1	urea	urea	PROPN
eurjchem-460	13	2	zinc	zinc	NOUN
eurjchem-460	13	3	chromite	chromite	NOUN
eurjchem-460	13	4	ethylene	ethylene	NOUN
eurjchem-460	13	5	glycol	glycol	NOUN
eurjchem-460	13	6	co‐precipitation	co‐precipitation	NOUN
eurjchem-460	13	7	cyclocondensation	cyclocondensation	NOUN
eurjchem-460	13	8	ethylene	ethylene	NOUN
eurjchem-460	13	9	carbonate	carbonate	NOUN
eurjchem-460	13	10	1	1	NUM
eurjchem-460	13	11	.	.	PUNCT
eurjchem-460	14	1	introduction	introduction	NOUN
eurjchem-460	14	2	carbon	carbon	NOUN
eurjchem-460	14	3	dioxide	dioxide	NOUN
eurjchem-460	14	4	is	be	AUX
eurjchem-460	14	5	a	a	DET
eurjchem-460	14	6	greenhouse	greenhouse	NOUN
eurjchem-460	14	7	gas	gas	NOUN
eurjchem-460	14	8	and	and	CCONJ
eurjchem-460	14	9	renewable	renewable	ADJ
eurjchem-460	14	10	source	source	NOUN
eurjchem-460	14	11	of	of	ADP
eurjchem-460	14	12	carbon	carbon	NOUN
eurjchem-460	14	13	.	.	PUNCT
eurjchem-460	15	1	in	in	ADP
eurjchem-460	15	2	the	the	DET
eurjchem-460	15	3	current	current	ADJ
eurjchem-460	15	4	decade	decade	NOUN
eurjchem-460	15	5	attempts	attempt	NOUN
eurjchem-460	15	6	have	have	AUX
eurjchem-460	15	7	therefore	therefore	ADV
eurjchem-460	15	8	been	be	AUX
eurjchem-460	15	9	made	make	VERB
eurjchem-460	15	10	to	to	PART
eurjchem-460	15	11	transform	transform	VERB
eurjchem-460	15	12	it	it	PRON
eurjchem-460	15	13	into	into	ADP
eurjchem-460	15	14	valuable	valuable	ADJ
eurjchem-460	15	15	chemicals	chemical	NOUN
eurjchem-460	15	16	.	.	PUNCT
eurjchem-460	16	1	however	however	ADV
eurjchem-460	16	2	,	,	PUNCT
eurjchem-460	16	3	because	because	SCONJ
eurjchem-460	16	4	of	of	ADP
eurjchem-460	16	5	its	its	PRON
eurjchem-460	16	6	high	high	ADJ
eurjchem-460	16	7	thermodynamic	thermodynamic	ADJ
eurjchem-460	16	8	stability	stability	NOUN
eurjchem-460	16	9	,	,	PUNCT
eurjchem-460	16	10	it	it	PRON
eurjchem-460	16	11	is	be	AUX
eurjchem-460	16	12	almost	almost	ADV
eurjchem-460	16	13	inert	inert	ADJ
eurjchem-460	16	14	to	to	ADP
eurjchem-460	16	15	large	large	ADJ
eurjchem-460	16	16	variety	variety	NOUN
eurjchem-460	16	17	of	of	ADP
eurjchem-460	16	18	chemicals	chemical	NOUN
eurjchem-460	16	19	and	and	CCONJ
eurjchem-460	16	20	only	only	ADV
eurjchem-460	16	21	highly	highly	ADV
eurjchem-460	16	22	strained	strain	VERB
eurjchem-460	16	23	molecules	molecule	NOUN
eurjchem-460	16	24	can	can	AUX
eurjchem-460	16	25	react	react	VERB
eurjchem-460	16	26	with	with	ADP
eurjchem-460	16	27	it	it	PRON
eurjchem-460	16	28	under	under	ADP
eurjchem-460	16	29	elevated	elevated	ADJ
eurjchem-460	16	30	temperature	temperature	NOUN
eurjchem-460	16	31	and	and	CCONJ
eurjchem-460	16	32	pressure	pressure	NOUN
eurjchem-460	16	33	.	.	PUNCT
eurjchem-460	17	1	this	this	PRON
eurjchem-460	17	2	is	be	AUX
eurjchem-460	17	3	the	the	DET
eurjchem-460	17	4	reason	reason	NOUN
eurjchem-460	17	5	why	why	SCONJ
eurjchem-460	17	6	only	only	ADV
eurjchem-460	17	7	limited	limited	ADJ
eurjchem-460	17	8	chemical	chemical	NOUN
eurjchem-460	17	9	processes	process	NOUN
eurjchem-460	17	10	utilize	utilize	VERB
eurjchem-460	17	11	it	it	PRON
eurjchem-460	17	12	as	as	ADP
eurjchem-460	17	13	a	a	DET
eurjchem-460	17	14	raw	raw	ADJ
eurjchem-460	17	15	material	material	NOUN
eurjchem-460	17	16	.	.	PUNCT
eurjchem-460	18	1	in	in	ADP
eurjchem-460	18	2	spite	spite	NOUN
eurjchem-460	18	3	of	of	ADP
eurjchem-460	18	4	this	this	DET
eurjchem-460	18	5	drawback	drawback	NOUN
eurjchem-460	18	6	,	,	PUNCT
eurjchem-460	18	7	success	success	NOUN
eurjchem-460	18	8	has	have	AUX
eurjchem-460	18	9	been	be	AUX
eurjchem-460	18	10	obtained	obtain	VERB
eurjchem-460	18	11	to	to	PART
eurjchem-460	18	12	transform	transform	VERB
eurjchem-460	18	13	carbon	carbon	NOUN
eurjchem-460	18	14	dioxide	dioxide	NOUN
eurjchem-460	18	15	into	into	ADP
eurjchem-460	18	16	dimethyl	dimethyl	NOUN
eurjchem-460	18	17	carbonate	carbonate	NOUN
eurjchem-460	18	18	,	,	PUNCT
eurjchem-460	18	19	cyclic	cyclic	ADJ
eurjchem-460	18	20	carbonates	carbonate	NOUN
eurjchem-460	18	21	,	,	PUNCT
eurjchem-460	18	22	polycarbonates	polycarbonate	NOUN
eurjchem-460	18	23	,	,	PUNCT
eurjchem-460	18	24	urea	urea	NOUN
eurjchem-460	18	25	and	and	CCONJ
eurjchem-460	18	26	urethane	urethane	NOUN
eurjchem-460	18	27	derivatives	derivative	NOUN
eurjchem-460	18	28	,	,	PUNCT
eurjchem-460	18	29	carboxylic	carboxylic	ADJ
eurjchem-460	18	30	acids	acid	NOUN
eurjchem-460	18	31	,	,	PUNCT
eurjchem-460	18	32	esters	ester	NOUN
eurjchem-460	18	33	,	,	PUNCT
eurjchem-460	18	34	lactones	lactone	NOUN
eurjchem-460	18	35	,	,	PUNCT
eurjchem-460	18	36	isocyanates	isocyanate	NOUN
eurjchem-460	18	37	and	and	CCONJ
eurjchem-460	18	38	many	many	ADJ
eurjchem-460	18	39	more	more	ADJ
eurjchem-460	18	40	chemicals	chemical	NOUN
eurjchem-460	18	41	[	[	X
eurjchem-460	18	42	1	1	NUM
eurjchem-460	18	43	]	]	PUNCT
eurjchem-460	18	44	.	.	PUNCT
eurjchem-460	19	1	cyclic	cyclic	ADJ
eurjchem-460	19	2	carbonates	carbonate	NOUN
eurjchem-460	19	3	find	find	VERB
eurjchem-460	19	4	applications	application	NOUN
eurjchem-460	19	5	as	as	ADP
eurjchem-460	19	6	reactive	reactive	ADJ
eurjchem-460	19	7	intermediates	intermediate	NOUN
eurjchem-460	19	8	and	and	CCONJ
eurjchem-460	19	9	as	as	ADP
eurjchem-460	19	10	inert	inert	ADJ
eurjchem-460	19	11	solvent	solvent	NOUN
eurjchem-460	19	12	.	.	PUNCT
eurjchem-460	20	1	these	these	PRON
eurjchem-460	20	2	can	can	AUX
eurjchem-460	20	3	be	be	AUX
eurjchem-460	20	4	used	use	VERB
eurjchem-460	20	5	to	to	PART
eurjchem-460	20	6	prepare	prepare	VERB
eurjchem-460	20	7	monomers	monomer	NOUN
eurjchem-460	20	8	,	,	PUNCT
eurjchem-460	20	9	polymers	polymer	NOUN
eurjchem-460	20	10	,	,	PUNCT
eurjchem-460	20	11	surfactants	surfactant	NOUN
eurjchem-460	20	12	,	,	PUNCT
eurjchem-460	20	13	plasticizers	plasticizer	NOUN
eurjchem-460	20	14	,	,	PUNCT
eurjchem-460	20	15	cross	cross	VERB
eurjchem-460	20	16	linking	link	VERB
eurjchem-460	20	17	agents	agent	NOUN
eurjchem-460	20	18	and	and	CCONJ
eurjchem-460	20	19	solvents	solvent	NOUN
eurjchem-460	21	1	[	[	X
eurjchem-460	21	2	2	2	NUM
eurjchem-460	21	3	]	]	PUNCT
eurjchem-460	21	4	.	.	PUNCT
eurjchem-460	22	1	cyclic	cyclic	ADJ
eurjchem-460	22	2	carbonates	carbonate	NOUN
eurjchem-460	22	3	are	be	AUX
eurjchem-460	22	4	also	also	ADV
eurjchem-460	22	5	used	use	VERB
eurjchem-460	22	6	as	as	ADP
eurjchem-460	22	7	electrolytes	electrolyte	NOUN
eurjchem-460	22	8	in	in	ADP
eurjchem-460	22	9	the	the	DET
eurjchem-460	22	10	lithium	lithium	NOUN
eurjchem-460	22	11	ion	ion	NOUN
eurjchem-460	22	12	rechargeable	rechargeable	NOUN
eurjchem-460	22	13	batteries	battery	NOUN
eurjchem-460	22	14	[	[	X
eurjchem-460	22	15	3‐5	3‐5	NUM
eurjchem-460	22	16	]	]	X
eurjchem-460	22	17	.	.	PUNCT
eurjchem-460	23	1	an	an	DET
eurjchem-460	23	2	important	important	ADJ
eurjchem-460	23	3	field	field	NOUN
eurjchem-460	23	4	in	in	ADP
eurjchem-460	23	5	green	green	ADJ
eurjchem-460	23	6	chemistry	chemistry	NOUN
eurjchem-460	23	7	is	be	AUX
eurjchem-460	23	8	to	to	PART
eurjchem-460	23	9	find	find	VERB
eurjchem-460	23	10	solvents	solvent	NOUN
eurjchem-460	23	11	which	which	PRON
eurjchem-460	23	12	can	can	AUX
eurjchem-460	23	13	replace	replace	VERB
eurjchem-460	23	14	the	the	DET
eurjchem-460	23	15	traditional	traditional	ADJ
eurjchem-460	23	16	hazardous	hazardous	ADJ
eurjchem-460	23	17	solvents	solvent	NOUN
eurjchem-460	23	18	.	.	PUNCT
eurjchem-460	24	1	owing	owe	VERB
eurjchem-460	24	2	to	to	ADP
eurjchem-460	24	3	their	their	PRON
eurjchem-460	24	4	biodegradability	biodegradability	NOUN
eurjchem-460	24	5	and	and	CCONJ
eurjchem-460	24	6	biocompatibility	biocompatibility	NOUN
eurjchem-460	24	7	[	[	X
eurjchem-460	24	8	6,7	6,7	NUM
eurjchem-460	24	9	]	]	PUNCT
eurjchem-460	24	10	,	,	PUNCT
eurjchem-460	24	11	low	low	ADJ
eurjchem-460	24	12	odour	odour	NOUN
eurjchem-460	24	13	level	level	NOUN
eurjchem-460	24	14	,	,	PUNCT
eurjchem-460	24	15	low	low	ADJ
eurjchem-460	24	16	toxicity	toxicity	NOUN
eurjchem-460	24	17	,	,	PUNCT
eurjchem-460	24	18	high	high	ADJ
eurjchem-460	24	19	dipole	dipole	NOUN
eurjchem-460	24	20	moment	moment	NOUN
eurjchem-460	24	21	,	,	PUNCT
eurjchem-460	24	22	and	and	CCONJ
eurjchem-460	24	23	high	high	ADJ
eurjchem-460	24	24	boiling	boiling	NOUN
eurjchem-460	24	25	and	and	CCONJ
eurjchem-460	24	26	flash	flash	NOUN
eurjchem-460	24	27	point	point	NOUN
eurjchem-460	24	28	,	,	PUNCT
eurjchem-460	24	29	cyclic	cyclic	ADJ
eurjchem-460	24	30	carbonates	carbonate	NOUN
eurjchem-460	24	31	are	be	AUX
eurjchem-460	24	32	emerging	emerge	VERB
eurjchem-460	24	33	as	as	ADP
eurjchem-460	24	34	promising	promise	VERB
eurjchem-460	24	35	environmental	environmental	ADJ
eurjchem-460	24	36	benign	benign	ADJ
eurjchem-460	24	37	solvents	solvent	NOUN
eurjchem-460	24	38	for	for	ADP
eurjchem-460	24	39	future	future	NOUN
eurjchem-460	24	40	.	.	PUNCT
eurjchem-460	25	1	recently	recently	ADV
eurjchem-460	25	2	,	,	PUNCT
eurjchem-460	25	3	wang	wang	PROPN
eurjchem-460	25	4	et	et	PROPN
eurjchem-460	25	5	al	al	PROPN
eurjchem-460	25	6	.	.	PUNCT
eurjchem-460	26	1	[	[	X
eurjchem-460	26	2	8	8	NUM
eurjchem-460	26	3	]	]	PUNCT
eurjchem-460	26	4	have	have	AUX
eurjchem-460	26	5	used	use	VERB
eurjchem-460	26	6	ethylene	ethylene	NOUN
eurjchem-460	26	7	carbonate	carbonate	NOUN
eurjchem-460	26	8	as	as	ADP
eurjchem-460	26	9	a	a	DET
eurjchem-460	26	10	unique	unique	ADJ
eurjchem-460	26	11	solvent	solvent	NOUN
eurjchem-460	26	12	for	for	ADP
eurjchem-460	26	13	palladium‐catalyzed	palladium‐catalyze	VERB
eurjchem-460	26	14	wacker	wacker	NOUN
eurjchem-460	26	15	oxidation	oxidation	NOUN
eurjchem-460	26	16	using	use	VERB
eurjchem-460	26	17	oxygen	oxygen	NOUN
eurjchem-460	26	18	as	as	ADP
eurjchem-460	26	19	sole	sole	ADJ
eurjchem-460	26	20	oxidant	oxidant	NOUN
eurjchem-460	26	21	.	.	PUNCT
eurjchem-460	27	1	traditionally	traditionally	ADV
eurjchem-460	27	2	,	,	PUNCT
eurjchem-460	27	3	these	these	DET
eurjchem-460	27	4	carbonates	carbonate	NOUN
eurjchem-460	27	5	are	be	AUX
eurjchem-460	27	6	prepared	prepare	VERB
eurjchem-460	27	7	by	by	ADP
eurjchem-460	27	8	reacting	react	VERB
eurjchem-460	27	9	toxic	toxic	ADJ
eurjchem-460	27	10	phosgenation	phosgenation	NOUN
eurjchem-460	27	11	with	with	ADP
eurjchem-460	27	12	alcohols	alcohol	NOUN
eurjchem-460	27	13	at	at	ADP
eurjchem-460	27	14	about	about	ADP
eurjchem-460	27	15	room	room	NOUN
eurjchem-460	27	16	temperature	temperature	NOUN
eurjchem-460	27	17	in	in	ADP
eurjchem-460	27	18	an	an	DET
eurjchem-460	27	19	anhydrous	anhydrous	ADJ
eurjchem-460	27	20	solvent	solvent	NOUN
eurjchem-460	27	21	containing	contain	VERB
eurjchem-460	27	22	excess	excess	NOUN
eurjchem-460	27	23	of	of	ADP
eurjchem-460	27	24	pyridine	pyridine	NOUN
eurjchem-460	27	25	.	.	PUNCT
eurjchem-460	28	1	although	although	SCONJ
eurjchem-460	28	2	the	the	DET
eurjchem-460	28	3	process	process	NOUN
eurjchem-460	28	4	is	be	AUX
eurjchem-460	28	5	accompanied	accompany	VERB
eurjchem-460	28	6	with	with	ADP
eurjchem-460	28	7	very	very	ADV
eurjchem-460	28	8	high	high	ADJ
eurjchem-460	28	9	yield	yield	NOUN
eurjchem-460	28	10	of	of	ADP
eurjchem-460	28	11	carbonates	carbonate	NOUN
eurjchem-460	28	12	,	,	PUNCT
eurjchem-460	28	13	the	the	DET
eurjchem-460	28	14	main	main	ADJ
eurjchem-460	28	15	drawback	drawback	NOUN
eurjchem-460	28	16	of	of	ADP
eurjchem-460	28	17	the	the	DET
eurjchem-460	28	18	process	process	NOUN
eurjchem-460	28	19	is	be	AUX
eurjchem-460	28	20	the	the	DET
eurjchem-460	28	21	use	use	NOUN
eurjchem-460	28	22	of	of	ADP
eurjchem-460	28	23	toxic	toxic	ADJ
eurjchem-460	28	24	and	and	CCONJ
eurjchem-460	28	25	hazardous	hazardous	ADJ
eurjchem-460	28	26	chemicals	chemical	NOUN
eurjchem-460	28	27	like	like	ADP
eurjchem-460	28	28	pyridine	pyridine	NOUN
eurjchem-460	28	29	and	and	CCONJ
eurjchem-460	28	30	phosgene	phosgene	NOUN
eurjchem-460	28	31	[	[	X
eurjchem-460	28	32	9	9	NUM
eurjchem-460	28	33	]	]	PUNCT
eurjchem-460	28	34	.	.	PUNCT
eurjchem-460	29	1	reaction	reaction	NOUN
eurjchem-460	29	2	of	of	ADP
eurjchem-460	29	3	co2	co2	NOUN
eurjchem-460	29	4	with	with	ADP
eurjchem-460	29	5	epoxides	epoxide	NOUN
eurjchem-460	29	6	is	be	AUX
eurjchem-460	29	7	another	another	DET
eurjchem-460	29	8	green	green	ADJ
eurjchem-460	29	9	process	process	NOUN
eurjchem-460	29	10	for	for	ADP
eurjchem-460	29	11	synthesis	synthesis	NOUN
eurjchem-460	29	12	of	of	ADP
eurjchem-460	29	13	cyclic	cyclic	ADJ
eurjchem-460	29	14	carbonates	carbonate	NOUN
eurjchem-460	29	15	and	and	CCONJ
eurjchem-460	29	16	fixation	fixation	NOUN
eurjchem-460	29	17	of	of	ADP
eurjchem-460	29	18	carbon	carbon	NOUN
eurjchem-460	29	19	dioxide	dioxide	NOUN
eurjchem-460	29	20	[	[	X
eurjchem-460	29	21	10‐23	10‐23	NUM
eurjchem-460	29	22	]	]	PUNCT
eurjchem-460	29	23	.	.	PUNCT
eurjchem-460	30	1	drawback	drawback	NOUN
eurjchem-460	30	2	with	with	ADP
eurjchem-460	30	3	this	this	DET
eurjchem-460	30	4	process	process	NOUN
eurjchem-460	30	5	is	be	AUX
eurjchem-460	30	6	that	that	SCONJ
eurjchem-460	30	7	it	it	PRON
eurjchem-460	30	8	requires	require	VERB
eurjchem-460	30	9	high	high	ADJ
eurjchem-460	30	10	pressure	pressure	NOUN
eurjchem-460	30	11	and	and	CCONJ
eurjchem-460	30	12	uses	use	VERB
eurjchem-460	30	13	epoxide	epoxide	NOUN
eurjchem-460	30	14	as	as	ADP
eurjchem-460	30	15	the	the	DET
eurjchem-460	30	16	starting	starting	NOUN
eurjchem-460	30	17	material	material	NOUN
eurjchem-460	30	18	.	.	PUNCT
eurjchem-460	31	1	a	a	DET
eurjchem-460	31	2	better	well	ADJ
eurjchem-460	31	3	route	route	NOUN
eurjchem-460	31	4	for	for	ADP
eurjchem-460	31	5	the	the	DET
eurjchem-460	31	6	synthesis	synthesis	NOUN
eurjchem-460	31	7	of	of	ADP
eurjchem-460	31	8	cyclic	cyclic	ADJ
eurjchem-460	31	9	carbonates	carbonate	NOUN
eurjchem-460	31	10	is	be	AUX
eurjchem-460	31	11	to	to	PART
eurjchem-460	31	12	transform	transform	VERB
eurjchem-460	31	13	co2	co2	NOUN
eurjchem-460	31	14	into	into	ADP
eurjchem-460	31	15	urea	urea	NOUN
eurjchem-460	31	16	and	and	CCONJ
eurjchem-460	31	17	then	then	ADV
eurjchem-460	31	18	react	react	VERB
eurjchem-460	31	19	urea	urea	NOUN
eurjchem-460	31	20	with	with	ADP
eurjchem-460	31	21	diols	diol	NOUN
eurjchem-460	31	22	,	,	PUNCT
eurjchem-460	31	23	at	at	ADP
eurjchem-460	31	24	about	about	ADP
eurjchem-460	31	25	atmospheric	atmospheric	ADJ
eurjchem-460	31	26	pressure	pressure	NOUN
eurjchem-460	31	27	.	.	PUNCT
eurjchem-460	32	1	chromite	chromite	NOUN
eurjchem-460	32	2	spinals	spinal	NOUN
eurjchem-460	32	3	formed	form	VERB
eurjchem-460	32	4	due	due	ADP
eurjchem-460	32	5	to	to	ADP
eurjchem-460	32	6	close	close	ADJ
eurjchem-460	32	7	packing	packing	NOUN
eurjchem-460	32	8	of	of	ADP
eurjchem-460	32	9	o2‐	o2‐	NOUN
eurjchem-460	32	10	anions	anion	NOUN
eurjchem-460	32	11	have	have	VERB
eurjchem-460	32	12	the	the	DET
eurjchem-460	32	13	general	general	ADJ
eurjchem-460	32	14	formula	formula	NOUN
eurjchem-460	32	15	a2+[b23+]o4	a2+[b23+]o4	NOUN
eurjchem-460	32	16	and	and	CCONJ
eurjchem-460	32	17	posses	posse	NOUN
eurjchem-460	32	18	tetrahedral	tetrahedral	ADJ
eurjchem-460	32	19	and	and	CCONJ
eurjchem-460	32	20	octahedral	octahedral	ADJ
eurjchem-460	32	21	interstitial	interstitial	ADJ
eurjchem-460	32	22	sites	site	NOUN
eurjchem-460	32	23	filled	fill	VERB
eurjchem-460	32	24	by	by	ADP
eurjchem-460	32	25	a2	a2	PROPN
eurjchem-460	32	26	+	+	NOUN
eurjchem-460	32	27	and	and	CCONJ
eurjchem-460	32	28	b3	b3	PROPN
eurjchem-460	32	29	+	+	PART
eurjchem-460	32	30	ions	ion	NOUN
eurjchem-460	32	31	,	,	PUNCT
eurjchem-460	32	32	respectively	respectively	ADV
eurjchem-460	32	33	.	.	PUNCT
eurjchem-460	33	1	ferrite	ferrite	NOUN
eurjchem-460	33	2	,	,	PUNCT
eurjchem-460	33	3	spinals	spinal	NOUN
eurjchem-460	33	4	have	have	AUX
eurjchem-460	33	5	been	be	AUX
eurjchem-460	33	6	found	find	VERB
eurjchem-460	33	7	to	to	PART
eurjchem-460	33	8	be	be	AUX
eurjchem-460	33	9	very	very	ADV
eurjchem-460	33	10	selective	selective	ADJ
eurjchem-460	33	11	catalysts	catalyst	NOUN
eurjchem-460	33	12	for	for	ADP
eurjchem-460	33	13	alkylation	alkylation	NOUN
eurjchem-460	33	14	of	of	ADP
eurjchem-460	33	15	aromatics	aromatic	NOUN
eurjchem-460	33	16	[	[	X
eurjchem-460	33	17	24‐28	24‐28	NUM
eurjchem-460	33	18	]	]	PUNCT
eurjchem-460	33	19	.	.	PUNCT
eurjchem-460	34	1	there	there	PRON
eurjchem-460	34	2	are	be	VERB
eurjchem-460	34	3	reports	report	NOUN
eurjchem-460	34	4	on	on	ADP
eurjchem-460	34	5	the	the	DET
eurjchem-460	34	6	synthesis	synthesis	NOUN
eurjchem-460	34	7	of	of	ADP
eurjchem-460	34	8	ethylene	ethylene	NOUN
eurjchem-460	34	9	carbonate	carbonate	NOUN
eurjchem-460	34	10	(	(	PUNCT
eurjchem-460	34	11	ec	ec	PROPN
eurjchem-460	34	12	)	)	PUNCT
eurjchem-460	35	1	[	[	X
eurjchem-460	35	2	29‐36	29‐36	NOUN
eurjchem-460	35	3	]	]	X
eurjchem-460	35	4	.	.	PUNCT
eurjchem-460	36	1	many	many	ADJ
eurjchem-460	36	2	of	of	ADP
eurjchem-460	36	3	them	they	PRON
eurjchem-460	36	4	use	use	VERB
eurjchem-460	36	5	ethylene	ethylene	NOUN
eurjchem-460	36	6	oxide	oxide	NOUN
eurjchem-460	36	7	as	as	ADP
eurjchem-460	36	8	raw	raw	ADJ
eurjchem-460	36	9	material	material	NOUN
eurjchem-460	36	10	[	[	X
eurjchem-460	36	11	29‐31	29‐31	X
eurjchem-460	36	12	]	]	PUNCT
eurjchem-460	36	13	.	.	PUNCT
eurjchem-460	37	1	su	su	PROPN
eurjchem-460	37	2	et	et	PROPN
eurjchem-460	37	3	al	al	PROPN
eurjchem-460	37	4	.	.	PUNCT
eurjchem-460	38	1	[	[	X
eurjchem-460	38	2	32	32	NUM
eurjchem-460	38	3	]	]	PUNCT
eurjchem-460	38	4	described	describe	VERB
eurjchem-460	38	5	reactions	reaction	NOUN
eurjchem-460	38	6	of	of	ADP
eurjchem-460	38	7	alkylene	alkylene	ADJ
eurjchem-460	38	8	glycols	glycol	NOUN
eurjchem-460	38	9	and	and	CCONJ
eurjchem-460	38	10	urea	urea	NOUN
eurjchem-460	38	11	to	to	PART
eurjchem-460	38	12	synthesise	synthesise	VERB
eurjchem-460	38	13	alkylene	alkylene	ADJ
eurjchem-460	38	14	carbonates	carbonate	NOUN
eurjchem-460	38	15	using	use	VERB
eurjchem-460	38	16	tin	tin	NOUN
eurjchem-460	38	17	containing	contain	VERB
eurjchem-460	38	18	catalysts	catalyst	NOUN
eurjchem-460	38	19	.	.	PUNCT
eurjchem-460	39	1	masaharu	masaharu	NOUN
eurjchem-460	39	2	et	et	PROPN
eurjchem-460	39	3	al	al	PROPN
eurjchem-460	39	4	.	.	PUNCT
eurjchem-460	40	1	[	[	X
eurjchem-460	40	2	33	33	NUM
eurjchem-460	40	3	]	]	PUNCT
eurjchem-460	40	4	have	have	AUX
eurjchem-460	40	5	described	describe	VERB
eurjchem-460	40	6	a	a	DET
eurjchem-460	40	7	method	method	NOUN
eurjchem-460	40	8	for	for	ADP
eurjchem-460	40	9	synthesis	synthesis	NOUN
eurjchem-460	40	10	of	of	ADP
eurjchem-460	40	11	alkylene	alkylene	ADJ
eurjchem-460	40	12	carbonates	carbonate	NOUN
eurjchem-460	40	13	from	from	ADP
eurjchem-460	40	14	alkene	alkene	ADJ
eurjchem-460	40	15	glycols	glycol	NOUN
eurjchem-460	40	16	and	and	CCONJ
eurjchem-460	40	17	urea	urea	NOUN
eurjchem-460	40	18	under	under	ADP
eurjchem-460	40	19	reduced	reduced	ADJ
eurjchem-460	40	20	pressure	pressure	NOUN
eurjchem-460	40	21	using	use	VERB
eurjchem-460	40	22	a	a	DET
eurjchem-460	40	23	catalyst	catalyst	NOUN
eurjchem-460	40	24	containing	contain	VERB
eurjchem-460	40	25	at	at	ADV
eurjchem-460	40	26	least	least	ADV
eurjchem-460	40	27	one	one	NUM
eurjchem-460	40	28	metal	metal	NOUN
eurjchem-460	40	29	selected	select	VERB
eurjchem-460	40	30	from	from	ADP
eurjchem-460	40	31	zinc	zinc	NOUN
eurjchem-460	40	32	,	,	PUNCT
eurjchem-460	40	33	magnesium	magnesium	NOUN
eurjchem-460	40	34	,	,	PUNCT
eurjchem-460	40	35	lead	lead	NOUN
eurjchem-460	40	36	and	and	CCONJ
eurjchem-460	40	37	calcium	calcium	NOUN
eurjchem-460	40	38	;	;	PUNCT
eurjchem-460	40	39	and	and	CCONJ
eurjchem-460	40	40	reported	report	VERB
eurjchem-460	40	41	a	a	DET
eurjchem-460	40	42	yield	yield	NOUN
eurjchem-460	40	43	of	of	ADP
eurjchem-460	40	44	ec	ec	PROPN
eurjchem-460	40	45	reached	reach	VERB
eurjchem-460	40	46	92.6	92.6	NUM
eurjchem-460	40	47	%	%	NOUN
eurjchem-460	40	48	.	.	PUNCT
eurjchem-460	41	1	236	236	NUM
eurjchem-460	41	2	bhadauria	bhadauria	NOUN
eurjchem-460	41	3	et	et	NOUN
eurjchem-460	41	4	al	al	PROPN
eurjchem-460	41	5	.	.	PUNCT
eurjchem-460	41	6	/	/	SYM
eurjchem-460	41	7	european	european	PROPN
eurjchem-460	41	8	journal	journal	PROPN
eurjchem-460	41	9	of	of	ADP
eurjchem-460	41	10	chemistry	chemistry	NOUN
eurjchem-460	41	11	3	3	NUM
eurjchem-460	41	12	(	(	PUNCT
eurjchem-460	41	13	2	2	NUM
eurjchem-460	41	14	)	)	PUNCT
eurjchem-460	41	15	(	(	PUNCT
eurjchem-460	41	16	2012	2012	NUM
eurjchem-460	41	17	)	)	PUNCT
eurjchem-460	41	18	235‐240	235‐240	NUM
eurjchem-460	41	19	table	table	NOUN
eurjchem-460	41	20	1	1	NUM
eurjchem-460	41	21	.	.	PUNCT
eurjchem-460	41	22	effect	effect	NOUN
eurjchem-460	41	23	of	of	ADP
eurjchem-460	41	24	precursor	precursor	NOUN
eurjchem-460	41	25	on	on	ADP
eurjchem-460	41	26	catalytic	catalytic	ADJ
eurjchem-460	41	27	composition	composition	NOUN
eurjchem-460	41	28	of	of	ADP
eurjchem-460	41	29	zinc	zinc	NOUN
eurjchem-460	41	30	/	/	SYM
eurjchem-460	41	31	chromium	chromium	NOUN
eurjchem-460	41	32	oxide	oxide	NOUN
eurjchem-460	41	33	.	.	PUNCT
eurjchem-460	42	1	catalyst	catalyst	NOUN
eurjchem-460	42	2	precursors	precursor	NOUN
eurjchem-460	42	3	precursor	precursor	NOUN
eurjchem-460	42	4	(	(	PUNCT
eurjchem-460	42	5	mol	mol	ADP
eurjchem-460	42	6	ratio	ratio	NOUN
eurjchem-460	42	7	)	)	PUNCT
eurjchem-460	42	8	expected	expect	VERB
eurjchem-460	42	9	catalyst	catalyst	NOUN
eurjchem-460	42	10	composition	composition	NOUN
eurjchem-460	42	11	zn	zn	PROPN
eurjchem-460	42	12	cr	cr	PROPN
eurjchem-460	42	13	zc‐1	zc‐1	PROPN
eurjchem-460	42	14	zn(no3)2·6h2o	zn(no3)2·6h2o	X
eurjchem-460	42	15	cl3cr·6h2o	cl3cr·6h2o	VERB
eurjchem-460	42	16	9:1	9:1	NUM
eurjchem-460	42	17	8.5	8.5	NUM
eurjchem-460	42	18	zno	zno	X
eurjchem-460	42	19	·	·	SYM
eurjchem-460	42	20	0.5	0.5	NUM
eurjchem-460	42	21	zncr2o4	zncr2o4	PROPN
eurjchem-460	42	22	zc‐2	zc‐2	PROPN
eurjchem-460	42	23	zn(no3)2·6h2o	zn(no3)2·6h2o	PROPN
eurjchem-460	42	24	cl3cr·6h2o	cl3cr·6h2o	VERB
eurjchem-460	42	25	7:3	7:3	NUM
eurjchem-460	42	26	5.5	5.5	NUM
eurjchem-460	42	27	zno	zno	X
eurjchem-460	42	28	·	·	SYM
eurjchem-460	42	29	1.5	1.5	NUM
eurjchem-460	42	30	zncr2o4	zncr2o4	NOUN
eurjchem-460	42	31	zc‐3	zc‐3	DET
eurjchem-460	42	32	zn(no3)2·6h2o	zn(no3)2·6h2o	NUM
eurjchem-460	42	33	cl3cr·6h2o	cl3cr·6h2o	VERB
eurjchem-460	42	34	5:5	5:5	NUM
eurjchem-460	42	35	2.5	2.5	NUM
eurjchem-460	42	36	zno	zno	X
eurjchem-460	42	37	·	·	SYM
eurjchem-460	42	38	2.5	2.5	NUM
eurjchem-460	42	39	zncr2o4	zncr2o4	NUM
eurjchem-460	42	40	zc‐4	zc‐4	PROPN
eurjchem-460	42	41	zn(no3)2·6h2o	zn(no3)2·6h2o	NUM
eurjchem-460	42	42	cl3cr·6h2o	cl3cr·6h2o	VERB
eurjchem-460	42	43	3:7	3:7	NUM
eurjchem-460	42	44	3.5	3.5	NUM
eurjchem-460	42	45	zncr2o4·0.5cr2o3	zncr2o4·0.5cr2o3	PROPN
eurjchem-460	42	46	zc‐5	zc‐5	NOUN
eurjchem-460	42	47	zn(no3)2·6h2o	zn(no3)2·6h2o	NOUN
eurjchem-460	42	48	cl3cr·6h2o	cl3cr·6h2o	VERB
eurjchem-460	42	49	1:2	1:2	NUM
eurjchem-460	42	50	zncr2o4	zncr2o4	NUM
eurjchem-460	42	51	table	table	NOUN
eurjchem-460	42	52	2	2	NUM
eurjchem-460	42	53	.	.	PUNCT
eurjchem-460	42	54	acidity	acidity	NOUN
eurjchem-460	42	55	,	,	PUNCT
eurjchem-460	42	56	mean	mean	ADJ
eurjchem-460	42	57	crystallite	crystallite	NOUN
eurjchem-460	42	58	size	size	NOUN
eurjchem-460	42	59	,	,	PUNCT
eurjchem-460	42	60	surface	surface	NOUN
eurjchem-460	42	61	area	area	NOUN
eurjchem-460	42	62	and	and	CCONJ
eurjchem-460	42	63	catalytic	catalytic	ADJ
eurjchem-460	42	64	activity	activity	NOUN
eurjchem-460	42	65	of	of	ADP
eurjchem-460	42	66	zno·cr2o3	zno·cr2o3	PROPN
eurjchem-460	42	67	.	.	PROPN
eurjchem-460	42	68	catalyst	catalyst	NOUN
eurjchem-460	42	69	acidity	acidity	NOUN
eurjchem-460	42	70	(	(	PUNCT
eurjchem-460	42	71	nh3	nh3	X
eurjchem-460	42	72	uptake	uptake	ADJ
eurjchem-460	42	73	mmol	mmol	NOUN
eurjchem-460	42	74	/	/	SYM
eurjchem-460	42	75	g	g	NOUN
eurjchem-460	42	76	)	)	PUNCT
eurjchem-460	42	77	total	total	ADJ
eurjchem-460	42	78	acidity	acidity	NOUN
eurjchem-460	42	79	mean	mean	NOUN
eurjchem-460	42	80	crystallite	crystallite	NOUN
eurjchem-460	42	81	size	size	NOUN
eurjchem-460	42	82	(	(	PUNCT
eurjchem-460	42	83	nm	nm	NOUN
eurjchem-460	42	84	)	)	PUNCT
eurjchem-460	42	85	surface	surface	NOUN
eurjchem-460	42	86	area	area	NOUN
eurjchem-460	42	87	(	(	PUNCT
eurjchem-460	42	88	m2	m2	PROPN
eurjchem-460	42	89	/	/	SYM
eurjchem-460	42	90	g	g	PROPN
eurjchem-460	42	91	)	)	PUNCT
eurjchem-460	42	92	catalytic	catalytic	ADJ
eurjchem-460	42	93	activity	activity	NOUN
eurjchem-460	42	94	473‐573	473‐573	NUM
eurjchem-460	43	1	k	k	NOUN
eurjchem-460	43	2	573‐673	573‐673	PROPN
eurjchem-460	43	3	k	k	PROPN
eurjchem-460	44	1	673‐773	673‐773	PROPN
eurjchem-460	44	2	k	k	PROPN
eurjchem-460	44	3	ec	ec	PROPN
eurjchem-460	44	4	yield	yield	NOUN
eurjchem-460	44	5	(	(	PUNCT
eurjchem-460	44	6	%	%	INTJ
eurjchem-460	44	7	)	)	PUNCT
eurjchem-460	44	8	zc‐1	zc‐1	PROPN
eurjchem-460	45	1	0.3	0.3	NUM
eurjchem-460	45	2	0.2	0.2	NUM
eurjchem-460	45	3	0.1	0.1	NUM
eurjchem-460	45	4	0.6	0.6	NUM
eurjchem-460	45	5	31.34	31.34	NUM
eurjchem-460	45	6	20.89	20.89	NUM
eurjchem-460	45	7	59.90	59.90	NUM
eurjchem-460	45	8	zc‐2	zc‐2	NUM
eurjchem-460	45	9	0.5	0.5	NUM
eurjchem-460	45	10	0.3	0.3	NUM
eurjchem-460	45	11	0.2	0.2	NUM
eurjchem-460	45	12	1.0	1.0	NUM
eurjchem-460	45	13	7.49	7.49	NUM
eurjchem-460	45	14	58.64	58.64	NUM
eurjchem-460	45	15	56.00	56.00	NUM
eurjchem-460	45	16	zc‐3	zc‐3	NOUN
eurjchem-460	45	17	0.4	0.4	NUM
eurjchem-460	45	18	0.2	0.2	NUM
eurjchem-460	45	19	0.3	0.3	NUM
eurjchem-460	45	20	0.9	0.9	NUM
eurjchem-460	45	21	4.87	4.87	NUM
eurjchem-460	45	22	66.30	66.30	NUM
eurjchem-460	45	23	40.50	40.50	NUM
eurjchem-460	45	24	zc‐4	zc‐4	NUM
eurjchem-460	45	25	0.4	0.4	NUM
eurjchem-460	45	26	0.2	0.2	NUM
eurjchem-460	45	27	0.2	0.2	NUM
eurjchem-460	45	28	0.8	0.8	NUM
eurjchem-460	45	29	4.08	4.08	NUM
eurjchem-460	45	30	157.67	157.67	NUM
eurjchem-460	45	31	34.54	34.54	NUM
eurjchem-460	45	32	zc‐5	zc‐5	NOUN
eurjchem-460	45	33	0.4	0.4	NUM
eurjchem-460	45	34	0.3	0.3	NUM
eurjchem-460	45	35	0.1	0.1	NUM
eurjchem-460	45	36	0.8	0.8	NUM
eurjchem-460	45	37	4.89	4.89	NUM
eurjchem-460	45	38	148.32	148.32	NUM
eurjchem-460	45	39	31.88	31.88	NUM
eurjchem-460	45	40	zno	zno	NOUN
eurjchem-460	45	41	56.00	56.00	NUM
eurjchem-460	45	42	82.35	82.35	NUM
eurjchem-460	45	43	reaction	reaction	NOUN
eurjchem-460	45	44	conditions	condition	NOUN
eurjchem-460	45	45	:	:	PUNCT
eurjchem-460	45	46	temperature	temperature	NOUN
eurjchem-460	45	47	:	:	PUNCT
eurjchem-460	45	48	423	423	NUM
eurjchem-460	45	49	k	k	NOUN
eurjchem-460	45	50	;	;	PUNCT
eurjchem-460	45	51	catalyst	catalyst	NOUN
eurjchem-460	45	52	concentration	concentration	NOUN
eurjchem-460	45	53	:	:	PUNCT
eurjchem-460	45	54	2	2	NUM
eurjchem-460	45	55	wt	wt	NOUN
eurjchem-460	45	56	.	.	NOUN
eurjchem-460	45	57	%	%	NOUN
eurjchem-460	45	58	;	;	PUNCT
eurjchem-460	45	59	ethylene	ethylene	NOUN
eurjchem-460	45	60	glycol	glycol	NOUN
eurjchem-460	45	61	/	/	SYM
eurjchem-460	45	62	urea	urea	NOUN
eurjchem-460	45	63	mole	mole	NOUN
eurjchem-460	45	64	ratio	ratio	NOUN
eurjchem-460	45	65	:	:	PUNCT
eurjchem-460	45	66	1.5	1.5	NUM
eurjchem-460	45	67	;	;	PUNCT
eurjchem-460	45	68	duration	duration	NOUN
eurjchem-460	45	69	of	of	ADP
eurjchem-460	45	70	the	the	DET
eurjchem-460	45	71	reaction	reaction	NOUN
eurjchem-460	45	72	:	:	PUNCT
eurjchem-460	45	73	2	2	NUM
eurjchem-460	45	74	h.	h.	NOUN
eurjchem-460	45	75	figure	figure	NOUN
eurjchem-460	45	76	1	1	NUM
eurjchem-460	45	77	.	.	PUNCT
eurjchem-460	45	78	experimental	experimental	ADJ
eurjchem-460	45	79	setup	setup	NOUN
eurjchem-460	45	80	for	for	ADP
eurjchem-460	45	81	lab	lab	NOUN
eurjchem-460	45	82	.	.	PUNCT
eurjchem-460	46	1	scale	scale	NOUN
eurjchem-460	46	2	syntheses	synthesis	NOUN
eurjchem-460	46	3	of	of	ADP
eurjchem-460	46	4	ec	ec	PROPN
eurjchem-460	46	5	.	.	PUNCT
eurjchem-460	47	1	1	1	X
eurjchem-460	47	2	.	.	X
eurjchem-460	47	3	heater	heater	NOUN
eurjchem-460	47	4	;	;	PUNCT
eurjchem-460	48	1	2	2	X
eurjchem-460	48	2	.	.	X
eurjchem-460	48	3	reactor	reactor	NOUN
eurjchem-460	48	4	;	;	PUNCT
eurjchem-460	48	5	3	3	X
eurjchem-460	48	6	.	.	X
eurjchem-460	48	7	condenser	condenser	NOUN
eurjchem-460	48	8	;	;	PUNCT
eurjchem-460	48	9	4	4	X
eurjchem-460	48	10	.	.	X
eurjchem-460	48	11	hcl	hcl	PROPN
eurjchem-460	48	12	trap	trap	NOUN
eurjchem-460	48	13	;	;	PUNCT
eurjchem-460	48	14	5	5	X
eurjchem-460	48	15	.	.	X
eurjchem-460	48	16	calcium	calcium	NOUN
eurjchem-460	48	17	chloride	chloride	NOUN
eurjchem-460	48	18	tower	tower	NOUN
eurjchem-460	48	19	;	;	PUNCT
eurjchem-460	48	20	6	6	X
eurjchem-460	48	21	.	.	X
eurjchem-460	48	22	ice	ice	NOUN
eurjchem-460	48	23	cooled	cool	VERB
eurjchem-460	48	24	empty	empty	ADJ
eurjchem-460	48	25	trap	trap	NOUN
eurjchem-460	48	26	.	.	PUNCT
eurjchem-460	49	1	li	li	PROPN
eurjchem-460	49	2	et	et	PROPN
eurjchem-460	49	3	al	al	PROPN
eurjchem-460	49	4	.	.	PUNCT
eurjchem-460	50	1	[	[	X
eurjchem-460	50	2	34	34	NUM
eurjchem-460	50	3	]	]	PUNCT
eurjchem-460	50	4	found	find	VERB
eurjchem-460	50	5	that	that	SCONJ
eurjchem-460	50	6	metal	metal	NOUN
eurjchem-460	50	7	oxide	oxide	NOUN
eurjchem-460	50	8	catalysts	catalyst	NOUN
eurjchem-460	50	9	with	with	ADP
eurjchem-460	50	10	appropriate	appropriate	ADJ
eurjchem-460	50	11	acidity	acidity	NOUN
eurjchem-460	50	12	and	and	CCONJ
eurjchem-460	50	13	basicity	basicity	NOUN
eurjchem-460	50	14	were	be	AUX
eurjchem-460	50	15	favourable	favourable	ADJ
eurjchem-460	50	16	for	for	ADP
eurjchem-460	50	17	the	the	DET
eurjchem-460	50	18	synthesis	synthesis	NOUN
eurjchem-460	50	19	of	of	ADP
eurjchem-460	50	20	cyclic	cyclic	ADJ
eurjchem-460	50	21	carbonate	carbonate	NOUN
eurjchem-460	50	22	.	.	PUNCT
eurjchem-460	51	1	zhao	zhao	PROPN
eurjchem-460	51	2	et	et	PROPN
eurjchem-460	51	3	al	al	PROPN
eurjchem-460	51	4	.	.	PUNCT
eurjchem-460	52	1	[	[	X
eurjchem-460	52	2	35	35	NUM
eurjchem-460	52	3	]	]	PUNCT
eurjchem-460	52	4	and	and	CCONJ
eurjchem-460	52	5	jia	jia	PROPN
eurjchem-460	52	6	et	et	PROPN
eurjchem-460	52	7	al	al	PROPN
eurjchem-460	52	8	.	.	PUNCT
eurjchem-460	53	1	[	[	X
eurjchem-460	53	2	36	36	NUM
eurjchem-460	53	3	]	]	X
eurjchem-460	53	4	prepared	prepare	VERB
eurjchem-460	53	5	zinc	zinc	NOUN
eurjchem-460	53	6	/	/	SYM
eurjchem-460	53	7	iron	iron	NOUN
eurjchem-460	53	8	oxide	oxide	NOUN
eurjchem-460	53	9	and	and	CCONJ
eurjchem-460	53	10	silica	silica	NOUN
eurjchem-460	53	11	supported	support	VERB
eurjchem-460	53	12	lead	lead	NOUN
eurjchem-460	53	13	catalysts	catalyst	NOUN
eurjchem-460	53	14	respectively	respectively	ADV
eurjchem-460	53	15	for	for	ADP
eurjchem-460	53	16	the	the	DET
eurjchem-460	53	17	synthesis	synthesis	NOUN
eurjchem-460	53	18	of	of	ADP
eurjchem-460	53	19	propylene	propylene	NOUN
eurjchem-460	53	20	carbonate	carbonate	NOUN
eurjchem-460	53	21	via	via	ADP
eurjchem-460	53	22	1	1	NUM
eurjchem-460	53	23	,	,	PUNCT
eurjchem-460	53	24	2‐	2‐	NUM
eurjchem-460	53	25	propylene	propylene	NOUN
eurjchem-460	53	26	glycol	glycol	NOUN
eurjchem-460	53	27	and	and	CCONJ
eurjchem-460	53	28	urea	urea	NOUN
eurjchem-460	53	29	.	.	PUNCT
eurjchem-460	54	1	there	there	PRON
eurjchem-460	54	2	is	be	VERB
eurjchem-460	54	3	one	one	NUM
eurjchem-460	54	4	cursory	cursory	NOUN
eurjchem-460	54	5	study	study	NOUN
eurjchem-460	54	6	on	on	ADP
eurjchem-460	54	7	the	the	DET
eurjchem-460	54	8	synthesis	synthesis	NOUN
eurjchem-460	54	9	of	of	ADP
eurjchem-460	54	10	ethylene	ethylene	NOUN
eurjchem-460	54	11	carbonate	carbonate	NOUN
eurjchem-460	54	12	from	from	ADP
eurjchem-460	54	13	ethylene	ethylene	NOUN
eurjchem-460	54	14	glycol	glycol	NOUN
eurjchem-460	54	15	and	and	CCONJ
eurjchem-460	54	16	urea	urea	NOUN
eurjchem-460	54	17	over	over	ADP
eurjchem-460	54	18	zno·fe2o3	zno·fe2o3	NOUN
eurjchem-460	54	19	catalyst	catalyst	NOUN
eurjchem-460	54	20	[	[	X
eurjchem-460	54	21	37	37	NUM
eurjchem-460	54	22	]	]	PUNCT
eurjchem-460	54	23	,	,	PUNCT
eurjchem-460	54	24	to	to	ADP
eurjchem-460	54	25	the	the	DET
eurjchem-460	54	26	best	good	ADJ
eurjchem-460	54	27	of	of	ADP
eurjchem-460	54	28	our	our	PRON
eurjchem-460	54	29	knowledge	knowledge	NOUN
eurjchem-460	54	30	there	there	PRON
eurjchem-460	54	31	seems	seem	VERB
eurjchem-460	54	32	to	to	PART
eurjchem-460	54	33	be	be	AUX
eurjchem-460	54	34	no	no	DET
eurjchem-460	54	35	report	report	NOUN
eurjchem-460	54	36	on	on	ADP
eurjchem-460	54	37	the	the	DET
eurjchem-460	54	38	synthesis	synthesis	NOUN
eurjchem-460	54	39	of	of	ADP
eurjchem-460	54	40	ethylene	ethylene	NOUN
eurjchem-460	54	41	carbonate	carbonate	NOUN
eurjchem-460	54	42	from	from	ADP
eurjchem-460	54	43	ethylene	ethylene	NOUN
eurjchem-460	54	44	glycol	glycol	NOUN
eurjchem-460	54	45	(	(	PUNCT
eurjchem-460	54	46	eg	eg	NOUN
eurjchem-460	54	47	)	)	PUNCT
eurjchem-460	54	48	and	and	CCONJ
eurjchem-460	54	49	urea	urea	NOUN
eurjchem-460	54	50	using	use	VERB
eurjchem-460	54	51	zno·cr2o3	zno·cr2o3	PROPN
eurjchem-460	54	52	as	as	ADP
eurjchem-460	54	53	a	a	DET
eurjchem-460	54	54	catalyst	catalyst	NOUN
eurjchem-460	54	55	system	system	NOUN
eurjchem-460	54	56	.	.	PUNCT
eurjchem-460	55	1	2	2	X
eurjchem-460	55	2	.	.	X
eurjchem-460	55	3	experimental	experimental	ADJ
eurjchem-460	55	4	2.1	2.1	NUM
eurjchem-460	55	5	.	.	PUNCT
eurjchem-460	55	6	catalyst	catalyst	NOUN
eurjchem-460	55	7	preparation	preparation	NOUN
eurjchem-460	55	8	zn(no3)2·6h2o	zn(no3)2·6h2o	NOUN
eurjchem-460	55	9	and	and	CCONJ
eurjchem-460	55	10	cl3cr·6h2o	cl3cr·6h2o	NOUN
eurjchem-460	55	11	are	be	AUX
eurjchem-460	55	12	taken	take	VERB
eurjchem-460	55	13	in	in	ADP
eurjchem-460	55	14	according	accord	VERB
eurjchem-460	55	15	to	to	ADP
eurjchem-460	55	16	table	table	NOUN
eurjchem-460	55	17	1	1	NUM
eurjchem-460	55	18	and	and	CCONJ
eurjchem-460	55	19	metal	metal	NOUN
eurjchem-460	55	20	salts	salt	NOUN
eurjchem-460	55	21	were	be	AUX
eurjchem-460	55	22	dissolved	dissolve	VERB
eurjchem-460	55	23	in	in	ADP
eurjchem-460	55	24	excess	excess	NOUN
eurjchem-460	55	25	of	of	ADP
eurjchem-460	55	26	distilled	distil	VERB
eurjchem-460	55	27	water	water	NOUN
eurjchem-460	55	28	(	(	PUNCT
eurjchem-460	55	29	salt	salt	NOUN
eurjchem-460	55	30	:	:	PUNCT
eurjchem-460	56	1	water	water	NOUN
eurjchem-460	56	2	wt	wt	PROPN
eurjchem-460	56	3	.	.	PUNCT
eurjchem-460	56	4	ratio	ratio	NOUN
eurjchem-460	56	5	was	be	AUX
eurjchem-460	56	6	kept	keep	VERB
eurjchem-460	56	7	nearly	nearly	ADV
eurjchem-460	56	8	1:300	1:300	NUM
eurjchem-460	56	9	)	)	PUNCT
eurjchem-460	56	10	and	and	CCONJ
eurjchem-460	56	11	a	a	DET
eurjchem-460	56	12	dilute	dilute	NOUN
eurjchem-460	56	13	solution	solution	NOUN
eurjchem-460	56	14	of	of	ADP
eurjchem-460	56	15	naoh	naoh	NOUN
eurjchem-460	56	16	was	be	AUX
eurjchem-460	56	17	added	add	VERB
eurjchem-460	56	18	with	with	ADP
eurjchem-460	56	19	constant	constant	ADJ
eurjchem-460	56	20	stirring	stirring	NOUN
eurjchem-460	56	21	until	until	SCONJ
eurjchem-460	56	22	the	the	DET
eurjchem-460	56	23	ph	ph	NOUN
eurjchem-460	56	24	of	of	ADP
eurjchem-460	56	25	the	the	DET
eurjchem-460	56	26	solution	solution	NOUN
eurjchem-460	56	27	was	be	AUX
eurjchem-460	56	28	8.5	8.5	NUM
eurjchem-460	56	29	.	.	PUNCT
eurjchem-460	57	1	the	the	DET
eurjchem-460	57	2	precipitate	precipitate	NOUN
eurjchem-460	57	3	was	be	AUX
eurjchem-460	57	4	further	far	ADV
eurjchem-460	57	5	digested	digest	VERB
eurjchem-460	57	6	at	at	ADP
eurjchem-460	57	7	353	353	NUM
eurjchem-460	57	8	k	k	NOUN
eurjchem-460	57	9	for	for	ADP
eurjchem-460	57	10	2	2	NUM
eurjchem-460	57	11	h.	h.	NOUN
eurjchem-460	57	12	and	and	CCONJ
eurjchem-460	57	13	repeatedly	repeatedly	ADV
eurjchem-460	57	14	washed	wash	VERB
eurjchem-460	57	15	with	with	ADP
eurjchem-460	57	16	distilled	distil	VERB
eurjchem-460	57	17	water	water	NOUN
eurjchem-460	57	18	until	until	ADP
eurjchem-460	57	19	free	free	ADJ
eurjchem-460	57	20	from	from	ADP
eurjchem-460	57	21	chloride	chloride	NOUN
eurjchem-460	57	22	and	and	CCONJ
eurjchem-460	57	23	nitrate	nitrate	NOUN
eurjchem-460	57	24	ions	ion	NOUN
eurjchem-460	57	25	.	.	PUNCT
eurjchem-460	58	1	finally	finally	ADV
eurjchem-460	58	2	the	the	DET
eurjchem-460	58	3	precipitate	precipitate	NOUN
eurjchem-460	58	4	was	be	AUX
eurjchem-460	58	5	oven	oven	VERB
eurjchem-460	58	6	dried	dry	VERB
eurjchem-460	58	7	and	and	CCONJ
eurjchem-460	58	8	calcined	calcine	VERB
eurjchem-460	58	9	at	at	ADP
eurjchem-460	58	10	723	723	NUM
eurjchem-460	58	11	k.	k.	NOUN
eurjchem-460	58	12	2.2	2.2	NUM
eurjchem-460	58	13	.	.	PUNCT
eurjchem-460	59	1	characterization	characterization	NOUN
eurjchem-460	59	2	of	of	ADP
eurjchem-460	59	3	the	the	DET
eurjchem-460	59	4	catalyst	catalyst	NOUN
eurjchem-460	59	5	the	the	DET
eurjchem-460	59	6	x‐ray	x‐ray	PROPN
eurjchem-460	59	7	diffraction	diffraction	PROPN
eurjchem-460	59	8	(	(	PUNCT
eurjchem-460	59	9	xrd	xrd	NOUN
eurjchem-460	59	10	)	)	PUNCT
eurjchem-460	59	11	measurements	measurement	NOUN
eurjchem-460	59	12	were	be	AUX
eurjchem-460	59	13	performed	perform	VERB
eurjchem-460	59	14	using	use	VERB
eurjchem-460	59	15	a	a	DET
eurjchem-460	59	16	rigaku	rigaku	NOUN
eurjchem-460	59	17	x‐ray	x‐ray	ADJ
eurjchem-460	59	18	powder	powder	NOUN
eurjchem-460	59	19	diffractometer	diffractometer	NOUN
eurjchem-460	59	20	equipped	equip	VERB
eurjchem-460	59	21	with	with	ADP
eurjchem-460	59	22	a	a	DET
eurjchem-460	59	23	graphite‐crystal	graphite‐crystal	ADJ
eurjchem-460	59	24	monochromator	monochromator	NOUN
eurjchem-460	59	25	(	(	PUNCT
eurjchem-460	59	26	for	for	ADP
eurjchem-460	59	27	the	the	DET
eurjchem-460	59	28	diffracted	diffract	VERB
eurjchem-460	59	29	beam	beam	NOUN
eurjchem-460	59	30	)	)	PUNCT
eurjchem-460	59	31	and	and	CCONJ
eurjchem-460	59	32	a	a	DET
eurjchem-460	59	33	scintillation	scintillation	NOUN
eurjchem-460	59	34	counter	counter	NOUN
eurjchem-460	59	35	:	:	PUNCT
eurjchem-460	59	36	cukα	cukα	ADJ
eurjchem-460	59	37	radiation	radiation	NOUN
eurjchem-460	59	38	with	with	ADP
eurjchem-460	59	39	wavelength	wavelength	NOUN
eurjchem-460	59	40	1.5406	1.5406	NUM
eurjchem-460	59	41	å	å	NOUN
eurjchem-460	59	42	was	be	AUX
eurjchem-460	59	43	used	use	VERB
eurjchem-460	59	44	in	in	ADP
eurjchem-460	59	45	the	the	DET
eurjchem-460	59	46	2θ	2θ	NUM
eurjchem-460	59	47	range	range	NOUN
eurjchem-460	60	1	10‐95	10‐95	NUM
eurjchem-460	60	2	å	å	X
eurjchem-460	60	3	.	.	PUNCT
eurjchem-460	61	1	the	the	DET
eurjchem-460	61	2	mean	mean	ADJ
eurjchem-460	61	3	crystallite	crystallite	NOUN
eurjchem-460	61	4	size	size	NOUN
eurjchem-460	61	5	was	be	AUX
eurjchem-460	61	6	determined	determine	VERB
eurjchem-460	61	7	by	by	ADP
eurjchem-460	61	8	measuring	measure	VERB
eurjchem-460	61	9	the	the	DET
eurjchem-460	61	10	broadening	broadening	NOUN
eurjchem-460	61	11	of	of	ADP
eurjchem-460	61	12	the	the	DET
eurjchem-460	61	13	peak	peak	NOUN
eurjchem-460	61	14	and	and	CCONJ
eurjchem-460	61	15	applying	apply	VERB
eurjchem-460	61	16	the	the	DET
eurjchem-460	61	17	debye	debye	ADJ
eurjchem-460	61	18	scherrer	scherrer	ADJ
eurjchem-460	61	19	equation	equation	NOUN
eurjchem-460	61	20	[	[	X
eurjchem-460	61	21	38	38	NUM
eurjchem-460	61	22	]	]	PUNCT
eurjchem-460	61	23	.	.	PUNCT
eurjchem-460	62	1	the	the	DET
eurjchem-460	62	2	surface	surface	NOUN
eurjchem-460	62	3	morphology	morphology	NOUN
eurjchem-460	62	4	of	of	ADP
eurjchem-460	62	5	the	the	DET
eurjchem-460	62	6	catalyst	catalyst	NOUN
eurjchem-460	62	7	was	be	AUX
eurjchem-460	62	8	observed	observe	VERB
eurjchem-460	62	9	with	with	ADP
eurjchem-460	62	10	a	a	DET
eurjchem-460	62	11	jeol	jeol	PROPN
eurjchem-460	62	12	jsm‐5600	jsm‐5600	PROPN
eurjchem-460	62	13	scanning	scan	VERB
eurjchem-460	62	14	electron	electron	NOUN
eurjchem-460	62	15	microscopy	microscopy	NOUN
eurjchem-460	62	16	system	system	NOUN
eurjchem-460	62	17	equipped	equip	VERB
eurjchem-460	62	18	with	with	ADP
eurjchem-460	62	19	an	an	DET
eurjchem-460	62	20	energy‐dispersive	energy‐dispersive	ADJ
eurjchem-460	62	21	x‐ray	x‐ray	ADJ
eurjchem-460	62	22	analysis	analysis	NOUN
eurjchem-460	62	23	(	(	PUNCT
eurjchem-460	62	24	sem‐edx	sem‐edx	NOUN
eurjchem-460	62	25	)	)	PUNCT
eurjchem-460	62	26	.	.	PUNCT
eurjchem-460	63	1	the	the	DET
eurjchem-460	63	2	samples	sample	NOUN
eurjchem-460	63	3	were	be	AUX
eurjchem-460	63	4	prepared	prepare	VERB
eurjchem-460	63	5	by	by	ADP
eurjchem-460	63	6	evaporating	evaporate	VERB
eurjchem-460	63	7	a	a	DET
eurjchem-460	63	8	drop	drop	NOUN
eurjchem-460	63	9	of	of	ADP
eurjchem-460	63	10	the	the	DET
eurjchem-460	63	11	sample	sample	NOUN
eurjchem-460	63	12	on	on	ADP
eurjchem-460	63	13	a	a	DET
eurjchem-460	63	14	carbon‐coated	carbon‐coate	VERB
eurjchem-460	63	15	copper	copper	NOUN
eurjchem-460	63	16	grid	grid	NOUN
eurjchem-460	63	17	.	.	PUNCT
eurjchem-460	64	1	all	all	DET
eurjchem-460	64	2	images	image	NOUN
eurjchem-460	64	3	were	be	AUX
eurjchem-460	64	4	obtained	obtain	VERB
eurjchem-460	64	5	in	in	ADP
eurjchem-460	64	6	the	the	DET
eurjchem-460	64	7	sem	sem	PROPN
eurjchem-460	64	8	mode	mode	NOUN
eurjchem-460	64	9	with	with	ADP
eurjchem-460	64	10	the	the	DET
eurjchem-460	64	11	emission	emission	NOUN
eurjchem-460	64	12	gun	gun	NOUN
eurjchem-460	64	13	operated	operate	VERB
eurjchem-460	64	14	at	at	ADP
eurjchem-460	64	15	an	an	DET
eurjchem-460	64	16	acceleration	acceleration	NOUN
eurjchem-460	64	17	voltage	voltage	NOUN
eurjchem-460	64	18	of	of	ADP
eurjchem-460	64	19	20	20	NUM
eurjchem-460	64	20	kv	kv	PROPN
eurjchem-460	64	21	.	.	PUNCT
eurjchem-460	65	1	bet	bet	PROPN
eurjchem-460	65	2	surface	surface	PROPN
eurjchem-460	65	3	area	area	NOUN
eurjchem-460	65	4	measurements	measurement	NOUN
eurjchem-460	65	5	were	be	AUX
eurjchem-460	65	6	made	make	VERB
eurjchem-460	65	7	using	use	VERB
eurjchem-460	65	8	a	a	DET
eurjchem-460	65	9	single	single	ADJ
eurjchem-460	65	10	point	point	NOUN
eurjchem-460	65	11	bet	bet	VERB
eurjchem-460	65	12	dynamic	dynamic	ADJ
eurjchem-460	65	13	method	method	NOUN
eurjchem-460	65	14	employing	employ	VERB
eurjchem-460	65	15	a	a	DET
eurjchem-460	65	16	smart	smart	ADJ
eurjchem-460	65	17	sorb	sorb	NOUN
eurjchem-460	65	18	93	93	NUM
eurjchem-460	65	19	instrument	instrument	NOUN
eurjchem-460	65	20	supplied	supply	VERB
eurjchem-460	65	21	by	by	ADP
eurjchem-460	65	22	smart	smart	ADJ
eurjchem-460	65	23	instrument	instrument	PROPN
eurjchem-460	65	24	co.	co.	PROPN
eurjchem-460	65	25	,	,	PUNCT
eurjchem-460	65	26	bombay	bombay	PROPN
eurjchem-460	65	27	.	.	PUNCT
eurjchem-460	66	1	ammonia	ammonia	NOUN
eurjchem-460	66	2	desorption	desorption	NOUN
eurjchem-460	66	3	experiments	experiment	NOUN
eurjchem-460	66	4	were	be	AUX
eurjchem-460	66	5	carried	carry	VERB
eurjchem-460	66	6	out	out	ADP
eurjchem-460	66	7	to	to	PART
eurjchem-460	66	8	measure	measure	VERB
eurjchem-460	66	9	the	the	DET
eurjchem-460	66	10	acidity	acidity	NOUN
eurjchem-460	66	11	of	of	ADP
eurjchem-460	66	12	the	the	DET
eurjchem-460	66	13	catalyst	catalyst	NOUN
eurjchem-460	66	14	using	use	VERB
eurjchem-460	66	15	ammonia	ammonia	NOUN
eurjchem-460	66	16	as	as	ADP
eurjchem-460	66	17	an	an	DET
eurjchem-460	66	18	adsorbate	adsorbate	NOUN
eurjchem-460	66	19	.	.	PUNCT
eurjchem-460	67	1	2.0	2.0	NUM
eurjchem-460	67	2	g	g	NOUN
eurjchem-460	67	3	of	of	ADP
eurjchem-460	67	4	catalyst	catalyst	NOUN
eurjchem-460	67	5	was	be	AUX
eurjchem-460	67	6	packed	pack	VERB
eurjchem-460	67	7	in	in	ADP
eurjchem-460	67	8	a	a	DET
eurjchem-460	67	9	pyrex	pyrex	NOUN
eurjchem-460	67	10	tube	tube	NOUN
eurjchem-460	67	11	down	down	ADP
eurjchem-460	67	12	flow	flow	NOUN
eurjchem-460	67	13	reactor	reactor	NOUN
eurjchem-460	67	14	and	and	CCONJ
eurjchem-460	67	15	heated	heat	VERB
eurjchem-460	67	16	to	to	ADP
eurjchem-460	67	17	673	673	NUM
eurjchem-460	67	18	k	k	NOUN
eurjchem-460	67	19	under	under	ADP
eurjchem-460	67	20	a	a	DET
eurjchem-460	67	21	nitrogen	nitrogen	NOUN
eurjchem-460	67	22	gas	gas	NOUN
eurjchem-460	67	23	flow	flow	NOUN
eurjchem-460	67	24	rate	rate	NOUN
eurjchem-460	67	25	of	of	ADP
eurjchem-460	67	26	0.5	0.5	NUM
eurjchem-460	67	27	cm3	cm3	NOUN
eurjchem-460	67	28	/	/	SYM
eurjchem-460	67	29	s	s	NOUN
eurjchem-460	67	30	for	for	ADP
eurjchem-460	67	31	3	3	NUM
eurjchem-460	67	32	h.	h.	NOUN
eurjchem-460	67	33	the	the	DET
eurjchem-460	67	34	reactor	reactor	NOUN
eurjchem-460	67	35	was	be	AUX
eurjchem-460	67	36	then	then	ADV
eurjchem-460	67	37	cooled	cool	VERB
eurjchem-460	67	38	to	to	ADP
eurjchem-460	67	39	298	298	NUM
eurjchem-460	67	40	k	k	NOUN
eurjchem-460	67	41	and	and	CCONJ
eurjchem-460	67	42	adsorption	adsorption	NOUN
eurjchem-460	67	43	conducted	conduct	VERB
eurjchem-460	67	44	at	at	ADP
eurjchem-460	67	45	that	that	DET
eurjchem-460	67	46	temperature	temperature	NOUN
eurjchem-460	67	47	by	by	ADP
eurjchem-460	67	48	exposing	expose	VERB
eurjchem-460	67	49	the	the	DET
eurjchem-460	67	50	sample	sample	NOUN
eurjchem-460	67	51	to	to	ADP
eurjchem-460	67	52	ammonia	ammonia	NOUN
eurjchem-460	67	53	for	for	SCONJ
eurjchem-460	67	54	2	2	NUM
eurjchem-460	67	55	h.	h.	NOUN
eurjchem-460	67	56	physically	physically	ADV
eurjchem-460	67	57	adsorbed	adsorb	VERB
eurjchem-460	67	58	ammonia	ammonia	NOUN
eurjchem-460	67	59	was	be	AUX
eurjchem-460	67	60	removed	remove	VERB
eurjchem-460	67	61	by	by	ADP
eurjchem-460	67	62	purging	purge	VERB
eurjchem-460	67	63	the	the	DET
eurjchem-460	67	64	sample	sample	NOUN
eurjchem-460	67	65	with	with	ADP
eurjchem-460	67	66	a	a	DET
eurjchem-460	67	67	nitrogen	nitrogen	NOUN
eurjchem-460	67	68	gas	gas	NOUN
eurjchem-460	67	69	(	(	PUNCT
eurjchem-460	67	70	flow	flow	NOUN
eurjchem-460	67	71	rate	rate	NOUN
eurjchem-460	67	72	0.5	0.5	NUM
eurjchem-460	67	73	cm3	cm3	PROPN
eurjchem-460	67	74	/	/	SYM
eurjchem-460	67	75	s	s	NOUN
eurjchem-460	67	76	)	)	PUNCT
eurjchem-460	67	77	at	at	ADP
eurjchem-460	67	78	353	353	NUM
eurjchem-460	67	79	k	k	NOUN
eurjchem-460	67	80	for	for	ADP
eurjchem-460	67	81	1	1	NUM
eurjchem-460	67	82	h.	h.	NOUN
eurjchem-460	67	83	the	the	DET
eurjchem-460	67	84	acid	acid	NOUN
eurjchem-460	67	85	strength	strength	NOUN
eurjchem-460	67	86	distribution	distribution	NOUN
eurjchem-460	67	87	was	be	AUX
eurjchem-460	67	88	obtained	obtain	VERB
eurjchem-460	67	89	by	by	ADP
eurjchem-460	67	90	raising	raise	VERB
eurjchem-460	67	91	the	the	DET
eurjchem-460	67	92	catalyst	catalyst	NOUN
eurjchem-460	67	93	temperature	temperature	NOUN
eurjchem-460	67	94	from	from	ADP
eurjchem-460	67	95	373‐773	373‐773	PROPN
eurjchem-460	67	96	k	k	NOUN
eurjchem-460	68	1	in	in	ADP
eurjchem-460	68	2	a	a	DET
eurjchem-460	68	3	flow	flow	NOUN
eurjchem-460	68	4	of	of	ADP
eurjchem-460	68	5	nitrogen	nitrogen	NOUN
eurjchem-460	68	6	gas	gas	NOUN
eurjchem-460	68	7	at	at	ADP
eurjchem-460	68	8	0.5	0.5	NUM
eurjchem-460	68	9	cm3	cm3	NOUN
eurjchem-460	68	10	s‐1and	s‐1and	CCONJ
eurjchem-460	68	11	absorbing	absorb	VERB
eurjchem-460	68	12	the	the	DET
eurjchem-460	68	13	ammonia	ammonia	NOUN
eurjchem-460	68	14	evolved	evolve	VERB
eurjchem-460	68	15	in	in	ADP
eurjchem-460	68	16	0.1	0.1	NUM
eurjchem-460	68	17	n	n	PRON
eurjchem-460	68	18	hcl	hcl	PROPN
eurjchem-460	68	19	.	.	PUNCT
eurjchem-460	69	1	quantitative	quantitative	ADJ
eurjchem-460	69	2	estimation	estimation	NOUN
eurjchem-460	69	3	was	be	AUX
eurjchem-460	69	4	made	make	VERB
eurjchem-460	69	5	by	by	ADP
eurjchem-460	69	6	titrating	titrate	VERB
eurjchem-460	69	7	the	the	DET
eurjchem-460	69	8	unreacted	unreacted	ADJ
eurjchem-460	69	9	hcl	hcl	PROPN
eurjchem-460	69	10	with	with	ADP
eurjchem-460	69	11	0.1	0.1	NUM
eurjchem-460	69	12	n	n	PRON
eurjchem-460	69	13	naoh	naoh	NOUN
eurjchem-460	69	14	in	in	ADP
eurjchem-460	69	15	different	different	ADJ
eurjchem-460	69	16	temperature	temperature	NOUN
eurjchem-460	69	17	ranges	range	NOUN
eurjchem-460	69	18	.	.	PUNCT
eurjchem-460	70	1	the	the	DET
eurjchem-460	70	2	results	result	NOUN
eurjchem-460	70	3	are	be	AUX
eurjchem-460	70	4	presented	present	VERB
eurjchem-460	70	5	in	in	ADP
eurjchem-460	70	6	table	table	NOUN
eurjchem-460	70	7	2	2	NUM
eurjchem-460	70	8	.	.	NOUN
eurjchem-460	70	9	2.3	2.3	NUM
eurjchem-460	70	10	.	.	PUNCT
eurjchem-460	71	1	experimental	experimental	ADJ
eurjchem-460	71	2	procedure	procedure	NOUN
eurjchem-460	71	3	the	the	DET
eurjchem-460	71	4	reaction	reaction	NOUN
eurjchem-460	71	5	was	be	AUX
eurjchem-460	71	6	carried	carry	VERB
eurjchem-460	71	7	out	out	ADP
eurjchem-460	71	8	in	in	ADP
eurjchem-460	71	9	a	a	DET
eurjchem-460	71	10	100	100	NUM
eurjchem-460	71	11	ml	ml	NOUN
eurjchem-460	71	12	,	,	PUNCT
eurjchem-460	71	13	three‐neck	three‐neck	NOUN
eurjchem-460	71	14	round‐	round‐	ADV
eurjchem-460	71	15	bottomed	bottom	VERB
eurjchem-460	71	16	flask	flask	NOUN
eurjchem-460	71	17	,	,	PUNCT
eurjchem-460	71	18	equipped	equip	VERB
eurjchem-460	71	19	with	with	ADP
eurjchem-460	71	20	a	a	DET
eurjchem-460	71	21	condenser	condenser	NOUN
eurjchem-460	71	22	and	and	CCONJ
eurjchem-460	71	23	a	a	DET
eurjchem-460	71	24	thermometer	thermometer	NOUN
eurjchem-460	71	25	.	.	PUNCT
eurjchem-460	72	1	the	the	DET
eurjchem-460	72	2	condenser	condenser	NOUN
eurjchem-460	72	3	was	be	AUX
eurjchem-460	72	4	connected	connect	VERB
eurjchem-460	72	5	to	to	ADP
eurjchem-460	72	6	a	a	DET
eurjchem-460	72	7	vacuum	vacuum	NOUN
eurjchem-460	72	8	pump	pump	NOUN
eurjchem-460	72	9	through	through	ADP
eurjchem-460	72	10	an	an	DET
eurjchem-460	72	11	hcl	hcl	PROPN
eurjchem-460	72	12	tower	tower	NOUN
eurjchem-460	72	13	and	and	CCONJ
eurjchem-460	72	14	an	an	DET
eurjchem-460	72	15	ice	ice	NOUN
eurjchem-460	72	16	cold	cold	ADJ
eurjchem-460	72	17	trape	trape	NOUN
eurjchem-460	72	18	,	,	PUNCT
eurjchem-460	72	19	to	to	PART
eurjchem-460	72	20	pump	pump	VERB
eurjchem-460	72	21	out	out	ADP
eurjchem-460	72	22	ammonia	ammonia	NOUN
eurjchem-460	72	23	gas	gas	NOUN
eurjchem-460	72	24	produced	produce	VERB
eurjchem-460	72	25	during	during	ADP
eurjchem-460	72	26	the	the	DET
eurjchem-460	72	27	reaction	reaction	NOUN
eurjchem-460	72	28	(	(	PUNCT
eurjchem-460	72	29	figure	figure	NOUN
eurjchem-460	72	30	1	1	NUM
eurjchem-460	72	31	)	)	PUNCT
eurjchem-460	72	32	.	.	PUNCT
eurjchem-460	73	1	the	the	DET
eurjchem-460	73	2	reactor	reactor	NOUN
eurjchem-460	73	3	was	be	AUX
eurjchem-460	73	4	charged	charge	VERB
eurjchem-460	73	5	with	with	ADP
eurjchem-460	73	6	ethylene	ethylene	NOUN
eurjchem-460	73	7	glycol	glycol	NOUN
eurjchem-460	73	8	and	and	CCONJ
eurjchem-460	73	9	urea	urea	NOUN
eurjchem-460	73	10	and	and	CCONJ
eurjchem-460	73	11	was	be	AUX
eurjchem-460	73	12	put	put	VERB
eurjchem-460	73	13	to	to	PART
eurjchem-460	73	14	reflux	reflux	VERB
eurjchem-460	73	15	at	at	ADP
eurjchem-460	73	16	423	423	NUM
eurjchem-460	73	17	k.	k.	NOUN
eurjchem-460	73	18	after	after	ADP
eurjchem-460	73	19	the	the	DET
eurjchem-460	73	20	completion	completion	NOUN
eurjchem-460	73	21	of	of	ADP
eurjchem-460	73	22	reaction	reaction	NOUN
eurjchem-460	73	23	,	,	PUNCT
eurjchem-460	73	24	the	the	DET
eurjchem-460	73	25	product	product	NOUN
eurjchem-460	73	26	was	be	AUX
eurjchem-460	73	27	filtered	filter	VERB
eurjchem-460	73	28	to	to	PART
eurjchem-460	73	29	separate	separate	VERB
eurjchem-460	73	30	the	the	DET
eurjchem-460	73	31	catalyst	catalyst	NOUN
eurjchem-460	73	32	.	.	PUNCT
eurjchem-460	74	1	the	the	DET
eurjchem-460	74	2	filtrate	filtrate	NOUN
eurjchem-460	74	3	was	be	AUX
eurjchem-460	74	4	cool	cool	ADJ
eurjchem-460	74	5	to	to	PART
eurjchem-460	74	6	room	room	VERB
eurjchem-460	74	7	temperature	temperature	NOUN
eurjchem-460	74	8	.	.	PUNCT
eurjchem-460	75	1	bhadauria	bhadauria	NOUN
eurjchem-460	75	2	et	et	PROPN
eurjchem-460	75	3	al	al	PROPN
eurjchem-460	75	4	.	.	PUNCT
eurjchem-460	75	5	/	/	SYM
eurjchem-460	75	6	european	european	PROPN
eurjchem-460	75	7	journal	journal	PROPN
eurjchem-460	75	8	of	of	ADP
eurjchem-460	75	9	chemistry	chemistry	NOUN
eurjchem-460	75	10	3	3	NUM
eurjchem-460	75	11	(	(	PUNCT
eurjchem-460	75	12	2	2	NUM
eurjchem-460	75	13	)	)	PUNCT
eurjchem-460	75	14	(	(	PUNCT
eurjchem-460	75	15	2012	2012	NUM
eurjchem-460	75	16	)	)	PUNCT
eurjchem-460	75	17	235‐240	235‐240	PROPN
eurjchem-460	75	18	237	237	NUM
eurjchem-460	75	19	2.4	2.4	NUM
eurjchem-460	75	20	.	.	PUNCT
eurjchem-460	76	1	identification	identification	NOUN
eurjchem-460	76	2	and	and	CCONJ
eurjchem-460	76	3	analysis	analysis	NOUN
eurjchem-460	76	4	of	of	ADP
eurjchem-460	76	5	product	product	NOUN
eurjchem-460	76	6	about	about	ADV
eurjchem-460	76	7	10	10	NUM
eurjchem-460	76	8	g	g	NOUN
eurjchem-460	76	9	of	of	ADP
eurjchem-460	76	10	solid	solid	ADJ
eurjchem-460	76	11	sample	sample	NOUN
eurjchem-460	76	12	was	be	AUX
eurjchem-460	76	13	collected	collect	VERB
eurjchem-460	76	14	.	.	PUNCT
eurjchem-460	77	1	its	its	PRON
eurjchem-460	77	2	melting	melting	NOUN
eurjchem-460	77	3	point	point	NOUN
eurjchem-460	77	4	was	be	AUX
eurjchem-460	77	5	determined	determine	VERB
eurjchem-460	77	6	to	to	PART
eurjchem-460	77	7	be	be	AUX
eurjchem-460	77	8	307	307	NUM
eurjchem-460	77	9	k.	k.	NOUN
eurjchem-460	78	1	an	an	DET
eurjchem-460	78	2	ir	ir	PROPN
eurjchem-460	78	3	spectrum	spectrum	NOUN
eurjchem-460	78	4	of	of	ADP
eurjchem-460	78	5	the	the	DET
eurjchem-460	78	6	solid	solid	ADJ
eurjchem-460	78	7	sample	sample	NOUN
eurjchem-460	78	8	recorded	record	VERB
eurjchem-460	78	9	at	at	ADP
eurjchem-460	78	10	shimadzu	shimadzu	ADJ
eurjchem-460	78	11	r‐460	r‐460	NOUN
eurjchem-460	78	12	spectrometer	spectrometer	NOUN
eurjchem-460	78	13	in	in	ADP
eurjchem-460	78	14	the	the	DET
eurjchem-460	78	15	range	range	NOUN
eurjchem-460	78	16	400‐4000	400‐4000	NUM
eurjchem-460	78	17	cm‐1	cm‐1	NOUN
eurjchem-460	78	18	shows	show	VERB
eurjchem-460	78	19	band	band	NOUN
eurjchem-460	78	20	at	at	ADP
eurjchem-460	78	21	1752	1752	NUM
eurjchem-460	78	22	cm‐1	cm‐1	NOUN
eurjchem-460	78	23	which	which	PRON
eurjchem-460	78	24	can	can	AUX
eurjchem-460	78	25	be	be	AUX
eurjchem-460	78	26	assign	assign	VERB
eurjchem-460	78	27	to	to	ADP
eurjchem-460	78	28	c	c	NOUN
eurjchem-460	78	29	=	=	VERB
eurjchem-460	78	30	o	o	NOUN
eurjchem-460	78	31	stretching	stretch	VERB
eurjchem-460	78	32	mode	mode	NOUN
eurjchem-460	78	33	.	.	PUNCT
eurjchem-460	79	1	quantitative	quantitative	ADJ
eurjchem-460	79	2	analysis	analysis	NOUN
eurjchem-460	79	3	of	of	ADP
eurjchem-460	79	4	the	the	DET
eurjchem-460	79	5	product	product	NOUN
eurjchem-460	79	6	mixture	mixture	NOUN
eurjchem-460	79	7	was	be	AUX
eurjchem-460	79	8	made	make	VERB
eurjchem-460	79	9	employing	employ	VERB
eurjchem-460	79	10	a	a	DET
eurjchem-460	79	11	gas	gas	NOUN
eurjchem-460	79	12	liquid	liquid	NOUN
eurjchem-460	79	13	chromatograph	chromatograph	NOUN
eurjchem-460	79	14	(	(	PUNCT
eurjchem-460	79	15	chemito	chemito	NOUN
eurjchem-460	79	16	gas	gas	NOUN
eurjchem-460	79	17	chromatograph	chromatograph	NOUN
eurjchem-460	79	18	7610	7610	NUM
eurjchem-460	79	19	)	)	PUNCT
eurjchem-460	79	20	equipped	equip	VERB
eurjchem-460	79	21	with	with	ADP
eurjchem-460	79	22	a	a	DET
eurjchem-460	79	23	flame	flame	NOUN
eurjchem-460	79	24	ionization	ionization	NOUN
eurjchem-460	79	25	detector	detector	NOUN
eurjchem-460	79	26	.	.	PUNCT
eurjchem-460	80	1	the	the	DET
eurjchem-460	80	2	conditions	condition	NOUN
eurjchem-460	80	3	of	of	ADP
eurjchem-460	80	4	gc	gc	PROPN
eurjchem-460	80	5	analysis	analysis	NOUN
eurjchem-460	80	6	were	be	AUX
eurjchem-460	80	7	:	:	PUNCT
eurjchem-460	80	8	fid	fid	NOUN
eurjchem-460	80	9	detector	detector	NOUN
eurjchem-460	80	10	,	,	PUNCT
eurjchem-460	80	11	temperature	temperature	NOUN
eurjchem-460	80	12	=	=	SYM
eurjchem-460	80	13	473	473	NUM
eurjchem-460	80	14	k	k	NOUN
eurjchem-460	80	15	;	;	PUNCT
eurjchem-460	80	16	injector	injector	NOUN
eurjchem-460	80	17	temperature	temperature	NOUN
eurjchem-460	80	18	,	,	PUNCT
eurjchem-460	80	19	473	473	NUM
eurjchem-460	80	20	k	k	NOUN
eurjchem-460	80	21	,	,	PUNCT
eurjchem-460	80	22	and	and	CCONJ
eurjchem-460	80	23	column	column	NOUN
eurjchem-460	80	24	temperature	temperature	NOUN
eurjchem-460	80	25	ranges	range	VERB
eurjchem-460	80	26	from	from	ADP
eurjchem-460	80	27	353	353	NUM
eurjchem-460	80	28	k	k	NOUN
eurjchem-460	80	29	to	to	ADP
eurjchem-460	80	30	473	473	NUM
eurjchem-460	80	31	k.	k.	NOUN
eurjchem-460	80	32	nitrogen	nitrogen	PROPN
eurjchem-460	80	33	was	be	AUX
eurjchem-460	80	34	used	use	VERB
eurjchem-460	80	35	as	as	ADP
eurjchem-460	80	36	a	a	DET
eurjchem-460	80	37	carrier	carrier	NOUN
eurjchem-460	80	38	gas	gas	NOUN
eurjchem-460	80	39	.	.	PUNCT
eurjchem-460	81	1	3	3	X
eurjchem-460	81	2	.	.	NOUN
eurjchem-460	81	3	results	result	NOUN
eurjchem-460	81	4	and	and	CCONJ
eurjchem-460	81	5	discussion	discussion	NOUN
eurjchem-460	81	6	3.1	3.1	NUM
eurjchem-460	81	7	.	.	PUNCT
eurjchem-460	81	8	catalyst	catalyst	NOUN
eurjchem-460	81	9	characterization	characterization	NOUN
eurjchem-460	81	10	the	the	DET
eurjchem-460	81	11	xrd	xrd	NOUN
eurjchem-460	81	12	pattern	pattern	NOUN
eurjchem-460	81	13	of	of	ADP
eurjchem-460	81	14	various	various	ADJ
eurjchem-460	81	15	catalysts	catalyst	NOUN
eurjchem-460	81	16	is	be	AUX
eurjchem-460	81	17	reproduced	reproduce	VERB
eurjchem-460	81	18	in	in	ADP
eurjchem-460	81	19	figure	figure	NOUN
eurjchem-460	81	20	2	2	NUM
eurjchem-460	81	21	.	.	PUNCT
eurjchem-460	82	1	although	although	SCONJ
eurjchem-460	82	2	,	,	PUNCT
eurjchem-460	82	3	most	most	ADJ
eurjchem-460	82	4	of	of	ADP
eurjchem-460	82	5	the	the	DET
eurjchem-460	82	6	xrd	xrd	NOUN
eurjchem-460	82	7	peaks	peak	NOUN
eurjchem-460	82	8	corresponds	correspond	VERB
eurjchem-460	82	9	to	to	ADP
eurjchem-460	82	10	zncr2o4	zncr2o4	NUM
eurjchem-460	82	11	spinel	spinel	NOUN
eurjchem-460	82	12	,	,	PUNCT
eurjchem-460	82	13	peak	peak	NOUN
eurjchem-460	82	14	at	at	ADP
eurjchem-460	82	15	θ	θ	PROPN
eurjchem-460	82	16	=	=	SYM
eurjchem-460	82	17	68.0	68.0	NUM
eurjchem-460	82	18	corresponds	correspond	NOUN
eurjchem-460	82	19	to	to	ADP
eurjchem-460	82	20	zno	zno	NOUN
eurjchem-460	82	21	,	,	PUNCT
eurjchem-460	82	22	while	while	SCONJ
eurjchem-460	82	23	that	that	PRON
eurjchem-460	82	24	appeared	appear	VERB
eurjchem-460	82	25	at	at	ADP
eurjchem-460	82	26	θ	θ	PROPN
eurjchem-460	82	27	=	=	SYM
eurjchem-460	82	28	36.2	36.2	NUM
eurjchem-460	82	29	correspond	correspond	NOUN
eurjchem-460	82	30	to	to	ADP
eurjchem-460	82	31	chromium	chromium	NOUN
eurjchem-460	82	32	oxide	oxide	NOUN
eurjchem-460	82	33	.	.	PUNCT
eurjchem-460	83	1	thus	thus	ADV
eurjchem-460	83	2	,	,	PUNCT
eurjchem-460	83	3	our	our	PRON
eurjchem-460	83	4	catalyst	catalyst	NOUN
eurjchem-460	83	5	system	system	NOUN
eurjchem-460	83	6	is	be	AUX
eurjchem-460	83	7	composed	compose	VERB
eurjchem-460	83	8	of	of	ADP
eurjchem-460	83	9	zno	zno	NOUN
eurjchem-460	84	1	[	[	X
eurjchem-460	84	2	39	39	NUM
eurjchem-460	84	3	]	]	PUNCT
eurjchem-460	84	4	,	,	PUNCT
eurjchem-460	84	5	cr2o3	cr2o3	PROPN
eurjchem-460	84	6	and	and	CCONJ
eurjchem-460	84	7	zncr2o4	zncr2o4	PROPN
eurjchem-460	84	8	.	.	PUNCT
eurjchem-460	85	1	the	the	DET
eurjchem-460	85	2	expected	expect	VERB
eurjchem-460	85	3	composition	composition	NOUN
eurjchem-460	85	4	of	of	ADP
eurjchem-460	85	5	all	all	DET
eurjchem-460	85	6	catalysts	catalyst	NOUN
eurjchem-460	85	7	is	be	AUX
eurjchem-460	85	8	listed	list	VERB
eurjchem-460	85	9	in	in	ADP
eurjchem-460	85	10	table	table	NOUN
eurjchem-460	85	11	1	1	NUM
eurjchem-460	85	12	.	.	PUNCT
eurjchem-460	86	1	the	the	DET
eurjchem-460	86	2	chromites	chromite	NOUN
eurjchem-460	86	3	composition	composition	NOUN
eurjchem-460	86	4	increases	increase	NOUN
eurjchem-460	86	5	with	with	ADP
eurjchem-460	86	6	increasing	increase	VERB
eurjchem-460	86	7	amount	amount	NOUN
eurjchem-460	86	8	of	of	ADP
eurjchem-460	86	9	chromium	chromium	NOUN
eurjchem-460	86	10	chloride	chloride	NOUN
eurjchem-460	86	11	.	.	PUNCT
eurjchem-460	87	1	this	this	PRON
eurjchem-460	87	2	is	be	AUX
eurjchem-460	87	3	also	also	ADV
eurjchem-460	87	4	reflected	reflect	VERB
eurjchem-460	87	5	in	in	ADP
eurjchem-460	87	6	the	the	DET
eurjchem-460	87	7	xrd	xrd	NOUN
eurjchem-460	87	8	pattern	pattern	NOUN
eurjchem-460	87	9	.	.	PUNCT
eurjchem-460	88	1	it	it	PRON
eurjchem-460	88	2	is	be	AUX
eurjchem-460	88	3	worth	worth	ADJ
eurjchem-460	88	4	noting	note	VERB
eurjchem-460	88	5	that	that	SCONJ
eurjchem-460	88	6	xrd	xrd	NOUN
eurjchem-460	88	7	pattern	pattern	NOUN
eurjchem-460	88	8	of	of	ADP
eurjchem-460	88	9	zc‐5	zc‐5	NOUN
eurjchem-460	88	10	correspond	correspond	VERB
eurjchem-460	88	11	to	to	ADP
eurjchem-460	88	12	single	single	ADJ
eurjchem-460	88	13	phase	phase	NOUN
eurjchem-460	88	14	zncr2o4	zncr2o4	NUM
eurjchem-460	88	15	and	and	CCONJ
eurjchem-460	88	16	match	match	VERB
eurjchem-460	88	17	well	well	ADV
eurjchem-460	88	18	with	with	ADP
eurjchem-460	88	19	jcpds	jcpds	PROPN
eurjchem-460	88	20	card	card	NOUN
eurjchem-460	88	21	no	no	INTJ
eurjchem-460	88	22	.	.	PUNCT
eurjchem-460	89	1	73‐1962	73‐1962	X
eurjchem-460	89	2	.	.	PUNCT
eurjchem-460	90	1	the	the	DET
eurjchem-460	90	2	sem	sem	NOUN
eurjchem-460	90	3	images	image	NOUN
eurjchem-460	90	4	of	of	ADP
eurjchem-460	90	5	three	three	NUM
eurjchem-460	90	6	typical	typical	ADJ
eurjchem-460	90	7	catalysts	catalyst	NOUN
eurjchem-460	90	8	zc‐1	zc‐1	PROPN
eurjchem-460	90	9	,	,	PUNCT
eurjchem-460	90	10	zc‐2	zc‐2	PROPN
eurjchem-460	90	11	,	,	PUNCT
eurjchem-460	90	12	zc‐3	zc‐3	PROPN
eurjchem-460	90	13	are	be	AUX
eurjchem-460	90	14	reproduced	reproduce	VERB
eurjchem-460	90	15	in	in	ADP
eurjchem-460	90	16	figure	figure	NOUN
eurjchem-460	90	17	3	3	NUM
eurjchem-460	90	18	.	.	PUNCT
eurjchem-460	91	1	the	the	DET
eurjchem-460	91	2	sem	sem	PROPN
eurjchem-460	91	3	picture	picture	NOUN
eurjchem-460	91	4	of	of	ADP
eurjchem-460	91	5	figure	figure	NOUN
eurjchem-460	91	6	3	3	NUM
eurjchem-460	91	7	(	(	PUNCT
eurjchem-460	91	8	a	a	NOUN
eurjchem-460	91	9	)	)	PUNCT
eurjchem-460	91	10	is	be	AUX
eurjchem-460	91	11	typical	typical	ADJ
eurjchem-460	91	12	to	to	ADP
eurjchem-460	91	13	that	that	PRON
eurjchem-460	91	14	of	of	ADP
eurjchem-460	91	15	zno	zno	NOUN
eurjchem-460	91	16	rods	rod	NOUN
eurjchem-460	91	17	.	.	PUNCT
eurjchem-460	92	1	with	with	ADP
eurjchem-460	92	2	increasing	increase	VERB
eurjchem-460	92	3	content	content	NOUN
eurjchem-460	92	4	of	of	ADP
eurjchem-460	92	5	cr2o3	cr2o3	PROPN
eurjchem-460	92	6	in	in	ADP
eurjchem-460	92	7	the	the	DET
eurjchem-460	92	8	catalyst	catalyst	NOUN
eurjchem-460	92	9	(	(	PUNCT
eurjchem-460	92	10	figure	figure	NOUN
eurjchem-460	92	11	3	3	NUM
eurjchem-460	92	12	(	(	PUNCT
eurjchem-460	92	13	b	b	NOUN
eurjchem-460	92	14	)	)	PUNCT
eurjchem-460	92	15	and	and	CCONJ
eurjchem-460	92	16	(	(	PUNCT
eurjchem-460	92	17	c	c	NOUN
eurjchem-460	92	18	)	)	PUNCT
eurjchem-460	92	19	)	)	PUNCT
eurjchem-460	93	1	the	the	DET
eurjchem-460	93	2	zno	zno	NOUN
eurjchem-460	93	3	rods	rod	NOUN
eurjchem-460	93	4	have	have	AUX
eurjchem-460	93	5	vanished	vanish	VERB
eurjchem-460	93	6	suggesting	suggest	VERB
eurjchem-460	93	7	formation	formation	NOUN
eurjchem-460	93	8	of	of	ADP
eurjchem-460	93	9	spinel	spinel	NOUN
eurjchem-460	93	10	structure	structure	NOUN
eurjchem-460	93	11	.	.	PUNCT
eurjchem-460	94	1	figure	figure	NOUN
eurjchem-460	94	2	2	2	NUM
eurjchem-460	94	3	.	.	PUNCT
eurjchem-460	95	1	the	the	DET
eurjchem-460	95	2	xrd	xrd	NOUN
eurjchem-460	95	3	pattern	pattern	NOUN
eurjchem-460	95	4	of	of	ADP
eurjchem-460	95	5	the	the	DET
eurjchem-460	95	6	various	various	ADJ
eurjchem-460	95	7	zno	zno	X
eurjchem-460	95	8	·	·	PUNCT
eurjchem-460	95	9	cr2o3	cr2o3	PROPN
eurjchem-460	95	10	catalysts	catalyst	NOUN
eurjchem-460	95	11	.	.	PUNCT
eurjchem-460	96	1	bet	bet	PROPN
eurjchem-460	96	2	surface	surface	PROPN
eurjchem-460	96	3	area	area	PROPN
eurjchem-460	96	4	records	record	NOUN
eurjchem-460	96	5	are	be	AUX
eurjchem-460	96	6	listed	list	VERB
eurjchem-460	96	7	in	in	ADP
eurjchem-460	96	8	table	table	NOUN
eurjchem-460	96	9	2	2	NUM
eurjchem-460	96	10	.	.	PUNCT
eurjchem-460	97	1	the	the	DET
eurjchem-460	97	2	surface	surface	NOUN
eurjchem-460	97	3	area	area	NOUN
eurjchem-460	97	4	increased	increase	VERB
eurjchem-460	97	5	with	with	ADP
eurjchem-460	97	6	increasing	increase	VERB
eurjchem-460	97	7	amount	amount	NOUN
eurjchem-460	97	8	of	of	ADP
eurjchem-460	97	9	cr2o3	cr2o3	PROPN
eurjchem-460	97	10	.	.	PUNCT
eurjchem-460	98	1	this	this	PRON
eurjchem-460	98	2	can	can	AUX
eurjchem-460	98	3	be	be	AUX
eurjchem-460	98	4	correlated	correlate	VERB
eurjchem-460	98	5	to	to	PART
eurjchem-460	98	6	decrease	decrease	VERB
eurjchem-460	98	7	in	in	ADP
eurjchem-460	98	8	the	the	DET
eurjchem-460	98	9	particle	particle	NOUN
eurjchem-460	98	10	size	size	NOUN
eurjchem-460	98	11	of	of	ADP
eurjchem-460	98	12	the	the	DET
eurjchem-460	98	13	catalysts	catalyst	NOUN
eurjchem-460	98	14	.	.	PUNCT
eurjchem-460	99	1	an	an	DET
eurjchem-460	99	2	inspection	inspection	NOUN
eurjchem-460	99	3	of	of	ADP
eurjchem-460	99	4	table	table	NOUN
eurjchem-460	99	5	2	2	NUM
eurjchem-460	99	6	suggests	suggest	VERB
eurjchem-460	99	7	all	all	DET
eurjchem-460	99	8	the	the	DET
eurjchem-460	99	9	catalysts	catalyst	NOUN
eurjchem-460	99	10	to	to	PART
eurjchem-460	99	11	possess	possess	VERB
eurjchem-460	99	12	acidic	acidic	ADJ
eurjchem-460	99	13	nature	nature	NOUN
eurjchem-460	99	14	.	.	PUNCT
eurjchem-460	100	1	acidity	acidity	NOUN
eurjchem-460	100	2	in	in	ADP
eurjchem-460	100	3	zno	zno	NOUN
eurjchem-460	100	4	has	have	AUX
eurjchem-460	100	5	been	be	AUX
eurjchem-460	100	6	shown	show	VERB
eurjchem-460	100	7	by	by	ADP
eurjchem-460	100	8	others	other	NOUN
eurjchem-460	100	9	also	also	ADV
eurjchem-460	101	1	[	[	X
eurjchem-460	101	2	40,41	40,41	NOUN
eurjchem-460	101	3	]	]	X
eurjchem-460	101	4	.	.	PUNCT
eurjchem-460	102	1	presence	presence	NOUN
eurjchem-460	102	2	of	of	ADP
eurjchem-460	102	3	acidity	acidity	NOUN
eurjchem-460	102	4	is	be	AUX
eurjchem-460	102	5	important	important	ADJ
eurjchem-460	102	6	for	for	ADP
eurjchem-460	102	7	adsorption	adsorption	NOUN
eurjchem-460	102	8	of	of	ADP
eurjchem-460	102	9	reactants	reactant	NOUN
eurjchem-460	102	10	.	.	PUNCT
eurjchem-460	103	1	3.2	3.2	NUM
eurjchem-460	103	2	.	.	PUNCT
eurjchem-460	103	3	performance	performance	NOUN
eurjchem-460	103	4	of	of	ADP
eurjchem-460	103	5	various	various	ADJ
eurjchem-460	103	6	catalysts	catalyst	NOUN
eurjchem-460	103	7	in	in	ADP
eurjchem-460	103	8	the	the	DET
eurjchem-460	103	9	cyclization	cyclization	NOUN
eurjchem-460	103	10	of	of	ADP
eurjchem-460	103	11	ethylene	ethylene	NOUN
eurjchem-460	103	12	glycol	glycol	NOUN
eurjchem-460	103	13	and	and	CCONJ
eurjchem-460	103	14	urea	urea	NOUN
eurjchem-460	103	15	to	to	ADP
eurjchem-460	103	16	ec	ec	PROPN
eurjchem-460	103	17	catalysts	catalyst	NOUN
eurjchem-460	103	18	with	with	ADP
eurjchem-460	103	19	their	their	PRON
eurjchem-460	103	20	performances	performance	NOUN
eurjchem-460	103	21	are	be	AUX
eurjchem-460	103	22	shown	show	VERB
eurjchem-460	103	23	in	in	ADP
eurjchem-460	103	24	table	table	NOUN
eurjchem-460	103	25	2	2	NUM
eurjchem-460	103	26	.	.	PUNCT
eurjchem-460	104	1	the	the	DET
eurjchem-460	104	2	order	order	NOUN
eurjchem-460	104	3	of	of	ADP
eurjchem-460	104	4	catalytic	catalytic	ADJ
eurjchem-460	104	5	activity	activity	NOUN
eurjchem-460	104	6	of	of	ADP
eurjchem-460	104	7	system	system	NOUN
eurjchem-460	104	8	toward	toward	ADP
eurjchem-460	104	9	overall	overall	ADJ
eurjchem-460	104	10	conversion	conversion	NOUN
eurjchem-460	104	11	was	be	AUX
eurjchem-460	104	12	observed	observe	VERB
eurjchem-460	104	13	to	to	PART
eurjchem-460	104	14	be	be	AUX
eurjchem-460	104	15	zc‐1	zc‐1	PROPN
eurjchem-460	104	16	>	>	X
eurjchem-460	105	1	zc‐2	zc‐2	PUNCT
eurjchem-460	105	2	>	>	PUNCT
eurjchem-460	105	3	zc‐3	zc‐3	X
eurjchem-460	105	4	>	>	X
eurjchem-460	105	5	zc‐	zc‐	PROPN
eurjchem-460	105	6	4	4	NUM
eurjchem-460	105	7	>	>	X
eurjchem-460	105	8	zc‐	zc‐	PROPN
eurjchem-460	105	9	5	5	NUM
eurjchem-460	105	10	.	.	PUNCT
eurjchem-460	106	1	the	the	DET
eurjchem-460	106	2	best	good	ADJ
eurjchem-460	106	3	activity	activity	NOUN
eurjchem-460	106	4	was	be	AUX
eurjchem-460	106	5	shown	show	VERB
eurjchem-460	106	6	by	by	ADP
eurjchem-460	106	7	zc‐1	zc‐1	PROPN
eurjchem-460	106	8	.	.	PUNCT
eurjchem-460	107	1	therefore	therefore	ADV
eurjchem-460	107	2	,	,	PUNCT
eurjchem-460	107	3	further	further	ADJ
eurjchem-460	107	4	studies	study	NOUN
eurjchem-460	107	5	were	be	AUX
eurjchem-460	107	6	performed	perform	VERB
eurjchem-460	107	7	on	on	ADP
eurjchem-460	107	8	this	this	DET
eurjchem-460	107	9	catalyst	catalyst	NOUN
eurjchem-460	107	10	.	.	PUNCT
eurjchem-460	108	1	(	(	PUNCT
eurjchem-460	108	2	a	a	X
eurjchem-460	108	3	)	)	PUNCT
eurjchem-460	108	4	(	(	PUNCT
eurjchem-460	108	5	b	b	X
eurjchem-460	108	6	)	)	PUNCT
eurjchem-460	108	7	(	(	PUNCT
eurjchem-460	108	8	c	c	X
eurjchem-460	108	9	)	)	PUNCT
eurjchem-460	108	10	figure	figure	NOUN
eurjchem-460	108	11	3	3	NUM
eurjchem-460	108	12	.	.	PUNCT
eurjchem-460	108	13	sem	sem	ADJ
eurjchem-460	108	14	images	image	NOUN
eurjchem-460	108	15	of	of	ADP
eurjchem-460	108	16	(	(	PUNCT
eurjchem-460	108	17	a	a	X
eurjchem-460	108	18	)	)	PUNCT
eurjchem-460	108	19	zc‐1	zc‐1	PROPN
eurjchem-460	109	1	(	(	PUNCT
eurjchem-460	109	2	b	b	X
eurjchem-460	109	3	)	)	PUNCT
eurjchem-460	109	4	zc‐3	zc‐3	NOUN
eurjchem-460	109	5	(	(	PUNCT
eurjchem-460	109	6	c	c	NOUN
eurjchem-460	109	7	)	)	PUNCT
eurjchem-460	109	8	zc‐5	zc‐5	NOUN
eurjchem-460	109	9	.	.	PUNCT
eurjchem-460	110	1	3.3	3.3	NUM
eurjchem-460	110	2	.	.	PUNCT
eurjchem-460	111	1	effect	effect	NOUN
eurjchem-460	111	2	of	of	ADP
eurjchem-460	111	3	temperature	temperature	NOUN
eurjchem-460	111	4	on	on	ADP
eurjchem-460	111	5	the	the	DET
eurjchem-460	111	6	synthesis	synthesis	NOUN
eurjchem-460	111	7	of	of	ADP
eurjchem-460	111	8	ec	ec	PROPN
eurjchem-460	111	9	the	the	DET
eurjchem-460	111	10	effect	effect	NOUN
eurjchem-460	111	11	of	of	ADP
eurjchem-460	111	12	temperature	temperature	NOUN
eurjchem-460	111	13	on	on	ADP
eurjchem-460	111	14	the	the	DET
eurjchem-460	111	15	cyclization	cyclization	NOUN
eurjchem-460	111	16	of	of	ADP
eurjchem-460	111	17	ec	ec	PROPN
eurjchem-460	111	18	is	be	AUX
eurjchem-460	111	19	shown	show	VERB
eurjchem-460	111	20	in	in	ADP
eurjchem-460	111	21	figure	figure	NOUN
eurjchem-460	111	22	4	4	NUM
eurjchem-460	111	23	.	.	PUNCT
eurjchem-460	112	1	conversion	conversion	NOUN
eurjchem-460	112	2	increased	increase	VERB
eurjchem-460	112	3	slowly	slowly	ADV
eurjchem-460	112	4	up	up	ADP
eurjchem-460	112	5	to	to	PART
eurjchem-460	112	6	400	400	NUM
eurjchem-460	112	7	k	k	NOUN
eurjchem-460	112	8	reached	reach	VERB
eurjchem-460	112	9	a	a	DET
eurjchem-460	112	10	maximum	maximum	NOUN
eurjchem-460	112	11	of	of	ADP
eurjchem-460	112	12	70	70	NUM
eurjchem-460	112	13	%	%	NOUN
eurjchem-460	112	14	at	at	ADP
eurjchem-460	112	15	423	423	NUM
eurjchem-460	112	16	k.	k.	NOUN
eurjchem-460	112	17	thus	thus	ADV
eurjchem-460	112	18	,	,	PUNCT
eurjchem-460	112	19	optimum	optimum	ADJ
eurjchem-460	112	20	temperature	temperature	NOUN
eurjchem-460	112	21	range	range	NOUN
eurjchem-460	112	22	of	of	ADP
eurjchem-460	112	23	cycloaddition	cycloaddition	NOUN
eurjchem-460	112	24	with	with	ADP
eurjchem-460	112	25	urea	urea	PROPN
eurjchem-460	112	26	over	over	ADP
eurjchem-460	112	27	zc‐1	zc‐1	PROPN
eurjchem-460	112	28	catalyst	catalyst	NOUN
eurjchem-460	112	29	seems	seem	VERB
eurjchem-460	112	30	to	to	PART
eurjchem-460	112	31	be	be	AUX
eurjchem-460	112	32	400‐	400‐	NUM
eurjchem-460	112	33	448	448	NUM
eurjchem-460	112	34	k.	k.	NOUN
eurjchem-460	113	1	maximum	maximum	PROPN
eurjchem-460	113	2	selectivity	selectivity	PROPN
eurjchem-460	113	3	was	be	AUX
eurjchem-460	113	4	also	also	ADV
eurjchem-460	113	5	found	find	VERB
eurjchem-460	113	6	in	in	ADP
eurjchem-460	113	7	the	the	DET
eurjchem-460	113	8	same	same	ADJ
eurjchem-460	113	9	temperature	temperature	NOUN
eurjchem-460	113	10	range	range	NOUN
eurjchem-460	113	11	.	.	PUNCT
eurjchem-460	114	1	figure	figure	NOUN
eurjchem-460	114	2	4	4	NUM
eurjchem-460	114	3	.	.	PUNCT
eurjchem-460	114	4	effect	effect	NOUN
eurjchem-460	114	5	of	of	ADP
eurjchem-460	114	6	reaction	reaction	NOUN
eurjchem-460	114	7	temperature	temperature	NOUN
eurjchem-460	114	8	on	on	ADP
eurjchem-460	114	9	ec	ec	PROPN
eurjchem-460	114	10	yield	yield	NOUN
eurjchem-460	114	11	.	.	PUNCT
eurjchem-460	115	1	reaction	reaction	NOUN
eurjchem-460	115	2	conditions	condition	NOUN
eurjchem-460	115	3	:	:	PUNCT
eurjchem-460	115	4	catalyst	catalyst	NOUN
eurjchem-460	115	5	concentration	concentration	NOUN
eurjchem-460	115	6	:	:	PUNCT
eurjchem-460	115	7	6	6	NUM
eurjchem-460	115	8	wt.%	wt.%	NOUN
eurjchem-460	115	9	(	(	PUNCT
eurjchem-460	115	10	zc‐1	zc‐1	PROPN
eurjchem-460	115	11	)	)	PUNCT
eurjchem-460	115	12	,	,	PUNCT
eurjchem-460	115	13	ethylene	ethylene	NOUN
eurjchem-460	115	14	glycol	glycol	NOUN
eurjchem-460	115	15	/	/	SYM
eurjchem-460	115	16	urea	urea	NOUN
eurjchem-460	115	17	mole	mole	NOUN
eurjchem-460	115	18	ratio	ratio	NOUN
eurjchem-460	115	19	:	:	PUNCT
eurjchem-460	115	20	1.5	1.5	NUM
eurjchem-460	115	21	,	,	PUNCT
eurjchem-460	115	22	duration	duration	NOUN
eurjchem-460	115	23	of	of	ADP
eurjchem-460	115	24	the	the	DET
eurjchem-460	115	25	reaction	reaction	NOUN
eurjchem-460	115	26	:	:	PUNCT
eurjchem-460	115	27	2	2	NUM
eurjchem-460	115	28	h.	h.	NOUN
eurjchem-460	115	29	3.4	3.4	NUM
eurjchem-460	115	30	.	.	PUNCT
eurjchem-460	116	1	effect	effect	NOUN
eurjchem-460	116	2	of	of	ADP
eurjchem-460	116	3	catalyst	catalyst	NOUN
eurjchem-460	116	4	concentration	concentration	NOUN
eurjchem-460	116	5	on	on	ADP
eurjchem-460	116	6	the	the	DET
eurjchem-460	116	7	reaction	reaction	NOUN
eurjchem-460	116	8	figure	figure	NOUN
eurjchem-460	116	9	5	5	NUM
eurjchem-460	116	10	presents	present	VERB
eurjchem-460	116	11	the	the	DET
eurjchem-460	116	12	effect	effect	NOUN
eurjchem-460	116	13	of	of	ADP
eurjchem-460	116	14	catalyst	catalyst	NOUN
eurjchem-460	116	15	concentration	concentration	NOUN
eurjchem-460	116	16	on	on	ADP
eurjchem-460	116	17	the	the	DET
eurjchem-460	116	18	cycloaddition	cycloaddition	NOUN
eurjchem-460	116	19	of	of	ADP
eurjchem-460	116	20	urea	urea	NOUN
eurjchem-460	116	21	with	with	ADP
eurjchem-460	116	22	eg	eg	NOUN
eurjchem-460	116	23	.	.	PUNCT
eurjchem-460	117	1	it	it	PRON
eurjchem-460	117	2	is	be	AUX
eurjchem-460	117	3	found	find	VERB
eurjchem-460	117	4	that	that	SCONJ
eurjchem-460	117	5	initial	initial	ADJ
eurjchem-460	117	6	increase	increase	NOUN
eurjchem-460	117	7	in	in	ADP
eurjchem-460	117	8	the	the	DET
eurjchem-460	117	9	catalyst	catalyst	NOUN
eurjchem-460	117	10	concentration	concentration	NOUN
eurjchem-460	117	11	leads	lead	VERB
eurjchem-460	117	12	to	to	PART
eurjchem-460	117	13	increase	increase	VERB
eurjchem-460	117	14	in	in	ADP
eurjchem-460	117	15	eg	eg	NOUN
eurjchem-460	117	16	conversion	conversion	NOUN
eurjchem-460	117	17	until	until	SCONJ
eurjchem-460	117	18	a	a	DET
eurjchem-460	117	19	limiting	limit	VERB
eurjchem-460	117	20	value	value	NOUN
eurjchem-460	117	21	is	be	AUX
eurjchem-460	117	22	reached	reach	VERB
eurjchem-460	117	23	.	.	PUNCT
eurjchem-460	118	1	a	a	DET
eurjchem-460	118	2	6	6	NUM
eurjchem-460	118	3	wt%	wt%	VERB
eurjchem-460	118	4	catalyst	catalyst	NOUN
eurjchem-460	118	5	is	be	AUX
eurjchem-460	118	6	found	find	VERB
eurjchem-460	118	7	to	to	PART
eurjchem-460	118	8	be	be	AUX
eurjchem-460	118	9	optimum	optimum	ADJ
eurjchem-460	118	10	eg	eg	NOUN
eurjchem-460	118	11	conversion	conversion	NOUN
eurjchem-460	118	12	with	with	ADP
eurjchem-460	118	13	an	an	DET
eurjchem-460	118	14	ec	ec	PROPN
eurjchem-460	118	15	yield	yield	NOUN
eurjchem-460	118	16	of	of	ADP
eurjchem-460	118	17	70	70	NUM
eurjchem-460	118	18	%	%	NOUN
eurjchem-460	118	19	.	.	PUNCT
eurjchem-460	119	1	238	238	NUM
eurjchem-460	119	2	bhadauria	bhadauria	NOUN
eurjchem-460	119	3	et	et	NOUN
eurjchem-460	119	4	al	al	PROPN
eurjchem-460	119	5	.	.	PUNCT
eurjchem-460	119	6	/	/	SYM
eurjchem-460	119	7	european	european	PROPN
eurjchem-460	119	8	journal	journal	PROPN
eurjchem-460	119	9	of	of	ADP
eurjchem-460	119	10	chemistry	chemistry	NOUN
eurjchem-460	119	11	3	3	NUM
eurjchem-460	119	12	(	(	PUNCT
eurjchem-460	119	13	2	2	NUM
eurjchem-460	119	14	)	)	PUNCT
eurjchem-460	119	15	(	(	PUNCT
eurjchem-460	119	16	2012	2012	NUM
eurjchem-460	119	17	)	)	PUNCT
eurjchem-460	119	18	235‐240	235‐240	NUM
eurjchem-460	119	19	table	table	NOUN
eurjchem-460	119	20	3	3	NUM
eurjchem-460	119	21	.	.	PUNCT
eurjchem-460	120	1	ir	ir	PROPN
eurjchem-460	120	2	observed	observe	VERB
eurjchem-460	120	3	bands	band	NOUN
eurjchem-460	120	4	(	(	PUNCT
eurjchem-460	120	5	cm‐1	cm‐1	NOUN
eurjchem-460	120	6	)	)	PUNCT
eurjchem-460	120	7	during	during	ADP
eurjchem-460	120	8	syntheses	synthesis	NOUN
eurjchem-460	120	9	of	of	ADP
eurjchem-460	120	10	ethylene	ethylene	NOUN
eurjchem-460	120	11	carbonate	carbonate	NOUN
eurjchem-460	120	12	.	.	PUNCT
eurjchem-460	121	1	sample	sample	NOUN
eurjchem-460	121	2	no	no	DET
eurjchem-460	121	3	stretching	stretch	VERB
eurjchem-460	121	4	ethylene	ethylene	NOUN
eurjchem-460	121	5	glycol	glycol	NOUN
eurjchem-460	121	6	urea	urea	NOUN
eurjchem-460	121	7	2‐hydroxyethyl	2‐hydroxyethyl	PROPN
eurjchem-460	121	8	carbamate	carbamate	PROPN
eurjchem-460	121	9	ethylene	ethylene	NOUN
eurjchem-460	121	10	carbonate	carbonate	NOUN
eurjchem-460	121	11	1	1	NUM
eurjchem-460	121	12	‐oh	‐oh	NOUN
eurjchem-460	121	13	3356	3356	NUM
eurjchem-460	121	14	‐	‐	ADP
eurjchem-460	121	15	3666	3666	NUM
eurjchem-460	121	16	‐	‐	ADV
eurjchem-460	121	17	2	2	NUM
eurjchem-460	121	18	c	c	NOUN
eurjchem-460	121	19	=	=	NOUN
eurjchem-460	121	20	o	o	NOUN
eurjchem-460	121	21	‐	‐	ADV
eurjchem-460	121	22	1625	1625	NUM
eurjchem-460	121	23	‐	‐	VERB
eurjchem-460	121	24	1800	1800	NUM
eurjchem-460	121	25	3	3	NUM
eurjchem-460	121	26	c‐o	c‐o	NOUN
eurjchem-460	121	27	‐	‐	VERB
eurjchem-460	121	28	‐	‐	ADV
eurjchem-460	121	29	‐	‐	VERB
eurjchem-460	121	30	1125	1125	NUM
eurjchem-460	121	31	figure	figure	NOUN
eurjchem-460	121	32	5	5	NUM
eurjchem-460	121	33	.	.	PUNCT
eurjchem-460	121	34	effect	effect	NOUN
eurjchem-460	121	35	of	of	ADP
eurjchem-460	121	36	catalyst	catalyst	NOUN
eurjchem-460	121	37	concentration	concentration	NOUN
eurjchem-460	121	38	on	on	ADP
eurjchem-460	121	39	the	the	DET
eurjchem-460	121	40	ec	ec	PROPN
eurjchem-460	121	41	yield	yield	NOUN
eurjchem-460	121	42	.	.	PUNCT
eurjchem-460	122	1	reaction	reaction	NOUN
eurjchem-460	122	2	conditions	condition	NOUN
eurjchem-460	122	3	:	:	PUNCT
eurjchem-460	122	4	temperature	temperature	NOUN
eurjchem-460	122	5	:	:	PUNCT
eurjchem-460	122	6	423	423	NUM
eurjchem-460	122	7	k	k	NOUN
eurjchem-460	122	8	,	,	PUNCT
eurjchem-460	122	9	ethylene	ethylene	NOUN
eurjchem-460	122	10	glycol	glycol	NOUN
eurjchem-460	122	11	/	/	SYM
eurjchem-460	122	12	urea	urea	NOUN
eurjchem-460	122	13	mole	mole	NOUN
eurjchem-460	122	14	ratio	ratio	NOUN
eurjchem-460	122	15	:	:	PUNCT
eurjchem-460	122	16	1.5	1.5	NUM
eurjchem-460	122	17	,	,	PUNCT
eurjchem-460	122	18	duration	duration	NOUN
eurjchem-460	122	19	of	of	ADP
eurjchem-460	122	20	the	the	DET
eurjchem-460	122	21	reaction	reaction	NOUN
eurjchem-460	122	22	:	:	PUNCT
eurjchem-460	122	23	2	2	NUM
eurjchem-460	122	24	h.	h.	NOUN
eurjchem-460	122	25	3.5	3.5	NUM
eurjchem-460	122	26	.	.	PUNCT
eurjchem-460	123	1	effect	effect	NOUN
eurjchem-460	123	2	of	of	ADP
eurjchem-460	123	3	molar	molar	ADJ
eurjchem-460	123	4	ratio	ratio	NOUN
eurjchem-460	123	5	on	on	ADP
eurjchem-460	123	6	the	the	DET
eurjchem-460	123	7	synthesis	synthesis	NOUN
eurjchem-460	123	8	of	of	ADP
eurjchem-460	123	9	ec	ec	PROPN
eurjchem-460	123	10	the	the	DET
eurjchem-460	123	11	effect	effect	NOUN
eurjchem-460	123	12	of	of	ADP
eurjchem-460	123	13	urea	urea	NOUN
eurjchem-460	123	14	/	/	SYM
eurjchem-460	123	15	eg	eg	NOUN
eurjchem-460	123	16	molar	molar	ADJ
eurjchem-460	123	17	ratio	ratio	NOUN
eurjchem-460	123	18	on	on	ADP
eurjchem-460	123	19	the	the	DET
eurjchem-460	123	20	eg	eg	PROPN
eurjchem-460	123	21	conversion	conversion	PROPN
eurjchem-460	123	22	and	and	CCONJ
eurjchem-460	123	23	ec	ec	PROPN
eurjchem-460	123	24	yield	yield	NOUN
eurjchem-460	123	25	is	be	AUX
eurjchem-460	123	26	depicted	depict	VERB
eurjchem-460	123	27	in	in	ADP
eurjchem-460	123	28	figure	figure	NOUN
eurjchem-460	123	29	6	6	NUM
eurjchem-460	123	30	.	.	PUNCT
eurjchem-460	124	1	a	a	DET
eurjchem-460	124	2	urea	urea	NOUN
eurjchem-460	124	3	/	/	SYM
eurjchem-460	124	4	eg	eg	NOUN
eurjchem-460	124	5	molar	molar	ADJ
eurjchem-460	124	6	ratio	ratio	NOUN
eurjchem-460	124	7	of	of	ADP
eurjchem-460	124	8	1:1.5	1:1.5	NUM
eurjchem-460	124	9	was	be	AUX
eurjchem-460	124	10	found	find	VERB
eurjchem-460	124	11	to	to	PART
eurjchem-460	124	12	be	be	AUX
eurjchem-460	124	13	optimum	optimum	ADJ
eurjchem-460	124	14	.	.	PUNCT
eurjchem-460	125	1	further	furth	ADJ
eurjchem-460	125	2	increase	increase	NOUN
eurjchem-460	125	3	in	in	ADP
eurjchem-460	125	4	the	the	DET
eurjchem-460	125	5	ratio	ratio	NOUN
eurjchem-460	125	6	led	lead	VERB
eurjchem-460	125	7	to	to	ADP
eurjchem-460	125	8	decreased	decrease	VERB
eurjchem-460	125	9	conversion	conversion	NOUN
eurjchem-460	125	10	due	due	ADP
eurjchem-460	125	11	to	to	ADP
eurjchem-460	125	12	insufficient	insufficient	ADJ
eurjchem-460	125	13	availability	availability	NOUN
eurjchem-460	125	14	of	of	ADP
eurjchem-460	125	15	urea	urea	NOUN
eurjchem-460	125	16	.	.	PUNCT
eurjchem-460	126	1	figure	figure	NOUN
eurjchem-460	126	2	6	6	NUM
eurjchem-460	126	3	.	.	PUNCT
eurjchem-460	127	1	effect	effect	NOUN
eurjchem-460	127	2	of	of	ADP
eurjchem-460	127	3	molar	molar	ADJ
eurjchem-460	127	4	ratio	ratio	NOUN
eurjchem-460	127	5	urea	urea	PROPN
eurjchem-460	127	6	/	/	SYM
eurjchem-460	127	7	ec	ec	PROPN
eurjchem-460	127	8	yield	yield	NOUN
eurjchem-460	127	9	.	.	PUNCT
eurjchem-460	128	1	reaction	reaction	NOUN
eurjchem-460	128	2	conditions	condition	NOUN
eurjchem-460	128	3	:	:	PUNCT
eurjchem-460	128	4	catalyst	catalyst	NOUN
eurjchem-460	128	5	:	:	PUNCT
eurjchem-460	129	1	zc‐1	zc‐1	NOUN
eurjchem-460	129	2	,	,	PUNCT
eurjchem-460	129	3	temperature	temperature	NOUN
eurjchem-460	129	4	:	:	PUNCT
eurjchem-460	129	5	423	423	NUM
eurjchem-460	129	6	k	k	NOUN
eurjchem-460	129	7	,	,	PUNCT
eurjchem-460	129	8	duration	duration	NOUN
eurjchem-460	129	9	of	of	ADP
eurjchem-460	129	10	the	the	DET
eurjchem-460	129	11	reaction	reaction	NOUN
eurjchem-460	129	12	:	:	PUNCT
eurjchem-460	129	13	2	2	NUM
eurjchem-460	129	14	h.	h.	NOUN
eurjchem-460	129	15	3.6	3.6	NUM
eurjchem-460	129	16	.	.	PUNCT
eurjchem-460	130	1	effect	effect	NOUN
eurjchem-460	130	2	of	of	ADP
eurjchem-460	130	3	time	time	NOUN
eurjchem-460	130	4	on	on	ADP
eurjchem-460	130	5	stream	stream	NOUN
eurjchem-460	130	6	on	on	ADP
eurjchem-460	130	7	the	the	DET
eurjchem-460	130	8	synthesis	synthesis	NOUN
eurjchem-460	130	9	of	of	ADP
eurjchem-460	130	10	ec	ec	PROPN
eurjchem-460	130	11	to	to	PART
eurjchem-460	130	12	investigate	investigate	VERB
eurjchem-460	130	13	the	the	DET
eurjchem-460	130	14	catalytic	catalytic	ADJ
eurjchem-460	130	15	activity	activity	NOUN
eurjchem-460	130	16	at	at	ADP
eurjchem-460	130	17	different	different	ADJ
eurjchem-460	130	18	time	time	NOUN
eurjchem-460	130	19	,	,	PUNCT
eurjchem-460	130	20	more	more	ADJ
eurjchem-460	130	21	experiments	experiment	NOUN
eurjchem-460	130	22	were	be	AUX
eurjchem-460	130	23	conducted	conduct	VERB
eurjchem-460	130	24	in	in	ADP
eurjchem-460	130	25	the	the	DET
eurjchem-460	130	26	range	range	NOUN
eurjchem-460	130	27	of	of	ADP
eurjchem-460	130	28	1‐4	1‐4	PROPN
eurjchem-460	130	29	h.	h.	NOUN
eurjchem-460	130	30	the	the	DET
eurjchem-460	130	31	result	result	NOUN
eurjchem-460	130	32	presented	present	VERB
eurjchem-460	130	33	graphically	graphically	ADV
eurjchem-460	130	34	in	in	ADP
eurjchem-460	130	35	figure	figure	NOUN
eurjchem-460	130	36	7	7	NUM
eurjchem-460	130	37	.	.	PUNCT
eurjchem-460	131	1	it	it	PRON
eurjchem-460	131	2	can	can	AUX
eurjchem-460	131	3	be	be	AUX
eurjchem-460	131	4	seen	see	VERB
eurjchem-460	131	5	that	that	SCONJ
eurjchem-460	131	6	the	the	DET
eurjchem-460	131	7	yield	yield	NOUN
eurjchem-460	131	8	of	of	ADP
eurjchem-460	131	9	ec	ec	PROPN
eurjchem-460	131	10	increased	increase	VERB
eurjchem-460	131	11	with	with	ADP
eurjchem-460	131	12	the	the	DET
eurjchem-460	131	13	reaction	reaction	NOUN
eurjchem-460	131	14	time	time	NOUN
eurjchem-460	131	15	,	,	PUNCT
eurjchem-460	131	16	but	but	CCONJ
eurjchem-460	131	17	the	the	DET
eurjchem-460	131	18	change	change	NOUN
eurjchem-460	131	19	was	be	AUX
eurjchem-460	131	20	not	not	PART
eurjchem-460	131	21	significant	significant	ADJ
eurjchem-460	131	22	after	after	ADP
eurjchem-460	131	23	about	about	ADV
eurjchem-460	131	24	3	3	NUM
eurjchem-460	131	25	h.	h.	NOUN
eurjchem-460	132	1	so	so	ADV
eurjchem-460	132	2	,	,	PUNCT
eurjchem-460	132	3	the	the	DET
eurjchem-460	132	4	optimum	optimum	ADJ
eurjchem-460	132	5	reaction	reaction	NOUN
eurjchem-460	132	6	time	time	NOUN
eurjchem-460	132	7	for	for	ADP
eurjchem-460	132	8	the	the	DET
eurjchem-460	132	9	reaction	reaction	NOUN
eurjchem-460	132	10	is	be	AUX
eurjchem-460	132	11	3	3	NUM
eurjchem-460	132	12	h.	h.	NOUN
eurjchem-460	132	13	in	in	ADP
eurjchem-460	132	14	these	these	DET
eurjchem-460	132	15	experiments	experiment	NOUN
eurjchem-460	132	16	recovered	recover	VERB
eurjchem-460	132	17	catalyst	catalyst	NOUN
eurjchem-460	132	18	were	be	AUX
eurjchem-460	132	19	used	use	VERB
eurjchem-460	132	20	.	.	PUNCT
eurjchem-460	133	1	therefore	therefore	ADV
eurjchem-460	133	2	,	,	PUNCT
eurjchem-460	133	3	these	these	DET
eurjchem-460	133	4	experiments	experiment	NOUN
eurjchem-460	133	5	demonstrate	demonstrate	VERB
eurjchem-460	133	6	the	the	DET
eurjchem-460	133	7	reusability	reusability	NOUN
eurjchem-460	133	8	of	of	ADP
eurjchem-460	133	9	the	the	DET
eurjchem-460	133	10	recovered	recover	VERB
eurjchem-460	133	11	catalysts	catalyst	NOUN
eurjchem-460	133	12	as	as	ADV
eurjchem-460	133	13	well	well	ADV
eurjchem-460	133	14	.	.	PUNCT
eurjchem-460	134	1	4	4	X
eurjchem-460	134	2	.	.	X
eurjchem-460	134	3	mechanism	mechanism	NOUN
eurjchem-460	134	4	the	the	DET
eurjchem-460	134	5	mechanism	mechanism	NOUN
eurjchem-460	134	6	of	of	ADP
eurjchem-460	134	7	the	the	DET
eurjchem-460	134	8	reaction	reaction	NOUN
eurjchem-460	134	9	being	be	AUX
eurjchem-460	134	10	proposed	propose	VERB
eurjchem-460	134	11	is	be	AUX
eurjchem-460	134	12	based	base	VERB
eurjchem-460	134	13	on	on	ADP
eurjchem-460	134	14	product	product	NOUN
eurjchem-460	134	15	analysis	analysis	NOUN
eurjchem-460	134	16	and	and	CCONJ
eurjchem-460	134	17	infrared	infrared	ADJ
eurjchem-460	134	18	record	record	NOUN
eurjchem-460	134	19	of	of	ADP
eurjchem-460	134	20	the	the	DET
eurjchem-460	134	21	reactants	reactant	NOUN
eurjchem-460	134	22	,	,	PUNCT
eurjchem-460	134	23	product	product	NOUN
eurjchem-460	134	24	and	and	CCONJ
eurjchem-460	134	25	reaction	reaction	NOUN
eurjchem-460	134	26	mixture	mixture	NOUN
eurjchem-460	134	27	at	at	ADP
eurjchem-460	134	28	different	different	ADJ
eurjchem-460	134	29	interval	interval	NOUN
eurjchem-460	134	30	of	of	ADP
eurjchem-460	134	31	time	time	NOUN
eurjchem-460	134	32	on	on	ADP
eurjchem-460	134	33	a	a	DET
eurjchem-460	134	34	shimadzu	shimadzu	ADJ
eurjchem-460	134	35	ir	ir	PROPN
eurjchem-460	134	36	spectrometer	spectrometer	NOUN
eurjchem-460	134	37	460	460	NUM
eurjchem-460	134	38	.	.	PUNCT
eurjchem-460	135	1	the	the	DET
eurjchem-460	135	2	bands	band	NOUN
eurjchem-460	135	3	observed	observe	VERB
eurjchem-460	135	4	in	in	ADP
eurjchem-460	135	5	the	the	DET
eurjchem-460	135	6	range	range	NOUN
eurjchem-460	135	7	3000‐	3000‐	NUM
eurjchem-460	135	8	4000	4000	NUM
eurjchem-460	135	9	cm‐1	cm‐1	NOUN
eurjchem-460	135	10	and	and	CCONJ
eurjchem-460	135	11	1600‐1900	1600‐1900	NUM
eurjchem-460	135	12	cm‐1	cm‐1	NOUN
eurjchem-460	135	13	are	be	AUX
eurjchem-460	135	14	listed	list	VERB
eurjchem-460	135	15	in	in	ADP
eurjchem-460	135	16	table	table	NOUN
eurjchem-460	135	17	3	3	NUM
eurjchem-460	135	18	.	.	PUNCT
eurjchem-460	136	1	the	the	DET
eurjchem-460	136	2	oh	oh	INTJ
eurjchem-460	136	3	stretching	stretch	VERB
eurjchem-460	136	4	mode	mode	NOUN
eurjchem-460	136	5	of	of	ADP
eurjchem-460	136	6	ethylene	ethylene	NOUN
eurjchem-460	136	7	glycol	glycol	NOUN
eurjchem-460	136	8	appeared	appear	VERB
eurjchem-460	136	9	at	at	ADP
eurjchem-460	136	10	3356	3356	NUM
eurjchem-460	136	11	cm‐1	cm‐1	NOUN
eurjchem-460	136	12	.	.	PUNCT
eurjchem-460	137	1	in	in	ADP
eurjchem-460	137	2	the	the	DET
eurjchem-460	137	3	reaction	reaction	NOUN
eurjchem-460	137	4	mixture	mixture	NOUN
eurjchem-460	137	5	a	a	DET
eurjchem-460	137	6	broad	broad	ADJ
eurjchem-460	137	7	band	band	NOUN
eurjchem-460	137	8	centered	center	VERB
eurjchem-460	137	9	around	around	ADP
eurjchem-460	137	10	3666	3666	NUM
eurjchem-460	137	11	cm‐1	cm‐1	NOUN
eurjchem-460	137	12	appeared	appear	VERB
eurjchem-460	137	13	which	which	PRON
eurjchem-460	137	14	loses	lose	VERB
eurjchem-460	137	15	its	its	PRON
eurjchem-460	137	16	intensity	intensity	NOUN
eurjchem-460	137	17	with	with	ADP
eurjchem-460	137	18	time	time	NOUN
eurjchem-460	137	19	.	.	PUNCT
eurjchem-460	138	1	figure	figure	VERB
eurjchem-460	138	2	7	7	NUM
eurjchem-460	138	3	.	.	PUNCT
eurjchem-460	138	4	effect	effect	NOUN
eurjchem-460	138	5	of	of	ADP
eurjchem-460	138	6	reaction	reaction	NOUN
eurjchem-460	138	7	time	time	NOUN
eurjchem-460	138	8	on	on	ADP
eurjchem-460	138	9	ec	ec	PROPN
eurjchem-460	138	10	yield	yield	NOUN
eurjchem-460	138	11	.	.	PUNCT
eurjchem-460	139	1	reaction	reaction	NOUN
eurjchem-460	139	2	conditions	condition	NOUN
eurjchem-460	139	3	:	:	PUNCT
eurjchem-460	139	4	temperature	temperature	NOUN
eurjchem-460	139	5	:	:	PUNCT
eurjchem-460	139	6	423	423	NUM
eurjchem-460	139	7	k	k	NOUN
eurjchem-460	139	8	,	,	PUNCT
eurjchem-460	139	9	catalyst	catalyst	NOUN
eurjchem-460	139	10	concentration	concentration	NOUN
eurjchem-460	139	11	:	:	PUNCT
eurjchem-460	139	12	6	6	NUM
eurjchem-460	139	13	wt	wt	NUM
eurjchem-460	139	14	%	%	NOUN
eurjchem-460	139	15	ethylene	ethylene	NOUN
eurjchem-460	139	16	glycol	glycol	NOUN
eurjchem-460	139	17	/	/	SYM
eurjchem-460	139	18	urea	urea	NOUN
eurjchem-460	139	19	mole	mole	NOUN
eurjchem-460	139	20	ratio	ratio	NOUN
eurjchem-460	139	21	:	:	PUNCT
eurjchem-460	139	22	1.5	1.5	NUM
eurjchem-460	139	23	.	.	PUNCT
eurjchem-460	140	1	this	this	DET
eurjchem-460	140	2	band	band	NOUN
eurjchem-460	140	3	has	have	AUX
eurjchem-460	140	4	been	be	AUX
eurjchem-460	140	5	assigned	assign	VERB
eurjchem-460	140	6	to	to	ADP
eurjchem-460	140	7	oh	oh	INTJ
eurjchem-460	140	8	stretching	stretch	VERB
eurjchem-460	140	9	band	band	NOUN
eurjchem-460	140	10	of	of	ADP
eurjchem-460	140	11	2‐	2‐	NUM
eurjchem-460	140	12	hydroxyethyl	hydroxyethyl	NOUN
eurjchem-460	140	13	carbamate	carbamate	NOUN
eurjchem-460	140	14	.	.	PUNCT
eurjchem-460	141	1	similarly	similarly	ADV
eurjchem-460	141	2	the	the	DET
eurjchem-460	141	3	c	c	NOUN
eurjchem-460	141	4	=	=	NOUN
eurjchem-460	141	5	o	o	NOUN
eurjchem-460	141	6	stretching	stretch	VERB
eurjchem-460	141	7	band	band	NOUN
eurjchem-460	141	8	of	of	ADP
eurjchem-460	141	9	urea	urea	NOUN
eurjchem-460	141	10	appears	appear	VERB
eurjchem-460	141	11	at	at	ADP
eurjchem-460	141	12	1625	1625	NUM
eurjchem-460	141	13	cm‐1	cm‐1	NOUN
eurjchem-460	141	14	.	.	PUNCT
eurjchem-460	142	1	ir	ir	PROPN
eurjchem-460	142	2	spectrum	spectrum	NOUN
eurjchem-460	142	3	of	of	ADP
eurjchem-460	142	4	the	the	DET
eurjchem-460	142	5	reaction	reaction	NOUN
eurjchem-460	142	6	mixture	mixture	NOUN
eurjchem-460	142	7	showed	show	VERB
eurjchem-460	142	8	a	a	DET
eurjchem-460	142	9	band	band	NOUN
eurjchem-460	142	10	at	at	ADP
eurjchem-460	142	11	1800	1800	NUM
eurjchem-460	142	12	cm‐1	cm‐1	NOUN
eurjchem-460	142	13	and	and	CCONJ
eurjchem-460	142	14	has	have	AUX
eurjchem-460	142	15	been	be	AUX
eurjchem-460	142	16	assigned	assign	VERB
eurjchem-460	142	17	to	to	ADP
eurjchem-460	142	18	c	c	NOUN
eurjchem-460	142	19	=	=	X
eurjchem-460	142	20	o	o	NOUN
eurjchem-460	142	21	stretching	stretch	VERB
eurjchem-460	142	22	mode	mode	NOUN
eurjchem-460	142	23	of	of	ADP
eurjchem-460	142	24	ethylene	ethylene	NOUN
eurjchem-460	142	25	carbonate	carbonate	NOUN
eurjchem-460	142	26	.	.	PUNCT
eurjchem-460	143	1	a	a	DET
eurjchem-460	143	2	shoulder	shoulder	NOUN
eurjchem-460	143	3	appeared	appear	VERB
eurjchem-460	143	4	at	at	ADP
eurjchem-460	143	5	1850	1850	NUM
eurjchem-460	143	6	cm‐1	cm‐1	NOUN
eurjchem-460	143	7	is	be	AUX
eurjchem-460	143	8	assigned	assign	VERB
eurjchem-460	143	9	to	to	ADP
eurjchem-460	143	10	c	c	NOUN
eurjchem-460	143	11	=	=	X
eurjchem-460	143	12	o	o	NOUN
eurjchem-460	143	13	stretching	stretch	VERB
eurjchem-460	143	14	mode	mode	NOUN
eurjchem-460	143	15	of	of	ADP
eurjchem-460	143	16	2‐hydroxyethyl	2‐hydroxyethyl	PROPN
eurjchem-460	143	17	carbamate	carbamate	PROPN
eurjchem-460	143	18	.	.	PUNCT
eurjchem-460	144	1	a	a	DET
eurjchem-460	144	2	plot	plot	NOUN
eurjchem-460	144	3	of	of	ADP
eurjchem-460	144	4	ethylene	ethylene	NOUN
eurjchem-460	144	5	carbonate	carbonate	NOUN
eurjchem-460	144	6	yield	yield	NOUN
eurjchem-460	144	7	and	and	CCONJ
eurjchem-460	144	8	concentration	concentration	NOUN
eurjchem-460	144	9	of	of	ADP
eurjchem-460	144	10	ethylene	ethylene	NOUN
eurjchem-460	144	11	glycol	glycol	NOUN
eurjchem-460	144	12	with	with	ADP
eurjchem-460	144	13	time	time	NOUN
eurjchem-460	144	14	is	be	AUX
eurjchem-460	144	15	shown	show	VERB
eurjchem-460	144	16	in	in	ADP
eurjchem-460	144	17	figure	figure	NOUN
eurjchem-460	144	18	7	7	NUM
eurjchem-460	144	19	.	.	PUNCT
eurjchem-460	145	1	the	the	DET
eurjchem-460	145	2	yield	yield	NOUN
eurjchem-460	145	3	increases	increase	VERB
eurjchem-460	145	4	with	with	ADP
eurjchem-460	145	5	time	time	NOUN
eurjchem-460	145	6	and	and	CCONJ
eurjchem-460	145	7	the	the	DET
eurjchem-460	145	8	concentration	concentration	NOUN
eurjchem-460	145	9	of	of	ADP
eurjchem-460	145	10	ethylene	ethylene	NOUN
eurjchem-460	145	11	glycol	glycol	NOUN
eurjchem-460	145	12	decrease	decrease	NOUN
eurjchem-460	145	13	with	with	ADP
eurjchem-460	145	14	time	time	NOUN
eurjchem-460	145	15	.	.	PUNCT
eurjchem-460	146	1	we	we	PRON
eurjchem-460	146	2	could	could	AUX
eurjchem-460	146	3	not	not	PART
eurjchem-460	146	4	observe	observe	VERB
eurjchem-460	146	5	any	any	DET
eurjchem-460	146	6	separate	separate	ADJ
eurjchem-460	146	7	peak	peak	NOUN
eurjchem-460	146	8	in	in	ADP
eurjchem-460	146	9	our	our	PRON
eurjchem-460	146	10	gc	gc	PROPN
eurjchem-460	146	11	analysis	analysis	NOUN
eurjchem-460	146	12	for	for	ADP
eurjchem-460	146	13	2‐hyroxyethyl	2‐hyroxyethyl	NUM
eurjchem-460	146	14	carbonate	carbonate	NOUN
eurjchem-460	146	15	.	.	PUNCT
eurjchem-460	147	1	idea	idea	NOUN
eurjchem-460	147	2	of	of	ADP
eurjchem-460	147	3	it	it	PRON
eurjchem-460	147	4	concentration	concentration	NOUN
eurjchem-460	147	5	was	be	AUX
eurjchem-460	147	6	therefore	therefore	ADV
eurjchem-460	147	7	made	make	VERB
eurjchem-460	147	8	from	from	ADP
eurjchem-460	147	9	the	the	DET
eurjchem-460	147	10	time	time	NOUN
eurjchem-460	147	11	record	record	NOUN
eurjchem-460	147	12	of	of	ADP
eurjchem-460	147	13	ir	ir	PROPN
eurjchem-460	147	14	intensity	intensity	NOUN
eurjchem-460	147	15	of	of	ADP
eurjchem-460	147	16	oh	oh	INTJ
eurjchem-460	147	17	stretching	stretch	VERB
eurjchem-460	147	18	mode	mode	NOUN
eurjchem-460	147	19	of	of	ADP
eurjchem-460	147	20	2‐hydroxyethyl	2‐hydroxyethyl	PROPN
eurjchem-460	147	21	carbamate	carbamate	PROPN
eurjchem-460	147	22	.	.	PUNCT
eurjchem-460	148	1	the	the	DET
eurjchem-460	148	2	records	record	NOUN
eurjchem-460	148	3	show	show	VERB
eurjchem-460	148	4	decrease	decrease	NOUN
eurjchem-460	148	5	in	in	ADP
eurjchem-460	148	6	the	the	DET
eurjchem-460	148	7	intensity	intensity	NOUN
eurjchem-460	148	8	of	of	ADP
eurjchem-460	148	9	this	this	DET
eurjchem-460	148	10	peak	peak	NOUN
eurjchem-460	148	11	.	.	PUNCT
eurjchem-460	149	1	it	it	PRON
eurjchem-460	149	2	seems	seem	VERB
eurjchem-460	149	3	2‐hydroxyethyl	2‐hydroxyethyl	PROPN
eurjchem-460	149	4	carbamate	carbamate	PROPN
eurjchem-460	149	5	is	be	AUX
eurjchem-460	149	6	rapidly	rapidly	ADV
eurjchem-460	149	7	formed	form	VERB
eurjchem-460	149	8	in	in	ADP
eurjchem-460	149	9	the	the	DET
eurjchem-460	149	10	beginning	beginning	NOUN
eurjchem-460	149	11	and	and	CCONJ
eurjchem-460	149	12	then	then	ADV
eurjchem-460	149	13	its	its	PRON
eurjchem-460	149	14	concentration	concentration	NOUN
eurjchem-460	149	15	decrease	decrease	NOUN
eurjchem-460	149	16	with	with	ADP
eurjchem-460	149	17	time	time	NOUN
eurjchem-460	149	18	.	.	PUNCT
eurjchem-460	150	1	it	it	PRON
eurjchem-460	150	2	seems	seem	VERB
eurjchem-460	150	3	urea	urea	NOUN
eurjchem-460	150	4	is	be	AUX
eurjchem-460	150	5	adsorbed	adsorb	VERB
eurjchem-460	150	6	on	on	ADP
eurjchem-460	150	7	the	the	DET
eurjchem-460	150	8	acidic	acidic	ADJ
eurjchem-460	150	9	catalyst	catalyst	NOUN
eurjchem-460	150	10	and	and	CCONJ
eurjchem-460	150	11	eg	eg	NOUN
eurjchem-460	150	12	remains	remain	VERB
eurjchem-460	150	13	in	in	ADP
eurjchem-460	150	14	gas	gas	NOUN
eurjchem-460	150	15	phase	phase	NOUN
eurjchem-460	150	16	.	.	PUNCT
eurjchem-460	151	1	due	due	ADP
eurjchem-460	151	2	to	to	ADP
eurjchem-460	151	3	adsorption	adsorption	NOUN
eurjchem-460	151	4	the	the	DET
eurjchem-460	151	5	ammine	ammine	NOUN
eurjchem-460	151	6	bond	bond	NOUN
eurjchem-460	151	7	is	be	AUX
eurjchem-460	151	8	weakened	weaken	VERB
eurjchem-460	151	9	,	,	PUNCT
eurjchem-460	151	10	reacts	react	VERB
eurjchem-460	151	11	with	with	ADP
eurjchem-460	151	12	eg	eg	NOUN
eurjchem-460	151	13	and	and	CCONJ
eurjchem-460	151	14	removed	remove	VERB
eurjchem-460	151	15	as	as	ADP
eurjchem-460	151	16	nh3	nh3	NOUN
eurjchem-460	151	17	giving	give	VERB
eurjchem-460	151	18	rise	rise	NOUN
eurjchem-460	151	19	to	to	ADP
eurjchem-460	151	20	the	the	DET
eurjchem-460	151	21	adsorbed	adsorb	VERB
eurjchem-460	151	22	specie	specie	PROPN
eurjchem-460	151	23	2‐hydroxyethyl	2‐hydroxyethyl	PROPN
eurjchem-460	151	24	carbamate	carbamate	PROPN
eurjchem-460	151	25	.	.	PUNCT
eurjchem-460	152	1	2‐hydroxyethyl	2‐hydroxyethyl	PROPN
eurjchem-460	152	2	carbamate	carbamate	PROPN
eurjchem-460	152	3	is	be	AUX
eurjchem-460	152	4	adsorbed	adsorb	VERB
eurjchem-460	152	5	on	on	ADP
eurjchem-460	152	6	catalyst	catalyst	NOUN
eurjchem-460	152	7	through	through	ADP
eurjchem-460	152	8	nitrogen	nitrogen	NOUN
eurjchem-460	152	9	atom	atom	NOUN
eurjchem-460	152	10	as	as	ADV
eurjchem-460	152	11	well	well	ADV
eurjchem-460	152	12	as	as	ADP
eurjchem-460	152	13	under‐	under‐	NOUN
eurjchem-460	152	14	goes	go	VERB
eurjchem-460	152	15	a	a	DET
eurjchem-460	152	16	conformational	conformational	ADJ
eurjchem-460	152	17	change	change	NOUN
eurjchem-460	152	18	to	to	ADP
eurjchem-460	152	19	the	the	DET
eurjchem-460	152	20	rotation	rotation	NOUN
eurjchem-460	152	21	about	about	ADP
eurjchem-460	152	22	c‐o	c‐o	NOUN
eurjchem-460	152	23	bond	bond	NOUN
eurjchem-460	152	24	to	to	PART
eurjchem-460	152	25	facilitate	facilitate	VERB
eurjchem-460	152	26	removal	removal	NOUN
eurjchem-460	152	27	of	of	ADP
eurjchem-460	152	28	second	second	ADJ
eurjchem-460	152	29	nh3	nh3	NOUN
eurjchem-460	152	30	molecule	molecule	NOUN
eurjchem-460	152	31	and	and	CCONJ
eurjchem-460	152	32	formation	formation	NOUN
eurjchem-460	152	33	of	of	ADP
eurjchem-460	152	34	the	the	DET
eurjchem-460	152	35	ethylene	ethylene	NOUN
eurjchem-460	152	36	carbonate	carbonate	NOUN
eurjchem-460	152	37	.	.	PUNCT
eurjchem-460	153	1	further	further	ADJ
eurjchem-460	153	2	clue	clue	NOUN
eurjchem-460	153	3	to	to	ADP
eurjchem-460	153	4	the	the	DET
eurjchem-460	153	5	reaction	reaction	NOUN
eurjchem-460	153	6	mechanism	mechanism	NOUN
eurjchem-460	153	7	was	be	AUX
eurjchem-460	153	8	obtained	obtain	VERB
eurjchem-460	153	9	by	by	ADP
eurjchem-460	153	10	modeling	modeling	NOUN
eurjchem-460	153	11	of	of	ADP
eurjchem-460	153	12	the	the	DET
eurjchem-460	153	13	transition	transition	NOUN
eurjchem-460	153	14	state	state	NOUN
eurjchem-460	153	15	for	for	ADP
eurjchem-460	153	16	the	the	DET
eurjchem-460	153	17	reaction	reaction	NOUN
eurjchem-460	153	18	under	under	ADP
eurjchem-460	153	19	qst2	qst2	ADJ
eurjchem-460	153	20	option	option	NOUN
eurjchem-460	153	21	of	of	ADP
eurjchem-460	153	22	the	the	DET
eurjchem-460	153	23	gaussian‐09	gaussian‐09	PROPN
eurjchem-460	153	24	suite	suite	NOUN
eurjchem-460	153	25	[	[	X
eurjchem-460	153	26	42	42	NUM
eurjchem-460	153	27	]	]	PUNCT
eurjchem-460	153	28	.	.	PUNCT
eurjchem-460	154	1	details	detail	NOUN
eurjchem-460	154	2	of	of	ADP
eurjchem-460	154	3	qst2	qst2	ADJ
eurjchem-460	154	4	option	option	NOUN
eurjchem-460	154	5	can	can	AUX
eurjchem-460	154	6	be	be	AUX
eurjchem-460	154	7	found	find	VERB
eurjchem-460	154	8	elsewhere	elsewhere	ADV
eurjchem-460	154	9	[	[	X
eurjchem-460	154	10	43	43	NUM
eurjchem-460	154	11	]	]	PUNCT
eurjchem-460	154	12	.	.	PUNCT
eurjchem-460	155	1	bhadauria	bhadauria	NOUN
eurjchem-460	155	2	et	et	PROPN
eurjchem-460	155	3	al	al	PROPN
eurjchem-460	155	4	.	.	PUNCT
eurjchem-460	155	5	/	/	SYM
eurjchem-460	155	6	european	european	PROPN
eurjchem-460	155	7	journal	journal	PROPN
eurjchem-460	155	8	of	of	ADP
eurjchem-460	155	9	chemistry	chemistry	NOUN
eurjchem-460	155	10	3	3	NUM
eurjchem-460	155	11	(	(	PUNCT
eurjchem-460	155	12	2	2	NUM
eurjchem-460	155	13	)	)	PUNCT
eurjchem-460	155	14	(	(	PUNCT
eurjchem-460	155	15	2012	2012	NUM
eurjchem-460	155	16	)	)	PUNCT
eurjchem-460	155	17	235‐240	235‐240	NUM
eurjchem-460	155	18	239	239	NUM
eurjchem-460	155	19	scheme	scheme	NOUN
eurjchem-460	155	20	1	1	NUM
eurjchem-460	155	21	the	the	DET
eurjchem-460	155	22	dft	dft	PROPN
eurjchem-460	155	23	molecular	molecular	ADJ
eurjchem-460	155	24	orbital	orbital	ADJ
eurjchem-460	155	25	calculations	calculation	NOUN
eurjchem-460	155	26	were	be	AUX
eurjchem-460	155	27	performed	perform	VERB
eurjchem-460	155	28	using	use	VERB
eurjchem-460	155	29	becke	becke	NOUN
eurjchem-460	155	30	’s	’s	PART
eurjchem-460	155	31	three	three	NUM
eurjchem-460	155	32	parameter	parameter	NOUN
eurjchem-460	155	33	hybrid	hybrid	NOUN
eurjchem-460	155	34	method	method	NOUN
eurjchem-460	155	35	with	with	ADP
eurjchem-460	155	36	the	the	DET
eurjchem-460	155	37	lee	lee	PROPN
eurjchem-460	155	38	,	,	PUNCT
eurjchem-460	155	39	yang	yang	PROPN
eurjchem-460	155	40	and	and	CCONJ
eurjchem-460	155	41	parr	parr	X
eurjchem-460	155	42	(	(	PUNCT
eurjchem-460	155	43	b3lyp	b3lyp	SYM
eurjchem-460	155	44	)	)	PUNCT
eurjchem-460	155	45	gradient	gradient	NOUN
eurjchem-460	155	46	corrected	correct	VERB
eurjchem-460	155	47	correlation	correlation	NOUN
eurjchem-460	155	48	function	function	NOUN
eurjchem-460	156	1	[	[	X
eurjchem-460	156	2	44	44	NUM
eurjchem-460	156	3	‐45	‐45	NOUN
eurjchem-460	156	4	]	]	X
eurjchem-460	156	5	.	.	PUNCT
eurjchem-460	157	1	an	an	DET
eurjchem-460	157	2	inspection	inspection	NOUN
eurjchem-460	157	3	of	of	ADP
eurjchem-460	157	4	table	table	NOUN
eurjchem-460	157	5	2	2	NUM
eurjchem-460	157	6	reveals	reveal	VERB
eurjchem-460	157	7	that	that	SCONJ
eurjchem-460	157	8	in	in	ADP
eurjchem-460	157	9	the	the	DET
eurjchem-460	157	10	present	present	ADJ
eurjchem-460	157	11	catalyst	catalyst	NOUN
eurjchem-460	157	12	system	system	NOUN
eurjchem-460	157	13	performance	performance	NOUN
eurjchem-460	157	14	of	of	ADP
eurjchem-460	157	15	the	the	DET
eurjchem-460	157	16	catalysts	catalyst	NOUN
eurjchem-460	157	17	increased	increase	VERB
eurjchem-460	157	18	with	with	ADP
eurjchem-460	157	19	increasing	increase	VERB
eurjchem-460	157	20	amount	amount	NOUN
eurjchem-460	157	21	of	of	ADP
eurjchem-460	157	22	zno	zno	NOUN
eurjchem-460	157	23	in	in	ADP
eurjchem-460	157	24	the	the	DET
eurjchem-460	157	25	catalyst	catalyst	NOUN
eurjchem-460	157	26	and	and	CCONJ
eurjchem-460	157	27	zc‐1	zc‐1	X
eurjchem-460	157	28	with	with	ADP
eurjchem-460	157	29	maximum	maximum	ADJ
eurjchem-460	157	30	amount	amount	NOUN
eurjchem-460	157	31	of	of	ADP
eurjchem-460	157	32	zno	zno	NOUN
eurjchem-460	157	33	came	come	VERB
eurjchem-460	157	34	out	out	ADP
eurjchem-460	157	35	to	to	PART
eurjchem-460	157	36	be	be	AUX
eurjchem-460	157	37	the	the	DET
eurjchem-460	157	38	best	good	ADJ
eurjchem-460	157	39	catalyst	catalyst	NOUN
eurjchem-460	157	40	.	.	PUNCT
eurjchem-460	158	1	li	li	PROPN
eurjchem-460	158	2	et	et	PROPN
eurjchem-460	158	3	al	al	PROPN
eurjchem-460	158	4	.	.	PUNCT
eurjchem-460	159	1	[	[	X
eurjchem-460	159	2	34	34	NUM
eurjchem-460	159	3	]	]	PUNCT
eurjchem-460	159	4	have	have	VERB
eurjchem-460	159	5	studies	study	NOUN
eurjchem-460	159	6	a	a	DET
eurjchem-460	159	7	series	series	NOUN
eurjchem-460	159	8	of	of	ADP
eurjchem-460	159	9	basic	basic	ADJ
eurjchem-460	159	10	and	and	CCONJ
eurjchem-460	159	11	acidic	acidic	ADJ
eurjchem-460	159	12	metal	metal	NOUN
eurjchem-460	159	13	oxides	oxide	NOUN
eurjchem-460	159	14	for	for	ADP
eurjchem-460	159	15	synthesis	synthesis	NOUN
eurjchem-460	159	16	of	of	ADP
eurjchem-460	159	17	cyclic	cyclic	ADJ
eurjchem-460	159	18	carbonates	carbonate	NOUN
eurjchem-460	159	19	from	from	ADP
eurjchem-460	159	20	urea	urea	NOUN
eurjchem-460	159	21	and	and	CCONJ
eurjchem-460	159	22	diols	diol	NOUN
eurjchem-460	159	23	and	and	CCONJ
eurjchem-460	159	24	found	find	VERB
eurjchem-460	159	25	zno	zno	NOUN
eurjchem-460	159	26	to	to	PART
eurjchem-460	159	27	be	be	AUX
eurjchem-460	159	28	most	most	ADV
eurjchem-460	159	29	active	active	ADJ
eurjchem-460	159	30	catalyst	catalyst	NOUN
eurjchem-460	159	31	for	for	ADP
eurjchem-460	159	32	such	such	ADJ
eurjchem-460	159	33	reactions	reaction	NOUN
eurjchem-460	159	34	.	.	PUNCT
eurjchem-460	160	1	these	these	DET
eurjchem-460	160	2	findings	finding	NOUN
eurjchem-460	160	3	suggest	suggest	VERB
eurjchem-460	160	4	zno	zno	NOUN
eurjchem-460	160	5	as	as	ADP
eurjchem-460	160	6	the	the	DET
eurjchem-460	160	7	active	active	ADJ
eurjchem-460	160	8	component	component	NOUN
eurjchem-460	160	9	of	of	ADP
eurjchem-460	160	10	the	the	DET
eurjchem-460	160	11	catalyst	catalyst	NOUN
eurjchem-460	160	12	.	.	PUNCT
eurjchem-460	161	1	the	the	DET
eurjchem-460	161	2	function	function	NOUN
eurjchem-460	161	3	of	of	ADP
eurjchem-460	161	4	zncr2o4	zncr2o4	PROPN
eurjchem-460	161	5	and	and	CCONJ
eurjchem-460	161	6	cr2o3	cr2o3	PROPN
eurjchem-460	161	7	seems	seem	VERB
eurjchem-460	161	8	to	to	PART
eurjchem-460	161	9	be	be	AUX
eurjchem-460	161	10	that	that	PRON
eurjchem-460	161	11	of	of	ADP
eurjchem-460	161	12	support	support	NOUN
eurjchem-460	161	13	/	/	SYM
eurjchem-460	161	14	promoters	promoter	NOUN
eurjchem-460	161	15	.	.	PUNCT
eurjchem-460	162	1	in	in	ADP
eurjchem-460	162	2	view	view	NOUN
eurjchem-460	162	3	of	of	ADP
eurjchem-460	162	4	these	these	DET
eurjchem-460	162	5	stoichiometric	stoichiometric	ADJ
eurjchem-460	162	6	cluster	cluster	NOUN
eurjchem-460	162	7	zn4o4	zn4o4	PROPN
eurjchem-460	162	8	having	having	AUX
eurjchem-460	162	9	least	least	ADJ
eurjchem-460	162	10	amount	amount	NOUN
eurjchem-460	162	11	of	of	ADP
eurjchem-460	162	12	dangling	dangle	VERB
eurjchem-460	162	13	bond	bond	NOUN
eurjchem-460	162	14	was	be	AUX
eurjchem-460	162	15	chosen	choose	VERB
eurjchem-460	162	16	as	as	ADP
eurjchem-460	162	17	the	the	DET
eurjchem-460	162	18	appropriate	appropriate	ADJ
eurjchem-460	162	19	model	model	NOUN
eurjchem-460	162	20	of	of	ADP
eurjchem-460	162	21	the	the	DET
eurjchem-460	162	22	catalyst	catalyst	NOUN
eurjchem-460	162	23	[	[	X
eurjchem-460	162	24	46‐48	46‐48	NOUN
eurjchem-460	162	25	]	]	PUNCT
eurjchem-460	162	26	for	for	ADP
eurjchem-460	162	27	gaussian	gaussian	ADJ
eurjchem-460	162	28	calculations	calculation	NOUN
eurjchem-460	162	29	.	.	PUNCT
eurjchem-460	163	1	modeling	modeling	NOUN
eurjchem-460	163	2	of	of	ADP
eurjchem-460	163	3	the	the	DET
eurjchem-460	163	4	reaction	reaction	NOUN
eurjchem-460	163	5	with	with	ADP
eurjchem-460	163	6	flat	flat	ADJ
eurjchem-460	163	7	adsorption	adsorption	NOUN
eurjchem-460	163	8	of	of	ADP
eurjchem-460	163	9	urea	urea	NOUN
eurjchem-460	163	10	and	and	CCONJ
eurjchem-460	163	11	ethylene	ethylene	NOUN
eurjchem-460	163	12	glycol	glycol	NOUN
eurjchem-460	163	13	was	be	AUX
eurjchem-460	163	14	so	so	ADV
eurjchem-460	163	15	crowded	crowded	ADJ
eurjchem-460	163	16	that	that	SCONJ
eurjchem-460	163	17	it	it	PRON
eurjchem-460	163	18	did	do	AUX
eurjchem-460	163	19	not	not	PART
eurjchem-460	163	20	converge	converge	VERB
eurjchem-460	163	21	even	even	ADV
eurjchem-460	163	22	for	for	ADP
eurjchem-460	163	23	reactant	reactant	NOUN
eurjchem-460	163	24	model	model	NOUN
eurjchem-460	163	25	.	.	PUNCT
eurjchem-460	164	1	these	these	PRON
eurjchem-460	164	2	rules	rule	VERB
eurjchem-460	164	3	out	out	ADP
eurjchem-460	164	4	the	the	DET
eurjchem-460	164	5	single	single	ADJ
eurjchem-460	164	6	step	step	NOUN
eurjchem-460	164	7	reaction	reaction	NOUN
eurjchem-460	164	8	giving	give	VERB
eurjchem-460	164	9	two	two	NUM
eurjchem-460	164	10	moles	mole	NOUN
eurjchem-460	164	11	of	of	ADP
eurjchem-460	164	12	ammonia	ammonia	NOUN
eurjchem-460	164	13	and	and	CCONJ
eurjchem-460	164	14	one	one	NUM
eurjchem-460	164	15	moles	mole	NOUN
eurjchem-460	164	16	of	of	ADP
eurjchem-460	164	17	ethylene	ethylene	NOUN
eurjchem-460	164	18	carbonate	carbonate	NOUN
eurjchem-460	164	19	.	.	PUNCT
eurjchem-460	165	1	attempts	attempt	NOUN
eurjchem-460	165	2	were	be	AUX
eurjchem-460	165	3	therefore	therefore	ADV
eurjchem-460	165	4	made	make	VERB
eurjchem-460	165	5	to	to	PART
eurjchem-460	165	6	model	model	VERB
eurjchem-460	165	7	these	these	DET
eurjchem-460	165	8	reactions	reaction	NOUN
eurjchem-460	165	9	as	as	ADP
eurjchem-460	165	10	a	a	DET
eurjchem-460	165	11	two	two	NUM
eurjchem-460	165	12	steps	step	NOUN
eurjchem-460	165	13	consecutive	consecutive	ADJ
eurjchem-460	165	14	reaction	reaction	NOUN
eurjchem-460	165	15	in	in	ADP
eurjchem-460	165	16	which	which	PRON
eurjchem-460	165	17	urea	urea	NOUN
eurjchem-460	165	18	and	and	CCONJ
eurjchem-460	165	19	eg	eg	NOUN
eurjchem-460	165	20	are	be	AUX
eurjchem-460	165	21	adsorbed	adsorb	VERB
eurjchem-460	165	22	on	on	ADP
eurjchem-460	165	23	neighboring	neighboring	NOUN
eurjchem-460	165	24	sites	site	NOUN
eurjchem-460	165	25	and	and	CCONJ
eurjchem-460	165	26	produce	produce	VERB
eurjchem-460	165	27	2‐	2‐	NUM
eurjchem-460	165	28	hydroxyethyl	hydroxyethyl	NOUN
eurjchem-460	165	29	carbamate	carbamate	NOUN
eurjchem-460	165	30	(	(	PUNCT
eurjchem-460	165	31	reaction	reaction	NOUN
eurjchem-460	165	32	1	1	NUM
eurjchem-460	165	33	)	)	PUNCT
eurjchem-460	165	34	.	.	PUNCT
eurjchem-460	166	1	2‐hydroxyethyl	2‐hydroxyethyl	PROPN
eurjchem-460	166	2	carbamate	carbamate	PROPN
eurjchem-460	166	3	is	be	AUX
eurjchem-460	166	4	further	far	ADV
eurjchem-460	166	5	adsorbed	adsorb	VERB
eurjchem-460	166	6	in	in	ADP
eurjchem-460	166	7	the	the	DET
eurjchem-460	166	8	second	second	ADJ
eurjchem-460	166	9	step	step	NOUN
eurjchem-460	166	10	to	to	PART
eurjchem-460	166	11	produce	produce	VERB
eurjchem-460	166	12	ethylene	ethylene	NOUN
eurjchem-460	166	13	carbonate	carbonate	NOUN
eurjchem-460	166	14	and	and	CCONJ
eurjchem-460	166	15	ammonia	ammonia	NOUN
eurjchem-460	166	16	(	(	PUNCT
eurjchem-460	166	17	reaction	reaction	NOUN
eurjchem-460	166	18	2	2	NUM
eurjchem-460	166	19	)	)	PUNCT
eurjchem-460	166	20	.	.	PUNCT
eurjchem-460	167	1	the	the	DET
eurjchem-460	167	2	potential	potential	ADJ
eurjchem-460	167	3	energy	energy	NOUN
eurjchem-460	167	4	surfaces	surface	NOUN
eurjchem-460	167	5	for	for	ADP
eurjchem-460	167	6	reaction	reaction	NOUN
eurjchem-460	167	7	1	1	NUM
eurjchem-460	167	8	and	and	CCONJ
eurjchem-460	167	9	2	2	NUM
eurjchem-460	167	10	are	be	AUX
eurjchem-460	167	11	shown	show	VERB
eurjchem-460	167	12	in	in	ADP
eurjchem-460	167	13	figure	figure	NOUN
eurjchem-460	167	14	8	8	NUM
eurjchem-460	167	15	.	.	PUNCT
eurjchem-460	168	1	figure	figure	NOUN
eurjchem-460	168	2	8	8	NUM
eurjchem-460	168	3	.	.	PUNCT
eurjchem-460	169	1	the	the	DET
eurjchem-460	169	2	potential	potential	ADJ
eurjchem-460	169	3	energy	energy	NOUN
eurjchem-460	169	4	surface	surface	NOUN
eurjchem-460	169	5	for	for	ADP
eurjchem-460	169	6	reactions	reaction	NOUN
eurjchem-460	169	7	(	(	PUNCT
eurjchem-460	169	8	a	a	X
eurjchem-460	169	9	)	)	PUNCT
eurjchem-460	169	10	eg+	eg+	NOUN
eurjchem-460	169	11	pg	pg	PROPN
eurjchem-460	170	1	=	=	PROPN
eurjchem-460	171	1	2‐hec	2‐hec	PROPN
eurjchem-460	172	1	+	+	CCONJ
eurjchem-460	172	2	nh3	nh3	NUM
eurjchem-460	172	3	and	and	CCONJ
eurjchem-460	172	4	(	(	PUNCT
eurjchem-460	172	5	b	b	NOUN
eurjchem-460	172	6	)	)	PUNCT
eurjchem-460	172	7	2‐hec	2‐hec	NUM
eurjchem-460	172	8	=	=	SYM
eurjchem-460	172	9	ec	ec	PROPN
eurjchem-460	172	10	+	+	CCONJ
eurjchem-460	172	11	nh3	nh3	PROPN
eurjchem-460	172	12	.	.	PROPN
eurjchem-460	172	13	r=	r=	PROPN
eurjchem-460	172	14	reactants	reactant	NOUN
eurjchem-460	172	15	,	,	PUNCT
eurjchem-460	172	16	p	p	NOUN
eurjchem-460	172	17	=	=	NOUN
eurjchem-460	172	18	products	product	NOUN
eurjchem-460	172	19	.	.	PUNCT
eurjchem-460	173	1	the	the	DET
eurjchem-460	173	2	activation	activation	NOUN
eurjchem-460	173	3	energies	energy	NOUN
eurjchem-460	173	4	for	for	ADP
eurjchem-460	173	5	reaction	reaction	NOUN
eurjchem-460	173	6	1	1	NUM
eurjchem-460	173	7	and	and	CCONJ
eurjchem-460	173	8	2	2	NUM
eurjchem-460	173	9	were	be	AUX
eurjchem-460	173	10	calculated	calculate	VERB
eurjchem-460	173	11	to	to	PART
eurjchem-460	173	12	be	be	AUX
eurjchem-460	173	13	94.1	94.1	NUM
eurjchem-460	173	14	and	and	CCONJ
eurjchem-460	173	15	7.4	7.4	NUM
eurjchem-460	173	16	kcal	kcal	NOUN
eurjchem-460	173	17	/	/	SYM
eurjchem-460	173	18	mol1	mol1	PROPN
eurjchem-460	173	19	respectively	respectively	ADV
eurjchem-460	173	20	suggesting	suggest	VERB
eurjchem-460	173	21	reaction	reaction	NOUN
eurjchem-460	173	22	2	2	NUM
eurjchem-460	173	23	to	to	PART
eurjchem-460	173	24	be	be	AUX
eurjchem-460	173	25	much	much	ADV
eurjchem-460	173	26	faster	fast	ADJ
eurjchem-460	173	27	than	than	ADP
eurjchem-460	173	28	reaction	reaction	NOUN
eurjchem-460	173	29	1	1	NUM
eurjchem-460	173	30	.	.	PUNCT
eurjchem-460	174	1	thus	thus	ADV
eurjchem-460	174	2	,	,	PUNCT
eurjchem-460	174	3	it	it	PRON
eurjchem-460	174	4	seems	seem	VERB
eurjchem-460	174	5	2‐	2‐	NUM
eurjchem-460	174	6	hydroxyethyl	hydroxyethyl	NOUN
eurjchem-460	174	7	carbamate	carbamate	PROPN
eurjchem-460	174	8	is	be	AUX
eurjchem-460	174	9	formed	form	VERB
eurjchem-460	174	10	in	in	ADP
eurjchem-460	174	11	reaction	reaction	NOUN
eurjchem-460	174	12	1	1	NUM
eurjchem-460	174	13	and	and	CCONJ
eurjchem-460	174	14	is	be	AUX
eurjchem-460	174	15	instantly	instantly	ADV
eurjchem-460	174	16	converted	convert	VERB
eurjchem-460	174	17	to	to	ADP
eurjchem-460	174	18	ec	ec	PROPN
eurjchem-460	174	19	.	.	PUNCT
eurjchem-460	175	1	the	the	DET
eurjchem-460	175	2	mechanism	mechanism	NOUN
eurjchem-460	175	3	consistent	consistent	ADJ
eurjchem-460	175	4	with	with	ADP
eurjchem-460	175	5	these	these	PRON
eurjchem-460	175	6	is	be	AUX
eurjchem-460	175	7	shown	show	VERB
eurjchem-460	175	8	in	in	ADP
eurjchem-460	175	9	scheme	scheme	NOUN
eurjchem-460	175	10	1	1	NUM
eurjchem-460	175	11	.	.	SYM
eurjchem-460	175	12	5	5	NUM
eurjchem-460	175	13	.	.	PUNCT
eurjchem-460	175	14	conclusions	conclusion	NOUN
eurjchem-460	175	15	zno.cr2o3	zno.cr2o3	NOUN
eurjchem-460	175	16	catalyst	catalyst	NOUN
eurjchem-460	175	17	has	have	AUX
eurjchem-460	175	18	been	be	AUX
eurjchem-460	175	19	used	use	VERB
eurjchem-460	175	20	for	for	ADP
eurjchem-460	175	21	the	the	DET
eurjchem-460	175	22	first	first	ADJ
eurjchem-460	175	23	time	time	NOUN
eurjchem-460	175	24	for	for	ADP
eurjchem-460	175	25	synthesis	synthesis	NOUN
eurjchem-460	175	26	of	of	ADP
eurjchem-460	175	27	ethylene	ethylene	NOUN
eurjchem-460	175	28	carbonate	carbonate	NOUN
eurjchem-460	175	29	from	from	ADP
eurjchem-460	175	30	ethylene	ethylene	NOUN
eurjchem-460	175	31	glycol	glycol	NOUN
eurjchem-460	175	32	and	and	CCONJ
eurjchem-460	175	33	urea	urea	NOUN
eurjchem-460	175	34	.	.	PUNCT
eurjchem-460	176	1	the	the	DET
eurjchem-460	176	2	operation	operation	NOUN
eurjchem-460	176	3	conditions	condition	NOUN
eurjchem-460	176	4	have	have	VERB
eurjchem-460	176	5	a	a	DET
eurjchem-460	176	6	significant	significant	ADJ
eurjchem-460	176	7	influence	influence	NOUN
eurjchem-460	176	8	on	on	ADP
eurjchem-460	176	9	the	the	DET
eurjchem-460	176	10	ec	ec	PROPN
eurjchem-460	176	11	yield	yield	NOUN
eurjchem-460	176	12	.	.	PUNCT
eurjchem-460	177	1	the	the	DET
eurjchem-460	177	2	experimental	experimental	ADJ
eurjchem-460	177	3	results	result	NOUN
eurjchem-460	177	4	indicated	indicate	VERB
eurjchem-460	177	5	that	that	SCONJ
eurjchem-460	177	6	the	the	DET
eurjchem-460	177	7	optimum	optimum	ADJ
eurjchem-460	177	8	reaction	reaction	NOUN
eurjchem-460	177	9	conditions	condition	NOUN
eurjchem-460	177	10	over	over	ADP
eurjchem-460	177	11	zc‐1	zc‐1	PROPN
eurjchem-460	177	12	were	be	AUX
eurjchem-460	177	13	urea/	urea/	NUM
eurjchem-460	177	14	eg	eg	NOUN
eurjchem-460	177	15	molar	molar	ADJ
eurjchem-460	177	16	ratio	ratio	NOUN
eurjchem-460	177	17	of	of	ADP
eurjchem-460	177	18	1:1.5	1:1.5	NUM
eurjchem-460	177	19	,	,	PUNCT
eurjchem-460	177	20	catalyst	catalyst	NOUN
eurjchem-460	177	21	concentration	concentration	NOUN
eurjchem-460	177	22	of	of	ADP
eurjchem-460	177	23	6	6	NUM
eurjchem-460	177	24	wt.%	wt.%	ADJ
eurjchem-460	177	25	,	,	PUNCT
eurjchem-460	177	26	reaction	reaction	NOUN
eurjchem-460	177	27	temperature	temperature	NOUN
eurjchem-460	177	28	of	of	ADP
eurjchem-460	177	29	425	425	NUM
eurjchem-460	177	30	k	k	NOUN
eurjchem-460	177	31	,	,	PUNCT
eurjchem-460	177	32	and	and	CCONJ
eurjchem-460	177	33	reaction	reaction	NOUN
eurjchem-460	177	34	time	time	NOUN
eurjchem-460	177	35	of	of	ADP
eurjchem-460	177	36	3	3	NUM
eurjchem-460	177	37	h.	h.	NOUN
eurjchem-460	177	38	a	a	DET
eurjchem-460	177	39	mechanism	mechanism	NOUN
eurjchem-460	177	40	of	of	ADP
eurjchem-460	177	41	the	the	DET
eurjchem-460	177	42	reaction	reaction	NOUN
eurjchem-460	177	43	assuming	assume	VERB
eurjchem-460	177	44	a	a	DET
eurjchem-460	177	45	consecutive	consecutive	ADJ
eurjchem-460	177	46	reaction	reaction	NOUN
eurjchem-460	177	47	is	be	AUX
eurjchem-460	177	48	proposed	propose	VERB
eurjchem-460	177	49	.	.	PUNCT
eurjchem-460	178	1	catalysts	catalyst	NOUN
eurjchem-460	178	2	can	can	AUX
eurjchem-460	178	3	be	be	AUX
eurjchem-460	178	4	easily	easily	ADV
eurjchem-460	178	5	regenerated	regenerate	VERB
eurjchem-460	178	6	in	in	ADP
eurjchem-460	178	7	situ	situ	NOUN
eurjchem-460	178	8	by	by	ADP
eurjchem-460	178	9	calcining	calcine	VERB
eurjchem-460	178	10	with	with	ADP
eurjchem-460	178	11	air	air	NOUN
eurjchem-460	178	12	at	at	ADP
eurjchem-460	178	13	773	773	NUM
eurjchem-460	178	14	k	k	NOUN
eurjchem-460	178	15	for	for	ADP
eurjchem-460	178	16	4	4	NUM
eurjchem-460	178	17	h.	h.	NOUN
eurjchem-460	178	18	acknowledgements	acknowledgement	NOUN
eurjchem-460	178	19	the	the	DET
eurjchem-460	178	20	authors	author	NOUN
eurjchem-460	178	21	wish	wish	VERB
eurjchem-460	178	22	to	to	PART
eurjchem-460	178	23	express	express	VERB
eurjchem-460	178	24	their	their	PRON
eurjchem-460	178	25	appreciation	appreciation	NOUN
eurjchem-460	178	26	to	to	ADP
eurjchem-460	178	27	university	university	NOUN
eurjchem-460	178	28	grants	grant	NOUN
eurjchem-460	178	29	commission‐department	commission‐department	ADJ
eurjchem-460	178	30	of	of	ADP
eurjchem-460	178	31	atomic	atomic	ADJ
eurjchem-460	178	32	energy‐	energy‐	PROPN
eurjchem-460	178	33	consortium	consortium	NOUN
eurjchem-460	178	34	for	for	ADP
eurjchem-460	178	35	scientific	scientific	ADJ
eurjchem-460	178	36	research	research	NOUN
eurjchem-460	178	37	(	(	PUNCT
eurjchem-460	178	38	ugc‐dae‐csr	ugc‐dae‐csr	NUM
eurjchem-460	178	39	)	)	PUNCT
eurjchem-460	178	40	,	,	PUNCT
eurjchem-460	178	41	indore	indore	NOUN
eurjchem-460	178	42	for	for	ADP
eurjchem-460	178	43	recording	recording	NOUN
eurjchem-460	178	44	xrd	xrd	NOUN
eurjchem-460	178	45	and	and	CCONJ
eurjchem-460	178	46	sem	sem	NOUN
eurjchem-460	178	47	measurements	measurement	NOUN
eurjchem-460	178	48	.	.	PUNCT
eurjchem-460	179	1	dr	dr	PROPN
eurjchem-460	179	2	.	.	PROPN
eurjchem-460	179	3	reena	reena	PROPN
eurjchem-460	179	4	dwivedi	dwivedi	PROPN
eurjchem-460	179	5	and	and	CCONJ
eurjchem-460	179	6	prabhakar	prabhakar	PROPN
eurjchem-460	179	7	sharma	sharma	PROPN
eurjchem-460	179	8	wish	wish	VERB
eurjchem-460	179	9	to	to	PART
eurjchem-460	179	10	thank	thank	VERB
eurjchem-460	179	11	department	department	PROPN
eurjchem-460	179	12	of	of	ADP
eurjchem-460	179	13	science	science	NOUN
eurjchem-460	179	14	and	and	CCONJ
eurjchem-460	179	15	technology	technology	NOUN
eurjchem-460	179	16	(	(	PUNCT
eurjchem-460	179	17	dst	dst	PROPN
eurjchem-460	179	18	)	)	PUNCT
eurjchem-460	179	19	,	,	PUNCT
eurjchem-460	179	20	new	new	PROPN
eurjchem-460	179	21	delhi	delhi	PROPN
eurjchem-460	179	22	and	and	CCONJ
eurjchem-460	179	23	madhya	madhya	PROPN
eurjchem-460	179	24	pradesh	pradesh	PROPN
eurjchem-460	179	25	council	council	PROPN
eurjchem-460	179	26	of	of	ADP
eurjchem-460	179	27	science	science	PROPN
eurjchem-460	179	28	&	&	CCONJ
eurjchem-460	179	29	technology	technology	PROPN
eurjchem-460	179	30	(	(	PUNCT
eurjchem-460	179	31	mpcst	mpcst	ADJ
eurjchem-460	179	32	)	)	PUNCT
eurjchem-460	179	33	,	,	PUNCT
eurjchem-460	179	34	bhopal	bhopal	NOUN
eurjchem-460	179	35	,	,	PUNCT
eurjchem-460	179	36	respectively	respectively	ADV
eurjchem-460	179	37	for	for	ADP
eurjchem-460	179	38	financial	financial	ADJ
eurjchem-460	179	39	supports	support	NOUN
eurjchem-460	179	40	.	.	PUNCT
eurjchem-460	180	1	references	reference	NOUN
eurjchem-460	180	2	[	[	X
eurjchem-460	180	3	1	1	NUM
eurjchem-460	180	4	]	]	PUNCT
eurjchem-460	180	5	.	.	PUNCT
eurjchem-460	181	1	sakakura	sakakura	PROPN
eurjchem-460	181	2	,	,	PUNCT
eurjchem-460	181	3	t.	t.	PROPN
eurjchem-460	181	4	;	;	PUNCT
eurjchem-460	181	5	choi	choi	PROPN
eurjchem-460	181	6	,	,	PUNCT
eurjchem-460	181	7	j.	j.	PROPN
eurjchem-460	181	8	;	;	PUNCT
eurjchem-460	181	9	yasuda	yasuda	PROPN
eurjchem-460	181	10	,	,	PUNCT
eurjchem-460	181	11	h.	h.	PROPN
eurjchem-460	181	12	chem	chem	PROPN
eurjchem-460	181	13	.	.	PUNCT
eurjchem-460	182	1	rev	rev	PROPN
eurjchem-460	182	2	.	.	PROPN
eurjchem-460	182	3	2007	2007	NUM
eurjchem-460	182	4	,	,	PUNCT
eurjchem-460	182	5	107	107	NUM
eurjchem-460	182	6	,	,	PUNCT
eurjchem-460	182	7	2365‐2387	2365‐2387	NUM
eurjchem-460	182	8	.	.	PUNCT
eurjchem-460	183	1	[	[	X
eurjchem-460	183	2	2	2	NUM
eurjchem-460	183	3	]	]	PUNCT
eurjchem-460	183	4	.	.	PUNCT
eurjchem-460	184	1	clements	clements	PROPN
eurjchem-460	184	2	,	,	PUNCT
eurjchem-460	184	3	j.	j.	PROPN
eurjchem-460	184	4	h.	h.	PROPN
eurjchem-460	184	5	ind	ind	PROPN
eurjchem-460	184	6	.	.	PUNCT
eurjchem-460	185	1	eng	eng	PROPN
eurjchem-460	185	2	.	.	PROPN
eurjchem-460	185	3	chem	chem	PROPN
eurjchem-460	185	4	.	.	PUNCT
eurjchem-460	186	1	res	re	NOUN
eurjchem-460	186	2	.	.	PROPN
eurjchem-460	186	3	2003	2003	NUM
eurjchem-460	186	4	,	,	PUNCT
eurjchem-460	186	5	42	42	NUM
eurjchem-460	186	6	,	,	PUNCT
eurjchem-460	186	7	663‐674	663‐674	NUM
eurjchem-460	186	8	.	.	PUNCT
eurjchem-460	187	1	[	[	X
eurjchem-460	187	2	3	3	NUM
eurjchem-460	187	3	]	]	PUNCT
eurjchem-460	187	4	.	.	PUNCT
eurjchem-460	188	1	balasubramanian	balasubramanian	PROPN
eurjchem-460	188	2	,	,	PUNCT
eurjchem-460	188	3	m.	m.	NOUN
eurjchem-460	188	4	;	;	PUNCT
eurjchem-460	188	5	lee	lee	PROPN
eurjchem-460	188	6	,	,	PUNCT
eurjchem-460	188	7	h.	h.	PROPN
eurjchem-460	188	8	s.	s.	PROPN
eurjchem-460	188	9	;	;	PUNCT
eurjchem-460	188	10	sun	sun	NOUN
eurjchem-460	188	11	,	,	PUNCT
eurjchem-460	188	12	x.	x.	PROPN
eurjchem-460	188	13	;	;	PUNCT
eurjchem-460	188	14	yang	yang	PROPN
eurjchem-460	188	15	,	,	PUNCT
eurjchem-460	188	16	x.	x.	PROPN
eurjchem-460	188	17	q.	q.	PROPN
eurjchem-460	188	18	;	;	PUNCT
eurjchem-460	188	19	moodenbaugh	moodenbaugh	PROPN
eurjchem-460	188	20	,	,	PUNCT
eurjchem-460	188	21	a.	a.	PROPN
eurjchem-460	188	22	r.	r.	PROPN
eurjchem-460	188	23	;	;	PUNCT
eurjchem-460	188	24	mcbreen	mcbreen	PROPN
eurjchem-460	188	25	,	,	PUNCT
eurjchem-460	188	26	j.	j.	PROPN
eurjchem-460	188	27	;	;	PUNCT
eurjchem-460	188	28	fischer	fischer	PROPN
eurjchem-460	188	29	,	,	PUNCT
eurjchem-460	188	30	d.	d.	PROPN
eurjchem-460	188	31	a.	a.	PROPN
eurjchem-460	188	32	;	;	PUNCT
eurjchem-460	188	33	fu	fu	PROPN
eurjchem-460	188	34	,	,	PUNCT
eurjchem-460	188	35	z.	z.	PROPN
eurjchem-460	188	36	electrochem	electrochem	PROPN
eurjchem-460	188	37	solid	solid	PROPN
eurjchem-460	188	38	st	st	PROPN
eurjchem-460	188	39	.	.	PROPN
eurjchem-460	188	40	2002	2002	NUM
eurjchem-460	188	41	,	,	PUNCT
eurjchem-460	188	42	5	5	NUM
eurjchem-460	188	43	,	,	PUNCT
eurjchem-460	188	44	a22‐	a22‐	ADJ
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eurjchem-460	188	46	.	.	PUNCT
eurjchem-460	189	1	[	[	X
eurjchem-460	189	2	4	4	NUM
eurjchem-460	189	3	]	]	PUNCT
eurjchem-460	189	4	.	.	PUNCT
eurjchem-460	190	1	chandrasekarani	chandrasekarani	PROPN
eurjchem-460	190	2	,	,	PUNCT
eurjchem-460	190	3	r.	r.	PROPN
eurjchem-460	190	4	;	;	PUNCT
eurjchem-460	190	5	koh	koh	PROPN
eurjchem-460	190	6	,	,	PUNCT
eurjchem-460	190	7	m.	m.	NOUN
eurjchem-460	190	8	;	;	PUNCT
eurjchem-460	190	9	ozhawa	ozhawa	PROPN
eurjchem-460	190	10	,	,	PUNCT
eurjchem-460	190	11	y.	y.	PROPN
eurjchem-460	190	12	;	;	PUNCT
eurjchem-460	190	13	aoyoma	aoyoma	PROPN
eurjchem-460	190	14	,	,	PUNCT
eurjchem-460	190	15	h.	h.	PROPN
eurjchem-460	190	16	;	;	PUNCT
eurjchem-460	190	17	nakajima	nakajima	PROPN
eurjchem-460	190	18	,	,	PUNCT
eurjchem-460	190	19	t.	t.	PROPN
eurjchem-460	190	20	j.	j.	PROPN
eurjchem-460	190	21	chem	chem	PROPN
eurjchem-460	190	22	.	.	PUNCT
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eurjchem-460	191	2	2009	2009	NUM
eurjchem-460	191	3	,	,	PUNCT
eurjchem-460	191	4	121	121	NUM
eurjchem-460	191	5	,	,	PUNCT
eurjchem-460	191	6	339‐346	339‐346	NUM
eurjchem-460	191	7	.	.	PUNCT
eurjchem-460	192	1	[	[	X
eurjchem-460	192	2	5	5	NUM
eurjchem-460	192	3	]	]	PUNCT
eurjchem-460	192	4	.	.	PUNCT
eurjchem-460	193	1	jie	jie	PROPN
eurjchem-460	193	2	,	,	PUNCT
eurjchem-460	193	3	l.	l.	PROPN
eurjchem-460	193	4	;	;	PUNCT
eurjchem-460	193	5	wanhao	wanhao	PROPN
eurjchem-460	193	6	,	,	PUNCT
eurjchem-460	193	7	y.	y.	PROPN
eurjchem-460	193	8	;	;	PUNCT
eurjchem-460	193	9	meng	meng	PROPN
eurjchem-460	193	10	,	,	PUNCT
eurjchem-460	193	11	y.	y.	PROPN
eurjchem-460	193	12	s.	s.	PROPN
eurjchem-460	193	13	;	;	PUNCT
eurjchem-460	193	14	yang	yang	PROPN
eurjchem-460	193	15	,	,	PUNCT
eurjchem-460	193	16	y.	y.	PROPN
eurjchem-460	193	17	j.	j.	PROPN
eurjchem-460	193	18	phys	phys	PROPN
eurjchem-460	193	19	.	.	PUNCT
eurjchem-460	194	1	chem	chem	PROPN
eurjchem-460	194	2	.	.	PUNCT
eurjchem-460	195	1	c	c	PROPN
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eurjchem-460	195	3	,	,	PUNCT
eurjchem-460	195	4	112	112	NUM
eurjchem-460	195	5	,	,	PUNCT
eurjchem-460	195	6	12550‐12556	12550‐12556	NUM
eurjchem-460	195	7	.	.	PUNCT
eurjchem-460	196	1	[	[	X
eurjchem-460	196	2	6	6	NUM
eurjchem-460	196	3	]	]	PUNCT
eurjchem-460	196	4	.	.	PUNCT
eurjchem-460	197	1	badsetan	badsetan	PROPN
eurjchem-460	197	2	,	,	PUNCT
eurjchem-460	197	3	m.	m.	NOUN
eurjchem-460	197	4	;	;	PUNCT
eurjchem-460	197	5	christenson	christenson	PROPN
eurjchem-460	197	6	,	,	PUNCT
eurjchem-460	197	7	e.	e.	PROPN
eurjchem-460	197	8	m.	m.	PROPN
eurjchem-460	197	9	;	;	PUNCT
eurjchem-460	197	10	unger	unger	PROPN
eurjchem-460	197	11	,	,	PUNCT
eurjchem-460	197	12	b.	b.	PROPN
eurjchem-460	197	13	;	;	PUNCT
eurjchem-460	197	14	ausborn	ausborn	VERB
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eurjchem-460	197	17	;	;	PUNCT
eurjchem-460	197	18	kissel	kissel	PROPN
eurjchem-460	197	19	,	,	PUNCT
eurjchem-460	197	20	t.	t.	PROPN
eurjchem-460	197	21	;	;	PUNCT
eurjchem-460	197	22	hiltener	hiltener	NOUN
eurjchem-460	197	23	,	,	PUNCT
eurjchem-460	197	24	a.	a.	NOUN
eurjchem-460	197	25	;	;	PUNCT
eurjchem-460	198	1	anderson	anderson	PROPN
eurjchem-460	198	2	,	,	PUNCT
eurjchem-460	198	3	j.	j.	PROPN
eurjchem-460	198	4	m.	m.	PROPN
eurjchem-460	198	5	j.	j.	PROPN
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eurjchem-460	198	9	,	,	PUNCT
eurjchem-460	198	10	93	93	NUM
eurjchem-460	198	11	,	,	PUNCT
eurjchem-460	198	12	259‐270	259‐270	NUM
eurjchem-460	198	13	.	.	PUNCT
eurjchem-460	199	1	[	[	X
eurjchem-460	199	2	7	7	NUM
eurjchem-460	199	3	]	]	PUNCT
eurjchem-460	199	4	.	.	PUNCT
eurjchem-460	200	1	shirahama	shirahama	PROPN
eurjchem-460	200	2	,	,	PUNCT
eurjchem-460	200	3	h.	h.	PROPN
eurjchem-460	200	4	;	;	PUNCT
eurjchem-460	200	5	kanetani	kanetani	PROPN
eurjchem-460	200	6	,	,	PUNCT
eurjchem-460	200	7	a.	a.	NOUN
eurjchem-460	200	8	;	;	PUNCT
eurjchem-460	200	9	yasuda	yasuda	PROPN
eurjchem-460	200	10	,	,	PUNCT
eurjchem-460	200	11	h.	h.	PROPN
eurjchem-460	200	12	polym	polym	PROPN
eurjchem-460	200	13	.	.	PUNCT
eurjchem-460	201	1	j.	j.	PROPN
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eurjchem-460	201	3	,	,	PUNCT
eurjchem-460	201	4	32	32	NUM
eurjchem-460	201	5	,	,	PUNCT
eurjchem-460	201	6	280‐286	280‐286	NUM
eurjchem-460	201	7	.	.	PUNCT
eurjchem-460	202	1	[	[	X
eurjchem-460	202	2	8	8	NUM
eurjchem-460	202	3	]	]	PUNCT
eurjchem-460	202	4	.	.	PUNCT
eurjchem-460	203	1	wang	wang	PROPN
eurjchem-460	203	2	,	,	PUNCT
eurjchem-460	203	3	j.	j.	PROPN
eurjchem-460	203	4	l.	l.	PROPN
eurjchem-460	203	5	;	;	PUNCT
eurjchem-460	203	6	he	he	PRON
eurjchem-460	203	7	,	,	PUNCT
eurjchem-460	203	8	l.	l.	PROPN
eurjchem-460	203	9	n.	n.	PROPN
eurjchem-460	203	10	;	;	PUNCT
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eurjchem-460	203	12	,	,	PUNCT
eurjchem-460	203	13	c.	c.	PROPN
eurjchem-460	203	14	x.	x.	PROPN
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eurjchem-460	203	17	,	,	PUNCT
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eurjchem-460	203	22	.	.	PUNCT
eurjchem-460	204	1	2009	2009	NUM
eurjchem-460	204	2	,	,	PUNCT
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eurjchem-460	204	4	,	,	PUNCT
eurjchem-460	204	5	1317‐	1317‐	NUM
eurjchem-460	204	6	1320	1320	NUM
eurjchem-460	204	7	.	.	PUNCT
eurjchem-460	205	1	[	[	X
eurjchem-460	205	2	9	9	NUM
eurjchem-460	205	3	]	]	PUNCT
eurjchem-460	205	4	.	.	PUNCT
eurjchem-460	206	1	shaikh	shaikh	PROPN
eurjchem-460	206	2	,	,	PUNCT
eurjchem-460	206	3	g.	g.	PROPN
eurjchem-460	206	4	;	;	PUNCT
eurjchem-460	206	5	sivram	sivram	PROPN
eurjchem-460	206	6	,	,	PUNCT
eurjchem-460	206	7	s.	s.	PROPN
eurjchem-460	206	8	chem	chem	PROPN
eurjchem-460	206	9	.	.	PUNCT
eurjchem-460	207	1	rev	rev	PROPN
eurjchem-460	207	2	.	.	PROPN
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eurjchem-460	207	4	,	,	PUNCT
eurjchem-460	207	5	96	96	NUM
eurjchem-460	207	6	,	,	PUNCT
eurjchem-460	207	7	951‐976	951‐976	NUM
eurjchem-460	207	8	.	.	PUNCT
eurjchem-460	208	1	[	[	X
eurjchem-460	208	2	10	10	NUM
eurjchem-460	208	3	]	]	PUNCT
eurjchem-460	208	4	.	.	PUNCT
eurjchem-460	209	1	ji	ji	PROPN
eurjchem-460	209	2	,	,	PUNCT
eurjchem-460	209	3	d.	d.	PROPN
eurjchem-460	209	4	;	;	PUNCT
eurjchem-460	209	5	xiaobing	xiaobing	PROPN
eurjchem-460	209	6	,	,	PUNCT
eurjchem-460	209	7	l.	l.	PROPN
eurjchem-460	209	8	;	;	PUNCT
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eurjchem-460	209	10	.	.	PUNCT
eurjchem-460	210	1	h.	h.	PROPN
eurjchem-460	210	2	appl	appl	PROPN
eurjchem-460	210	3	.	.	PUNCT
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eurjchem-460	211	2	.	.	PUNCT
eurjchem-460	212	1	a	a	DET
eurjchem-460	212	2	:	:	PUNCT
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eurjchem-460	212	6	,	,	PUNCT
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eurjchem-460	212	8	,	,	PUNCT
eurjchem-460	212	9	329‐333	329‐333	NUM
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eurjchem-460	213	3	]	]	PUNCT
eurjchem-460	213	4	.	.	PUNCT
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eurjchem-460	213	6	,	,	PUNCT
eurjchem-460	213	7	a.	a.	NOUN
eurjchem-460	213	8	;	;	PUNCT
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eurjchem-460	213	10	,	,	PUNCT
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eurjchem-460	213	12	;	;	PUNCT
eurjchem-460	213	13	jacobs	jacobs	PROPN
eurjchem-460	213	14	,	,	PUNCT
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eurjchem-460	213	18	,	,	PUNCT
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eurjchem-460	213	20	d.	d.	PROPN
eurjchem-460	213	21	appl	appl	PROPN
eurjchem-460	213	22	.	.	PUNCT
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eurjchem-460	214	2	.	.	PUNCT
eurjchem-460	215	1	a	a	DET
eurjchem-460	215	2	:	:	PUNCT
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eurjchem-460	215	4	.	.	PROPN
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eurjchem-460	215	6	,	,	PUNCT
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eurjchem-460	215	8	,	,	PUNCT
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eurjchem-460	215	10	.	.	PUNCT
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eurjchem-460	216	3	]	]	PUNCT
eurjchem-460	216	4	.	.	PUNCT
eurjchem-460	217	1	jagtap	jagtap	PROPN
eurjchem-460	217	2	,	,	PUNCT
eurjchem-460	217	3	s.	s.	PROPN
eurjchem-460	217	4	;	;	PUNCT
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eurjchem-460	217	6	,	,	PUNCT
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eurjchem-460	217	8	;	;	PUNCT
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eurjchem-460	217	10	,	,	PUNCT
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eurjchem-460	217	12	;	;	PUNCT
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eurjchem-460	217	14	,	,	PUNCT
eurjchem-460	217	15	b.	b.	PROPN
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eurjchem-460	217	17	.	.	PUNCT
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eurjchem-460	218	2	.	.	PUNCT
eurjchem-460	219	1	2006	2006	NUM
eurjchem-460	219	2	,	,	PUNCT
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eurjchem-460	219	4	,	,	PUNCT
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eurjchem-460	219	6	.	.	PUNCT
eurjchem-460	220	1	[	[	X
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eurjchem-460	220	3	]	]	PUNCT
eurjchem-460	220	4	.	.	PUNCT
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eurjchem-460	220	6	,	,	PUNCT
eurjchem-460	220	7	r.	r.	PROPN
eurjchem-460	220	8	;	;	PUNCT
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eurjchem-460	220	10	,	,	PUNCT
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eurjchem-460	220	12	;	;	PUNCT
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eurjchem-460	220	14	,	,	PUNCT
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eurjchem-460	220	16	j.	j.	PROPN
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eurjchem-460	220	18	.	.	PROPN
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eurjchem-460	221	2	,	,	PUNCT
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eurjchem-460	221	4	,	,	PUNCT
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eurjchem-460	221	6	.	.	PUNCT
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eurjchem-460	222	3	]	]	SYM
eurjchem-460	222	4	.	.	PUNCT
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eurjchem-460	223	2	,	,	PUNCT
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eurjchem-460	223	4	;	;	PUNCT
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eurjchem-460	223	6	,	,	PUNCT
eurjchem-460	223	7	e.	e.	PROPN
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eurjchem-460	223	9	;	;	PUNCT
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eurjchem-460	223	13	;	;	PUNCT
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eurjchem-460	223	17	kore	kore	PROPN
eurjchem-460	223	18	.	.	PUNCT
eurjchem-460	224	1	chem	chem	PROPN
eurjchem-460	224	2	.	.	PUNCT
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eurjchem-460	225	2	.	.	PUNCT
eurjchem-460	226	1	2006	2006	NUM
eurjchem-460	226	2	,	,	PUNCT
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eurjchem-460	226	4	,	,	PUNCT
eurjchem-460	226	5	1171‐	1171‐	NUM
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eurjchem-460	226	7	.	.	PUNCT
eurjchem-460	227	1	[	[	X
eurjchem-460	227	2	15	15	NUM
eurjchem-460	227	3	]	]	PUNCT
eurjchem-460	227	4	.	.	PUNCT
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eurjchem-460	228	2	,	,	PUNCT
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eurjchem-460	228	4	;	;	PUNCT
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eurjchem-460	228	6	,	,	PUNCT
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eurjchem-460	228	8	;	;	PUNCT
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eurjchem-460	228	10	,	,	PUNCT
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eurjchem-460	228	12	;	;	PUNCT
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eurjchem-460	228	14	,	,	PUNCT
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eurjchem-460	228	17	.	.	PUNCT
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eurjchem-460	229	2	.	.	PUNCT
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eurjchem-460	229	4	,	,	PUNCT
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eurjchem-460	229	6	,	,	PUNCT
eurjchem-460	229	7	2561‐	2561‐	NUM
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eurjchem-460	229	9	.	.	PUNCT
eurjchem-460	230	1	[	[	X
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eurjchem-460	230	4	.	.	PUNCT
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eurjchem-460	231	2	,	,	PUNCT
eurjchem-460	231	3	d.	d.	PROPN
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eurjchem-460	231	5	;	;	PUNCT
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eurjchem-460	231	7	,	,	PUNCT
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eurjchem-460	231	11	.	.	PUNCT
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eurjchem-460	232	2	.	.	PUNCT
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eurjchem-460	233	2	.	.	PROPN
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eurjchem-460	233	4	,	,	PUNCT
eurjchem-460	233	5	153	153	NUM
eurjchem-460	233	6	,	,	PUNCT
eurjchem-460	233	7	155‐174	155‐174	NUM
eurjchem-460	233	8	.	.	PUNCT
eurjchem-460	234	1	[	[	X
eurjchem-460	234	2	17	17	NUM
eurjchem-460	234	3	]	]	PUNCT
eurjchem-460	234	4	.	.	PUNCT
eurjchem-460	235	1	tomishige	tomishige	PROPN
eurjchem-460	235	2	,	,	PUNCT
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eurjchem-460	235	4	;	;	PUNCT
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eurjchem-460	235	6	,	,	PUNCT
eurjchem-460	235	7	h.	h.	PROPN
eurjchem-460	235	8	;	;	PUNCT
eurjchem-460	235	9	yoshida	yoshida	PROPN
eurjchem-460	235	10	,	,	PUNCT
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eurjchem-460	235	12	;	;	PUNCT
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eurjchem-460	237	2	,	,	PUNCT
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eurjchem-460	243	6	,	,	PUNCT
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eurjchem-460	244	3	,	,	PUNCT
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eurjchem-460	248	14	,	,	PUNCT
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eurjchem-460	249	2	,	,	PUNCT
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eurjchem-460	249	6	.	.	PUNCT
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eurjchem-460	250	3	]	]	PUNCT
eurjchem-460	250	4	.	.	PUNCT
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eurjchem-460	251	2	,	,	PUNCT
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eurjchem-460	251	7	,	,	PUNCT
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eurjchem-460	255	2	,	,	PUNCT
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eurjchem-460	257	25	;	;	PUNCT
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eurjchem-460	257	27	,	,	PUNCT
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eurjchem-460	277	6	,	,	PUNCT
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eurjchem-460	277	8	,	,	PUNCT
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eurjchem-460	277	10	.	.	PUNCT
eurjchem-460	278	1	[	[	X
eurjchem-460	278	2	29	29	NUM
eurjchem-460	278	3	]	]	PUNCT
eurjchem-460	278	4	.	.	PUNCT
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eurjchem-460	279	2	,	,	PUNCT
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eurjchem-460	279	7	,	,	PUNCT
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eurjchem-460	279	11	s	s	PART
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eurjchem-460	279	14	,	,	PUNCT
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eurjchem-460	279	16	.	.	PUNCT
eurjchem-460	280	1	[	[	X
eurjchem-460	280	2	30	30	NUM
eurjchem-460	280	3	]	]	PUNCT
eurjchem-460	280	4	.	.	PUNCT
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eurjchem-460	281	2	,	,	PUNCT
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eurjchem-460	281	7	,	,	PUNCT
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eurjchem-460	281	11	s	s	PROPN
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eurjchem-460	281	14	,	,	PUNCT
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eurjchem-460	281	16	.	.	PUNCT
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eurjchem-460	282	17	)	)	PUNCT
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eurjchem-460	284	3	]	]	PUNCT
eurjchem-460	284	4	.	.	PUNCT
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eurjchem-460	284	6	,	,	PUNCT
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eurjchem-460	284	11	,	,	PUNCT
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eurjchem-460	284	20	,	,	PUNCT
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eurjchem-460	284	25	4233221	4233221	NUM
eurjchem-460	284	26	,	,	PUNCT
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eurjchem-460	284	28	.	.	PUNCT
eurjchem-460	285	1	[	[	X
eurjchem-460	285	2	32	32	NUM
eurjchem-460	285	3	]	]	SYM
eurjchem-460	285	4	.	.	PUNCT
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eurjchem-460	286	2	,	,	PUNCT
eurjchem-460	286	3	w.	w.	PROPN
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eurjchem-460	286	5	;	;	PUNCT
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eurjchem-460	286	7	,	,	PUNCT
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eurjchem-460	287	3	e	e	PROPN
eurjchem-460	288	1	p	p	NOUN
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eurjchem-460	288	3	0443758	0443758	NUM
eurjchem-460	288	4	a1	a1	NOUN
eurjchem-460	288	5	,	,	PUNCT
eurjchem-460	288	6	1991	1991	NUM
eurjchem-460	288	7	.	.	PUNCT
eurjchem-460	289	1	[	[	X
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eurjchem-460	289	3	]	]	PUNCT
eurjchem-460	289	4	.	.	PUNCT
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eurjchem-460	290	2	,	,	PUNCT
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eurjchem-460	290	4	;	;	PUNCT
eurjchem-460	290	5	takashi	takashi	PROPN
eurjchem-460	290	6	,	,	PUNCT
eurjchem-460	290	7	o.	o.	PROPN
eurjchem-460	290	8	;	;	PUNCT
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eurjchem-460	290	10	,	,	PUNCT
eurjchem-460	290	11	k.	k.	PROPN
eurjchem-460	290	12	;	;	PUNCT
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eurjchem-460	290	14	,	,	PUNCT
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eurjchem-460	290	16	;	;	PUNCT
eurjchem-460	290	17	kenlchi	kenlchi	PROPN
eurjchem-460	290	18	,	,	PUNCT
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eurjchem-460	291	1	e.	e.	PROPN
eurjchem-460	291	2	p.	p.	PROPN
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eurjchem-460	291	4	0581131	0581131	NUM
eurjchem-460	291	5	a2	a2	PROPN
eurjchem-460	291	6	,	,	PUNCT
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eurjchem-460	291	8	.	.	PUNCT
eurjchem-460	292	1	[	[	X
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eurjchem-460	292	3	]	]	PUNCT
eurjchem-460	292	4	.	.	PUNCT
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eurjchem-460	293	2	,	,	PUNCT
eurjchem-460	293	3	q.	q.	PROPN
eurjchem-460	293	4	b.	b.	PROPN
eurjchem-460	293	5	;	;	PUNCT
eurjchem-460	293	6	zhang	zhang	PROPN
eurjchem-460	293	7	,	,	PUNCT
eurjchem-460	293	8	w.	w.	PROPN
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eurjchem-460	293	10	;	;	PUNCT
eurjchem-460	293	11	zhao	zhao	X
eurjchem-460	293	12	,	,	PUNCT
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eurjchem-460	293	14	;	;	PUNCT
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eurjchem-460	293	20	,	,	PUNCT
eurjchem-460	293	21	y.	y.	PROPN
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eurjchem-460	294	2	,	,	PUNCT
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eurjchem-460	294	4	,	,	PUNCT
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eurjchem-460	294	6	,	,	PUNCT
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eurjchem-460	294	8	.	.	PUNCT
eurjchem-460	295	1	[	[	X
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eurjchem-460	295	3	]	]	SYM
eurjchem-460	295	4	.	.	PUNCT
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eurjchem-460	296	2	,	,	PUNCT
eurjchem-460	296	3	x.	x.	PROPN
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eurjchem-460	296	5	;	;	PUNCT
eurjchem-460	296	6	jia	jia	PROPN
eurjchem-460	296	7	,	,	PUNCT
eurjchem-460	296	8	z.	z.	PROPN
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eurjchem-460	296	10	;	;	PUNCT
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eurjchem-460	296	12	,	,	PUNCT
eurjchem-460	296	13	y.	y.	PROPN
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eurjchem-460	296	16	.	.	PUNCT
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eurjchem-460	297	2	.	.	PUNCT
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eurjchem-460	297	4	.	.	PUNCT
eurjchem-460	298	1	2006	2006	NUM
eurjchem-460	298	2	,	,	PUNCT
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eurjchem-460	298	4	,	,	PUNCT
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eurjchem-460	298	7	.	.	PUNCT
eurjchem-460	299	1	[	[	X
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eurjchem-460	299	3	]	]	PUNCT
eurjchem-460	299	4	.	.	PUNCT
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eurjchem-460	300	2	,	,	PUNCT
eurjchem-460	300	3	z.	z.	PROPN
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eurjchem-460	300	5	;	;	PUNCT
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eurjchem-460	300	7	,	,	PUNCT
eurjchem-460	300	8	x.	x.	PROPN
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eurjchem-460	300	10	;	;	PUNCT
eurjchem-460	300	11	an	an	PRON
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eurjchem-460	300	13	h.	h.	PROPN
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eurjchem-460	300	17	,	,	PUNCT
eurjchem-460	300	18	c.	c.	PROPN
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eurjchem-460	300	22	,	,	PUNCT
eurjchem-460	300	23	y.	y.	PROPN
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eurjchem-460	300	26	.	.	PUNCT
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eurjchem-460	301	2	.	.	PUNCT
eurjchem-460	302	1	2006	2006	NUM
eurjchem-460	302	2	,	,	PUNCT
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eurjchem-460	302	4	,	,	PUNCT
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eurjchem-460	302	6	.	.	PUNCT
eurjchem-460	303	1	[	[	X
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eurjchem-460	303	3	]	]	PUNCT
eurjchem-460	303	4	.	.	PUNCT
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eurjchem-460	304	2	,	,	PUNCT
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eurjchem-460	304	4	;	;	PUNCT
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eurjchem-460	304	6	,	,	PUNCT
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eurjchem-460	304	8	;	;	PUNCT
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eurjchem-460	304	10	,	,	PUNCT
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eurjchem-460	304	12	;	;	PUNCT
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eurjchem-460	304	14	,	,	PUNCT
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eurjchem-460	304	16	;	;	PUNCT
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eurjchem-460	304	18	,	,	PUNCT
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eurjchem-460	304	22	.	.	PUNCT
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eurjchem-460	305	2	.	.	PUNCT
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eurjchem-460	305	4	.	.	PROPN
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eurjchem-460	305	6	,	,	PUNCT
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eurjchem-460	305	8	,	,	PUNCT
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eurjchem-460	305	10	.	.	PUNCT
eurjchem-460	306	1	[	[	X
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eurjchem-460	306	3	]	]	PUNCT
eurjchem-460	306	4	.	.	PUNCT
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eurjchem-460	307	5	,	,	PUNCT
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eurjchem-460	307	7	.	.	PUNCT
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eurjchem-460	308	4	.	.	PUNCT
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eurjchem-460	309	2	,	,	PUNCT
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eurjchem-460	309	4	;	;	PUNCT
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eurjchem-460	309	6	,	,	PUNCT
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eurjchem-460	309	9	;	;	PUNCT
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eurjchem-460	309	19	,	,	PUNCT
eurjchem-460	309	20	h.	h.	PROPN
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eurjchem-460	309	23	,	,	PUNCT
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eurjchem-460	310	1	[	[	X
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eurjchem-460	310	4	.	.	PUNCT
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eurjchem-460	311	7	,	,	PUNCT
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eurjchem-460	311	11	.	.	PUNCT
eurjchem-460	312	1	acta	acta	PROPN
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eurjchem-460	312	3	,	,	PUNCT
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eurjchem-460	312	5	,	,	PUNCT
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eurjchem-460	312	7	.	.	PUNCT
eurjchem-460	313	1	[	[	X
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eurjchem-460	313	3	]	]	PUNCT
eurjchem-460	313	4	.	.	PUNCT
eurjchem-460	314	1	lavalley	lavalley	PROPN
eurjchem-460	314	2	,	,	PUNCT
eurjchem-460	314	3	j.	j.	PROPN
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eurjchem-460	314	5	;	;	PUNCT
eurjchem-460	314	6	saussey	saussey	PROPN
eurjchem-460	314	7	,	,	PUNCT
eurjchem-460	314	8	j.	j.	PROPN
eurjchem-460	314	9	;	;	PUNCT
eurjchem-460	314	10	bovet	bovet	PROPN
eurjchem-460	314	11	,	,	PUNCT
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eurjchem-460	314	13	j.	j.	PROPN
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eurjchem-460	314	17	.	.	PUNCT
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eurjchem-460	315	2	,	,	PUNCT
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eurjchem-460	315	4	,	,	PUNCT
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eurjchem-460	315	6	.	.	PUNCT
eurjchem-460	316	1	[	[	X
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eurjchem-460	316	3	]	]	PUNCT
eurjchem-460	316	4	.	.	PUNCT
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eurjchem-460	316	6	,	,	PUNCT
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eurjchem-460	316	9	;	;	PUNCT
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eurjchem-460	316	11	,	,	PUNCT
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eurjchem-460	316	14	;	;	PUNCT
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eurjchem-460	316	16	,	,	PUNCT
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eurjchem-460	316	21	,	,	PUNCT
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eurjchem-460	316	24	;	;	PUNCT
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eurjchem-460	316	26	,	,	PUNCT
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eurjchem-460	316	29	;	;	PUNCT
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eurjchem-460	316	40	,	,	PUNCT
eurjchem-460	316	41	v.	v.	PROPN
eurjchem-460	316	42	;	;	PUNCT
eurjchem-460	316	43	mennucci	mennucci	PROPN
eurjchem-460	316	44	,	,	PUNCT
eurjchem-460	316	45	b.	b.	PROPN
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eurjchem-460	316	47	petersson	petersson	PROPN
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eurjchem-460	316	49	g.	g.	PROPN
eurjchem-460	316	50	a.	a.	PROPN
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eurjchem-460	316	52	nakatsuji	nakatsuji	PROPN
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eurjchem-460	316	54	h.	h.	PROPN
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eurjchem-460	316	56	caricato	caricato	PROPN
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eurjchem-460	316	60	li	li	PROPN
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eurjchem-460	316	62	x.	x.	PROPN
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eurjchem-460	316	66	h.	h.	PROPN
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eurjchem-460	316	84	j.	j.	PROPN
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eurjchem-460	316	126	h.	h.	PROPN
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eurjchem-460	316	140	;	;	PUNCT
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eurjchem-460	316	156	e.	e.	PROPN
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eurjchem-460	316	158	kudin	kudin	PROPN
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eurjchem-460	316	160	k.	k.	PROPN
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eurjchem-460	316	182	k.	k.	PROPN
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eurjchem-460	316	184	rendell	rendell	PROPN
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eurjchem-460	316	239	j.	j.	PROPN
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eurjchem-460	316	241	gomperts	gomperts	PROPN
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eurjchem-460	329	6	111‐	111‐	NUM
eurjchem-460	329	7	116	116	NUM
eurjchem-460	329	8	.	.	PUNCT
eurjchem-460	330	1	[	[	X
eurjchem-460	330	2	47	47	NUM
eurjchem-460	330	3	]	]	PUNCT
eurjchem-460	330	4	.	.	PUNCT
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eurjchem-460	331	2	,	,	PUNCT
eurjchem-460	331	3	x.	x.	PROPN
eurjchem-460	331	4	;	;	PUNCT
eurjchem-460	331	5	xu	xu	PROPN
eurjchem-460	331	6	,	,	PUNCT
eurjchem-460	331	7	x.	x.	PROPN
eurjchem-460	331	8	;	;	PUNCT
eurjchem-460	331	9	wang	wang	PROPN
eurjchem-460	331	10	,	,	PUNCT
eurjchem-460	331	11	n.	n.	PROPN
eurjchem-460	331	12	;	;	PUNCT
eurjchem-460	331	13	zhang	zhang	PROPN
eurjchem-460	331	14	,	,	PUNCT
eurjchem-460	331	15	q.	q.	PROPN
eurjchem-460	331	16	j.	j.	PROPN
eurjchem-460	331	17	phys	phys	PROPN
eurjchem-460	331	18	.	.	PUNCT
eurjchem-460	332	1	chem	chem	PROPN
eurjchem-460	332	2	.	.	PUNCT
eurjchem-460	333	1	b	b	NOUN
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eurjchem-460	333	3	,	,	PUNCT
eurjchem-460	333	4	103	103	NUM
eurjchem-460	333	5	,	,	PUNCT
eurjchem-460	333	6	2689‐	2689‐	NUM
eurjchem-460	333	7	2695	2695	NUM
eurjchem-460	333	8	.	.	PUNCT
eurjchem-460	334	1	[	[	X
eurjchem-460	334	2	48	48	NUM
eurjchem-460	334	3	]	]	PUNCT
eurjchem-460	334	4	.	.	PUNCT
eurjchem-460	335	1	lu	lu	PROPN
eurjchem-460	335	2	,	,	PUNCT
eurjchem-460	335	3	x.	x.	PROPN
eurjchem-460	335	4	;	;	PUNCT
eurjchem-460	335	5	xin	xin	PROPN
eurjchem-460	335	6	,	,	PUNCT
eurjchem-460	335	7	x.	x.	PROPN
eurjchem-460	335	8	;	;	PUNCT
eurjchem-460	335	9	wang	wang	PROPN
eurjchem-460	335	10	,	,	PUNCT
eurjchem-460	335	11	n.	n.	PROPN
eurjchem-460	335	12	;	;	PUNCT
eurjchem-460	335	13	zhang	zhang	PROPN
eurjchem-460	335	14	,	,	PUNCT
eurjchem-460	335	15	q.	q.	PROPN
eurjchem-460	335	16	ehara	ehara	PROPN
eurjchem-460	335	17	,	,	PUNCT
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eurjchem-460	335	19	;	;	PUNCT
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eurjchem-460	335	21	,	,	PUNCT
eurjchem-460	335	22	h.	h.	PROPN
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eurjchem-460	335	24	.	.	PUNCT
eurjchem-460	336	1	phys	phy	NOUN
eurjchem-460	336	2	.	.	PUNCT
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eurjchem-460	337	2	.	.	PUNCT
eurjchem-460	338	1	1998	1998	NUM
eurjchem-460	338	2	,	,	PUNCT
eurjchem-460	338	3	291	291	NUM
eurjchem-460	338	4	,	,	PUNCT
eurjchem-460	338	5	445‐452	445‐452	PROPN
eurjchem-460	338	6	.	.	PUNCT