Jtam.dvi JOURNAL OF THEORETICAL AND APPLIED MECHANICS 50, 1, pp. 301-319, Warsaw 2012 50th anniversary of JTAM ON COMBINED SPATIAL AND TEMPORAL INSTABILITIES OF ELECTRICALLY DRIVEN JETS WITH CONSTANT OR VARIABLE APPLIED FIELD Saulo Orizaga Daniel N. Riahi University of Texas-Pan American, Department of Mathematics, Edinburg, USA e-mail: driahi@utpa.edu We investigate the problem of combined spatial and temporal instabili- ties of electrically driven viscous jets with finite electrical conductivity in the presence of either constant or variable applied electric field.Ama- thematical model leads to a lengthy equation for the unknown spatial growth rate and temporal growth rate of the disturbances.This equation is solved numerically usingNewton’smethod.We investigated two cases of water jets and glycerol jets. For water jets and in the case of either constant or variable applied field, we found two newmodes of instabili- ties which grow simultaneously in time and space and lead to significant reduction in the jet radius.However, in the case of glycerol jets, we found two new modes of instabilities in the presence of constant applied field but only onemode of instability in the presence of variable applied field. For the glycerol jets, the combined temporal and spatial instabilities are less stronger and lead to an increase in the jet radius. The instabilities for both types of water and glycerol jets were found to be restricted to particular domain in their wavelength and were enhanced with the strength of the electric field. Keywords: temporal instability, spatial instability, jet flow, electric field, jet instability 1. Introduction In this paper, we consider the problem of combined spatial and temporal in- stabilities of electrically forced cylindrical jets of a viscous fluid with finite electrical conductivity and in the presence of an externally imposed constant 302 S. Orizaga, D.N. Riahi or variable electric field. The investigations of electrically forced jets are im- portant particularly in applications such as those to electrospraying (Baily, 1988) and electrospinning (Hohman et al., 2001a, 2001b). Electrospinning is a technology that uses electric fields to produce and control small fibers. The aim is at producing non-woven materials that are unparalleled in their poro- sity, high surface area, and the fineness and uniformity of their fibers. Such a technology has been used in a number of areas including bioengineering, tis- sue engineering, nano-electronics and in filtration media. Electrospraying is a technology that uses electric field to produce and control sprays of very small drops. The aim is at producing very small drops that are uniform in size and are of chargedmacromolecules in the gas phase. This technology also has been used in several areas including ink jet printing and the fuel injection process. There have been a number of theoretical, computational and experimen- tal studies of free shear flows and jets instabilities in the absence of electrical effects (Michalke, 1965; Drazin and Reid, 1981; Tam and Thies, 1993; Soder- berg, 2003;Healey, 2008) and in the presence of electrical effects (Taylor, 1969; Reneker et al., 2000; Shkadov and Shutov, 2001; Hohman et al., 2001a, 2001b; Li and Xia, 2004; Yu et al., 2004; Riahi, 2009; Orizaga and Riahi, 2009). Riahi (2009) followed amodeling approach analog to that due to Hohman et al. (2001a) and investigated analytically spatial instability of electrically forced jets with an applied variable field but under a restricted condition of neutral temporal stability and idealistic cases of a jet of zero electrical conduc- tivity or a jet of infinite electrical conductivity andwith certain restrictions on the frequency of the disturbances. He detected two spatial modes of instabili- ty, each of which was enhanced with increasing the strength of the externally imposed applied electric field. Thesemodeswere existed under certain restric- ted ranges of the axial wave number of disturbances, and, in particular, did not exist if the axial wave number was sufficiently small. Later, Orizaga and Riahi (2009) followed amodeling approach similar to that carried out byRiahi (2009) for the spatial instability of the electrically forced jet and again under a neutral temporal stability condition, but they investigated numerically using Newton’s method (Anderson et al., 1984) to determine results based on a set of fluid parameters for the jet with finite conductivity and under a constant or variable applied field. Orizaga and Riahi (2009) found two new modes of spatial instabilities. One of these modes was enhanced by the strength of the applied field, while the other mode decays with increasing the applied field. The growth rates of both modes increased mostly with decreasing the axial wavelength of the disturbances. For the case of a variable applied field, they found the growth rates of the spatial instability modes to be higher than the On combined spatial and temporal instabilities... 303 corresponding ones for the constant applied field, provided the strength of the applied field was not too small. In the present study, we first use a method of approach similar to that employed in Riahi (2009) and Orizaga and Riahi (2009) to arrive at a ma- thematical model for the realistic electrically driven viscous jets with finite conductivity, under externally imposed constant or variable applied field and with no restriction on the neutral stability boundary for the time variation of the superimposed perturbations. Here we consider more realistic jet flow instabilities, where the perturbations grow naturally and simultaneously both in time and space, and so no idealistic marginal stability conditions in time or in space are imposed on themathematical modeling of the jet flow instability system. We derive the dispersion relation which relates the growth rates of the spatial and temporal instabilities of the growing disturbances to the wave number in the axial direction, the frequency and the non-dimensional parame- ters of the model.We solve numerically the dispersion relation for the spatial and temporal growth rates of the growing disturbances using Newton’s me- thod (Anderson et al., 1984). We found a number of interesting results which were qualitatively different from the earlier studies (Riahi, 2009; Orizaga and Riahi, 2009) where the jet perturbations were not allowed to grow in time. In particular, we found new modes of instability which grow simultaneously in time and space. For the two investigated cases of glycerol and water jets, the growth rates of themodes of instabilities were increased as the strength of the electric fieldwas increased.For the case ofwater jet, the temporal growth rates were increasedmostly, while the spatial growth rates were increasedmostly in the case of glycerol jet. The spatial and temporal growth rates for either water jet or glycerol jet decrease mostly with decreasing the axial wave number of the disturbances. For the case of variable applied field, the growth rates of temporal and spatial growing disturbances were found to be mostly higher than the corresponding ones for the case of constant applied field. 2. Formulation and analysis The present mathematical modeling of the electrically driven jets is based on the governing electrohydrodynamic equations (Melcher and Taylor, 1969), whichwere already described in some details inRiahi (2009) andOrizaga and Riahi (2009) and, thus, will not be repeated here. Here we briefly describe the physical system and the correspondingmathematical model and refer the reader to these two references for details. A cylindrical, axisymmetric, New- 304 S. Orizaga, D.N. Riahi tonian and incompressible fluid jet is considered to be moving axially with passive air as the external fluid. The governing equations are used in a cy- lindrical coordinate system with the origin at the center of section where the jet is emitted with the axial z-axis along the axis of the jet. The modeling was based on the approximation that the jet is long and slender in the axial direction with the large length scale in the axial direction in comparison to that in the radial direction, so that a perturbation expansion is used in the small jet aspect ratio. Expanding the dependent variables in the Taylor series in the radial variable r, using such expansions in the full governing axisym- metric system, keeping only the leading terms and non-dimensionalizing the resulting equations, four relatively simple model equations are obtained for the dependent variables h, v, σ and E as functions of t and z. Here h is the radius of the jet cross section, v is the axial velocity, σ is the surface charge, E is the induced electric field and t is the time variable. These equations con- tain three non-dimensional parameters, which are the conductivity parameter K∗ =K0{ρr30/[γβ(ε̃)2]}0.5, the charge induction parameter β = ε/ε̃−1 and the viscosity parameter ν∗ = [ν2ρ/(γr0)] 0.5. Here r0 is radius of the cross- sectional area of the nozzle exit at z =0, γ is the surface tension, K0 is the reference conductivity, ε/(4π) is the permittivity constant in the jet, ϑε/(4π) is the permittivity constant in the air, ρ is the fluid density and ν is the kinematic viscosity. Next, the electrostatic equilibrium solution for the four model equations, referred to as the basic state solution, is considered as the one around which perturbations can grow in time and space. The basic state solution for each of the dependent variables, which is designated with a subscript b, is given below hb =1 vb =0 σb =σ0 Eb = Ω K̃(z) =Ω ( 1− 8σ0π Ω √ β z ) (2.1) where both Ω and σ0 are constant quantities. Here σ0 is the background free charge density.We set δ=8σ0π/(Ω √ β) to be a small parameter (δ≪ 1) and consider a series expansion in powers of δ for all the dependent variables for the case of variable applied field. In this paper, we investigate the cases where the applied electric field can be either constant (δ = 0) or variable (δ 6= 0). We consider each dependent variable as sum of its basic state solution plus a small perturbation, which is assumed to be oscillatory in time and in the axial variable. Thus, we write (h,v,σ,E) = (hb,vb,σb,Eb)+(h1,v1,σ1,E1) (2.2) On combined spatial and temporal instabilities... 305 where the perturbation quantities, which are designated with subscript 1, are given by (h1,v1,σ1,E1)= (h ′,v′,σ′,E′)exp[(f+iω)t+(s+ik)z] (2.3) Here (h′,v′,σ′,E′) are small constants, i is the pure imaginary number √ −1, f is the temporal growth rate of the growing disturbances, ω is the frequency, s is the spatial growth rate of the growing disturbances and k is the axial wave number. Using (2.1)-(2.3) in the fourmodel equations, we linearize with respect to the amplitude of perturbation, consider the lowest order in δ (for the variable applied field case) and divide each equation by the exponential function exp[(f+iω)t+(s+ik)z].We then obtain 4 linear algebraic equations for the unknown constants h′, v′, σ′ and E′. To obtain non-trivial (non-zero) values of these constants, the 4× 4 determinant of the coefficients of these unknownsmust be zero, which yields the following dispersion relation 1 2 (k2−1−s2−2iks)(k2−s2−2iks) [ (iω+f)A+ 4πK∗√ β ] +(k2−s2−2iks) [ (f+iω) (12πν∗K∗√ β + ω2 4π ) + ω2K∗A√ β ] − (ω− if)2 {4πK∗√ β +[(f+iω)+3ν∗(k2−s2−2iks)]A } +(k− is)2 [ 2(f+iω)Aπσ0 ( 1+ ln0.89k 2+Λ ) + 4πK∗√ β ( 2πσ20 −Ωσ0(s+ik) 4+(ln0.89k)−1 (k− is)2 √ β )] =0 (2.4) where A=1− 2 β(k− is)2 ln 1 χ Λ=−β(k− is)2 ln0.89k χ= 1 0.89k It can be seen from lengthy complex equation (2.4) that the spatial growth rate s and temporal growth rate f can be found for given values of the para- meters, k and ω. The effects of the unknowns s and f are highly nonlinear in (2.4), and, in particular, it turns out that the solution for s alone with f =0 in (2.4) is quite different from the corresponding solution for swith f 6=0 as our generated data for the two cases verified such outcome. 306 S. Orizaga, D.N. Riahi 3. Results and discussion Dispersion relation (2.4) is investigated for both variable and constant applied field cases. For the variable applied field, where δ 6= 0, we assume that δ is small of order about 0.1, and here both Ω and β cannot take zero value, so that we set 0 < σ0 ¬ 0.1, which turns out to keep the maximum value of δ of order 0.1 in the range of values for the rest of the parameters that are considered in the present study. For the constant applied field case, we set σ0 =0. In this Section, we describe each of the cases that we investigated and provide and discuss the corresponding results. In the present computation, we consider 2 types of fluids for the jet, which can be representatives for those used in the experimental investigation for the problem such as water and a type of glycerol. For such fluids, we set representative values of the parameters to be K∗ = 19.60, ν∗(glycerol) = =9.05384, ν∗(water)= 0.00608, and β=77.00. In addition, σ0 = 0 for the constant applied field and σ0 = 0.10 for the variable applied field.We then used (2.4) and carried outNewton’smethod to generate data for spatial and temporal growth rates, for different values of Ω and for both variable and constant applied field cases. The results are briefly presented in the following two sub-sections. 3.1. The case of water jet For Ω =1, we found two new modes of instabilities, each of which grows in both time and space. Thesemodes of instability were present for both cases of constant and variable applied field. The first mode of instability, referred here to asmode I, favors relatively smaller values of the axial wave number k, while the second mode of instability, referred to as mode II, favors relatively larger values of k. For the case of variable applied field, the temporal growth rate for both modes increases with the axial wave number k in the domain 0.04 < k < 0.38, while the spatial growth rate decreases with increasing k for mode I in 0.36 < k < 0.46 and increases shapely with k for mode II in 0.70 < k < 0.74. For the case of constant applied field, the temporal growth rate increases slowly with k for mode I in 0.10 < k < 0.28) and increases sharply with k for mode II in 0.56 < k < 0.58, while the spatial growth rate decreases sharply with increasing k for mode I in 0.32 < k < 0.34 and increases with k for mode II in 0.48 6.4, the amplitudes of the perturba- tions for v1 and h1 are sufficiently large that the present linear theory ceases to be valid. In addition and most importantly, it is seen that the jet radius On combined spatial and temporal instabilities... 311 perturbation can become negative for z > 5.6 and the magnitude increases rapidly with increasing z. Using this result together with (2.1)1 and (2.2), it implies significant reduction in the jet radius by the instabilities of mode I. This result can have important implicationwith respect to the electrospinning applications and making use of instabilities in a controlling manner for pro- duction of very small- andnano-scale fibers.Figure 8 presents variations of the perturbation quantities for mode I of combined spatial and temporal instabi- lities versus time variable t for σ0 = 0.1, s = 1.3460, k = 0.38, f = 0.9619 and Ω=4 but at one given axial location (z=1). Again it can be seen that, for example, for t > 5.4, the amplitude of v1 and E1 are sufficiently large that the linear theory ceases to be valid. In addition, temporal instability of mode I also exhibits significant reduction in the jet radius, which is enhanced with increasing time. From the results presented in the Figs.7 and 8, which were for the case of variable applied field, it can be concluded that combined spatial and temporal instabilities exhibit both significant reduction in the jet radius and a higher sensitivity of the jet flowwith respect to the disturbances that can grow simultaneously in time and in space. We also generated simi- lar data for the case of constant applied field and found that the spatial and temporal instabilities are more effective and enhanced in the case of variable applied field. Fig. 8. Perturbation quantities h1 (thin solid line), v1 (dashed line), σ1 (thick solid line) and E1 (dotted line) versus the axial variable t for water jet with Ω=4, σ0 =0.1, z=1, k=0.38, s=1.3460 and f =0.9619 3.2. The case of glycerol jet For Ω = 1, we found two modes of combined temporal and spatial in- stabilities similar to modes I and II described earlier in the case of water (sub-section 3.1) that were present for the case of constant applied field. For 312 S. Orizaga, D.N. Riahi this case, the growth rates s increase with the axial wave number in either 0.14 < k < 0.26 or 0.92 < k < 0.96, while the growth rates f remain quite small and non-monotonic for k in either 0.24 5.5, the amplitudes of perturbations for σ1 and h1 are sufficiently large that the present linear theory ceases to be valid. In addition, it can be seen that in contrast to the case ofwater jet, the glycerol jet radius is enhanced by themode of instability. Figure 16 presents variations of the perturbations versus time t for Ω = 4, k=0.16, σ0 =0.1, s=1.6251 and f =0.0280 but for a given location in the axial direction (z=1). Again it can be seen that, for example, for t> 55, the 316 S. Orizaga, D.N. Riahi amplitude of E1 is sufficiently large that the linear theory ceases to be valid. It is also seen that the jet radius is increasedwith time. Comparing the results presented in Figs.7, 8, 15 and 16, it can be concluded that in the presence of variable applied field, combined spatial and temporal instabilities exhibit higher strength and sensitivity and can lead to significant reduction in the jet radius, while such instabilities exhibit lower strength and sensitivity and lead to an increase in the jet radius in the case of glycerol jets. Our additional collected data for the constant applied field and for both water and glycerol jets lead to similar conclusions stated above. Fig. 16. Perturbation quantities h1 (thin solid line), v1 (dashed line), σ1 (thick solid line) and E1 (dotted line) versus the axial variable t for glycerol jet with Ω=4, σ0 =0.1, z=1, k=0.16, s=1.6251 and f =0.0280 4. Concluding remarks Mathematical modeling and numerical investigation of combined linear spa- tial and temporal instabilities of electro-hydrodynamic system for electrically forced slender viscous and finite conducting jet flows with externally imposed either constant or variable applied field were carried out. We were able to uncover two new modes of instabilities in the case of water jet in presence of either constant or variable applied field. For the case of glycerol jet, we found two modes of combined temporal and spatial instabilities under the imposed constant applied field and only one such a mode in the case of variable ap- plied field. For the case of variable applied field, only one mode of instability was found for the glycerol jet. The detected temporal-spatial instabilities were found to reduce significantly the jet radius and exhibit higher strength and On combined spatial and temporal instabilities... 317 sensitivity in the water jet cases, in which the jet radius is enhanced and in- stabilities are less strong with lower sensitivity in the case of glycerol jets. In addition, it was found that the instability modes are more effective mostly in the case of variable applied field. In regard to the relevance of the present detectedmodes of combined tem- poral and spatial to the available experimental results (Taylor, 1969; Hoh- man et al., 2001a,b) and in applications, we note that for electrically for- ced jets, Taylor (1969) documented the presence of axisymmetric instabilities at lower values of the strength of the applied field and non-axisymmentric whipping modes of instabilities at higher values of the field strength. Hoh- man et al. (2001a,b) observed experimentally axisymmetric excitations and growth in time as well as thickening blobs along the axial direction, and instabilities appeared to grow in time as well as they move downstream. These observations indicate the presence of axisymmetric instabilities and also temporally and spatially growing disturbances in the jet flow. Since non-axisymmetric whipping modes of instabilities have also been observed to be strong leading to significant jet radius reduction and ultimately bre- ak up the jets (Hohman et al., 2001b), it was thought that the whipping mode is the important instability mechanism for jet radius reduction and the corresponding advantage for controlling such instability in order to pro- duce higher quality fibers of very small- and nano-scale size. However, the present results for the axisymmetric modes of combined temporal and spa- tial instabilities in water jets, that can lead to significant reduction in the jet radius, could stimulate future investigations for ways to make use of such results in an optimized manner to production of higher quality fiber materials. Further extensions of the present study that are planned by the second author to be investigated in future, are the cases of combined spatial and temporal instabilities due to the non-axisymmetric disturbances.As is evident from the well known experiments by Taylor (1969) that the electrically forced jets can be non-axisymmetric and whip for sufficiently large values of the strengthof the electric field,we can expect that combined spatial and temporal instabilities due to the non-axisymmetric disturbances can dominate over the corresponding axisymmetric ones if Ω is sufficiently large. Acknowledgement This researchwas supported by a research grant fromUTPA-FRC. 318 S. Orizaga, D.N. Riahi References 1. Anderson D.A., Tannehill R.H., Pletcher R.H., 1984, Computational Fluid Mechanics and Heat Transfer, Hemisphere Publishing Corporation, New York 2. Baily A.G., 1988,Electro-Static Spraying of Liquid, Wiley, NewYork 3. Drazin P.G., Reid W.H., 1981,Hydrodynamic Stability, Cambridge Univer- sity Press, UK 4. Healey J.J., 2008, Inviscid axisymmetric absolute instability of swirling jets, Journal of Fluid Mechanics, 613, 1-33 5. Hohman M. M., Shin M., Rutledge G., Brenner M.P., 2001a, Electro- spinning and electrically forced jets. I. Stability theory,Phys. of Fluids, 13, 8, 2201-2220 6. Hohman M.M., Shin M., Rutledge G., Brenner M.P., 2001b, Electro- spinning and electrically forced jets. II. Applications, Phys. of Fluids, 13, 8, 2221-2236 7. Li D., Xia Y., 2004, Direct fabrication of composite and ceramic hollow na- nofibers by electrospinning,Nano Letters, 4, 933-938 8. 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Soderberg D.L., 2003, Absolute and convective instability of a relaxational plane liquid jet, Journal of Fluid Mechanics, 439, 89-119 15. Tam C.K.W., Thies A.T., 1993, Instability of rectangular jet, Journal of Fluid Mechanics, 248, 425-448 16. Taylor G.I., 1969, Electrically driven jets, Proceedings of the Royal Society of London, Series A, 313, 453-475 On combined spatial and temporal instabilities... 319 17. Yu J.H., Fridrikh S.V., Rutledge G.C., 2004, Production of sub- micrometer diameter fibers by two-fluid electrospinning, Advanced Materials, 16, 1562-1566 O złożonych, przestrzenno-czasowych niestabilnościach elektrycznie indukowanych strumieni w stałym i zmiennym polu Streszczenie Autorzy prezentują problem złożonych przestrzenno-czasowych niestabilności elektrycznie indukowanych strumieni wiskotycznych o skończonej przewodności elek- trycznej w obecności stałego albo zmiennego pola. Model matematyczny sprowadzo- no do skomplikowanego równania, w którym niewiadomą jest czasowe i przestrzenne tempo wzrostu zakłóceń w strumieniu. Równanie to rozwiązano numerycznie, uży- wając metody Newtona. Zbadano dwa przypadki – dla strumienia wody i gliceryny. Dla wody, niezależnie od tego, czy pole elektryczne jest stałe, czy zmienne, wykryto dwie nowepostacie niestabilności rosnących równocześniew czasie i przestrzeni, które znacznie ograniczająpromień strumienia.Wprzypadku gliceryny, dwie nowepostacie niestabilności znaleziono tylko przy stałympolu elektrycznym.Wpolu zmiennym za- obserwowano jedną postać.Dla gliceryny, złożoneniestabilności przestrzenno-czasowe wykazują słabszą intensywność i zwiększają promień strumienia. Niezależnie od ro- dzaju ośrodka, niestabilności te ograniczają się do pewnego zakresu długości falowej i wzrastają z natężeniem pola elektrycznego. Manuscript received August 9, 2010; accepted for print June 20, 2011